Articles | Volume 15, issue 12
https://doi.org/10.5194/gmd-15-4881-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/gmd-15-4881-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Model description paper
| 
27 Jun 2022
Model description paper |
| 27 Jun 2022
| 27 Jun 2022
Description and evaluation of the tropospheric aerosol scheme in the Integrated Forecasting System (IFS-AER, cycle 47R1) of ECMWF
HYGEOS, Lille, France
Zak Kipling
European Centre for Medium-Range Weather Forecasts, Reading, UK
Vincent Huijnen
Royal Netherlands Meteorological Institute, De Bilt, the Netherlands
Johannes Flemming
European Centre for Medium-Range Weather Forecasts, Reading, UK
Pierre Nabat
Météo-France, Toulouse, France
Martine Michou
Météo-France, Toulouse, France
Melanie Ades
European Centre for Medium-Range Weather Forecasts, Reading, UK
Richard Engelen
European Centre for Medium-Range Weather Forecasts, Reading, UK
Vincent-Henri Peuch
European Centre for Medium-Range Weather Forecasts, Reading, UK
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Atmos. Chem. Phys., 22, 11009–11032, https://doi.org/10.5194/acp-22-11009-2022, https://doi.org/10.5194/acp-22-11009-2022, 2022
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Vincent Huijnen, Philippe Le Sager, Marcus O. Köhler, Glenn Carver, Samuel Rémy, Johannes Flemming, Simon Chabrillat, Quentin Errera, and Twan van Noije
Geosci. Model Dev., 15, 6221–6241, https://doi.org/10.5194/gmd-15-6221-2022, https://doi.org/10.5194/gmd-15-6221-2022, 2022
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We report on the first implementation of atmospheric chemistry and aerosol as part of the OpenIFS model, based on the CAMS global model. We give an overview of the model and evaluate two reference model configurations, with and without the stratospheric chemistry extension, against a variety of observational datasets. This OpenIFS version with atmospheric composition components is open to the scientific user community under a standard OpenIFS license.
Maria Sand, Bjørn H. Samset, Gunnar Myhre, Jonas Gliß, Susanne E. Bauer, Huisheng Bian, Mian Chin, Ramiro Checa-Garcia, Paul Ginoux, Zak Kipling, Alf Kirkevåg, Harri Kokkola, Philippe Le Sager, Marianne T. Lund, Hitoshi Matsui, Twan van Noije, Dirk J. L. Olivié, Samuel Remy, Michael Schulz, Philip Stier, Camilla W. Stjern, Toshihiko Takemura, Kostas Tsigaridis, Svetlana G. Tsyro, and Duncan Watson-Parris
Atmos. Chem. Phys., 21, 15929–15947, https://doi.org/10.5194/acp-21-15929-2021, https://doi.org/10.5194/acp-21-15929-2021, 2021
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Absorption of shortwave radiation by aerosols can modify precipitation and clouds but is poorly constrained in models. A total of 15 different aerosol models from AeroCom phase III have reported total aerosol absorption, and for the first time, 11 of these models have reported in a consistent experiment the contributions to absorption from black carbon, dust, and organic aerosol. Here, we document the model diversity in aerosol absorption.
Anthony C. Jones, Adrian Hill, Samuel Remy, N. Luke Abraham, Mohit Dalvi, Catherine Hardacre, Alan J. Hewitt, Ben Johnson, Jane P. Mulcahy, and Steven T. Turnock
Atmos. Chem. Phys., 21, 15901–15927, https://doi.org/10.5194/acp-21-15901-2021, https://doi.org/10.5194/acp-21-15901-2021, 2021
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EGUsphere, https://doi.org/10.5194/egusphere-2026-4322, https://doi.org/10.5194/egusphere-2026-4322, 2026
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Paolo Andreozzi, Mark D. Fielding, Robin J. Hogan, Richard M. Forbes, Adrian A. Hill, Samuel Rémy, Birger Bohn, and Ulrich Löhnert
Atmos. Chem. Phys., 26, 11309–11338, https://doi.org/10.5194/acp-26-11309-2026, https://doi.org/10.5194/acp-26-11309-2026, 2026
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Bosi Sheng, Massimo A. Bollasina, Alexandre S. Gagnon, Laura J. Wilcox, Thomas P. S. Reynolds, Christopher T. S. Beckett, Haolin Wang, Qingxiang Li, Pierre Nabat, Robert J. Allen, Bjørn H. Samset, Joonas Merikanto, Geeta G. Persad, Toshihiko Takemura, Kostas Tsigaridis, Sharar Ahmadi, Maxwell T. Elling, Knut von Salzen, Daniel M. Westervelt, Naga Oshima, and Tsuyoshi Koshiro
EGUsphere, https://doi.org/10.5194/egusphere-2026-2198, https://doi.org/10.5194/egusphere-2026-2198, 2026
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Dylan B. A. Jones, Lucas Prates, Zhen Qu, William Y. Y. Cheng, Kazuyuki Miyazaki, Takashi Sekiya, Antje Inness, Rajesh Kumar, Xiao Tang, Helen Worden, Gerbrand Koren, and Vincent Huijnen
Atmos. Chem. Phys., 26, 6655–6682, https://doi.org/10.5194/acp-26-6655-2026, https://doi.org/10.5194/acp-26-6655-2026, 2026
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We evaluate five chemical reanalysis products to assess their potential to provide useful information on tropospheric ozone variability. We find that the reanalyses produce consistent information on ozone variations in the free troposphere, but have large discrepancies at the surface. The results suggests that improvements in the reanalyses are needed to better exploit the assimilated observations to enhance the utility of the reanalysis products at the surface.
Eliza K. Duncan, George Jordan, Paul Kim, James M. Haywood, Duncan Watson-Parris, Ben Johnson, Alistair Sellar, Zak Kipling, João Teixeira, Florent Malavelle, and Daniel G. Partridge
EGUsphere, https://doi.org/10.5194/egusphere-2026-1043, https://doi.org/10.5194/egusphere-2026-1043, 2026
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The 2014–15 Holuhraun eruption offers a natural experiment to assess how well climate models can capture the changes in aerosol associated with the plume. We investigate the aerosol lifecycle during transport to identify key differences in climate models' representation of aerosol processes, which could affect the models’ ability to capture changes in cloud properties. Our study highlights the importance of the representation of boundary layer nucleation processes in climate models.
Glenn-Michael Oomen, Jean-François Müller, Trissevgeni Stavrakou, Isabelle De Smedt, Vincent Huijnen, Flora Kluge, Antje Inness, and Johannes Flemming
EGUsphere, https://doi.org/10.5194/egusphere-2026-2362, https://doi.org/10.5194/egusphere-2026-2362, 2026
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Isoprene is a commonly emitted organic gas emitted by trees. In this work, we strongly simplified the chemical mechanism through parametric fitting, which helps scientists study air pollution and climate more efficiently. By comparing it with a detailed model and satellite observations, we show that the simplified version produces very similar results. This means faster calculations are possible without losing accuracy, improving studies of emissions and air quality worldwide.
Quentin Errera, Marc Op de beeck, Stefan Bender, Johannes Flemming, Bernd Funke, Alex Hoffmann, Michael Höpfner, Nathaniel Livesey, Gabriele Poli, Didier Pieroux, Piera Raspollini, and Björn-Martin Sinnhuber
Atmos. Meas. Tech., 19, 2601–2620, https://doi.org/10.5194/amt-19-2601-2026, https://doi.org/10.5194/amt-19-2601-2026, 2026
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The Changing Atmosphere Infra-Red Tomography Explorer (CAIRT) is a satellite mission concept developed to observe, among other, the gradient of ozone and water vapour in the upper troposphere and lower stratosphere where these species have their largest radiative impact. By simulating CAIRT observations and measuring their constrain on an atmospheric model using data assimilation, this study shows that CAIRT specifications are adequate to fulfil this objective.
Tim Butler, Tabish Ansari, Claudio A. Belis, Elisa Bergas-Masso, Willem van Caspel, Hilde Fagerli, Johannes Flemming, Marta Garcia Vivanco, Paul Griffiths, Douglas S. Hamilton, Coralina Hernandez Trujillo, Lena Höglund-Isaksson, Vincent Huijnen, Matthew Kasoar, Johannes W. Kaiser, Gerbrand Koren, Zbigniew Klimont, Florian Lindl, Aura Lupascu, Mariano Mertens, Martijn Schaap, Steven T. Turnock, Oliver Wild, Philipp Weiss, Jacek Kaminski, Rosa Wu, and Terry Keating
EGUsphere, https://doi.org/10.5194/egusphere-2026-1367, https://doi.org/10.5194/egusphere-2026-1367, 2026
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Air pollution travels across continents, meaning emissions in one region can affect air quality far away. To better understand this, scientists from many groups are planning to run coordinated computer simulations of the atmosphere. By comparing results across models and emission scenarios, the planned study will show how pollution moves between regions and which sources matter most, helping governments design more effective air quality policies.
