Articles | Volume 13, issue 3
https://doi.org/10.5194/gmd-13-977-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/gmd-13-977-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Model description paper
| 
06 Mar 2020
Model description paper |
| 06 Mar 2020
| 06 Mar 2020
Beijing Climate Center Earth System Model version 1 (BCC-ESM1): model description and evaluation of aerosol simulations
Beijing Climate Center, China Meteorological Administration, Beijing, China
Fang Zhang
Beijing Climate Center, China Meteorological Administration, Beijing, China
Jie Zhang
Beijing Climate Center, China Meteorological Administration, Beijing, China
Weihua Jie
Beijing Climate Center, China Meteorological Administration, Beijing, China
Yanwu Zhang
Beijing Climate Center, China Meteorological Administration, Beijing, China
Fanghua Wu
Beijing Climate Center, China Meteorological Administration, Beijing, China
Laurent Li
Beijing Climate Center, China Meteorological Administration, Beijing, China
Laboratoire de Météorologie Dynamique, IPSL, CNRS, Sorbonne
Université, Ecole Normale Supérieure, Ecole Polytechnique, Paris,
France
Jinghui Yan
Beijing Climate Center, China Meteorological Administration, Beijing, China
Xiaohong Liu
Texas A&M University, College Station, TX 77843, USA
Laboratory for Climate and Ocean-Atmosphere Studies, Department of
Atmospheric and Oceanic Sciences, School of Physics, Peking University,
Beijing, China
Haiyue Tan
Laboratory for Climate and Ocean-Atmosphere Studies, Department of
Atmospheric and Oceanic Sciences, School of Physics, Peking University,
Beijing, China
Lin Zhang
Laboratory for Climate and Ocean-Atmosphere Studies, Department of
Atmospheric and Oceanic Sciences, School of Physics, Peking University,
Beijing, China
University of Iowa, Iowa City, IA 52242, USA
National Center for Atmospheric Research, P.O. Box 3000, Boulder,
CO 80307-3000, USA
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This study explores how urban green spaces in Guangzhou influence ozone levels. By using advanced models, we found that natural emissions from these areas can significantly affect air quality. Our results suggest the design and planning of urban green spaces should not only consider aesthetics and social factors but also their environmental impacts on air quality.
Natalie M. Mahowald, Longlei Li, Julius Vira, Marje Prank, Douglas S. Hamilton, Hitoshi Matsui, Ron L. Miller, Louis Lu, Ezgi Akyuz, Daphne Meidan, Peter G. Hess, Heikki Lihavainen, Christine Wiedinmyer, Jenny Hand, Maria Grazia Alaimo, Célia Alves, Andres Alastuey, Paulo Artaxo, Africa Barreto, Francisco Barraza, Silvia Becagli, Giulia Calzolai, Shankararaman Chellam, Ying Chen, Patrick Chuang, David D. Cohen, Cristina Colombi, Evangelia Diapouli, Gaetano Dongarra, Konstantinos Eleftheriadis, Johann Engelbrecht, Corinne Galy-Lacaux, Cassandra Gaston, Dario Gomez, Yenny González Ramos, Roy M. Harrison, Chris Heyes, Barak Herut, Philip Hopke, Christoph Hüglin, Maria Kanakidou, Zsofia Kertesz, Zbigniew Klimont, Katriina Kyllönen, Fabrice Lambert, Xiaohong Liu, Remi Losno, Franco Lucarelli, Willy Maenhaut, Beatrice Marticorena, Randall V. Martin, Nikolaos Mihalopoulos, Yasser Morera-Gomez, Adina Paytan, Joseph Prospero, Sergio Rodríguez, Patricia Smichowski, Daniela Varrica, Brenna Walsh, Crystal Weagle, and Xi Zhao
EGUsphere, https://doi.org/10.5194/egusphere-2024-1617, https://doi.org/10.5194/egusphere-2024-1617, 2024
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Aerosol particles are an important part of the Earth system, but their concentrations are spatially and temporally heterogeneous, as well as variable in size and composition. Here we present a new compilation of PM2.5 and PM10 aerosol observations, focusing on the spatial variability across different observational stations, including composition, and demonstrate a method for comparing the datasets to model output.
Fangxuan Ren, Jintai Lin, Chenghao Xu, Jamiu A. Adeniran, Jingxu Wang, Randall V. Martin, Aaron van Donkelaar, Melanie S. Hammer, Larry W. Horowitz, Steven T. Turnock, Naga Oshima, Jie Zhang, Susanne Bauer, Kostas Tsigaridis, Øyvind Seland, Pierre Nabat, David Neubauer, Gary Strand, Twan van Noije, Philippe Le Sager, and Toshihiko Takemura
Geosci. Model Dev., 17, 4821–4836, https://doi.org/10.5194/gmd-17-4821-2024, https://doi.org/10.5194/gmd-17-4821-2024, 2024
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We evaluate the performance of 14 CMIP6 ESMs in simulating total PM2.5 and its 5 components over China during 2000–2014. PM2.5 and its components are underestimated in almost all models, except that black carbon (BC) and sulfate are overestimated in two models, respectively. The underestimation is the largest for organic carbon (OC) and the smallest for BC. Models reproduce the observed spatial pattern for OC, sulfate, nitrate and ammonium well, yet the agreement is poorer for BC.
Ziming Ke, Qi Tang, Jean-Christoophe Golaz, Xiaohong Liu, and Hailong Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-1612, https://doi.org/10.5194/egusphere-2024-1612, 2024
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By treating volcanic emission interactively, model results improve simulated temperature variability, showing better correlations for 1940–1959 and 1960–1979, and reveals how volcanic activity influences cloud behavior and climate.
Mariya Petrenko, Ralph Kahn, Mian Chin, Susanne E. Bauer, Tommi Bergman, Huisheng Bian, Gabriele Curci, Ben Johnson, Johannes Kaiser, Zak Kipling, Harri Kokkola, Xiaohong Liu, Keren Mezuman, Tero Mielonen, Gunnar Myhre, Xiaohua Pan, Anna Protonotariou, Samuel Remy, Ragnhild Bieltvedt Skeie, Philip Stier, Toshihiko Takemura, Kostas Tsigaridis, Hailong Wang, Duncan Watson-Parris, and Kai Zhang
EGUsphere, https://doi.org/10.5194/egusphere-2024-1487, https://doi.org/10.5194/egusphere-2024-1487, 2024
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We compared smoke plume simulations from 11 global models to each other and to satellite smoke-amount observations, aimed at constraining smoke source strength. In regions where plumes are thick and background aerosol is low, models and satellites compare well. However, the input emission inventory tends to underestimate in many places, and particle property and loss-rate assumptions vary enormously among models, causing uncertainties that require systematic in-situ measurements to resolve.
Hannah Nesser, Daniel J. Jacob, Joannes D. Maasakkers, Alba Lorente, Zichong Chen, Xiao Lu, Lu Shen, Zhen Qu, Melissa P. Sulprizio, Margaux Winter, Shuang Ma, A. Anthony Bloom, John R. Worden, Robert N. Stavins, and Cynthia A. Randles
Atmos. Chem. Phys., 24, 5069–5091, https://doi.org/10.5194/acp-24-5069-2024, https://doi.org/10.5194/acp-24-5069-2024, 2024
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We quantify 2019 methane emissions in the contiguous US (CONUS) at a ≈ 25 km × 25 km resolution using satellite methane observations. We find a 13 % upward correction to the 2023 US Environmental Protection Agency (EPA) Greenhouse Gas Emissions Inventory (GHGI) for 2019, with large corrections to individual states, urban areas, and landfills. This may present a challenge for US climate policies and goals, many of which target significant reductions in methane emissions.
Hao Wang, Xiaohong Liu, Chenglai Wu, and Guangxing Lin
Atmos. Chem. Phys., 24, 3309–3328, https://doi.org/10.5194/acp-24-3309-2024, https://doi.org/10.5194/acp-24-3309-2024, 2024
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We quantified different global- and regional-scale drivers of biogenic volatile organic compound (BVOC) emission trends over the past 20 years. The results show that global greening trends significantly boost BVOC emissions and deforestation reduces BVOC emissions in South America and Southeast Asia. Elevated temperature in Europe and increased soil moisture in East and South Asia enhance BVOC emissions. The results deepen our understanding of long-term BVOC emission trends in hotspots.
Yiming Wang, Haolin Wang, Yujie Qin, Xinqi Xu, Guowen He, Nanxi Liu, Shengjie Miao, Xiao Lu, Haichao Wang, and Shaojia Fan
Atmos. Chem. Phys., 24, 2267–2285, https://doi.org/10.5194/acp-24-2267-2024, https://doi.org/10.5194/acp-24-2267-2024, 2024
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We conducted a vertical measurement of winter PM2.5 using a mobile multi-lidar system in four cities. Combined with the surface PM2.5 data, the ERA5 reanalysis data, and GEOS-Chem simulations during Dec 2018–Feb 2019, we found that transport nocturnal PM2.5 enhancement by subsidence (T-NPES) events widely occurred with high frequencies in plains regions in eastern China but happened less often in basin regions like Xi’an and Chengdu. We propose a conceptual model of the T-NPES events.
Natalie M. Mahowald, Longlei Li, Julius Vira, Marje Prank, Douglas S. Hamilton, Hitoshi Matsui, Ron L. Miller, Louis Lu, Ezgi Akyuz, Daphne Meidan, Peter Hess, Heikki Lihavainen, Christine Wiedinmyer, Jenny Hand, Maria Grazia Alaimo, Célia Alves, Andres Alastuey, Paulo Artaxo, Africa Barreto, Francisco Barraza, Silvia Becagli, Giulia Calzolai, Shankarararman Chellam, Ying Chen, Patrick Chuang, David D. Cohen, Cristina Colombi, Evangelia Diapouli, Gaetano Dongarra, Konstantinos Eleftheriadis, Corinne Galy-Lacaux, Cassandra Gaston, Dario Gomez, Yenny González Ramos, Hannele Hakola, Roy M. Harrison, Chris Heyes, Barak Herut, Philip Hopke, Christoph Hüglin, Maria Kanakidou, Zsofia Kertesz, Zbiginiw Klimont, Katriina Kyllönen, Fabrice Lambert, Xiaohong Liu, Remi Losno, Franco Lucarelli, Willy Maenhaut, Beatrice Marticorena, Randall V. Martin, Nikolaos Mihalopoulos, Yasser Morera-Gomez, Adina Paytan, Joseph Prospero, Sergio Rodríguez, Patricia Smichowski, Daniela Varrica, Brenna Walsh, Crystal Weagle, and Xi Zhao
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-1, https://doi.org/10.5194/essd-2024-1, 2024
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Aerosol particles can interact with incoming solar radiation and outgoing long wave radiation, change cloud properties, affect photochemistry, impact surface air quality, and when deposited impact surface albedo of snow and ice, and modulate carbon dioxide uptake by the land and ocean. Here we present a new compilation of aerosol observations including composition, a methodology for comparing the datasets to model output, and show the implications of these results using one model.
Yinbao Jin, Yiming Liu, Xiao Lu, Xiaoyang Chen, Ao Shen, Haofan Wang, Yinping Cui, Yifei Xu, Siting Li, Jian Liu, Ming Zhang, Yingying Ma, and Qi Fan
Atmos. Chem. Phys., 24, 367–395, https://doi.org/10.5194/acp-24-367-2024, https://doi.org/10.5194/acp-24-367-2024, 2024
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This study aims to address these issues by evaluating eight independent biomass burning (BB) emission inventories (GFED, FINN1.5, FINN2.5 MOS, FINN2.5 MOSVIS, GFAS, FEER, QFED, and IS4FIRES) using the WRF-Chem model and analyzing their impact on aerosol optical properties (AOPs) and direct radiative forcing (DRF) during wildfire events in peninsular Southeast Asia (PSEA) that occurred in March 2019.
Hyerim Kim, Xi Chen, Jun Wang, Zhendong Lu, Meng Zhou, Gregory Carmichael, Sang Seo Park, and Jhoon Kim
EGUsphere, https://doi.org/10.5194/egusphere-2023-3115, https://doi.org/10.5194/egusphere-2023-3115, 2024
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We compare aerosol layer height (ALH) derived from satellite platforms (GEMS, EPIC, TROPOMI). Validation against CALIOP shows high correlation for EPIC and TROPOMI (R > 0.7, overestimation ~0.8 km), while GEMS displays minimal bias (0.1 km) with a lower correlation (R = 0.64). Categorizing GEMS ALH with UVAI ≥ 3 improves agreement. GEMS exhibits a narrower ALH range and lower mean value than TROPOMI and EPIC. Diurnal variation of EPIC and GEMS ALH aligns with the boundary layer development.
Simone Tilmes, Michael J. Mills, Yunqian Zhu, Charles G. Bardeen, Francis Vitt, Pengfei Yu, David Fillmore, Xiaohong Liu, Brian Toon, and Terry Deshler
Geosci. Model Dev., 16, 6087–6125, https://doi.org/10.5194/gmd-16-6087-2023, https://doi.org/10.5194/gmd-16-6087-2023, 2023
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We implemented an alternative aerosol scheme in the high- and low-top model versions of the Community Earth System Model Version 2 (CESM2) with a more detailed description of tropospheric and stratospheric aerosol size distributions than the existing aerosol model. This development enables the comparison of different aerosol schemes with different complexity in the same model framework. It identifies improvements compared to a range of observations in both the troposphere and stratosphere.
Guowen He, Cheng He, Haofan Wang, Xiao Lu, Chenglei Pei, Xiaonuan Qiu, Chenxi Liu, Yiming Wang, Nanxi Liu, Jinpu Zhang, Lei Lei, Yiming Liu, Haichao Wang, Tao Deng, Qi Fan, and Shaojia Fan
Atmos. Chem. Phys., 23, 13107–13124, https://doi.org/10.5194/acp-23-13107-2023, https://doi.org/10.5194/acp-23-13107-2023, 2023
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We analyze nighttime ozone in the lower boundary layer (up to 500 m) from the 2017–2019 measurements at the Canton Tower and the WRF-CMAQ model. We identify a strong ability of the residual layer to store daytime ozone in the convective mixing layer, investigate the chemical and meteorological factors controlling nighttime ozone in the residual layer, and quantify the contribution of nighttime ozone in the residual layer to both the nighttime and the following day’s surface ozone air quality.
Qindan Zhu, Bryan Place, Eva Y. Pfannerstill, Sha Tong, Huanxin Zhang, Jun Wang, Clara M. Nussbaumer, Paul Wooldridge, Benjamin C. Schulze, Caleb Arata, Anthony Bucholtz, John H. Seinfeld, Allen H. Goldstein, and Ronald C. Cohen
Atmos. Chem. Phys., 23, 9669–9683, https://doi.org/10.5194/acp-23-9669-2023, https://doi.org/10.5194/acp-23-9669-2023, 2023
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Nitrogen oxide (NOx) is a hazardous air pollutant, and it is the precursor of short-lived climate forcers like tropospheric ozone and aerosol particles. While NOx emissions from transportation has been strictly regulated, soil NOx emissions are overlooked. We use the airborne flux measurements to observe NOx emissions from highways and urban and cultivated soil land cover types. We show non-negligible soil NOx emissions, which are significantly underestimated in current model simulations.
Haofan Wang, Jiaxin Qiu, Yiming Liu, Qi Fan, Xiao Lu, Yang Zhang, Kai Wu, Ao Shen, Yifei Xu, Yinbao Jin, Yuqi Zhu, Jiayin Sun, and Haolin Wang
EGUsphere, https://doi.org/10.5194/egusphere-2023-1309, https://doi.org/10.5194/egusphere-2023-1309, 2023
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This tool improves existing methods by providing temporal and species allocation modules and enabling emission file generation in advance for any time period. The tool is also capable of vertical plane distribution for high altitude emissions and accurately tracks road-related emissions, an area overlooked by other tools. It utilizes 50 % of the CPU capacity for efficient parallel processing during allocation.
Kaiyue Zhou, Wen Xu, Lin Zhang, Mingrui Ma, Xuejun Liu, and Yu Zhao
Atmos. Chem. Phys., 23, 8531–8551, https://doi.org/10.5194/acp-23-8531-2023, https://doi.org/10.5194/acp-23-8531-2023, 2023
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We developed a dataset of the long-term (2005–2020) variabilities of China’s nitrogen and sulfur deposition, with multiple statistical models that combine available observations and chemistry transport modeling. We demonstrated the strong impact of human activities and national pollution control actions on the spatiotemporal changes in deposition and indicated a relatively small benefit of emission abatement on deposition (and thereby ecological risk) for China compared to Europe and the USA.
Hejun Hu, Haichao Wang, Keding Lu, Jie Wang, Zelong Zheng, Xuezhen Xu, Tianyu Zhai, Xiaorui Chen, Xiao Lu, Wenxing Fu, Xin Li, Limin Zeng, Min Hu, Yuanhang Zhang, and Shaojia Fan
Atmos. Chem. Phys., 23, 8211–8223, https://doi.org/10.5194/acp-23-8211-2023, https://doi.org/10.5194/acp-23-8211-2023, 2023
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Nitrate radical chemistry is critical to the degradation of volatile organic compounds (VOCs) and secondary organic aerosol formation. This work investigated the level, seasonal variation, and trend of nitrate radical reactivity towards volatile organic compounds (kNO3) in Beijing. We show the key role of isoprene and styrene in regulating seasonal variation in kNO3 and rebuild a long-term record of kNO3 based on the reported VOC measurements.
Daniel J. Varon, Daniel J. Jacob, Benjamin Hmiel, Ritesh Gautam, David R. Lyon, Mark Omara, Melissa Sulprizio, Lu Shen, Drew Pendergrass, Hannah Nesser, Zhen Qu, Zachary R. Barkley, Natasha L. Miles, Scott J. Richardson, Kenneth J. Davis, Sudhanshu Pandey, Xiao Lu, Alba Lorente, Tobias Borsdorff, Joannes D. Maasakkers, and Ilse Aben
Atmos. Chem. Phys., 23, 7503–7520, https://doi.org/10.5194/acp-23-7503-2023, https://doi.org/10.5194/acp-23-7503-2023, 2023
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We use TROPOMI satellite observations to quantify weekly methane emissions from the US Permian oil and gas basin from May 2018 to October 2020. We find that Permian emissions are highly variable, with diverse economic and activity drivers. The most important drivers during our study period were new well development and natural gas price. Permian methane intensity averaged 4.6 % and decreased by 1 % per year.
Ruijun Dang, Daniel J. Jacob, Viral Shah, Sebastian D. Eastham, Thibaud M. Fritz, Loretta J. Mickley, Tianjia Liu, Yi Wang, and Jun Wang
Atmos. Chem. Phys., 23, 6271–6284, https://doi.org/10.5194/acp-23-6271-2023, https://doi.org/10.5194/acp-23-6271-2023, 2023
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We use the GEOS-Chem model to better understand the magnitude and trend in free tropospheric NO2 over the contiguous US. Model underestimate of background NO2 is largely corrected by considering aerosol nitrate photolysis. Increase in aircraft emissions affects satellite retrievals by altering the NO2 shape factor, and this effect is expected to increase in future. We show the importance of properly accounting for the free tropospheric background in interpreting NO2 observations from space.
Zichong Chen, Daniel J. Jacob, Ritesh Gautam, Mark Omara, Robert N. Stavins, Robert C. Stowe, Hannah Nesser, Melissa P. Sulprizio, Alba Lorente, Daniel J. Varon, Xiao Lu, Lu Shen, Zhen Qu, Drew C. Pendergrass, and Sarah Hancock
Atmos. Chem. Phys., 23, 5945–5967, https://doi.org/10.5194/acp-23-5945-2023, https://doi.org/10.5194/acp-23-5945-2023, 2023
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We quantify methane emissions from individual countries in the Middle East and North Africa by inverse analysis of 2019 TROPOMI satellite observations of atmospheric methane. We show that the ability to simply relate oil/gas emissions to activity metrics is compromised by stochastic nature of local infrastructure and management practices. We find that the industry target for oil/gas methane intensity is achievable through associated gas capture, modern infrastructure, and centralized operations.
Laura C. Jackson, Eduardo Alastrué de Asenjo, Katinka Bellomo, Gokhan Danabasoglu, Helmuth Haak, Aixue Hu, Johann Jungclaus, Warren Lee, Virna L. Meccia, Oleg Saenko, Andrew Shao, and Didier Swingedouw
Geosci. Model Dev., 16, 1975–1995, https://doi.org/10.5194/gmd-16-1975-2023, https://doi.org/10.5194/gmd-16-1975-2023, 2023
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The Atlantic meridional overturning circulation (AMOC) has an important impact on the climate. There are theories that freshening of the ocean might cause the AMOC to cross a tipping point (TP) beyond which recovery is difficult; however, it is unclear whether TPs exist in global climate models. Here, we outline a set of experiments designed to explore AMOC tipping points and sensitivity to additional freshwater input as part of the North Atlantic Hosing Model Intercomparison Project (NAHosMIP).
Di Wang, Lide Tian, Camille Risi, Xuejie Wang, Jiangpeng Cui, Gabriel J. Bowen, Kei Yoshimura, Zhongwang Wei, and Laurent Z. X. Li
Atmos. Chem. Phys., 23, 3409–3433, https://doi.org/10.5194/acp-23-3409-2023, https://doi.org/10.5194/acp-23-3409-2023, 2023
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To better understand the spatial and temporal distribution of vapor isotopes, we present two vehicle-based spatially continuous snapshots of the near-surface vapor isotopes in China during the pre-monsoon and monsoon periods. These observations are explained well by different moisture sources and processes along the air mass trajectories. Our results suggest that proxy records need to be interpreted in the context of regional systems and sources of moisture.
