Articles | Volume 16, issue 4
https://doi.org/10.5194/gmd-16-1359-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/gmd-16-1359-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Methods for assessment of models
| 
27 Feb 2023
Methods for assessment of models |
| 27 Feb 2023
| 27 Feb 2023
Incorporation of aerosol into the COSPv2 satellite lidar simulator for climate model evaluation
Marine Bonazzola
CORRESPONDING AUTHOR
Laboratoire de Météorologie Dynamique, École
Polytechnique, Palaiseau, France
Hélène Chepfer
Laboratoire de Météorologie Dynamique, École
Polytechnique, Palaiseau, France
Po-Lun Ma
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, WA, USA
Johannes Quaas
Institute for Meteorology, Universität Leipzig, Leipzig, Germany
David M. Winker
Langley Research Center, NASA, Hampton, VA, USA
Artem Feofilov
Laboratoire de Météorologie Dynamique, École
Polytechnique, Palaiseau, France
Nick Schutgens
Faculty of Sciences, Department of Earth Sciences, Vrije Universiteit Amsterdam, Amsterdam, the Netherlands
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Yannick Emanuel Anders, Karoline Block, Mira Pöhlker, and Johannes Quaas
EGUsphere, https://doi.org/10.5194/egusphere-2026-1404, https://doi.org/10.5194/egusphere-2026-1404, 2026
This preprint is open for discussion and under review for Geoscientific Model Development (GMD).
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Particles in the atmosphere can trigger the formation of cloud droplets, affecting cloud properties and climate. This study evaluates a new global dataset of these particles with measurements from 25 sites around the world. The variability in time and space and their conditional formation behaviour is analysed. The authors identify systematic biases and introduce a simple correction based on observations that greatly improves the dataset’s accuracy.
Jean Lac, Hélène Chepfer, Matthew D. Shupe, and Hannes Griesche
Atmos. Chem. Phys., 26, 4189–4213, https://doi.org/10.5194/acp-26-4189-2026, https://doi.org/10.5194/acp-26-4189-2026, 2026
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Satellite observations show that Arctic spring experiences a rapid increase in liquid-containing clouds over sea ice. Our study shows that this transition is mostly driven by warmer temperatures in early spring than in late spring, favoring more liquid clouds formation, rather than a limited moisture source in early spring. It suggests that, in the future, this transition is likely to occur earlier in spring considering the rapid Arctic warming.
Jerome D. Fast, Balwinder Singh, Oscar Diaz-Ibarra, Jeff Johnson, Chandru Dhandapani, Brian Gaudet, Taufiq Hassan, Meng Huang, Jaelyn Litzinger, James Overfelt, Kyle Pressel, Michael Schmidt, Shuaiqi Tang, Adam C. Varble, Hui Wan, Mingxuan Wu, Kai Zhang, and Po-Lun Ma
EGUsphere, https://doi.org/10.5194/egusphere-2026-1538, https://doi.org/10.5194/egusphere-2026-1538, 2026
This preprint is open for discussion and under review for Geoscientific Model Development (GMD).
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We ported a prognostic representation of aerosols to C++ and integrated it into an Earth system model that runs on powerful GPU supercomputers. The code conversion approach keeps the same detailed physics as the Fortran version, was carefully tested, and results show that new code produces aerosol simulations consistent with real‑world data over the central U.S. in spring 2016. Future work will optimize the code for GPUs so to reduce the overall computational time.
Tobias Braun, Sara M. Vallejo-Bernal, Norbert Marwan, Juergen Kurths, Johannes Quaas, Albert Díaz-Guilera, Luis Gimeno, and Miguel D. Mahecha
EGUsphere, https://doi.org/10.21203/rs.3.rs-7482510/v2, https://doi.org/10.21203/rs.3.rs-7482510/v2, 2026
This preprint is open for discussion and under review for Earth System Dynamics (ESD).
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Atmospheric rivers (ARs) move vast amounts of water through the atmosphere and often cause weather extremes, yet they are usually studied as regional events. Using 84 years of mapped AR trajectories, we reveal the global "roadmap" of ARs, a transport network of high-activity hubs, sparse atmospheric highways & hierarchical basins. Our approach shows how water vapor is systematically channelled through an atmospheric transport network, offering new ways to study changes in the global water cycle.
Johannes Mülmenstädt and Po-Lun Ma
EGUsphere, https://doi.org/10.5194/egusphere-2026-748, https://doi.org/10.5194/egusphere-2026-748, 2026
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Aerosols emitted by human activities change the planetary energy budget by, among other mechanisms, changing how much liquid water is contained in clouds and thus their reflectance. Different lines of evidence (observations and models) disagree on the sign of the liquid water change even though they agree on the sign of the correlation between aerosols and liquid water in present-day internal variability. We show one way that observations can constrain models to resolve this disagreement.
Sergey Khaykin, Michaël Sicard, Thierry Leblanc, Tetsu Sakai, Nickolay Balugin, Gwenaël Berthet, Stëphane Chevrier, Fernando Chouza, Artem Feofilov, Dominique Gantois, Sophie Godin-Beekmann, Arezki Haddouche, Yoshitaka Jin, Isamu Morino, Nicolas Kadygrov, Thomas Lecas, Ben Liley, Richard Querel, Ghasssan Taha, and Vladimir Yushkov
Atmos. Chem. Phys., 26, 607–622, https://doi.org/10.5194/acp-26-607-2026, https://doi.org/10.5194/acp-26-607-2026, 2026
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In April 2024, the Ruang volcano in Indonesia sent large amounts of gas and particles high into the atmosphere, which then spread worldwide. Using the new European EarthCARE satellite and its advanced laser instrument ATLID (Atmospheric LIDar), together with ground and balloon observations, we tracked how these particles doubled levels in the tropics and spread into both hemispheres. The study shows ATLID’s power to reveal how eruptions can affect climate, clouds, and ozone for more than a year.
Zacharie Titus, Marine Bonazzola, Hélène Chepfer, Artem G. Feofilov, Marie-Laure Roussel, Benjamin Witschas, and Sophie Bastin
Atmos. Chem. Phys., 26, 443–475, https://doi.org/10.5194/acp-26-443-2026, https://doi.org/10.5194/acp-26-443-2026, 2026
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Aeolus spaceborne Doppler Wind Lidar observes perfectly co-located vertical profiles of clouds and vertical profiles of horizontal wind that can be used to study cloud-wind interactions. At regional scale, we show that over the Indian Ocean, high cloud fractions increase when the Tropical Easterly Jet is active. At a smaller scale, we observe for the first time from space differences in the wind profiles within the cloud and its surrounding clear sky, that can be imputed to convective motions.
Yusuf A. Bhatti, Duncan Watson-Parris, Leighton A. Regayre, Hailing Jia, David Neubauer, Ulas Im, Carl Svenhag, Nick Schutgens, Athanasios Tsikerdekis, Athanasios Nenes, Muhammed Irfan, Bastiaan van Diedenhoven, Ardit Arifi, Guangliang Fu, and Otto P. Hasekamp
Atmos. Chem. Phys., 26, 269–293, https://doi.org/10.5194/acp-26-269-2026, https://doi.org/10.5194/acp-26-269-2026, 2026
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Aerosols (small airborne particles) impact Earth's climate, but their extent is unknown. By running climate model simulations and using machine learning to emulate millions of additional variants with different settings, we found that natural emissions like sea spray and sulfur are key sources of uncertainty in climate predictions. Our work shows that understanding these natural processes better can help improve climate models and make future climate projections more accurate.
Marie-Laure Roussel, Hélène Chepfer, Zacharie Titus, and Marine Bonazzola
Atmos. Chem. Phys., 26, 117–134, https://doi.org/10.5194/acp-26-117-2026, https://doi.org/10.5194/acp-26-117-2026, 2026
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Clouds are crucial for understanding and predicting climate, yet their processes remain uncertain in global models. We reproduced detailed observations from a lidar and a wind-lidar using an advanced instrument simulator to evaluate how well the model represents clouds. A dedicated module was developed for the wind-lidar. Both instruments reveal comparable cloud biases, confirming its value for improving model evaluation and enabling consistent multi-decade assessments with more recent sensors.
Matthew W. Christensen, Andrew Geiss, Adam C. Varble, and Po-Lun Ma
Atmos. Chem. Phys., 26, 59–76, https://doi.org/10.5194/acp-26-59-2026, https://doi.org/10.5194/acp-26-59-2026, 2026
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We used satellite data and machine learning to better understand how tiny particles in the atmosphere affect clouds and their brightness. At higher spatial resolution, we discovered a new “M”-shaped pattern in the relationship between cloud water and droplet concentration unlike the inverted-V shape observed at coarsely gridded scales. Cloud water increases more with droplet concentration when rain is present. These findings support the development of next-generation atmospheric models.