Michael Kahnert, Melanie Ades, Mickaël Bacles, Johannes Flemming, Vincent Guidard, Alexander Haefele, Robin J. Hogan, Samuel Rémy, and Eric Sauvageat
EGUsphere, https://doi.org/10.5194/egusphere-2025-6077, https://doi.org/10.5194/egusphere-2025-6077, 2026
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The Copernicus Atmosphere Monitoring Service (CAMS) provides quality-controlled information related to air quality and health. We explore the possibility to constrain the CAMS global forecasting model by use of ground-based observations of laser light backscattered by particulate matter. We find that the vertical distribution of particulate matter can be predicted more faithfully with this approach, which can have implications for air quality forecasts provided by CAMS to end users.
Anna Moustaka, Antonis Gkikas, Stavros-Andreas Logothetis, Johannes Flemming, Samuel Rémy, Melanie Ades, Angela Benedetti, Kleareti Tourpali, Vassilis Amiridis, and Stelios Kazadzis
EGUsphere, https://doi.org/10.5194/egusphere-2026-1107, https://doi.org/10.5194/egusphere-2026-1107, 2026
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Qinren Shi, Philippe Ciais, Nicolas Megel, Xavier Bonnemaizon, Rohith Teja Mittakola, Richard Engelen, and Chuanlong Zhou
Earth Syst. Sci. Data, 18, 927–944, https://doi.org/10.5194/essd-18-927-2026, https://doi.org/10.5194/essd-18-927-2026, 2026
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This study developed high-resolution maps (100 m × 100 m) showing how much carbon dioxide is emitted from cars and trucks in 20 European cities every hour. Using anonymous GPS signals from vehicles, we tracked traffic CO2 emission patterns throughout the year 2023. The results show that emissions vary significantly between cities and across different days and seasons. This method could help cities monitor on-road emissions in real time and design better strategies to reduce them.
Jason E. Williams, Swen Metzger, Samuel Rémy, Vincent Huijnen, and Johannes Flemming
Geosci. Model Dev., 18, 9913–9943, https://doi.org/10.5194/gmd-18-9913-2025, https://doi.org/10.5194/gmd-18-9913-2025, 2025
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One of the main constituents of Particulate Matter at the surface are Secondary Inorganic Aerosols (SIA) which are influenced by both anthropogenic emissions and the acidity of clouds and aerosols. This study shows improvements in introduced into the IFS-COMPO (Integrated Forecast System-COMPOsition) simulating the surface concentrations of SIA and the resulting changes in the total wet deposition for Europe, the US and South-East Asia.
Simon Chabrillat, Samuel Rémy, Quentin Errera, Vincent Huijnen, Christine Bingen, Jonas Debosscher, François Hendrick, Swen Metzger, Adrien Mora, Daniele Minganti, Marc Op de beek, Léa Reisenfeld, Jason E. Williams, Henk Eskes, and Johannes Flemming
Geosci. Model Dev., 18, 8973–9014, https://doi.org/10.5194/gmd-18-8973-2025, https://doi.org/10.5194/gmd-18-8973-2025, 2025
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We document the forecasts of the composition of the stratosphere by the Copernicus Atmosphere Monitoring Service. The model's predictions are compared with satellite measurements over a recent period, during polar ozone depletion events, and after the Mount Pinatubo volcanic eruption. The system performs well for sulfate aerosols, ozone and several other key gases but not as well for several nitrogen-containing gases. Chemical processes in aerosols and polar clouds should be improved.
Sini Talvinen, Paul Kim, Emanuele Tovazzi, Eemeli Holopainen, Roxana Cremer, Thomas Kühn, Harri Kokkola, Zak Kipling, David Neubauer, João C. Teixeira, Alistair Sellar, Duncan Watson-Parris, Yang Yang, Jialei Zhu, Srinath Krishnan, Annele Virtanen, and Daniel G. Partridge
Atmos. Chem. Phys., 25, 14449–14478, https://doi.org/10.5194/acp-25-14449-2025, https://doi.org/10.5194/acp-25-14449-2025, 2025
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Climate models struggle to predict how clouds and aerosols interact, affecting Earth’s energy balance. This study compares models to observations to see how they describe effects of clouds and rain on aerosols. While both models show similar overall trends, seasonal differences emerged. These, however, align with differences in key variables participating in cloud formation. The study provides insights on how to improve the representation of aerosol-cloud interactions in climate models.
Léon Roussel, Marie Dumont, Marion Réveillet, Delphine Six, Marin Kneib, Pierre Nabat, Kévin Fourteau, Diego Monteiro, Simon Gascoin, Emmanuel Thibert, Antoine Rabatel, Jean-Emmanuel Sicart, Mylène Bonnefoy, Luc Piard, Olivier Laarman, Bruno Jourdain, Mathieu Fructus, Matthieu Vernay, and Matthieu Lafaysse
The Cryosphere, 19, 5201–5230, https://doi.org/10.5194/tc-19-5201-2025, https://doi.org/10.5194/tc-19-5201-2025, 2025
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Saharan dust deposits frequently turn alpine glaciers orange. Mineral dust reduces snow albedo and increases snow and glaciers melt rate. Using physical modeling, we quantified the impact of dust on the Argentière Glacier over the period 2019–2022. We found that the contribution of mineral dust to the melt represents between 8 % and 16 % of Argentière Glacier summer melt. At specific locations, the impact of dust over one year can rise to an equivalent of 1.2 m of melted ice.
George Jordan, Florent Malavelle, Jim Haywood, Ying Chen, Ben Johnson, Daniel Partridge, Amy Peace, Eliza Duncan, Duncan Watson-Parris, David Neubauer, Anton Laakso, Martine Michou, and Pierre Nabat
Atmos. Chem. Phys., 25, 13393–13428, https://doi.org/10.5194/acp-25-13393-2025, https://doi.org/10.5194/acp-25-13393-2025, 2025
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The 2014–15 Holuhraun eruption created a vast aerosol plume that acted as a natural experiment to assess how well climate models capture changes in cloud properties due to increased aerosol. We find that climate models represent the observed shift to smaller, more numerous cloud droplets well. However, climate models diverge in their aerosol-induced changes to large-scale cloud properties, particularly cloud liquid water content. Our study shows that Holuhraun had a cooling effect on the Earth.
Augustin Colette, Gaëlle Collin, François Besson, Etienne Blot, Vincent Guidard, Frédérik Meleux, Adrien Royer, Valentin Petiot, Claire Miller, Oihana Fermond, Alizé Jeant, Mario Adani, Joaquim Arteta, Anna Benedictow, Robert Bergström, Dene Bowdalo, Jorgen Brandt, Gino Briganti, Ana C. Carvalho, Jesper Heile Christensen, Florian Couvidat, Ilaria D'Elia, Massimo D'Isidoro, Hugo Denier van der Gon, Gaël Descombes, Enza Di Tomaso, John Douros, Jeronimo Escribano, Henk Eskes, Hilde Fagerli, Yalda Fatahi, Johannes Flemming, Elmar Friese, Lise Frohn, Michael Gauss, Camilla Geels, Guido Guarnieri, Marc Guevara, Antoine Guion, Jonathan Guth, Risto Hänninen, Kaj Hansen, Ulas Im, Ruud Janssen, Marine Jeoffrion, Mathieu Joly, Luke Jones, Oriol Jorba, Evgeni Kadantsev, Michael Kahnert, Jacek W. Kaminski, Rostislav Kouznetsov, Richard Kranenburg, Jeroen Kuenen, Anne Caroline Lange, Joachim Langner, Victor Lannuque, Francesca Macchia, Astrid Manders, Mihaela Mircea, Agnes Nyiri, Miriam Olid, Carlos Pérez García-Pando, Yuliia Palamarchuk, Antonio Piersanti, Blandine Raux, Miha Razinger, Lennard Robertson, Arjo Segers, Martijn Schaap, Pilvi Siljamo, David Simpson, Mikhail Sofiev, Anders Stangel, Joanna Struzewska, Carles Tena, Renske Timmermans, Thanos Tsikerdekis, Svetlana Tsyro, Svyatoslav Tyuryakov, Anthony Ung, Andreas Uppstu, Alvaro Valdebenito, Peter van Velthoven, Lina Vitali, Zhuyun Ye, Vincent-Henri Peuch, and Laurence Rouïl
Geosci. Model Dev., 18, 6835–6883, https://doi.org/10.5194/gmd-18-6835-2025, https://doi.org/10.5194/gmd-18-6835-2025, 2025
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The Copernicus Atmosphere Monitoring Service – Regional Production delivers daily forecasts, analyses, and reanalyses of air quality in Europe. The service relies on a distributed modelling production by 11 leading European modelling teams following stringent requirements with an operational design that has no equivalent in the world. All the products are free, open, and quality-assured and disseminated with a high level of reliability.