Jing Wei, Zhanqing Li, Jun Wang, Can Li, Pawan Gupta, and Maureen Cribb
Atmos. Chem. Phys., 23, 1511–1532, https://doi.org/10.5194/acp-23-1511-2023, https://doi.org/10.5194/acp-23-1511-2023, 2023
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This study estimated the daily seamless 10 km ambient gaseous pollutants (NO2, SO2, and CO) across China using machine learning with extensive input variables measured on monitors, satellites, and models. Our dataset yields a high data quality via cross-validation at varying spatiotemporal scales and outperforms most previous related studies, making it most helpful to future (especially short-term) air pollution and environmental health-related studies.
Yuan Zhang, Devaraju Narayanappa, Philippe Ciais, Wei Li, Daniel Goll, Nicolas Vuichard, Martin G. De Kauwe, Laurent Li, and Fabienne Maignan
Geosci. Model Dev., 15, 9111–9125, https://doi.org/10.5194/gmd-15-9111-2022, https://doi.org/10.5194/gmd-15-9111-2022, 2022
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There are a few studies to examine if current models correctly represented the complex processes of transpiration. Here, we use a coefficient Ω, which indicates if transpiration is mainly controlled by vegetation processes or by turbulence, to evaluate the ORCHIDEE model. We found a good performance of ORCHIDEE, but due to compensation of biases in different processes, we also identified how different factors control Ω and where the model is wrong. Our method is generic to evaluate other models.
Cheng He, Xiao Lu, Haolin Wang, Haichao Wang, Yan Li, Guowen He, Yuanping He, Yurun Wang, Youlang Zhang, Yiming Liu, Qi Fan, and Shaojia Fan
Atmos. Chem. Phys., 22, 15243–15261, https://doi.org/10.5194/acp-22-15243-2022, https://doi.org/10.5194/acp-22-15243-2022, 2022
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We report that nocturnal ozone enhancement (NOE) events are observed at a high annual frequency of 41 % over 800 sites in China in 2014–2019 (about 50 % higher than that over Europe or the US). High daytime ozone provides a rich ozone source in the nighttime residual layer, determining the overall high frequency of NOE events in China, and enhanced atmospheric mixing then triggers NOE events by allowing the ozone-rich air in the residual layer to be mixed into the nighttime boundary layer.
Longlei Li, Natalie M. Mahowald, Jasper F. Kok, Xiaohong Liu, Mingxuan Wu, Danny M. Leung, Douglas S. Hamilton, Louisa K. Emmons, Yue Huang, Neil Sexton, Jun Meng, and Jessica Wan
Geosci. Model Dev., 15, 8181–8219, https://doi.org/10.5194/gmd-15-8181-2022, https://doi.org/10.5194/gmd-15-8181-2022, 2022
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This study advances mineral dust parameterizations in the Community Atmospheric Model (CAM; version 6.1). Efforts include 1) incorporating a more physically based dust emission scheme; 2) updating the dry deposition scheme; and 3) revising the gravitational settling velocity to account for dust asphericity. Substantial improvements achieved with these updates can help accurately quantify dust–climate interactions using CAM, such as the dust-radiation and dust–cloud interactions.
Gonzalo A. Ferrada, Meng Zhou, Jun Wang, Alexei Lyapustin, Yujie Wang, Saulo R. Freitas, and Gregory R. Carmichael
Geosci. Model Dev., 15, 8085–8109, https://doi.org/10.5194/gmd-15-8085-2022, https://doi.org/10.5194/gmd-15-8085-2022, 2022
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The smoke from fires is composed of different compounds that interact with the atmosphere and can create poor air-quality episodes. Here, we present a new fire inventory based on satellite observations from the Visible Infrared Imaging Radiometer Suite (VIIRS). We named this inventory the VIIRS-based Fire Emission Inventory (VFEI). Advantages of VFEI are its high resolution (~500 m) and that it provides information for many species. VFEI is publicly available and has provided data since 2012.
Haolin Wang, Xiao Lu, Daniel J. Jacob, Owen R. Cooper, Kai-Lan Chang, Ke Li, Meng Gao, Yiming Liu, Bosi Sheng, Kai Wu, Tongwen Wu, Jie Zhang, Bastien Sauvage, Philippe Nédélec, Romain Blot, and Shaojia Fan
Atmos. Chem. Phys., 22, 13753–13782, https://doi.org/10.5194/acp-22-13753-2022, https://doi.org/10.5194/acp-22-13753-2022, 2022
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We report significant global tropospheric ozone increases in 1995–2017 based on extensive aircraft and ozonesonde observations. Using GEOS-Chem (Goddard Earth Observing System chemistry model) multi-decadal global simulations, we find that changes in global anthropogenic emissions, in particular the rapid increases in aircraft emissions, contribute significantly to the increases in tropospheric ozone and resulting radiative impact.
Lu Shen, Ritesh Gautam, Mark Omara, Daniel Zavala-Araiza, Joannes D. Maasakkers, Tia R. Scarpelli, Alba Lorente, David Lyon, Jianxiong Sheng, Daniel J. Varon, Hannah Nesser, Zhen Qu, Xiao Lu, Melissa P. Sulprizio, Steven P. Hamburg, and Daniel J. Jacob
Atmos. Chem. Phys., 22, 11203–11215, https://doi.org/10.5194/acp-22-11203-2022, https://doi.org/10.5194/acp-22-11203-2022, 2022
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We use 22 months of TROPOMI satellite observations to quantity methane emissions from the oil (O) and natural gas (G) sector in the US and Canada at the scale of both individual basins as well as country-wide aggregates. We find that O/G-related methane emissions are underestimated in these inventories by 80 % for the US and 40 % for Canada, and 70 % of the underestimate in the US is from five O/G basins, including Permian, Haynesville, Anadarko, Eagle Ford, and Barnett.
Zichong Chen, Daniel J. Jacob, Hannah Nesser, Melissa P. Sulprizio, Alba Lorente, Daniel J. Varon, Xiao Lu, Lu Shen, Zhen Qu, Elise Penn, and Xueying Yu
Atmos. Chem. Phys., 22, 10809–10826, https://doi.org/10.5194/acp-22-10809-2022, https://doi.org/10.5194/acp-22-10809-2022, 2022
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We quantify methane emissions in China and contributions from different sectors by inverse analysis of 2019 TROPOMI satellite observations of atmospheric methane. We find that anthropogenic methane emissions for China are underestimated in the national inventory. Our estimate of emissions indicates a small life-cycle loss rate, implying net climate benefits from the current
coal-to-gasenergy transition in China. However, this small loss rate can be misleading given China's high gas imports.
Daniel J. Varon, Daniel J. Jacob, Melissa Sulprizio, Lucas A. Estrada, William B. Downs, Lu Shen, Sarah E. Hancock, Hannah Nesser, Zhen Qu, Elise Penn, Zichong Chen, Xiao Lu, Alba Lorente, Ashutosh Tewari, and Cynthia A. Randles
Geosci. Model Dev., 15, 5787–5805, https://doi.org/10.5194/gmd-15-5787-2022, https://doi.org/10.5194/gmd-15-5787-2022, 2022
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Reducing atmospheric methane emissions is critical to slow near-term climate change. Globally surveying satellite instruments like the TROPOspheric Monitoring Instrument (TROPOMI) have unique capabilities for monitoring atmospheric methane around the world. Here we present a user-friendly cloud-computing tool that enables researchers and stakeholders to quantify methane emissions across user-selected regions of interest using TROPOMI satellite observations.
Kai Zhang, Wentao Zhang, Hui Wan, Philip J. Rasch, Steven J. Ghan, Richard C. Easter, Xiangjun Shi, Yong Wang, Hailong Wang, Po-Lun Ma, Shixuan Zhang, Jian Sun, Susannah M. Burrows, Manish Shrivastava, Balwinder Singh, Yun Qian, Xiaohong Liu, Jean-Christophe Golaz, Qi Tang, Xue Zheng, Shaocheng Xie, Wuyin Lin, Yan Feng, Minghuai Wang, Jin-Ho Yoon, and L. Ruby Leung
Atmos. Chem. Phys., 22, 9129–9160, https://doi.org/10.5194/acp-22-9129-2022, https://doi.org/10.5194/acp-22-9129-2022, 2022
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Here we analyze the effective aerosol forcing simulated by E3SM version 1 using both century-long free-running and short nudged simulations. The aerosol forcing in E3SMv1 is relatively large compared to other models, mainly due to the large indirect aerosol effect. Aerosol-induced changes in liquid and ice cloud properties in E3SMv1 have a strong correlation. The aerosol forcing estimates in E3SMv1 are sensitive to the parameterization changes in both liquid and ice cloud processes.
Peter Hitchcock, Amy Butler, Andrew Charlton-Perez, Chaim I. Garfinkel, Tim Stockdale, James Anstey, Dann Mitchell, Daniela I. V. Domeisen, Tongwen Wu, Yixiong Lu, Daniele Mastrangelo, Piero Malguzzi, Hai Lin, Ryan Muncaster, Bill Merryfield, Michael Sigmond, Baoqiang Xiang, Liwei Jia, Yu-Kyung Hyun, Jiyoung Oh, Damien Specq, Isla R. Simpson, Jadwiga H. Richter, Cory Barton, Jeff Knight, Eun-Pa Lim, and Harry Hendon
Geosci. Model Dev., 15, 5073–5092, https://doi.org/10.5194/gmd-15-5073-2022, https://doi.org/10.5194/gmd-15-5073-2022, 2022
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This paper describes an experimental protocol focused on sudden stratospheric warmings to be carried out by subseasonal forecast modeling centers. These will allow for inter-model comparisons of these major disruptions to the stratospheric polar vortex and their impacts on the near-surface flow. The protocol will lead to new insights into the contribution of the stratosphere to subseasonal forecast skill and new approaches to the dynamical attribution of extreme events.
Chenhong Zhou, Fan Wang, Yike Guo, Cheng Liu, Dongsheng Ji, Yuesi Wang, Xiaobin Xu, Xiao Lu, Yan Wang, Gregory Carmichael, and Meng Gao
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2022-187, https://doi.org/10.5194/essd-2022-187, 2022
Manuscript not accepted for further review
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We develop an eXtreme Gradient Boosting (XGBoost) model integrating high-resolution meteorological data, satellite retrievals of trace gases, etc. to provide reconstructed daily ground-level O3 over 2005–2021 in China. It can facilitate climatological, ecological, and health research. The dataset is freely available at Zenodo (https://zenodo.org/record/6507706#.Yo8hKujP13g; Zhou, 2022).
Susannah M. Burrows, Richard C. Easter, Xiaohong Liu, Po-Lun Ma, Hailong Wang, Scott M. Elliott, Balwinder Singh, Kai Zhang, and Philip J. Rasch
Atmos. Chem. Phys., 22, 5223–5251, https://doi.org/10.5194/acp-22-5223-2022, https://doi.org/10.5194/acp-22-5223-2022, 2022
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Sea spray particles are composed of a mixture of salts and organic substances from oceanic microorganisms. In prior work, our team developed an approach connecting sea spray chemistry to ocean biology, called OCEANFILMS. Here we describe its implementation within an Earth system model, E3SM. We show that simulated sea spray chemistry is consistent with observed seasonal cycles and that sunlight reflected by simulated Southern Ocean clouds increases, consistent with analysis of satellite data.
Po-Lun Ma, Bryce E. Harrop, Vincent E. Larson, Richard B. Neale, Andrew Gettelman, Hugh Morrison, Hailong Wang, Kai Zhang, Stephen A. Klein, Mark D. Zelinka, Yuying Zhang, Yun Qian, Jin-Ho Yoon, Christopher R. Jones, Meng Huang, Sheng-Lun Tai, Balwinder Singh, Peter A. Bogenschutz, Xue Zheng, Wuyin Lin, Johannes Quaas, Hélène Chepfer, Michael A. Brunke, Xubin Zeng, Johannes Mülmenstädt, Samson Hagos, Zhibo Zhang, Hua Song, Xiaohong Liu, Michael S. Pritchard, Hui Wan, Jingyu Wang, Qi Tang, Peter M. Caldwell, Jiwen Fan, Larry K. Berg, Jerome D. Fast, Mark A. Taylor, Jean-Christophe Golaz, Shaocheng Xie, Philip J. Rasch, and L. Ruby Leung
Geosci. Model Dev., 15, 2881–2916, https://doi.org/10.5194/gmd-15-2881-2022, https://doi.org/10.5194/gmd-15-2881-2022, 2022
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An alternative set of parameters for E3SM Atmospheric Model version 1 has been developed based on a tuning strategy that focuses on clouds. When clouds in every regime are improved, other aspects of the model are also improved, even though they are not the direct targets for calibration. The recalibrated model shows a lower sensitivity to anthropogenic aerosols and surface warming, suggesting potential improvements to the simulated climate in the past and future.
Henry Bowman, Steven Turnock, Susanne E. Bauer, Kostas Tsigaridis, Makoto Deushi, Naga Oshima, Fiona M. O'Connor, Larry Horowitz, Tongwen Wu, Jie Zhang, Dagmar Kubistin, and David D. Parrish
Atmos. Chem. Phys., 22, 3507–3524, https://doi.org/10.5194/acp-22-3507-2022, https://doi.org/10.5194/acp-22-3507-2022, 2022
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A full understanding of ozone in the troposphere requires investigation of its temporal variability over all timescales. Model simulations show that the northern midlatitude ozone seasonal cycle shifted with industrial development (1850–2014), with an increasing magnitude and a later summer peak. That shift reached a maximum in the mid-1980s, followed by a reversal toward the preindustrial cycle. The few available observations, beginning in the 1970s, are consistent with the model simulations.
Tia R. Scarpelli, Daniel J. Jacob, Shayna Grossman, Xiao Lu, Zhen Qu, Melissa P. Sulprizio, Yuzhong Zhang, Frances Reuland, Deborah Gordon, and John R. Worden
Atmos. Chem. Phys., 22, 3235–3249, https://doi.org/10.5194/acp-22-3235-2022, https://doi.org/10.5194/acp-22-3235-2022, 2022
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We present a spatially explicit version of the national inventories of oil, gas, and coal methane emissions as submitted by individual countries to the United Nations Framework Convention on Climate Change (UNFCCC) in 2021. We then use atmospheric modeling to compare our inventory emissions to atmospheric methane observations with the goal of identifying potential under- and overestimates of oil–gas methane emissions in the national inventories.
Yang Shi, Xiaohong Liu, Mingxuan Wu, Xi Zhao, Ziming Ke, and Hunter Brown
Atmos. Chem. Phys., 22, 2909–2935, https://doi.org/10.5194/acp-22-2909-2022, https://doi.org/10.5194/acp-22-2909-2022, 2022
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We perform a modeling study to evaluate the contribution to Arctic dust loading and ice-nucleating particle (INP) population from high-latitude local and low-latitude dust. High-latitude dust has a large contribution in the lower troposphere, while low-latitude dust dominates the upper troposphere. The high-latitude dust INPs result in a net cooling effect on the Arctic surface by glaciating mixed-phase clouds. Our results highlight the contribution of high-latitude dust to the Arctic climate.
Dianyi Li, Drew Shindell, Dian Ding, Xiao Lu, Lin Zhang, and Yuqiang Zhang
Atmos. Chem. Phys., 22, 2625–2638, https://doi.org/10.5194/acp-22-2625-2022, https://doi.org/10.5194/acp-22-2625-2022, 2022
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In this study, we applied chemical transport model simulation with the latest annual anthropogenic emission inventory to study the long-term trend of ozone-induced crop production losses from 2010 to 2017 in China. We find that overall the ozone-induced crop production loss in China is significant and the annual average economic losses for wheat, rice, maize, and soybean in China are USD 9.55 billion, USD 8.53 billion, USD 2.23 billion, and USD 1.16 billion respectively, over the 8 years.
Xi Zhao and Xiaohong Liu
Atmos. Chem. Phys., 22, 2585–2600, https://doi.org/10.5194/acp-22-2585-2022, https://doi.org/10.5194/acp-22-2585-2022, 2022
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The goal of this study is to investigate the relative importance and interactions of primary and secondary ice production in the Arctic mixed-phase clouds. Our results show that the SIP is not only a result of ice crystals produced from ice nucleation, but also competes with the ice production; conversely, strong ice nucleation also suppresses SIP.
Ka Ming Fung, Colette L. Heald, Jesse H. Kroll, Siyuan Wang, Duseong S. Jo, Andrew Gettelman, Zheng Lu, Xiaohong Liu, Rahul A. Zaveri, Eric C. Apel, Donald R. Blake, Jose-Luis Jimenez, Pedro Campuzano-Jost, Patrick R. Veres, Timothy S. Bates, John E. Shilling, and Maria Zawadowicz
Atmos. Chem. Phys., 22, 1549–1573, https://doi.org/10.5194/acp-22-1549-2022, https://doi.org/10.5194/acp-22-1549-2022, 2022
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Understanding the natural aerosol burden in the preindustrial era is crucial for us to assess how atmospheric aerosols affect the Earth's radiative budgets. Our study explores how a detailed description of dimethyl sulfide (DMS) oxidation (implemented in the Community Atmospheric Model version 6 with chemistry, CAM6-chem) could help us better estimate the present-day and preindustrial concentrations of sulfate and other relevant chemicals, as well as the resulting aerosol radiative impacts.
Haiyue Tan, Lin Zhang, Xiao Lu, Yuanhong Zhao, Bo Yao, Robert J. Parker, and Hartmut Boesch
Atmos. Chem. Phys., 22, 1229–1249, https://doi.org/10.5194/acp-22-1229-2022, https://doi.org/10.5194/acp-22-1229-2022, 2022
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Methane is the second most important anthropogenic greenhouse gas. Understanding methane emissions and concentration growth over China in the past decade is important to support its mitigation. This study analyzes the contributions of methane emissions from different regions and sources over the globe to methane changes over China in 2007–2018. Our results show strong international transport influences and emphasize the need of intensive methane measurements covering eastern China.
Xiao Lu, Daniel J. Jacob, Haolin Wang, Joannes D. Maasakkers, Yuzhong Zhang, Tia R. Scarpelli, Lu Shen, Zhen Qu, Melissa P. Sulprizio, Hannah Nesser, A. Anthony Bloom, Shuang Ma, John R. Worden, Shaojia Fan, Robert J. Parker, Hartmut Boesch, Ritesh Gautam, Deborah Gordon, Michael D. Moran, Frances Reuland, Claudia A. Octaviano Villasana, and Arlyn Andrews
Atmos. Chem. Phys., 22, 395–418, https://doi.org/10.5194/acp-22-395-2022, https://doi.org/10.5194/acp-22-395-2022, 2022
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We evaluate methane emissions and trends for 2010–2017 in the gridded national emission inventories for the United States, Canada, and Mexico by inversion of in situ and satellite methane observations. We find that anthropogenic methane emissions for all three countries are underestimated in the national inventories, largely driven by oil emissions. Anthropogenic methane emissions in the US peak in 2014, in contrast to the report of a steadily decreasing trend over 2010–2017 from the US EPA.
Jie Zhang, Kalli Furtado, Steven T. Turnock, Jane P. Mulcahy, Laura J. Wilcox, Ben B. Booth, David Sexton, Tongwen Wu, Fang Zhang, and Qianxia Liu
Atmos. Chem. Phys., 21, 18609–18627, https://doi.org/10.5194/acp-21-18609-2021, https://doi.org/10.5194/acp-21-18609-2021, 2021
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The CMIP6 ESMs systematically underestimate TAS anomalies in the NH midlatitudes, especially from 1960 to 1990. The anomalous cooling is concurrent in time and space with anthropogenic SO2 emissions. The spurious drop in TAS is attributed to the overestimated aerosol concentrations. The aerosol forcing sensitivity cannot well explain the inter-model spread of PHC biases. And the cloud-amount term accounts for most of the inter-model spread in aerosol forcing sensitivity.
Youwen Sun, Hao Yin, Xiao Lu, Justus Notholt, Mathias Palm, Cheng Liu, Yuan Tian, and Bo Zheng
Atmos. Chem. Phys., 21, 18589–18608, https://doi.org/10.5194/acp-21-18589-2021, https://doi.org/10.5194/acp-21-18589-2021, 2021
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This study uses high-resolution nested-grid GEOS-Chem simulation, the eXtreme Gradient Boosting (XGBoost) machine learning method, and the exposure–response relationship to determine the drivers and evaluate the health risks of the unexpected surface O3 enhancements over the Sichuan Basin in 2020. These unexpected O3 enhancements were induced by meteorological anomalies and caused dramatically high health risks.
Zhonghua Zheng, Matthew West, Lei Zhao, Po-Lun Ma, Xiaohong Liu, and Nicole Riemer
Atmos. Chem. Phys., 21, 17727–17741, https://doi.org/10.5194/acp-21-17727-2021, https://doi.org/10.5194/acp-21-17727-2021, 2021
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Aerosol mixing state is an important emergent property that affects aerosol radiative forcing and aerosol–cloud interactions, but it has not been easy to constrain this property globally. We present a framework for evaluating the error in aerosol mixing state induced by aerosol representation assumptions, which is one of the important contributors to structural uncertainty in aerosol models. Our study provides insights into potential improvements to model process representation for aerosols.
