Articles | Volume 6, issue 3
https://doi.org/10.5194/gmd-6-765-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/gmd-6-765-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Development and technical paper
| 
05 Jun 2013
Development and technical paper |
| 05 Jun 2013
Sensitivity of remote aerosol distributions to representation of cloud–aerosol interactions in a global climate model
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory (PNNL), Richland, Washington, USA
R. C. Easter
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory (PNNL), Richland, Washington, USA
P. J. Rasch
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory (PNNL), Richland, Washington, USA
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory (PNNL), Richland, Washington, USA
X. Liu
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory (PNNL), Richland, Washington, USA
S. J. Ghan
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory (PNNL), Richland, Washington, USA
Y. Qian
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory (PNNL), Richland, Washington, USA
J.-H. Yoon
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory (PNNL), Richland, Washington, USA
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory (PNNL), Richland, Washington, USA
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory (PNNL), Richland, Washington, USA
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Dalei Hao, Gautam Bisht, Karl Rittger, Edward Bair, Cenlin He, Huilin Huang, Cheng Dang, Timbo Stillinger, Yu Gu, Hailong Wang, Yun Qian, and L. Ruby Leung
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Yang Yang, Liangying Zeng, Hailong Wang, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 22, 14489–14502, https://doi.org/10.5194/acp-22-14489-2022, https://doi.org/10.5194/acp-22-14489-2022, 2022
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Kai Zhang, Wentao Zhang, Hui Wan, Philip J. Rasch, Steven J. Ghan, Richard C. Easter, Xiangjun Shi, Yong Wang, Hailong Wang, Po-Lun Ma, Shixuan Zhang, Jian Sun, Susannah M. Burrows, Manish Shrivastava, Balwinder Singh, Yun Qian, Xiaohong Liu, Jean-Christophe Golaz, Qi Tang, Xue Zheng, Shaocheng Xie, Wuyin Lin, Yan Feng, Minghuai Wang, Jin-Ho Yoon, and L. Ruby Leung
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Here we analyze the effective aerosol forcing simulated by E3SM version 1 using both century-long free-running and short nudged simulations. The aerosol forcing in E3SMv1 is relatively large compared to other models, mainly due to the large indirect aerosol effect. Aerosol-induced changes in liquid and ice cloud properties in E3SMv1 have a strong correlation. The aerosol forcing estimates in E3SMv1 are sensitive to the parameterization changes in both liquid and ice cloud processes.
Jiyuan Gao, Yang Yang, Hailong Wang, Pinya Wang, Huimin Li, Mengyun Li, Lili Ren, Xu Yue, and Hong Liao
Atmos. Chem. Phys., 22, 7131–7142, https://doi.org/10.5194/acp-22-7131-2022, https://doi.org/10.5194/acp-22-7131-2022, 2022
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Xue Zheng, Qing Li, Tian Zhou, Qi Tang, Luke P. Van Roekel, Jean-Christophe Golaz, Hailong Wang, and Philip Cameron-Smith
Geosci. Model Dev., 15, 3941–3967, https://doi.org/10.5194/gmd-15-3941-2022, https://doi.org/10.5194/gmd-15-3941-2022, 2022
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We document the model experiments for the future climate projection by E3SMv1.0. At the highest future emission scenario, E3SMv1.0 projects a strong surface warming with rapid changes in the atmosphere, ocean, sea ice, and land runoff. Specifically, we detect a significant polar amplification and accelerated warming linked to the unmasking of the aerosol effects. The impact of greenhouse gas forcing is examined in different climate components.
Susannah M. Burrows, Richard C. Easter, Xiaohong Liu, Po-Lun Ma, Hailong Wang, Scott M. Elliott, Balwinder Singh, Kai Zhang, and Philip J. Rasch
Atmos. Chem. Phys., 22, 5223–5251, https://doi.org/10.5194/acp-22-5223-2022, https://doi.org/10.5194/acp-22-5223-2022, 2022
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Sea spray particles are composed of a mixture of salts and organic substances from oceanic microorganisms. In prior work, our team developed an approach connecting sea spray chemistry to ocean biology, called OCEANFILMS. Here we describe its implementation within an Earth system model, E3SM. We show that simulated sea spray chemistry is consistent with observed seasonal cycles and that sunlight reflected by simulated Southern Ocean clouds increases, consistent with analysis of satellite data.
Po-Lun Ma, Bryce E. Harrop, Vincent E. Larson, Richard B. Neale, Andrew Gettelman, Hugh Morrison, Hailong Wang, Kai Zhang, Stephen A. Klein, Mark D. Zelinka, Yuying Zhang, Yun Qian, Jin-Ho Yoon, Christopher R. Jones, Meng Huang, Sheng-Lun Tai, Balwinder Singh, Peter A. Bogenschutz, Xue Zheng, Wuyin Lin, Johannes Quaas, Hélène Chepfer, Michael A. Brunke, Xubin Zeng, Johannes Mülmenstädt, Samson Hagos, Zhibo Zhang, Hua Song, Xiaohong Liu, Michael S. Pritchard, Hui Wan, Jingyu Wang, Qi Tang, Peter M. Caldwell, Jiwen Fan, Larry K. Berg, Jerome D. Fast, Mark A. Taylor, Jean-Christophe Golaz, Shaocheng Xie, Philip J. Rasch, and L. Ruby Leung
Geosci. Model Dev., 15, 2881–2916, https://doi.org/10.5194/gmd-15-2881-2022, https://doi.org/10.5194/gmd-15-2881-2022, 2022
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An alternative set of parameters for E3SM Atmospheric Model version 1 has been developed based on a tuning strategy that focuses on clouds. When clouds in every regime are improved, other aspects of the model are also improved, even though they are not the direct targets for calibration. The recalibrated model shows a lower sensitivity to anthropogenic aerosols and surface warming, suggesting potential improvements to the simulated climate in the past and future.
Hossein Dadashazar, Majid Alipanah, Miguel Ricardo A. Hilario, Ewan Crosbie, Simon Kirschler, Hongyu Liu, Richard H. Moore, Andrew J. Peters, Amy Jo Scarino, Michael Shook, K. Lee Thornhill, Christiane Voigt, Hailong Wang, Edward Winstead, Bo Zhang, Luke Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 21, 16121–16141, https://doi.org/10.5194/acp-21-16121-2021, https://doi.org/10.5194/acp-21-16121-2021, 2021
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This study investigates precipitation impacts on long-range transport of North American outflow over the western North Atlantic Ocean (WNAO). Results demonstrate that precipitation scavenging plays a significant role in modifying surface aerosol concentrations over the WNAO, especially in winter and spring due to large-scale scavenging processes. This study highlights how precipitation impacts surface aerosol properties with relevance for other marine regions vulnerable to continental outflow.
Lili Ren, Yang Yang, Hailong Wang, Pinya Wang, Lei Chen, Jia Zhu, and Hong Liao
Atmos. Chem. Phys., 21, 15431–15445, https://doi.org/10.5194/acp-21-15431-2021, https://doi.org/10.5194/acp-21-15431-2021, 2021
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Due to the COVID-19 pandemic, human activities were strictly restricted in China. Even though anthropogenic aerosol emissions largely decreased, haze events still occurred. Our results shows that PM2.5 over the North China Plain is largely contributed by local sources. For other regions in China, PM2.5 is largely contributed from nonlocal sources. As emission reduction is a future goal, aerosol long-range transport and unfavorable meteorology are increasingly important to air quality.
Liangying Zeng, Yang Yang, Hailong Wang, Jing Wang, Jing Li, Lili Ren, Huimin Li, Yang Zhou, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 21, 10745–10761, https://doi.org/10.5194/acp-21-10745-2021, https://doi.org/10.5194/acp-21-10745-2021, 2021
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Using an aerosol–climate model, the impacts of El Niño with different durations on aerosols in China are examined. The modulation on aerosol concentrations and haze days by short-duration El Niño events is 2–3 times more than that by long-duration El Niño events in China. The frequency of short-duration El Niño has been increasing significantly in recent decades, suggesting that El Niño events have exerted increasingly intense modulation on aerosol pollution in China over the past few decades.
Hossein Dadashazar, David Painemal, Majid Alipanah, Michael Brunke, Seethala Chellappan, Andrea F. Corral, Ewan Crosbie, Simon Kirschler, Hongyu Liu, Richard H. Moore, Claire Robinson, Amy Jo Scarino, Michael Shook, Kenneth Sinclair, K. Lee Thornhill, Christiane Voigt, Hailong Wang, Edward Winstead, Xubin Zeng, Luke Ziemba, Paquita Zuidema, and Armin Sorooshian
Atmos. Chem. Phys., 21, 10499–10526, https://doi.org/10.5194/acp-21-10499-2021, https://doi.org/10.5194/acp-21-10499-2021, 2021
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This study investigates the seasonal cycle of cloud drop number concentration (Nd) over the western North Atlantic Ocean (WNAO) using multiple datasets. Reasons for the puzzling discrepancy between the seasonal cycles of Nd and aerosol concentration were identified. Results indicate that Nd is highest in winter (when aerosol proxy values are often lowest) due to conditions both linked to cold-air outbreaks and that promote greater droplet activation.
Mingxuan Wu, Xiaohong Liu, Hongbin Yu, Hailong Wang, Yang Shi, Kang Yang, Anton Darmenov, Chenglai Wu, Zhien Wang, Tao Luo, Yan Feng, and Ziming Ke
Atmos. Chem. Phys., 20, 13835–13855, https://doi.org/10.5194/acp-20-13835-2020, https://doi.org/10.5194/acp-20-13835-2020, 2020
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The spatiotemporal distributions of dust aerosol simulated by global climate models (GCMs) are highly uncertain. In this study, we evaluate dust extinction profiles, optical depth, and surface concentrations simulated in three GCMs and one reanalysis against multiple satellite retrievals and surface observations to gain process-level understanding. Our results highlight the importance of correctly representing dust emission, dry/wet deposition, and size distribution in GCMs.
Bethany Sutherland, Ben Kravitz, Philip J. Rasch, and Hailong Wang
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2020-228, https://doi.org/10.5194/gmd-2020-228, 2020
Preprint withdrawn
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Through a cascade of physical mechanisms, a change in one location can trigger a response in a different location. These responses and the mechanisms that cause them are difficult to detect. Here we propose a method, using global climate models, to detect possible relationships between changes in one region and responses throughout the globe caused by that change. A change in the Pacific ocean is used as a test case to determine the effectiveness of the method.
Lili Ren, Yang Yang, Hailong Wang, Rudong Zhang, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 20, 9067–9085, https://doi.org/10.5194/acp-20-9067-2020, https://doi.org/10.5194/acp-20-9067-2020, 2020
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Observations show that the concentrations of Arctic aerosols have declined since the early 1980s, which potentially contributed to the recent, rapid Arctic warming. We found that changes in sulfate and black carbon aerosols over the midlatitudes of the Northern Hemisphere had a larger impact on Arctic temperature than other regions and that the aerosol-induced temperature change explained approximately 20 % of the observed Arctic warming during 1980–2018.
Yufei Zou, Yuhang Wang, Zuowei Xie, Hailong Wang, and Philip J. Rasch
Atmos. Chem. Phys., 20, 4999–5017, https://doi.org/10.5194/acp-20-4999-2020, https://doi.org/10.5194/acp-20-4999-2020, 2020
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We analyze the relationship between winter air stagnation and pollution extremes over eastern China and preceding Arctic sea ice loss based on climate modeling and dynamic diagnoses. We find significant increases in both the probability and intensity of air stagnation extremes in the modeling result driven by regional sea ice and sea surface temperature changes over the Pacific sector of the Arctic. We reveal the considerable impact of the Arctic climate change on mid-latitude weather extremes.
Yang Yang, Sijia Lou, Hailong Wang, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 20, 2579–2590, https://doi.org/10.5194/acp-20-2579-2020, https://doi.org/10.5194/acp-20-2579-2020, 2020
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Aerosol concentration decreased in Europe during 1980–2018, of which 7 % was induced by the changes in non-European emissions. Aerosols transported from other source regions are increasingly important to air quality in Europe. Contributions to the sulfate radiative forcing over Europe from both European and non-European emissions should decrease at a comparable rate in the next three decades. Future changes in non-European emissions are important in causing regional climate change in Europe.
Hailong Wang, Jeremy G. Fyke, Jan T. M. Lenaerts, Jesse M. Nusbaumer, Hansi Singh, David Noone, Philip J. Rasch, and Rudong Zhang
The Cryosphere, 14, 429–444, https://doi.org/10.5194/tc-14-429-2020, https://doi.org/10.5194/tc-14-429-2020, 2020
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Using a climate model with unique water source tagging, we found that sea-ice anomalies in the Southern Ocean and accompanying SST changes have a significant influence on Antarctic precipitation and its source attribution through their direct impact on moisture sources and indirect impact on moisture transport. This study also highlights the importance of atmospheric dynamics in affecting the thermodynamic impact of sea-ice anomalies on regional Antarctic precipitation.
Edward Gryspeerdt, Johannes Mülmenstädt, Andrew Gettelman, Florent F. Malavelle, Hugh Morrison, David Neubauer, Daniel G. Partridge, Philip Stier, Toshihiko Takemura, Hailong Wang, Minghuai Wang, and Kai Zhang
Atmos. Chem. Phys., 20, 613–623, https://doi.org/10.5194/acp-20-613-2020, https://doi.org/10.5194/acp-20-613-2020, 2020
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Aerosol radiative forcing is a key uncertainty in our understanding of the human forcing of the climate, with much of this uncertainty coming from aerosol impacts on clouds. Observation-based estimates of the radiative forcing are typically smaller than those from global models, but it is not clear if they are more reliable. This work shows how the forcing components in global climate models can be identified, highlighting similarities between the two methods and areas for future investigation.
Hongbin Yu, Yang Yang, Hailong Wang, Qian Tan, Mian Chin, Robert C. Levy, Lorraine A. Remer, Steven J. Smith, Tianle Yuan, and Yingxi Shi
Atmos. Chem. Phys., 20, 139–161, https://doi.org/10.5194/acp-20-139-2020, https://doi.org/10.5194/acp-20-139-2020, 2020
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Emissions and long-range transport of mineral dust and
combustion-related aerosol from burning fossil fuels and biomass vary from year to year, driven by the evolution of the economy and changes in meteorological conditions and environmental regulations. This study offers both satellite and model perspectives on interannual variability and possible trends in combustion aerosol and dust in major continental outflow regions over the past 15 years (2003–2017).
George S. Fanourgakis, Maria Kanakidou, Athanasios Nenes, Susanne E. Bauer, Tommi Bergman, Ken S. Carslaw, Alf Grini, Douglas S. Hamilton, Jill S. Johnson, Vlassis A. Karydis, Alf Kirkevåg, John K. Kodros, Ulrike Lohmann, Gan Luo, Risto Makkonen, Hitoshi Matsui, David Neubauer, Jeffrey R. Pierce, Julia Schmale, Philip Stier, Kostas Tsigaridis, Twan van Noije, Hailong Wang, Duncan Watson-Parris, Daniel M. Westervelt, Yang Yang, Masaru Yoshioka, Nikos Daskalakis, Stefano Decesari, Martin Gysel-Beer, Nikos Kalivitis, Xiaohong Liu, Natalie M. Mahowald, Stelios Myriokefalitakis, Roland Schrödner, Maria Sfakianaki, Alexandra P. Tsimpidi, Mingxuan Wu, and Fangqun Yu
Atmos. Chem. Phys., 19, 8591–8617, https://doi.org/10.5194/acp-19-8591-2019, https://doi.org/10.5194/acp-19-8591-2019, 2019
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Effects of aerosols on clouds are important for climate studies but are among the largest uncertainties in climate projections. This study evaluates the skill of global models to simulate aerosol, cloud condensation nuclei (CCN) and cloud droplet number concentrations (CDNCs). Model results show reduced spread in CDNC compared to CCN due to the negative correlation between the sensitivities of CDNC to aerosol number concentration (air pollution) and updraft velocity (atmospheric dynamics).
Chandan Sarangi, Yun Qian, Karl Rittger, Kathryn J. Bormann, Ying Liu, Hailong Wang, Hui Wan, Guangxing Lin, and Thomas H. Painter
Atmos. Chem. Phys., 19, 7105–7128, https://doi.org/10.5194/acp-19-7105-2019, https://doi.org/10.5194/acp-19-7105-2019, 2019
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Radiative forcing induced by deposition of light-absorbing particles (LAPs) on snow is an important surface forcing. Here, we have used high-resolution WRF-Chem (coupled with online snow–LAP–radiation model) simulations for 2013–2014 to estimate the spatial variation in LAP-induced snow albedo darkening effect in high-mountain Asia. Significant improvement in simulated LAP–snow properties with use of a higher spatial resolution for the same model configuration is illustrated over this region.
Yang Yang, Steven J. Smith, Hailong Wang, Catrin M. Mills, and Philip J. Rasch
Atmos. Chem. Phys., 19, 2405–2420, https://doi.org/10.5194/acp-19-2405-2019, https://doi.org/10.5194/acp-19-2405-2019, 2019
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Black carbon (BC) particles exert a potentially large warming influence on the
Earth system. We evaluate regional climate responses, non-linearity, and short-term transient responses to BC emission perturbations. We found that climate responses do not scale linearity with emissions and BC impacts temperature much faster than greenhouse gas forcing. Removing present-day BC emissions results in discernible surface temperature changes for only limited regions of the globe.
Anna Possner, Hailong Wang, Robert Wood, Ken Caldeira, and Thomas P. Ackerman
Atmos. Chem. Phys., 18, 17475–17488, https://doi.org/10.5194/acp-18-17475-2018, https://doi.org/10.5194/acp-18-17475-2018, 2018
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We quantify aerosol–cloud radiative interactions in a regime of deep open-cell stratocumuli (boundary layer depth 1.5 km), a regime which remains largely unexplored within this context and yet is more dominant than cases of shallow stratocumuli previously studied. We simulate substantial increases in albedo in a regime where ship tracks are not found and argue that such changes may escape detection and attribution through remote sensing due to the large natural variability in the system.
Ben Kravitz, Philip J. Rasch, Hailong Wang, Alan Robock, Corey Gabriel, Olivier Boucher, Jason N. S. Cole, Jim Haywood, Duoying Ji, Andy Jones, Andrew Lenton, John C. Moore, Helene Muri, Ulrike Niemeier, Steven Phipps, Hauke Schmidt, Shingo Watanabe, Shuting Yang, and Jin-Ho Yoon
Atmos. Chem. Phys., 18, 13097–13113, https://doi.org/10.5194/acp-18-13097-2018, https://doi.org/10.5194/acp-18-13097-2018, 2018
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Marine cloud brightening has been proposed as a means of geoengineering/climate intervention, or deliberately altering the climate system to offset anthropogenic climate change. In idealized simulations that highlight contrasts between land and ocean, we find that the globe warms, including the ocean due to transport of heat from land. This study reinforces that no net energy input into the Earth system does not mean that temperature will necessarily remain unchanged.
Kai Zhang, Philip J. Rasch, Mark A. Taylor, Hui Wan, Ruby Leung, Po-Lun Ma, Jean-Christophe Golaz, Jon Wolfe, Wuyin Lin, Balwinder Singh, Susannah Burrows, Jin-Ho Yoon, Hailong Wang, Yun Qian, Qi Tang, Peter Caldwell, and Shaocheng Xie
Geosci. Model Dev., 11, 1971–1988, https://doi.org/10.5194/gmd-11-1971-2018, https://doi.org/10.5194/gmd-11-1971-2018, 2018
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The conservation of total water is an important numerical feature for global Earth system models. Even small conservation problems in the water budget can lead to systematic errors in century-long simulations for sea level rise projection. This study quantifies and reduces various sources of water conservation error in the atmosphere component of the Energy Exascale Earth System Model.
Hewen Niu, Shichang Kang, Hailong Wang, Rudong Zhang, Xixi Lu, Yun Qian, Rukumesh Paudyal, Shijin Wang, Xiaofei Shi, and Xingguo Yan
Atmos. Chem. Phys., 18, 6441–6460, https://doi.org/10.5194/acp-18-6441-2018, https://doi.org/10.5194/acp-18-6441-2018, 2018
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Deposition of light-absorbing carbonaceous aerosol on the surface of glaciers can greatly alter the energy fluxes of glaciers. Two years of continuous observations of carbonaceous aerosols in a glacierized region are analyzed. We mainly studied the light absorption properties of carbonaceous aerosol and have employed a global aerosol–climate model to estimate source attributions of atmospheric black carbon.
Jeremy Fyke, Jan T. M. Lenaerts, and Hailong Wang
The Cryosphere, 11, 2595–2609, https://doi.org/10.5194/tc-11-2595-2017, https://doi.org/10.5194/tc-11-2595-2017, 2017
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In this CESM modeling study, we uncover regional relationships in snowfall across Antarctica that are corroborated by regional modeling and ice core records. These relationships are driven by variability in large-scale atmospheric moisture transport and dampen overall Antarctic snowfall variability, with implications for Antarctic-sourced sea level variability and detection of an emergent anthropogenic signal in Antarctic mass trends.
Yang Yang, Hailong Wang, Steven J. Smith, Richard Easter, Po-Lun Ma, Yun Qian, Hongbin Yu, Can Li, and Philip J. Rasch
Atmos. Chem. Phys., 17, 8903–8922, https://doi.org/10.5194/acp-17-8903-2017, https://doi.org/10.5194/acp-17-8903-2017, 2017
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Sulfate has significant impacts on air quality and climate. Local sulfate pollution could result from remote influences, making domestic mitigation efforts inefficient. Using CESM with a sulfur source-tagging technique, we found that, over regions with relatively low emissions, sulfate concentrations are primarily attributed to non-local sources and sulfate indirect radiative forcing over the Southern Hemisphere is more sensitive to emission perturbation than the polluted Northern Hemisphere.
Shi Zhong, Yun Qian, Chun Zhao, Ruby Leung, Hailong Wang, Ben Yang, Jiwen Fan, Huiping Yan, Xiu-Qun Yang, and Dongqing Liu
Atmos. Chem. Phys., 17, 5439–5457, https://doi.org/10.5194/acp-17-5439-2017, https://doi.org/10.5194/acp-17-5439-2017, 2017
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An online climate–chemistry coupled model (WRF-Chem) is integrated for 5 years at cloud-permitting scale to quantify the impacts of urbanization-induced changes in land cover and pollutants emission on regional climate in the Yangtze River Delta region in eastern China. Urbanization over this region increases the frequency of extreme precipitation and heat wave in summer. The results could help China government in making policies in mitigating the environmental impact of urbanization.