Thomas Drugé, Pierre Nabat, Martine Michou, and Marc Mallet
Atmos. Chem. Phys., 25, 11651–11671, https://doi.org/10.5194/acp-25-11651-2025, https://doi.org/10.5194/acp-25-11651-2025, 2025
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This atmospheric modelling study focuses on the radiative and climatic impacts of coarse-aerosol scattering in the long-wave range. The impact of this process on several climate variables is studied, showing, in particular, significant changes in long-wave radiation and daily surface minimum temperature. Other changes in atmospheric fields are also simulated. The findings of this study highlight the importance of incorporating aerosol scattering in the long-wave spectrum in climate models.
Yunqian Zhu, Hideharu Akiyoshi, Valentina Aquila, Elizabeth Asher, Ewa M. Bednarz, Slimane Bekki, Christoph Brühl, Amy H. Butler, Parker Case, Simon Chabrillat, Gabriel Chiodo, Margot Clyne, Peter R. Colarco, Sandip Dhomse, Lola Falletti, Eric Fleming, Ben Johnson, Andrin Jörimann, Mahesh Kovilakam, Gerbrand Koren, Ales Kuchar, Nicolas Lebas, Qing Liang, Cheng-Cheng Liu, Graham Mann, Michael Manyin, Marion Marchand, Olaf Morgenstern, Paul Newman, Luke D. Oman, Freja F. Østerstrøm, Yifeng Peng, David Plummer, Ilaria Quaglia, William Randel, Samuel Rémy, Takashi Sekiya, Stephen Steenrod, Timofei Sukhodolov, Simone Tilmes, Kostas Tsigaridis, Rei Ueyama, Daniele Visioni, Xinyue Wang, Shingo Watanabe, Yousuke Yamashita, Pengfei Yu, Wandi Yu, Jun Zhang, and Zhihong Zhuo
Geosci. Model Dev., 18, 5487–5512, https://doi.org/10.5194/gmd-18-5487-2025, https://doi.org/10.5194/gmd-18-5487-2025, 2025
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To understand the climate impact of the 2022 Hunga volcanic eruption, we developed a climate model–observation comparison project. The paper describes the protocols and models that participate in the experiments. We designed several experiments to achieve our goals of this activity: (1) to evaluate the climate model performance and (2) to understand the Earth system responses to this eruption.
Anam M. Khan, Olivia E. Clifton, Jesse O. Bash, Sam Bland, Nathan Booth, Philip Cheung, Lisa Emberson, Johannes Flemming, Erick Fredj, Stefano Galmarini, Laurens Ganzeveld, Orestis Gazetas, Ignacio Goded, Christian Hogrefe, Christopher D. Holmes, László Horváth, Vincent Huijnen, Qian Li, Paul A. Makar, Ivan Mammarella, Giovanni Manca, J. William Munger, Juan L. Pérez-Camanyo, Jonathan Pleim, Limei Ran, Roberto San Jose, Donna Schwede, Sam J. Silva, Ralf Staebler, Shihan Sun, Amos P. K. Tai, Eran Tas, Timo Vesala, Tamás Weidinger, Zhiyong Wu, Leiming Zhang, and Paul C. Stoy
Atmos. Chem. Phys., 25, 8613–8635, https://doi.org/10.5194/acp-25-8613-2025, https://doi.org/10.5194/acp-25-8613-2025, 2025
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Vegetation removes tropospheric ozone through stomatal uptake, and accurately modeling the stomatal uptake of ozone is important for modeling dry deposition and air quality. We evaluated the stomatal component of ozone dry deposition modeled by atmospheric chemistry models at six sites. We find that models and observation-based estimates agree at times during the growing season at all sites, but some models overestimated the stomatal component during the dry summers at a seasonally dry site.
Matthieu Dabrowski, José Mennesson, Jérôme Riedi, Chaabane Djeraba, and Pierre Nabat
Geosci. Model Dev., 18, 3707–3733, https://doi.org/10.5194/gmd-18-3707-2025, https://doi.org/10.5194/gmd-18-3707-2025, 2025
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This work focuses on the prediction of aerosol concentration values at the ground level, which are a strong indicator of air quality, using artificial neural networks. A study of different variables and their efficiency as inputs for these models is also proposed and reveals that the best results are obtained when using all of them. Comparison between network architectures and information fusion methods allows for the extraction of knowledge on the most efficient methods in the context of this study.
Martin Cussac, Martine Michou, Pierre Nabat, Béatrice Josse, and Sophie Pelletier
EGUsphere, https://doi.org/10.5194/egusphere-2025-1933, https://doi.org/10.5194/egusphere-2025-1933, 2025
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This study evaluates three chemistry schemes of varying complexity, one mainly stratospheric and two tropospheric-stratospheric, in the latest version of the climate model ARPEGE-Climat. Stratospheric ozone and water vapour are better represented. Despite issues with carbon monoxide in one scheme and with winter nitrogen species in the other, tropospheric ozone is overall realistically simulated. These modelling evolutions strengthen future research on chemistry-climate interactions.
Takashi Sekiya, Emanuele Emili, Kazuyuki Miyazaki, Antje Inness, Zhen Qu, R. Bradley Pierce, Dylan Jones, Helen Worden, William Y. Y. Cheng, Vincent Huijnen, and Gerbrand Koren
Atmos. Chem. Phys., 25, 2243–2268, https://doi.org/10.5194/acp-25-2243-2025, https://doi.org/10.5194/acp-25-2243-2025, 2025
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Five global chemical reanalysis datasets were used to assess the relative impacts of assimilating satellite ozone and its precursor measurements on tropospheric ozone analyses for 2010. The multiple reanalysis system comparison allows an evaluation of the dependency of the impacts on different reanalysis systems. The results suggested the importance of satellite ozone and its precursor measurements for improving ozone analysis in the whole troposphere, with varying magnitudes among the systems.
Mariya Petrenko, Ralph Kahn, Mian Chin, Susanne E. Bauer, Tommi Bergman, Huisheng Bian, Gabriele Curci, Ben Johnson, Johannes W. Kaiser, Zak Kipling, Harri Kokkola, Xiaohong Liu, Keren Mezuman, Tero Mielonen, Gunnar Myhre, Xiaohua Pan, Anna Protonotariou, Samuel Remy, Ragnhild Bieltvedt Skeie, Philip Stier, Toshihiko Takemura, Kostas Tsigaridis, Hailong Wang, Duncan Watson-Parris, and Kai Zhang
Atmos. Chem. Phys., 25, 1545–1567, https://doi.org/10.5194/acp-25-1545-2025, https://doi.org/10.5194/acp-25-1545-2025, 2025
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We compared smoke plume simulations from 11 global models to each other and to satellite smoke amount observations aimed at constraining smoke source strength. In regions where plumes are thick and background aerosol is low, models and satellites compare well. However, the input emission inventory tends to underestimate in many places, and particle property and loss rate assumptions vary enormously among models, causing uncertainties that require systematic in situ measurements to resolve.
Gabriel Chesnoiu, Isabelle Chiapello, Nicolas Ferlay, Pierre Nabat, Marc Mallet, and Véronique Riffault
Atmos. Chem. Phys., 25, 1307–1331, https://doi.org/10.5194/acp-25-1307-2025, https://doi.org/10.5194/acp-25-1307-2025, 2025
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The ALADIN regional climate model at 12.5 km resolution allows us to study the evolution of surface solar radiation (SSR) and key associated atmospheric parameters. Over northern France and Benelux, influenced by anthropogenic aerosols and cloudy conditions, regional evaluation of recent hindcast simulations shows satisfying results and high spatial variability. Future SSR evolution by the end of the century for two contrasting CMIP6 scenarios highlights large decreases in SSR for SSP3-7.0.