Jianqi Zhao, Xiaoyan Ma, Johannes Quaas, and Tong Yang
Atmos. Chem. Phys., 25, 17701–17723, https://doi.org/10.5194/acp-25-17701-2025, https://doi.org/10.5194/acp-25-17701-2025, 2025
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We use the chemistry version of the Weather Research and Forecasting model coupled with spectral bin microphysics to investigate how meteorological conditions impact aerosol–cloud interactions (ACI) under different pollution regimes. Our findings highlight the changes in aerosol effects on clouds and precipitation under varying thermodynamic conditions, as well as the sensitivity of ACI to meteorological conditions under different pollution regimes, which help to clarify the mechanisms behind the nonlinear variation of ACI with environmental conditions.
Tom Eames, Nick Schutgens, Eleftherios Ioannidis, Ivar R. van der Velde, Max J. van Gerrevink, Roland Vernooij, and Guido R. van der Werf
Atmos. Chem. Phys., 25, 17429–17453, https://doi.org/10.5194/acp-25-17429-2025, https://doi.org/10.5194/acp-25-17429-2025, 2025
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Prescribed burning is used as a landscape management tool in southern African savannas. By deliberately changing the timing of fires in this region, the climate effect (radiative forcing) of a fire season can be altered. We show that by burning earlier in the dry season a small climate cooling effect can be achieved, similar to that of a 10 % reduction in global commercial aviation emissions. Local effects must be considered before implementing a fire regime shift for climate change mitigation.
Travis D. Toth, Marian B. Clayton, Zhujun Li, David Painemal, Sharon D. Rodier, Jayanta Kar, Tyler J. Thorsen, Richard A. Ferrare, Mark A. Vaughan, Jason L. Tackett, Huisheng Bian, Mian Chin, Anne E. Garnier, Ellsworth J. Welton, Robert A. Ryan, Charles R. Trepte, and David M. Winker
Atmos. Meas. Tech., 18, 6765–6793, https://doi.org/10.5194/amt-18-6765-2025, https://doi.org/10.5194/amt-18-6765-2025, 2025
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NASA's CALIPSO satellite mission observed aerosols (airborne particles) globally from 2006 to 2023. Its final data products update improves its aerosol optical parameters over oceans by adjusting for regional and seasonal differences in a new measurement-model synergistic approach. This results in a more realistic aerosol characterization, specifically near coastlines (where sea salt mixes with pollution), with potential impacts to future studies of science applications (e.g., climate effects).
Sudhakar Dipu, Johannes Mülmenstädt, and Johannes Quaas
EGUsphere, https://doi.org/10.5194/egusphere-2025-5064, https://doi.org/10.5194/egusphere-2025-5064, 2025
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High-resolution Large-Eddy Simulations (LES) are used to examine how aerosols affect liquid water path (LWP) sensitivity in non-precipitating liquid clouds. Two cases, 1985 (high aerosol) and 2013 (low aerosol), show a non-linear Nd–LWP relationship with a shift from positive to negative sensitivity at higher Nd under high aerosol loading. Enhanced cloud-top entrainment, evaporation, and heating drive this shift, highlighting aerosol impact on cloud microphysics and thermodynamics.
Zacharie Titus, Marine Bonazzola, Hélène Chepfer, Artem Feofilov, and Marie-Laure Roussel
EGUsphere, https://doi.org/10.5194/egusphere-2025-5335, https://doi.org/10.5194/egusphere-2025-5335, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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In this paper, we use satellite observations to study the relationships between profiles of clouds and profiles of wind from June to October around India. We found that thin clouds between 14 and 17 km are transported over the Arabian Sea by fast westward winds. We also show that the wind can be modified by 3 m/s because of the presence of deep convective clouds that spread out between 14 and 17 km of altitude. We discuss the implications of these interactions in a warming climate.
Naser Mahfouz, Hassan Beydoun, Johannes Mülmenstädt, Noel Keen, Adam C. Varble, Luca Bertagna, Peter Bogenschutz, Andrew Bradley, Matthew W. Christensen, T. Conrad Clevenger, Aaron Donahue, Jerome Fast, James Foucar, Jean-Christophe Golaz, Oksana Guba, Walter Hannah, Benjamin Hillman, Robert Jacob, Wuyin Lin, Po-Lun Ma, Yun Qian, Balwinder Singh, Christopher Terai, Hailong Wang, Mingxuan Wu, Kai Zhang, Andrew Gettelman, Mark Taylor, L. Ruby Leung, Peter Caldwell, and Susannah Burrows
Atmos. Chem. Phys., 25, 15105–15120, https://doi.org/10.5194/acp-25-15105-2025, https://doi.org/10.5194/acp-25-15105-2025, 2025
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Our study assesses the aerosol effective radiative forcing in a global cloud-resolving atmosphere model at ultra-high resolution. We demonstrate that global aerosol forcing signal can be robustly reproduced across resolutions when aerosol activation processes are carefully parameterized. Further, we argue that simplified prescribed aerosol schemes will open the door for further process/mechanism studies under controlled conditions.
Jason L. Tackett, Robert A. Ryan, Anne E. Garnier, Jayanta Kar, Brian J. Getzewich, Xia Cai, Mark A. Vaughan, Charles R. Trepte, Ron Verhappen, David M. Winker, and Kam-Pui A. Lee
Atmos. Meas. Tech., 18, 6211–6231, https://doi.org/10.5194/amt-18-6211-2025, https://doi.org/10.5194/amt-18-6211-2025, 2025
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The spaceborne atmospheric lidar CALIOP experienced an increasing number of intermittent low energy laser pulses in the final seven years of the 17-year long CALIPSO mission. Low energy pulses degraded the quality of retrievals in affected profiles. This paper describes low energy mitigation (LEM) algorithms that remove affected data and minimize data loss. LEM is demonstrated to correct calibration biases, reduce false feature detections, and restore the integrity of the CALIOP data record.
Charlotte Lange and Johannes Quaas
Atmos. Chem. Phys., 25, 10337–10359, https://doi.org/10.5194/acp-25-10337-2025, https://doi.org/10.5194/acp-25-10337-2025, 2025
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We studied how the Earth’s climate system adjusts to sudden changes in the energy budget by analysing data of four climate models, which simulated a 4 % reduction in incoming solar energy. We found rapid cooling of the atmosphere and shifts in cloud cover and atmospheric circulation patterns like land–sea circulation. Our research helps to better understand cloud adjustments, which are a major source of uncertainty in climate models. This can improve future climate predictions.
August Thomasson, Pontus Roldin, Nick Schutgens, Babitha George, Hugo Denier van der Gon, Guillaume Monteil, and Marko Scholze
EGUsphere, https://doi.org/10.5194/egusphere-2025-1568, https://doi.org/10.5194/egusphere-2025-1568, 2025
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We present top-down black carbon emissions estimates in Europe based on surface observations of concentrations at 24 rural sites from 2021. The annual emissions are 411 ± 10 Gg, overall 18 % higher compared to a traditional bottom-up estimate. Emissions are higher in for instance eastern Europe and the Iberian peninsula but lower in Poland and Italy. Validation with independent observations show overall better match and the uncertainties are reduced.
Sajedeh Marjani, Sina Mehrdad, and Johannes Quaas
EGUsphere, https://doi.org/10.5194/egusphere-2025-1847, https://doi.org/10.5194/egusphere-2025-1847, 2025
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A large part of aviation's climate impact comes from persistent contrails, not just carbon dioxide. This study examined how they evolve under different ice-supersaturated conditions, usually with background clouds. Using high-resolution simulations, we found that contrail growth depends on both the thickness of the supersaturated layer and available water vapor. Contrails can alter surrounding clouds and contribute to warming. Simple thresholds are not enough to predict their impact.
Goutam Choudhury, Karoline Block, Mahnoosh Haghighatnasab, Johannes Quaas, Tom Goren, and Matthias Tesche
Atmos. Chem. Phys., 25, 3841–3856, https://doi.org/10.5194/acp-25-3841-2025, https://doi.org/10.5194/acp-25-3841-2025, 2025
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Aerosol particles in the atmosphere increase cloud reflectivity, thereby cooling the Earth. Accurate global measurements of these particles are crucial for estimating this cooling effect. This study compares and harmonizes two newly developed global aerosol datasets, offering insights for their future use and refinement. We identify pristine oceans as a significant source of uncertainty in the datasets and, therefore, in quantifying the role of aerosols in Earth's climate.