Ruqian Miao, Qi Chen, Manish Shrivastava, Youfan Chen, Lin Zhang, Jianlin Hu, Yan Zheng, and Keren Liao
Atmos. Chem. Phys., 21, 16183–16201, https://doi.org/10.5194/acp-21-16183-2021, https://doi.org/10.5194/acp-21-16183-2021, 2021
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We apply process-based and observation-constrained schemes to simulate organic aerosol in China and conduct comprehensive model–observation comparisons. The results show that anthropogenic semivolatile and intermediate-volatility organic compounds (SVOCs and IVOCs) are the main sources of secondary organic aerosol (SOA) in polluted regions, for which the residential sector is perhaps the predominant contributor. The hydroxyl radical level is also important for SOA modeling in polluted regions.
Zhen Qu, Daniel J. Jacob, Lu Shen, Xiao Lu, Yuzhong Zhang, Tia R. Scarpelli, Hannah Nesser, Melissa P. Sulprizio, Joannes D. Maasakkers, A. Anthony Bloom, John R. Worden, Robert J. Parker, and Alba L. Delgado
Atmos. Chem. Phys., 21, 14159–14175, https://doi.org/10.5194/acp-21-14159-2021, https://doi.org/10.5194/acp-21-14159-2021, 2021
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The recent launch of TROPOMI offers an unprecedented opportunity to quantify the methane budget from a top-down perspective. We use TROPOMI and the more mature GOSAT methane observations to estimate methane emissions and get consistent global budgets. However, TROPOMI shows biases over regions where surface albedo is small and provides less information for the coarse-resolution inversion due to the larger error correlations and spatial variations in the number of observations.
Yixiong Lu, Tongwen Wu, Yubin Li, and Ben Yang
Geosci. Model Dev., 14, 5183–5204, https://doi.org/10.5194/gmd-14-5183-2021, https://doi.org/10.5194/gmd-14-5183-2021, 2021
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The spurious precipitation in the tropical southeastern Pacific and southern Atlantic is one of the most prominent systematic biases in coupled atmosphere–ocean general circulation models. This study significantly promotes the marine stratus simulation and largely alleviates the excessive precipitation biases through improving parameterizations of boundary-layer turbulence and shallow convection, providing an effective solution to the long-standing bias in the tropical precipitation simulation.
Youwen Sun, Hao Yin, Cheng Liu, Emmanuel Mahieu, Justus Notholt, Yao Té, Xiao Lu, Mathias Palm, Wei Wang, Changgong Shan, Qihou Hu, Min Qin, Yuan Tian, and Bo Zheng
Atmos. Chem. Phys., 21, 11759–11779, https://doi.org/10.5194/acp-21-11759-2021, https://doi.org/10.5194/acp-21-11759-2021, 2021
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The variability, sources, and transport of ethane (C2H6) over eastern China from 2015 to 2020 were studied using ground-based Fourier transform infrared (FTIR) spectroscopy and GEOS-Chem simulations. C2H6 variability is driven by both meteorological and emission factors. The reduction in C2H6 in recent years over eastern China points to air quality improvement in China.
Yadong Lei, Xu Yue, Hong Liao, Lin Zhang, Yang Yang, Hao Zhou, Chenguang Tian, Cheng Gong, Yimian Ma, Lan Gao, and Yang Cao
Atmos. Chem. Phys., 21, 11531–11543, https://doi.org/10.5194/acp-21-11531-2021, https://doi.org/10.5194/acp-21-11531-2021, 2021
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We present the first estimate of ozone enhancement by fire emissions through ozone–vegetation interactions using a fully coupled chemistry–vegetation model (GC-YIBs). In fire-prone areas, fire-induced ozone causes a positive feedback to surface ozone mainly because of the inhibition effects on stomatal conductance.
Meng Gao, Yang Yang, Hong Liao, Bin Zhu, Yuxuan Zhang, Zirui Liu, Xiao Lu, Chen Wang, Qiming Zhou, Yuesi Wang, Qiang Zhang, Gregory R. Carmichael, and Jianlin Hu
Atmos. Chem. Phys., 21, 11405–11421, https://doi.org/10.5194/acp-21-11405-2021, https://doi.org/10.5194/acp-21-11405-2021, 2021
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Light absorption and radiative forcing of black carbon (BC) is influenced by both BC itself and its interactions with other aerosol chemical compositions. In this study, we used the online coupled WRF-Chem model to examine how emission control measures during the Asian-Pacific Economic Cooperation (APEC) conference affect the mixing state and light absorption of BC and the associated implications for BC-PBL interactions.
David D. Parrish, Richard G. Derwent, Steven T. Turnock, Fiona M. O'Connor, Johannes Staehelin, Susanne E. Bauer, Makoto Deushi, Naga Oshima, Kostas Tsigaridis, Tongwen Wu, and Jie Zhang
Atmos. Chem. Phys., 21, 9669–9679, https://doi.org/10.5194/acp-21-9669-2021, https://doi.org/10.5194/acp-21-9669-2021, 2021
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The few ozone measurements made before the 1980s indicate that industrial development increased ozone concentrations by a factor of ~ 2 at northern midlatitudes, which are now larger than at southern midlatitudes. This difference was much smaller, and likely reversed, in the pre-industrial atmosphere. Earth system models find similar increases, but not higher pre-industrial ozone in the south. This disagreement may indicate that modeled natural ozone sources and/or deposition loss are inadequate.
Youwen Sun, Hao Yin, Yuan Cheng, Qianggong Zhang, Bo Zheng, Justus Notholt, Xiao Lu, Cheng Liu, Yuan Tian, and Jianguo Liu
Atmos. Chem. Phys., 21, 9201–9222, https://doi.org/10.5194/acp-21-9201-2021, https://doi.org/10.5194/acp-21-9201-2021, 2021
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We quantified the variability, source, and transport of urban CO over the Himalayas and Tibetan Plateau (HTP) by using measurement, model simulation, and the analysis of meteorological fields. Urban CO over the HTP is dominated by anthropogenic and biomass burning emissions from local, South Asia and East Asia, and oxidation sources. The decreasing trends in surface CO since 2015 in most cities over the HTP are attributed to the reduction in local and transported CO emissions in recent years.
Tongwen Wu, Rucong Yu, Yixiong Lu, Weihua Jie, Yongjie Fang, Jie Zhang, Li Zhang, Xiaoge Xin, Laurent Li, Zaizhi Wang, Yiming Liu, Fang Zhang, Fanghua Wu, Min Chu, Jianglong Li, Weiping Li, Yanwu Zhang, Xueli Shi, Wenyan Zhou, Junchen Yao, Xiangwen Liu, He Zhao, Jinghui Yan, Min Wei, Wei Xue, Anning Huang, Yaocun Zhang, Yu Zhang, Qi Shu, and Aixue Hu
Geosci. Model Dev., 14, 2977–3006, https://doi.org/10.5194/gmd-14-2977-2021, https://doi.org/10.5194/gmd-14-2977-2021, 2021
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This paper presents the high-resolution version of the Beijing Climate Center (BCC) Climate System Model, BCC-CSM2-HR, and describes its climate simulation performance including the atmospheric temperature and wind; precipitation; and the tropical climate phenomena such as TC, MJO, QBO, and ENSO. BCC-CSM2-HR is our model version contributing to the HighResMIP. We focused on its updates and differential characteristics from its predecessor, the medium-resolution version BCC-CSM2-MR.
Jing Wei, Zhanqing Li, Rachel T. Pinker, Jun Wang, Lin Sun, Wenhao Xue, Runze Li, and Maureen Cribb
Atmos. Chem. Phys., 21, 7863–7880, https://doi.org/10.5194/acp-21-7863-2021, https://doi.org/10.5194/acp-21-7863-2021, 2021
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This study developed a space-time Light Gradient Boosting Machine (STLG) model to derive the high-temporal-resolution (1 h) and high-quality PM2.5 dataset in China (i.e., ChinaHighPM2.5) at a 5 km spatial resolution from the Himawari-8 Advanced Himawari Imager aerosol products. Our model outperforms most previous related studies with a much lower computation burden in terms of speed and memory, making it most suitable for real-time air pollution monitoring in China.
Youwen Sun, Hao Yin, Cheng Liu, Lin Zhang, Yuan Cheng, Mathias Palm, Justus Notholt, Xiao Lu, Corinne Vigouroux, Bo Zheng, Wei Wang, Nicholas Jones, Changong Shan, Min Qin, Yuan Tian, Qihou Hu, Fanhao Meng, and Jianguo Liu
Atmos. Chem. Phys., 21, 6365–6387, https://doi.org/10.5194/acp-21-6365-2021, https://doi.org/10.5194/acp-21-6365-2021, 2021
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This study mapped the drivers of HCHO variability from 2015 to 2019 over eastern China. Hydroxyl (OH) radical production rates from HCHO photolysis were evaluated. The relative contributions of emitted and photochemical sources to the observed HCHO abundance were analyzed. Contributions of various emission sources and geographical regions to the observed HCHO summertime enhancements were determined.
Yuan Zhang, Olivier Boucher, Philippe Ciais, Laurent Li, and Nicolas Bellouin
Geosci. Model Dev., 14, 2029–2039, https://doi.org/10.5194/gmd-14-2029-2021, https://doi.org/10.5194/gmd-14-2029-2021, 2021
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We investigated different methods to reconstruct spatiotemporal distribution of the fraction of diffuse radiation (Fdf) to qualify the aerosol impacts on GPP using the ORCHIDEE_DF land surface model. We find that climatological-averaging methods which dampen the variability of Fdf can cause significant bias in the modeled diffuse radiation impacts on GPP. Better methods to reconstruct Fdf are recommended.
Xi Zhao, Xiaohong Liu, Vaughan T. J. Phillips, and Sachin Patade
Atmos. Chem. Phys., 21, 5685–5703, https://doi.org/10.5194/acp-21-5685-2021, https://doi.org/10.5194/acp-21-5685-2021, 2021
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Arctic mixed-phase clouds significantly influence the energy budget of the Arctic. We show that a climate model considering secondary ice production (SIP) can explain the observed cloud ice number concentrations, vertical distribution pattern, and probability density distribution of ice crystal number concentrations. The mixed-phase cloud occurrence and phase partitioning are also improved.
James Keeble, Birgit Hassler, Antara Banerjee, Ramiro Checa-Garcia, Gabriel Chiodo, Sean Davis, Veronika Eyring, Paul T. Griffiths, Olaf Morgenstern, Peer Nowack, Guang Zeng, Jiankai Zhang, Greg Bodeker, Susannah Burrows, Philip Cameron-Smith, David Cugnet, Christopher Danek, Makoto Deushi, Larry W. Horowitz, Anne Kubin, Lijuan Li, Gerrit Lohmann, Martine Michou, Michael J. Mills, Pierre Nabat, Dirk Olivié, Sungsu Park, Øyvind Seland, Jens Stoll, Karl-Hermann Wieners, and Tongwen Wu
Atmos. Chem. Phys., 21, 5015–5061, https://doi.org/10.5194/acp-21-5015-2021, https://doi.org/10.5194/acp-21-5015-2021, 2021
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Stratospheric ozone and water vapour are key components of the Earth system; changes to both have important impacts on global and regional climate. We evaluate changes to these species from 1850 to 2100 in the new generation of CMIP6 models. There is good agreement between the multi-model mean and observations, although there is substantial variation between the individual models. The future evolution of both ozone and water vapour is strongly dependent on the assumed future emissions scenario.
Xiao Lu, Daniel J. Jacob, Yuzhong Zhang, Joannes D. Maasakkers, Melissa P. Sulprizio, Lu Shen, Zhen Qu, Tia R. Scarpelli, Hannah Nesser, Robert M. Yantosca, Jianxiong Sheng, Arlyn Andrews, Robert J. Parker, Hartmut Boesch, A. Anthony Bloom, and Shuang Ma
Atmos. Chem. Phys., 21, 4637–4657, https://doi.org/10.5194/acp-21-4637-2021, https://doi.org/10.5194/acp-21-4637-2021, 2021
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We use an analytical solution to the Bayesian inverse problem to quantitatively compare and combine the information from satellite and in situ observations, and to estimate global methane budget and their trends over the 2010–2017 period. We find that satellite and in situ observations are to a large extent complementary in the inversion for estimating global methane budget, and reveal consistent corrections of regional anthropogenic and wetland methane emissions relative to the prior inventory.
Joannes D. Maasakkers, Daniel J. Jacob, Melissa P. Sulprizio, Tia R. Scarpelli, Hannah Nesser, Jianxiong Sheng, Yuzhong Zhang, Xiao Lu, A. Anthony Bloom, Kevin W. Bowman, John R. Worden, and Robert J. Parker
Atmos. Chem. Phys., 21, 4339–4356, https://doi.org/10.5194/acp-21-4339-2021, https://doi.org/10.5194/acp-21-4339-2021, 2021
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We use 2010–2015 GOSAT satellite observations of atmospheric methane over North America in a high-resolution inversion to estimate methane emissions. We find general consistency with the gridded EPA inventory but higher oil and gas production emissions, with oil production emissions twice as large as in the latest EPA Greenhouse Gas Inventory. We find lower wetland emissions than predicted by WetCHARTs and a small increasing trend in the eastern US, apparently related to unconventional oil/gas.
Yuzhong Zhang, Daniel J. Jacob, Xiao Lu, Joannes D. Maasakkers, Tia R. Scarpelli, Jian-Xiong Sheng, Lu Shen, Zhen Qu, Melissa P. Sulprizio, Jinfeng Chang, A. Anthony Bloom, Shuang Ma, John Worden, Robert J. Parker, and Hartmut Boesch
Atmos. Chem. Phys., 21, 3643–3666, https://doi.org/10.5194/acp-21-3643-2021, https://doi.org/10.5194/acp-21-3643-2021, 2021
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We use 2010–2018 satellite observations of atmospheric methane to interpret the factors controlling atmospheric methane and its accelerating increase during the period. The 2010–2018 increase in global methane emissions is driven by tropical and boreal wetlands and tropical livestock (South Asia, Africa, Brazil), with an insignificant positive trend in emissions from the fossil fuel sector. The peak methane growth rates in 2014–2015 are also contributed by low OH and high fire emissions.
Zun Yin, Catherine Ottlé, Philippe Ciais, Feng Zhou, Xuhui Wang, Polcher Jan, Patrice Dumas, Shushi Peng, Laurent Li, Xudong Zhou, Yan Bo, Yi Xi, and Shilong Piao
Hydrol. Earth Syst. Sci., 25, 1133–1150, https://doi.org/10.5194/hess-25-1133-2021, https://doi.org/10.5194/hess-25-1133-2021, 2021
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We improved the irrigation module in a land surface model ORCHIDEE and developed a dam operation model with the aim to investigate how irrigation and dams affect the streamflow fluctuations of the Yellow River. Results show that irrigation mainly reduces the annual river flow. The dam operation, however, mainly affects streamflow variation. By considering two generic operation rules, flood control and base flow guarantee, our dam model can sustainably improve the simulation accuracy.
Zhongjing Jiang, Jing Li, Xiao Lu, Cheng Gong, Lin Zhang, and Hong Liao
Atmos. Chem. Phys., 21, 2601–2613, https://doi.org/10.5194/acp-21-2601-2021, https://doi.org/10.5194/acp-21-2601-2021, 2021
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This study demonstrates that the intensity of the western Pacific subtropical high (WPSH), a major synoptic pattern in the northern Pacific during summer, can induce a dipole change in surface ozone pollution over eastern China. Ozone concentration increases in the north and decreases in the south during the strong WPSH phase, and vice versa. The change in chemical processes associated with the WPSH change plays a decisive role, whereas the natural emission of ozone precursors accounts for ~ 30 %.
Xi Zhao, Xiaohong Liu, Susannah M. Burrows, and Yang Shi
Atmos. Chem. Phys., 21, 2305–2327, https://doi.org/10.5194/acp-21-2305-2021, https://doi.org/10.5194/acp-21-2305-2021, 2021
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Organic sea spray particles influence aerosol and cloud processes over the ocean. This study introduces the emission, cloud droplet activation, and ice nucleation (IN) of marine organic aerosol (MOA) into the Community Earth System Model. Our results indicate that MOA IN particles dominate primary ice nucleation below 400 hPa over the Southern Ocean and Arctic boundary layer. MOA enhances cloud forcing over the Southern Ocean in the austral winter and summer.
Ryan Patnaude, Minghui Diao, Xiaohong Liu, and Suqian Chu
Atmos. Chem. Phys., 21, 1835–1859, https://doi.org/10.5194/acp-21-1835-2021, https://doi.org/10.5194/acp-21-1835-2021, 2021
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A comprehensive, in situ observation dataset of cirrus clouds was developed based on seven field campaigns, ranging from 87° N–75° S. The observations were compared with a global climate model. Several key factors for cirrus cloud formation were examined, including thermodynamics, dynamics, aerosol indirect effects and geographical locations. Model biases include lower ice mass concentrations, smaller ice crystals and weaker aerosol indirect effects.
Gillian D. Thornhill, William J. Collins, Ryan J. Kramer, Dirk Olivié, Ragnhild B. Skeie, Fiona M. O'Connor, Nathan Luke Abraham, Ramiro Checa-Garcia, Susanne E. Bauer, Makoto Deushi, Louisa K. Emmons, Piers M. Forster, Larry W. Horowitz, Ben Johnson, James Keeble, Jean-Francois Lamarque, Martine Michou, Michael J. Mills, Jane P. Mulcahy, Gunnar Myhre, Pierre Nabat, Vaishali Naik, Naga Oshima, Michael Schulz, Christopher J. Smith, Toshihiko Takemura, Simone Tilmes, Tongwen Wu, Guang Zeng, and Jie Zhang
Atmos. Chem. Phys., 21, 853–874, https://doi.org/10.5194/acp-21-853-2021, https://doi.org/10.5194/acp-21-853-2021, 2021
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This paper is a study of how different constituents in the atmosphere, such as aerosols and gases like methane and ozone, affect the energy balance in the atmosphere. Different climate models were run using the same inputs to allow an easy comparison of the results and to understand where the models differ. We found the effect of aerosols is to reduce warming in the atmosphere, but this effect varies between models. Reactions between gases are also important in affecting climate.
Steven T. Turnock, Robert J. Allen, Martin Andrews, Susanne E. Bauer, Makoto Deushi, Louisa Emmons, Peter Good, Larry Horowitz, Jasmin G. John, Martine Michou, Pierre Nabat, Vaishali Naik, David Neubauer, Fiona M. O'Connor, Dirk Olivié, Naga Oshima, Michael Schulz, Alistair Sellar, Sungbo Shim, Toshihiko Takemura, Simone Tilmes, Kostas Tsigaridis, Tongwen Wu, and Jie Zhang
Atmos. Chem. Phys., 20, 14547–14579, https://doi.org/10.5194/acp-20-14547-2020, https://doi.org/10.5194/acp-20-14547-2020, 2020
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A first assessment is made of the historical and future changes in air pollutants from models participating in the 6th Coupled Model Intercomparison Project (CMIP6). Substantial benefits to future air quality can be achieved in future scenarios that implement measures to mitigate climate and involve reductions in air pollutant emissions, particularly methane. However, important differences are shown between models in the future regional projection of air pollutants under the same scenario.
Lena R. Boysen, Victor Brovkin, Julia Pongratz, David M. Lawrence, Peter Lawrence, Nicolas Vuichard, Philippe Peylin, Spencer Liddicoat, Tomohiro Hajima, Yanwu Zhang, Matthias Rocher, Christine Delire, Roland Séférian, Vivek K. Arora, Lars Nieradzik, Peter Anthoni, Wim Thiery, Marysa M. Laguë, Deborah Lawrence, and Min-Hui Lo
Biogeosciences, 17, 5615–5638, https://doi.org/10.5194/bg-17-5615-2020, https://doi.org/10.5194/bg-17-5615-2020, 2020
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We find a biogeophysically induced global cooling with strong carbon losses in a 20 million square kilometre idealized deforestation experiment performed by nine CMIP6 Earth system models. It takes many decades for the temperature signal to emerge, with non-local effects playing an important role. Despite a consistent experimental setup, models diverge substantially in their climate responses. This study offers unprecedented insights for understanding land use change effects in CMIP6 models.
Mingxuan Wu, Xiaohong Liu, Hongbin Yu, Hailong Wang, Yang Shi, Kang Yang, Anton Darmenov, Chenglai Wu, Zhien Wang, Tao Luo, Yan Feng, and Ziming Ke
Atmos. Chem. Phys., 20, 13835–13855, https://doi.org/10.5194/acp-20-13835-2020, https://doi.org/10.5194/acp-20-13835-2020, 2020
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The spatiotemporal distributions of dust aerosol simulated by global climate models (GCMs) are highly uncertain. In this study, we evaluate dust extinction profiles, optical depth, and surface concentrations simulated in three GCMs and one reanalysis against multiple satellite retrievals and surface observations to gain process-level understanding. Our results highlight the importance of correctly representing dust emission, dry/wet deposition, and size distribution in GCMs.
Yuan Zhang, Ana Bastos, Fabienne Maignan, Daniel Goll, Olivier Boucher, Laurent Li, Alessandro Cescatti, Nicolas Vuichard, Xiuzhi Chen, Christof Ammann, M. Altaf Arain, T. Andrew Black, Bogdan Chojnicki, Tomomichi Kato, Ivan Mammarella, Leonardo Montagnani, Olivier Roupsard, Maria J. Sanz, Lukas Siebicke, Marek Urbaniak, Francesco Primo Vaccari, Georg Wohlfahrt, Will Woodgate, and Philippe Ciais
Geosci. Model Dev., 13, 5401–5423, https://doi.org/10.5194/gmd-13-5401-2020, https://doi.org/10.5194/gmd-13-5401-2020, 2020
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We improved the ORCHIDEE LSM by distinguishing diffuse and direct light in canopy and evaluated the new model with observations from 159 sites. Compared with the old model, the new model has better sunny GPP and reproduced the diffuse light fertilization effect observed at flux sites. Our simulations also indicate different mechanisms causing the observed GPP enhancement under cloudy conditions at different times. The new model has the potential to study large-scale impacts of aerosol changes.