Yang Yang, Hailong Wang, Steven J. Smith, Po-Lun Ma, and Philip J. Rasch
Atmos. Chem. Phys., 17, 4319–4336, https://doi.org/10.5194/acp-17-4319-2017, https://doi.org/10.5194/acp-17-4319-2017, 2017
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The source attributions of black carbon (BC) in China are quantified using the Community Earth System Model by source tagging. BC impacts neighboring regions greatly. Transport is important in increasing BC during regional polluted days. Emissions outside China contribute 35 % of BC direct radiative forcing in China. Efficiency analysis shows that reduction in BC emissions over eastern China could have a greater benefit for regional air quality in China, especially in the winter haze season.
Ben Kravitz, Douglas G. MacMartin, Philip J. Rasch, and Hailong Wang
Atmos. Chem. Phys., 17, 2525–2541, https://doi.org/10.5194/acp-17-2525-2017, https://doi.org/10.5194/acp-17-2525-2017, 2017
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We introduce system identification techniques to climate science wherein multiple dynamic input–output relationships can be simultaneously characterized in a single simulation. This method, involving multiple small perturbations (in space and time) of an input field while monitoring output fields to quantify responses, allows for identification of different timescales of climate response to forcing without substantially pushing the climate far away from a steady state.
Ben Kravitz, Douglas G. MacMartin, Hailong Wang, and Philip J. Rasch
Earth Syst. Dynam., 7, 469–497, https://doi.org/10.5194/esd-7-469-2016, https://doi.org/10.5194/esd-7-469-2016, 2016
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Most simulations of solar geoengineering prescribe a particular strategy and evaluate its modeled effects. Here we first choose example climate objectives and then design a strategy to meet those objectives in climate models. We show that certain objectives can be met simultaneously even in the presence of uncertainty, and the strategy for meeting those objectives can be ported to other models. This is part of a broader illustration of how uncertainties in solar geoengineering can be managed.
N. I. Kristiansen, A. Stohl, D. J. L. Olivié, B. Croft, O. A. Søvde, H. Klein, T. Christoudias, D. Kunkel, S. J. Leadbetter, Y. H. Lee, K. Zhang, K. Tsigaridis, T. Bergman, N. Evangeliou, H. Wang, P.-L. Ma, R. C. Easter, P. J. Rasch, X. Liu, G. Pitari, G. Di Genova, S. Y. Zhao, Y. Balkanski, S. E. Bauer, G. S. Faluvegi, H. Kokkola, R. V. Martin, J. R. Pierce, M. Schulz, D. Shindell, H. Tost, and H. Zhang
Atmos. Chem. Phys., 16, 3525–3561, https://doi.org/10.5194/acp-16-3525-2016, https://doi.org/10.5194/acp-16-3525-2016, 2016
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Processes affecting aerosol removal from the atmosphere are not fully understood. In this study we investigate to what extent atmospheric transport models can reproduce observed loss of aerosols. We compare measurements of radioactive isotopes, that attached to ambient sulfate aerosols during the 2011 Fukushima nuclear accident, to 19 models using identical emissions. Results indicate aerosol removal that is too fast in most models, and apply to aerosols that have undergone long-range transport.
Shipeng Zhang, Minghuai Wang, Steven J. Ghan, Aijun Ding, Hailong Wang, Kai Zhang, David Neubauer, Ulrike Lohmann, Sylvaine Ferrachat, Toshihiko Takeamura, Andrew Gettelman, Hugh Morrison, Yunha Lee, Drew T. Shindell, Daniel G. Partridge, Philip Stier, Zak Kipling, and Congbin Fu
Atmos. Chem. Phys., 16, 2765–2783, https://doi.org/10.5194/acp-16-2765-2016, https://doi.org/10.5194/acp-16-2765-2016, 2016
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The variation of aerosol indirect effects (AIE) in several climate models is investigated across different dynamical regimes. Regimes with strong large-scale ascent are shown to be as important as stratocumulus regimes in studying AIE. AIE over regions with high monthly large-scale surface precipitation rate contributes the most to the total aerosol indirect forcing. These results point to the need to reduce the uncertainty in AIE in different dynamical regimes.
X. Liu, P.-L. Ma, H. Wang, S. Tilmes, B. Singh, R. C. Easter, S. J. Ghan, and P. J. Rasch
Geosci. Model Dev., 9, 505–522, https://doi.org/10.5194/gmd-9-505-2016, https://doi.org/10.5194/gmd-9-505-2016, 2016
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In this study, we describe and evaluate a new four-mode version of the Modal Aerosol Module (MAM4) in the Community Atmosphere Model version 5 (CAM5). Compared to the current three-mode version of MAM in CAM5, MAM4 significantly improves the simulation of seasonal variation of BC concentrations in the polar regions, by increasing the BC concentrations in all seasons and particularly in cold seasons.
R. Zhang, H. Wang, D. A. Hegg, Y. Qian, S. J. Doherty, C. Dang, P.-L. Ma, P. J. Rasch, and Q. Fu
Atmos. Chem. Phys., 15, 12805–12822, https://doi.org/10.5194/acp-15-12805-2015, https://doi.org/10.5194/acp-15-12805-2015, 2015
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We use a global climate model with an explicit source tagging technique to quantify contributions of emissions from various geographical regions and sectors to BC in North America. Model results are evaluated against measurements of near-surface and in-snow BC. We found strong spatial variations of BC and its radiative forcing that can be quantitatively attributed to the various source origins, and also identified a significant source of BC in snow that is likely missing in most climate models.
B. Kravitz, A. Robock, S. Tilmes, O. Boucher, J. M. English, P. J. Irvine, A. Jones, M. G. Lawrence, M. MacCracken, H. Muri, J. C. Moore, U. Niemeier, S. J. Phipps, J. Sillmann, T. Storelvmo, H. Wang, and S. Watanabe
Geosci. Model Dev., 8, 3379–3392, https://doi.org/10.5194/gmd-8-3379-2015, https://doi.org/10.5194/gmd-8-3379-2015, 2015
R. Zhang, H. Wang, Y. Qian, P. J. Rasch, R. C. Easter, P.-L. Ma, B. Singh, J. Huang, and Q. Fu
Atmos. Chem. Phys., 15, 6205–6223, https://doi.org/10.5194/acp-15-6205-2015, https://doi.org/10.5194/acp-15-6205-2015, 2015
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We use the CAM5 model with a novel source-tagging technique to characterize the fate of BC particles emitted from various geographical regions and sectors and their transport pathways to the Himalayas and Tibetan Plateau (HTP). We show a comprehensive picture of the seasonal and regional dependence of BC source attributions, and find strong seasonal and spatial variations in BC-in-snow radiative forcing in the HTP that can be quantitatively attributed to the various regional/sectoral sources.
M. Wang, B. Xu, J. Cao, X. Tie, H. Wang, R. Zhang, Y. Qian, P. J. Rasch, S. Zhao, G. Wu, H. Zhao, D. R. Joswiak, J. Li, and Y. Xie
Atmos. Chem. Phys., 15, 1191–1204, https://doi.org/10.5194/acp-15-1191-2015, https://doi.org/10.5194/acp-15-1191-2015, 2015
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Carbonaceous aerosols recorded in a Tibetan glacier present a distinct seasonal dependence and an increasing trend after 1980, which has important implications for the accelerated glacier melting. We use a global aerosol--climate model to quantify the aerosol source--receptor relationships, showing that emissions in South Asia had the largest contribution. The emission inventories and historical fuel consumption in South Asia are consistent with our ice-core analysis and model results.
C. Zhao, Z. Hu, Y. Qian, L. Ruby Leung, J. Huang, M. Huang, J. Jin, M. G. Flanner, R. Zhang, H. Wang, H. Yan, Z. Lu, and D. G. Streets
Atmos. Chem. Phys., 14, 11475–11491, https://doi.org/10.5194/acp-14-11475-2014, https://doi.org/10.5194/acp-14-11475-2014, 2014
C. Zhao, X. Liu, Y. Qian, J. Yoon, Z. Hou, G. Lin, S. McFarlane, H. Wang, B. Yang, P.-L. Ma, H. Yan, and J. Bao
Atmos. Chem. Phys., 13, 10969–10987, https://doi.org/10.5194/acp-13-10969-2013, https://doi.org/10.5194/acp-13-10969-2013, 2013
Katherine Smith, Alice M. Barthel, LeAnn M. Conlon, Luke P. Van Roekel, Anthony Bartoletti, Jean-Christophe Golez, Chengzhu Zhang, Carolyn Branecky Begeman, James J. Benedict, Gautum Bisht, Yan Feng, Walter Hannah, Bryce E. Harrop, Nicole Jeffery, Wuyin Lin, Po-Lun Ma, Mathew E. Maltrud, Mark R. Petersen, Balwinder Singh, Qi Tang, Teklu Tesfa, Jonathan D. Wolfe, Shaocheng Xie, Xue Zheng, Karthik Balaguru, Oluwayemi Garuba, Peter Gleckler, Aixue Hu, Jiwoo Lee, Ben Moore-Maley, and Ana C. Ordonez
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-149, https://doi.org/10.5194/gmd-2024-149, 2024
Preprint under review for GMD
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Version 2.1 of the U.S. Department of Energy's Energy Exascale Earth System Model (E3SM) adds the Fox-Kemper et al. (2011) mixed layer eddy parameterization, which restratifies the ocean surface layer through an overturning streamfunction. Results include surface layer biases reduction in temperature, salinity, and sea-ice extent in the North Atlantic, a small strengthening of the Atlantic Meridional Overturning Circulation, and improvements in many atmospheric climatological variables.
Allen Hu, Xiaohong Liu, Ziming Ke, Benjamin Wagman, Hunter Brown, Zheng Lu, Diana Bull, and Kara Peterson
EGUsphere, https://doi.org/10.5194/egusphere-2024-2227, https://doi.org/10.5194/egusphere-2024-2227, 2024
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Volcanic eruptions have a major effect on temperature throughout the atmosphere and can be studied as a proxy for geo-engineering. The aerosol module in the Energy Exascale Earth System Model (E3SM) was originally intended for simulation of tropospheric aerosols and has problems handling stratospheric sulfate aerosols due to volcanic eruptions. We have made alterations to the aerosol module to overcome these problems, with simulation results more closely reproducing observations.
Ye Liu, Yun Qian, Larry K. Berg, Zhe Feng, Jianfeng Li, Jingyi Chen, and Zhao Yang
Atmos. Chem. Phys., 24, 8165–8181, https://doi.org/10.5194/acp-24-8165-2024, https://doi.org/10.5194/acp-24-8165-2024, 2024
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Deep convection under various large-scale meteorological patterns (LSMPs) shows distinct precipitation features. In southeastern Texas, mesoscale convective systems (MCSs) contribute significantly to precipitation year-round, while isolated deep convection (IDC) is prominent in summer and fall. Self-organizing maps (SOMs) reveal convection can occur without large-scale lifting or moisture convergence. MCSs and IDC events have distinct life cycles influenced by specific LSMPs.
Hunter York Brown, Benjamin Wagman, Diana Bull, Kara Peterson, Benjamin Hillman, Xiaohong Liu, Ziming Ke, and Lin Lin
Geosci. Model Dev., 17, 5087–5121, https://doi.org/10.5194/gmd-17-5087-2024, https://doi.org/10.5194/gmd-17-5087-2024, 2024
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Explosive volcanic eruptions lead to long-lived, microscopic particles in the upper atmosphere which act to cool the Earth's surface by reflecting the Sun's light back to space. We include and test this process in a global climate model, E3SM. E3SM is tested against satellite and balloon observations of the 1991 eruption of Mt. Pinatubo, showing that with these particles in the model we reasonably recreate Pinatubo and its global effects. We also explore how particle size leads to these effects.
Johannes Mülmenstädt, Edward Gryspeerdt, Sudhakar Dipu, Johannes Quaas, Andrew S. Ackerman, Ann M. Fridlind, Florian Tornow, Susanne E. Bauer, Andrew Gettelman, Yi Ming, Youtong Zheng, Po-Lun Ma, Hailong Wang, Kai Zhang, Matthew W. Christensen, Adam C. Varble, L. Ruby Leung, Xiaohong Liu, David Neubauer, Daniel G. Partridge, Philip Stier, and Toshihiko Takemura
Atmos. Chem. Phys., 24, 7331–7345, https://doi.org/10.5194/acp-24-7331-2024, https://doi.org/10.5194/acp-24-7331-2024, 2024
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Human activities release copious amounts of small particles called aerosols into the atmosphere. These particles change how much sunlight clouds reflect to space, an important human perturbation of the climate, whose magnitude is highly uncertain. We found that the latest climate models show a negative correlation but a positive causal relationship between aerosols and cloud water. This means we need to be very careful when we interpret observational studies that can only see correlation.
Jianfeng Li, Andrew Geiss, Zhe Feng, L. Ruby Leung, Yun Qian, and Wenjun Cui
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-112, https://doi.org/10.5194/essd-2024-112, 2024
Preprint under review for ESSD
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We develop a high-resolution (4 km and hourly) observational derecho dataset over the United States east of the Rocky Mountains from 2004 to 2021 by using a mesoscale convective system dataset, bow echo detection based on a machine learning method, hourly gust speed measurements, and physically based identification criteria.
Natalie M. Mahowald, Longlei Li, Julius Vira, Marje Prank, Douglas S. Hamilton, Hitoshi Matsui, Ron L. Miller, Louis Lu, Ezgi Akyuz, Daphne Meidan, Peter G. Hess, Heikki Lihavainen, Christine Wiedinmyer, Jenny Hand, Maria Grazia Alaimo, Célia Alves, Andres Alastuey, Paulo Artaxo, Africa Barreto, Francisco Barraza, Silvia Becagli, Giulia Calzolai, Shankararaman Chellam, Ying Chen, Patrick Chuang, David D. Cohen, Cristina Colombi, Evangelia Diapouli, Gaetano Dongarra, Konstantinos Eleftheriadis, Johann Engelbrecht, Corinne Galy-Lacaux, Cassandra Gaston, Dario Gomez, Yenny González Ramos, Roy M. Harrison, Chris Heyes, Barak Herut, Philip Hopke, Christoph Hüglin, Maria Kanakidou, Zsofia Kertesz, Zbigniew Klimont, Katriina Kyllönen, Fabrice Lambert, Xiaohong Liu, Remi Losno, Franco Lucarelli, Willy Maenhaut, Beatrice Marticorena, Randall V. Martin, Nikolaos Mihalopoulos, Yasser Morera-Gomez, Adina Paytan, Joseph Prospero, Sergio Rodríguez, Patricia Smichowski, Daniela Varrica, Brenna Walsh, Crystal Weagle, and Xi Zhao
EGUsphere, https://doi.org/10.5194/egusphere-2024-1617, https://doi.org/10.5194/egusphere-2024-1617, 2024
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Aerosol particles are an important part of the Earth system, but their concentrations are spatially and temporally heterogeneous, as well as variable in size and composition. Here we present a new compilation of PM2.5 and PM10 aerosol observations, focusing on the spatial variability across different observational stations, including composition, and demonstrate a method for comparing the datasets to model output.
Huilin Huang, Yun Qian, Gautam Bisht, Jiali Wang, Tirthankar Chakraborty, Dalei Hao, Jianfeng Li, Travis Thurber, Balwinder Singh, Zhao Yang, Ye Liu, Pengfei Xue, William Sacks, Ethan Coon, and Robert Hetland
EGUsphere, https://doi.org/10.5194/egusphere-2024-1555, https://doi.org/10.5194/egusphere-2024-1555, 2024
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We integrate E3SM land model (ELM) with the WRF Model through the Lightweight Infrastructure for Land Atmosphere Coupling (LILAC) – Earth System Modeling Framework (ESMF). This framework includes a top-level driver, LILAC, for variable communication between WRF and ELM, and ESMF caps for ELM initialization, execution, and finalization. The LILAC-ESMF framework maintains the integrity of the ELM’s source code structure and facilitates the transfer of future developments in LSMs to WRF-ELM.
Ziming Ke, Qi Tang, Jean-Christoophe Golaz, Xiaohong Liu, and Hailong Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-1612, https://doi.org/10.5194/egusphere-2024-1612, 2024
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By treating volcanic emission interactively, model results improve simulated temperature variability, showing better correlations for 1940–1959 and 1960–1979, and reveals how volcanic activity influences cloud behavior and climate.
Yang Yang, Shaoxuan Mou, Hailong Wang, Pinya Wang, Baojie Li, and Hong Liao
Atmos. Chem. Phys., 24, 6509–6523, https://doi.org/10.5194/acp-24-6509-2024, https://doi.org/10.5194/acp-24-6509-2024, 2024
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The variations in anthropogenic aerosol concentrations and source contributions and their subsequent radiative impact in major emission regions during historical periods are quantified based on an aerosol-tagging system in E3SMv1. Due to the industrial development and implementation of economic policies, sources of anthropogenic aerosols show different variations, which has important implications for pollution prevention and control measures and decision-making for global collaboration.
Mariya Petrenko, Ralph Kahn, Mian Chin, Susanne E. Bauer, Tommi Bergman, Huisheng Bian, Gabriele Curci, Ben Johnson, Johannes Kaiser, Zak Kipling, Harri Kokkola, Xiaohong Liu, Keren Mezuman, Tero Mielonen, Gunnar Myhre, Xiaohua Pan, Anna Protonotariou, Samuel Remy, Ragnhild Bieltvedt Skeie, Philip Stier, Toshihiko Takemura, Kostas Tsigaridis, Hailong Wang, Duncan Watson-Parris, and Kai Zhang
EGUsphere, https://doi.org/10.5194/egusphere-2024-1487, https://doi.org/10.5194/egusphere-2024-1487, 2024
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We compared smoke plume simulations from 11 global models to each other and to satellite smoke-amount observations, aimed at constraining smoke source strength. In regions where plumes are thick and background aerosol is low, models and satellites compare well. However, the input emission inventory tends to underestimate in many places, and particle property and loss-rate assumptions vary enormously among models, causing uncertainties that require systematic in-situ measurements to resolve.
Charlotte M. Beall, Po-Lun Ma, Matthew W. Christensen, Johannes Mülmenstädt, Adam Varble, Kentaroh Suzuki, and Takuro Michibata
Atmos. Chem. Phys., 24, 5287–5302, https://doi.org/10.5194/acp-24-5287-2024, https://doi.org/10.5194/acp-24-5287-2024, 2024
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Single-layer warm liquid clouds cover nearly one-third of the Earth's surface, and uncertainties regarding the impact of aerosols on their radiative properties pose a significant challenge to climate prediction. Here, we demonstrate how satellite observations can be used to constrain Earth system model estimates of the radiative forcing from the interactions of aerosols with clouds due to warm rain processes.
Taufiq Hassan, Kai Zhang, Jianfeng Li, Balwinder Singh, Shixuan Zhang, Hailong Wang, and Po-Lun Ma
Geosci. Model Dev., 17, 3507–3532, https://doi.org/10.5194/gmd-17-3507-2024, https://doi.org/10.5194/gmd-17-3507-2024, 2024
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Anthropogenic aerosol emissions are an essential part of global aerosol models. Significant errors can exist from the loss of emission heterogeneity. We introduced an emission treatment that significantly improved aerosol emission heterogeneity in high-resolution model simulations, with improvements in simulated aerosol surface concentrations. The emission treatment will provide a more accurate representation of aerosol emissions and their effects on climate.
Hongyu Liu, Bo Zhang, Richard H. Moore, Luke D. Ziemba, Richard A. Ferrare, Hyundeok Choi, Armin Sorooshian, David Painemal, Hailong Wang, Michael A. Shook, Amy Jo Scarino, Johnathan W. Hair, Ewan C. Crosbie, Marta A. Fenn, Taylor J. Shingler, Chris A. Hostetler, Gao Chen, Mary M. Kleb, Gan Luo, Fangqun Yu, Jason L. Tackett, Mark A. Vaughan, Yongxiang Hu, Glenn S. Diskin, John B. Nowak, Joshua P. DiGangi, Yonghoon Choi, Christoph A. Keller, and Matthew S. Johnson
EGUsphere, https://doi.org/10.5194/egusphere-2024-1127, https://doi.org/10.5194/egusphere-2024-1127, 2024
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We use the GEOS-Chem model to simulate aerosols over the western North Atlantic Ocean (WNAO) during the winter and summer campaigns of ACTIVATE 2020. Model results are evaluated against in situ and remote sensing measurements from two aircraft as well as ground-based and satellite observations. The improved understanding of the aerosol life cycle, composition, transport pathways, and distribution has important implications for characterizing aerosol-cloud-meteorology interactions over the WNAO.
Weiming Ma, Hailong Wang, Gang Chen, Yun Qian, Ian Baxter, Yiling Huo, and Mark W. Seefeldt
Atmos. Chem. Phys., 24, 4451–4472, https://doi.org/10.5194/acp-24-4451-2024, https://doi.org/10.5194/acp-24-4451-2024, 2024
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Extreme warming events with surface temperature going above 0°C can occur in the high-Arctic winter. Although reanalysis data show that these events were short-lived and occurred rarely during 1980–2021, they have become more frequent, stronger, and longer lasting latterly. A dipole pattern, comprising high- and low-pressure systems, is found to be the key in driving them. These findings have implications for the recent changes in sea ice, hydrological cycle, and ecosystem over the Arctic.
Philip Rasch, Haruki Hirasawa, Mingxuan Wu, Sarah Doherty, Robert Wood, Hailong Wang, Andy Jones, James Haywood, and Hansi Singh
EGUsphere, https://doi.org/10.5194/egusphere-2024-1031, https://doi.org/10.5194/egusphere-2024-1031, 2024
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We introduce a protocol to compare computer climate simulations to better understand a proposed strategy intended to counter warming & climate impacts from greenhouse gas increases. The strategy slightly changes clouds in 6 ocean regions to reflect more sunlight & cool Earth. Example changes in clouds & climate are shown for 3 climate models. Clouds change differently between the models, but precipitation and surface temperature changes are similar when their cooling effects are made similar.
John T. Fasullo, Jean-Christophe Golaz, Julie M. Caron, Nan Rosenbloom, Gerald A. Meehl, Warren Strand, Sasha Glanville, Samantha Stevenson, Maria Molina, Christine A. Shields, Chengzhu Zhang, James Benedict, Hailong Wang, and Tony Bartoletti
Earth Syst. Dynam., 15, 367–386, https://doi.org/10.5194/esd-15-367-2024, https://doi.org/10.5194/esd-15-367-2024, 2024
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Climate model large ensembles provide a unique and invaluable means for estimating the climate response to external forcing agents and quantify contrasts in model structure. Here, an overview of the Energy Exascale Earth System Model (E3SM) version 2 large ensemble is given along with comparisons to large ensembles from E3SM version 1 and versions 1 and 2 of the Community Earth System Model. The paper provides broad and important context for users of these ensembles.
Andrew Geiss and Po-Lun Ma
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-30, https://doi.org/10.5194/gmd-2024-30, 2024
Revised manuscript has not been submitted
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Particles in the Earth’s atmosphere strongly impact the planet’s energy budget and atmosphere simulations require accurately representing their interaction with light. This work introduces two approaches to representing light scattering by small particles. The first is a scattering simulation based on Mie theory implemented in Python. The second is a neural network emulator that is more accurate than existing methods and is fast enough to be used in climate and weather simulations.