Andrew Geiss and Po-Lun Ma
Geosci. Model Dev., 18, 1809–1827, https://doi.org/10.5194/gmd-18-1809-2025, https://doi.org/10.5194/gmd-18-1809-2025, 2025
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Particles in the Earth's atmosphere strongly impact the planet's energy budget, and atmosphere simulations require accurate representation of their interaction with light. This work introduces two approaches to represent light scattering by small particles. The first is a scattering simulator based on Mie theory implemented in Python. The second is a neural network emulator that is more accurate than existing methods and is fast enough to be used in climate and weather simulations.
Katherine M. Smith, Alice M. Barthel, LeAnn M. Conlon, Luke P. Van Roekel, Anthony Bartoletti, Jean-Christophe Golaz, Chengzhu Zhang, Carolyn Branecky Begeman, James J. Benedict, Gautam Bisht, Yan Feng, Walter Hannah, Bryce E. Harrop, Nicole Jeffery, Wuyin Lin, Po-Lun Ma, Mathew E. Maltrud, Mark R. Petersen, Balwinder Singh, Qi Tang, Teklu Tesfa, Jonathan D. Wolfe, Shaocheng Xie, Xue Zheng, Karthik Balaguru, Oluwayemi Garuba, Peter Gleckler, Aixue Hu, Jiwoo Lee, Ben Moore-Maley, and Ana C. Ordoñez
Geosci. Model Dev., 18, 1613–1633, https://doi.org/10.5194/gmd-18-1613-2025, https://doi.org/10.5194/gmd-18-1613-2025, 2025
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Version 2.1 of the U.S. Department of Energy's Energy Exascale Earth System Model (E3SM) adds the Fox-Kemper et al. (2011) mixed-layer eddy parameterization, which restratifies the ocean surface layer through an overturning streamfunction. Results include surface layer bias reduction in temperature, salinity, and sea ice extent in the North Atlantic; a small strengthening of the Atlantic meridional overturning circulation; and improvements to many atmospheric climatological variables.
Brandon M. Duran, Casey J. Wall, Nicholas J. Lutsko, Takuro Michibata, Po-Lun Ma, Yi Qin, Margaret L. Duffy, Brian Medeiros, and Matvey Debolskiy
Atmos. Chem. Phys., 25, 2123–2146, https://doi.org/10.5194/acp-25-2123-2025, https://doi.org/10.5194/acp-25-2123-2025, 2025
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We use satellite simulator data generated by global climate models to investigate how aerosol particles impact the radiative properties of liquid clouds. Specifically, we quantify the radiative perturbations arising from aerosol-driven changes in the number density of cloud droplets, the vertically integrated cloud water mass, and the cloud amount. Our results show that, in models, aerosol effects on the number density of cloud droplets contribute the most to anthropogenic climate forcing.
Johannes Mülmenstädt, Andrew S. Ackerman, Ann M. Fridlind, Meng Huang, Po-Lun Ma, Naser Mahfouz, Susanne E. Bauer, Susannah M. Burrows, Matthew W. Christensen, Sudhakar Dipu, Andrew Gettelman, L. Ruby Leung, Florian Tornow, Johannes Quaas, Adam C. Varble, Hailong Wang, Kai Zhang, and Youtong Zheng
Atmos. Chem. Phys., 24, 13633–13652, https://doi.org/10.5194/acp-24-13633-2024, https://doi.org/10.5194/acp-24-13633-2024, 2024
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Stratocumulus clouds play a large role in Earth's climate by reflecting incoming solar energy back to space. Turbulence at stratocumulus cloud top mixes in dry, warm air, which can lead to cloud dissipation. This process is challenging for coarse-resolution global models to represent. We show that global models nevertheless agree well with our process understanding. Global models also think the process is less important for the climate than other lines of evidence have led us to conclude.
Jianqi Zhao, Xiaoyan Ma, and Johannes Quaas
EGUsphere, https://doi.org/10.5194/egusphere-2024-3662, https://doi.org/10.5194/egusphere-2024-3662, 2024
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We conduct a comparative analysis of aerosol-cloud responses in liquid-phase clouds under different aerosol and meteorological conditions based on simulations using the WRF-Chem-SBM model. Our findings highlight the different effects of aerosols on clouds and precipitation, as well as variations in the roles of aerosol and meteorological factors influencing aerosol-cloud interactions, in different environment.
Iris Papakonstantinou-Presvelou and Johannes Quaas
EGUsphere, https://doi.org/10.5194/egusphere-2024-3293, https://doi.org/10.5194/egusphere-2024-3293, 2024
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As the Arctic warms and the sea ice retreats, more open ocean is exposed, changing how aerosols impact clouds. Our previous 10-year satellite analysis found higher ice crystal numbers over sea ice than over ocean. Using model simulations and aircraft observations we identify here two factors as potential causes at colder temperatures; ice nucleating particles over sea ice and blowing snow. With further sea ice loss, these processes may weaken, leading to fewer ice particles in the future.
Sina Mehrdad, Dörthe Handorf, Ines Höschel, Khalil Karami, Johannes Quaas, Sudhakar Dipu, and Christoph Jacobi
Weather Clim. Dynam., 5, 1223–1268, https://doi.org/10.5194/wcd-5-1223-2024, https://doi.org/10.5194/wcd-5-1223-2024, 2024
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This study introduces a novel deep learning (DL) approach to analyze how regional radiative forcing in Europe impacts the Arctic climate. By integrating atmospheric poleward energy transport with DL-based clustering of atmospheric patterns and attributing anomalies to specific clusters, our method reveals crucial, nuanced interactions within the climate system, enhancing our understanding of intricate climate dynamics.
Julien Lenhardt, Johannes Quaas, Dino Sejdinovic, and Daniel Klocke
EGUsphere, https://doi.org/10.5194/egusphere-2024-2724, https://doi.org/10.5194/egusphere-2024-2724, 2024
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Clouds come in various shapes and sizes and constitute a fundamental element of the Earth’s climate system. Different cloud types show variable impacts on climate change. We present a new cloud type classification method called CloudViT relying on spatial patterns of cloud properties obtained from satellite data using machine learning. We can thus help understanding the effects of different cloud types on climate change.
Julien Lenhardt, Johannes Quaas, and Dino Sejdinovic
Atmos. Meas. Tech., 17, 5655–5677, https://doi.org/10.5194/amt-17-5655-2024, https://doi.org/10.5194/amt-17-5655-2024, 2024
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Clouds play a key role in the regulation of the Earth's climate. Aspects like the height of their base are of essential interest to quantify their radiative effects but remain difficult to derive from satellite data. In this study, we combine observations from the surface and satellite retrievals of cloud properties to build a robust and accurate method to retrieve the cloud base height, based on a computer vision model and ordinal regression.
Jianqi Zhao, Xiaoyan Ma, Johannes Quaas, and Hailing Jia
Atmos. Chem. Phys., 24, 9101–9118, https://doi.org/10.5194/acp-24-9101-2024, https://doi.org/10.5194/acp-24-9101-2024, 2024
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We explore aerosol–cloud interactions in liquid-phase clouds over eastern China and its adjacent ocean in winter based on the WRF-Chem–SBM model, which couples a spectral-bin microphysics scheme and an online aerosol module. Our study highlights the differences in aerosol–cloud interactions between land and ocean and between precipitation clouds and non-precipitation clouds, and it differentiates and quantifies their underlying mechanisms.
Alexander Kutepov and Artem Feofilov
Geosci. Model Dev., 17, 5331–5347, https://doi.org/10.5194/gmd-17-5331-2024, https://doi.org/10.5194/gmd-17-5331-2024, 2024
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Infrared CO2 cooling of the middle and upper atmosphere is increasing. We developed a new routine for very fast and accurate calculations of this cooling in general circulation models. The new algorithm accounts for non-local thermodynamic equilibrium and is about 1000 times faster than the standard matrix algorithms. It is based on advanced techniques for non-equilibrium emission calculations in stellar atmospheres, which so far have not been used in Earth’s and planetary atmospheres.
Johannes Mülmenstädt, Edward Gryspeerdt, Sudhakar Dipu, Johannes Quaas, Andrew S. Ackerman, Ann M. Fridlind, Florian Tornow, Susanne E. Bauer, Andrew Gettelman, Yi Ming, Youtong Zheng, Po-Lun Ma, Hailong Wang, Kai Zhang, Matthew W. Christensen, Adam C. Varble, L. Ruby Leung, Xiaohong Liu, David Neubauer, Daniel G. Partridge, Philip Stier, and Toshihiko Takemura
Atmos. Chem. Phys., 24, 7331–7345, https://doi.org/10.5194/acp-24-7331-2024, https://doi.org/10.5194/acp-24-7331-2024, 2024
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Human activities release copious amounts of small particles called aerosols into the atmosphere. These particles change how much sunlight clouds reflect to space, an important human perturbation of the climate, whose magnitude is highly uncertain. We found that the latest climate models show a negative correlation but a positive causal relationship between aerosols and cloud water. This means we need to be very careful when we interpret observational studies that can only see correlation.