Ke Li, Daniel J. Jacob, Lu Shen, Xiao Lu, Isabelle De Smedt, and Hong Liao
Atmos. Chem. Phys., 20, 11423–11433, https://doi.org/10.5194/acp-20-11423-2020, https://doi.org/10.5194/acp-20-11423-2020, 2020
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Surface summer ozone increased in China from 2013 to 2019 despite new governmental efforts targeting ozone pollution. We find that the ozone increase is mostly due to anthropogenic drivers, although meteorology also plays a role. Further analysis for the North China Plain shows that PM2.5 continued to decrease through 2019, while emissions of volatile organic compounds (VOCs) stayed flat. This could explain the anthropogenic increase in ozone, as PM2.5 scavenges the radical precursors of ozone.
Stefan Rahimi, Xiaohong Liu, Chun Zhao, Zheng Lu, and Zachary J. Lebo
Atmos. Chem. Phys., 20, 10911–10935, https://doi.org/10.5194/acp-20-10911-2020, https://doi.org/10.5194/acp-20-10911-2020, 2020
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Dark particles emitted to the atmosphere can absorb sunlight and heat the air. As these particles settle, they may darken the surface, especially over snow-covered regions like the Rocky Mountains. This darkening of the surface may lead to changes in snowpack, affecting the local meteorology and hydrology. We seek to evaluate whether these light-absorbing particles more prominently affect this region through their atmospheric presence or their on-snow presence.
Chenglai Wu, Zhaohui Lin, and Xiaohong Liu
Atmos. Chem. Phys., 20, 10401–10425, https://doi.org/10.5194/acp-20-10401-2020, https://doi.org/10.5194/acp-20-10401-2020, 2020
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This study provides a comprehensive evaluation of the global dust cycle in 15 models participating in the fifth phase of the Coupled Model Intercomparison Project (CMIP5). We assess the global budget and associated uncertainties. We also quantify the discrepancies in each model. The results highlight the large uncertainties in both the locations and intensities of dust emission. Our study will serve as a useful reference for model communities and help further model improvements.
Xiao Lu, Lin Zhang, Tongwen Wu, Michael S. Long, Jun Wang, Daniel J. Jacob, Fang Zhang, Jie Zhang, Sebastian D. Eastham, Lu Hu, Lei Zhu, Xiong Liu, and Min Wei
Geosci. Model Dev., 13, 3817–3838, https://doi.org/10.5194/gmd-13-3817-2020, https://doi.org/10.5194/gmd-13-3817-2020, 2020
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This study presents the development and evaluation of a new climate chemistry model, BCC-GEOS-Chem v1.0, which couples the GEOS-Chem chemical transport model as an atmospheric chemistry component in the Beijing Climate Center atmospheric general circulation model. A 3-year (2012–2014) simulation of BCC-GEOS-Chem v1.0 shows that the model captures well the spatiotemporal distributions of tropospheric ozone, other gaseous pollutants, and aerosols.
Tong Sha, Xiaoyan Ma, Jun Wang, Rong Tian, Jianqi Zhao, Fang Cao, and Yan-Lin Zhang
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-760, https://doi.org/10.5194/acp-2020-760, 2020
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Most numerical models perform poorly on simulating the inorganic chemical components in PM2.5 (sulfate, nitrate, and ammonium (SNA)), generally underestimate sulfate but overestimate nitrate concentrations in haze events. Our work aims at investigating the role of cloud water in simulating SNA. We find that the uncertainties of cloud water can lead to model bias in simulating SNA, and can be reduced by constraining the modeled cloud water with MODIS satellite observations.
Vivek K. Arora, Anna Katavouta, Richard G. Williams, Chris D. Jones, Victor Brovkin, Pierre Friedlingstein, Jörg Schwinger, Laurent Bopp, Olivier Boucher, Patricia Cadule, Matthew A. Chamberlain, James R. Christian, Christine Delire, Rosie A. Fisher, Tomohiro Hajima, Tatiana Ilyina, Emilie Joetzjer, Michio Kawamiya, Charles D. Koven, John P. Krasting, Rachel M. Law, David M. Lawrence, Andrew Lenton, Keith Lindsay, Julia Pongratz, Thomas Raddatz, Roland Séférian, Kaoru Tachiiri, Jerry F. Tjiputra, Andy Wiltshire, Tongwen Wu, and Tilo Ziehn
Biogeosciences, 17, 4173–4222, https://doi.org/10.5194/bg-17-4173-2020, https://doi.org/10.5194/bg-17-4173-2020, 2020
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Since the preindustrial period, land and ocean have taken up about half of the carbon emitted into the atmosphere by humans. Comparison of different earth system models with the carbon cycle allows us to assess how carbon uptake by land and ocean differs among models. This yields an estimate of uncertainty in our understanding of how land and ocean respond to increasing atmospheric CO2. This paper summarizes results from two such model intercomparison projects that use an idealized scenario.
Robert J. Allen, Steven Turnock, Pierre Nabat, David Neubauer, Ulrike Lohmann, Dirk Olivié, Naga Oshima, Martine Michou, Tongwen Wu, Jie Zhang, Toshihiko Takemura, Michael Schulz, Kostas Tsigaridis, Susanne E. Bauer, Louisa Emmons, Larry Horowitz, Vaishali Naik, Twan van Noije, Tommi Bergman, Jean-Francois Lamarque, Prodromos Zanis, Ina Tegen, Daniel M. Westervelt, Philippe Le Sager, Peter Good, Sungbo Shim, Fiona O'Connor, Dimitris Akritidis, Aristeidis K. Georgoulias, Makoto Deushi, Lori T. Sentman, Jasmin G. John, Shinichiro Fujimori, and William J. Collins
Atmos. Chem. Phys., 20, 9641–9663, https://doi.org/10.5194/acp-20-9641-2020, https://doi.org/10.5194/acp-20-9641-2020, 2020
Haipeng Lin, Xu Feng, Tzung-May Fu, Heng Tian, Yaping Ma, Lijuan Zhang, Daniel J. Jacob, Robert M. Yantosca, Melissa P. Sulprizio, Elizabeth W. Lundgren, Jiawei Zhuang, Qiang Zhang, Xiao Lu, Lin Zhang, Lu Shen, Jianping Guo, Sebastian D. Eastham, and Christoph A. Keller
Geosci. Model Dev., 13, 3241–3265, https://doi.org/10.5194/gmd-13-3241-2020, https://doi.org/10.5194/gmd-13-3241-2020, 2020
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Online coupling of meteorology and chemistry models often presents maintenance issues with hard-wired coding. We present WRF-GC, an one-way online coupling of the WRF meteorological model and GEOS-Chem atmospheric chemistry model for regional atmospheric chemistry and air quality modeling. Our coupling structure allows future versions of either parent model to be immediately integrated into WRF-GC. The WRF-GC model was able to well reproduce regional PM2.5 with greater computational efficiency.
Yi Wang, Jun Wang, Xiaoguang Xu, Daven K. Henze, Zhen Qu, and Kai Yang
Atmos. Chem. Phys., 20, 6631–6650, https://doi.org/10.5194/acp-20-6631-2020, https://doi.org/10.5194/acp-20-6631-2020, 2020
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The use of OMPS satellite observations to inverse-model SO2 and NO2 emissions is presented through the GEOS-Chem adjoint modeling framework. The work is illustrated over China. The robustness of the results is studied through separate and joint inversions of SO2 and NO2 and the consideration of NH3 uncertainty. Independent validation is performed with OMI SO2 and NO2 data. It is shown that simultaneous inversion of NO2 and SO2 from OMPS provides an effective way to rapidly update emissions.
Yi Wang, Jun Wang, Meng Zhou, Daven K. Henze, Cui Ge, and Wei Wang
Atmos. Chem. Phys., 20, 6651–6670, https://doi.org/10.5194/acp-20-6651-2020, https://doi.org/10.5194/acp-20-6651-2020, 2020
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We developed four different methods to downscale SO2 and NO2 emissions derived from OMPS satellite observations (in Part 1) for regional air quality modeling at a spatial resolution that is finer than satellite observations. The VIIRS (city lights), TROPOMI, and OMI satellite data as well as surface data are used to evaluate the model. The method of using the top-down emissions from the past month for the air quality forecast in the present month is also shown to have practical merit.
Tristan Vadsaria, Laurent Li, Gilles Ramstein, and Jean-Claude Dutay
Geosci. Model Dev., 13, 2337–2354, https://doi.org/10.5194/gmd-13-2337-2020, https://doi.org/10.5194/gmd-13-2337-2020, 2020
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This article aims to reproduce the Early Holocene climate over the Mediterranean basin, characterized with a large reorganization of the Mediterranean thermohaline circulation. In order to reduce the demand of strong computation resources, a comprehensive global-to-regional model architecture is developed and validated against paleo data. Beyond the case study shown here, this platform may be applied to a large number of paleoclimate contexts.
Youwen Sun, Cheng Liu, Lin Zhang, Mathias Palm, Justus Notholt, Hao Yin, Corinne Vigouroux, Erik Lutsch, Wei Wang, Changong Shan, Thomas Blumenstock, Tomoo Nagahama, Isamu Morino, Emmanuel Mahieu, Kimberly Strong, Bavo Langerock, Martine De Mazière, Qihou Hu, Huifang Zhang, Christof Petri, and Jianguo Liu
Atmos. Chem. Phys., 20, 5437–5456, https://doi.org/10.5194/acp-20-5437-2020, https://doi.org/10.5194/acp-20-5437-2020, 2020
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We present multiyear time series of ground-based Fourier-transform infrared spectroscopy measurements of HCN in densely populated eastern China. The seasonality and interannual variability of tropospheric HCN columns were investigated. The potential sources that drive the observed HCN seasonality and interannual variability were determined using a GEOS-Chem tagged CO simulation, global fire maps, and potential source contribution function values calculated using HYSPLIT back trajectories.
Meng Gao, Jinhui Gao, Bin Zhu, Rajesh Kumar, Xiao Lu, Shaojie Song, Yuzhong Zhang, Beixi Jia, Peng Wang, Gufran Beig, Jianlin Hu, Qi Ying, Hongliang Zhang, Peter Sherman, and Michael B. McElroy
Atmos. Chem. Phys., 20, 4399–4414, https://doi.org/10.5194/acp-20-4399-2020, https://doi.org/10.5194/acp-20-4399-2020, 2020
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A regional fully coupled meteorology–chemistry model, Weather Research and Forecasting model with Chemistry (WRF-Chem), was employed to study the seasonality of ozone (O3) pollution and its sources in both China and India.
Yadong Lei, Xu Yue, Hong Liao, Cheng Gong, and Lin Zhang
Geosci. Model Dev., 13, 1137–1153, https://doi.org/10.5194/gmd-13-1137-2020, https://doi.org/10.5194/gmd-13-1137-2020, 2020
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We coupled a dynamic vegetation model YIBs with the chemical transport model GEOS-Chem to develop a new tool for studying interactions between atmospheric chemistry and biosphere. Within this framework, leaf area index and stomatal conductance are predicted for chemical simulations. In turn, surface ozone causes negative impacts to plant growth and the consequent dry deposition. Such interactions are important for air pollution prediction but ignored in most of current chemical models.
Andrew E. Kiss, Andrew McC. Hogg, Nicholas Hannah, Fabio Boeira Dias, Gary B. Brassington, Matthew A. Chamberlain, Christopher Chapman, Peter Dobrohotoff, Catia M. Domingues, Earl R. Duran, Matthew H. England, Russell Fiedler, Stephen M. Griffies, Aidan Heerdegen, Petra Heil, Ryan M. Holmes, Andreas Klocker, Simon J. Marsland, Adele K. Morrison, James Munroe, Maxim Nikurashin, Peter R. Oke, Gabriela S. Pilo, Océane Richet, Abhishek Savita, Paul Spence, Kial D. Stewart, Marshall L. Ward, Fanghua Wu, and Xihan Zhang
Geosci. Model Dev., 13, 401–442, https://doi.org/10.5194/gmd-13-401-2020, https://doi.org/10.5194/gmd-13-401-2020, 2020
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We describe new computer model configurations which simulate the global ocean and sea ice at three resolutions. The coarsest resolution is suitable for multi-century climate projection experiments, whereas the finest resolution is designed for more detailed studies over time spans of decades. The paper provides technical details of the model configurations and an assessment of their performance relative to observations.
Xiaohua Pan, Charles Ichoku, Mian Chin, Huisheng Bian, Anton Darmenov, Peter Colarco, Luke Ellison, Tom Kucsera, Arlindo da Silva, Jun Wang, Tomohiro Oda, and Ge Cui
Atmos. Chem. Phys., 20, 969–994, https://doi.org/10.5194/acp-20-969-2020, https://doi.org/10.5194/acp-20-969-2020, 2020
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The differences between these six BB emission datasets are large. Our study found that (1) most current biomass burning (BB) aerosol emission datasets derived from satellite observations lead to the underestimation of aerosol optical depth (AOD) in this model in the biomass-burning-dominated regions and (2) it is important to accurately estimate both the magnitudes and spatial patterns of regional BB emissions in order for a model using these emissions to reproduce observed AOD levels.
Jun Zhu, Xiangao Xia, Huizheng Che, Jun Wang, Zhiyuan Cong, Tianliang Zhao, Shichang Kang, Xuelei Zhang, Xingna Yu, and Yanlin Zhang
Atmos. Chem. Phys., 19, 14637–14656, https://doi.org/10.5194/acp-19-14637-2019, https://doi.org/10.5194/acp-19-14637-2019, 2019
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The long-term temporal–spatial variations of the aerosol optical properties over the Tibetan Plateau (TP) based on the multiple ground-based sun photometer sites and the MODIS product are presented. Besides, the aerosol pollution and aerosol transport processes over the TP are also analyzed by the observations and models. The results in this region could help reduce the assessment uncertainties of aerosol radiative forcing and provide more information on aerosol transportation.
Fang Li, Maria Val Martin, Meinrat O. Andreae, Almut Arneth, Stijn Hantson, Johannes W. Kaiser, Gitta Lasslop, Chao Yue, Dominique Bachelet, Matthew Forrest, Erik Kluzek, Xiaohong Liu, Stephane Mangeon, Joe R. Melton, Daniel S. Ward, Anton Darmenov, Thomas Hickler, Charles Ichoku, Brian I. Magi, Stephen Sitch, Guido R. van der Werf, Christine Wiedinmyer, and Sam S. Rabin
Atmos. Chem. Phys., 19, 12545–12567, https://doi.org/10.5194/acp-19-12545-2019, https://doi.org/10.5194/acp-19-12545-2019, 2019
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Fire emissions are critical for atmospheric composition, climate, carbon cycle, and air quality. We provide the first global multi-model fire emission reconstructions for 1700–2012, including carbon and 33 species of trace gases and aerosols, based on the nine state-of-the-art global fire models that participated in FireMIP. We also provide information on the recent status and limitations of the model-based reconstructions and identify the main uncertainty sources in their long-term changes.
Stefan Rahimi, Xiaohong Liu, Chenglai Wu, William K. Lau, Hunter Brown, Mingxuan Wu, and Yun Qian
Atmos. Chem. Phys., 19, 12025–12049, https://doi.org/10.5194/acp-19-12025-2019, https://doi.org/10.5194/acp-19-12025-2019, 2019
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Light-absorbing particles impact the Earth system in a variety of ways. They can warm the atmosphere by their very presence, or they can warm the atmosphere after they deposit on snow, warm it, and warm the overlying atmosphere. This paper focuses on these two processes as they pertain to black carbon and dust's impacts on the South Asian monsoon. It will be shown that these two aerosols have a significant effect on the monsoon.
Steven D. Miller, Louie D. Grasso, Qijing Bian, Sonia M. Kreidenweis, Jack F. Dostalek, Jeremy E. Solbrig, Jennifer Bukowski, Susan C. van den Heever, Yi Wang, Xiaoguang Xu, Jun Wang, Annette L. Walker, Ting-Chi Wu, Milija Zupanski, Christine Chiu, and Jeffrey S. Reid
Atmos. Meas. Tech., 12, 5101–5118, https://doi.org/10.5194/amt-12-5101-2019, https://doi.org/10.5194/amt-12-5101-2019, 2019
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Satellite–based detection of lofted mineral via infrared–window channels, well established in the literature, faces significant challenges in the presence of atmospheric moisture. Here, we consider a case featuring the juxtaposition of two dust plumes embedded within dry and moist air masses. The case is considered from the vantage points of numerical modeling, multi–sensor observations, and radiative transfer theory arriving at a new method for mitigating the water vapor masking effect.
Douglas S. Hamilton, Rachel A. Scanza, Yan Feng, Joseph Guinness, Jasper F. Kok, Longlei Li, Xiaohong Liu, Sagar D. Rathod, Jessica S. Wan, Mingxuan Wu, and Natalie M. Mahowald
Geosci. Model Dev., 12, 3835–3862, https://doi.org/10.5194/gmd-12-3835-2019, https://doi.org/10.5194/gmd-12-3835-2019, 2019
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MIMI v1.0 was designed for use within Earth system models to simulate the 3-D emission, atmospheric processing, and deposition of iron and its soluble fraction. Understanding the iron cycle is important due to its role as an essential micronutrient for ocean phytoplankton; its supply limits primary productivity in many of the world's oceans. Human activity has perturbed the iron cycle, and MIMI is capable of diagnosing many of these impacts; hence, it is important for future climate studies.
Stephen M. Saleeby, Susan C. van den Heever, Jennie Bukowski, Annette L. Walker, Jeremy E. Solbrig, Samuel A. Atwood, Qijing Bian, Sonia M. Kreidenweis, Yi Wang, Jun Wang, and Steven D. Miller
Atmos. Chem. Phys., 19, 10279–10301, https://doi.org/10.5194/acp-19-10279-2019, https://doi.org/10.5194/acp-19-10279-2019, 2019
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This study seeks to understand how intense dust storms impact the heating and cooling of the land surface and atmosphere. Dust storms that are intense enough to substantially impact visibility can also alter how much sunlight reaches the surface during the day and how much heat is trapped in the atmosphere at night. These radiation changes can impact the temperature of the atmosphere and impact the weather in the vicinity.
Jiarui Wu, Naifang Bei, Bo Hu, Suixin Liu, Meng Zhou, Qiyuan Wang, Xia Li, Lang Liu, Tian Feng, Zirui Liu, Yichen Wang, Junji Cao, Xuexi Tie, Jun Wang, Luisa T. Molina, and Guohui Li
Atmos. Chem. Phys., 19, 8703–8719, https://doi.org/10.5194/acp-19-8703-2019, https://doi.org/10.5194/acp-19-8703-2019, 2019
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In the present study, simulations during a persistent and heavy haze pollution episode from 5 December 2015 to 4 January 2016 in the North China Plain (NCP) were performed using the WRF-Chem model to comprehensively quantify contributions of the aerosol shortwave radiative feedback (ARF) to near-surface PM2.5 mass concentrations. During the episode, the ARF deteriorates the haze pollution, increasing the near-surface PM2.5 concentration in the NCP by 10.2 μg m−3 (7.8 %) on average.
Jiarui Wu, Naifang Bei, Bo Hu, Suixin Liu, Meng Zhou, Qiyuan Wang, Xia Li, Lang Liu, Tian Feng, Zirui Liu, Yichen Wang, Junji Cao, Xuexi Tie, Jun Wang, Luisa T. Molina, and Guohui Li
Atmos. Chem. Phys., 19, 8721–8739, https://doi.org/10.5194/acp-19-8721-2019, https://doi.org/10.5194/acp-19-8721-2019, 2019
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The near-surface PM2.5 contribution of the ALW total effect is 17.5 % in NCP, indicating that ALW plays an important role in the PM2.5 formation during the wintertime haze pollution. Moreover, the ALW-HET overwhelmingly dominates the PM2.5 enhancement due to the ALW. The ALW does not consistently enhance near-surface [PM2.5] with increasing RH. When the RH exceeds 80 %, the contribution of the ALW begins to decrease, which is caused by the high occurrence frequencies of precipitation.
George S. Fanourgakis, Maria Kanakidou, Athanasios Nenes, Susanne E. Bauer, Tommi Bergman, Ken S. Carslaw, Alf Grini, Douglas S. Hamilton, Jill S. Johnson, Vlassis A. Karydis, Alf Kirkevåg, John K. Kodros, Ulrike Lohmann, Gan Luo, Risto Makkonen, Hitoshi Matsui, David Neubauer, Jeffrey R. Pierce, Julia Schmale, Philip Stier, Kostas Tsigaridis, Twan van Noije, Hailong Wang, Duncan Watson-Parris, Daniel M. Westervelt, Yang Yang, Masaru Yoshioka, Nikos Daskalakis, Stefano Decesari, Martin Gysel-Beer, Nikos Kalivitis, Xiaohong Liu, Natalie M. Mahowald, Stelios Myriokefalitakis, Roland Schrödner, Maria Sfakianaki, Alexandra P. Tsimpidi, Mingxuan Wu, and Fangqun Yu
Atmos. Chem. Phys., 19, 8591–8617, https://doi.org/10.5194/acp-19-8591-2019, https://doi.org/10.5194/acp-19-8591-2019, 2019
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Effects of aerosols on clouds are important for climate studies but are among the largest uncertainties in climate projections. This study evaluates the skill of global models to simulate aerosol, cloud condensation nuclei (CCN) and cloud droplet number concentrations (CDNCs). Model results show reduced spread in CDNC compared to CCN due to the negative correlation between the sensitivities of CDNC to aerosol number concentration (air pollution) and updraft velocity (atmospheric dynamics).
