Articles | Volume 11, issue 6
https://doi.org/10.5194/gmd-11-2049-2018
https://doi.org/10.5194/gmd-11-2049-2018
Development and technical paper
 | 
05 Jun 2018
Development and technical paper |  | 05 Jun 2018

An advanced method of contributing emissions to short-lived chemical species (OH and HO2): the TAGGING 1.1 submodel based on the Modular Earth Submodel System (MESSy 2.53)

Vanessa S. Rieger, Mariano Mertens, and Volker Grewe

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Cited articles

Butler, T., Lawrence, M., Taraborrelli, D., and Lelieveld, J.: Multi-day ozone production potential of volatile organic compounds calculated with a tagging approach, Atmos. Environ., 45, 4082–4090, https://doi.org/10.1016/j.atmosenv.2011.03.040, 2011. a
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Coates, J. and Butler, T. M.: A comparison of chemical mechanisms using tagged ozone production potential (TOPP) analysis, Atmos. Chem. Phys., 15, 8795–8808, https://doi.org/10.5194/acp-15-8795-2015, 2015. a
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To reduce the climate impact of human activities, it is crucial to attribute changes in atmospheric gases to anthropogenic emissions. We present an advanced method to determine the contribution of emissions to OH and HO2 concentrations. Compared to the former version, it contains the main reactions of the OH and HO2 chemistry in the troposphere and stratosphere, introduces the tagging of the H radical and closes the budget of the sum of all contributions and the total concentration.