David Winker, Xia Cai, Mark Vaughan, Anne Garnier, Brian Magill, Melody Avery, and Brian Getzewich
Earth Syst. Sci. Data, 16, 2831–2855, https://doi.org/10.5194/essd-16-2831-2024, https://doi.org/10.5194/essd-16-2831-2024, 2024
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Clouds play important roles in both weather and climate. In this paper we describe version 1.0 of a unique global ice cloud data product derived from over 12 years of global spaceborne lidar measurements. This monthly gridded product provides a unique vertically resolved characterization of the occurrence and properties, optical and physical, of thin ice clouds and the tops of deep convective clouds. It should provide significant value for cloud research and model evaluation.
Charlotte M. Beall, Po-Lun Ma, Matthew W. Christensen, Johannes Mülmenstädt, Adam Varble, Kentaroh Suzuki, and Takuro Michibata
Atmos. Chem. Phys., 24, 5287–5302, https://doi.org/10.5194/acp-24-5287-2024, https://doi.org/10.5194/acp-24-5287-2024, 2024
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Single-layer warm liquid clouds cover nearly one-third of the Earth's surface, and uncertainties regarding the impact of aerosols on their radiative properties pose a significant challenge to climate prediction. Here, we demonstrate how satellite observations can be used to constrain Earth system model estimates of the radiative forcing from the interactions of aerosols with clouds due to warm rain processes.
Taufiq Hassan, Kai Zhang, Jianfeng Li, Balwinder Singh, Shixuan Zhang, Hailong Wang, and Po-Lun Ma
Geosci. Model Dev., 17, 3507–3532, https://doi.org/10.5194/gmd-17-3507-2024, https://doi.org/10.5194/gmd-17-3507-2024, 2024
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Anthropogenic aerosol emissions are an essential part of global aerosol models. Significant errors can exist from the loss of emission heterogeneity. We introduced an emission treatment that significantly improved aerosol emission heterogeneity in high-resolution model simulations, with improvements in simulated aerosol surface concentrations. The emission treatment will provide a more accurate representation of aerosol emissions and their effects on climate.
Bjorn Stevens, Stefan Adami, Tariq Ali, Hartwig Anzt, Zafer Aslan, Sabine Attinger, Jaana Bäck, Johanna Baehr, Peter Bauer, Natacha Bernier, Bob Bishop, Hendryk Bockelmann, Sandrine Bony, Guy Brasseur, David N. Bresch, Sean Breyer, Gilbert Brunet, Pier Luigi Buttigieg, Junji Cao, Christelle Castet, Yafang Cheng, Ayantika Dey Choudhury, Deborah Coen, Susanne Crewell, Atish Dabholkar, Qing Dai, Francisco Doblas-Reyes, Dale Durran, Ayoub El Gaidi, Charlie Ewen, Eleftheria Exarchou, Veronika Eyring, Florencia Falkinhoff, David Farrell, Piers M. Forster, Ariane Frassoni, Claudia Frauen, Oliver Fuhrer, Shahzad Gani, Edwin Gerber, Debra Goldfarb, Jens Grieger, Nicolas Gruber, Wilco Hazeleger, Rolf Herken, Chris Hewitt, Torsten Hoefler, Huang-Hsiung Hsu, Daniela Jacob, Alexandra Jahn, Christian Jakob, Thomas Jung, Christopher Kadow, In-Sik Kang, Sarah Kang, Karthik Kashinath, Katharina Kleinen-von Königslöw, Daniel Klocke, Uta Kloenne, Milan Klöwer, Chihiro Kodama, Stefan Kollet, Tobias Kölling, Jenni Kontkanen, Steve Kopp, Michal Koran, Markku Kulmala, Hanna Lappalainen, Fakhria Latifi, Bryan Lawrence, June Yi Lee, Quentin Lejeun, Christian Lessig, Chao Li, Thomas Lippert, Jürg Luterbacher, Pekka Manninen, Jochem Marotzke, Satoshi Matsouoka, Charlotte Merchant, Peter Messmer, Gero Michel, Kristel Michielsen, Tomoki Miyakawa, Jens Müller, Ramsha Munir, Sandeep Narayanasetti, Ousmane Ndiaye, Carlos Nobre, Achim Oberg, Riko Oki, Tuba Özkan-Haller, Tim Palmer, Stan Posey, Andreas Prein, Odessa Primus, Mike Pritchard, Julie Pullen, Dian Putrasahan, Johannes Quaas, Krishnan Raghavan, Venkatachalam Ramaswamy, Markus Rapp, Florian Rauser, Markus Reichstein, Aromar Revi, Sonakshi Saluja, Masaki Satoh, Vera Schemann, Sebastian Schemm, Christina Schnadt Poberaj, Thomas Schulthess, Cath Senior, Jagadish Shukla, Manmeet Singh, Julia Slingo, Adam Sobel, Silvina Solman, Jenna Spitzer, Philip Stier, Thomas Stocker, Sarah Strock, Hang Su, Petteri Taalas, John Taylor, Susann Tegtmeier, Georg Teutsch, Adrian Tompkins, Uwe Ulbrich, Pier-Luigi Vidale, Chien-Ming Wu, Hao Xu, Najibullah Zaki, Laure Zanna, Tianjun Zhou, and Florian Ziemen
Earth Syst. Sci. Data, 16, 2113–2122, https://doi.org/10.5194/essd-16-2113-2024, https://doi.org/10.5194/essd-16-2113-2024, 2024
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To manage Earth in the Anthropocene, new tools, new institutions, and new forms of international cooperation will be required. Earth Virtualization Engines is proposed as an international federation of centers of excellence to empower all people to respond to the immense and urgent challenges posed by climate change.
Sabine Doktorowski, Jan Kretzschmar, Johannes Quaas, Marc Salzmann, and Odran Sourdeval
Geosci. Model Dev., 17, 3099–3110, https://doi.org/10.5194/gmd-17-3099-2024, https://doi.org/10.5194/gmd-17-3099-2024, 2024
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Especially over the midlatitudes, precipitation is mainly formed via the ice phase. In this study we focus on the initial snow formation process in the ICON-AES, the aggregation process. We use a stochastical approach for the aggregation parameterization and investigate the influence in the ICON-AES. Therefore, a distribution function of cloud ice is created, which is evaluated with satellite data. The new approach leads to cloud ice loss and an improvement in the process rate bias.
Yu Yao, Po-Lun Ma, Yi Qin, Matthew W. Christensen, Hui Wan, Kai Zhang, Balwinder Singh, Meng Huang, and Mikhail Ovchinnikov
EGUsphere, https://doi.org/10.5194/egusphere-2024-523, https://doi.org/10.5194/egusphere-2024-523, 2024
Preprint withdrawn
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Giant aerosols have substantial effects on warm rain formation. However, it remains challenging to quantify the impact of giant particles at global scale. In this work, we applied earth system model to investigate its impacts by implementing new giant aerosol treatments to consider its physical process. We found this approach substantially affect liquid cloud and improved model's precipitation response to aerosols. Our findings demonstrate the significant impact of giant aerosols on climate.
Kirsten L. Findell, Zun Yin, Eunkyo Seo, Paul A. Dirmeyer, Nathan P. Arnold, Nathaniel Chaney, Megan D. Fowler, Meng Huang, David M. Lawrence, Po-Lun Ma, and Joseph A. Santanello Jr.
Geosci. Model Dev., 17, 1869–1883, https://doi.org/10.5194/gmd-17-1869-2024, https://doi.org/10.5194/gmd-17-1869-2024, 2024
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We outline a request for sub-daily data to accurately capture the process-level connections between land states, surface fluxes, and the boundary layer response. This high-frequency model output will allow for more direct comparison with observational field campaigns on process-relevant timescales, enable demonstration of inter-model spread in land–atmosphere coupling processes, and aid in targeted identification of sources of deficiencies and opportunities for improvement of the models.