Xiao Lu, Lin Zhang, Youfan Chen, Mi Zhou, Bo Zheng, Ke Li, Yiming Liu, Jintai Lin, Tzung-May Fu, and Qiang Zhang
Atmos. Chem. Phys., 19, 8339–8361, https://doi.org/10.5194/acp-19-8339-2019, https://doi.org/10.5194/acp-19-8339-2019, 2019
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Severe and deteriorating surface ozone pollution over major Chinese cities has become an emerging environmental concern in China. This study assesses the source contributions (including anthropogenic, background, and individual natural sources) and meteorological influences of surface ozone over China in 2016–2017 using the GEOS-Chem chemical transport model at high horizontal resolution with the most up-to-date Chinese anthropogenic emission inventory.
Xiaoguang Xu, Jun Wang, Yi Wang, Jing Zeng, Omar Torres, Jeffrey S. Reid, Steven D. Miller, J. Vanderlei Martins, and Lorraine A. Remer
Atmos. Meas. Tech., 12, 3269–3288, https://doi.org/10.5194/amt-12-3269-2019, https://doi.org/10.5194/amt-12-3269-2019, 2019
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Detecting aerosol layer height from space is challenging. The traditional method relies on active sensors such as lidar that provide the detailed vertical structure of the aerosol profile but is costly with limited spatial coverage (more than 1 year is needed for global coverage). Here we developed a passive remote sensing technique that uses backscattered sunlight to retrieve smoke aerosol layer height over both water and vegetated surfaces from a sensor 1.5 million kilometers from the Earth.
Jingyuan Shao, Qianjie Chen, Yuxuan Wang, Xiao Lu, Pengzhen He, Yele Sun, Viral Shah, Randall V. Martin, Sajeev Philip, Shaojie Song, Yue Zhao, Zhouqing Xie, Lin Zhang, and Becky Alexander
Atmos. Chem. Phys., 19, 6107–6123, https://doi.org/10.5194/acp-19-6107-2019, https://doi.org/10.5194/acp-19-6107-2019, 2019
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Sulfate is a key species contributing to particle formation and growth during wintertime Chinese haze events. This study combines observations and modeling of oxygen isotope signatures in sulfate aerosol to investigate its formation mechanisms, with a focus on heterogeneous production on aerosol surface via H2O2, O3, and NO2 and trace metal catalyzed oxidation. Contributions from different formation pathways are presented.
Zhenying Xu, Mingxu Liu, Minsi Zhang, Yu Song, Shuxiao Wang, Lin Zhang, Tingting Xu, Tiantian Wang, Caiqing Yan, Tian Zhou, Yele Sun, Yuepeng Pan, Min Hu, Mei Zheng, and Tong Zhu
Atmos. Chem. Phys., 19, 5605–5613, https://doi.org/10.5194/acp-19-5605-2019, https://doi.org/10.5194/acp-19-5605-2019, 2019
Tongwen Wu, Yixiong Lu, Yongjie Fang, Xiaoge Xin, Laurent Li, Weiping Li, Weihua Jie, Jie Zhang, Yiming Liu, Li Zhang, Fang Zhang, Yanwu Zhang, Fanghua Wu, Jianglong Li, Min Chu, Zaizhi Wang, Xueli Shi, Xiangwen Liu, Min Wei, Anning Huang, Yaocun Zhang, and Xiaohong Liu
Geosci. Model Dev., 12, 1573–1600, https://doi.org/10.5194/gmd-12-1573-2019, https://doi.org/10.5194/gmd-12-1573-2019, 2019
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This work presents advancements of the BCC model transition from CMIP5 to CMIP6, especially in the model resolution and its physics. Compared with BCC CMIP5 models, the BCC CMIP6 model shows significant improvements in historical simulations in many aspects including tropospheric air temperature and circulation at global and regional scales in East Asia, climate variability at different timescales (QBO, MJO, and diurnal cycle of precipitation), and the long-term trend of global air temperature.
Huanxin Zhang, Jun Wang, Lorena Castro García, Jing Zeng, Connor Dennhardt, Yang Liu, and Nickolay A. Krotkov
Atmos. Chem. Phys., 19, 2165–2181, https://doi.org/10.5194/acp-19-2165-2019, https://doi.org/10.5194/acp-19-2165-2019, 2019
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OMU-based surface erythemal UV irradiance is compared with ground observations in the United States from 2005 to 2017. We reveal that the assumption of constant atmospheric conditions between OMI overpass time and local solar noon time may not fully represent the real atmosphere and the peaks of surface UV are not always at local solar noon because of cloud effects. Future geostationary satellites (e.g., TEMPO) would reduce sampling bias and improve trend analysis of surface UV estimate.
Sophie Bastin, Philippe Drobinski, Marjolaine Chiriaco, Olivier Bock, Romain Roehrig, Clemente Gallardo, Dario Conte, Marta Domínguez Alonso, Laurent Li, Piero Lionello, and Ana C. Parracho
Atmos. Chem. Phys., 19, 1471–1490, https://doi.org/10.5194/acp-19-1471-2019, https://doi.org/10.5194/acp-19-1471-2019, 2019
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This paper uses colocated observations of temperature, precipitation and humidity to investigate the triggering of precipitation. It shows that there is a critical value of humidity above which precipitation picks up. This critical value depends on T and varies spatially. It also analyses how this dependency is reproduced in regional climate simulations over Europe. Models with too little and too light precipitation have both lower critical value of humidity and higher probability to exceed it.
Julien Beaumet, Gerhard Krinner, Michel Déqué, Rein Haarsma, and Laurent Li
Geosci. Model Dev., 12, 321–342, https://doi.org/10.5194/gmd-12-321-2019, https://doi.org/10.5194/gmd-12-321-2019, 2019
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Oceanic surface conditions coming from coupled ocean–atmosphere global climate models bear considerable biases over the historical climate. We review and present new methods for bias correcting sea surface temperatures and sea-ice concentration coming from such models in order to use them as boundary conditions for atmospheric-only GCMs. For sea ice, we propose a new analogue method which allows us to reproduce more physically consistent future bias-corrected sea-ice concentration maps.
Milija Zupanski, Anton Kliewer, Ting-Chi Wu, Karina Apodaca, Qijing Bian, Sam Atwood, Yi Wang, Jun Wang, and Steven D. Miller
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2019-2, https://doi.org/10.5194/acp-2019-2, 2019
Revised manuscript not accepted
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The problem of under-observed aerosol observations and in particular the vertical distribution of aerosols is addressed using a strongly coupled atmosphere-aerosol data assimilation system. In the strongly coupled system the atmospheric observations, which are more numerous in general, can impact the aerosol initial conditions. In an application over a coastal zone, results indicate that atmospheric observations have a positive impact on aerosols.
Mingxu Liu, Xin Huang, Yu Song, Tingting Xu, Shuxiao Wang, Zhijun Wu, Min Hu, Lin Zhang, Qiang Zhang, Yuepeng Pan, Xuejun Liu, and Tong Zhu
Atmos. Chem. Phys., 18, 17933–17943, https://doi.org/10.5194/acp-18-17933-2018, https://doi.org/10.5194/acp-18-17933-2018, 2018
Ting-Chi Wu, Milija Zupanski, Stephen Saleeby, Anton Kliewer, Lewis Grasso, Qijing Bian, Samuel A. Atwood, Yi Wang, and Jun Wang
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2018-1249, https://doi.org/10.5194/acp-2018-1249, 2018
Revised manuscript not accepted
Hunter Brown, Xiaohong Liu, Yan Feng, Yiquan Jiang, Mingxuan Wu, Zheng Lu, Chenglai Wu, Shane Murphy, and Rudra Pokhrel
Atmos. Chem. Phys., 18, 17745–17768, https://doi.org/10.5194/acp-18-17745-2018, https://doi.org/10.5194/acp-18-17745-2018, 2018
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In climate models, organic carbon (OC) in wildfire smoke has been treated as an atmospheric cooling component by reflecting sunlight back to space. This study incorporates the observationally identified absorbing brown carbon component of OC into the Community Earth System Model, improving the agreement between the model and observations and effectively increasing absorption of solar radiation. This change contributes to altered atmospheric dynamics and changes in cloud cover in the model.
Shan Li, Laurent Li, and Hervé Le Treut
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2018-257, https://doi.org/10.5194/gmd-2018-257, 2018
Preprint withdrawn
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Newtonian relaxation allowing RCM (regional climate model) to follow GCM (global climate model) is a widely-used technique for climate downscaling and regional weather forecasting. It is thoroughly assessed in an idealized framework for both synoptic variability and long-term mean climate. LMDz is a GCM, but it can be configured as a RCM. It thus acts as both GCM and RCM. The experimental set-up “Master versus Slave” considers GCM as the reference to assess behaviors of RCM.
Yangyang Zhang, Aohan Tang, Dandan Wang, Qingqing Wang, Katie Benedict, Lin Zhang, Duanyang Liu, Yi Li, Jeffrey L. Collett Jr., Yele Sun, and Xuejun Liu
Atmos. Chem. Phys., 18, 16385–16398, https://doi.org/10.5194/acp-18-16385-2018, https://doi.org/10.5194/acp-18-16385-2018, 2018
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Our study is the first to continually monitor the vertical concentration profile of NH3 in urban Beijing. Weekly concentrations averaged 13.3 ± 4.8 μg m−3. The highest NH3 concentrations were always observed between 32 and 63 m, decreasing toward the surface and toward higher altitudes. Our results demonstrate a NH3 rich atmosphere in urban Beijing, from the ground to at least 320 m. Regional transport from the south (intensive agricultural regions) contributed high NH3 concentrations in Beijing.
Anton Kliewer, Milija Zupanski, Qijing Bian, Sam Atwood, Yi Wang, and Jun Wang
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2018-1156, https://doi.org/10.5194/acp-2018-1156, 2018
Revised manuscript not accepted
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This research is focused on improving numerical weather prediction by including data regarding aerosols in the atmosphere. Using weather prediction models along with data assimilation (the process of marrying observations with a model prediction), a better representation of the atmosphere can be described. As no model or observational platform is ever perfect, the aerosol observations have to be de-biased (adjusting for systematic error). Here we look at two such methods.
Benjamin S. Grandey, Daniel Rothenberg, Alexander Avramov, Qinjian Jin, Hsiang-He Lee, Xiaohong Liu, Zheng Lu, Samuel Albani, and Chien Wang
Atmos. Chem. Phys., 18, 15783–15810, https://doi.org/10.5194/acp-18-15783-2018, https://doi.org/10.5194/acp-18-15783-2018, 2018
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Anthropogenic emissions of aerosol particles likely cool the climate system. We investigate the uncertainty in the strength of the cooling effect by exploring the representation of aerosols in a global climate model. We conclude that the specific representation of aerosols in global climate models has important implications for climate modelling. Important factors include the representation of aerosol mixing state, size distribution, and optical properties.
Elizabeth M. Lennartson, Jun Wang, Juping Gu, Lorena Castro Garcia, Cui Ge, Meng Gao, Myungje Choi, Pablo E. Saide, Gregory R. Carmichael, Jhoon Kim, and Scott J. Janz
Atmos. Chem. Phys., 18, 15125–15144, https://doi.org/10.5194/acp-18-15125-2018, https://doi.org/10.5194/acp-18-15125-2018, 2018
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This paper is among the first to study the diurnal variations of AOD, PM2.5, and their relationships in South Korea. We show that the PM2.5–AOD relationship has strong diurnal variations, and, hence, using AOD data retrieved from geostationary satellite can improve the monitoring of surface PM2.5 air quality on a daily basis as well as constrain the diurnal variation of aerosol emission.
Hansen Cao, Tzung-May Fu, Lin Zhang, Daven K. Henze, Christopher Chan Miller, Christophe Lerot, Gonzalo González Abad, Isabelle De Smedt, Qiang Zhang, Michel van Roozendael, François Hendrick, Kelly Chance, Jie Li, Junyu Zheng, and Yuanhong Zhao
Atmos. Chem. Phys., 18, 15017–15046, https://doi.org/10.5194/acp-18-15017-2018, https://doi.org/10.5194/acp-18-15017-2018, 2018
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Our top-down estimates for annual total Chinese NMVOC emissions was 30.7 to 49.5 Tg y−1, including 16.4 to 23.6 Tg y−1 from anthropogenic sources, 12.2 to 22.8 Tg y−1 from biogenic sources, and 2.08 to 3.13 Tg y−1 from biomass burning. Our four inversions consistently showed that the emissions of Chinese anthropogenic NMVOC precursors of glyoxal were larger than the a priori estimates. The glyoxal and formaldehyde constraints helped distinguish the NMVOC species from different sources.
Alf Kirkevåg, Alf Grini, Dirk Olivié, Øyvind Seland, Kari Alterskjær, Matthias Hummel, Inger H. H. Karset, Anna Lewinschal, Xiaohong Liu, Risto Makkonen, Ingo Bethke, Jan Griesfeller, Michael Schulz, and Trond Iversen
Geosci. Model Dev., 11, 3945–3982, https://doi.org/10.5194/gmd-11-3945-2018, https://doi.org/10.5194/gmd-11-3945-2018, 2018
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A new aerosol treatment is described and tested in a global climate model. With updated emissions, aerosol chemistry, and microphysics compared to its predecessor, black carbon (BC) mass concentrations aloft better fit observations, surface concentrations of BC and sea salt are less biased, and sulfate and mineral dust slightly more, while the results for organics are inconclusive. Man-made aerosols now yield a stronger cooling effect on climate that is strong compared to results from IPCC.
Wen Xu, Lei Liu, Miaomiao Cheng, Yuanhong Zhao, Lin Zhang, Yuepeng Pan, Xiuming Zhang, Baojing Gu, Yi Li, Xiuying Zhang, Jianlin Shen, Li Lu, Xiaosheng Luo, Yu Zhao, Zhaozhong Feng, Jeffrey L. Collett Jr., Fusuo Zhang, and Xuejun Liu
Atmos. Chem. Phys., 18, 10931–10954, https://doi.org/10.5194/acp-18-10931-2018, https://doi.org/10.5194/acp-18-10931-2018, 2018
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Our main results demonstrate that atmospheric Nr pollution in eastern China is more serious in the northern region than in the southern region. Any effects of current emission controls are not yet apparent in Nr pollution. NH3 emissions from fertilizer use were the largest contributor (36 %) to total inorganic Nr deposition. Our results provide useful information for policy-makers that mitigation of NH3 emissions should be a priority to tackle serious N deposition.
Nan Li, Qingyang He, Jim Greenberg, Alex Guenther, Jingyi Li, Junji Cao, Jun Wang, Hong Liao, Qiyuan Wang, and Qiang Zhang
Atmos. Chem. Phys., 18, 7489–7507, https://doi.org/10.5194/acp-18-7489-2018, https://doi.org/10.5194/acp-18-7489-2018, 2018
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O3 pollution has been increasing in most Chinese cities in recent years. Our study reveals that the synergistic impact of individual source contributions to O3 formation should be considered in the formation of air pollution control strategies, especially for big cities in the vicinity of forests.
Jennifer Kaiser, Daniel J. Jacob, Lei Zhu, Katherine R. Travis, Jenny A. Fisher, Gonzalo González Abad, Lin Zhang, Xuesong Zhang, Alan Fried, John D. Crounse, Jason M. St. Clair, and Armin Wisthaler
Atmos. Chem. Phys., 18, 5483–5497, https://doi.org/10.5194/acp-18-5483-2018, https://doi.org/10.5194/acp-18-5483-2018, 2018
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Isoprene emissions from vegetation have a large effect on atmospheric chemistry and air quality. Here we use the adjoint of GEOS-Chem in an inversion of OMI formaldehyde observations to produce top-down estimates of isoprene emissions in the southeast US during the summer of 2013. We find that MEGAN v2.1 is biased high on average by 40 %. Our downward correction of isoprene emissions leads to a small reduction in modeled surface O3 and decreases the contribution of isoprene to organic aerosol.
Xiao Lu, Lin Zhang, Xiong Liu, Meng Gao, Yuanhong Zhao, and Jingyuan Shao
Atmos. Chem. Phys., 18, 3101–3118, https://doi.org/10.5194/acp-18-3101-2018, https://doi.org/10.5194/acp-18-3101-2018, 2018
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Deteriorating tropospheric ozone pollution over India may not only affect local human health and vegetation but also perturb global ozone distribution. This study analyzes the processes controlling lower tropospheric ozone over India using OMI satellite observations (2006–2014) and model simulations (1990–2010). We show that the South Asian monsoon largely controls the seasonal cycle and interannual variability of Indian lower tropospheric ozone via changes in ozone production and transport.
Tianyi Fan, Xiaohong Liu, Po-Lun Ma, Qiang Zhang, Zhanqing Li, Yiquan Jiang, Fang Zhang, Chuanfeng Zhao, Xin Yang, Fang Wu, and Yuying Wang
Atmos. Chem. Phys., 18, 1395–1417, https://doi.org/10.5194/acp-18-1395-2018, https://doi.org/10.5194/acp-18-1395-2018, 2018
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We found that 22–28 % of the low AOD bias in eastern China simulated by the Community Atmosphere Model version 5 can be improved by using a new emission inventory. The concentrations of primary aerosols are closely related to the emission, while the seasonal variations of secondary aerosols depend more on atmospheric processes. This study highlights the importance of improving both the emission and atmospheric processes in modeling the atmospheric aerosols and their radiative effects.
Bin Zhao, Kuo-Nan Liou, Yu Gu, Jonathan H. Jiang, Qinbin Li, Rong Fu, Lei Huang, Xiaohong Liu, Xiangjun Shi, Hui Su, and Cenlin He
Atmos. Chem. Phys., 18, 1065–1078, https://doi.org/10.5194/acp-18-1065-2018, https://doi.org/10.5194/acp-18-1065-2018, 2018
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The interactions between aerosols and ice clouds represent one of the largest uncertainties among anthropogenic forcings on climate change. We find that the responses of ice crystal effective radius, a key parameter determining ice clouds' net radiative effect, to aerosol loadings are modulated by water vapor amount and vary from a significant negative correlation in moist conditions (consistent with the “Twomey effect” for liquid clouds) to a strong positive correlation in dry conditions.
Chenglai Wu, Xiaohong Liu, Zhaohui Lin, Stefan R. Rahimi-Esfarjani, and Zheng Lu
Atmos. Chem. Phys., 18, 511–533, https://doi.org/10.5194/acp-18-511-2018, https://doi.org/10.5194/acp-18-511-2018, 2018
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This study utilizes the newly developed variable-resolution Community Earth System Model (VR-CESM) with a refined high resolution (0.125º) to quantify the impacts of absorbing aerosol (BC and dust) deposition on snowpack and hydrologic cycles in the Rocky Mountains. BC and dust in snow significantly reduce the snowpack around the mountains. BC and dust in snow also accelerate the hydrologic cycles in the mountainous regions, with runoff increased in spring but reduced in summer.
Lin Zhang, Youfan Chen, Yuanhong Zhao, Daven K. Henze, Liye Zhu, Yu Song, Fabien Paulot, Xuejun Liu, Yuepeng Pan, Yi Lin, and Binxiang Huang
Atmos. Chem. Phys., 18, 339–355, https://doi.org/10.5194/acp-18-339-2018, https://doi.org/10.5194/acp-18-339-2018, 2018
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Substantial differences exist in current estimates of agricultural ammonia emissions in China, hindering understanding of their environmental consequences. This study applies both bottom-up and top-down methods to better quantify agricultural ammonia sources in China using observations from satellite and surface networks interpreted by a chemical transport model. Our estimate of annual Chinese anthropogenic ammonia emission is 11.7 tg (teragram) for 2008 with a strong seasonality peak in summer.
Yawen Liu, Kai Zhang, Yun Qian, Yuhang Wang, Yufei Zou, Yongjia Song, Hui Wan, Xiaohong Liu, and Xiu-Qun Yang
Atmos. Chem. Phys., 18, 31–47, https://doi.org/10.5194/acp-18-31-2018, https://doi.org/10.5194/acp-18-31-2018, 2018
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Fire aerosols have large impact on weather and climate through their effect on clouds and radiation, but it is difficult to quantify. Here we investigated the short-term effective radiative forcing of fire aerosols using the nudged hindcast ensemble simulations from global aerosol-climate model. Results show large effects of fire aerosols on both liquid and ice cloud and large ensemble spread of regional mean shortwave cloud radiative forcing over southern Mexico and the central US.
Yuxuan Wang, Yuanyu Xie, Wenhao Dong, Yi Ming, Jun Wang, and Lu Shen
Atmos. Chem. Phys., 17, 12827–12843, https://doi.org/10.5194/acp-17-12827-2017, https://doi.org/10.5194/acp-17-12827-2017, 2017
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Besides the well-known large impact on agriculture and water resources, drought is associated with significant adverse effects on air quality. Drought-induced degradation of air quality is largely due to natural processes, offsetting the effort of anthropogenic emission reduction during the past decades. Such adverse impacts should be included in modeling processes under current and future climate for mitigation policy.