Johannes Mülmenstädt, Andrew S. Ackerman, Ann M. Fridlind, Meng Huang, Po-Lun Ma, Naser Mahfouz, Susanne E. Bauer, Susannah M. Burrows, Matthew W. Christensen, Sudhakar Dipu, Andrew Gettelman, L. Ruby Leung, Florian Tornow, Johannes Quaas, Adam C. Varble, Hailong Wang, Kai Zhang, and Youtong Zheng
EGUsphere, https://doi.org/10.5194/egusphere-2024-778, https://doi.org/10.5194/egusphere-2024-778, 2024
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Stratocumulus clouds play a large role in Earth's climate by reflecting incoming solar energy back to space. Turbulence at stratocumulus cloud top mixes in drier, warmer air, which can lead to a reduction in cloud. This process is challenging for coarse-resolution global models to represent. We show that global models nevertheless agree well with our process understanding. Global models also think the process is less important for the climate than other lines of evidence had led us to conclude.
Hao Wang, Xiaohong Liu, Chenglai Wu, and Guangxing Lin
Atmos. Chem. Phys., 24, 3309–3328, https://doi.org/10.5194/acp-24-3309-2024, https://doi.org/10.5194/acp-24-3309-2024, 2024
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We quantified different global- and regional-scale drivers of biogenic volatile organic compound (BVOC) emission trends over the past 20 years. The results show that global greening trends significantly boost BVOC emissions and deforestation reduces BVOC emissions in South America and Southeast Asia. Elevated temperature in Europe and increased soil moisture in East and South Asia enhance BVOC emissions. The results deepen our understanding of long-term BVOC emission trends in hotspots.
Yawen Liu, Yun Qian, Philip J. Rasch, Kai Zhang, Lai-yung Ruby Leung, Yuhang Wang, Minghuai Wang, Hailong Wang, Xin Huang, and Xiu-Qun Yang
Atmos. Chem. Phys., 24, 3115–3128, https://doi.org/10.5194/acp-24-3115-2024, https://doi.org/10.5194/acp-24-3115-2024, 2024
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Fire management has long been a challenge. Here we report that spring-peak fire activity over southern Mexico and Central America (SMCA) has a distinct quasi-biennial signal by measuring multiple fire metrics. This signal is initially driven by quasi-biennial variability in precipitation and is further amplified by positive feedback of fire–precipitation interaction at short timescales. This work highlights the importance of fire–climate interactions in shaping fires on an interannual scale.
Yu Yao, Po-Lun Ma, Yi Qin, Matthew W. Christensen, Hui Wan, Kai Zhang, Balwinder Singh, Meng Huang, and Mikhail Ovchinnikov
EGUsphere, https://doi.org/10.5194/egusphere-2024-523, https://doi.org/10.5194/egusphere-2024-523, 2024
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Giant aerosols have substantial effects on warm rain formation. However, it remains challenging to quantify the impact of giant particles at global scale. In this work, we applied earth system model to investigate its impacts by implementing new giant aerosol treatments to consider its physical process. We found this approach substantially affect liquid cloud and improved model's precipitation response to aerosols. Our findings demonstrate the significant impact of giant aerosols on climate.
Kirsten L. Findell, Zun Yin, Eunkyo Seo, Paul A. Dirmeyer, Nathan P. Arnold, Nathaniel Chaney, Megan D. Fowler, Meng Huang, David M. Lawrence, Po-Lun Ma, and Joseph A. Santanello Jr.
Geosci. Model Dev., 17, 1869–1883, https://doi.org/10.5194/gmd-17-1869-2024, https://doi.org/10.5194/gmd-17-1869-2024, 2024
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We outline a request for sub-daily data to accurately capture the process-level connections between land states, surface fluxes, and the boundary layer response. This high-frequency model output will allow for more direct comparison with observational field campaigns on process-relevant timescales, enable demonstration of inter-model spread in land–atmosphere coupling processes, and aid in targeted identification of sources of deficiencies and opportunities for improvement of the models.
Chen Zhang, John J. Cassano, Mark Seefeldt, Hailong Wang, Weiming Ma, and Wen-wen Tung
EGUsphere, https://doi.org/10.5194/egusphere-2024-320, https://doi.org/10.5194/egusphere-2024-320, 2024
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An atmospheric river (AR) is a long, narrow corridor of moisture transport in the atmosphere. ARs are crucial for moisture and heat transport into the polar regions. Our study examines the role of ARs on the surface energy budget (SEB) in the Arctic. The results reveal distinct seasonality and land-sea-sea ice contrasts due to the impacts of ARs on the SEB. The conclusions provide greater insights into the current and future role of ARs on the Arctic climate system.
Hui Wan, Kai Zhang, Christopher J. Vogl, Carol S. Woodward, Richard C. Easter, Philip J. Rasch, Yan Feng, and Hailong Wang
Geosci. Model Dev., 17, 1387–1407, https://doi.org/10.5194/gmd-17-1387-2024, https://doi.org/10.5194/gmd-17-1387-2024, 2024
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Sophisticated numerical models of the Earth's atmosphere include representations of many physical and chemical processes. In numerical simulations, these processes need to be calculated in a certain sequence. This study reveals the weaknesses of the sequence of calculations used for aerosol processes in a global atmosphere model. A revision of the sequence is proposed and its impacts on the simulated global aerosol climatology are evaluated.
Jianfeng Li, Kai Zhang, Taufiq Hassan, Shixuan Zhang, Po-Lun Ma, Balwinder Singh, Qiyang Yan, and Huilin Huang
Geosci. Model Dev., 17, 1327–1347, https://doi.org/10.5194/gmd-17-1327-2024, https://doi.org/10.5194/gmd-17-1327-2024, 2024
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By comparing E3SM simulations with and without regional refinement, we find that model horizontal grid spacing considerably affects the simulated aerosol mass budget, aerosol–cloud interactions, and the effective radiative forcing of anthropogenic aerosols. The study identifies the critical physical processes strongly influenced by model resolution. It also highlights the benefit of applying regional refinement in future modeling studies at higher or even convection-permitting resolutions.
Xinyue Shao, Minghuai Wang, Xinyi Dong, Yaman Liu, Wenxiang Shen, Stephen Arnold, Leighton Regayre, Meinrat Andreae, Mira Pöhlker, Duseong Jo, Man Yue, and Ken Carslaw
EGUsphere, https://doi.org/10.5194/egusphere-2024-401, https://doi.org/10.5194/egusphere-2024-401, 2024
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Highly oxygenated organic molecules (HOMs) play an important role in atmospheric new particle formation (NPF). By explicitly coupling the chemical mechanism of HOMs and a comprehensive nucleation scheme in a global climate model. The updated model shows better agreement with measurements of nucleation rate, growth rate, NPF event frequency. Our results reveal that HOMs-driven NPF leads to a considerable increase in particle and cloud condensation nuclei burden globally.
Huisheng Bian, Mian Chin, Peter R. Colarco, Eric C. Apel, Donald R. Blake, Karl Froyd, Rebecca S. Hornbrook, Jose Jimenez, Pedro Campuzano Jost, Michael Lawler, Mingxu Liu, Marianne Tronstad Lund, Hitoshi Matsui, Benjamin A. Nault, Joyce E. Penner, Andrew W. Rollins, Gregory Schill, Ragnhild B. Skeie, Hailong Wang, Lu Xu, Kai Zhang, and Jialei Zhu
Atmos. Chem. Phys., 24, 1717–1741, https://doi.org/10.5194/acp-24-1717-2024, https://doi.org/10.5194/acp-24-1717-2024, 2024
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This work studies sulfur in the remote troposphere at global and seasonal scales using aircraft measurements and multi-model simulations. The goal is to understand the sulfur cycle over remote oceans, spread of model simulations, and observation–model discrepancies. Such an understanding and comparison with real observations are crucial to narrow down the uncertainties in model sulfur simulations and improve understanding of the sulfur cycle in atmospheric air quality, climate, and ecosystems.
Natalie M. Mahowald, Longlei Li, Julius Vira, Marje Prank, Douglas S. Hamilton, Hitoshi Matsui, Ron L. Miller, Louis Lu, Ezgi Akyuz, Daphne Meidan, Peter Hess, Heikki Lihavainen, Christine Wiedinmyer, Jenny Hand, Maria Grazia Alaimo, Célia Alves, Andres Alastuey, Paulo Artaxo, Africa Barreto, Francisco Barraza, Silvia Becagli, Giulia Calzolai, Shankarararman Chellam, Ying Chen, Patrick Chuang, David D. Cohen, Cristina Colombi, Evangelia Diapouli, Gaetano Dongarra, Konstantinos Eleftheriadis, Corinne Galy-Lacaux, Cassandra Gaston, Dario Gomez, Yenny González Ramos, Hannele Hakola, Roy M. Harrison, Chris Heyes, Barak Herut, Philip Hopke, Christoph Hüglin, Maria Kanakidou, Zsofia Kertesz, Zbiginiw Klimont, Katriina Kyllönen, Fabrice Lambert, Xiaohong Liu, Remi Losno, Franco Lucarelli, Willy Maenhaut, Beatrice Marticorena, Randall V. Martin, Nikolaos Mihalopoulos, Yasser Morera-Gomez, Adina Paytan, Joseph Prospero, Sergio Rodríguez, Patricia Smichowski, Daniela Varrica, Brenna Walsh, Crystal Weagle, and Xi Zhao
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-1, https://doi.org/10.5194/essd-2024-1, 2024
Preprint withdrawn
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Aerosol particles can interact with incoming solar radiation and outgoing long wave radiation, change cloud properties, affect photochemistry, impact surface air quality, and when deposited impact surface albedo of snow and ice, and modulate carbon dioxide uptake by the land and ocean. Here we present a new compilation of aerosol observations including composition, a methodology for comparing the datasets to model output, and show the implications of these results using one model.
Yang Yang, Yang Zhou, Hailong Wang, Mengyun Li, Huimin Li, Pinya Wang, Xu Yue, Ke Li, Jia Zhu, and Hong Liao
Atmos. Chem. Phys., 24, 1177–1191, https://doi.org/10.5194/acp-24-1177-2024, https://doi.org/10.5194/acp-24-1177-2024, 2024
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This study reveals that extreme ozone pollution over the North China Plain and Yangtze River Delta is due to the chemical production related to hot and dry conditions, and the regional transport explains the ozone pollution over the Sichuan Basin and Pearl River Delta. The frequency of meteorological conditions of the extreme ozone pollution increases from the past to the future. The sustainable scenario is the optimal path to retaining clean air in China in the future.
Yuying Zhang, Shaocheng Xie, Yi Qin, Wuyin Lin, Jean-Christophe Golaz, Xue Zheng, Po-Lun Ma, Yun Qian, Qi Tang, Christopher R. Terai, and Meng Zhang
Geosci. Model Dev., 17, 169–189, https://doi.org/10.5194/gmd-17-169-2024, https://doi.org/10.5194/gmd-17-169-2024, 2024
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We performed systematic evaluation of clouds simulated in the Energy
Exascale Earth System Model (E3SMv2) to document model performance and understand what updates in E3SMv2 have caused changes in clouds from E3SMv1 to E3SMv2. We find that stratocumulus clouds along the subtropical west coast of continents are dramatically improved, primarily due to the retuning done in CLUBB. This study offers additional insights into clouds simulated in E3SMv2 and will benefit future E3SM developments.
Exascale Earth System Model (E3SMv2) to document model performance and understand what updates in E3SMv2 have caused changes in clouds from E3SMv1 to E3SMv2. We find that stratocumulus clouds along the subtropical west coast of continents are dramatically improved, primarily due to the retuning done in CLUBB. This study offers additional insights into clouds simulated in E3SMv2 and will benefit future E3SM developments.
Shuaiqi Tang, Hailong Wang, Xiang-Yu Li, Jingyi Chen, Armin Sorooshian, Xubin Zeng, Ewan Crosbie, Kenneth L. Thornhill, Luke D. Ziemba, and Christiane Voigt
EGUsphere, https://doi.org/10.5194/egusphere-2023-3149, https://doi.org/10.5194/egusphere-2023-3149, 2024
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We examined marine boundary-layer clouds and their interactions with aerosols in the E3SM single-column model (SCM) for a case study. The SCM shows good agreement in simulating the clouds with high-resolution models. It reproduces the relationship between cloud droplet and aerosol particle number concentrations as produced in global models. However, the relationship between cloud liquid water and droplet number concentration are different, which warrants further investigation.
Jim M. Haywood, Andy Jones, Anthony C. Jones, Paul Halloran, and Philip J. Rasch
Atmos. Chem. Phys., 23, 15305–15324, https://doi.org/10.5194/acp-23-15305-2023, https://doi.org/10.5194/acp-23-15305-2023, 2023
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The difficulties in ameliorating global warming and the associated climate change via conventional mitigation are well documented, with all climate model scenarios exceeding 1.5 °C above the preindustrial level in the near future. There is therefore a growing interest in geoengineering to reflect a greater proportion of sunlight back to space and offset some of the global warming. We use a state-of-the-art Earth-system model to investigate two of the most prominent geoengineering strategies.
Hamza Ahsan, Hailong Wang, Jingbo Wu, Mingxuan Wu, Steven J. Smith, Susanne Bauer, Harrison Suchyta, Dirk Olivié, Gunnar Myhre, Hitoshi Matsui, Huisheng Bian, Jean-François Lamarque, Ken Carslaw, Larry Horowitz, Leighton Regayre, Mian Chin, Michael Schulz, Ragnhild Bieltvedt Skeie, Toshihiko Takemura, and Vaishali Naik
Atmos. Chem. Phys., 23, 14779–14799, https://doi.org/10.5194/acp-23-14779-2023, https://doi.org/10.5194/acp-23-14779-2023, 2023
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We examine the impact of the assumed effective height of SO2 injection, SO2 and BC emission seasonality, and the assumed fraction of SO2 emissions injected as SO4 on climate and chemistry model results. We find that the SO2 injection height has a large impact on surface SO2 concentrations and, in some models, radiative flux. These assumptions are a
hiddensource of inter-model variability and may be leading to bias in some climate model results.
Shuaiqi Tang, Adam C. Varble, Jerome D. Fast, Kai Zhang, Peng Wu, Xiquan Dong, Fan Mei, Mikhail Pekour, Joseph C. Hardin, and Po-Lun Ma
Geosci. Model Dev., 16, 6355–6376, https://doi.org/10.5194/gmd-16-6355-2023, https://doi.org/10.5194/gmd-16-6355-2023, 2023
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To assess the ability of Earth system model (ESM) predictions, we developed a tool called ESMAC Diags to understand how aerosols, clouds, and aerosol–cloud interactions are represented in ESMs. This paper describes its version 2 functionality. We compared the model predictions with measurements taken by planes, ships, satellites, and ground instruments over four regions across the world. Results show that this new tool can help identify model problems and guide future development of ESMs.
Simone Tilmes, Michael J. Mills, Yunqian Zhu, Charles G. Bardeen, Francis Vitt, Pengfei Yu, David Fillmore, Xiaohong Liu, Brian Toon, and Terry Deshler
Geosci. Model Dev., 16, 6087–6125, https://doi.org/10.5194/gmd-16-6087-2023, https://doi.org/10.5194/gmd-16-6087-2023, 2023
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We implemented an alternative aerosol scheme in the high- and low-top model versions of the Community Earth System Model Version 2 (CESM2) with a more detailed description of tropospheric and stratospheric aerosol size distributions than the existing aerosol model. This development enables the comparison of different aerosol schemes with different complexity in the same model framework. It identifies improvements compared to a range of observations in both the troposphere and stratosphere.
Adam C. Varble, Po-Lun Ma, Matthew W. Christensen, Johannes Mülmenstädt, Shuaiqi Tang, and Jerome Fast
Atmos. Chem. Phys., 23, 13523–13553, https://doi.org/10.5194/acp-23-13523-2023, https://doi.org/10.5194/acp-23-13523-2023, 2023
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We evaluate how clouds change in response to changing atmospheric particle (aerosol) concentrations in a climate model and find that the model-predicted cloud brightness increases too much as aerosols increase because the cloud drop number increases too much. Excessive drizzle in the model mutes this difference. Many differences between observational and model estimates are explained by varying assumptions of how much liquid has been lost in clouds, which impacts the estimated cloud drop number.
Armin Sorooshian, Mikhail D. Alexandrov, Adam D. Bell, Ryan Bennett, Grace Betito, Sharon P. Burton, Megan E. Buzanowicz, Brian Cairns, Eduard V. Chemyakin, Gao Chen, Yonghoon Choi, Brian L. Collister, Anthony L. Cook, Andrea F. Corral, Ewan C. Crosbie, Bastiaan van Diedenhoven, Joshua P. DiGangi, Glenn S. Diskin, Sanja Dmitrovic, Eva-Lou Edwards, Marta A. Fenn, Richard A. Ferrare, David van Gilst, Johnathan W. Hair, David B. Harper, Miguel Ricardo A. Hilario, Chris A. Hostetler, Nathan Jester, Michael Jones, Simon Kirschler, Mary M. Kleb, John M. Kusterer, Sean Leavor, Joseph W. Lee, Hongyu Liu, Kayla McCauley, Richard H. Moore, Joseph Nied, Anthony Notari, John B. Nowak, David Painemal, Kasey E. Phillips, Claire E. Robinson, Amy Jo Scarino, Joseph S. Schlosser, Shane T. Seaman, Chellappan Seethala, Taylor J. Shingler, Michael A. Shook, Kenneth A. Sinclair, William L. Smith Jr., Douglas A. Spangenberg, Snorre A. Stamnes, Kenneth L. Thornhill, Christiane Voigt, Holger Vömel, Andrzej P. Wasilewski, Hailong Wang, Edward L. Winstead, Kira Zeider, Xubin Zeng, Bo Zhang, Luke D. Ziemba, and Paquita Zuidema
Earth Syst. Sci. Data, 15, 3419–3472, https://doi.org/10.5194/essd-15-3419-2023, https://doi.org/10.5194/essd-15-3419-2023, 2023
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The NASA Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) produced a unique dataset for research into aerosol–cloud–meteorology interactions. HU-25 Falcon and King Air aircraft conducted systematic and spatially coordinated flights over the northwest Atlantic Ocean. This paper describes the ACTIVATE flight strategy, instrument and complementary dataset products, data access and usage details, and data application notes.
Qi Tang, Jean-Christophe Golaz, Luke P. Van Roekel, Mark A. Taylor, Wuyin Lin, Benjamin R. Hillman, Paul A. Ullrich, Andrew M. Bradley, Oksana Guba, Jonathan D. Wolfe, Tian Zhou, Kai Zhang, Xue Zheng, Yunyan Zhang, Meng Zhang, Mingxuan Wu, Hailong Wang, Cheng Tao, Balwinder Singh, Alan M. Rhoades, Yi Qin, Hong-Yi Li, Yan Feng, Yuying Zhang, Chengzhu Zhang, Charles S. Zender, Shaocheng Xie, Erika L. Roesler, Andrew F. Roberts, Azamat Mametjanov, Mathew E. Maltrud, Noel D. Keen, Robert L. Jacob, Christiane Jablonowski, Owen K. Hughes, Ryan M. Forsyth, Alan V. Di Vittorio, Peter M. Caldwell, Gautam Bisht, Renata B. McCoy, L. Ruby Leung, and David C. Bader
Geosci. Model Dev., 16, 3953–3995, https://doi.org/10.5194/gmd-16-3953-2023, https://doi.org/10.5194/gmd-16-3953-2023, 2023
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High-resolution simulations are superior to low-resolution ones in capturing regional climate changes and climate extremes. However, uniformly reducing the grid size of a global Earth system model is too computationally expensive. We provide an overview of the fully coupled regionally refined model (RRM) of E3SMv2 and document a first-of-its-kind set of climate production simulations using RRM at an economic cost. The key to this success is our innovative hybrid time step method.
Aishwarya Raman, Thomas Hill, Paul J. DeMott, Balwinder Singh, Kai Zhang, Po-Lun Ma, Mingxuan Wu, Hailong Wang, Simon P. Alexander, and Susannah M. Burrows
Atmos. Chem. Phys., 23, 5735–5762, https://doi.org/10.5194/acp-23-5735-2023, https://doi.org/10.5194/acp-23-5735-2023, 2023
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Ice-nucleating particles (INPs) play an important role in cloud processes and associated precipitation. Yet, INPs are not accurately represented in climate models. This study attempts to uncover these gaps by comparing model-simulated INP concentrations against field campaign measurements in the SO for an entire year, 2017–2018. Differences in INP concentrations and variability between the model and observations have major implications for modeling cloud properties in high latitudes.
Pengwei Li, Yang Yang, Hailong Wang, Su Li, Ke Li, Pinya Wang, Baojie Li, and Hong Liao
Atmos. Chem. Phys., 23, 5403–5417, https://doi.org/10.5194/acp-23-5403-2023, https://doi.org/10.5194/acp-23-5403-2023, 2023
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We use a novel technique that can attribute O3 to precursors to investigate O3 changes in the United States during 1995–2019. We found that the US domestic energy and surface transportation emission reductions are primarily responsible for the O3 decrease in summer. In winter, factors such as nitrogen oxide emission reduction in the context of its inhibition of ozone production, increased aviation and shipping activities, and large-scale circulation changes contribute to the O3 increases.
Andrew Geiss, Po-Lun Ma, Balwinder Singh, and Joseph C. Hardin
Geosci. Model Dev., 16, 2355–2370, https://doi.org/10.5194/gmd-16-2355-2023, https://doi.org/10.5194/gmd-16-2355-2023, 2023
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Atmospheric aerosols play a critical role in Earth's climate, but it is too computationally expensive to directly model their interaction with radiation in climate simulations. This work develops a new neural-network-based parameterization of aerosol optical properties for use in the Energy Exascale Earth System Model that is much more accurate than the current one; it also introduces a unique model optimization method that involves randomly generating neural network architectures.
Matthew W. Christensen, Po-Lun Ma, Peng Wu, Adam C. Varble, Johannes Mülmenstädt, and Jerome D. Fast
Atmos. Chem. Phys., 23, 2789–2812, https://doi.org/10.5194/acp-23-2789-2023, https://doi.org/10.5194/acp-23-2789-2023, 2023
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An increase in aerosol concentration (tiny airborne particles) is shown to suppress rainfall and increase the abundance of droplets in clouds passing over Graciosa Island in the Azores. Cloud drops remain affected by aerosol for several days across thousands of kilometers in satellite data. Simulations from an Earth system model show good agreement, but differences in the amount of cloud water and its extent remain despite modifications to model parameters that control the warm-rain process.