Marc Mallet, Aurore Voldoire, Fabien Solmon, Pierre Nabat, Thomas Drugé, and Romain Roehrig
Atmos. Chem. Phys., 24, 12509–12535, https://doi.org/10.5194/acp-24-12509-2024, https://doi.org/10.5194/acp-24-12509-2024, 2024
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This study investigates the interactions between smoke aerosols and climate in tropical Africa using a coupled ocean–atmosphere–aerosol climate model. The work shows that smoke plumes have a significant impact by increasing the low-cloud fraction, decreasing the ocean and continental surface temperature and reducing the precipitation of coastal western Africa. It also highlights the role of the ocean temperature response and its feedbacks for the September–November season.
Samuel Rémy, Swen Metzger, Vincent Huijnen, Jason E. Williams, and Johannes Flemming
Geosci. Model Dev., 17, 7539–7567, https://doi.org/10.5194/gmd-17-7539-2024, https://doi.org/10.5194/gmd-17-7539-2024, 2024
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In this paper we describe the development of the future operational cycle 49R1 of the IFS-COMPO system, used for operational forecasts of atmospheric composition in the CAMS project, and focus on the implementation of the thermodynamical model EQSAM4Clim version 12. The implementation of EQSAM4Clim significantly improves the simulated secondary inorganic aerosol surface concentration. The new aerosol and precipitation acidity diagnostics showed good agreement against observational datasets.
Jorge E. Pachón, Mariel A. Opazo, Pablo Lichtig, Nicolas Huneeus, Idir Bouarar, Guy Brasseur, Cathy W. Y. Li, Johannes Flemming, Laurent Menut, Camilo Menares, Laura Gallardo, Michael Gauss, Mikhail Sofiev, Rostislav Kouznetsov, Julia Palamarchuk, Andreas Uppstu, Laura Dawidowski, Nestor Y. Rojas, María de Fátima Andrade, Mario E. Gavidia-Calderón, Alejandro H. Delgado Peralta, and Daniel Schuch
Geosci. Model Dev., 17, 7467–7512, https://doi.org/10.5194/gmd-17-7467-2024, https://doi.org/10.5194/gmd-17-7467-2024, 2024
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Latin America (LAC) has some of the most populated urban areas in the world, with high levels of air pollution. Air quality management in LAC has been traditionally focused on surveillance and building emission inventories. This study performed the first intercomparison and model evaluation in LAC, with interesting and insightful findings for the region. A multiscale modeling ensemble chain was assembled as a first step towards an air quality forecasting system.
Ana Maria Roxana Petrescu, Glen P. Peters, Richard Engelen, Sander Houweling, Dominik Brunner, Aki Tsuruta, Bradley Matthews, Prabir K. Patra, Dmitry Belikov, Rona L. Thompson, Lena Höglund-Isaksson, Wenxin Zhang, Arjo J. Segers, Giuseppe Etiope, Giancarlo Ciotoli, Philippe Peylin, Frédéric Chevallier, Tuula Aalto, Robbie M. Andrew, David Bastviken, Antoine Berchet, Grégoire Broquet, Giulia Conchedda, Stijn N. C. Dellaert, Hugo Denier van der Gon, Johannes Gütschow, Jean-Matthieu Haussaire, Ronny Lauerwald, Tiina Markkanen, Jacob C. A. van Peet, Isabelle Pison, Pierre Regnier, Espen Solum, Marko Scholze, Maria Tenkanen, Francesco N. Tubiello, Guido R. van der Werf, and John R. Worden
Earth Syst. Sci. Data, 16, 4325–4350, https://doi.org/10.5194/essd-16-4325-2024, https://doi.org/10.5194/essd-16-4325-2024, 2024
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This study provides an overview of data availability from observation- and inventory-based CH4 emission estimates. It systematically compares them and provides recommendations for robust comparisons, aiming to steadily engage more parties in using observational methods to complement their UNFCCC submissions. Anticipating improvements in atmospheric modelling and observations, future developments need to resolve knowledge gaps in both approaches and to better quantify remaining uncertainty.
Henk Eskes, Athanasios Tsikerdekis, Melanie Ades, Mihai Alexe, Anna Carlin Benedictow, Yasmine Bennouna, Lewis Blake, Idir Bouarar, Simon Chabrillat, Richard Engelen, Quentin Errera, Johannes Flemming, Sebastien Garrigues, Jan Griesfeller, Vincent Huijnen, Luka Ilić, Antje Inness, John Kapsomenakis, Zak Kipling, Bavo Langerock, Augustin Mortier, Mark Parrington, Isabelle Pison, Mikko Pitkänen, Samuel Remy, Andreas Richter, Anja Schoenhardt, Michael Schulz, Valerie Thouret, Thorsten Warneke, Christos Zerefos, and Vincent-Henri Peuch
Atmos. Chem. Phys., 24, 9475–9514, https://doi.org/10.5194/acp-24-9475-2024, https://doi.org/10.5194/acp-24-9475-2024, 2024
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The Copernicus Atmosphere Monitoring Service (CAMS) provides global analyses and forecasts of aerosols and trace gases in the atmosphere. On 27 June 2023 a major upgrade, Cy48R1, became operational. Comparisons with in situ, surface remote sensing, aircraft, and balloon and satellite observations show that the new CAMS system is a significant improvement. The results quantify the skill of CAMS to forecast impactful events, such as wildfires, dust storms and air pollution peaks.
Sören Johansson, Michael Höpfner, Felix Friedl-Vallon, Norbert Glatthor, Thomas Gulde, Vincent Huijnen, Anne Kleinert, Erik Kretschmer, Guido Maucher, Tom Neubert, Hans Nordmeyer, Christof Piesch, Peter Preusse, Martin Riese, Björn-Martin Sinnhuber, Jörn Ungermann, Gerald Wetzel, and Wolfgang Woiwode
Atmos. Chem. Phys., 24, 8125–8138, https://doi.org/10.5194/acp-24-8125-2024, https://doi.org/10.5194/acp-24-8125-2024, 2024
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We present airborne infrared limb sounding GLORIA measurements of ammonia (NH3) in the upper troposphere of air masses within the Asian monsoon and of those connected with biomass burning. Comparing CAMS (Copernicus Atmosphere Monitoring Service) model data, we find that the model reproduces the measured enhanced NH3 within the Asian monsoon well but not that within biomass burning plumes, where no enhanced NH3 is measured in the upper troposphere but considerable amounts are simulated by CAMS.
Alkiviadis Kalisoras, Aristeidis K. Georgoulias, Dimitris Akritidis, Robert J. Allen, Vaishali Naik, Chaincy Kuo, Sophie Szopa, Pierre Nabat, Dirk Olivié, Twan van Noije, Philippe Le Sager, David Neubauer, Naga Oshima, Jane Mulcahy, Larry W. Horowitz, and Prodromos Zanis
Atmos. Chem. Phys., 24, 7837–7872, https://doi.org/10.5194/acp-24-7837-2024, https://doi.org/10.5194/acp-24-7837-2024, 2024
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Effective radiative forcing (ERF) is a metric for estimating how human activities and natural agents change the energy flow into and out of the Earth’s climate system. We investigate the anthropogenic aerosol ERF, and we estimate the contribution of individual processes to the total ERF using simulations from Earth system models within the Coupled Model Intercomparison Project Phase 6 (CMIP6). Our findings highlight that aerosol–cloud interactions drive ERF variability during the last 150 years.
Claire L. Ryder, Clément Bézier, Helen F. Dacre, Rory Clarkson, Vassilis Amiridis, Eleni Marinou, Emmanouil Proestakis, Zak Kipling, Angela Benedetti, Mark Parrington, Samuel Rémy, and Mark Vaughan
Nat. Hazards Earth Syst. Sci., 24, 2263–2284, https://doi.org/10.5194/nhess-24-2263-2024, https://doi.org/10.5194/nhess-24-2263-2024, 2024
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Desert dust poses a hazard to aircraft via degradation of engine components. This has financial implications for the aviation industry and results in increased fuel burn with climate impacts. Here we quantify dust ingestion by aircraft engines at airports worldwide. We find Dubai and Delhi in summer are among the dustiest airports, where substantial engine degradation would occur after 1000 flights. Dust ingestion can be reduced by changing take-off times and the altitude of holding patterns.