Maria Sand, Bjørn H. Samset, Yves Balkanski, Susanne Bauer, Nicolas Bellouin, Terje K. Berntsen, Huisheng Bian, Mian Chin, Thomas Diehl, Richard Easter, Steven J. Ghan, Trond Iversen, Alf Kirkevåg, Jean-François Lamarque, Guangxing Lin, Xiaohong Liu, Gan Luo, Gunnar Myhre, Twan van Noije, Joyce E. Penner, Michael Schulz, Øyvind Seland, Ragnhild B. Skeie, Philip Stier, Toshihiko Takemura, Kostas Tsigaridis, Fangqun Yu, Kai Zhang, and Hua Zhang
Atmos. Chem. Phys., 17, 12197–12218, https://doi.org/10.5194/acp-17-12197-2017, https://doi.org/10.5194/acp-17-12197-2017, 2017
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The role of aerosols in the changing polar climate is not well understood and the aerosols are poorly constrained in the models. In this study we have compared output from 16 different aerosol models with available observations at both poles. We show that the model median is representative of the observations, but the model spread is large. The Arctic direct aerosol radiative effect over the industrial area is positive during spring due to black carbon and negative during summer due to sulfate.
Hongyan Zhao, Xin Li, Qiang Zhang, Xujia Jiang, Jintai Lin, Glen P. Peters, Meng Li, Guannan Geng, Bo Zheng, Hong Huo, Lin Zhang, Haikun Wang, Steven J. Davis, and Kebin He
Atmos. Chem. Phys., 17, 10367–10381, https://doi.org/10.5194/acp-17-10367-2017, https://doi.org/10.5194/acp-17-10367-2017, 2017
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Effective and efficient control of air pollution relies upon an understanding of the pollution sources. We conduct an interdisciplinary study and find that 33 % of China’s PM2.5-related premature mortality in 2010 were caused by production emission in other regions; 56 % of the mortality was related to consumption in other regions. Multilateral and multi-stage cooperation under a regional sustainable development framework is in urgent need to mitigate air pollution and related health impacts.
Yuanhong Zhao, Lin Zhang, Amos P. K. Tai, Youfan Chen, and Yuepeng Pan
Atmos. Chem. Phys., 17, 9781–9796, https://doi.org/10.5194/acp-17-9781-2017, https://doi.org/10.5194/acp-17-9781-2017, 2017
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Human activities have substantially enhanced atmospheric deposition of reactive nitrogen, inducing complex environmental consequences. This study presents a first quantitative investigation of how anthropogenic nitrogen deposition could impact surface ozone air quality through surface–atmosphere exchange processes. We find important surface ozone changes driven by nitrogen deposition, which can be comparable with those due to historical climate and land use changes.
Chenglai Wu, Xiaohong Liu, Minghui Diao, Kai Zhang, Andrew Gettelman, Zheng Lu, Joyce E. Penner, and Zhaohui Lin
Atmos. Chem. Phys., 17, 4731–4749, https://doi.org/10.5194/acp-17-4731-2017, https://doi.org/10.5194/acp-17-4731-2017, 2017
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This study utilizes a novel approach to directly compare the CAM5-simulated cloud macro- and microphysics with the collocated HIPPO observations for the period of 2009 to 2011. The model cannot capture the large spatial variabilities of observed RH, which is responsible for much of the model missing low-level warm clouds. A large portion of the RH bias results from the discrepancy in water vapor. The model underestimates the observed number concentration and ice water content.
Wen Xu, Wei Song, Yangyang Zhang, Xuejun Liu, Lin Zhang, Yuanhong Zhao, Duanyang Liu, Aohan Tang, Daowei Yang, Dandan Wang, Zhang Wen, Yuepeng Pan, David Fowler, Jeffrey L. Collett Jr., Jan Willem Erisman, Keith Goulding, Yi Li, and Fusuo Zhang
Atmos. Chem. Phys., 17, 31–46, https://doi.org/10.5194/acp-17-31-2017, https://doi.org/10.5194/acp-17-31-2017, 2017
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This paper evaluates the effectiveness of emission control measures implemented in Beijing during the Parade Blue period by integrating our own results, official-released data and modeling data. We demonstrate that emission control measures make a major contribution to air quality improvement in Beijing and surrounding regions. We conclude a joint local and regional control of secondary aerosol precursors to be key to curbing air pollution in Beijing.
Yiquan Jiang, Zheng Lu, Xiaohong Liu, Yun Qian, Kai Zhang, Yuhang Wang, and Xiu-Qun Yang
Atmos. Chem. Phys., 16, 14805–14824, https://doi.org/10.5194/acp-16-14805-2016, https://doi.org/10.5194/acp-16-14805-2016, 2016
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Aerosols from open fires could significantly perturb the global radiation balance and induce climate change. In this study, the CAM5 global climate model is used to investigate the spatial and seasonal characteristics of radiative effects due to fire aerosol–radiation interactions, fire aerosol-cloud interactions and fire aerosol-surface albedo interactions, including radiative effects from all fire aerosols, fire black carbon and fire particulate organic matter.
Xiao Lu, Lin Zhang, Xu Yue, Jiachen Zhang, Daniel A. Jaffe, Andreas Stohl, Yuanhong Zhao, and Jingyuan Shao
Atmos. Chem. Phys., 16, 14687–14702, https://doi.org/10.5194/acp-16-14687-2016, https://doi.org/10.5194/acp-16-14687-2016, 2016
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Increasing wildfire activities in the mountainous western US may present a challenge for the region to attain a recently revised ozone air quality standard in summer. We quantify the wildfire influence on the ozone variability, trends, and number of high ozone days over this region in summers 1989–2010 using a Lagrangian dispersion model and statistical regression models.
Cheng Zhou, Joyce E. Penner, Guangxing Lin, Xiaohong Liu, and Minghuai Wang
Atmos. Chem. Phys., 16, 12411–12424, https://doi.org/10.5194/acp-16-12411-2016, https://doi.org/10.5194/acp-16-12411-2016, 2016
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We examined the different ice nucleation parameterization factors that affect the simulated ice number concentrations in cirrus clouds in the upper troposphere using the CAM5 model. We examined the effect from three different updraft velocities (from low to high), two different water vapour accommodation coefficients (α = 0.1 or 1), the effect of including vapour deposition onto pre-existing ice particles during ice nucleation, and the effect of including SOA as heterogeneous ice nuclei.
Shouguo Ding, Jun Wang, and Xiaoguang Xu
Atmos. Meas. Tech., 9, 2077–2092, https://doi.org/10.5194/amt-9-2077-2016, https://doi.org/10.5194/amt-9-2077-2016, 2016
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Knowledge on the vertical distribution of aerosols in the atmospheric is important for studying aerosol impacts on air quality and climate change. The polarization measurements in O2 A and B bands is shown here theoretically to have rich information for characterizing aerosol vertical profile over land. This paper presents a passive remote sensing technique supplementary to the existing technique to retrieve aerosol vertical distribution over land from space.
N. I. Kristiansen, A. Stohl, D. J. L. Olivié, B. Croft, O. A. Søvde, H. Klein, T. Christoudias, D. Kunkel, S. J. Leadbetter, Y. H. Lee, K. Zhang, K. Tsigaridis, T. Bergman, N. Evangeliou, H. Wang, P.-L. Ma, R. C. Easter, P. J. Rasch, X. Liu, G. Pitari, G. Di Genova, S. Y. Zhao, Y. Balkanski, S. E. Bauer, G. S. Faluvegi, H. Kokkola, R. V. Martin, J. R. Pierce, M. Schulz, D. Shindell, H. Tost, and H. Zhang
Atmos. Chem. Phys., 16, 3525–3561, https://doi.org/10.5194/acp-16-3525-2016, https://doi.org/10.5194/acp-16-3525-2016, 2016
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Processes affecting aerosol removal from the atmosphere are not fully understood. In this study we investigate to what extent atmospheric transport models can reproduce observed loss of aerosols. We compare measurements of radioactive isotopes, that attached to ambient sulfate aerosols during the 2011 Fukushima nuclear accident, to 19 models using identical emissions. Results indicate aerosol removal that is too fast in most models, and apply to aerosols that have undergone long-range transport.
Zak Kipling, Philip Stier, Colin E. Johnson, Graham W. Mann, Nicolas Bellouin, Susanne E. Bauer, Tommi Bergman, Mian Chin, Thomas Diehl, Steven J. Ghan, Trond Iversen, Alf Kirkevåg, Harri Kokkola, Xiaohong Liu, Gan Luo, Twan van Noije, Kirsty J. Pringle, Knut von Salzen, Michael Schulz, Øyvind Seland, Ragnhild B. Skeie, Toshihiko Takemura, Kostas Tsigaridis, and Kai Zhang
Atmos. Chem. Phys., 16, 2221–2241, https://doi.org/10.5194/acp-16-2221-2016, https://doi.org/10.5194/acp-16-2221-2016, 2016
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The vertical distribution of atmospheric aerosol is an important factor in its effects on climate. In this study we use a sophisticated model of the many interacting processes affecting aerosol in the atmosphere to show that the vertical distribution is typically dominated by only a few of these processes. Constraining these physical processes may help to reduce the large differences between models. However, the important processes are not always the same for different types of aerosol.
Kai Zhang, Chun Zhao, Hui Wan, Yun Qian, Richard C. Easter, Steven J. Ghan, Koichi Sakaguchi, and Xiaohong Liu
Geosci. Model Dev., 9, 607–632, https://doi.org/10.5194/gmd-9-607-2016, https://doi.org/10.5194/gmd-9-607-2016, 2016
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A sub-grid treatment based on Weibull distribution is introduced to CAM5 to take into account the impact of unresolved variability of surface wind speed on sea salt and dust emissions. Simulations show that sub-grid wind variability has relatively small impacts on the global mean sea salt emissions, but considerable influence on dust emissions. Dry convective eddies and mesoscale flows associated with complex topography are the major causes of dust emission enhancement.
X. Liu, P.-L. Ma, H. Wang, S. Tilmes, B. Singh, R. C. Easter, S. J. Ghan, and P. J. Rasch
Geosci. Model Dev., 9, 505–522, https://doi.org/10.5194/gmd-9-505-2016, https://doi.org/10.5194/gmd-9-505-2016, 2016
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In this study, we describe and evaluate a new four-mode version of the Modal Aerosol Module (MAM4) in the Community Atmosphere Model version 5 (CAM5). Compared to the current three-mode version of MAM in CAM5, MAM4 significantly improves the simulation of seasonal variation of BC concentrations in the polar regions, by increasing the BC concentrations in all seasons and particularly in cold seasons.
W. Xu, X. S. Luo, Y. P. Pan, L. Zhang, A. H. Tang, J. L. Shen, Y. Zhang, K. H. Li, Q. H. Wu, D. W. Yang, Y. Y. Zhang, J. Xue, W. Q. Li, Q. Q. Li, L. Tang, S. H. Lu, T. Liang, Y. A. Tong, P. Liu, Q. Zhang, Z. Q. Xiong, X. J. Shi, L. H. Wu, W. Q. Shi, K. Tian, X. H. Zhong, K. Shi, Q. Y. Tang, L. J. Zhang, J. L. Huang, C. E. He, F. H. Kuang, B. Zhu, H. Liu, X. Jin, Y. J. Xin, X. K. Shi, E. Z. Du, A. J. Dore, S. Tang, J. L. Collett Jr., K. Goulding, Y. X. Sun, J. Ren, F. S. Zhang, and X. J. Liu
Atmos. Chem. Phys., 15, 12345–12360, https://doi.org/10.5194/acp-15-12345-2015, https://doi.org/10.5194/acp-15-12345-2015, 2015
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The annual average concentrations (1.3-47.0µg N m-3) and dry plus wet/bulk deposition fluxes (2.9-83.3kg N ha-1 yr-1) of inorganic Nr species ranked by land use as urban > rural > background sites and by regions as north China > southeast China > southwest China > northeast China > northwest China > Tibetan Plateau, reflecting the impact of anthropogenic Nr emission. Average dry and wet/bulk N deposition fluxes were 20.6 ± 11.2 and 19.3 ± 9.2kg kg N ha-1 yr-1 across China, respectively.
Y. Zhao, L. Zhang, Y. Pan, Y. Wang, F. Paulot, and D. K. Henze
Atmos. Chem. Phys., 15, 10905–10924, https://doi.org/10.5194/acp-15-10905-2015, https://doi.org/10.5194/acp-15-10905-2015, 2015
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Rapid Asian industrialization has led to increased atmospheric nitrogen deposition downwind. This work analyzes the sources and processes controlling atmospheric nitrogen deposition to the northwestern Pacific. Both nitrogen emissions and meteorology, largely controlled by the East Asian Monsoon, determine the seasonality of nitrogen deposition. Ascribing deposition over the marginal seas to nitrogen sources from different regions and sectors shows important contribution from fertilizer use.
W. Tao, J. Liu, G. A. Ban-Weiss, D. A. Hauglustaine, L. Zhang, Q. Zhang, Y. Cheng, Y. Yu, and S. Tao
Atmos. Chem. Phys., 15, 8597–8614, https://doi.org/10.5194/acp-15-8597-2015, https://doi.org/10.5194/acp-15-8597-2015, 2015
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We examine the responses of a range of meteorological and air quality indicators to the expansion of urban land using WRF/Chem. Sensitivity studies indicate that the responses of pollutant concentrations to the spatial extent of urbanization are linear near the surface but nonlinear at higher altitudes. The results of process analysis demonstrate that urban heat island circulation and a deeper boundary layer with stronger turbulent intensities play a significant role in relocating pollutants.
S. Tilmes, J.-F. Lamarque, L. K. Emmons, D. E. Kinnison, P.-L. Ma, X. Liu, S. Ghan, C. Bardeen, S. Arnold, M. Deeter, F. Vitt, T. Ryerson, J. W. Elkins, F. Moore, J. R. Spackman, and M. Val Martin
Geosci. Model Dev., 8, 1395–1426, https://doi.org/10.5194/gmd-8-1395-2015, https://doi.org/10.5194/gmd-8-1395-2015, 2015
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The Community Atmosphere Model (CAM), version 5, is now coupled to extensive tropospheric and stratospheric chemistry, called CAM5-chem, and is available in addition to CAM4-chem in the Community Earth System Model (CESM) version 1.2. Both configurations are well suited as tools for atmospheric chemistry modeling studies in the troposphere and lower stratosphere.
X. Shi, X. Liu, and K. Zhang
Atmos. Chem. Phys., 15, 1503–1520, https://doi.org/10.5194/acp-15-1503-2015, https://doi.org/10.5194/acp-15-1503-2015, 2015
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The ice nucleation scheme in the Community Atmosphere Model (CAM5) was improved by considering the effects of pre-existing ice crystals and some other modifications. Subsequently, the comparison between different ice nucleation parameterizations is investigated. Experiment using the ice nucleation parameterization of Kärcher et al. (2006) predicts a much smaller anthropogenic aerosol indirect forcing than that using the parameterizations of Liu and Penner (2005) and Barahona and Nenes (2009).
R. A. Scanza, N. Mahowald, S. Ghan, C. S. Zender, J. F. Kok, X. Liu, Y. Zhang, and S. Albani
Atmos. Chem. Phys., 15, 537–561, https://doi.org/10.5194/acp-15-537-2015, https://doi.org/10.5194/acp-15-537-2015, 2015
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The main purpose of this study was to build a framework in the Community Atmosphere Models version 4 and 5 within the Community Earth System Model to simulate dust aerosols as their component minerals. With this framework, we investigate the direct radiative forcing that results from the mineral speciation. We find that adding mineralogy results in a small positive forcing at the top of the atmosphere, while simulations without mineralogy have a small negative forcing.
Y.-Y. Yan, J.-T. Lin, Y. Kuang, D. Yang, and L. Zhang
Atmos. Chem. Phys., 14, 12649–12663, https://doi.org/10.5194/acp-14-12649-2014, https://doi.org/10.5194/acp-14-12649-2014, 2014
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Limited by coarse resolutions, global chemical transport models cannot well capture small-scale nonlinear processes. To alleviate the problem, we develop a two-way coupled system to integrate the global GEOS-Chem model and its three high-resolution nested models covering Asia, Europe and North America. Confirmed by comparisons with observations, the coupled system improves upon the global model with a 10% increase in global tropospheric CO, a 4% decrease in OH and a 4% increase in MCF lifetime.