Jianfeng Li, Kai Zhang, Taufiq Hassan, Shixuan Zhang, Po-Lun Ma, Balwinder Singh, Qiyang Yan, and Huilin Huang
Geosci. Model Dev., 17, 1327–1347, https://doi.org/10.5194/gmd-17-1327-2024, https://doi.org/10.5194/gmd-17-1327-2024, 2024
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By comparing E3SM simulations with and without regional refinement, we find that model horizontal grid spacing considerably affects the simulated aerosol mass budget, aerosol–cloud interactions, and the effective radiative forcing of anthropogenic aerosols. The study identifies the critical physical processes strongly influenced by model resolution. It also highlights the benefit of applying regional refinement in future modeling studies at higher or even convection-permitting resolutions.
Karoline Block, Mahnoosh Haghighatnasab, Daniel G. Partridge, Philip Stier, and Johannes Quaas
Earth Syst. Sci. Data, 16, 443–470, https://doi.org/10.5194/essd-16-443-2024, https://doi.org/10.5194/essd-16-443-2024, 2024
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Aerosols being able to act as condensation nuclei for cloud droplets (CCNs) are a key element in cloud formation but very difficult to determine. In this study we present a new global vertically resolved CCN dataset for various humidity conditions and aerosols. It is obtained using an atmospheric model (CAMS reanalysis) that is fed by satellite observations of light extinction (AOD). We investigate and evaluate the abundance of CCNs in the atmosphere and their temporal and spatial occurrence.
Yuying Zhang, Shaocheng Xie, Yi Qin, Wuyin Lin, Jean-Christophe Golaz, Xue Zheng, Po-Lun Ma, Yun Qian, Qi Tang, Christopher R. Terai, and Meng Zhang
Geosci. Model Dev., 17, 169–189, https://doi.org/10.5194/gmd-17-169-2024, https://doi.org/10.5194/gmd-17-169-2024, 2024
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We performed systematic evaluation of clouds simulated in the Energy
Exascale Earth System Model (E3SMv2) to document model performance and understand what updates in E3SMv2 have caused changes in clouds from E3SMv1 to E3SMv2. We find that stratocumulus clouds along the subtropical west coast of continents are dramatically improved, primarily due to the retuning done in CLUBB. This study offers additional insights into clouds simulated in E3SMv2 and will benefit future E3SM developments.
Exascale Earth System Model (E3SMv2) to document model performance and understand what updates in E3SMv2 have caused changes in clouds from E3SMv1 to E3SMv2. We find that stratocumulus clouds along the subtropical west coast of continents are dramatically improved, primarily due to the retuning done in CLUBB. This study offers additional insights into clouds simulated in E3SMv2 and will benefit future E3SM developments.
Shuaiqi Tang, Adam C. Varble, Jerome D. Fast, Kai Zhang, Peng Wu, Xiquan Dong, Fan Mei, Mikhail Pekour, Joseph C. Hardin, and Po-Lun Ma
Geosci. Model Dev., 16, 6355–6376, https://doi.org/10.5194/gmd-16-6355-2023, https://doi.org/10.5194/gmd-16-6355-2023, 2023
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To assess the ability of Earth system model (ESM) predictions, we developed a tool called ESMAC Diags to understand how aerosols, clouds, and aerosol–cloud interactions are represented in ESMs. This paper describes its version 2 functionality. We compared the model predictions with measurements taken by planes, ships, satellites, and ground instruments over four regions across the world. Results show that this new tool can help identify model problems and guide future development of ESMs.
Adam C. Varble, Po-Lun Ma, Matthew W. Christensen, Johannes Mülmenstädt, Shuaiqi Tang, and Jerome Fast
Atmos. Chem. Phys., 23, 13523–13553, https://doi.org/10.5194/acp-23-13523-2023, https://doi.org/10.5194/acp-23-13523-2023, 2023
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We evaluate how clouds change in response to changing atmospheric particle (aerosol) concentrations in a climate model and find that the model-predicted cloud brightness increases too much as aerosols increase because the cloud drop number increases too much. Excessive drizzle in the model mutes this difference. Many differences between observational and model estimates are explained by varying assumptions of how much liquid has been lost in clouds, which impacts the estimated cloud drop number.
Olivia Linke, Johannes Quaas, Finja Baumer, Sebastian Becker, Jan Chylik, Sandro Dahlke, André Ehrlich, Dörthe Handorf, Christoph Jacobi, Heike Kalesse-Los, Luca Lelli, Sina Mehrdad, Roel A. J. Neggers, Johannes Riebold, Pablo Saavedra Garfias, Niklas Schnierstein, Matthew D. Shupe, Chris Smith, Gunnar Spreen, Baptiste Verneuil, Kameswara S. Vinjamuri, Marco Vountas, and Manfred Wendisch
Atmos. Chem. Phys., 23, 9963–9992, https://doi.org/10.5194/acp-23-9963-2023, https://doi.org/10.5194/acp-23-9963-2023, 2023
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Lapse rate feedback (LRF) is a major driver of the Arctic amplification (AA) of climate change. It arises because the warming is stronger at the surface than aloft. Several processes can affect the LRF in the Arctic, such as the omnipresent temperature inversion. Here, we compare multimodel climate simulations to Arctic-based observations from a large research consortium to broaden our understanding of these processes, find synergy among them, and constrain the Arctic LRF and AA.
Athanasios Tsikerdekis, Otto P. Hasekamp, Nick A. J. Schutgens, and Qirui Zhong
Atmos. Chem. Phys., 23, 9495–9524, https://doi.org/10.5194/acp-23-9495-2023, https://doi.org/10.5194/acp-23-9495-2023, 2023
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Aerosols are tiny particles of different substances (species) that can be emitted into the atmosphere by natural processes or by anthropogenic activities. However, the actual aerosol emission amount per species is highly uncertain. Thus in this work we correct the aerosol emissions used to drive a global aerosol–climate model using satellite observations through a process called data assimilation. These more accurate aerosol emissions can lead to a more accurate weather and climate prediction.
Hao Luo, Johannes Quaas, and Yong Han
Atmos. Chem. Phys., 23, 8169–8186, https://doi.org/10.5194/acp-23-8169-2023, https://doi.org/10.5194/acp-23-8169-2023, 2023
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Clouds exhibit a wide range of vertical structures with varying microphysical and radiative properties. We show a global survey of spatial distribution, vertical extent and radiative effect of various classified cloud vertical structures using joint satellite observations from the new CCCM datasets during 2007–2010. Moreover, the long-term trends in CVSs are investigated based on different CMIP6 future scenarios to capture the cloud variations with different, increasing anthropogenic forcings.
Artem G. Feofilov, Hélène Chepfer, Vincent Noël, and Frederic Szczap
Atmos. Meas. Tech., 16, 3363–3390, https://doi.org/10.5194/amt-16-3363-2023, https://doi.org/10.5194/amt-16-3363-2023, 2023
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The response of clouds to human-induced climate warming remains the largest source of uncertainty in model predictions of climate. We consider cloud retrievals from spaceborne observations, the existing CALIOP lidar and future ATLID lidar; show how they compare for the same scenes; and discuss the advantage of adding a new lidar for detecting cloud changes in the long run. We show that ATLID's advanced technology should allow for better detecting thinner clouds during daytime than before.
Aishwarya Raman, Thomas Hill, Paul J. DeMott, Balwinder Singh, Kai Zhang, Po-Lun Ma, Mingxuan Wu, Hailong Wang, Simon P. Alexander, and Susannah M. Burrows
Atmos. Chem. Phys., 23, 5735–5762, https://doi.org/10.5194/acp-23-5735-2023, https://doi.org/10.5194/acp-23-5735-2023, 2023
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Ice-nucleating particles (INPs) play an important role in cloud processes and associated precipitation. Yet, INPs are not accurately represented in climate models. This study attempts to uncover these gaps by comparing model-simulated INP concentrations against field campaign measurements in the SO for an entire year, 2017–2018. Differences in INP concentrations and variability between the model and observations have major implications for modeling cloud properties in high latitudes.
Andrew Geiss, Po-Lun Ma, Balwinder Singh, and Joseph C. Hardin
Geosci. Model Dev., 16, 2355–2370, https://doi.org/10.5194/gmd-16-2355-2023, https://doi.org/10.5194/gmd-16-2355-2023, 2023
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Atmospheric aerosols play a critical role in Earth's climate, but it is too computationally expensive to directly model their interaction with radiation in climate simulations. This work develops a new neural-network-based parameterization of aerosol optical properties for use in the Energy Exascale Earth System Model that is much more accurate than the current one; it also introduces a unique model optimization method that involves randomly generating neural network architectures.