Sarah Tinorua, Cyrielle Denjean, Pierre Nabat, Véronique Pont, Mathilde Arnaud, Thierry Bourrianne, Maria Dias Alves, and Eric Gardrat
Atmos. Meas. Tech., 17, 3897–3915, https://doi.org/10.5194/amt-17-3897-2024, https://doi.org/10.5194/amt-17-3897-2024, 2024
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The three most widely used techniques for measuring black carbon (BC) have been deployed continuously for 2 years at a French high-altitude research station. Despite a similar temporal variation in the BC load, we found significant biases by up to a factor of 8 between the three instruments. This study raises questions about the relevance of using these instruments for specific background sites, as well as the processing of their data, which can vary according to the atmospheric conditions.
Swen Metzger, Samuel Rémy, Jason E. Williams, Vincent Huijnen, and Johannes Flemming
Geosci. Model Dev., 17, 5009–5021, https://doi.org/10.5194/gmd-17-5009-2024, https://doi.org/10.5194/gmd-17-5009-2024, 2024
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EQSAM4Clim has recently been revised to provide an accurate and efficient method for calculating the acidity of atmospheric particles. It is based on an analytical concept that is sufficiently fast and free of numerical noise, which makes it attractive for air quality forecasting. Version 12 allows the calculation of aerosol composition based on the gas–liquid–solid and the reduced gas–liquid partitioning with the associated water uptake for both cases, including the acidity of the aerosols.
Fangxuan Ren, Jintai Lin, Chenghao Xu, Jamiu A. Adeniran, Jingxu Wang, Randall V. Martin, Aaron van Donkelaar, Melanie S. Hammer, Larry W. Horowitz, Steven T. Turnock, Naga Oshima, Jie Zhang, Susanne Bauer, Kostas Tsigaridis, Øyvind Seland, Pierre Nabat, David Neubauer, Gary Strand, Twan van Noije, Philippe Le Sager, and Toshihiko Takemura
Geosci. Model Dev., 17, 4821–4836, https://doi.org/10.5194/gmd-17-4821-2024, https://doi.org/10.5194/gmd-17-4821-2024, 2024
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We evaluate the performance of 14 CMIP6 ESMs in simulating total PM2.5 and its 5 components over China during 2000–2014. PM2.5 and its components are underestimated in almost all models, except that black carbon (BC) and sulfate are overestimated in two models, respectively. The underestimation is the largest for organic carbon (OC) and the smallest for BC. Models reproduce the observed spatial pattern for OC, sulfate, nitrate and ammonium well, yet the agreement is poorer for BC.
Peng Xian, Jeffrey S. Reid, Melanie Ades, Angela Benedetti, Peter R. Colarco, Arlindo da Silva, Tom F. Eck, Johannes Flemming, Edward J. Hyer, Zak Kipling, Samuel Rémy, Tsuyoshi Thomas Sekiyama, Taichu Tanaka, Keiya Yumimoto, and Jianglong Zhang
Atmos. Chem. Phys., 24, 6385–6411, https://doi.org/10.5194/acp-24-6385-2024, https://doi.org/10.5194/acp-24-6385-2024, 2024
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The study compares and evaluates monthly AOD of four reanalyses (RA) and their consensus (i.e., ensemble mean). The basic verification characteristics of these RA versus both AERONET and MODIS retrievals are presented. The study discusses the strength of each RA and identifies regions where divergence and challenges are prominent. The RA consensus usually performs very well on a global scale in terms of how well it matches the observational data, making it a good choice for various applications.
Adrianus de Laat, Vincent Huijnen, Niels Andela, and Matthias Forkel
EGUsphere, https://doi.org/10.5194/egusphere-2024-732, https://doi.org/10.5194/egusphere-2024-732, 2024
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This study assesses state-of-the art and more advanced and innovative satellite-observation-based (bottom-up) wildfire emission estimates. They are evaluated by comparison with satellite observation of single fire emission plumes. Results indicate that more advanced fire emission estimates – more information – are more realistic but that especially for a limited number of very large fires certain differences remain – for unknown reasons.
Sarah Tinorua, Cyrielle Denjean, Pierre Nabat, Thierry Bourrianne, Véronique Pont, François Gheusi, and Emmanuel Leclerc
Atmos. Chem. Phys., 24, 1801–1824, https://doi.org/10.5194/acp-24-1801-2024, https://doi.org/10.5194/acp-24-1801-2024, 2024
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At a French high-altitude site, where many complex interactions between black carbon (BC), radiation, clouds and snow impact climate, 2 years of refractive BC (rBC) and aerosol optical and microphysical measurements have been made. We observed strong seasonal rBC properties variations, with an enhanced absorption in summer compared to winter. The combination of rBC emission sources, transport pathways, atmospheric dynamics and chemical processes explains the rBC light absorption seasonality.
Zhipeng Qu, David P. Donovan, Howard W. Barker, Jason N. S. Cole, Mark W. Shephard, and Vincent Huijnen
Atmos. Meas. Tech., 16, 4927–4946, https://doi.org/10.5194/amt-16-4927-2023, https://doi.org/10.5194/amt-16-4927-2023, 2023
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The EarthCARE satellite mission Level 2 algorithm development requires realistic 3D cloud and aerosol scenes along the satellite orbits. One of the best ways to produce these scenes is to use a high-resolution numerical weather prediction model to simulate atmospheric conditions at 250 m horizontal resolution. This paper describes the production and validation of three EarthCARE test scenes.
Sebastien Garrigues, Melanie Ades, Samuel Remy, Johannes Flemming, Zak Kipling, Istvan Laszlo, Mark Parrington, Antje Inness, Roberto Ribas, Luke Jones, Richard Engelen, and Vincent-Henri Peuch
Atmos. Chem. Phys., 23, 10473–10487, https://doi.org/10.5194/acp-23-10473-2023, https://doi.org/10.5194/acp-23-10473-2023, 2023
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The Copernicus Atmosphere Monitoring Service (CAMS) provides global monitoring of aerosols using the ECMWF forecast model constrained by the assimilation of satellite aerosol optical depth (AOD). This work aims at evaluating the assimilation of the NOAA VIIRS AOD product in the ECMWF model. It shows that the introduction of VIIRS in the CAMS data assimilation system enhances the accuracy of the aerosol analysis, particularly over Europe and desert and maritime sites.
Olivia E. Clifton, Donna Schwede, Christian Hogrefe, Jesse O. Bash, Sam Bland, Philip Cheung, Mhairi Coyle, Lisa Emberson, Johannes Flemming, Erick Fredj, Stefano Galmarini, Laurens Ganzeveld, Orestis Gazetas, Ignacio Goded, Christopher D. Holmes, László Horváth, Vincent Huijnen, Qian Li, Paul A. Makar, Ivan Mammarella, Giovanni Manca, J. William Munger, Juan L. Pérez-Camanyo, Jonathan Pleim, Limei Ran, Roberto San Jose, Sam J. Silva, Ralf Staebler, Shihan Sun, Amos P. K. Tai, Eran Tas, Timo Vesala, Tamás Weidinger, Zhiyong Wu, and Leiming Zhang
Atmos. Chem. Phys., 23, 9911–9961, https://doi.org/10.5194/acp-23-9911-2023, https://doi.org/10.5194/acp-23-9911-2023, 2023
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A primary sink of air pollutants is dry deposition. Dry deposition estimates differ across the models used to simulate atmospheric chemistry. Here, we introduce an effort to examine dry deposition schemes from atmospheric chemistry models. We provide our approach’s rationale, document the schemes, and describe datasets used to drive and evaluate the schemes. We also launch the analysis of results by evaluating against observations and identifying the processes leading to model–model differences.
Anna Agustí-Panareda, Jérôme Barré, Sébastien Massart, Antje Inness, Ilse Aben, Melanie Ades, Bianca C. Baier, Gianpaolo Balsamo, Tobias Borsdorff, Nicolas Bousserez, Souhail Boussetta, Michael Buchwitz, Luca Cantarello, Cyril Crevoisier, Richard Engelen, Henk Eskes, Johannes Flemming, Sébastien Garrigues, Otto Hasekamp, Vincent Huijnen, Luke Jones, Zak Kipling, Bavo Langerock, Joe McNorton, Nicolas Meilhac, Stefan Noël, Mark Parrington, Vincent-Henri Peuch, Michel Ramonet, Miha Razinger, Maximilian Reuter, Roberto Ribas, Martin Suttie, Colm Sweeney, Jérôme Tarniewicz, and Lianghai Wu
Atmos. Chem. Phys., 23, 3829–3859, https://doi.org/10.5194/acp-23-3829-2023, https://doi.org/10.5194/acp-23-3829-2023, 2023
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We present a global dataset of atmospheric CO2 and CH4, the two most important human-made greenhouse gases, which covers almost 2 decades (2003–2020). It is produced by combining satellite data of CO2 and CH4 with a weather and air composition prediction model, and it has been carefully evaluated against independent observations to ensure validity and point out deficiencies to the user. This dataset can be used for scientific studies in the field of climate change and the global carbon cycle.