Marine Bonazzola, Hélène Chepfer, Po-Lun Ma, Johannes Quaas, David M. Winker, Artem Feofilov, and Nick Schutgens
Geosci. Model Dev., 16, 1359–1377, https://doi.org/10.5194/gmd-16-1359-2023, https://doi.org/10.5194/gmd-16-1359-2023, 2023
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Aerosol has a large impact on climate. Using a lidar aerosol simulator ensures consistent comparisons between modeled and observed aerosol. We present a lidar aerosol simulator that applies a cloud masking and an aerosol detection threshold. We estimate the lidar signals that would be observed at 532 nm by the Cloud-Aerosol Lidar with Orthogonal Polarization overflying the atmosphere predicted by a climate model. Our comparison at the seasonal timescale shows a discrepancy in the Southern Ocean.
Chandan Sarangi, Yun Qian, L. Ruby Leung, Yang Zhang, Yufei Zou, and Yuhang Wang
Atmos. Chem. Phys., 23, 1769–1783, https://doi.org/10.5194/acp-23-1769-2023, https://doi.org/10.5194/acp-23-1769-2023, 2023
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We show that for air quality, the densely populated eastern US may see even larger impacts of wildfires due to long-distance smoke transport and associated positive climatic impacts, partially compensating the improvements from regulations on anthropogenic emissions. This study highlights the tension between natural and anthropogenic contributions and the non-local nature of air pollution that complicate regulatory strategies for improving future regional air quality for human health.
Mengyun Li, Yang Yang, Hailong Wang, Huimin Li, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 23, 1533–1544, https://doi.org/10.5194/acp-23-1533-2023, https://doi.org/10.5194/acp-23-1533-2023, 2023
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Using the GEOS-Chem model, the impact of the quasi-biennial oscillation (QBO) on summertime tropospheric O3 in China is investigated. In the warm phases of sea surface temperature anomalies over the eastern tropical Pacific, the QBO has a significant positive correlation with near-surface O3 concentrations over central China. The QBO impacts on O3 pollution in China are mainly a result of changing vertical transport of O3.
Huimin Li, Yang Yang, Jianbing Jin, Hailong Wang, Ke Li, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 23, 1131–1145, https://doi.org/10.5194/acp-23-1131-2023, https://doi.org/10.5194/acp-23-1131-2023, 2023
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Future climate change will aggravate ozone pollution in Asia, especially in high-forcing scenarios. Ozone pollution in China will expand from North China to South China and extend into the cold season in a warmer future. The emphasis of this work is to quantify the impacts of future climate change on O3 pollution in Asia, which is of great significance for future O3 pollution mitigation strategies.
Younjoo J. Lee, Wieslaw Maslowski, John J. Cassano, Jaclyn Clement Kinney, Anthony P. Craig, Samy Kamal, Robert Osinski, Mark W. Seefeldt, Julienne Stroeve, and Hailong Wang
The Cryosphere, 17, 233–253, https://doi.org/10.5194/tc-17-233-2023, https://doi.org/10.5194/tc-17-233-2023, 2023
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During 1979–2020, four winter polynyas occurred in December 1986 and February 2011, 2017, and 2018 north of Greenland. Instead of ice melting due to the anomalous warm air intrusion, the extreme wind forcing resulted in greater ice transport offshore. Based on the two ensemble runs, representing a 1980s thicker ice vs. a 2010s thinner ice, a dominant cause of these winter polynyas stems from internal variability of atmospheric forcing rather than from the forced response to a warming climate.
Dalei Hao, Gautam Bisht, Karl Rittger, Edward Bair, Cenlin He, Huilin Huang, Cheng Dang, Timbo Stillinger, Yu Gu, Hailong Wang, Yun Qian, and L. Ruby Leung
Geosci. Model Dev., 16, 75–94, https://doi.org/10.5194/gmd-16-75-2023, https://doi.org/10.5194/gmd-16-75-2023, 2023
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Snow with the highest albedo of land surface plays a vital role in Earth’s surface energy budget and water cycle. This study accounts for the impacts of snow grain shape and mixing state of light-absorbing particles with snow on snow albedo in the E3SM land model. The findings advance our understanding of the role of snow grain shape and mixing state of LAP–snow in land surface processes and offer guidance for improving snow simulations and radiative forcing estimates in Earth system models.
Huilin Huang, Yun Qian, Ye Liu, Cenlin He, Jianyu Zheng, Zhibo Zhang, and Antonis Gkikas
Atmos. Chem. Phys., 22, 15469–15488, https://doi.org/10.5194/acp-22-15469-2022, https://doi.org/10.5194/acp-22-15469-2022, 2022
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Using a clustering method developed in the field of artificial neural networks, we identify four typical dust transport patterns across the Sierra Nevada, associated with the mesoscale and regional-scale wind circulations. Our results highlight the connection between dust transport and dominant weather patterns, which can be used to understand dust transport in a changing climate.
Longlei Li, Natalie M. Mahowald, Jasper F. Kok, Xiaohong Liu, Mingxuan Wu, Danny M. Leung, Douglas S. Hamilton, Louisa K. Emmons, Yue Huang, Neil Sexton, Jun Meng, and Jessica Wan
Geosci. Model Dev., 15, 8181–8219, https://doi.org/10.5194/gmd-15-8181-2022, https://doi.org/10.5194/gmd-15-8181-2022, 2022
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This study advances mineral dust parameterizations in the Community Atmospheric Model (CAM; version 6.1). Efforts include 1) incorporating a more physically based dust emission scheme; 2) updating the dry deposition scheme; and 3) revising the gravitational settling velocity to account for dust asphericity. Substantial improvements achieved with these updates can help accurately quantify dust–climate interactions using CAM, such as the dust-radiation and dust–cloud interactions.
Yang Yang, Liangying Zeng, Hailong Wang, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 22, 14489–14502, https://doi.org/10.5194/acp-22-14489-2022, https://doi.org/10.5194/acp-22-14489-2022, 2022
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Using an aerosol–climate model, dust pollution in China affected by different spatial and temporal types of El Niño are examined. Both eastern and central Pacific El Niño and short-duration El Niño increase winter dust concentrations over northern China, while long-duration El Niño decreases concentrations. Only long-duration El Niño events can significantly affect dust over China in the following spring. This study has profound implications for air pollution control and dust storm prediction.
Meng Huang, Po-Lun Ma, Nathaniel W. Chaney, Dalei Hao, Gautam Bisht, Megan D. Fowler, Vincent E. Larson, and L. Ruby Leung
Geosci. Model Dev., 15, 6371–6384, https://doi.org/10.5194/gmd-15-6371-2022, https://doi.org/10.5194/gmd-15-6371-2022, 2022
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The land surface in one grid cell may be diverse in character. This study uses an explicit way to account for that subgrid diversity in a state-of-the-art Earth system model (ESM) and explores its implications for the overlying atmosphere. We find that the shallow clouds are increased significantly with the land surface diversity. Our work highlights the importance of accurately representing the land surface and its interaction with the atmosphere in next-generation ESMs.
Kai Zhang, Wentao Zhang, Hui Wan, Philip J. Rasch, Steven J. Ghan, Richard C. Easter, Xiangjun Shi, Yong Wang, Hailong Wang, Po-Lun Ma, Shixuan Zhang, Jian Sun, Susannah M. Burrows, Manish Shrivastava, Balwinder Singh, Yun Qian, Xiaohong Liu, Jean-Christophe Golaz, Qi Tang, Xue Zheng, Shaocheng Xie, Wuyin Lin, Yan Feng, Minghuai Wang, Jin-Ho Yoon, and L. Ruby Leung
Atmos. Chem. Phys., 22, 9129–9160, https://doi.org/10.5194/acp-22-9129-2022, https://doi.org/10.5194/acp-22-9129-2022, 2022
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Here we analyze the effective aerosol forcing simulated by E3SM version 1 using both century-long free-running and short nudged simulations. The aerosol forcing in E3SMv1 is relatively large compared to other models, mainly due to the large indirect aerosol effect. Aerosol-induced changes in liquid and ice cloud properties in E3SMv1 have a strong correlation. The aerosol forcing estimates in E3SMv1 are sensitive to the parameterization changes in both liquid and ice cloud processes.
Jiyuan Gao, Yang Yang, Hailong Wang, Pinya Wang, Huimin Li, Mengyun Li, Lili Ren, Xu Yue, and Hong Liao
Atmos. Chem. Phys., 22, 7131–7142, https://doi.org/10.5194/acp-22-7131-2022, https://doi.org/10.5194/acp-22-7131-2022, 2022
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China has been implementing a sequence of policies for clean air since the year 2013. The aerosol decline produced a 0.09 ± 0.10°C warming during 2013–2017 estimated in this study, and the increase in ozone in the lower troposphere during this time period accelerated the warming, leading to a total 0.16 ± 0.15°C temperature increase in eastern China. Residential emission reductions led to a cooling effect because of a substantial decrease in light-absorbing aerosols.
Shuaiqi Tang, Jerome D. Fast, Kai Zhang, Joseph C. Hardin, Adam C. Varble, John E. Shilling, Fan Mei, Maria A. Zawadowicz, and Po-Lun Ma
Geosci. Model Dev., 15, 4055–4076, https://doi.org/10.5194/gmd-15-4055-2022, https://doi.org/10.5194/gmd-15-4055-2022, 2022
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We developed an Earth system model (ESM) diagnostics package to compare various types of aerosol properties simulated in ESMs with aircraft, ship, and surface measurements from six field campaigns across spatial scales. The diagnostics package is coded and organized to be flexible and modular for future extension to other field campaign datasets and adapted to higher-resolution model simulations. Future releases will include comprehensive cloud and aerosol–cloud interaction diagnostics.
Xue Zheng, Qing Li, Tian Zhou, Qi Tang, Luke P. Van Roekel, Jean-Christophe Golaz, Hailong Wang, and Philip Cameron-Smith
Geosci. Model Dev., 15, 3941–3967, https://doi.org/10.5194/gmd-15-3941-2022, https://doi.org/10.5194/gmd-15-3941-2022, 2022
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We document the model experiments for the future climate projection by E3SMv1.0. At the highest future emission scenario, E3SMv1.0 projects a strong surface warming with rapid changes in the atmosphere, ocean, sea ice, and land runoff. Specifically, we detect a significant polar amplification and accelerated warming linked to the unmasking of the aerosol effects. The impact of greenhouse gas forcing is examined in different climate components.
Susannah M. Burrows, Richard C. Easter, Xiaohong Liu, Po-Lun Ma, Hailong Wang, Scott M. Elliott, Balwinder Singh, Kai Zhang, and Philip J. Rasch
Atmos. Chem. Phys., 22, 5223–5251, https://doi.org/10.5194/acp-22-5223-2022, https://doi.org/10.5194/acp-22-5223-2022, 2022
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Sea spray particles are composed of a mixture of salts and organic substances from oceanic microorganisms. In prior work, our team developed an approach connecting sea spray chemistry to ocean biology, called OCEANFILMS. Here we describe its implementation within an Earth system model, E3SM. We show that simulated sea spray chemistry is consistent with observed seasonal cycles and that sunlight reflected by simulated Southern Ocean clouds increases, consistent with analysis of satellite data.
Hui Wan, Kai Zhang, Philip J. Rasch, Vincent E. Larson, Xubin Zeng, Shixuan Zhang, and Ross Dixon
Geosci. Model Dev., 15, 3205–3231, https://doi.org/10.5194/gmd-15-3205-2022, https://doi.org/10.5194/gmd-15-3205-2022, 2022
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This paper describes a tool embedded in a global climate model for sampling atmospheric conditions and monitoring physical processes as a numerical simulation is being carried out. The tool facilitates process-level model evaluation by allowing the users to select a wide range of quantities and processes to monitor at run time without having to do tedious ad hoc coding.
Po-Lun Ma, Bryce E. Harrop, Vincent E. Larson, Richard B. Neale, Andrew Gettelman, Hugh Morrison, Hailong Wang, Kai Zhang, Stephen A. Klein, Mark D. Zelinka, Yuying Zhang, Yun Qian, Jin-Ho Yoon, Christopher R. Jones, Meng Huang, Sheng-Lun Tai, Balwinder Singh, Peter A. Bogenschutz, Xue Zheng, Wuyin Lin, Johannes Quaas, Hélène Chepfer, Michael A. Brunke, Xubin Zeng, Johannes Mülmenstädt, Samson Hagos, Zhibo Zhang, Hua Song, Xiaohong Liu, Michael S. Pritchard, Hui Wan, Jingyu Wang, Qi Tang, Peter M. Caldwell, Jiwen Fan, Larry K. Berg, Jerome D. Fast, Mark A. Taylor, Jean-Christophe Golaz, Shaocheng Xie, Philip J. Rasch, and L. Ruby Leung
Geosci. Model Dev., 15, 2881–2916, https://doi.org/10.5194/gmd-15-2881-2022, https://doi.org/10.5194/gmd-15-2881-2022, 2022
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An alternative set of parameters for E3SM Atmospheric Model version 1 has been developed based on a tuning strategy that focuses on clouds. When clouds in every regime are improved, other aspects of the model are also improved, even though they are not the direct targets for calibration. The recalibrated model shows a lower sensitivity to anthropogenic aerosols and surface warming, suggesting potential improvements to the simulated climate in the past and future.
Sally S.-C. Wang, Yun Qian, L. Ruby Leung, and Yang Zhang
Atmos. Chem. Phys., 22, 3445–3468, https://doi.org/10.5194/acp-22-3445-2022, https://doi.org/10.5194/acp-22-3445-2022, 2022
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This study develops an interpretable machine learning (ML) model predicting monthly PM2.5 fire emission over the contiguous US at 0.25° resolution and compares the prediction skills of the ML and process-based models. The comparison facilitates attributions of model biases and better understanding of the strengths and uncertainties in the two types of models at regional scales, for informing future model development and their applications in fire emission projection.
Yang Shi, Xiaohong Liu, Mingxuan Wu, Xi Zhao, Ziming Ke, and Hunter Brown
Atmos. Chem. Phys., 22, 2909–2935, https://doi.org/10.5194/acp-22-2909-2022, https://doi.org/10.5194/acp-22-2909-2022, 2022
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We perform a modeling study to evaluate the contribution to Arctic dust loading and ice-nucleating particle (INP) population from high-latitude local and low-latitude dust. High-latitude dust has a large contribution in the lower troposphere, while low-latitude dust dominates the upper troposphere. The high-latitude dust INPs result in a net cooling effect on the Arctic surface by glaciating mixed-phase clouds. Our results highlight the contribution of high-latitude dust to the Arctic climate.
Artem G. Feofilov, Hélène Chepfer, Vincent Noël, Rodrigo Guzman, Cyprien Gindre, Po-Lun Ma, and Marjolaine Chiriaco
Atmos. Meas. Tech., 15, 1055–1074, https://doi.org/10.5194/amt-15-1055-2022, https://doi.org/10.5194/amt-15-1055-2022, 2022
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Space-borne lidars have been providing invaluable information of atmospheric optical properties since 2006, and new lidar missions are on the way to ensure continuous observations. In this work, we compare the clouds estimated from space-borne ALADIN and CALIOP lidar observations. The analysis of collocated data shows that the agreement between the retrieved clouds is good up to 3 km height. Above that, ALADIN detects 40 % less clouds than CALIOP, except for polar stratospheric clouds (PSCs).
Xi Zhao and Xiaohong Liu
Atmos. Chem. Phys., 22, 2585–2600, https://doi.org/10.5194/acp-22-2585-2022, https://doi.org/10.5194/acp-22-2585-2022, 2022
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The goal of this study is to investigate the relative importance and interactions of primary and secondary ice production in the Arctic mixed-phase clouds. Our results show that the SIP is not only a result of ice crystals produced from ice nucleation, but also competes with the ice production; conversely, strong ice nucleation also suppresses SIP.
Ka Ming Fung, Colette L. Heald, Jesse H. Kroll, Siyuan Wang, Duseong S. Jo, Andrew Gettelman, Zheng Lu, Xiaohong Liu, Rahul A. Zaveri, Eric C. Apel, Donald R. Blake, Jose-Luis Jimenez, Pedro Campuzano-Jost, Patrick R. Veres, Timothy S. Bates, John E. Shilling, and Maria Zawadowicz
Atmos. Chem. Phys., 22, 1549–1573, https://doi.org/10.5194/acp-22-1549-2022, https://doi.org/10.5194/acp-22-1549-2022, 2022
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Understanding the natural aerosol burden in the preindustrial era is crucial for us to assess how atmospheric aerosols affect the Earth's radiative budgets. Our study explores how a detailed description of dimethyl sulfide (DMS) oxidation (implemented in the Community Atmospheric Model version 6 with chemistry, CAM6-chem) could help us better estimate the present-day and preindustrial concentrations of sulfate and other relevant chemicals, as well as the resulting aerosol radiative impacts.
Ye Liu, Yun Qian, and Larry K. Berg
Wind Energ. Sci., 7, 37–51, https://doi.org/10.5194/wes-7-37-2022, https://doi.org/10.5194/wes-7-37-2022, 2022
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Uncertainties in initial conditions (ICs) decrease the accuracy of wind speed forecasts. We find that IC uncertainties can alter wind speed by modulating the weather system. IC uncertainties in local thermal gradient and large-scale circulation jointly contribute to wind speed forecast uncertainties. Wind forecast accuracy in the Columbia River Basin is confined by initial uncertainties in a few specific regions, providing useful information for more intense measurement and modeling studies.
Matthew W. Christensen, Andrew Gettelman, Jan Cermak, Guy Dagan, Michael Diamond, Alyson Douglas, Graham Feingold, Franziska Glassmeier, Tom Goren, Daniel P. Grosvenor, Edward Gryspeerdt, Ralph Kahn, Zhanqing Li, Po-Lun Ma, Florent Malavelle, Isabel L. McCoy, Daniel T. McCoy, Greg McFarquhar, Johannes Mülmenstädt, Sandip Pal, Anna Possner, Adam Povey, Johannes Quaas, Daniel Rosenfeld, Anja Schmidt, Roland Schrödner, Armin Sorooshian, Philip Stier, Velle Toll, Duncan Watson-Parris, Robert Wood, Mingxi Yang, and Tianle Yuan
Atmos. Chem. Phys., 22, 641–674, https://doi.org/10.5194/acp-22-641-2022, https://doi.org/10.5194/acp-22-641-2022, 2022
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Trace gases and aerosols (tiny airborne particles) are released from a variety of point sources around the globe. Examples include volcanoes, industrial chimneys, forest fires, and ship stacks. These sources provide opportunistic experiments with which to quantify the role of aerosols in modifying cloud properties. We review the current state of understanding on the influence of aerosol on climate built from the wide range of natural and anthropogenic laboratories investigated in recent decades.
Zhonghua Zheng, Matthew West, Lei Zhao, Po-Lun Ma, Xiaohong Liu, and Nicole Riemer
Atmos. Chem. Phys., 21, 17727–17741, https://doi.org/10.5194/acp-21-17727-2021, https://doi.org/10.5194/acp-21-17727-2021, 2021
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Aerosol mixing state is an important emergent property that affects aerosol radiative forcing and aerosol–cloud interactions, but it has not been easy to constrain this property globally. We present a framework for evaluating the error in aerosol mixing state induced by aerosol representation assumptions, which is one of the important contributors to structural uncertainty in aerosol models. Our study provides insights into potential improvements to model process representation for aerosols.
Hossein Dadashazar, Majid Alipanah, Miguel Ricardo A. Hilario, Ewan Crosbie, Simon Kirschler, Hongyu Liu, Richard H. Moore, Andrew J. Peters, Amy Jo Scarino, Michael Shook, K. Lee Thornhill, Christiane Voigt, Hailong Wang, Edward Winstead, Bo Zhang, Luke Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 21, 16121–16141, https://doi.org/10.5194/acp-21-16121-2021, https://doi.org/10.5194/acp-21-16121-2021, 2021
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This study investigates precipitation impacts on long-range transport of North American outflow over the western North Atlantic Ocean (WNAO). Results demonstrate that precipitation scavenging plays a significant role in modifying surface aerosol concentrations over the WNAO, especially in winter and spring due to large-scale scavenging processes. This study highlights how precipitation impacts surface aerosol properties with relevance for other marine regions vulnerable to continental outflow.
Lili Ren, Yang Yang, Hailong Wang, Pinya Wang, Lei Chen, Jia Zhu, and Hong Liao
Atmos. Chem. Phys., 21, 15431–15445, https://doi.org/10.5194/acp-21-15431-2021, https://doi.org/10.5194/acp-21-15431-2021, 2021
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Due to the COVID-19 pandemic, human activities were strictly restricted in China. Even though anthropogenic aerosol emissions largely decreased, haze events still occurred. Our results shows that PM2.5 over the North China Plain is largely contributed by local sources. For other regions in China, PM2.5 is largely contributed from nonlocal sources. As emission reduction is a future goal, aerosol long-range transport and unfavorable meteorology are increasingly important to air quality.
Yongkang Xue, Tandong Yao, Aaron A. Boone, Ismaila Diallo, Ye Liu, Xubin Zeng, William K. M. Lau, Shiori Sugimoto, Qi Tang, Xiaoduo Pan, Peter J. van Oevelen, Daniel Klocke, Myung-Seo Koo, Tomonori Sato, Zhaohui Lin, Yuhei Takaya, Constantin Ardilouze, Stefano Materia, Subodh K. Saha, Retish Senan, Tetsu Nakamura, Hailan Wang, Jing Yang, Hongliang Zhang, Mei Zhao, Xin-Zhong Liang, J. David Neelin, Frederic Vitart, Xin Li, Ping Zhao, Chunxiang Shi, Weidong Guo, Jianping Tang, Miao Yu, Yun Qian, Samuel S. P. Shen, Yang Zhang, Kun Yang, Ruby Leung, Yuan Qiu, Daniele Peano, Xin Qi, Yanling Zhan, Michael A. Brunke, Sin Chan Chou, Michael Ek, Tianyi Fan, Hong Guan, Hai Lin, Shunlin Liang, Helin Wei, Shaocheng Xie, Haoran Xu, Weiping Li, Xueli Shi, Paulo Nobre, Yan Pan, Yi Qin, Jeff Dozier, Craig R. Ferguson, Gianpaolo Balsamo, Qing Bao, Jinming Feng, Jinkyu Hong, Songyou Hong, Huilin Huang, Duoying Ji, Zhenming Ji, Shichang Kang, Yanluan Lin, Weiguang Liu, Ryan Muncaster, Patricia de Rosnay, Hiroshi G. Takahashi, Guiling Wang, Shuyu Wang, Weicai Wang, Xu Zhou, and Yuejian Zhu
Geosci. Model Dev., 14, 4465–4494, https://doi.org/10.5194/gmd-14-4465-2021, https://doi.org/10.5194/gmd-14-4465-2021, 2021
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The subseasonal prediction of extreme hydroclimate events such as droughts/floods has remained stubbornly low for years. This paper presents a new international initiative which, for the first time, introduces spring land surface temperature anomalies over high mountains to improve precipitation prediction through remote effects of land–atmosphere interactions. More than 40 institutions worldwide are participating in this effort. The experimental protocol and preliminary results are presented.