Samuel Kwakye, Heike Kalesse-Los, Maximilian Maahn, Patric Seifert, Roel van Klink, Christian Wirth, and Johannes Quaas
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2023-69, https://doi.org/10.5194/amt-2023-69, 2023
Publication in AMT not foreseen
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Insect numbers in the atmosphere can be calculated using polarimetric weather radar but they have to be identified and separated from other echoes, especially weather phenomena. Here, the separation is demonstrated using three machine-learning algorithms and insect count data from suction traps and the nature of radar measurements of different radar echoes is revealed. Random forest is the best separating algorithm and insect echoes radar measurements are distinct.
Jianqi Zhao, Xiaoyan Ma, Johannes Quaas, and Hailing Jia
EGUsphere, https://doi.org/10.5194/egusphere-2023-331, https://doi.org/10.5194/egusphere-2023-331, 2023
Preprint archived
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We improve the ability of WRF-Chem model to simulate aerosol-cloud physical and chemical processes by coupling a spectral-bin cloud microphysics scheme and online aerosol module, and consequently explore the aerosol-cloud interactions over eastern China and its adjacent ocean in boreal winter. Our study highlights the differences in aerosol-cloud interactions between land and ocean, precipitation clouds and non-precipitation clouds, and differentiates and quantifies their underlying mechanisms.
Matthew W. Christensen, Po-Lun Ma, Peng Wu, Adam C. Varble, Johannes Mülmenstädt, and Jerome D. Fast
Atmos. Chem. Phys., 23, 2789–2812, https://doi.org/10.5194/acp-23-2789-2023, https://doi.org/10.5194/acp-23-2789-2023, 2023
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An increase in aerosol concentration (tiny airborne particles) is shown to suppress rainfall and increase the abundance of droplets in clouds passing over Graciosa Island in the Azores. Cloud drops remain affected by aerosol for several days across thousands of kilometers in satellite data. Simulations from an Earth system model show good agreement, but differences in the amount of cloud water and its extent remain despite modifications to model parameters that control the warm-rain process.
Jason L. Tackett, Jayanta Kar, Mark A. Vaughan, Brian J. Getzewich, Man-Hae Kim, Jean-Paul Vernier, Ali H. Omar, Brian E. Magill, Michael C. Pitts, and David M. Winker
Atmos. Meas. Tech., 16, 745–768, https://doi.org/10.5194/amt-16-745-2023, https://doi.org/10.5194/amt-16-745-2023, 2023
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The accurate identification of aerosol types in the stratosphere is important to characterize their impacts on the Earth climate system. The space-borne lidar on board CALIPSO is well-posed to identify aerosols in the stratosphere from volcanic eruptions and major wildfire events. This paper describes improvements implemented in the version 4.5 CALIPSO data release to more accurately discriminate between volcanic ash, sulfate, and smoke within the stratosphere.
Alberto Caldas-Alvarez, Markus Augenstein, Georgy Ayzel, Klemens Barfus, Ribu Cherian, Lisa Dillenardt, Felix Fauer, Hendrik Feldmann, Maik Heistermann, Alexia Karwat, Frank Kaspar, Heidi Kreibich, Etor Emanuel Lucio-Eceiza, Edmund P. Meredith, Susanna Mohr, Deborah Niermann, Stephan Pfahl, Florian Ruff, Henning W. Rust, Lukas Schoppa, Thomas Schwitalla, Stella Steidl, Annegret H. Thieken, Jordis S. Tradowsky, Volker Wulfmeyer, and Johannes Quaas
Nat. Hazards Earth Syst. Sci., 22, 3701–3724, https://doi.org/10.5194/nhess-22-3701-2022, https://doi.org/10.5194/nhess-22-3701-2022, 2022
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In a warming climate, extreme precipitation events are becoming more frequent. To advance our knowledge on such phenomena, we present a multidisciplinary analysis of a selected case study that took place on 29 June 2017 in the Berlin metropolitan area. Our analysis provides evidence of the extremeness of the case from the atmospheric and the impacts perspectives as well as new insights on the physical mechanisms of the event at the meteorological and climate scales.
Johannes Quaas, Hailing Jia, Chris Smith, Anna Lea Albright, Wenche Aas, Nicolas Bellouin, Olivier Boucher, Marie Doutriaux-Boucher, Piers M. Forster, Daniel Grosvenor, Stuart Jenkins, Zbigniew Klimont, Norman G. Loeb, Xiaoyan Ma, Vaishali Naik, Fabien Paulot, Philip Stier, Martin Wild, Gunnar Myhre, and Michael Schulz
Atmos. Chem. Phys., 22, 12221–12239, https://doi.org/10.5194/acp-22-12221-2022, https://doi.org/10.5194/acp-22-12221-2022, 2022
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Pollution particles cool climate and offset part of the global warming. However, they are washed out by rain and thus their effect responds quickly to changes in emissions. We show multiple datasets to demonstrate that aerosol emissions and their concentrations declined in many regions influenced by human emissions, as did the effects on clouds. Consequently, the cooling impact on the Earth energy budget became smaller. This change in trend implies a relative warming.
Qirui Zhong, Nick Schutgens, Guido van der Werf, Twan van Noije, Kostas Tsigaridis, Susanne E. Bauer, Tero Mielonen, Alf Kirkevåg, Øyvind Seland, Harri Kokkola, Ramiro Checa-Garcia, David Neubauer, Zak Kipling, Hitoshi Matsui, Paul Ginoux, Toshihiko Takemura, Philippe Le Sager, Samuel Rémy, Huisheng Bian, Mian Chin, Kai Zhang, Jialei Zhu, Svetlana G. Tsyro, Gabriele Curci, Anna Protonotariou, Ben Johnson, Joyce E. Penner, Nicolas Bellouin, Ragnhild B. Skeie, and Gunnar Myhre
Atmos. Chem. Phys., 22, 11009–11032, https://doi.org/10.5194/acp-22-11009-2022, https://doi.org/10.5194/acp-22-11009-2022, 2022
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Aerosol optical depth (AOD) errors for biomass burning aerosol (BBA) are evaluated in 18 global models against satellite datasets. Notwithstanding biases in satellite products, they allow model evaluations. We observe large and diverse model biases due to errors in BBA. Further interpretations of AOD diversities suggest large biases exist in key processes for BBA which require better constraining. These results can contribute to further model improvement and development.
Meng Huang, Po-Lun Ma, Nathaniel W. Chaney, Dalei Hao, Gautam Bisht, Megan D. Fowler, Vincent E. Larson, and L. Ruby Leung
Geosci. Model Dev., 15, 6371–6384, https://doi.org/10.5194/gmd-15-6371-2022, https://doi.org/10.5194/gmd-15-6371-2022, 2022
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The land surface in one grid cell may be diverse in character. This study uses an explicit way to account for that subgrid diversity in a state-of-the-art Earth system model (ESM) and explores its implications for the overlying atmosphere. We find that the shallow clouds are increased significantly with the land surface diversity. Our work highlights the importance of accurately representing the land surface and its interaction with the atmosphere in next-generation ESMs.
Bernd Heinold, Holger Baars, Boris Barja, Matthew Christensen, Anne Kubin, Kevin Ohneiser, Kerstin Schepanski, Nick Schutgens, Fabian Senf, Roland Schrödner, Diego Villanueva, and Ina Tegen
Atmos. Chem. Phys., 22, 9969–9985, https://doi.org/10.5194/acp-22-9969-2022, https://doi.org/10.5194/acp-22-9969-2022, 2022
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The extreme 2019–2020 Australian wildfires produced massive smoke plumes lofted into the lower stratosphere by pyrocumulonimbus convection. Most climate models do not adequately simulate the injection height of such intense fires. By combining aerosol-climate modeling with prescribed pyroconvective smoke injection and lidar observations, this study shows the importance of the representation of the most extreme wildfire events for estimating the atmospheric energy budget.
Roland Vernooij, Patrik Winiger, Martin Wooster, Tercia Strydom, Laurent Poulain, Ulrike Dusek, Mark Grosvenor, Gareth J. Roberts, Nick Schutgens, and Guido R. van der Werf
Atmos. Meas. Tech., 15, 4271–4294, https://doi.org/10.5194/amt-15-4271-2022, https://doi.org/10.5194/amt-15-4271-2022, 2022
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Landscape fires are a substantial emitter of greenhouse gases and aerosols. Previous studies have indicated savanna emission factors to be highly variable. Improving fire emission estimates, and understanding future climate- and human-induced changes in fire regimes, requires in situ measurements. We present a drone-based method that enables the collection of a large amount of high-quality emission factor measurements that do not have the biases of aircraft or surface measurements.