John Douros, Henk Eskes, Jos van Geffen, K. Folkert Boersma, Steven Compernolle, Gaia Pinardi, Anne-Marlene Blechschmidt, Vincent-Henri Peuch, Augustin Colette, and Pepijn Veefkind
Geosci. Model Dev., 16, 509–534, https://doi.org/10.5194/gmd-16-509-2023, https://doi.org/10.5194/gmd-16-509-2023, 2023
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We focus on the challenges associated with comparing atmospheric composition models with satellite products such as tropospheric NO2 columns. The aim is to highlight the methodological difficulties and propose sound ways of doing such comparisons. Building on the comparisons, a new satellite product is proposed and made available, which takes advantage of higher-resolution, regional atmospheric modelling to improve estimates of troposheric NO2 columns over Europe.
Stijn Naus, Lucas G. Domingues, Maarten Krol, Ingrid T. Luijkx, Luciana V. Gatti, John B. Miller, Emanuel Gloor, Sourish Basu, Caio Correia, Gerbrand Koren, Helen M. Worden, Johannes Flemming, Gabrielle Pétron, and Wouter Peters
Atmos. Chem. Phys., 22, 14735–14750, https://doi.org/10.5194/acp-22-14735-2022, https://doi.org/10.5194/acp-22-14735-2022, 2022
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We assimilate MOPITT CO satellite data in the TM5-4D-Var inverse modelling framework to estimate Amazon fire CO emissions for 2003–2018. We show that fire emissions have decreased over the analysis period, coincident with a decrease in deforestation rates. However, interannual variations in fire emissions are large, and they correlate strongly with soil moisture. Our results reveal an important role for robust, top-down fire CO emissions in quantifying and attributing Amazon fire intensity.
Sebastien Garrigues, Samuel Remy, Julien Chimot, Melanie Ades, Antje Inness, Johannes Flemming, Zak Kipling, Istvan Laszlo, Angela Benedetti, Roberto Ribas, Soheila Jafariserajehlou, Bertrand Fougnie, Shobha Kondragunta, Richard Engelen, Vincent-Henri Peuch, Mark Parrington, Nicolas Bousserez, Margarita Vazquez Navarro, and Anna Agusti-Panareda
Atmos. Chem. Phys., 22, 14657–14692, https://doi.org/10.5194/acp-22-14657-2022, https://doi.org/10.5194/acp-22-14657-2022, 2022
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The Copernicus Atmosphere Monitoring Service (CAMS) provides global monitoring of aerosols using the ECMWF forecast model constrained by the assimilation of satellite aerosol optical depth (AOD). This work aims at evaluating two new satellite AODs to enhance the CAMS aerosol global forecast. It highlights the spatial and temporal differences between the satellite AOD products at the model spatial resolution, which is essential information to design multi-satellite AOD data assimilation schemes.
Antje Inness, Ilse Aben, Melanie Ades, Tobias Borsdorff, Johannes Flemming, Luke Jones, Jochen Landgraf, Bavo Langerock, Philippe Nedelec, Mark Parrington, and Roberto Ribas
Atmos. Chem. Phys., 22, 14355–14376, https://doi.org/10.5194/acp-22-14355-2022, https://doi.org/10.5194/acp-22-14355-2022, 2022
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The Copernicus Atmosphere Monitoring Service (CAMS) provides daily global air quality forecasts to users worldwide. One of the species of interest is carbon monoxide (CO), an important trace gas in the atmosphere with anthropogenic and natural sources, produced by incomplete combustion, for example, by wildfires. This paper looks at how well CAMS can model CO in the atmosphere and shows that the fields can be improved when blending CO data from the TROPOMI instrument with the CAMS model.
Thomas Drugé, Pierre Nabat, Marc Mallet, Martine Michou, Samuel Rémy, and Oleg Dubovik
Atmos. Chem. Phys., 22, 12167–12205, https://doi.org/10.5194/acp-22-12167-2022, https://doi.org/10.5194/acp-22-12167-2022, 2022
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This study presents the implementation of brown carbon in the atmospheric component of the CNRM global climate model and particularly in its aerosol scheme TACTIC. Several simulations were carried out with this climate model, over the period 2000–2014, to evaluate the model by comparison with different reference datasets (PARASOL-GRASP, OMI-OMAERUVd, MACv2, FMI_SAT, AERONET) and to analyze the brown carbon radiative and climatic effects.
Sini Isokääntä, Paul Kim, Santtu Mikkonen, Thomas Kühn, Harri Kokkola, Taina Yli-Juuti, Liine Heikkinen, Krista Luoma, Tuukka Petäjä, Zak Kipling, Daniel Partridge, and Annele Virtanen
Atmos. Chem. Phys., 22, 11823–11843, https://doi.org/10.5194/acp-22-11823-2022, https://doi.org/10.5194/acp-22-11823-2022, 2022
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This research employs air mass history analysis and observations to study how clouds and precipitation affect atmospheric aerosols during transport to a boreal forest site. The mass concentrations of studied chemical species showed exponential decrease as a function of accumulated rain along the air mass route. Our analysis revealed in-cloud sulfate formation, while no major changes in organic mass were seen. Most of the in-cloud-formed sulfate could be assigned to particle sizes above 200 nm.
Qirui Zhong, Nick Schutgens, Guido van der Werf, Twan van Noije, Kostas Tsigaridis, Susanne E. Bauer, Tero Mielonen, Alf Kirkevåg, Øyvind Seland, Harri Kokkola, Ramiro Checa-Garcia, David Neubauer, Zak Kipling, Hitoshi Matsui, Paul Ginoux, Toshihiko Takemura, Philippe Le Sager, Samuel Rémy, Huisheng Bian, Mian Chin, Kai Zhang, Jialei Zhu, Svetlana G. Tsyro, Gabriele Curci, Anna Protonotariou, Ben Johnson, Joyce E. Penner, Nicolas Bellouin, Ragnhild B. Skeie, and Gunnar Myhre
Atmos. Chem. Phys., 22, 11009–11032, https://doi.org/10.5194/acp-22-11009-2022, https://doi.org/10.5194/acp-22-11009-2022, 2022
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Aerosol optical depth (AOD) errors for biomass burning aerosol (BBA) are evaluated in 18 global models against satellite datasets. Notwithstanding biases in satellite products, they allow model evaluations. We observe large and diverse model biases due to errors in BBA. Further interpretations of AOD diversities suggest large biases exist in key processes for BBA which require better constraining. These results can contribute to further model improvement and development.
Vincent Huijnen, Philippe Le Sager, Marcus O. Köhler, Glenn Carver, Samuel Rémy, Johannes Flemming, Simon Chabrillat, Quentin Errera, and Twan van Noije
Geosci. Model Dev., 15, 6221–6241, https://doi.org/10.5194/gmd-15-6221-2022, https://doi.org/10.5194/gmd-15-6221-2022, 2022
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We report on the first implementation of atmospheric chemistry and aerosol as part of the OpenIFS model, based on the CAMS global model. We give an overview of the model and evaluate two reference model configurations, with and without the stratospheric chemistry extension, against a variety of observational datasets. This OpenIFS version with atmospheric composition components is open to the scientific user community under a standard OpenIFS license.
Peng Xian, Jianglong Zhang, Norm T. O'Neill, Travis D. Toth, Blake Sorenson, Peter R. Colarco, Zak Kipling, Edward J. Hyer, James R. Campbell, Jeffrey S. Reid, and Keyvan Ranjbar
Atmos. Chem. Phys., 22, 9915–9947, https://doi.org/10.5194/acp-22-9915-2022, https://doi.org/10.5194/acp-22-9915-2022, 2022
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The study provides baseline Arctic spring and summertime aerosol optical depth climatology, trend, and extreme event statistics from 2003 to 2019 using a combination of aerosol reanalyses, remote sensing, and ground observations. Biomass burning smoke has an overwhelming contribution to black carbon (an efficient climate forcer) compared to anthropogenic sources. Burning's large interannual variability and increasing summer trend have important implications for the Arctic climate.