Liangying Zeng, Yang Yang, Hailong Wang, Jing Wang, Jing Li, Lili Ren, Huimin Li, Yang Zhou, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 21, 10745–10761, https://doi.org/10.5194/acp-21-10745-2021, https://doi.org/10.5194/acp-21-10745-2021, 2021
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Using an aerosol–climate model, the impacts of El Niño with different durations on aerosols in China are examined. The modulation on aerosol concentrations and haze days by short-duration El Niño events is 2–3 times more than that by long-duration El Niño events in China. The frequency of short-duration El Niño has been increasing significantly in recent decades, suggesting that El Niño events have exerted increasingly intense modulation on aerosol pollution in China over the past few decades.
Hossein Dadashazar, David Painemal, Majid Alipanah, Michael Brunke, Seethala Chellappan, Andrea F. Corral, Ewan Crosbie, Simon Kirschler, Hongyu Liu, Richard H. Moore, Claire Robinson, Amy Jo Scarino, Michael Shook, Kenneth Sinclair, K. Lee Thornhill, Christiane Voigt, Hailong Wang, Edward Winstead, Xubin Zeng, Luke Ziemba, Paquita Zuidema, and Armin Sorooshian
Atmos. Chem. Phys., 21, 10499–10526, https://doi.org/10.5194/acp-21-10499-2021, https://doi.org/10.5194/acp-21-10499-2021, 2021
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This study investigates the seasonal cycle of cloud drop number concentration (Nd) over the western North Atlantic Ocean (WNAO) using multiple datasets. Reasons for the puzzling discrepancy between the seasonal cycles of Nd and aerosol concentration were identified. Results indicate that Nd is highest in winter (when aerosol proxy values are often lowest) due to conditions both linked to cold-air outbreaks and that promote greater droplet activation.
Raghavendra Krishnamurthy, Rob K. Newsom, Larry K. Berg, Heng Xiao, Po-Lun Ma, and David D. Turner
Atmos. Meas. Tech., 14, 4403–4424, https://doi.org/10.5194/amt-14-4403-2021, https://doi.org/10.5194/amt-14-4403-2021, 2021
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Planetary boundary layer (PBL) height is a critical parameter in atmospheric models. Continuous PBL height measurements from remote sensing measurements are important to understand various boundary layer mechanisms, especially during daytime and evening transition periods. Due to several limitations in existing methodologies to detect PBL height from a Doppler lidar, in this study, a machine learning (ML) approach is tested. The ML model is observed to improve the accuracy by over 50 %.
Sam J. Silva, Po-Lun Ma, Joseph C. Hardin, and Daniel Rothenberg
Geosci. Model Dev., 14, 3067–3077, https://doi.org/10.5194/gmd-14-3067-2021, https://doi.org/10.5194/gmd-14-3067-2021, 2021
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The activation of aerosol into cloud droplets is an important but uncertain process in the Earth system. The physical and chemical interactions that govern this process are too computationally expensive to explicitly resolve in modern Earth system models. Here, we demonstrate how hybrid machine learning approaches can provide a potential path forward, enabling the representation of the more detailed physics and chemistry at a reduced computational cost while still retaining physical information.
Yaman Liu, Xinyi Dong, Minghuai Wang, Louisa K. Emmons, Yawen Liu, Yuan Liang, Xiao Li, and Manish Shrivastava
Atmos. Chem. Phys., 21, 8003–8021, https://doi.org/10.5194/acp-21-8003-2021, https://doi.org/10.5194/acp-21-8003-2021, 2021
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Secondary organic aerosol (SOA) is considered one of the most important uncertainties in climate modeling. We evaluate SOA performance in the Community Earth System Model version 2.1 (CESM2.1) configured with the Community Atmosphere Model version 6 with chemistry (CAM6-Chem) through a long-term simulation (1988–2019) with observations in the United States, which indicates monoterpene-formed SOA contributes most to the overestimation of SOA at the surface and underestimation in the upper air.
Xi Zhao, Xiaohong Liu, Vaughan T. J. Phillips, and Sachin Patade
Atmos. Chem. Phys., 21, 5685–5703, https://doi.org/10.5194/acp-21-5685-2021, https://doi.org/10.5194/acp-21-5685-2021, 2021
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Arctic mixed-phase clouds significantly influence the energy budget of the Arctic. We show that a climate model considering secondary ice production (SIP) can explain the observed cloud ice number concentrations, vertical distribution pattern, and probability density distribution of ice crystal number concentrations. The mixed-phase cloud occurrence and phase partitioning are also improved.
Hui Wan, Shixuan Zhang, Philip J. Rasch, Vincent E. Larson, Xubin Zeng, and Huiping Yan
Geosci. Model Dev., 14, 1921–1948, https://doi.org/10.5194/gmd-14-1921-2021, https://doi.org/10.5194/gmd-14-1921-2021, 2021
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Numerical models used in weather and climate research and prediction unavoidably contain numerical errors resulting from temporal discretization, and the impact of such errors can be substantial. Complex process interactions often make it difficult to pinpoint the exact sources of such errors. This study uses a series of sensitivity experiments to identify components in a global atmosphere model that are responsible for time step sensitivities in various cloud regimes.
Duseong S. Jo, Alma Hodzic, Louisa K. Emmons, Simone Tilmes, Rebecca H. Schwantes, Michael J. Mills, Pedro Campuzano-Jost, Weiwei Hu, Rahul A. Zaveri, Richard C. Easter, Balwinder Singh, Zheng Lu, Christiane Schulz, Johannes Schneider, John E. Shilling, Armin Wisthaler, and Jose L. Jimenez
Atmos. Chem. Phys., 21, 3395–3425, https://doi.org/10.5194/acp-21-3395-2021, https://doi.org/10.5194/acp-21-3395-2021, 2021
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Secondary organic aerosol (SOA) is a major component of submicron particulate matter, but there are a lot of uncertainties in the future prediction of SOA. We used CESM 2.1 to investigate future IEPOX SOA concentration changes. The explicit chemistry predicted substantial changes in IEPOX SOA depending on the future scenario, but the parameterization predicted weak changes due to simplified chemistry, which shows the importance of correct physicochemical dependencies in future SOA prediction.
Jianfeng Li, Zhe Feng, Yun Qian, and L. Ruby Leung
Earth Syst. Sci. Data, 13, 827–856, https://doi.org/10.5194/essd-13-827-2021, https://doi.org/10.5194/essd-13-827-2021, 2021
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Deep convection has different properties at different scales. We develop a 4 km h−1 observational data product of mesoscale convective systems and isolated deep convection in the United States from 2004–2017. We find that both types of convective systems contribute significantly to precipitation east of the Rocky Mountains but with distinct spatiotemporal characteristics. The data product will be useful for observational analyses and model evaluations of convection events at different scales.
Xi Zhao, Xiaohong Liu, Susannah M. Burrows, and Yang Shi
Atmos. Chem. Phys., 21, 2305–2327, https://doi.org/10.5194/acp-21-2305-2021, https://doi.org/10.5194/acp-21-2305-2021, 2021
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Organic sea spray particles influence aerosol and cloud processes over the ocean. This study introduces the emission, cloud droplet activation, and ice nucleation (IN) of marine organic aerosol (MOA) into the Community Earth System Model. Our results indicate that MOA IN particles dominate primary ice nucleation below 400 hPa over the Southern Ocean and Arctic boundary layer. MOA enhances cloud forcing over the Southern Ocean in the austral winter and summer.
Ryan Patnaude, Minghui Diao, Xiaohong Liu, and Suqian Chu
Atmos. Chem. Phys., 21, 1835–1859, https://doi.org/10.5194/acp-21-1835-2021, https://doi.org/10.5194/acp-21-1835-2021, 2021
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A comprehensive, in situ observation dataset of cirrus clouds was developed based on seven field campaigns, ranging from 87° N–75° S. The observations were compared with a global climate model. Several key factors for cirrus cloud formation were examined, including thermodynamics, dynamics, aerosol indirect effects and geographical locations. Model biases include lower ice mass concentrations, smaller ice crystals and weaker aerosol indirect effects.
Jingyu Wang, Jiwen Fan, Robert A. Houze Jr., Stella R. Brodzik, Kai Zhang, Guang J. Zhang, and Po-Lun Ma
Geosci. Model Dev., 14, 719–734, https://doi.org/10.5194/gmd-14-719-2021, https://doi.org/10.5194/gmd-14-719-2021, 2021
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This paper presents an evaluation of the E3SM model against NEXRAD radar observations for the warm seasons during 2014–2016. The COSP forward simulator package is implemented in the model to generate radar reflectivity, and the NEXRAD observations are coarsened to the model resolution for comparison. The model severely underestimates the reflectivity above 4 km. Sensitivity tests on the parameters from cumulus parameterization and cloud microphysics do not improve this model bias.
Johannes Quaas, Antti Arola, Brian Cairns, Matthew Christensen, Hartwig Deneke, Annica M. L. Ekman, Graham Feingold, Ann Fridlind, Edward Gryspeerdt, Otto Hasekamp, Zhanqing Li, Antti Lipponen, Po-Lun Ma, Johannes Mülmenstädt, Athanasios Nenes, Joyce E. Penner, Daniel Rosenfeld, Roland Schrödner, Kenneth Sinclair, Odran Sourdeval, Philip Stier, Matthias Tesche, Bastiaan van Diedenhoven, and Manfred Wendisch
Atmos. Chem. Phys., 20, 15079–15099, https://doi.org/10.5194/acp-20-15079-2020, https://doi.org/10.5194/acp-20-15079-2020, 2020
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Anthropogenic pollution particles – aerosols – serve as cloud condensation nuclei and thus increase cloud droplet concentration and the clouds' reflection of sunlight (a cooling effect on climate). This Twomey effect is poorly constrained by models and requires satellite data for better quantification. The review summarizes the challenges in properly doing so and outlines avenues for progress towards a better use of aerosol retrievals and better retrievals of droplet concentrations.
Mingxuan Wu, Xiaohong Liu, Hongbin Yu, Hailong Wang, Yang Shi, Kang Yang, Anton Darmenov, Chenglai Wu, Zhien Wang, Tao Luo, Yan Feng, and Ziming Ke
Atmos. Chem. Phys., 20, 13835–13855, https://doi.org/10.5194/acp-20-13835-2020, https://doi.org/10.5194/acp-20-13835-2020, 2020
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The spatiotemporal distributions of dust aerosol simulated by global climate models (GCMs) are highly uncertain. In this study, we evaluate dust extinction profiles, optical depth, and surface concentrations simulated in three GCMs and one reanalysis against multiple satellite retrievals and surface observations to gain process-level understanding. Our results highlight the importance of correctly representing dust emission, dry/wet deposition, and size distribution in GCMs.
Stefan Rahimi, Xiaohong Liu, Chun Zhao, Zheng Lu, and Zachary J. Lebo
Atmos. Chem. Phys., 20, 10911–10935, https://doi.org/10.5194/acp-20-10911-2020, https://doi.org/10.5194/acp-20-10911-2020, 2020
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Dark particles emitted to the atmosphere can absorb sunlight and heat the air. As these particles settle, they may darken the surface, especially over snow-covered regions like the Rocky Mountains. This darkening of the surface may lead to changes in snowpack, affecting the local meteorology and hydrology. We seek to evaluate whether these light-absorbing particles more prominently affect this region through their atmospheric presence or their on-snow presence.
Chenglai Wu, Zhaohui Lin, and Xiaohong Liu
Atmos. Chem. Phys., 20, 10401–10425, https://doi.org/10.5194/acp-20-10401-2020, https://doi.org/10.5194/acp-20-10401-2020, 2020
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This study provides a comprehensive evaluation of the global dust cycle in 15 models participating in the fifth phase of the Coupled Model Intercomparison Project (CMIP5). We assess the global budget and associated uncertainties. We also quantify the discrepancies in each model. The results highlight the large uncertainties in both the locations and intensities of dust emission. Our study will serve as a useful reference for model communities and help further model improvements.
Bethany Sutherland, Ben Kravitz, Philip J. Rasch, and Hailong Wang
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2020-228, https://doi.org/10.5194/gmd-2020-228, 2020
Preprint withdrawn
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Through a cascade of physical mechanisms, a change in one location can trigger a response in a different location. These responses and the mechanisms that cause them are difficult to detect. Here we propose a method, using global climate models, to detect possible relationships between changes in one region and responses throughout the globe caused by that change. A change in the Pacific ocean is used as a test case to determine the effectiveness of the method.
Lili Ren, Yang Yang, Hailong Wang, Rudong Zhang, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 20, 9067–9085, https://doi.org/10.5194/acp-20-9067-2020, https://doi.org/10.5194/acp-20-9067-2020, 2020
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Observations show that the concentrations of Arctic aerosols have declined since the early 1980s, which potentially contributed to the recent, rapid Arctic warming. We found that changes in sulfate and black carbon aerosols over the midlatitudes of the Northern Hemisphere had a larger impact on Arctic temperature than other regions and that the aerosol-induced temperature change explained approximately 20 % of the observed Arctic warming during 1980–2018.
Yi Zeng, Minghuai Wang, Chun Zhao, Siyu Chen, Zhoukun Liu, Xin Huang, and Yang Gao
Geosci. Model Dev., 13, 2125–2147, https://doi.org/10.5194/gmd-13-2125-2020, https://doi.org/10.5194/gmd-13-2125-2020, 2020
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Dust aerosol can impact many processes of the Earth system, but large uncertainties still remain in dust simulations. In this study, we investigated dust simulation sensitivity to two dust emission schemes and three dry deposition schemes using WRF-Chem. An optimal combination of dry deposition scheme and dust emission scheme has been identified to best simulate the dust storm in comparison with observation. Our results highlight the importance of dry deposition schemes for dust simulation.
Yufei Zou, Yuhang Wang, Zuowei Xie, Hailong Wang, and Philip J. Rasch
Atmos. Chem. Phys., 20, 4999–5017, https://doi.org/10.5194/acp-20-4999-2020, https://doi.org/10.5194/acp-20-4999-2020, 2020
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We analyze the relationship between winter air stagnation and pollution extremes over eastern China and preceding Arctic sea ice loss based on climate modeling and dynamic diagnoses. We find significant increases in both the probability and intensity of air stagnation extremes in the modeling result driven by regional sea ice and sea surface temperature changes over the Pacific sector of the Arctic. We reveal the considerable impact of the Arctic climate change on mid-latitude weather extremes.
Tongwen Wu, Fang Zhang, Jie Zhang, Weihua Jie, Yanwu Zhang, Fanghua Wu, Laurent Li, Jinghui Yan, Xiaohong Liu, Xiao Lu, Haiyue Tan, Lin Zhang, Jun Wang, and Aixue Hu
Geosci. Model Dev., 13, 977–1005, https://doi.org/10.5194/gmd-13-977-2020, https://doi.org/10.5194/gmd-13-977-2020, 2020
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This paper describes the first version of the Beijing Climate Center (BCC) fully coupled Earth System Model with interactive atmospheric chemistry and aerosols (BCC-ESM1). It is one of the models at the BCC for the Coupled Model Intercomparison Project Phase 6 (CMIP6). The CMIP6 Aerosol Chemistry Model Intercomparison Project (AerChemMIP) experiment using BCC-ESM1 has been finished. The evaluations show an overall good agreement between BCC-ESM1 simulations and observations in the 20th century.
Yang Yang, Sijia Lou, Hailong Wang, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 20, 2579–2590, https://doi.org/10.5194/acp-20-2579-2020, https://doi.org/10.5194/acp-20-2579-2020, 2020
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Aerosol concentration decreased in Europe during 1980–2018, of which 7 % was induced by the changes in non-European emissions. Aerosols transported from other source regions are increasingly important to air quality in Europe. Contributions to the sulfate radiative forcing over Europe from both European and non-European emissions should decrease at a comparable rate in the next three decades. Future changes in non-European emissions are important in causing regional climate change in Europe.
Hailong Wang, Jeremy G. Fyke, Jan T. M. Lenaerts, Jesse M. Nusbaumer, Hansi Singh, David Noone, Philip J. Rasch, and Rudong Zhang
The Cryosphere, 14, 429–444, https://doi.org/10.5194/tc-14-429-2020, https://doi.org/10.5194/tc-14-429-2020, 2020
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Using a climate model with unique water source tagging, we found that sea-ice anomalies in the Southern Ocean and accompanying SST changes have a significant influence on Antarctic precipitation and its source attribution through their direct impact on moisture sources and indirect impact on moisture transport. This study also highlights the importance of atmospheric dynamics in affecting the thermodynamic impact of sea-ice anomalies on regional Antarctic precipitation.
Yufei Zou, Yuhang Wang, Yun Qian, Hanqin Tian, Jia Yang, and Ernesto Alvarado
Atmos. Chem. Phys., 20, 995–1020, https://doi.org/10.5194/acp-20-995-2020, https://doi.org/10.5194/acp-20-995-2020, 2020
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Fire is a natural phenomenon that has a long history of interactions with the environment and human activity. The complex interactions were less represented in previous fire and climate models. Here we use a new global fire model with improved modeling capability to study how fire responds and contributes to climate change. The modeling results show increased global fire activity in the future driven by climate change, which in turn modulates local and remote climate and ecosystems.
Edward Gryspeerdt, Johannes Mülmenstädt, Andrew Gettelman, Florent F. Malavelle, Hugh Morrison, David Neubauer, Daniel G. Partridge, Philip Stier, Toshihiko Takemura, Hailong Wang, Minghuai Wang, and Kai Zhang
Atmos. Chem. Phys., 20, 613–623, https://doi.org/10.5194/acp-20-613-2020, https://doi.org/10.5194/acp-20-613-2020, 2020
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Aerosol radiative forcing is a key uncertainty in our understanding of the human forcing of the climate, with much of this uncertainty coming from aerosol impacts on clouds. Observation-based estimates of the radiative forcing are typically smaller than those from global models, but it is not clear if they are more reliable. This work shows how the forcing components in global climate models can be identified, highlighting similarities between the two methods and areas for future investigation.
Hongbin Yu, Yang Yang, Hailong Wang, Qian Tan, Mian Chin, Robert C. Levy, Lorraine A. Remer, Steven J. Smith, Tianle Yuan, and Yingxi Shi
Atmos. Chem. Phys., 20, 139–161, https://doi.org/10.5194/acp-20-139-2020, https://doi.org/10.5194/acp-20-139-2020, 2020
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Emissions and long-range transport of mineral dust and
combustion-related aerosol from burning fossil fuels and biomass vary from year to year, driven by the evolution of the economy and changes in meteorological conditions and environmental regulations. This study offers both satellite and model perspectives on interannual variability and possible trends in combustion aerosol and dust in major continental outflow regions over the past 15 years (2003–2017).
Johannes Mülmenstädt, Edward Gryspeerdt, Marc Salzmann, Po-Lun Ma, Sudhakar Dipu, and Johannes Quaas
Atmos. Chem. Phys., 19, 15415–15429, https://doi.org/10.5194/acp-19-15415-2019, https://doi.org/10.5194/acp-19-15415-2019, 2019
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The effect of aerosol–cloud interactions (ACIs) on Earth's energy budget continues to be highly uncertain. We decompose the effective radiative forcing by ACIs (ERFaci) into the instantaneous forcing due to anthropogenic increases in the number of cloud droplets and fast responses of cloud properties to the droplet number perturbation in the ECHAM–HAMMOZ aerosol–climate model. This decomposition maps onto the IPCC's Fifth Assessment Report analysis of ERFaci more directly than previous work.
Zhiyuan Hu, Jianping Huang, Chun Zhao, Yuanyuan Ma, Qinjian Jin, Yun Qian, L. Ruby Leung, Jianrong Bi, and Jianmin Ma
Atmos. Chem. Phys., 19, 12709–12730, https://doi.org/10.5194/acp-19-12709-2019, https://doi.org/10.5194/acp-19-12709-2019, 2019
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This study investigates aerosol chemical compositions and relative contributions to total aerosols in the western US. The results show that trans-Pacific aerosols have a maximum concentration in the boreal spring, with the greatest contribution from dust. Over western North America, the trans-Pacific aerosols dominate the column-integrated aerosol mass and number concentration. However, near the surface, aerosols mainly originated from local emissions.
Fang Li, Maria Val Martin, Meinrat O. Andreae, Almut Arneth, Stijn Hantson, Johannes W. Kaiser, Gitta Lasslop, Chao Yue, Dominique Bachelet, Matthew Forrest, Erik Kluzek, Xiaohong Liu, Stephane Mangeon, Joe R. Melton, Daniel S. Ward, Anton Darmenov, Thomas Hickler, Charles Ichoku, Brian I. Magi, Stephen Sitch, Guido R. van der Werf, Christine Wiedinmyer, and Sam S. Rabin
Atmos. Chem. Phys., 19, 12545–12567, https://doi.org/10.5194/acp-19-12545-2019, https://doi.org/10.5194/acp-19-12545-2019, 2019
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Fire emissions are critical for atmospheric composition, climate, carbon cycle, and air quality. We provide the first global multi-model fire emission reconstructions for 1700–2012, including carbon and 33 species of trace gases and aerosols, based on the nine state-of-the-art global fire models that participated in FireMIP. We also provide information on the recent status and limitations of the model-based reconstructions and identify the main uncertainty sources in their long-term changes.
Stefan Rahimi, Xiaohong Liu, Chenglai Wu, William K. Lau, Hunter Brown, Mingxuan Wu, and Yun Qian
Atmos. Chem. Phys., 19, 12025–12049, https://doi.org/10.5194/acp-19-12025-2019, https://doi.org/10.5194/acp-19-12025-2019, 2019
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Light-absorbing particles impact the Earth system in a variety of ways. They can warm the atmosphere by their very presence, or they can warm the atmosphere after they deposit on snow, warm it, and warm the overlying atmosphere. This paper focuses on these two processes as they pertain to black carbon and dust's impacts on the South Asian monsoon. It will be shown that these two aerosols have a significant effect on the monsoon.
Douglas S. Hamilton, Rachel A. Scanza, Yan Feng, Joseph Guinness, Jasper F. Kok, Longlei Li, Xiaohong Liu, Sagar D. Rathod, Jessica S. Wan, Mingxuan Wu, and Natalie M. Mahowald
Geosci. Model Dev., 12, 3835–3862, https://doi.org/10.5194/gmd-12-3835-2019, https://doi.org/10.5194/gmd-12-3835-2019, 2019
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MIMI v1.0 was designed for use within Earth system models to simulate the 3-D emission, atmospheric processing, and deposition of iron and its soluble fraction. Understanding the iron cycle is important due to its role as an essential micronutrient for ocean phytoplankton; its supply limits primary productivity in many of the world's oceans. Human activity has perturbed the iron cycle, and MIMI is capable of diagnosing many of these impacts; hence, it is important for future climate studies.