Kai Zhang, Wentao Zhang, Hui Wan, Philip J. Rasch, Steven J. Ghan, Richard C. Easter, Xiangjun Shi, Yong Wang, Hailong Wang, Po-Lun Ma, Shixuan Zhang, Jian Sun, Susannah M. Burrows, Manish Shrivastava, Balwinder Singh, Yun Qian, Xiaohong Liu, Jean-Christophe Golaz, Qi Tang, Xue Zheng, Shaocheng Xie, Wuyin Lin, Yan Feng, Minghuai Wang, Jin-Ho Yoon, and L. Ruby Leung
Atmos. Chem. Phys., 22, 9129–9160, https://doi.org/10.5194/acp-22-9129-2022, https://doi.org/10.5194/acp-22-9129-2022, 2022
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Here we analyze the effective aerosol forcing simulated by E3SM version 1 using both century-long free-running and short nudged simulations. The aerosol forcing in E3SMv1 is relatively large compared to other models, mainly due to the large indirect aerosol effect. Aerosol-induced changes in liquid and ice cloud properties in E3SMv1 have a strong correlation. The aerosol forcing estimates in E3SMv1 are sensitive to the parameterization changes in both liquid and ice cloud processes.
Ovid O. Krüger, Bruna A. Holanda, Sourangsu Chowdhury, Andrea Pozzer, David Walter, Christopher Pöhlker, Maria Dolores Andrés Hernández, John P. Burrows, Christiane Voigt, Jos Lelieveld, Johannes Quaas, Ulrich Pöschl, and Mira L. Pöhlker
Atmos. Chem. Phys., 22, 8683–8699, https://doi.org/10.5194/acp-22-8683-2022, https://doi.org/10.5194/acp-22-8683-2022, 2022
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The abrupt reduction in human activities during the first COVID-19 lockdown created unprecedented atmospheric conditions. We took the opportunity to quantify changes in black carbon (BC) as a major anthropogenic air pollutant. Therefore, we measured BC on board a research aircraft over Europe during the lockdown and compared the results to measurements from 2017. With model simulations we account for different weather conditions and find a lockdown-related decrease in BC of 41 %.
Mahnoosh Haghighatnasab, Jan Kretzschmar, Karoline Block, and Johannes Quaas
Atmos. Chem. Phys., 22, 8457–8472, https://doi.org/10.5194/acp-22-8457-2022, https://doi.org/10.5194/acp-22-8457-2022, 2022
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The impact of aerosols emitted by the Holuhraun volcanic eruption on liquid clouds was assessed from a pair of cloud-system-resolving simulations along with satellite retrievals. Inside and outside the plume were compared in terms of their statistical distributions. Analyses indicated enhancement for cloud droplet number concentration inside the volcano plume in model simulations and satellite retrievals, while there was on average a small effect on both liquid water path and cloud fraction.
Assia Arouf, Hélène Chepfer, Thibault Vaillant de Guélis, Marjolaine Chiriaco, Matthew D. Shupe, Rodrigo Guzman, Artem Feofilov, Patrick Raberanto, Tristan S. L'Ecuyer, Seiji Kato, and Michael R. Gallagher
Atmos. Meas. Tech., 15, 3893–3923, https://doi.org/10.5194/amt-15-3893-2022, https://doi.org/10.5194/amt-15-3893-2022, 2022
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We proposed new estimates of the surface longwave (LW) cloud radiative effect (CRE) derived from observations collected by a space-based lidar on board the CALIPSO satellite and radiative transfer computations. Our estimate appropriately captures the surface LW CRE annual variability over bright polar surfaces, and it provides a dataset more than 13 years long.
Enza Di Tomaso, Jerónimo Escribano, Sara Basart, Paul Ginoux, Francesca Macchia, Francesca Barnaba, Francesco Benincasa, Pierre-Antoine Bretonnière, Arnau Buñuel, Miguel Castrillo, Emilio Cuevas, Paola Formenti, María Gonçalves, Oriol Jorba, Martina Klose, Lucia Mona, Gilbert Montané Pinto, Michail Mytilinaios, Vincenzo Obiso, Miriam Olid, Nick Schutgens, Athanasios Votsis, Ernest Werner, and Carlos Pérez García-Pando
Earth Syst. Sci. Data, 14, 2785–2816, https://doi.org/10.5194/essd-14-2785-2022, https://doi.org/10.5194/essd-14-2785-2022, 2022
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MONARCH reanalysis of desert dust aerosols extends the existing observation-based information for mineral dust monitoring by providing 3-hourly upper-air, surface and total column key geophysical variables of the dust cycle over Northern Africa, the Middle East and Europe, at a 0.1° horizontal resolution in a rotated grid, from 2007 to 2016. This work provides evidence of the high accuracy of this data set and its suitability for air quality and health and climate service applications.
Hailing Jia, Johannes Quaas, Edward Gryspeerdt, Christoph Böhm, and Odran Sourdeval
Atmos. Chem. Phys., 22, 7353–7372, https://doi.org/10.5194/acp-22-7353-2022, https://doi.org/10.5194/acp-22-7353-2022, 2022
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Aerosol–cloud interaction is the most uncertain component of the anthropogenic forcing of the climate. By combining satellite and reanalysis data, we show that the strength of the Twomey effect (S) increases remarkably with vertical velocity. Both the confounding effect of aerosol–precipitation interaction and the lack of vertical co-location between aerosol and cloud are found to overestimate S, whereas the retrieval biases in aerosol and cloud appear to underestimate S.
Shuaiqi Tang, Jerome D. Fast, Kai Zhang, Joseph C. Hardin, Adam C. Varble, John E. Shilling, Fan Mei, Maria A. Zawadowicz, and Po-Lun Ma
Geosci. Model Dev., 15, 4055–4076, https://doi.org/10.5194/gmd-15-4055-2022, https://doi.org/10.5194/gmd-15-4055-2022, 2022
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We developed an Earth system model (ESM) diagnostics package to compare various types of aerosol properties simulated in ESMs with aircraft, ship, and surface measurements from six field campaigns across spatial scales. The diagnostics package is coded and organized to be flexible and modular for future extension to other field campaign datasets and adapted to higher-resolution model simulations. Future releases will include comprehensive cloud and aerosol–cloud interaction diagnostics.
Susannah M. Burrows, Richard C. Easter, Xiaohong Liu, Po-Lun Ma, Hailong Wang, Scott M. Elliott, Balwinder Singh, Kai Zhang, and Philip J. Rasch
Atmos. Chem. Phys., 22, 5223–5251, https://doi.org/10.5194/acp-22-5223-2022, https://doi.org/10.5194/acp-22-5223-2022, 2022
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Sea spray particles are composed of a mixture of salts and organic substances from oceanic microorganisms. In prior work, our team developed an approach connecting sea spray chemistry to ocean biology, called OCEANFILMS. Here we describe its implementation within an Earth system model, E3SM. We show that simulated sea spray chemistry is consistent with observed seasonal cycles and that sunlight reflected by simulated Southern Ocean clouds increases, consistent with analysis of satellite data.
Athanasios Tsikerdekis, Nick A. J. Schutgens, Guangliang Fu, and Otto P. Hasekamp
Geosci. Model Dev., 15, 3253–3279, https://doi.org/10.5194/gmd-15-3253-2022, https://doi.org/10.5194/gmd-15-3253-2022, 2022
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In our study we quantify the ability of the future satellite sensor SPEXone, part of the NASA PACE mission, to estimate aerosol emissions. The sensor will be able to retrieve accurate information of aerosol light extinction and most importantly light absorption. We simulate SPEXone spatial coverage and combine it with an aerosol model. We found that SPEXone will be able to estimate species-specific (e.g. dust, sea salt, organic or black carbon, sulfates) aerosol emissions very accurately.
Po-Lun Ma, Bryce E. Harrop, Vincent E. Larson, Richard B. Neale, Andrew Gettelman, Hugh Morrison, Hailong Wang, Kai Zhang, Stephen A. Klein, Mark D. Zelinka, Yuying Zhang, Yun Qian, Jin-Ho Yoon, Christopher R. Jones, Meng Huang, Sheng-Lun Tai, Balwinder Singh, Peter A. Bogenschutz, Xue Zheng, Wuyin Lin, Johannes Quaas, Hélène Chepfer, Michael A. Brunke, Xubin Zeng, Johannes Mülmenstädt, Samson Hagos, Zhibo Zhang, Hua Song, Xiaohong Liu, Michael S. Pritchard, Hui Wan, Jingyu Wang, Qi Tang, Peter M. Caldwell, Jiwen Fan, Larry K. Berg, Jerome D. Fast, Mark A. Taylor, Jean-Christophe Golaz, Shaocheng Xie, Philip J. Rasch, and L. Ruby Leung
Geosci. Model Dev., 15, 2881–2916, https://doi.org/10.5194/gmd-15-2881-2022, https://doi.org/10.5194/gmd-15-2881-2022, 2022
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An alternative set of parameters for E3SM Atmospheric Model version 1 has been developed based on a tuning strategy that focuses on clouds. When clouds in every regime are improved, other aspects of the model are also improved, even though they are not the direct targets for calibration. The recalibrated model shows a lower sensitivity to anthropogenic aerosols and surface warming, suggesting potential improvements to the simulated climate in the past and future.