S. Yu, R. Mathur, J. Pleim, D. Wong, R. Gilliam, K. Alapaty, C. Zhao, and X. Liu
Atmos. Chem. Phys., 14, 11247–11285, https://doi.org/10.5194/acp-14-11247-2014, https://doi.org/10.5194/acp-14-11247-2014, 2014
K. Tsigaridis, N. Daskalakis, M. Kanakidou, P. J. Adams, P. Artaxo, R. Bahadur, Y. Balkanski, S. E. Bauer, N. Bellouin, A. Benedetti, T. Bergman, T. K. Berntsen, J. P. Beukes, H. Bian, K. S. Carslaw, M. Chin, G. Curci, T. Diehl, R. C. Easter, S. J. Ghan, S. L. Gong, A. Hodzic, C. R. Hoyle, T. Iversen, S. Jathar, J. L. Jimenez, J. W. Kaiser, A. Kirkevåg, D. Koch, H. Kokkola, Y. H Lee, G. Lin, X. Liu, G. Luo, X. Ma, G. W. Mann, N. Mihalopoulos, J.-J. Morcrette, J.-F. Müller, G. Myhre, S. Myriokefalitakis, N. L. Ng, D. O'Donnell, J. E. Penner, L. Pozzoli, K. J. Pringle, L. M. Russell, M. Schulz, J. Sciare, Ø. Seland, D. T. Shindell, S. Sillman, R. B. Skeie, D. Spracklen, T. Stavrakou, S. D. Steenrod, T. Takemura, P. Tiitta, S. Tilmes, H. Tost, T. van Noije, P. G. van Zyl, K. von Salzen, F. Yu, Z. Wang, Z. Wang, R. A. Zaveri, H. Zhang, K. Zhang, Q. Zhang, and X. Zhang
Atmos. Chem. Phys., 14, 10845–10895, https://doi.org/10.5194/acp-14-10845-2014, https://doi.org/10.5194/acp-14-10845-2014, 2014
Y. Wang, X. Liu, C. Hoose, and B. Wang
Atmos. Chem. Phys., 14, 10411–10430, https://doi.org/10.5194/acp-14-10411-2014, https://doi.org/10.5194/acp-14-10411-2014, 2014
K. Zhang, H. Wan, X. Liu, S. J. Ghan, G. J. Kooperman, P.-L. Ma, P. J. Rasch, D. Neubauer, and U. Lohmann
Atmos. Chem. Phys., 14, 8631–8645, https://doi.org/10.5194/acp-14-8631-2014, https://doi.org/10.5194/acp-14-8631-2014, 2014
L. Zhang, D. J. Jacob, X. Yue, N. V. Downey, D. A. Wood, and D. Blewitt
Atmos. Chem. Phys., 14, 5295–5309, https://doi.org/10.5194/acp-14-5295-2014, https://doi.org/10.5194/acp-14-5295-2014, 2014
G. W. Mann, K. S. Carslaw, C. L. Reddington, K. J. Pringle, M. Schulz, A. Asmi, D. V. Spracklen, D. A. Ridley, M. T. Woodhouse, L. A. Lee, K. Zhang, S. J. Ghan, R. C. Easter, X. Liu, P. Stier, Y. H. Lee, P. J. Adams, H. Tost, J. Lelieveld, S. E. Bauer, K. Tsigaridis, T. P. C. van Noije, A. Strunk, E. Vignati, N. Bellouin, M. Dalvi, C. E. Johnson, T. Bergman, H. Kokkola, K. von Salzen, F. Yu, G. Luo, A. Petzold, J. Heintzenberg, A. Clarke, J. A. Ogren, J. Gras, U. Baltensperger, U. Kaminski, S. G. Jennings, C. D. O'Dowd, R. M. Harrison, D. C. S. Beddows, M. Kulmala, Y. Viisanen, V. Ulevicius, N. Mihalopoulos, V. Zdimal, M. Fiebig, H.-C. Hansson, E. Swietlicki, and J. S. Henzing
Atmos. Chem. Phys., 14, 4679–4713, https://doi.org/10.5194/acp-14-4679-2014, https://doi.org/10.5194/acp-14-4679-2014, 2014
P.-L. Ma, P. J. Rasch, J. D. Fast, R. C. Easter, W. I. Gustafson Jr., X. Liu, S. J. Ghan, and B. Singh
Geosci. Model Dev., 7, 755–778, https://doi.org/10.5194/gmd-7-755-2014, https://doi.org/10.5194/gmd-7-755-2014, 2014
K. E. O. Todd-Brown, J. T. Randerson, F. Hopkins, V. Arora, T. Hajima, C. Jones, E. Shevliakova, J. Tjiputra, E. Volodin, T. Wu, Q. Zhang, and S. D. Allison
Biogeosciences, 11, 2341–2356, https://doi.org/10.5194/bg-11-2341-2014, https://doi.org/10.5194/bg-11-2341-2014, 2014
M. S. Long, W. C. Keene, R. C. Easter, R. Sander, X. Liu, A. Kerkweg, and D. Erickson
Atmos. Chem. Phys., 14, 3397–3425, https://doi.org/10.5194/acp-14-3397-2014, https://doi.org/10.5194/acp-14-3397-2014, 2014
G. C. M. Vinken, K. F. Boersma, A. van Donkelaar, and L. Zhang
Atmos. Chem. Phys., 14, 1353–1369, https://doi.org/10.5194/acp-14-1353-2014, https://doi.org/10.5194/acp-14-1353-2014, 2014
C. Ge, J. Wang, and J. S. Reid
Atmos. Chem. Phys., 14, 159–174, https://doi.org/10.5194/acp-14-159-2014, https://doi.org/10.5194/acp-14-159-2014, 2014
B. S. Meland, X. Xu, D. K. Henze, and J. Wang
Atmos. Meas. Tech., 6, 3441–3457, https://doi.org/10.5194/amt-6-3441-2013, https://doi.org/10.5194/amt-6-3441-2013, 2013
C. Zhao, X. Liu, Y. Qian, J. Yoon, Z. Hou, G. Lin, S. McFarlane, H. Wang, B. Yang, P.-L. Ma, H. Yan, and J. Bao
Atmos. Chem. Phys., 13, 10969–10987, https://doi.org/10.5194/acp-13-10969-2013, https://doi.org/10.5194/acp-13-10969-2013, 2013
R. A. Ellis, D. J. Jacob, M. P. Sulprizio, L. Zhang, C. D. Holmes, B. A. Schichtel, T. Blett, E. Porter, L. H. Pardo, and J. A. Lynch
Atmos. Chem. Phys., 13, 9083–9095, https://doi.org/10.5194/acp-13-9083-2013, https://doi.org/10.5194/acp-13-9083-2013, 2013
H. Wang, R. C. Easter, P. J. Rasch, M. Wang, X. Liu, S. J. Ghan, Y. Qian, J.-H. Yoon, P.-L. Ma, and V. Vinoj
Geosci. Model Dev., 6, 765–782, https://doi.org/10.5194/gmd-6-765-2013, https://doi.org/10.5194/gmd-6-765-2013, 2013
K. Zhang, X. Liu, M. Wang, J. M. Comstock, D. L. Mitchell, S. Mishra, and G. G. Mace
Atmos. Chem. Phys., 13, 4963–4982, https://doi.org/10.5194/acp-13-4963-2013, https://doi.org/10.5194/acp-13-4963-2013, 2013
D. T. Shindell, J.-F. Lamarque, M. Schulz, M. Flanner, C. Jiao, M. Chin, P. J. Young, Y. H. Lee, L. Rotstayn, N. Mahowald, G. Milly, G. Faluvegi, Y. Balkanski, W. J. Collins, A. J. Conley, S. Dalsoren, R. Easter, S. Ghan, L. Horowitz, X. Liu, G. Myhre, T. Nagashima, V. Naik, S. T. Rumbold, R. Skeie, K. Sudo, S. Szopa, T. Takemura, A. Voulgarakis, J.-H. Yoon, and F. Lo
Atmos. Chem. Phys., 13, 2939–2974, https://doi.org/10.5194/acp-13-2939-2013, https://doi.org/10.5194/acp-13-2939-2013, 2013
B. H. Samset, G. Myhre, M. Schulz, Y. Balkanski, S. Bauer, T. K. Berntsen, H. Bian, N. Bellouin, T. Diehl, R. C. Easter, S. J. Ghan, T. Iversen, S. Kinne, A. Kirkevåg, J.-F. Lamarque, G. Lin, X. Liu, J. E. Penner, Ø. Seland, R. B. Skeie, P. Stier, T. Takemura, K. Tsigaridis, and K. Zhang
Atmos. Chem. Phys., 13, 2423–2434, https://doi.org/10.5194/acp-13-2423-2013, https://doi.org/10.5194/acp-13-2423-2013, 2013
M. S. Long, W. C. Keene, R. Easter, R. Sander, A. Kerkweg, D. Erickson, X. Liu, and S. Ghan
Geosci. Model Dev., 6, 255–262, https://doi.org/10.5194/gmd-6-255-2013, https://doi.org/10.5194/gmd-6-255-2013, 2013
J. Wang, S. Park, J. Zeng, C. Ge, K. Yang, S. Carn, N. Krotkov, and A. H. Omar
Atmos. Chem. Phys., 13, 1895–1912, https://doi.org/10.5194/acp-13-1895-2013, https://doi.org/10.5194/acp-13-1895-2013, 2013
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The need for carbon-emissions-driven climate projections in CMIP7
Robust handling of extremes in quantile mapping – “Murder your darlings”
A protocol for model intercomparison of impacts of marine cloud brightening climate intervention
An extensible perturbed parameter ensemble for the Community Atmosphere Model version 6
Coupling the regional climate model ICON-CLM v2.6.6 to the Earth system model GCOAST-AHOI v2.0 using OASIS3-MCT v4.0
A fully coupled solid-particle microphysics scheme for stratospheric aerosol injections within the aerosol–chemistry–climate model SOCOL-AERv2
An improved representation of aerosol in the ECMWF IFS-COMPO 49R1 through the integration of EQSAM4Climv12 – a first attempt at simulating aerosol acidity
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Impact of ocean vertical-mixing parameterization on Arctic sea ice and upper-ocean properties using the NEMO-SI3 model
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A new lightning scheme in the Canadian Atmospheric Model (CanAM5.1): implementation, evaluation, and projections of lightning and fire in future climates
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Benjamin M. Sanderson, Ben B. B. Booth, John Dunne, Veronika Eyring, Rosie A. Fisher, Pierre Friedlingstein, Matthew J. Gidden, Tomohiro Hajima, Chris D. Jones, Colin G. Jones, Andrew King, Charles D. Koven, David M. Lawrence, Jason Lowe, Nadine Mengis, Glen P. Peters, Joeri Rogelj, Chris Smith, Abigail C. Snyder, Isla R. Simpson, Abigail L. S. Swann, Claudia Tebaldi, Tatiana Ilyina, Carl-Friedrich Schleussner, Roland Séférian, Bjørn H. Samset, Detlef van Vuuren, and Sönke Zaehle
Geosci. Model Dev., 17, 8141–8172, https://doi.org/10.5194/gmd-17-8141-2024, https://doi.org/10.5194/gmd-17-8141-2024, 2024
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We discuss how, in order to provide more relevant guidance for climate policy, coordinated climate experiments should adopt a greater focus on simulations where Earth system models are provided with carbon emissions from fossil fuels together with land use change instructions, rather than past approaches that have largely focused on experiments with prescribed atmospheric carbon dioxide concentrations. We discuss how these goals might be achieved in coordinated climate modeling experiments.
Peter Berg, Thomas Bosshard, Denica Bozhinova, Lars Bärring, Joakim Löw, Carolina Nilsson, Gustav Strandberg, Johan Södling, Johan Thuresson, Renate Wilcke, and Wei Yang
Geosci. Model Dev., 17, 8173–8179, https://doi.org/10.5194/gmd-17-8173-2024, https://doi.org/10.5194/gmd-17-8173-2024, 2024
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When bias adjusting climate model data using quantile mapping, one needs to prescribe what to do at the tails of the distribution, where a larger data range is likely encountered outside of the calibration period. The end result is highly dependent on the method used. We show that, to avoid discontinuities in the time series, one needs to exclude data in the calibration range to also activate the extrapolation functionality in that time period.
Philip J. Rasch, Haruki Hirasawa, Mingxuan Wu, Sarah J. Doherty, Robert Wood, Hailong Wang, Andy Jones, James Haywood, and Hansi Singh
Geosci. Model Dev., 17, 7963–7994, https://doi.org/10.5194/gmd-17-7963-2024, https://doi.org/10.5194/gmd-17-7963-2024, 2024
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We introduce a protocol to compare computer climate simulations to better understand a proposed strategy intended to counter warming and climate impacts from greenhouse gas increases. This slightly changes clouds in six ocean regions to reflect more sunlight and cool the Earth. Example changes in clouds and climate are shown for three climate models. Cloud changes differ between the models, but precipitation and surface temperature changes are similar when their cooling effects are made similar.
Trude Eidhammer, Andrew Gettelman, Katherine Thayer-Calder, Duncan Watson-Parris, Gregory Elsaesser, Hugh Morrison, Marcus van Lier-Walqui, Ci Song, and Daniel McCoy
Geosci. Model Dev., 17, 7835–7853, https://doi.org/10.5194/gmd-17-7835-2024, https://doi.org/10.5194/gmd-17-7835-2024, 2024
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We describe a dataset where 45 parameters related to cloud processes in the Community Earth System Model version 2 (CESM2) Community Atmosphere Model version 6 (CAM6) are perturbed. Three sets of perturbed parameter ensembles (263 members) were created: current climate, preindustrial aerosol loading and future climate with sea surface temperature increased by 4 K.
Ha Thi Minh Ho-Hagemann, Vera Maurer, Stefan Poll, and Irina Fast
Geosci. Model Dev., 17, 7815–7834, https://doi.org/10.5194/gmd-17-7815-2024, https://doi.org/10.5194/gmd-17-7815-2024, 2024
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The regional Earth system model GCOAST-AHOI v2.0 that includes the regional climate model ICON-CLM coupled to the ocean model NEMO and the hydrological discharge model HD via the OASIS3-MCT coupler can be a useful tool for conducting long-term regional climate simulations over the EURO-CORDEX domain. The new OASIS3-MCT coupling interface implemented in ICON-CLM makes it more flexible for coupling to an external ocean model and an external hydrological discharge model.
Sandro Vattioni, Rahel Weber, Aryeh Feinberg, Andrea Stenke, John A. Dykema, Beiping Luo, Georgios A. Kelesidis, Christian A. Bruun, Timofei Sukhodolov, Frank N. Keutsch, Thomas Peter, and Gabriel Chiodo
Geosci. Model Dev., 17, 7767–7793, https://doi.org/10.5194/gmd-17-7767-2024, https://doi.org/10.5194/gmd-17-7767-2024, 2024
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We quantified impacts and efficiency of stratospheric solar climate intervention via solid particle injection. Microphysical interactions of solid particles with the sulfur cycle were interactively coupled to the heterogeneous chemistry scheme and the radiative transfer code of an aerosol–chemistry–climate model. Compared to injection of SO2 we only find a stronger cooling efficiency for solid particles when normalizing to the aerosol load but not when normalizing to the injection rate.
Samuel Rémy, Swen Metzger, Vincent Huijnen, Jason E. Williams, and Johannes Flemming
Geosci. Model Dev., 17, 7539–7567, https://doi.org/10.5194/gmd-17-7539-2024, https://doi.org/10.5194/gmd-17-7539-2024, 2024
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In this paper we describe the development of the future operational cycle 49R1 of the IFS-COMPO system, used for operational forecasts of atmospheric composition in the CAMS project, and focus on the implementation of the thermodynamical model EQSAM4Clim version 12. The implementation of EQSAM4Clim significantly improves the simulated secondary inorganic aerosol surface concentration. The new aerosol and precipitation acidity diagnostics showed good agreement against observational datasets.
Maximillian Van Wyk de Vries, Tom Matthews, L. Baker Perry, Nirakar Thapa, and Rob Wilby
Geosci. Model Dev., 17, 7629–7643, https://doi.org/10.5194/gmd-17-7629-2024, https://doi.org/10.5194/gmd-17-7629-2024, 2024
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This paper introduces the AtsMOS workflow, a new tool for improving weather forecasts in mountainous areas. By combining advanced statistical techniques with local weather data, AtsMOS can provide more accurate predictions of weather conditions. Using data from Mount Everest as an example, AtsMOS has shown promise in better forecasting hazardous weather conditions, making it a valuable tool for communities in mountainous regions and beyond.
Sofia Allende, Anne Marie Treguier, Camille Lique, Clément de Boyer Montégut, François Massonnet, Thierry Fichefet, and Antoine Barthélemy
Geosci. Model Dev., 17, 7445–7466, https://doi.org/10.5194/gmd-17-7445-2024, https://doi.org/10.5194/gmd-17-7445-2024, 2024
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We study the parameters of the turbulent-kinetic-energy mixed-layer-penetration scheme in the NEMO model with regard to sea-ice-covered regions of the Arctic Ocean. This evaluation reveals the impact of these parameters on mixed-layer depth, sea surface temperature and salinity, and ocean stratification. Our findings demonstrate significant impacts on sea ice thickness and sea ice concentration, emphasizing the need for accurately representing ocean mixing to understand Arctic climate dynamics.
Sabin I. Taranu, David M. Lawrence, Yoshihide Wada, Ting Tang, Erik Kluzek, Sam Rabin, Yi Yao, Steven J. De Hertog, Inne Vanderkelen, and Wim Thiery
Geosci. Model Dev., 17, 7365–7399, https://doi.org/10.5194/gmd-17-7365-2024, https://doi.org/10.5194/gmd-17-7365-2024, 2024
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In this study, we improved a climate model by adding the representation of water use sectors such as domestic, industry, and agriculture. This new feature helps us understand how water is used and supplied in various areas. We tested our model from 1971 to 2010 and found that it accurately identifies areas with water scarcity. By modelling the competition between sectors when water availability is limited, the model helps estimate the intensity and extent of individual sectors' water shortages.
Cynthia Whaley, Montana Etten-Bohm, Courtney Schumacher, Ayodeji Akingunola, Vivek Arora, Jason Cole, Michael Lazare, David Plummer, Knut von Salzen, and Barbara Winter
Geosci. Model Dev., 17, 7141–7155, https://doi.org/10.5194/gmd-17-7141-2024, https://doi.org/10.5194/gmd-17-7141-2024, 2024
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This paper describes how lightning was added as a process in the Canadian Earth System Model in order to interactively respond to climate changes. As lightning is an important cause of global wildfires, this new model development allows for more realistic projections of how wildfires may change in the future, responding to a changing climate.
Erik Gustafsson, Bo G. Gustafsson, Martijn Hermans, Christoph Humborg, and Christian Stranne
Geosci. Model Dev., 17, 7157–7179, https://doi.org/10.5194/gmd-17-7157-2024, https://doi.org/10.5194/gmd-17-7157-2024, 2024
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Methane (CH4) cycling in the Baltic Proper is studied through model simulations, enabling a first estimate of key CH4 fluxes. A preliminary budget identifies benthic CH4 release as the dominant source and two main sinks: CH4 oxidation in the water (92 % of sinks) and outgassing to the atmosphere (8 % of sinks). This study addresses CH4 emissions from coastal seas and is a first step toward understanding the relative importance of open-water outgassing compared with local coastal hotspots.
Tridib Banerjee, Patrick Scholz, Sergey Danilov, Knut Klingbeil, and Dmitry Sidorenko
Geosci. Model Dev., 17, 7051–7065, https://doi.org/10.5194/gmd-17-7051-2024, https://doi.org/10.5194/gmd-17-7051-2024, 2024
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In this paper we propose a new alternative to one of the functionalities of the sea ice model FESOM2. The alternative we propose allows the model to capture and simulate fast changes in quantities like sea surface elevation more accurately. We also demonstrate that the new alternative is faster and more adept at taking advantages of highly parallelized computing infrastructure. We therefore show that this new alternative is a great addition to the sea ice model FESOM2.
Yuwen Fan, Zhao Yang, Min-Hui Lo, Jina Hur, and Eun-Soon Im
Geosci. Model Dev., 17, 6929–6947, https://doi.org/10.5194/gmd-17-6929-2024, https://doi.org/10.5194/gmd-17-6929-2024, 2024
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Irrigated agriculture in the North China Plain (NCP) has a significant impact on the local climate. To better understand this impact, we developed a specialized model specifically for the NCP region. This model allows us to simulate the double-cropping vegetation and the dynamic irrigation practices that are commonly employed in the NCP. This model shows improved performance in capturing the general crop growth, such as crop stages, biomass, crop yield, and vegetation greenness.
Ed Blockley, Emma Fiedler, Jeff Ridley, Luke Roberts, Alex West, Dan Copsey, Daniel Feltham, Tim Graham, David Livings, Clement Rousset, David Schroeder, and Martin Vancoppenolle
Geosci. Model Dev., 17, 6799–6817, https://doi.org/10.5194/gmd-17-6799-2024, https://doi.org/10.5194/gmd-17-6799-2024, 2024
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This paper documents the sea ice model component of the latest Met Office coupled model configuration, which will be used as the physical basis for UK contributions to CMIP7. Documentation of science options used in the configuration are given along with a brief model evaluation. This is the first UK configuration to use NEMO’s new SI3 sea ice model. We provide details on how SI3 was adapted to work with Met Office coupling methodology and documentation of coupling processes in the model.
Jean-François Lemieux, William H. Lipscomb, Anthony Craig, David A. Bailey, Elizabeth C. Hunke, Philippe Blain, Till A. S. Rasmussen, Mats Bentsen, Frédéric Dupont, David Hebert, and Richard Allard
Geosci. Model Dev., 17, 6703–6724, https://doi.org/10.5194/gmd-17-6703-2024, https://doi.org/10.5194/gmd-17-6703-2024, 2024
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We present the latest version of the CICE model. It solves equations that describe the dynamics and the growth and melt of sea ice. To do so, the domain is divided into grid cells and variables are positioned at specific locations in the cells. A new implementation (C-grid) is presented, with the velocity located on cell edges. Compared to the previous B-grid, the C-grid allows for a natural coupling with some oceanic and atmospheric models. It also allows for ice transport in narrow channels.
Rachid El Montassir, Olivier Pannekoucke, and Corentin Lapeyre
Geosci. Model Dev., 17, 6657–6681, https://doi.org/10.5194/gmd-17-6657-2024, https://doi.org/10.5194/gmd-17-6657-2024, 2024
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This study introduces a novel approach that combines physics and artificial intelligence (AI) for improved cloud cover forecasting. This approach outperforms traditional deep learning (DL) methods in producing realistic and physically consistent results while requiring less training data. This architecture provides a promising solution to overcome the limitations of classical AI methods and contributes to open up new possibilities for combining physical knowledge with deep learning models.
Marit Sandstad, Borgar Aamaas, Ane Nordlie Johansen, Marianne Tronstad Lund, Glen Philip Peters, Bjørn Hallvard Samset, Benjamin Mark Sanderson, and Ragnhild Bieltvedt Skeie
Geosci. Model Dev., 17, 6589–6625, https://doi.org/10.5194/gmd-17-6589-2024, https://doi.org/10.5194/gmd-17-6589-2024, 2024
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The CICERO-SCM has existed as a Fortran model since 1999 that calculates the radiative forcing and concentrations from emissions and is an upwelling diffusion energy balance model of the ocean that calculates temperature change. In this paper, we describe an updated version ported to Python and publicly available at https://github.com/ciceroOslo/ciceroscm (https://doi.org/10.5281/zenodo.10548720). This version contains functionality for parallel runs and automatic calibration.
Zheng Xiang, Yongkang Xue, Weidong Guo, Melannie D. Hartman, Ye Liu, and William J. Parton
Geosci. Model Dev., 17, 6437–6464, https://doi.org/10.5194/gmd-17-6437-2024, https://doi.org/10.5194/gmd-17-6437-2024, 2024
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A process-based plant carbon (C)–nitrogen (N) interface coupling framework has been developed which mainly focuses on plant resistance and N-limitation effects on photosynthesis, plant respiration, and plant phenology. A dynamic C / N ratio is introduced to represent plant resistance and self-adjustment. The framework has been implemented in a coupled biophysical-ecosystem–biogeochemical model, and testing results show a general improvement in simulating plant properties with this framework.
Yangke Liu, Qing Bao, Bian He, Xiaofei Wu, Jing Yang, Yimin Liu, Guoxiong Wu, Tao Zhu, Siyuan Zhou, Yao Tang, Ankang Qu, Yalan Fan, Anling Liu, Dandan Chen, Zhaoming Luo, Xing Hu, and Tongwen Wu
Geosci. Model Dev., 17, 6249–6275, https://doi.org/10.5194/gmd-17-6249-2024, https://doi.org/10.5194/gmd-17-6249-2024, 2024
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We give an overview of the Institute of Atmospheric Physics–Chinese Academy of Sciences subseasonal-to-seasonal ensemble forecasting system and Madden–Julian Oscillation forecast evaluation of the system. Compared to other S2S models, the IAP-CAS model has its benefits but also biases, i.e., underdispersive ensemble, overestimated amplitude, and faster propagation speed when forecasting MJO. We provide a reason for these biases and prospects for further improvement of this system in the future.
Laurent Brodeau, Pierre Rampal, Einar Ólason, and Véronique Dansereau
Geosci. Model Dev., 17, 6051–6082, https://doi.org/10.5194/gmd-17-6051-2024, https://doi.org/10.5194/gmd-17-6051-2024, 2024
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A new brittle sea ice rheology, BBM, has been implemented into the sea ice component of NEMO. We describe how a new spatial discretization framework was introduced to achieve this. A set of idealized and realistic ocean and sea ice simulations of the Arctic have been performed using BBM and the standard viscous–plastic rheology of NEMO. When compared to satellite data, our simulations show that our implementation of BBM leads to a fairly good representation of sea ice deformations.
Joseph P. Hollowed, Christiane Jablonowski, Hunter Y. Brown, Benjamin R. Hillman, Diana L. Bull, and Joseph L. Hart
Geosci. Model Dev., 17, 5913–5938, https://doi.org/10.5194/gmd-17-5913-2024, https://doi.org/10.5194/gmd-17-5913-2024, 2024
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Large volcanic eruptions deposit material in the upper atmosphere, which is capable of altering temperature and wind patterns of Earth's atmosphere for subsequent years. This research describes a new method of simulating these effects in an idealized, efficient atmospheric model. A volcanic eruption of sulfur dioxide is described with a simplified set of physical rules, which eventually cools the planetary surface. This model has been designed as a test bed for climate attribution studies.