George S. Fanourgakis, Maria Kanakidou, Athanasios Nenes, Susanne E. Bauer, Tommi Bergman, Ken S. Carslaw, Alf Grini, Douglas S. Hamilton, Jill S. Johnson, Vlassis A. Karydis, Alf Kirkevåg, John K. Kodros, Ulrike Lohmann, Gan Luo, Risto Makkonen, Hitoshi Matsui, David Neubauer, Jeffrey R. Pierce, Julia Schmale, Philip Stier, Kostas Tsigaridis, Twan van Noije, Hailong Wang, Duncan Watson-Parris, Daniel M. Westervelt, Yang Yang, Masaru Yoshioka, Nikos Daskalakis, Stefano Decesari, Martin Gysel-Beer, Nikos Kalivitis, Xiaohong Liu, Natalie M. Mahowald, Stelios Myriokefalitakis, Roland Schrödner, Maria Sfakianaki, Alexandra P. Tsimpidi, Mingxuan Wu, and Fangqun Yu
Atmos. Chem. Phys., 19, 8591–8617, https://doi.org/10.5194/acp-19-8591-2019, https://doi.org/10.5194/acp-19-8591-2019, 2019
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Effects of aerosols on clouds are important for climate studies but are among the largest uncertainties in climate projections. This study evaluates the skill of global models to simulate aerosol, cloud condensation nuclei (CCN) and cloud droplet number concentrations (CDNCs). Model results show reduced spread in CDNC compared to CCN due to the negative correlation between the sensitivities of CDNC to aerosol number concentration (air pollution) and updraft velocity (atmospheric dynamics).
Qi Tang, Stephen A. Klein, Shaocheng Xie, Wuyin Lin, Jean-Christophe Golaz, Erika L. Roesler, Mark A. Taylor, Philip J. Rasch, David C. Bader, Larry K. Berg, Peter Caldwell, Scott E. Giangrande, Richard B. Neale, Yun Qian, Laura D. Riihimaki, Charles S. Zender, Yuying Zhang, and Xue Zheng
Geosci. Model Dev., 12, 2679–2706, https://doi.org/10.5194/gmd-12-2679-2019, https://doi.org/10.5194/gmd-12-2679-2019, 2019
Chandan Sarangi, Yun Qian, Karl Rittger, Kathryn J. Bormann, Ying Liu, Hailong Wang, Hui Wan, Guangxing Lin, and Thomas H. Painter
Atmos. Chem. Phys., 19, 7105–7128, https://doi.org/10.5194/acp-19-7105-2019, https://doi.org/10.5194/acp-19-7105-2019, 2019
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Radiative forcing induced by deposition of light-absorbing particles (LAPs) on snow is an important surface forcing. Here, we have used high-resolution WRF-Chem (coupled with online snow–LAP–radiation model) simulations for 2013–2014 to estimate the spatial variation in LAP-induced snow albedo darkening effect in high-mountain Asia. Significant improvement in simulated LAP–snow properties with use of a higher spatial resolution for the same model configuration is illustrated over this region.
Tongwen Wu, Yixiong Lu, Yongjie Fang, Xiaoge Xin, Laurent Li, Weiping Li, Weihua Jie, Jie Zhang, Yiming Liu, Li Zhang, Fang Zhang, Yanwu Zhang, Fanghua Wu, Jianglong Li, Min Chu, Zaizhi Wang, Xueli Shi, Xiangwen Liu, Min Wei, Anning Huang, Yaocun Zhang, and Xiaohong Liu
Geosci. Model Dev., 12, 1573–1600, https://doi.org/10.5194/gmd-12-1573-2019, https://doi.org/10.5194/gmd-12-1573-2019, 2019
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This work presents advancements of the BCC model transition from CMIP5 to CMIP6, especially in the model resolution and its physics. Compared with BCC CMIP5 models, the BCC CMIP6 model shows significant improvements in historical simulations in many aspects including tropospheric air temperature and circulation at global and regional scales in East Asia, climate variability at different timescales (QBO, MJO, and diurnal cycle of precipitation), and the long-term trend of global air temperature.
Yang Yang, Steven J. Smith, Hailong Wang, Catrin M. Mills, and Philip J. Rasch
Atmos. Chem. Phys., 19, 2405–2420, https://doi.org/10.5194/acp-19-2405-2019, https://doi.org/10.5194/acp-19-2405-2019, 2019
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Black carbon (BC) particles exert a potentially large warming influence on the
Earth system. We evaluate regional climate responses, non-linearity, and short-term transient responses to BC emission perturbations. We found that climate responses do not scale linearity with emissions and BC impacts temperature much faster than greenhouse gas forcing. Removing present-day BC emissions results in discernible surface temperature changes for only limited regions of the globe.
Zhibo Zhang, Hua Song, Po-Lun Ma, Vincent E. Larson, Minghuai Wang, Xiquan Dong, and Jianwu Wang
Atmos. Chem. Phys., 19, 1077–1096, https://doi.org/10.5194/acp-19-1077-2019, https://doi.org/10.5194/acp-19-1077-2019, 2019
Ge Zhang, Yang Gao, Wenju Cai, L. Ruby Leung, Shuxiao Wang, Bin Zhao, Minghuai Wang, Huayao Shan, Xiaohong Yao, and Huiwang Gao
Atmos. Chem. Phys., 19, 565–576, https://doi.org/10.5194/acp-19-565-2019, https://doi.org/10.5194/acp-19-565-2019, 2019
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Based on observed data, this study reveals a distinct seesaw feature of abnormally high and low PM2.5 concentrations in December 2015 and January 2016 over North China. The mechanism of the seesaw pattern was found to be linked to a super El Niño and the Arctic Oscillation (AO). During the mature phase of El Niño in December 2015, the weakened East Asian winter monsoon favors strong haze formation; however, the circulation pattern was reversed in the next month due to the phase change of the AO.
Hunter Brown, Xiaohong Liu, Yan Feng, Yiquan Jiang, Mingxuan Wu, Zheng Lu, Chenglai Wu, Shane Murphy, and Rudra Pokhrel
Atmos. Chem. Phys., 18, 17745–17768, https://doi.org/10.5194/acp-18-17745-2018, https://doi.org/10.5194/acp-18-17745-2018, 2018
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In climate models, organic carbon (OC) in wildfire smoke has been treated as an atmospheric cooling component by reflecting sunlight back to space. This study incorporates the observationally identified absorbing brown carbon component of OC into the Community Earth System Model, improving the agreement between the model and observations and effectively increasing absorption of solar radiation. This change contributes to altered atmospheric dynamics and changes in cloud cover in the model.
Anna Possner, Hailong Wang, Robert Wood, Ken Caldeira, and Thomas P. Ackerman
Atmos. Chem. Phys., 18, 17475–17488, https://doi.org/10.5194/acp-18-17475-2018, https://doi.org/10.5194/acp-18-17475-2018, 2018
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We quantify aerosol–cloud radiative interactions in a regime of deep open-cell stratocumuli (boundary layer depth 1.5 km), a regime which remains largely unexplored within this context and yet is more dominant than cases of shallow stratocumuli previously studied. We simulate substantial increases in albedo in a regime where ship tracks are not found and argue that such changes may escape detection and attribution through remote sensing due to the large natural variability in the system.
Jiahui Zhang, Dao-Yi Gong, Rui Mao, Jing Yang, Ziyin Zhang, and Yun Qian
Atmos. Chem. Phys., 18, 16775–16791, https://doi.org/10.5194/acp-18-16775-2018, https://doi.org/10.5194/acp-18-16775-2018, 2018
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The Chinese Spring Festival (also known as the Chinese New Year or Lunar New Year) is the most important festival in China. This paper reports that during the Chinese Spring Festival, the precipitation over southern China has been significantly reduced. The precipitation reduction is due to anomalous northerly winds. We suppose that anomalous atmospheric circulation is likely related to the human activity during holidays. It is an interesting phenomenon.
Benjamin S. Grandey, Daniel Rothenberg, Alexander Avramov, Qinjian Jin, Hsiang-He Lee, Xiaohong Liu, Zheng Lu, Samuel Albani, and Chien Wang
Atmos. Chem. Phys., 18, 15783–15810, https://doi.org/10.5194/acp-18-15783-2018, https://doi.org/10.5194/acp-18-15783-2018, 2018
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Anthropogenic emissions of aerosol particles likely cool the climate system. We investigate the uncertainty in the strength of the cooling effect by exploring the representation of aerosols in a global climate model. We conclude that the specific representation of aerosols in global climate models has important implications for climate modelling. Important factors include the representation of aerosol mixing state, size distribution, and optical properties.
Alf Kirkevåg, Alf Grini, Dirk Olivié, Øyvind Seland, Kari Alterskjær, Matthias Hummel, Inger H. H. Karset, Anna Lewinschal, Xiaohong Liu, Risto Makkonen, Ingo Bethke, Jan Griesfeller, Michael Schulz, and Trond Iversen
Geosci. Model Dev., 11, 3945–3982, https://doi.org/10.5194/gmd-11-3945-2018, https://doi.org/10.5194/gmd-11-3945-2018, 2018
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A new aerosol treatment is described and tested in a global climate model. With updated emissions, aerosol chemistry, and microphysics compared to its predecessor, black carbon (BC) mass concentrations aloft better fit observations, surface concentrations of BC and sea salt are less biased, and sulfate and mineral dust slightly more, while the results for organics are inconclusive. Man-made aerosols now yield a stronger cooling effect on climate that is strong compared to results from IPCC.
Ben Kravitz, Philip J. Rasch, Hailong Wang, Alan Robock, Corey Gabriel, Olivier Boucher, Jason N. S. Cole, Jim Haywood, Duoying Ji, Andy Jones, Andrew Lenton, John C. Moore, Helene Muri, Ulrike Niemeier, Steven Phipps, Hauke Schmidt, Shingo Watanabe, Shuting Yang, and Jin-Ho Yoon
Atmos. Chem. Phys., 18, 13097–13113, https://doi.org/10.5194/acp-18-13097-2018, https://doi.org/10.5194/acp-18-13097-2018, 2018
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Marine cloud brightening has been proposed as a means of geoengineering/climate intervention, or deliberately altering the climate system to offset anthropogenic climate change. In idealized simulations that highlight contrasts between land and ocean, we find that the globe warms, including the ocean due to transport of heat from land. This study reinforces that no net energy input into the Earth system does not mean that temperature will necessarily remain unchanged.
Cenlin He, Mark G. Flanner, Fei Chen, Michael Barlage, Kuo-Nan Liou, Shichang Kang, Jing Ming, and Yun Qian
Atmos. Chem. Phys., 18, 11507–11527, https://doi.org/10.5194/acp-18-11507-2018, https://doi.org/10.5194/acp-18-11507-2018, 2018
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Snow albedo plays a key role in the Earth and climate system. It can be affected by impurities and snow properties. This study implements new parameterizations into a widely used snow model to account for effects of snow shape and black carbon–snow mixing state on snow albedo reduction in the Tibetan Plateau. This study points toward an imperative need for extensive measurements and improved model characterization of snow grain shape and aerosol–snow mixing state in Tibet and elsewhere.
Hua Song, Zhibo Zhang, Po-Lun Ma, Steven Ghan, and Minghuai Wang
Geosci. Model Dev., 11, 3147–3158, https://doi.org/10.5194/gmd-11-3147-2018, https://doi.org/10.5194/gmd-11-3147-2018, 2018
Kai Zhang, Philip J. Rasch, Mark A. Taylor, Hui Wan, Ruby Leung, Po-Lun Ma, Jean-Christophe Golaz, Jon Wolfe, Wuyin Lin, Balwinder Singh, Susannah Burrows, Jin-Ho Yoon, Hailong Wang, Yun Qian, Qi Tang, Peter Caldwell, and Shaocheng Xie
Geosci. Model Dev., 11, 1971–1988, https://doi.org/10.5194/gmd-11-1971-2018, https://doi.org/10.5194/gmd-11-1971-2018, 2018
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The conservation of total water is an important numerical feature for global Earth system models. Even small conservation problems in the water budget can lead to systematic errors in century-long simulations for sea level rise projection. This study quantifies and reduces various sources of water conservation error in the atmosphere component of the Energy Exascale Earth System Model.
Hewen Niu, Shichang Kang, Hailong Wang, Rudong Zhang, Xixi Lu, Yun Qian, Rukumesh Paudyal, Shijin Wang, Xiaofei Shi, and Xingguo Yan
Atmos. Chem. Phys., 18, 6441–6460, https://doi.org/10.5194/acp-18-6441-2018, https://doi.org/10.5194/acp-18-6441-2018, 2018
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Deposition of light-absorbing carbonaceous aerosol on the surface of glaciers can greatly alter the energy fluxes of glaciers. Two years of continuous observations of carbonaceous aerosols in a glacierized region are analyzed. We mainly studied the light absorption properties of carbonaceous aerosol and have employed a global aerosol–climate model to estimate source attributions of atmospheric black carbon.
Longtao Wu, Yu Gu, Jonathan H. Jiang, Hui Su, Nanpeng Yu, Chun Zhao, Yun Qian, Bin Zhao, Kuo-Nan Liou, and Yong-Sang Choi
Atmos. Chem. Phys., 18, 5529–5547, https://doi.org/10.5194/acp-18-5529-2018, https://doi.org/10.5194/acp-18-5529-2018, 2018
Heming Bai, Cheng Gong, Minghuai Wang, Zhibo Zhang, and Tristan L'Ecuyer
Atmos. Chem. Phys., 18, 1763–1783, https://doi.org/10.5194/acp-18-1763-2018, https://doi.org/10.5194/acp-18-1763-2018, 2018
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Precipitation susceptibility to aerosol perturbation plays a key role in understanding aerosol–cloud interactions and for constraining aerosol indirect effects. Here, multisensor aerosol and cloud products from A-Train satellites are analyzed to estimate precipitation susceptibility. Compared to precipitation intensity susceptibility, precipitation frequency susceptibility demonstrates relatively robust features across different retrieval products.
Tianyi Fan, Xiaohong Liu, Po-Lun Ma, Qiang Zhang, Zhanqing Li, Yiquan Jiang, Fang Zhang, Chuanfeng Zhao, Xin Yang, Fang Wu, and Yuying Wang
Atmos. Chem. Phys., 18, 1395–1417, https://doi.org/10.5194/acp-18-1395-2018, https://doi.org/10.5194/acp-18-1395-2018, 2018
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We found that 22–28 % of the low AOD bias in eastern China simulated by the Community Atmosphere Model version 5 can be improved by using a new emission inventory. The concentrations of primary aerosols are closely related to the emission, while the seasonal variations of secondary aerosols depend more on atmospheric processes. This study highlights the importance of improving both the emission and atmospheric processes in modeling the atmospheric aerosols and their radiative effects.
Bin Zhao, Kuo-Nan Liou, Yu Gu, Jonathan H. Jiang, Qinbin Li, Rong Fu, Lei Huang, Xiaohong Liu, Xiangjun Shi, Hui Su, and Cenlin He
Atmos. Chem. Phys., 18, 1065–1078, https://doi.org/10.5194/acp-18-1065-2018, https://doi.org/10.5194/acp-18-1065-2018, 2018
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The interactions between aerosols and ice clouds represent one of the largest uncertainties among anthropogenic forcings on climate change. We find that the responses of ice crystal effective radius, a key parameter determining ice clouds' net radiative effect, to aerosol loadings are modulated by water vapor amount and vary from a significant negative correlation in moist conditions (consistent with the “Twomey effect” for liquid clouds) to a strong positive correlation in dry conditions.
Chenglai Wu, Xiaohong Liu, Zhaohui Lin, Stefan R. Rahimi-Esfarjani, and Zheng Lu
Atmos. Chem. Phys., 18, 511–533, https://doi.org/10.5194/acp-18-511-2018, https://doi.org/10.5194/acp-18-511-2018, 2018
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This study utilizes the newly developed variable-resolution Community Earth System Model (VR-CESM) with a refined high resolution (0.125º) to quantify the impacts of absorbing aerosol (BC and dust) deposition on snowpack and hydrologic cycles in the Rocky Mountains. BC and dust in snow significantly reduce the snowpack around the mountains. BC and dust in snow also accelerate the hydrologic cycles in the mountainous regions, with runoff increased in spring but reduced in summer.
Yawen Liu, Kai Zhang, Yun Qian, Yuhang Wang, Yufei Zou, Yongjia Song, Hui Wan, Xiaohong Liu, and Xiu-Qun Yang
Atmos. Chem. Phys., 18, 31–47, https://doi.org/10.5194/acp-18-31-2018, https://doi.org/10.5194/acp-18-31-2018, 2018
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Fire aerosols have large impact on weather and climate through their effect on clouds and radiation, but it is difficult to quantify. Here we investigated the short-term effective radiative forcing of fire aerosols using the nudged hindcast ensemble simulations from global aerosol-climate model. Results show large effects of fire aerosols on both liquid and ice cloud and large ensemble spread of regional mean shortwave cloud radiative forcing over southern Mexico and the central US.
Jeremy Fyke, Jan T. M. Lenaerts, and Hailong Wang
The Cryosphere, 11, 2595–2609, https://doi.org/10.5194/tc-11-2595-2017, https://doi.org/10.5194/tc-11-2595-2017, 2017
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In this CESM modeling study, we uncover regional relationships in snowfall across Antarctica that are corroborated by regional modeling and ice core records. These relationships are driven by variability in large-scale atmospheric moisture transport and dampen overall Antarctic snowfall variability, with implications for Antarctic-sourced sea level variability and detection of an emergent anthropogenic signal in Antarctic mass trends.
Maria Sand, Bjørn H. Samset, Yves Balkanski, Susanne Bauer, Nicolas Bellouin, Terje K. Berntsen, Huisheng Bian, Mian Chin, Thomas Diehl, Richard Easter, Steven J. Ghan, Trond Iversen, Alf Kirkevåg, Jean-François Lamarque, Guangxing Lin, Xiaohong Liu, Gan Luo, Gunnar Myhre, Twan van Noije, Joyce E. Penner, Michael Schulz, Øyvind Seland, Ragnhild B. Skeie, Philip Stier, Toshihiko Takemura, Kostas Tsigaridis, Fangqun Yu, Kai Zhang, and Hua Zhang
Atmos. Chem. Phys., 17, 12197–12218, https://doi.org/10.5194/acp-17-12197-2017, https://doi.org/10.5194/acp-17-12197-2017, 2017
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The role of aerosols in the changing polar climate is not well understood and the aerosols are poorly constrained in the models. In this study we have compared output from 16 different aerosol models with available observations at both poles. We show that the model median is representative of the observations, but the model spread is large. The Arctic direct aerosol radiative effect over the industrial area is positive during spring due to black carbon and negative during summer due to sulfate.
Louis Marelle, Jean-Christophe Raut, Kathy S. Law, Larry K. Berg, Jerome D. Fast, Richard C. Easter, Manish Shrivastava, and Jennie L. Thomas
Geosci. Model Dev., 10, 3661–3677, https://doi.org/10.5194/gmd-10-3661-2017, https://doi.org/10.5194/gmd-10-3661-2017, 2017
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We develop the WRF-Chem 3.5.1 model to improve simulations of aerosols and ozone in the Arctic. Both species are important air pollutants and climate forcers, but models often struggle to reproduce observations in the Arctic. Our developments concern pollutant emissions, mixing, chemistry, and removal, including processes related to snow and sea ice. The effect of these changes are quantitatively validated against observations, showing significant improvements compared to the original model.
Jean-Christophe Raut, Louis Marelle, Jerome D. Fast, Jennie L. Thomas, Bernadett Weinzierl, Katharine S. Law, Larry K. Berg, Anke Roiger, Richard C. Easter, Katharina Heimerl, Tatsuo Onishi, Julien Delanoë, and Hans Schlager
Atmos. Chem. Phys., 17, 10969–10995, https://doi.org/10.5194/acp-17-10969-2017, https://doi.org/10.5194/acp-17-10969-2017, 2017
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We study the cross-polar transport of plumes from Siberian fires to the Arctic in summer, both in terms of transport pathways and efficiency of deposition processes. Those plumes containing soot may originate from anthropogenic and biomass burning sources in mid-latitude regions and may impact the Arctic climate by depositing on snow and ice surfaces. We evaluate the role of the respective source contributions, investigate the transport of plumes and treat pathway-dependent removal of particles.
Yang Yang, Hailong Wang, Steven J. Smith, Richard Easter, Po-Lun Ma, Yun Qian, Hongbin Yu, Can Li, and Philip J. Rasch
Atmos. Chem. Phys., 17, 8903–8922, https://doi.org/10.5194/acp-17-8903-2017, https://doi.org/10.5194/acp-17-8903-2017, 2017
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Sulfate has significant impacts on air quality and climate. Local sulfate pollution could result from remote influences, making domestic mitigation efforts inefficient. Using CESM with a sulfur source-tagging technique, we found that, over regions with relatively low emissions, sulfate concentrations are primarily attributed to non-local sources and sulfate indirect radiative forcing over the Southern Hemisphere is more sensitive to emission perturbation than the polluted Northern Hemisphere.
Shi Zhong, Yun Qian, Chun Zhao, Ruby Leung, Hailong Wang, Ben Yang, Jiwen Fan, Huiping Yan, Xiu-Qun Yang, and Dongqing Liu
Atmos. Chem. Phys., 17, 5439–5457, https://doi.org/10.5194/acp-17-5439-2017, https://doi.org/10.5194/acp-17-5439-2017, 2017
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An online climate–chemistry coupled model (WRF-Chem) is integrated for 5 years at cloud-permitting scale to quantify the impacts of urbanization-induced changes in land cover and pollutants emission on regional climate in the Yangtze River Delta region in eastern China. Urbanization over this region increases the frequency of extreme precipitation and heat wave in summer. The results could help China government in making policies in mitigating the environmental impact of urbanization.
Chenglai Wu, Xiaohong Liu, Minghui Diao, Kai Zhang, Andrew Gettelman, Zheng Lu, Joyce E. Penner, and Zhaohui Lin
Atmos. Chem. Phys., 17, 4731–4749, https://doi.org/10.5194/acp-17-4731-2017, https://doi.org/10.5194/acp-17-4731-2017, 2017
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This study utilizes a novel approach to directly compare the CAM5-simulated cloud macro- and microphysics with the collocated HIPPO observations for the period of 2009 to 2011. The model cannot capture the large spatial variabilities of observed RH, which is responsible for much of the model missing low-level warm clouds. A large portion of the RH bias results from the discrepancy in water vapor. The model underestimates the observed number concentration and ice water content.