Jason E. Williams, Vincent Huijnen, Idir Bouarar, Mehdi Meziane, Timo Schreurs, Sophie Pelletier, Virginie Marécal, Beatrice Josse, and Johannes Flemming
Geosci. Model Dev., 15, 4657–4687, https://doi.org/10.5194/gmd-15-4657-2022, https://doi.org/10.5194/gmd-15-4657-2022, 2022
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The global CAMS air quality model is used for providing tropospheric ozone information to end users. This paper updates the chemical mechanism employed (CBA) and compares it against two other mechanisms (MOCAGE, MOZART) and a multi-decadal dataset based on a previous version of CBA. We perform extensive validation for the US using multiple surface and aircraft datasets, providing an assessment of biases and the extent of correlation across different seasons during 2014.
Marc Guevara, Hervé Petetin, Oriol Jorba, Hugo Denier van der Gon, Jeroen Kuenen, Ingrid Super, Jukka-Pekka Jalkanen, Elisa Majamäki, Lasse Johansson, Vincent-Henri Peuch, and Carlos Pérez García-Pando
Earth Syst. Sci. Data, 14, 2521–2552, https://doi.org/10.5194/essd-14-2521-2022, https://doi.org/10.5194/essd-14-2521-2022, 2022
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To control the spread of the COVID-19 disease, European governments implemented mobility restriction measures that resulted in an unprecedented drop in anthropogenic emissions. This work presents a dataset of emission adjustment factors that allows quantifying changes in 2020 European primary emissions per country and pollutant sector at the daily scale. The resulting dataset can be used as input in modelling studies aiming at quantifying the impact of COVID-19 on air quality levels.
Dimitris Akritidis, Andrea Pozzer, Johannes Flemming, Antje Inness, Philippe Nédélec, and Prodromos Zanis
Atmos. Chem. Phys., 22, 6275–6289, https://doi.org/10.5194/acp-22-6275-2022, https://doi.org/10.5194/acp-22-6275-2022, 2022
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We perform a process-oriented evaluation of Copernicus Atmosphere Monitoring Service (CAMS) reanalysis (CAMSRA) O3 over Europe using WOUDC (World Ozone and Ultraviolet Radiation Data Centre) ozonesondes and IAGOS (In-service Aircraft for a Global Observing System) aircraft measurements. Chemical data assimilation assists CAMSRA to reproduce the observed O3 increases in the troposphere during the examined folding events, but it mostly results in O3 overestimation in the upper troposphere.
Joe McNorton, Nicolas Bousserez, Anna Agustí-Panareda, Gianpaolo Balsamo, Luca Cantarello, Richard Engelen, Vincent Huijnen, Antje Inness, Zak Kipling, Mark Parrington, and Roberto Ribas
Atmos. Chem. Phys., 22, 5961–5981, https://doi.org/10.5194/acp-22-5961-2022, https://doi.org/10.5194/acp-22-5961-2022, 2022
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Concentrations of atmospheric methane continue to grow, in recent years at an increasing rate, for unknown reasons. Using newly available satellite observations and a state-of-the-art weather prediction model we perform global estimates of emissions from hotspots at high resolution. Results show that the system can accurately report on biases in national inventories and is used to conclude that the early COVID-19 slowdown period (March–June 2020) had little impact on global methane emissions.
Simone Tilmes, Daniele Visioni, Andy Jones, James Haywood, Roland Séférian, Pierre Nabat, Olivier Boucher, Ewa Monica Bednarz, and Ulrike Niemeier
Atmos. Chem. Phys., 22, 4557–4579, https://doi.org/10.5194/acp-22-4557-2022, https://doi.org/10.5194/acp-22-4557-2022, 2022
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This study assesses the impacts of climate interventions, using stratospheric sulfate aerosol and solar dimming on stratospheric ozone, based on three Earth system models with interactive stratospheric chemistry. The climate interventions have been applied to a high emission (baseline) scenario in order to reach global surface temperatures of a medium emission scenario. We find significant increases and decreases in total column ozone, depending on regions and seasons.
Beatriz M. Monge-Sanz, Alessio Bozzo, Nicholas Byrne, Martyn P. Chipperfield, Michail Diamantakis, Johannes Flemming, Lesley J. Gray, Robin J. Hogan, Luke Jones, Linus Magnusson, Inna Polichtchouk, Theodore G. Shepherd, Nils Wedi, and Antje Weisheimer
Atmos. Chem. Phys., 22, 4277–4302, https://doi.org/10.5194/acp-22-4277-2022, https://doi.org/10.5194/acp-22-4277-2022, 2022
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The stratosphere is emerging as one of the keys to improve tropospheric weather and climate predictions. This study provides evidence of the role the stratospheric ozone layer plays in improving weather predictions at different timescales. Using a new ozone modelling approach suitable for high-resolution global models that provide operational forecasts from days to seasons, we find significant improvements in stratospheric meteorological fields and stratosphere–troposphere coupling.
Andy Jones, Jim M. Haywood, Adam A. Scaife, Olivier Boucher, Matthew Henry, Ben Kravitz, Thibaut Lurton, Pierre Nabat, Ulrike Niemeier, Roland Séférian, Simone Tilmes, and Daniele Visioni
Atmos. Chem. Phys., 22, 2999–3016, https://doi.org/10.5194/acp-22-2999-2022, https://doi.org/10.5194/acp-22-2999-2022, 2022
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Simulations by six Earth-system models of geoengineering by introducing sulfuric acid aerosols into the tropical stratosphere are compared. A robust impact on the northern wintertime North Atlantic Oscillation is found, exacerbating precipitation reduction over parts of southern Europe. In contrast, the models show no consistency with regard to impacts on the Quasi-Biennial Oscillation, although results do indicate a risk that the oscillation could become locked into a permanent westerly phase.
Antje Inness, Melanie Ades, Dimitris Balis, Dmitry Efremenko, Johannes Flemming, Pascal Hedelt, Maria-Elissavet Koukouli, Diego Loyola, and Roberto Ribas
Geosci. Model Dev., 15, 971–994, https://doi.org/10.5194/gmd-15-971-2022, https://doi.org/10.5194/gmd-15-971-2022, 2022
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This paper describes the way that the Copernicus Atmosphere Monitoring Service (CAMS) produces forecasts of volcanic SO2. These forecasts are provided routinely every day. They are created by blending SO2 data from satellite instruments (TROPOMI and GOME-2) with the CAMS model. We show that the quality of the CAMS SO2 forecasts can be improved if additional information about the height of volcanic plumes is provided in the satellite data.
Sarah J. Doherty, Pablo E. Saide, Paquita Zuidema, Yohei Shinozuka, Gonzalo A. Ferrada, Hamish Gordon, Marc Mallet, Kerry Meyer, David Painemal, Steven G. Howell, Steffen Freitag, Amie Dobracki, James R. Podolske, Sharon P. Burton, Richard A. Ferrare, Calvin Howes, Pierre Nabat, Gregory R. Carmichael, Arlindo da Silva, Kristina Pistone, Ian Chang, Lan Gao, Robert Wood, and Jens Redemann
Atmos. Chem. Phys., 22, 1–46, https://doi.org/10.5194/acp-22-1-2022, https://doi.org/10.5194/acp-22-1-2022, 2022
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Between July and October, biomass burning smoke is advected over the southeastern Atlantic Ocean, leading to climate forcing. Model calculations of forcing by this plume vary significantly in both magnitude and sign. This paper compares aerosol and cloud properties observed during three NASA ORACLES field campaigns to the same in four models. It quantifies modeled biases in properties key to aerosol direct radiative forcing and evaluates how these biases propagate to biases in forcing.
Song Liu, Pieter Valks, Gaia Pinardi, Jian Xu, Ka Lok Chan, Athina Argyrouli, Ronny Lutz, Steffen Beirle, Ehsan Khorsandi, Frank Baier, Vincent Huijnen, Alkiviadis Bais, Sebastian Donner, Steffen Dörner, Myrto Gratsea, François Hendrick, Dimitris Karagkiozidis, Kezia Lange, Ankie J. M. Piters, Julia Remmers, Andreas Richter, Michel Van Roozendael, Thomas Wagner, Mark Wenig, and Diego G. Loyola
Atmos. Meas. Tech., 14, 7297–7327, https://doi.org/10.5194/amt-14-7297-2021, https://doi.org/10.5194/amt-14-7297-2021, 2021
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In this work, an improved tropospheric NO2 retrieval algorithm from TROPOMI measurements over Europe is presented. The stratospheric estimation is implemented with correction for the dependency of the stratospheric NO2 on the viewing geometry. The AMF calculation is implemented using improved surface albedo, a priori NO2 profiles, and cloud correction. The improved tropospheric NO2 data show good correlations with ground-based MAX-DOAS measurements.