Hong Li, Yi Yang, Jian Sun, Yuan Jiang, Ruhui Gan, and Qian Xie
Geosci. Model Dev., 17, 5883–5896, https://doi.org/10.5194/gmd-17-5883-2024, https://doi.org/10.5194/gmd-17-5883-2024, 2024
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Vertical atmospheric motions play a vital role in convective-scale precipitation forecasts by connecting atmospheric dynamics with cloud development. A three-dimensional variational vertical velocity assimilation scheme is developed within the high-resolution CMA-MESO model, utilizing the adiabatic Richardson equation as the observation operator. A 10 d continuous run and an individual case study demonstrate improved forecasts, confirming the scheme's effectiveness.
Matthias Nützel, Laura Stecher, Patrick Jöckel, Franziska Winterstein, Martin Dameris, Michael Ponater, Phoebe Graf, and Markus Kunze
Geosci. Model Dev., 17, 5821–5849, https://doi.org/10.5194/gmd-17-5821-2024, https://doi.org/10.5194/gmd-17-5821-2024, 2024
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We extended the infrastructure of our modelling system to enable the use of an additional radiation scheme. After calibrating the model setups to the old and the new radiation scheme, we find that the simulation with the new scheme shows considerable improvements, e.g. concerning the cold-point temperature and stratospheric water vapour. Furthermore, perturbations of radiative fluxes associated with greenhouse gas changes, e.g. of methane, tend to be improved when the new scheme is employed.
Yibing Wang, Xianhong Xie, Bowen Zhu, Arken Tursun, Fuxiao Jiang, Yao Liu, Dawei Peng, and Buyun Zheng
Geosci. Model Dev., 17, 5803–5819, https://doi.org/10.5194/gmd-17-5803-2024, https://doi.org/10.5194/gmd-17-5803-2024, 2024
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Urban expansion intensifies challenges like urban heat and urban dry islands. To address this, we developed an urban module, VIC-urban, in the Variable Infiltration Capacity (VIC) model. Tested in Beijing, VIC-urban accurately simulated turbulent heat fluxes, runoff, and land surface temperature. We provide a reliable tool for large-scale simulations considering urban environment and a systematic urban modelling framework within VIC, offering crucial insights for urban planners and designers.
Jeremy Carter, Erick A. Chacón-Montalván, and Amber Leeson
Geosci. Model Dev., 17, 5733–5757, https://doi.org/10.5194/gmd-17-5733-2024, https://doi.org/10.5194/gmd-17-5733-2024, 2024
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Climate models are essential tools in the study of climate change and its wide-ranging impacts on life on Earth. However, the output is often afflicted with some bias. In this paper, a novel model is developed to predict and correct bias in the output of climate models. The model captures uncertainty in the correction and explicitly models underlying spatial correlation between points. These features are of key importance for climate change impact assessments and resulting decision-making.
Anna Martin, Veronika Gayler, Benedikt Steil, Klaus Klingmüller, Patrick Jöckel, Holger Tost, Jos Lelieveld, and Andrea Pozzer
Geosci. Model Dev., 17, 5705–5732, https://doi.org/10.5194/gmd-17-5705-2024, https://doi.org/10.5194/gmd-17-5705-2024, 2024
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The study evaluates the land surface and vegetation model JSBACHv4 as a replacement for the simplified submodel SURFACE in EMAC. JSBACH mitigates earlier problems of soil dryness, which are critical for vegetation modelling. When analysed using different datasets, the coupled model shows strong correlations of key variables, such as land surface temperature, surface albedo and radiation flux. The versatility of the model increases significantly, while the overall performance does not degrade.
Hugo Banderier, Christian Zeman, David Leutwyler, Stefan Rüdisühli, and Christoph Schär
Geosci. Model Dev., 17, 5573–5586, https://doi.org/10.5194/gmd-17-5573-2024, https://doi.org/10.5194/gmd-17-5573-2024, 2024
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We investigate the effects of reduced-precision arithmetic in a state-of-the-art regional climate model by studying the results of 10-year-long simulations. After this time, the results of the reduced precision and the standard implementation are hardly different. This should encourage the use of reduced precision in climate models to exploit the speedup and memory savings it brings. The methodology used in this work can help researchers verify reduced-precision implementations of their model.
David Fuchs, Steven C. Sherwood, Abhnil Prasad, Kirill Trapeznikov, and Jim Gimlett
Geosci. Model Dev., 17, 5459–5475, https://doi.org/10.5194/gmd-17-5459-2024, https://doi.org/10.5194/gmd-17-5459-2024, 2024
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Machine learning (ML) of unresolved processes offers many new possibilities for improving weather and climate models, but integrating ML into the models has been an engineering challenge, and there are performance issues. We present a new software plugin for this integration, TorchClim, that is scalable and flexible and thereby allows a new level of experimentation with the ML approach. We also provide guidance on ML training and demonstrate a skillful hybrid ML atmosphere model.
Minjin Lee, Charles A. Stock, John P. Dunne, and Elena Shevliakova
Geosci. Model Dev., 17, 5191–5224, https://doi.org/10.5194/gmd-17-5191-2024, https://doi.org/10.5194/gmd-17-5191-2024, 2024
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Modeling global freshwater solid and nutrient loads, in both magnitude and form, is imperative for understanding emerging eutrophication problems. Such efforts, however, have been challenged by the difficulty of balancing details of freshwater biogeochemical processes with limited knowledge, input, and validation datasets. Here we develop a global freshwater model that resolves intertwined algae, solid, and nutrient dynamics and provide performance assessment against measurement-based estimates.
Hunter York Brown, Benjamin Wagman, Diana Bull, Kara Peterson, Benjamin Hillman, Xiaohong Liu, Ziming Ke, and Lin Lin
Geosci. Model Dev., 17, 5087–5121, https://doi.org/10.5194/gmd-17-5087-2024, https://doi.org/10.5194/gmd-17-5087-2024, 2024
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Explosive volcanic eruptions lead to long-lived, microscopic particles in the upper atmosphere which act to cool the Earth's surface by reflecting the Sun's light back to space. We include and test this process in a global climate model, E3SM. E3SM is tested against satellite and balloon observations of the 1991 eruption of Mt. Pinatubo, showing that with these particles in the model we reasonably recreate Pinatubo and its global effects. We also explore how particle size leads to these effects.
Deifilia Aurora To, Julian Quinting, Gholam Ali Hoshyaripour, Markus Götz, Achim Streit, and Charlotte Debus
EGUsphere, https://doi.org/10.5194/egusphere-2024-1714, https://doi.org/10.5194/egusphere-2024-1714, 2024
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Pangu-Weather is a breakthrough machine learning model in medium-range weather forecasting that considers three-dimensional atmospheric information. We show that using a simpler 2D framework improves robustness, speeds up training, and reduces computational needs by 20–30%. We introduce a training procedure that varies the importance of atmospheric variables over time to speed up training convergence. Decreasing computational demand increases accessibility of training and working with the model.
Carl Svenhag, Moa K. Sporre, Tinja Olenius, Daniel Yazgi, Sara M. Blichner, Lars P. Nieradzik, and Pontus Roldin
Geosci. Model Dev., 17, 4923–4942, https://doi.org/10.5194/gmd-17-4923-2024, https://doi.org/10.5194/gmd-17-4923-2024, 2024
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Our research shows the importance of modeling new particle formation (NPF) and growth of particles in the atmosphere on a global scale, as they influence the outcomes of clouds and our climate. With the global model EC-Earth3 we show that using a new method for NPF modeling, which includes new detailed processes with NH3 and H2SO4, significantly impacts the number of particles in the air and clouds and changes the radiation balance of the same magnitude as anthropogenic greenhouse emissions.
Mengjie Han, Qing Zhao, Xili Wang, Ying-Ping Wang, Philippe Ciais, Haicheng Zhang, Daniel S. Goll, Lei Zhu, Zhe Zhao, Zhixuan Guo, Chen Wang, Wei Zhuang, Fengchang Wu, and Wei Li
Geosci. Model Dev., 17, 4871–4890, https://doi.org/10.5194/gmd-17-4871-2024, https://doi.org/10.5194/gmd-17-4871-2024, 2024
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The impact of biochar (BC) on soil organic carbon (SOC) dynamics is not represented in most land carbon models used for assessing land-based climate change mitigation. Our study develops a BC model that incorporates our current understanding of BC effects on SOC based on a soil carbon model (MIMICS). The BC model can reproduce the SOC changes after adding BC, providing a useful tool to couple dynamic land models to evaluate the effectiveness of BC application for CO2 removal from the atmosphere.
Kalyn Dorheim, Skylar Gering, Robert Gieseke, Corinne Hartin, Leeya Pressburger, Alexey N. Shiklomanov, Steven J. Smith, Claudia Tebaldi, Dawn L. Woodard, and Ben Bond-Lamberty
Geosci. Model Dev., 17, 4855–4869, https://doi.org/10.5194/gmd-17-4855-2024, https://doi.org/10.5194/gmd-17-4855-2024, 2024
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Hector is an easy-to-use, global climate–carbon cycle model. With its quick run time, Hector can provide climate information from a run in a fraction of a second. Hector models on a global and annual basis. Here, we present an updated version of the model, Hector V3. In this paper, we document Hector’s new features. Hector V3 is capable of reproducing historical observations, and its future temperature projections are consistent with those of more complex models.
Fangxuan Ren, Jintai Lin, Chenghao Xu, Jamiu A. Adeniran, Jingxu Wang, Randall V. Martin, Aaron van Donkelaar, Melanie S. Hammer, Larry W. Horowitz, Steven T. Turnock, Naga Oshima, Jie Zhang, Susanne Bauer, Kostas Tsigaridis, Øyvind Seland, Pierre Nabat, David Neubauer, Gary Strand, Twan van Noije, Philippe Le Sager, and Toshihiko Takemura
Geosci. Model Dev., 17, 4821–4836, https://doi.org/10.5194/gmd-17-4821-2024, https://doi.org/10.5194/gmd-17-4821-2024, 2024
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We evaluate the performance of 14 CMIP6 ESMs in simulating total PM2.5 and its 5 components over China during 2000–2014. PM2.5 and its components are underestimated in almost all models, except that black carbon (BC) and sulfate are overestimated in two models, respectively. The underestimation is the largest for organic carbon (OC) and the smallest for BC. Models reproduce the observed spatial pattern for OC, sulfate, nitrate and ammonium well, yet the agreement is poorer for BC.
Yi Xi, Chunjing Qiu, Yuan Zhang, Dan Zhu, Shushi Peng, Gustaf Hugelius, Jinfeng Chang, Elodie Salmon, and Philippe Ciais
Geosci. Model Dev., 17, 4727–4754, https://doi.org/10.5194/gmd-17-4727-2024, https://doi.org/10.5194/gmd-17-4727-2024, 2024
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The ORCHIDEE-MICT model can simulate the carbon cycle and hydrology at a sub-grid scale but energy budgets only at a grid scale. This paper assessed the implementation of a multi-tiling energy budget approach in ORCHIDEE-MICT and found warmer surface and soil temperatures, higher soil moisture, and more soil organic carbon across the Northern Hemisphere compared with the original version.
Maria Rosa Russo, Sadie L. Bartholomew, David Hassell, Alex M. Mason, Erica Neininger, A. James Perman, David A. J. Sproson, Duncan Watson-Parris, and Nathan Luke Abraham
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-73, https://doi.org/10.5194/gmd-2024-73, 2024
Revised manuscript accepted for GMD
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Observational data and modelling capabilities are expanding in recent years, but there are still barriers preventing these two data sources to be used in synergy. Proper comparison requires generating, storing and handling a large amount of data. This manuscript describes the first step in the development of a new set of software tools, the ‘VISION toolkit’, which can enable the easy and efficient integration of observational and model data required for model evaluation.
Georgia Lazoglou, Theo Economou, Christina Anagnostopoulou, George Zittis, Anna Tzyrkalli, Pantelis Georgiades, and Jos Lelieveld
Geosci. Model Dev., 17, 4689–4703, https://doi.org/10.5194/gmd-17-4689-2024, https://doi.org/10.5194/gmd-17-4689-2024, 2024
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This study focuses on the important issue of the drizzle bias effect in regional climate models, described by an over-prediction of the number of rainy days while underestimating associated precipitation amounts. For this purpose, two distinct methodologies are applied and rigorously evaluated. These results are encouraging for using the multivariate machine learning method random forest to increase the accuracy of climate models concerning the projection of the number of wet days.
Xu Yue, Hao Zhou, Chenguang Tian, Yimian Ma, Yihan Hu, Cheng Gong, Hui Zheng, and Hong Liao
Geosci. Model Dev., 17, 4621–4642, https://doi.org/10.5194/gmd-17-4621-2024, https://doi.org/10.5194/gmd-17-4621-2024, 2024
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We develop the interactive Model for Air Pollution and Land Ecosystems (iMAPLE). The model considers the full coupling between carbon and water cycles, dynamic fire emissions, wetland methane emissions, biogenic volatile organic compound emissions, and trait-based ozone vegetation damage. Evaluations show that iMAPLE is a useful tool for the study of the interactions among climate, chemistry, and ecosystems.
Malte Meinshausen, Carl-Friedrich Schleussner, Kathleen Beyer, Greg Bodeker, Olivier Boucher, Josep G. Canadell, John S. Daniel, Aïda Diongue-Niang, Fatima Driouech, Erich Fischer, Piers Forster, Michael Grose, Gerrit Hansen, Zeke Hausfather, Tatiana Ilyina, Jarmo S. Kikstra, Joyce Kimutai, Andrew D. King, June-Yi Lee, Chris Lennard, Tabea Lissner, Alexander Nauels, Glen P. Peters, Anna Pirani, Gian-Kasper Plattner, Hans Pörtner, Joeri Rogelj, Maisa Rojas, Joyashree Roy, Bjørn H. Samset, Benjamin M. Sanderson, Roland Séférian, Sonia Seneviratne, Christopher J. Smith, Sophie Szopa, Adelle Thomas, Diana Urge-Vorsatz, Guus J. M. Velders, Tokuta Yokohata, Tilo Ziehn, and Zebedee Nicholls
Geosci. Model Dev., 17, 4533–4559, https://doi.org/10.5194/gmd-17-4533-2024, https://doi.org/10.5194/gmd-17-4533-2024, 2024
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The scientific community is considering new scenarios to succeed RCPs and SSPs for the next generation of Earth system model runs to project future climate change. To contribute to that effort, we reflect on relevant policy and scientific research questions and suggest categories for representative emission pathways. These categories are tailored to the Paris Agreement long-term temperature goal, high-risk outcomes in the absence of further climate policy and worlds “that could have been”.
Seung H. Baek, Paul A. Ullrich, Bo Dong, and Jiwoo Lee
EGUsphere, https://doi.org/10.5194/egusphere-2024-1456, https://doi.org/10.5194/egusphere-2024-1456, 2024
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We evaluate downscaled products by examining locally relevant covariances during convective and frontal precipitation events. Common statistical downscaling techniques preserve expected covariances during convective precipitation. However, they dampen future intensification of frontal precipitation captured in global climate models and dynamical downscaling. This suggests statistical downscaling may not fully resolve non-stationary hydrologic processes as compared to dynamical downscaling.
Emmanuel Nyenah, Petra Döll, Daniel S. Katz, and Robert Reinecke
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-97, https://doi.org/10.5194/gmd-2024-97, 2024
Revised manuscript accepted for GMD
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Research software is crucial for scientific progress but is often developed by scientists with limited training, time, and funding, leading to software that is hard to understand, (re)use, modify, and maintain. Our study across 10 research sectors highlights strengths in version control, open-source licensing, and documentation while emphasizing the need for containerization and code quality. Recommendations include workshops, code quality metrics, funding, and adherence to FAIR standards.
Yilin Fang, Hoang Viet Tran, and L. Ruby Leung
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-70, https://doi.org/10.5194/gmd-2024-70, 2024
Revised manuscript accepted for GMD
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Hurricanes may worsen the water quality in the lower Mississippi River Basin (LMRB) by increasing nutrient runoff. We found that runoff parameterizations greatly affect nitrate-nitrogen runoff simulated using an Earth system land model. Our simulations predicted increased nitrogen runoff in LMRB during Hurricane Ida in 2021, but less pronounced than the observations, indicating areas for model improvement to better understand and manage nutrient runoff loss during hurricanes in the region.
Giovanni G. Seijo-Ellis, Donata Giglio, Gustavo M. Marques, and Frank O. Bryan
EGUsphere, https://doi.org/10.5194/egusphere-2024-1378, https://doi.org/10.5194/egusphere-2024-1378, 2024
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A CESM/MOM6 regional configuration of the Caribbean Sea was developed as a response to the rising need of high-resolution models for climate impact studies. The configuration is validated for the period of 2000–2020 and improves significant errors in a low resolution model. Oceanic properties are well represented. Patterns of freshwater associated with the Amazon river are well captured and the mean flows across the multiple passages in the Caribbean Sea agree with observations.
Ross Mower, Ethan D. Gutmann, Glen E. Liston, Jessica Lundquist, and Soren Rasmussen
Geosci. Model Dev., 17, 4135–4154, https://doi.org/10.5194/gmd-17-4135-2024, https://doi.org/10.5194/gmd-17-4135-2024, 2024
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Higher-resolution model simulations are better at capturing winter snowpack changes across space and time. However, increasing resolution also increases the computational requirements. This work provides an overview of changes made to a distributed snow-evolution modeling system (SnowModel) to allow it to leverage high-performance computing resources. Continental simulations that were previously estimated to take 120 d can now be performed in 5 h.
Catherine Guiavarc'h, Dave Storkey, Adam T. Blaker, Ed Blockley, Alex Megann, Helene T. Hewitt, Michael J. Bell, Daley Calvert, Dan Copsey, Bablu Sinha, Sophia Moreton, Pierre Mathiot, and Bo An
EGUsphere, https://doi.org/10.5194/egusphere-2024-805, https://doi.org/10.5194/egusphere-2024-805, 2024
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GOSI9 is the new UK’s hierarchy of global ocean and sea ice models. Developed as part of a collaboration between several UK research institutes it will be used for various applications such as weather forecast and climate prediction. The models, based on NEMO, are available at three resolutions 1°, ¼° and 1/12°. GOSI9 improves upon previous version by reducing global temperature and salinity biases and enhancing the representation of the Arctic sea ice and of the Antarctic Circumpolar Current.
Jiaxu Guo, Juepeng Zheng, Yidan Xu, Haohuan Fu, Wei Xue, Lanning Wang, Lin Gan, Ping Gao, Wubing Wan, Xianwei Wu, Zhitao Zhang, Liang Hu, Gaochao Xu, and Xilong Che
Geosci. Model Dev., 17, 3975–3992, https://doi.org/10.5194/gmd-17-3975-2024, https://doi.org/10.5194/gmd-17-3975-2024, 2024
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To enhance the efficiency of experiments using SCAM, we train a learning-based surrogate model to facilitate large-scale sensitivity analysis and tuning of combinations of multiple parameters. Employing a hybrid method, we investigate the joint sensitivity of multi-parameter combinations across typical cases, identifying the most sensitive three-parameter combination out of 11. Subsequently, we conduct a tuning process aimed at reducing output errors in these cases.
Yung-Yao Lan, Huang-Hsiung Hsu, and Wan-Ling Tseng
Geosci. Model Dev., 17, 3897–3918, https://doi.org/10.5194/gmd-17-3897-2024, https://doi.org/10.5194/gmd-17-3897-2024, 2024
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This study uses the CAM5–SIT coupled model to investigate the effects of SST feedback frequency on the MJO simulations with intervals at 30 min, 1, 3, 6, 12, 18, 24, and 30 d. The simulations become increasingly unrealistic as the frequency of the SST feedback decreases. Our results suggest that more spontaneous air--sea interaction (e.g., ocean response within 3 d in this study) with high vertical resolution in the ocean model is key to the realistic simulation of the MJO.
Jiwoo Lee, Peter J. Gleckler, Min-Seop Ahn, Ana Ordonez, Paul A. Ullrich, Kenneth R. Sperber, Karl E. Taylor, Yann Y. Planton, Eric Guilyardi, Paul Durack, Celine Bonfils, Mark D. Zelinka, Li-Wei Chao, Bo Dong, Charles Doutriaux, Chengzhu Zhang, Tom Vo, Jason Boutte, Michael F. Wehner, Angeline G. Pendergrass, Daehyun Kim, Zeyu Xue, Andrew T. Wittenberg, and John Krasting
Geosci. Model Dev., 17, 3919–3948, https://doi.org/10.5194/gmd-17-3919-2024, https://doi.org/10.5194/gmd-17-3919-2024, 2024
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We introduce an open-source software, the PCMDI Metrics Package (PMP), developed for a comprehensive comparison of Earth system models (ESMs) with real-world observations. Using diverse metrics evaluating climatology, variability, and extremes simulated in thousands of simulations from the Coupled Model Intercomparison Project (CMIP), PMP aids in benchmarking model improvements across generations. PMP also enables efficient tracking of performance evolutions during ESM developments.
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Short summary
This paper describes the first version of the Beijing Climate Center (BCC) fully coupled Earth System Model with interactive atmospheric chemistry and aerosols (BCC-ESM1). It is one of the models at the BCC for the Coupled Model Intercomparison Project Phase 6 (CMIP6). The CMIP6 Aerosol Chemistry Model Intercomparison Project (AerChemMIP) experiment using BCC-ESM1 has been finished. The evaluations show an overall good agreement between BCC-ESM1 simulations and observations in the 20th century.
This paper describes the first version of the Beijing Climate Center (BCC) fully coupled Earth...