Yang Yang, Hailong Wang, Steven J. Smith, Po-Lun Ma, and Philip J. Rasch
Atmos. Chem. Phys., 17, 4319–4336, https://doi.org/10.5194/acp-17-4319-2017, https://doi.org/10.5194/acp-17-4319-2017, 2017
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The source attributions of black carbon (BC) in China are quantified using the Community Earth System Model by source tagging. BC impacts neighboring regions greatly. Transport is important in increasing BC during regional polluted days. Emissions outside China contribute 35 % of BC direct radiative forcing in China. Efficiency analysis shows that reduction in BC emissions over eastern China could have a greater benefit for regional air quality in China, especially in the winter haze season.
Ben Kravitz, Douglas G. MacMartin, Philip J. Rasch, and Hailong Wang
Atmos. Chem. Phys., 17, 2525–2541, https://doi.org/10.5194/acp-17-2525-2017, https://doi.org/10.5194/acp-17-2525-2017, 2017
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We introduce system identification techniques to climate science wherein multiple dynamic input–output relationships can be simultaneously characterized in a single simulation. This method, involving multiple small perturbations (in space and time) of an input field while monitoring output fields to quantify responses, allows for identification of different timescales of climate response to forcing without substantially pushing the climate far away from a steady state.
Hui Wan, Kai Zhang, Philip J. Rasch, Balwinder Singh, Xingyuan Chen, and Jim Edwards
Geosci. Model Dev., 10, 537–552, https://doi.org/10.5194/gmd-10-537-2017, https://doi.org/10.5194/gmd-10-537-2017, 2017
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Solution reproductibility testing is an important task for assuring the software quality of a climate model. A new method is developed using the concept of numerical convergence with respect to temporal resolution. The method is objective, easy to implement, and computationally efficient. This paper describes the new test and demonstrates its utility in the Community Atmosphere Model version 5 (CAM5).
Yiquan Jiang, Zheng Lu, Xiaohong Liu, Yun Qian, Kai Zhang, Yuhang Wang, and Xiu-Qun Yang
Atmos. Chem. Phys., 16, 14805–14824, https://doi.org/10.5194/acp-16-14805-2016, https://doi.org/10.5194/acp-16-14805-2016, 2016
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Aerosols from open fires could significantly perturb the global radiation balance and induce climate change. In this study, the CAM5 global climate model is used to investigate the spatial and seasonal characteristics of radiative effects due to fire aerosol–radiation interactions, fire aerosol-cloud interactions and fire aerosol-surface albedo interactions, including radiative effects from all fire aerosols, fire black carbon and fire particulate organic matter.
Tianjun Zhou, Andrew G. Turner, James L. Kinter, Bin Wang, Yun Qian, Xiaolong Chen, Bo Wu, Bin Wang, Bo Liu, Liwei Zou, and Bian He
Geosci. Model Dev., 9, 3589–3604, https://doi.org/10.5194/gmd-9-3589-2016, https://doi.org/10.5194/gmd-9-3589-2016, 2016
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This paper tells why to launch the Global Monsoons Model Inter-comparison Project (GMMIP) and how to achieve its scientific goals on monsoon variability. It addresses the scientific questions to be answered, describes three tiered experiments comprehensively and proposes a basic analysis framework to guide future research. It will help the monsoon research communities to understand the objectives of the GMMIP and the modelling groups involved in the GMMIP conduct the experiments successfully.
Cheng Zhou, Joyce E. Penner, Guangxing Lin, Xiaohong Liu, and Minghuai Wang
Atmos. Chem. Phys., 16, 12411–12424, https://doi.org/10.5194/acp-16-12411-2016, https://doi.org/10.5194/acp-16-12411-2016, 2016
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We examined the different ice nucleation parameterization factors that affect the simulated ice number concentrations in cirrus clouds in the upper troposphere using the CAM5 model. We examined the effect from three different updraft velocities (from low to high), two different water vapour accommodation coefficients (α = 0.1 or 1), the effect of including vapour deposition onto pre-existing ice particles during ice nucleation, and the effect of including SOA as heterogeneous ice nuclei.
Xin Huang, Aijun Ding, Lixia Liu, Qiang Liu, Ke Ding, Xiaorui Niu, Wei Nie, Zheng Xu, Xuguang Chi, Minghuai Wang, Jianning Sun, Weidong Guo, and Congbin Fu
Atmos. Chem. Phys., 16, 10063–10082, https://doi.org/10.5194/acp-16-10063-2016, https://doi.org/10.5194/acp-16-10063-2016, 2016
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We conducted a comprehensive modelling work to understand the impact of biomass burning on synoptic weather during agricultural burning season in East China. We demonstrated that the numerical model with fire emission, chemical processes, and aerosol–meteorology online coupled could reproduce the change of air temperature and precipitation induced by air pollution during this event. This study highlights the importance of including human activities in numerical-model-based weather forecast.
Chun Zhao, Maoyi Huang, Jerome D. Fast, Larry K. Berg, Yun Qian, Alex Guenther, Dasa Gu, Manish Shrivastava, Ying Liu, Stacy Walters, Gabriele Pfister, Jiming Jin, John E. Shilling, and Carsten Warneke
Geosci. Model Dev., 9, 1959–1976, https://doi.org/10.5194/gmd-9-1959-2016, https://doi.org/10.5194/gmd-9-1959-2016, 2016
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In this study, the latest version of MEGAN is coupled within CLM4 in WRF-Chem. In this implementation, MEGAN shares a consistent vegetation map with CLM4. This improved modeling framework is used to investigate the impact of two land surface schemes on BVOCs and examine the sensitivity of BVOCs to vegetation distributions in California. This study indicates that more effort is needed to obtain the most appropriate and accurate land cover data sets for climate and air quality models.
Ben Kravitz, Douglas G. MacMartin, Hailong Wang, and Philip J. Rasch
Earth Syst. Dynam., 7, 469–497, https://doi.org/10.5194/esd-7-469-2016, https://doi.org/10.5194/esd-7-469-2016, 2016
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Most simulations of solar geoengineering prescribe a particular strategy and evaluate its modeled effects. Here we first choose example climate objectives and then design a strategy to meet those objectives in climate models. We show that certain objectives can be met simultaneously even in the presence of uncertainty, and the strategy for meeting those objectives can be ported to other models. This is part of a broader illustration of how uncertainties in solar geoengineering can be managed.
Zhiyuan Hu, Chun Zhao, Jianping Huang, L. Ruby Leung, Yun Qian, Hongbin Yu, Lei Huang, and Olga V. Kalashnikova
Geosci. Model Dev., 9, 1725–1746, https://doi.org/10.5194/gmd-9-1725-2016, https://doi.org/10.5194/gmd-9-1725-2016, 2016
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This study conducts the simulation of WRF-Chem with the quasi-global configuration for 2010–2014, and evaluates the simulation with multiple observation datasets for the first time. This study demonstrates that the WRF-Chem quasi-global simulation can be used for investigating trans-Pacific transport of aerosols and providing reasonable inflow chemical boundaries for the western USA to further understand the impact of transported pollutants on the regional air quality and climate.
N. I. Kristiansen, A. Stohl, D. J. L. Olivié, B. Croft, O. A. Søvde, H. Klein, T. Christoudias, D. Kunkel, S. J. Leadbetter, Y. H. Lee, K. Zhang, K. Tsigaridis, T. Bergman, N. Evangeliou, H. Wang, P.-L. Ma, R. C. Easter, P. J. Rasch, X. Liu, G. Pitari, G. Di Genova, S. Y. Zhao, Y. Balkanski, S. E. Bauer, G. S. Faluvegi, H. Kokkola, R. V. Martin, J. R. Pierce, M. Schulz, D. Shindell, H. Tost, and H. Zhang
Atmos. Chem. Phys., 16, 3525–3561, https://doi.org/10.5194/acp-16-3525-2016, https://doi.org/10.5194/acp-16-3525-2016, 2016
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Processes affecting aerosol removal from the atmosphere are not fully understood. In this study we investigate to what extent atmospheric transport models can reproduce observed loss of aerosols. We compare measurements of radioactive isotopes, that attached to ambient sulfate aerosols during the 2011 Fukushima nuclear accident, to 19 models using identical emissions. Results indicate aerosol removal that is too fast in most models, and apply to aerosols that have undergone long-range transport.
Shipeng Zhang, Minghuai Wang, Steven J. Ghan, Aijun Ding, Hailong Wang, Kai Zhang, David Neubauer, Ulrike Lohmann, Sylvaine Ferrachat, Toshihiko Takeamura, Andrew Gettelman, Hugh Morrison, Yunha Lee, Drew T. Shindell, Daniel G. Partridge, Philip Stier, Zak Kipling, and Congbin Fu
Atmos. Chem. Phys., 16, 2765–2783, https://doi.org/10.5194/acp-16-2765-2016, https://doi.org/10.5194/acp-16-2765-2016, 2016
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The variation of aerosol indirect effects (AIE) in several climate models is investigated across different dynamical regimes. Regimes with strong large-scale ascent are shown to be as important as stratocumulus regimes in studying AIE. AIE over regions with high monthly large-scale surface precipitation rate contributes the most to the total aerosol indirect forcing. These results point to the need to reduce the uncertainty in AIE in different dynamical regimes.
Xin Huang, Luxi Zhou, Aijun Ding, Ximeng Qi, Wei Nie, Minghuai Wang, Xuguang Chi, Tuukka Petäjä, Veli-Matti Kerminen, Pontus Roldin, Anton Rusanen, Markku Kulmala, and Michael Boy
Atmos. Chem. Phys., 16, 2477–2492, https://doi.org/10.5194/acp-16-2477-2016, https://doi.org/10.5194/acp-16-2477-2016, 2016
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By combining a regional model and a box model, this study simulates new particle formation in Nanjing, China, when the air masses were affected by anthropogenic activities, biogenic emissions, or mixed ocean and continental sources. The simulations reveal that biogenic organic compounds play a vital role in growth of newly formed clusters. This novel combination of two models makes it possible to accomplish new particle formation simulation without direct measurements of all chemical species.
Zak Kipling, Philip Stier, Colin E. Johnson, Graham W. Mann, Nicolas Bellouin, Susanne E. Bauer, Tommi Bergman, Mian Chin, Thomas Diehl, Steven J. Ghan, Trond Iversen, Alf Kirkevåg, Harri Kokkola, Xiaohong Liu, Gan Luo, Twan van Noije, Kirsty J. Pringle, Knut von Salzen, Michael Schulz, Øyvind Seland, Ragnhild B. Skeie, Toshihiko Takemura, Kostas Tsigaridis, and Kai Zhang
Atmos. Chem. Phys., 16, 2221–2241, https://doi.org/10.5194/acp-16-2221-2016, https://doi.org/10.5194/acp-16-2221-2016, 2016
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The vertical distribution of atmospheric aerosol is an important factor in its effects on climate. In this study we use a sophisticated model of the many interacting processes affecting aerosol in the atmosphere to show that the vertical distribution is typically dominated by only a few of these processes. Constraining these physical processes may help to reduce the large differences between models. However, the important processes are not always the same for different types of aerosol.
Kai Zhang, Chun Zhao, Hui Wan, Yun Qian, Richard C. Easter, Steven J. Ghan, Koichi Sakaguchi, and Xiaohong Liu
Geosci. Model Dev., 9, 607–632, https://doi.org/10.5194/gmd-9-607-2016, https://doi.org/10.5194/gmd-9-607-2016, 2016
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A sub-grid treatment based on Weibull distribution is introduced to CAM5 to take into account the impact of unresolved variability of surface wind speed on sea salt and dust emissions. Simulations show that sub-grid wind variability has relatively small impacts on the global mean sea salt emissions, but considerable influence on dust emissions. Dry convective eddies and mesoscale flows associated with complex topography are the major causes of dust emission enhancement.
X. Liu, P.-L. Ma, H. Wang, S. Tilmes, B. Singh, R. C. Easter, S. J. Ghan, and P. J. Rasch
Geosci. Model Dev., 9, 505–522, https://doi.org/10.5194/gmd-9-505-2016, https://doi.org/10.5194/gmd-9-505-2016, 2016
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In this study, we describe and evaluate a new four-mode version of the Modal Aerosol Module (MAM4) in the Community Atmosphere Model version 5 (CAM5). Compared to the current three-mode version of MAM in CAM5, MAM4 significantly improves the simulation of seasonal variation of BC concentrations in the polar regions, by increasing the BC concentrations in all seasons and particularly in cold seasons.
K. Thayer-Calder, A. Gettelman, C. Craig, S. Goldhaber, P. A. Bogenschutz, C.-C. Chen, H. Morrison, J. Höft, E. Raut, B. M. Griffin, J. K. Weber, V. E. Larson, M. C. Wyant, M. Wang, Z. Guo, and S. J. Ghan
Geosci. Model Dev., 8, 3801–3821, https://doi.org/10.5194/gmd-8-3801-2015, https://doi.org/10.5194/gmd-8-3801-2015, 2015
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This study evaluates a unified cloud parameterization and a Monte Carlo microphysics interface that is implemented in CAM v5.3. We show mean climate and tropical variability results from global simulations. The model has a degradation in precipitation skill but improvements in shortwave cloud forcing, liquid water path, long-wave cloud forcing, precipitable water, and tropical wave simulation. We also show estimation of computational expense and sensitivity to number of subcolumns.
R. Zhang, H. Wang, D. A. Hegg, Y. Qian, S. J. Doherty, C. Dang, P.-L. Ma, P. J. Rasch, and Q. Fu
Atmos. Chem. Phys., 15, 12805–12822, https://doi.org/10.5194/acp-15-12805-2015, https://doi.org/10.5194/acp-15-12805-2015, 2015
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We use a global climate model with an explicit source tagging technique to quantify contributions of emissions from various geographical regions and sectors to BC in North America. Model results are evaluated against measurements of near-surface and in-snow BC. We found strong spatial variations of BC and its radiative forcing that can be quantitatively attributed to the various source origins, and also identified a significant source of BC in snow that is likely missing in most climate models.
A. Lupascu, R. Easter, R. Zaveri, M. Shrivastava, M. Pekour, J. Tomlinson, Q. Yang, H. Matsui, A. Hodzic, Q. Zhang, and J. D. Fast
Atmos. Chem. Phys., 15, 12283–12313, https://doi.org/10.5194/acp-15-12283-2015, https://doi.org/10.5194/acp-15-12283-2015, 2015
B. Kravitz, A. Robock, S. Tilmes, O. Boucher, J. M. English, P. J. Irvine, A. Jones, M. G. Lawrence, M. MacCracken, H. Muri, J. C. Moore, U. Niemeier, S. J. Phipps, J. Sillmann, T. Storelvmo, H. Wang, and S. Watanabe
Geosci. Model Dev., 8, 3379–3392, https://doi.org/10.5194/gmd-8-3379-2015, https://doi.org/10.5194/gmd-8-3379-2015, 2015
R. Zhang, H. Wang, Y. Qian, P. J. Rasch, R. C. Easter, P.-L. Ma, B. Singh, J. Huang, and Q. Fu
Atmos. Chem. Phys., 15, 6205–6223, https://doi.org/10.5194/acp-15-6205-2015, https://doi.org/10.5194/acp-15-6205-2015, 2015
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We use the CAM5 model with a novel source-tagging technique to characterize the fate of BC particles emitted from various geographical regions and sectors and their transport pathways to the Himalayas and Tibetan Plateau (HTP). We show a comprehensive picture of the seasonal and regional dependence of BC source attributions, and find strong seasonal and spatial variations in BC-in-snow radiative forcing in the HTP that can be quantitatively attributed to the various regional/sectoral sources.
S. Tilmes, J.-F. Lamarque, L. K. Emmons, D. E. Kinnison, P.-L. Ma, X. Liu, S. Ghan, C. Bardeen, S. Arnold, M. Deeter, F. Vitt, T. Ryerson, J. W. Elkins, F. Moore, J. R. Spackman, and M. Val Martin
Geosci. Model Dev., 8, 1395–1426, https://doi.org/10.5194/gmd-8-1395-2015, https://doi.org/10.5194/gmd-8-1395-2015, 2015
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The Community Atmosphere Model (CAM), version 5, is now coupled to extensive tropospheric and stratospheric chemistry, called CAM5-chem, and is available in addition to CAM4-chem in the Community Earth System Model (CESM) version 1.2. Both configurations are well suited as tools for atmospheric chemistry modeling studies in the troposphere and lower stratosphere.
L. K. Berg, M. Shrivastava, R. C. Easter, J. D. Fast, E. G. Chapman, Y. Liu, and R. A. Ferrare
Geosci. Model Dev., 8, 409–429, https://doi.org/10.5194/gmd-8-409-2015, https://doi.org/10.5194/gmd-8-409-2015, 2015
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This work presents a new methodology for representing regional-scale impacts of cloud processing on both aerosol and trace gases in sub-grid-scale convective clouds. Using the new methodology, we can better simulate the aerosol lifecycle over large areas. The results presented in this work highlight the potential change in column-integrated amounts of black carbon, organic aerosol, and sulfate aerosol, which were found to range from -50% for black carbon to +40% for sulfate.
X. Shi, X. Liu, and K. Zhang
Atmos. Chem. Phys., 15, 1503–1520, https://doi.org/10.5194/acp-15-1503-2015, https://doi.org/10.5194/acp-15-1503-2015, 2015
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The ice nucleation scheme in the Community Atmosphere Model (CAM5) was improved by considering the effects of pre-existing ice crystals and some other modifications. Subsequently, the comparison between different ice nucleation parameterizations is investigated. Experiment using the ice nucleation parameterization of Kärcher et al. (2006) predicts a much smaller anthropogenic aerosol indirect forcing than that using the parameterizations of Liu and Penner (2005) and Barahona and Nenes (2009).
M. Wang, B. Xu, J. Cao, X. Tie, H. Wang, R. Zhang, Y. Qian, P. J. Rasch, S. Zhao, G. Wu, H. Zhao, D. R. Joswiak, J. Li, and Y. Xie
Atmos. Chem. Phys., 15, 1191–1204, https://doi.org/10.5194/acp-15-1191-2015, https://doi.org/10.5194/acp-15-1191-2015, 2015
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Carbonaceous aerosols recorded in a Tibetan glacier present a distinct seasonal dependence and an increasing trend after 1980, which has important implications for the accelerated glacier melting. We use a global aerosol--climate model to quantify the aerosol source--receptor relationships, showing that emissions in South Asia had the largest contribution. The emission inventories and historical fuel consumption in South Asia are consistent with our ice-core analysis and model results.
R. A. Scanza, N. Mahowald, S. Ghan, C. S. Zender, J. F. Kok, X. Liu, Y. Zhang, and S. Albani
Atmos. Chem. Phys., 15, 537–561, https://doi.org/10.5194/acp-15-537-2015, https://doi.org/10.5194/acp-15-537-2015, 2015
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The main purpose of this study was to build a framework in the Community Atmosphere Models version 4 and 5 within the Community Earth System Model to simulate dust aerosols as their component minerals. With this framework, we investigate the direct radiative forcing that results from the mineral speciation. We find that adding mineralogy results in a small positive forcing at the top of the atmosphere, while simulations without mineralogy have a small negative forcing.
R. L. Storer, B. M. Griffin, J. Höft, J. K. Weber, E. Raut, V. E. Larson, M. Wang, and P. J. Rasch
Geosci. Model Dev., 8, 1–19, https://doi.org/10.5194/gmd-8-1-2015, https://doi.org/10.5194/gmd-8-1-2015, 2015
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Representing clouds in climate models is a challenging problem. It is particularly difficult to represent deep convective clouds and, historically, deep convective parameterization is separate from the representation of other cloud types. Here we use a single-column cloud model to simulate three deep convective cases, and two shallow cloud cases. The results look reasonable, demonstrating that it may be possible to use one parameterization within a climate model for all cloud types.
S. M. Burrows, O. Ogunro, A. A. Frossard, L. M. Russell, P. J. Rasch, and S. M. Elliott
Atmos. Chem. Phys., 14, 13601–13629, https://doi.org/10.5194/acp-14-13601-2014, https://doi.org/10.5194/acp-14-13601-2014, 2014
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The air over the ocean is full of sea spray particles ejected by bubbles that burst in the wake of breaking waves. The smallest of such particles, less than a micrometer in diameter, include organic matter derived from ocean biota. This paper introduces a method to calculate the chemical composition of spray particles. Ocean organic matter is divided into several classes using a global model. Basic chemistry relationships predict the amount of organic material in emitted spray.
B. H. Samset, G. Myhre, A. Herber, Y. Kondo, S.-M. Li, N. Moteki, M. Koike, N. Oshima, J. P. Schwarz, Y. Balkanski, S. E. Bauer, N. Bellouin, T. K. Berntsen, H. Bian, M. Chin, T. Diehl, R. C. Easter, S. J. Ghan, T. Iversen, A. Kirkevåg, J.-F. Lamarque, G. Lin, X. Liu, J. E. Penner, M. Schulz, Ø. Seland, R. B. Skeie, P. Stier, T. Takemura, K. Tsigaridis, and K. Zhang
Atmos. Chem. Phys., 14, 12465–12477, https://doi.org/10.5194/acp-14-12465-2014, https://doi.org/10.5194/acp-14-12465-2014, 2014
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Far from black carbon (BC) emission sources, present climate models are unable to reproduce flight measurements. By comparing recent models with data, we find that the atmospheric lifetime of BC may be overestimated in models. By adjusting modeled BC concentrations to measurements in remote regions - over oceans and at high altitudes - we arrive at a reduced estimate for BC radiative forcing over the industrial era.