Margarita Choulga, Greet Janssens-Maenhout, Ingrid Super, Efisio Solazzo, Anna Agusti-Panareda, Gianpaolo Balsamo, Nicolas Bousserez, Monica Crippa, Hugo Denier van der Gon, Richard Engelen, Diego Guizzardi, Jeroen Kuenen, Joe McNorton, Gabriel Oreggioni, and Antoon Visschedijk
Earth Syst. Sci. Data, 13, 5311–5335, https://doi.org/10.5194/essd-13-5311-2021, https://doi.org/10.5194/essd-13-5311-2021, 2021
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People worry that growing man-made carbon dioxide (CO2) concentrations lead to climate change. Global models, use of observations, and datasets can help us better understand behaviour of CO2. Here a tool to compute uncertainty in man-made CO2 sources per country per year and month is presented. An example of all sources separated into seven groups (intensive and average energy, industry, humans, ground and air transport, others) is presented. Results will be used to predict CO2 concentrations.
Hugues Brenot, Nicolas Theys, Lieven Clarisse, Jeroen van Gent, Daniel R. Hurtmans, Sophie Vandenbussche, Nikolaos Papagiannopoulos, Lucia Mona, Timo Virtanen, Andreas Uppstu, Mikhail Sofiev, Luca Bugliaro, Margarita Vázquez-Navarro, Pascal Hedelt, Michelle Maree Parks, Sara Barsotti, Mauro Coltelli, William Moreland, Simona Scollo, Giuseppe Salerno, Delia Arnold-Arias, Marcus Hirtl, Tuomas Peltonen, Juhani Lahtinen, Klaus Sievers, Florian Lipok, Rolf Rüfenacht, Alexander Haefele, Maxime Hervo, Saskia Wagenaar, Wim Som de Cerff, Jos de Laat, Arnoud Apituley, Piet Stammes, Quentin Laffineur, Andy Delcloo, Robertson Lennart, Carl-Herbert Rokitansky, Arturo Vargas, Markus Kerschbaum, Christian Resch, Raimund Zopp, Matthieu Plu, Vincent-Henri Peuch, Michel Van Roozendael, and Gerhard Wotawa
Nat. Hazards Earth Syst. Sci., 21, 3367–3405, https://doi.org/10.5194/nhess-21-3367-2021, https://doi.org/10.5194/nhess-21-3367-2021, 2021
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The purpose of the EUNADICS-AV (European Natural Airborne Disaster Information and Coordination System for Aviation) prototype early warning system (EWS) is to develop the combined use of harmonised data products from satellite, ground-based and in situ instruments to produce alerts of airborne hazards (volcanic, dust, smoke and radionuclide clouds), satisfying the requirement of aviation air traffic management (ATM) stakeholders (https://cordis.europa.eu/project/id/723986).
Anthony C. Jones, Adrian Hill, Samuel Remy, N. Luke Abraham, Mohit Dalvi, Catherine Hardacre, Alan J. Hewitt, Ben Johnson, Jane P. Mulcahy, and Steven T. Turnock
Atmos. Chem. Phys., 21, 15901–15927, https://doi.org/10.5194/acp-21-15901-2021, https://doi.org/10.5194/acp-21-15901-2021, 2021
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Ammonium nitrate is hard to model because it forms and evaporates rapidly. One approach is to relate its equilibrium concentration to temperature, humidity, and the amount of nitric acid and ammonia gases. Using this approach, we limit the rate at which equilibrium is reached using various condensation rates in a climate model. We show that ammonium nitrate concentrations are highly sensitive to the condensation rate. Our results will help improve the representation of nitrate in climate models.
Maria Sand, Bjørn H. Samset, Gunnar Myhre, Jonas Gliß, Susanne E. Bauer, Huisheng Bian, Mian Chin, Ramiro Checa-Garcia, Paul Ginoux, Zak Kipling, Alf Kirkevåg, Harri Kokkola, Philippe Le Sager, Marianne T. Lund, Hitoshi Matsui, Twan van Noije, Dirk J. L. Olivié, Samuel Remy, Michael Schulz, Philip Stier, Camilla W. Stjern, Toshihiko Takemura, Kostas Tsigaridis, Svetlana G. Tsyro, and Duncan Watson-Parris
Atmos. Chem. Phys., 21, 15929–15947, https://doi.org/10.5194/acp-21-15929-2021, https://doi.org/10.5194/acp-21-15929-2021, 2021
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Absorption of shortwave radiation by aerosols can modify precipitation and clouds but is poorly constrained in models. A total of 15 different aerosol models from AeroCom phase III have reported total aerosol absorption, and for the first time, 11 of these models have reported in a consistent experiment the contributions to absorption from black carbon, dust, and organic aerosol. Here, we document the model diversity in aerosol absorption.
Xinxin Ye, Pargoal Arab, Ravan Ahmadov, Eric James, Georg A. Grell, Bradley Pierce, Aditya Kumar, Paul Makar, Jack Chen, Didier Davignon, Greg R. Carmichael, Gonzalo Ferrada, Jeff McQueen, Jianping Huang, Rajesh Kumar, Louisa Emmons, Farren L. Herron-Thorpe, Mark Parrington, Richard Engelen, Vincent-Henri Peuch, Arlindo da Silva, Amber Soja, Emily Gargulinski, Elizabeth Wiggins, Johnathan W. Hair, Marta Fenn, Taylor Shingler, Shobha Kondragunta, Alexei Lyapustin, Yujie Wang, Brent Holben, David M. Giles, and Pablo E. Saide
Atmos. Chem. Phys., 21, 14427–14469, https://doi.org/10.5194/acp-21-14427-2021, https://doi.org/10.5194/acp-21-14427-2021, 2021
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Wildfire smoke has crucial impacts on air quality, while uncertainties in the numerical forecasts remain significant. We present an evaluation of 12 real-time forecasting systems. Comparison of predicted smoke emissions suggests a large spread in magnitudes, with temporal patterns deviating from satellite detections. The performance for AOD and surface PM2.5 and their discrepancies highlighted the role of accurately represented spatiotemporal emission profiles in improving smoke forecasts.
Alex Resovsky, Michel Ramonet, Leonard Rivier, Jerome Tarniewicz, Philippe Ciais, Martin Steinbacher, Ivan Mammarella, Meelis Mölder, Michal Heliasz, Dagmar Kubistin, Matthias Lindauer, Jennifer Müller-Williams, Sebastien Conil, and Richard Engelen
Atmos. Meas. Tech., 14, 6119–6135, https://doi.org/10.5194/amt-14-6119-2021, https://doi.org/10.5194/amt-14-6119-2021, 2021
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We present a technical description of a statistical methodology for extracting synoptic- and seasonal-length anomalies from greenhouse gas time series. The definition of what represents an anomalous signal is somewhat subjective, which we touch on throughout the paper. We show, however, that the method performs reasonably well in extracting portions of time series influenced by significant North Atlantic Oscillation weather episodes and continent-wide terrestrial biospheric aberrations.
Cited articles
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Forecasting global atmospheric CO2, Atmos. Chem. Phys., 14, 11959–11983, https://doi.org/10.5194/acp-14-11959-2014, 2014. a
Agusti-Panareda, A., Diamantakis, M., Bayona, V., Klappenbach, F., and Butz, A.:
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Whitecap coverage from satellite measurements: A first step toward modeling the variability of oceanic whitecaps, J. Geophys. Res., 111, C03017, https://doi.org/10.1029/2005JC003158, 2006. a
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Short summary
This article describes a new version of IFS-AER, the tropospheric aerosol scheme used to provide global aerosol products within the Copernicus Atmosphere Monitoring Service (CAMS) cycle. Several components of the model have been updated, such as the dynamical dust and sea salt aerosol emission schemes. New deposition schemes have also been incorporated but are not yet used operationally. This new version of IFS-AER has been evaluated and shown to have a greater skill than previous versions.
This article describes a new version of IFS-AER, the tropospheric aerosol scheme used to provide...