Thibault Vaillant de Guélis, Gérard Ancellet, Anne Garnier, Laurent C.-Labonnote, Jacques Pelon, Mark A. Vaughan, Zhaoyan Liu, and David M. Winker
Atmos. Meas. Tech., 15, 1931–1956, https://doi.org/10.5194/amt-15-1931-2022, https://doi.org/10.5194/amt-15-1931-2022, 2022
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A new IIR-based cloud and aerosol discrimination (CAD) algorithm is developed using the IIR brightness temperature differences for cloud and aerosol features confidently identified by the CALIOP version 4 CAD algorithm. IIR classifications agree with the majority of V4 cloud identifications, reduce the ambiguity in a notable fraction of
not confidentV4 cloud classifications, and correct a few V4 misclassifications of cloud layers identified as dense dust or elevated smoke layers by CALIOP.
Artem G. Feofilov, Hélène Chepfer, Vincent Noël, Rodrigo Guzman, Cyprien Gindre, Po-Lun Ma, and Marjolaine Chiriaco
Atmos. Meas. Tech., 15, 1055–1074, https://doi.org/10.5194/amt-15-1055-2022, https://doi.org/10.5194/amt-15-1055-2022, 2022
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Space-borne lidars have been providing invaluable information of atmospheric optical properties since 2006, and new lidar missions are on the way to ensure continuous observations. In this work, we compare the clouds estimated from space-borne ALADIN and CALIOP lidar observations. The analysis of collocated data shows that the agreement between the retrieved clouds is good up to 3 km height. Above that, ALADIN detects 40 % less clouds than CALIOP, except for polar stratospheric clouds (PSCs).
Michael R. Gallagher, Matthew D. Shupe, Hélène Chepfer, and Tristan L'Ecuyer
The Cryosphere, 16, 435–450, https://doi.org/10.5194/tc-16-435-2022, https://doi.org/10.5194/tc-16-435-2022, 2022
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By using direct observations of snowfall and mass changes, the variability of daily snowfall mass input to the Greenland ice sheet is quantified for the first time. With new methods we conclude that cyclones west of Greenland in summer contribute the most snowfall, with 1.66 Gt per occurrence. These cyclones are contextualized in the broader Greenland climate, and snowfall is validated against mass changes to verify the results. Snowfall and mass change observations are shown to agree well.
Matthew W. Christensen, Andrew Gettelman, Jan Cermak, Guy Dagan, Michael Diamond, Alyson Douglas, Graham Feingold, Franziska Glassmeier, Tom Goren, Daniel P. Grosvenor, Edward Gryspeerdt, Ralph Kahn, Zhanqing Li, Po-Lun Ma, Florent Malavelle, Isabel L. McCoy, Daniel T. McCoy, Greg McFarquhar, Johannes Mülmenstädt, Sandip Pal, Anna Possner, Adam Povey, Johannes Quaas, Daniel Rosenfeld, Anja Schmidt, Roland Schrödner, Armin Sorooshian, Philip Stier, Velle Toll, Duncan Watson-Parris, Robert Wood, Mingxi Yang, and Tianle Yuan
Atmos. Chem. Phys., 22, 641–674, https://doi.org/10.5194/acp-22-641-2022, https://doi.org/10.5194/acp-22-641-2022, 2022
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Trace gases and aerosols (tiny airborne particles) are released from a variety of point sources around the globe. Examples include volcanoes, industrial chimneys, forest fires, and ship stacks. These sources provide opportunistic experiments with which to quantify the role of aerosols in modifying cloud properties. We review the current state of understanding on the influence of aerosol on climate built from the wide range of natural and anthropogenic laboratories investigated in recent decades.
Zhonghua Zheng, Matthew West, Lei Zhao, Po-Lun Ma, Xiaohong Liu, and Nicole Riemer
Atmos. Chem. Phys., 21, 17727–17741, https://doi.org/10.5194/acp-21-17727-2021, https://doi.org/10.5194/acp-21-17727-2021, 2021
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Aerosol mixing state is an important emergent property that affects aerosol radiative forcing and aerosol–cloud interactions, but it has not been easy to constrain this property globally. We present a framework for evaluating the error in aerosol mixing state induced by aerosol representation assumptions, which is one of the important contributors to structural uncertainty in aerosol models. Our study provides insights into potential improvements to model process representation for aerosols.
Silke Trömel, Clemens Simmer, Ulrich Blahak, Armin Blanke, Sabine Doktorowski, Florian Ewald, Michael Frech, Mathias Gergely, Martin Hagen, Tijana Janjic, Heike Kalesse-Los, Stefan Kneifel, Christoph Knote, Jana Mendrok, Manuel Moser, Gregor Köcher, Kai Mühlbauer, Alexander Myagkov, Velibor Pejcic, Patric Seifert, Prabhakar Shrestha, Audrey Teisseire, Leonie von Terzi, Eleni Tetoni, Teresa Vogl, Christiane Voigt, Yuefei Zeng, Tobias Zinner, and Johannes Quaas
Atmos. Chem. Phys., 21, 17291–17314, https://doi.org/10.5194/acp-21-17291-2021, https://doi.org/10.5194/acp-21-17291-2021, 2021
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The article introduces the ACP readership to ongoing research in Germany on cloud- and precipitation-related process information inherent in polarimetric radar measurements, outlines pathways to inform atmospheric models with radar-based information, and points to remaining challenges towards an improved fusion of radar polarimetry and atmospheric modelling.
Raghavendra Krishnamurthy, Rob K. Newsom, Larry K. Berg, Heng Xiao, Po-Lun Ma, and David D. Turner
Atmos. Meas. Tech., 14, 4403–4424, https://doi.org/10.5194/amt-14-4403-2021, https://doi.org/10.5194/amt-14-4403-2021, 2021
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Planetary boundary layer (PBL) height is a critical parameter in atmospheric models. Continuous PBL height measurements from remote sensing measurements are important to understand various boundary layer mechanisms, especially during daytime and evening transition periods. Due to several limitations in existing methodologies to detect PBL height from a Doppler lidar, in this study, a machine learning (ML) approach is tested. The ML model is observed to improve the accuracy by over 50 %.
Sam J. Silva, Po-Lun Ma, Joseph C. Hardin, and Daniel Rothenberg
Geosci. Model Dev., 14, 3067–3077, https://doi.org/10.5194/gmd-14-3067-2021, https://doi.org/10.5194/gmd-14-3067-2021, 2021
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The activation of aerosol into cloud droplets is an important but uncertain process in the Earth system. The physical and chemical interactions that govern this process are too computationally expensive to explicitly resolve in modern Earth system models. Here, we demonstrate how hybrid machine learning approaches can provide a potential path forward, enabling the representation of the more detailed physics and chemistry at a reduced computational cost while still retaining physical information.
Nick Schutgens, Oleg Dubovik, Otto Hasekamp, Omar Torres, Hiren Jethva, Peter J. T. Leonard, Pavel Litvinov, Jens Redemann, Yohei Shinozuka, Gerrit de Leeuw, Stefan Kinne, Thomas Popp, Michael Schulz, and Philip Stier
Atmos. Chem. Phys., 21, 6895–6917, https://doi.org/10.5194/acp-21-6895-2021, https://doi.org/10.5194/acp-21-6895-2021, 2021
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Absorptive aerosol has a potentially large impact on climate change. We evaluate and intercompare four global satellite datasets of absorptive aerosol optical depth (AAOD) and single-scattering albedo (SSA). We show that these datasets show reasonable correlations with the AErosol RObotic NETwork (AERONET) reference, although significant biases remain. In a follow-up paper we show that these observations nevertheless can be used for model evaluation.
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Short summary
Aerosol has a large impact on climate. Using a lidar aerosol simulator ensures consistent comparisons between modeled and observed aerosol. We present a lidar aerosol simulator that applies a cloud masking and an aerosol detection threshold. We estimate the lidar signals that would be observed at 532 nm by the Cloud-Aerosol Lidar with Orthogonal Polarization overflying the atmosphere predicted by a climate model. Our comparison at the seasonal timescale shows a discrepancy in the Southern Ocean.
Aerosol has a large impact on climate. Using a lidar aerosol simulator ensures consistent...