C. Zhao, Z. Hu, Y. Qian, L. Ruby Leung, J. Huang, M. Huang, J. Jin, M. G. Flanner, R. Zhang, H. Wang, H. Yan, Z. Lu, and D. G. Streets
Atmos. Chem. Phys., 14, 11475–11491, https://doi.org/10.5194/acp-14-11475-2014, https://doi.org/10.5194/acp-14-11475-2014, 2014
S. Yu, R. Mathur, J. Pleim, D. Wong, R. Gilliam, K. Alapaty, C. Zhao, and X. Liu
Atmos. Chem. Phys., 14, 11247–11285, https://doi.org/10.5194/acp-14-11247-2014, https://doi.org/10.5194/acp-14-11247-2014, 2014
K. Tsigaridis, N. Daskalakis, M. Kanakidou, P. J. Adams, P. Artaxo, R. Bahadur, Y. Balkanski, S. E. Bauer, N. Bellouin, A. Benedetti, T. Bergman, T. K. Berntsen, J. P. Beukes, H. Bian, K. S. Carslaw, M. Chin, G. Curci, T. Diehl, R. C. Easter, S. J. Ghan, S. L. Gong, A. Hodzic, C. R. Hoyle, T. Iversen, S. Jathar, J. L. Jimenez, J. W. Kaiser, A. Kirkevåg, D. Koch, H. Kokkola, Y. H Lee, G. Lin, X. Liu, G. Luo, X. Ma, G. W. Mann, N. Mihalopoulos, J.-J. Morcrette, J.-F. Müller, G. Myhre, S. Myriokefalitakis, N. L. Ng, D. O'Donnell, J. E. Penner, L. Pozzoli, K. J. Pringle, L. M. Russell, M. Schulz, J. Sciare, Ø. Seland, D. T. Shindell, S. Sillman, R. B. Skeie, D. Spracklen, T. Stavrakou, S. D. Steenrod, T. Takemura, P. Tiitta, S. Tilmes, H. Tost, T. van Noije, P. G. van Zyl, K. von Salzen, F. Yu, Z. Wang, Z. Wang, R. A. Zaveri, H. Zhang, K. Zhang, Q. Zhang, and X. Zhang
Atmos. Chem. Phys., 14, 10845–10895, https://doi.org/10.5194/acp-14-10845-2014, https://doi.org/10.5194/acp-14-10845-2014, 2014
Y. Wang, X. Liu, C. Hoose, and B. Wang
Atmos. Chem. Phys., 14, 10411–10430, https://doi.org/10.5194/acp-14-10411-2014, https://doi.org/10.5194/acp-14-10411-2014, 2014
H. Wan, P. J. Rasch, K. Zhang, Y. Qian, H. Yan, and C. Zhao
Geosci. Model Dev., 7, 1961–1977, https://doi.org/10.5194/gmd-7-1961-2014, https://doi.org/10.5194/gmd-7-1961-2014, 2014
K. Zhang, H. Wan, X. Liu, S. J. Ghan, G. J. Kooperman, P.-L. Ma, P. J. Rasch, D. Neubauer, and U. Lohmann
Atmos. Chem. Phys., 14, 8631–8645, https://doi.org/10.5194/acp-14-8631-2014, https://doi.org/10.5194/acp-14-8631-2014, 2014
R. A. Zaveri, R. C. Easter, J. E. Shilling, and J. H. Seinfeld
Atmos. Chem. Phys., 14, 5153–5181, https://doi.org/10.5194/acp-14-5153-2014, https://doi.org/10.5194/acp-14-5153-2014, 2014
G. W. Mann, K. S. Carslaw, C. L. Reddington, K. J. Pringle, M. Schulz, A. Asmi, D. V. Spracklen, D. A. Ridley, M. T. Woodhouse, L. A. Lee, K. Zhang, S. J. Ghan, R. C. Easter, X. Liu, P. Stier, Y. H. Lee, P. J. Adams, H. Tost, J. Lelieveld, S. E. Bauer, K. Tsigaridis, T. P. C. van Noije, A. Strunk, E. Vignati, N. Bellouin, M. Dalvi, C. E. Johnson, T. Bergman, H. Kokkola, K. von Salzen, F. Yu, G. Luo, A. Petzold, J. Heintzenberg, A. Clarke, J. A. Ogren, J. Gras, U. Baltensperger, U. Kaminski, S. G. Jennings, C. D. O'Dowd, R. M. Harrison, D. C. S. Beddows, M. Kulmala, Y. Viisanen, V. Ulevicius, N. Mihalopoulos, V. Zdimal, M. Fiebig, H.-C. Hansson, E. Swietlicki, and J. S. Henzing
Atmos. Chem. Phys., 14, 4679–4713, https://doi.org/10.5194/acp-14-4679-2014, https://doi.org/10.5194/acp-14-4679-2014, 2014
P.-L. Ma, P. J. Rasch, J. D. Fast, R. C. Easter, W. I. Gustafson Jr., X. Liu, S. J. Ghan, and B. Singh
Geosci. Model Dev., 7, 755–778, https://doi.org/10.5194/gmd-7-755-2014, https://doi.org/10.5194/gmd-7-755-2014, 2014
M. S. Long, W. C. Keene, R. C. Easter, R. Sander, X. Liu, A. Kerkweg, and D. Erickson
Atmos. Chem. Phys., 14, 3397–3425, https://doi.org/10.5194/acp-14-3397-2014, https://doi.org/10.5194/acp-14-3397-2014, 2014
C. Jiao, M. G. Flanner, Y. Balkanski, S. E. Bauer, N. Bellouin, T. K. Berntsen, H. Bian, K. S. Carslaw, M. Chin, N. De Luca, T. Diehl, S. J. Ghan, T. Iversen, A. Kirkevåg, D. Koch, X. Liu, G. W. Mann, J. E. Penner, G. Pitari, M. Schulz, Ø. Seland, R. B. Skeie, S. D. Steenrod, P. Stier, T. Takemura, K. Tsigaridis, T. van Noije, Y. Yun, and K. Zhang
Atmos. Chem. Phys., 14, 2399–2417, https://doi.org/10.5194/acp-14-2399-2014, https://doi.org/10.5194/acp-14-2399-2014, 2014
C. Zhao, X. Liu, Y. Qian, J. Yoon, Z. Hou, G. Lin, S. McFarlane, H. Wang, B. Yang, P.-L. Ma, H. Yan, and J. Bao
Atmos. Chem. Phys., 13, 10969–10987, https://doi.org/10.5194/acp-13-10969-2013, https://doi.org/10.5194/acp-13-10969-2013, 2013
C. Zhao, S. Chen, L. R. Leung, Y. Qian, J. F. Kok, R. A. Zaveri, and J. Huang
Atmos. Chem. Phys., 13, 10733–10753, https://doi.org/10.5194/acp-13-10733-2013, https://doi.org/10.5194/acp-13-10733-2013, 2013
J. Brioude, D. Arnold, A. Stohl, M. Cassiani, D. Morton, P. Seibert, W. Angevine, S. Evan, A. Dingwell, J. D. Fast, R. C. Easter, I. Pisso, J. Burkhart, and G. Wotawa
Geosci. Model Dev., 6, 1889–1904, https://doi.org/10.5194/gmd-6-1889-2013, https://doi.org/10.5194/gmd-6-1889-2013, 2013
S. J. Ghan
Atmos. Chem. Phys., 13, 9971–9974, https://doi.org/10.5194/acp-13-9971-2013, https://doi.org/10.5194/acp-13-9971-2013, 2013
J.-F. Lamarque, F. Dentener, J. McConnell, C.-U. Ro, M. Shaw, R. Vet, D. Bergmann, P. Cameron-Smith, S. Dalsoren, R. Doherty, G. Faluvegi, S. J. Ghan, B. Josse, Y. H. Lee, I. A. MacKenzie, D. Plummer, D. T. Shindell, R. B. Skeie, D. S. Stevenson, S. Strode, G. Zeng, M. Curran, D. Dahl-Jensen, S. Das, D. Fritzsche, and M. Nolan
Atmos. Chem. Phys., 13, 7997–8018, https://doi.org/10.5194/acp-13-7997-2013, https://doi.org/10.5194/acp-13-7997-2013, 2013
H. Wan, P. J. Rasch, K. Zhang, J. Kazil, and L. R. Leung
Geosci. Model Dev., 6, 861–874, https://doi.org/10.5194/gmd-6-861-2013, https://doi.org/10.5194/gmd-6-861-2013, 2013
K. Zhang, X. Liu, M. Wang, J. M. Comstock, D. L. Mitchell, S. Mishra, and G. G. Mace
Atmos. Chem. Phys., 13, 4963–4982, https://doi.org/10.5194/acp-13-4963-2013, https://doi.org/10.5194/acp-13-4963-2013, 2013
P. Stier, N. A. J. Schutgens, N. Bellouin, H. Bian, O. Boucher, M. Chin, S. Ghan, N. Huneeus, S. Kinne, G. Lin, X. Ma, G. Myhre, J. E. Penner, C. A. Randles, B. Samset, M. Schulz, T. Takemura, F. Yu, H. Yu, and C. Zhou
Atmos. Chem. Phys., 13, 3245–3270, https://doi.org/10.5194/acp-13-3245-2013, https://doi.org/10.5194/acp-13-3245-2013, 2013
D. T. Shindell, J.-F. Lamarque, M. Schulz, M. Flanner, C. Jiao, M. Chin, P. J. Young, Y. H. Lee, L. Rotstayn, N. Mahowald, G. Milly, G. Faluvegi, Y. Balkanski, W. J. Collins, A. J. Conley, S. Dalsoren, R. Easter, S. Ghan, L. Horowitz, X. Liu, G. Myhre, T. Nagashima, V. Naik, S. T. Rumbold, R. Skeie, K. Sudo, S. Szopa, T. Takemura, A. Voulgarakis, J.-H. Yoon, and F. Lo
Atmos. Chem. Phys., 13, 2939–2974, https://doi.org/10.5194/acp-13-2939-2013, https://doi.org/10.5194/acp-13-2939-2013, 2013
Y. H. Lee, J.-F. Lamarque, M. G. Flanner, C. Jiao, D. T. Shindell, T. Berntsen, M. M. Bisiaux, J. Cao, W. J. Collins, M. Curran, R. Edwards, G. Faluvegi, S. Ghan, L. W. Horowitz, J. R. McConnell, J. Ming, G. Myhre, T. Nagashima, V. Naik, S. T. Rumbold, R. B. Skeie, K. Sudo, T. Takemura, F. Thevenon, B. Xu, and J.-H. Yoon
Atmos. Chem. Phys., 13, 2607–2634, https://doi.org/10.5194/acp-13-2607-2013, https://doi.org/10.5194/acp-13-2607-2013, 2013
B. H. Samset, G. Myhre, M. Schulz, Y. Balkanski, S. Bauer, T. K. Berntsen, H. Bian, N. Bellouin, T. Diehl, R. C. Easter, S. J. Ghan, T. Iversen, S. Kinne, A. Kirkevåg, J.-F. Lamarque, G. Lin, X. Liu, J. E. Penner, Ø. Seland, R. B. Skeie, P. Stier, T. Takemura, K. Tsigaridis, and K. Zhang
Atmos. Chem. Phys., 13, 2423–2434, https://doi.org/10.5194/acp-13-2423-2013, https://doi.org/10.5194/acp-13-2423-2013, 2013
M. S. Long, W. C. Keene, R. Easter, R. Sander, A. Kerkweg, D. Erickson, X. Liu, and S. Ghan
Geosci. Model Dev., 6, 255–262, https://doi.org/10.5194/gmd-6-255-2013, https://doi.org/10.5194/gmd-6-255-2013, 2013
A. Kirkevåg, T. Iversen, Ø. Seland, C. Hoose, J. E. Kristjánsson, H. Struthers, A. M. L. Ekman, S. Ghan, J. Griesfeller, E. D. Nilsson, and M. Schulz
Geosci. Model Dev., 6, 207–244, https://doi.org/10.5194/gmd-6-207-2013, https://doi.org/10.5194/gmd-6-207-2013, 2013
J.-F. Lamarque, D. T. Shindell, B. Josse, P. J. Young, I. Cionni, V. Eyring, D. Bergmann, P. Cameron-Smith, W. J. Collins, R. Doherty, S. Dalsoren, G. Faluvegi, G. Folberth, S. J. Ghan, L. W. Horowitz, Y. H. Lee, I. A. MacKenzie, T. Nagashima, V. Naik, D. Plummer, M. Righi, S. T. Rumbold, M. Schulz, R. B. Skeie, D. S. Stevenson, S. Strode, K. Sudo, S. Szopa, A. Voulgarakis, and G. Zeng
Geosci. Model Dev., 6, 179–206, https://doi.org/10.5194/gmd-6-179-2013, https://doi.org/10.5194/gmd-6-179-2013, 2013
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Marit Sandstad, Borgar Aamaas, Ane Nordlie Johansen, Marianne Tronstad Lund, Glen Philip Peters, Bjørn Hallvard Samset, Benjamin Mark Sanderson, and Ragnhild Bieltvedt Skeie
Geosci. Model Dev., 17, 6589–6625, https://doi.org/10.5194/gmd-17-6589-2024, https://doi.org/10.5194/gmd-17-6589-2024, 2024
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The CICERO-SCM has existed as a Fortran model since 1999 that calculates the radiative forcing and concentrations from emissions and is an upwelling diffusion energy balance model of the ocean that calculates temperature change. In this paper, we describe an updated version ported to Python and publicly available at https://github.com/ciceroOslo/ciceroscm (https://doi.org/10.5281/zenodo.10548720). This version contains functionality for parallel runs and automatic calibration.
Zheng Xiang, Yongkang Xue, Weidong Guo, Melannie D. Hartman, Ye Liu, and William J. Parton
Geosci. Model Dev., 17, 6437–6464, https://doi.org/10.5194/gmd-17-6437-2024, https://doi.org/10.5194/gmd-17-6437-2024, 2024
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A process-based plant carbon (C)–nitrogen (N) interface coupling framework has been developed which mainly focuses on plant resistance and N-limitation effects on photosynthesis, plant respiration, and plant phenology. A dynamic C / N ratio is introduced to represent plant resistance and self-adjustment. The framework has been implemented in a coupled biophysical-ecosystem–biogeochemical model, and testing results show a general improvement in simulating plant properties with this framework.
Yangke Liu, Qing Bao, Bian He, Xiaofei Wu, Jing Yang, Yimin Liu, Guoxiong Wu, Tao Zhu, Siyuan Zhou, Yao Tang, Ankang Qu, Yalan Fan, Anling Liu, Dandan Chen, Zhaoming Luo, Xing Hu, and Tongwen Wu
Geosci. Model Dev., 17, 6249–6275, https://doi.org/10.5194/gmd-17-6249-2024, https://doi.org/10.5194/gmd-17-6249-2024, 2024
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We give an overview of the Institute of Atmospheric Physics–Chinese Academy of Sciences subseasonal-to-seasonal ensemble forecasting system and Madden–Julian Oscillation forecast evaluation of the system. Compared to other S2S models, the IAP-CAS model has its benefits but also biases, i.e., underdispersive ensemble, overestimated amplitude, and faster propagation speed when forecasting MJO. We provide a reason for these biases and prospects for further improvement of this system in the future.
Laurent Brodeau, Pierre Rampal, Einar Ólason, and Véronique Dansereau
Geosci. Model Dev., 17, 6051–6082, https://doi.org/10.5194/gmd-17-6051-2024, https://doi.org/10.5194/gmd-17-6051-2024, 2024
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A new brittle sea ice rheology, BBM, has been implemented into the sea ice component of NEMO. We describe how a new spatial discretization framework was introduced to achieve this. A set of idealized and realistic ocean and sea ice simulations of the Arctic have been performed using BBM and the standard viscous–plastic rheology of NEMO. When compared to satellite data, our simulations show that our implementation of BBM leads to a fairly good representation of sea ice deformations.
Joseph P. Hollowed, Christiane Jablonowski, Hunter Y. Brown, Benjamin R. Hillman, Diana L. Bull, and Joseph L. Hart
Geosci. Model Dev., 17, 5913–5938, https://doi.org/10.5194/gmd-17-5913-2024, https://doi.org/10.5194/gmd-17-5913-2024, 2024
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Large volcanic eruptions deposit material in the upper atmosphere, which is capable of altering temperature and wind patterns of Earth's atmosphere for subsequent years. This research describes a new method of simulating these effects in an idealized, efficient atmospheric model. A volcanic eruption of sulfur dioxide is described with a simplified set of physical rules, which eventually cools the planetary surface. This model has been designed as a test bed for climate attribution studies.
Hong Li, Yi Yang, Jian Sun, Yuan Jiang, Ruhui Gan, and Qian Xie
Geosci. Model Dev., 17, 5883–5896, https://doi.org/10.5194/gmd-17-5883-2024, https://doi.org/10.5194/gmd-17-5883-2024, 2024
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Vertical atmospheric motions play a vital role in convective-scale precipitation forecasts by connecting atmospheric dynamics with cloud development. A three-dimensional variational vertical velocity assimilation scheme is developed within the high-resolution CMA-MESO model, utilizing the adiabatic Richardson equation as the observation operator. A 10 d continuous run and an individual case study demonstrate improved forecasts, confirming the scheme's effectiveness.
Matthias Nützel, Laura Stecher, Patrick Jöckel, Franziska Winterstein, Martin Dameris, Michael Ponater, Phoebe Graf, and Markus Kunze
Geosci. Model Dev., 17, 5821–5849, https://doi.org/10.5194/gmd-17-5821-2024, https://doi.org/10.5194/gmd-17-5821-2024, 2024
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We extended the infrastructure of our modelling system to enable the use of an additional radiation scheme. After calibrating the model setups to the old and the new radiation scheme, we find that the simulation with the new scheme shows considerable improvements, e.g. concerning the cold-point temperature and stratospheric water vapour. Furthermore, perturbations of radiative fluxes associated with greenhouse gas changes, e.g. of methane, tend to be improved when the new scheme is employed.
Yibing Wang, Xianhong Xie, Bowen Zhu, Arken Tursun, Fuxiao Jiang, Yao Liu, Dawei Peng, and Buyun Zheng
Geosci. Model Dev., 17, 5803–5819, https://doi.org/10.5194/gmd-17-5803-2024, https://doi.org/10.5194/gmd-17-5803-2024, 2024
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Urban expansion intensifies challenges like urban heat and urban dry islands. To address this, we developed an urban module, VIC-urban, in the Variable Infiltration Capacity (VIC) model. Tested in Beijing, VIC-urban accurately simulated turbulent heat fluxes, runoff, and land surface temperature. We provide a reliable tool for large-scale simulations considering urban environment and a systematic urban modelling framework within VIC, offering crucial insights for urban planners and designers.
Jeremy Carter, Erick A. Chacón-Montalván, and Amber Leeson
Geosci. Model Dev., 17, 5733–5757, https://doi.org/10.5194/gmd-17-5733-2024, https://doi.org/10.5194/gmd-17-5733-2024, 2024
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Climate models are essential tools in the study of climate change and its wide-ranging impacts on life on Earth. However, the output is often afflicted with some bias. In this paper, a novel model is developed to predict and correct bias in the output of climate models. The model captures uncertainty in the correction and explicitly models underlying spatial correlation between points. These features are of key importance for climate change impact assessments and resulting decision-making.
Anna Martin, Veronika Gayler, Benedikt Steil, Klaus Klingmüller, Patrick Jöckel, Holger Tost, Jos Lelieveld, and Andrea Pozzer
Geosci. Model Dev., 17, 5705–5732, https://doi.org/10.5194/gmd-17-5705-2024, https://doi.org/10.5194/gmd-17-5705-2024, 2024
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The study evaluates the land surface and vegetation model JSBACHv4 as a replacement for the simplified submodel SURFACE in EMAC. JSBACH mitigates earlier problems of soil dryness, which are critical for vegetation modelling. When analysed using different datasets, the coupled model shows strong correlations of key variables, such as land surface temperature, surface albedo and radiation flux. The versatility of the model increases significantly, while the overall performance does not degrade.
Hugo Banderier, Christian Zeman, David Leutwyler, Stefan Rüdisühli, and Christoph Schär
Geosci. Model Dev., 17, 5573–5586, https://doi.org/10.5194/gmd-17-5573-2024, https://doi.org/10.5194/gmd-17-5573-2024, 2024
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We investigate the effects of reduced-precision arithmetic in a state-of-the-art regional climate model by studying the results of 10-year-long simulations. After this time, the results of the reduced precision and the standard implementation are hardly different. This should encourage the use of reduced precision in climate models to exploit the speedup and memory savings it brings. The methodology used in this work can help researchers verify reduced-precision implementations of their model.
David Fuchs, Steven C. Sherwood, Abhnil Prasad, Kirill Trapeznikov, and Jim Gimlett
Geosci. Model Dev., 17, 5459–5475, https://doi.org/10.5194/gmd-17-5459-2024, https://doi.org/10.5194/gmd-17-5459-2024, 2024
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Machine learning (ML) of unresolved processes offers many new possibilities for improving weather and climate models, but integrating ML into the models has been an engineering challenge, and there are performance issues. We present a new software plugin for this integration, TorchClim, that is scalable and flexible and thereby allows a new level of experimentation with the ML approach. We also provide guidance on ML training and demonstrate a skillful hybrid ML atmosphere model.
Minjin Lee, Charles A. Stock, John P. Dunne, and Elena Shevliakova
Geosci. Model Dev., 17, 5191–5224, https://doi.org/10.5194/gmd-17-5191-2024, https://doi.org/10.5194/gmd-17-5191-2024, 2024
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Modeling global freshwater solid and nutrient loads, in both magnitude and form, is imperative for understanding emerging eutrophication problems. Such efforts, however, have been challenged by the difficulty of balancing details of freshwater biogeochemical processes with limited knowledge, input, and validation datasets. Here we develop a global freshwater model that resolves intertwined algae, solid, and nutrient dynamics and provide performance assessment against measurement-based estimates.
Hunter York Brown, Benjamin Wagman, Diana Bull, Kara Peterson, Benjamin Hillman, Xiaohong Liu, Ziming Ke, and Lin Lin
Geosci. Model Dev., 17, 5087–5121, https://doi.org/10.5194/gmd-17-5087-2024, https://doi.org/10.5194/gmd-17-5087-2024, 2024
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Explosive volcanic eruptions lead to long-lived, microscopic particles in the upper atmosphere which act to cool the Earth's surface by reflecting the Sun's light back to space. We include and test this process in a global climate model, E3SM. E3SM is tested against satellite and balloon observations of the 1991 eruption of Mt. Pinatubo, showing that with these particles in the model we reasonably recreate Pinatubo and its global effects. We also explore how particle size leads to these effects.
Carl Svenhag, Moa K. Sporre, Tinja Olenius, Daniel Yazgi, Sara M. Blichner, Lars P. Nieradzik, and Pontus Roldin
Geosci. Model Dev., 17, 4923–4942, https://doi.org/10.5194/gmd-17-4923-2024, https://doi.org/10.5194/gmd-17-4923-2024, 2024
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Our research shows the importance of modeling new particle formation (NPF) and growth of particles in the atmosphere on a global scale, as they influence the outcomes of clouds and our climate. With the global model EC-Earth3 we show that using a new method for NPF modeling, which includes new detailed processes with NH3 and H2SO4, significantly impacts the number of particles in the air and clouds and changes the radiation balance of the same magnitude as anthropogenic greenhouse emissions.
Mengjie Han, Qing Zhao, Xili Wang, Ying-Ping Wang, Philippe Ciais, Haicheng Zhang, Daniel S. Goll, Lei Zhu, Zhe Zhao, Zhixuan Guo, Chen Wang, Wei Zhuang, Fengchang Wu, and Wei Li
Geosci. Model Dev., 17, 4871–4890, https://doi.org/10.5194/gmd-17-4871-2024, https://doi.org/10.5194/gmd-17-4871-2024, 2024
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The impact of biochar (BC) on soil organic carbon (SOC) dynamics is not represented in most land carbon models used for assessing land-based climate change mitigation. Our study develops a BC model that incorporates our current understanding of BC effects on SOC based on a soil carbon model (MIMICS). The BC model can reproduce the SOC changes after adding BC, providing a useful tool to couple dynamic land models to evaluate the effectiveness of BC application for CO2 removal from the atmosphere.