Articles | Volume 16, issue 9
https://doi.org/10.5194/gmd-16-2649-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/gmd-16-2649-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Model description paper
| 
17 May 2023
Model description paper |
| 17 May 2023
| 17 May 2023
The 3D biogeochemical marine mercury cycling model MERCY v2.0 – linking atmospheric Hg to methylmercury in fish
Johannes Bieser
CORRESPONDING AUTHOR
Institute of Coastal Systems – Analysis and Modeling, Helmholtz-Zentrum Hereon,
Max-Planck-Str. 1, 21502 Geesthacht, Germany
David J. Amptmeijer
Institute of Coastal Systems – Analysis and Modeling, Helmholtz-Zentrum Hereon,
Max-Planck-Str. 1, 21502 Geesthacht, Germany
Ute Daewel
Institute of Coastal Systems – Analysis and Modeling, Helmholtz-Zentrum Hereon,
Max-Planck-Str. 1, 21502 Geesthacht, Germany
Joachim Kuss
Department of Marine Chemistry, Leibniz Institute for Baltic Sea Research, Seestraße 15, 18119 Rostock, Germany
Anne L. Soerensen
Department of Environmental
Research and Monitoring, Swedish Museum of Natural History, Stockholm, Sweden
Corinna Schrum
Institute of Coastal Systems – Analysis and Modeling, Helmholtz-Zentrum Hereon,
Max-Planck-Str. 1, 21502 Geesthacht, Germany
Institute of Oceanography, Universität Hamburg, Mittelweg
177, 20146 Hamburg, Germany
Related authors
Danilo Custódio, Katrine Aspmo Pfaffhuber, T. Gerard Spain, Fidel F. Pankratov, Iana Strigunova, Koketso Molepo, Henrik Skov, Johannes Bieser, and Ralf Ebinghaus
Atmos. Chem. Phys., 22, 3827–3840, https://doi.org/10.5194/acp-22-3827-2022, https://doi.org/10.5194/acp-22-3827-2022, 2022
Short summary
Short summary
As a poison in the air that we breathe and the food that we eat, mercury is a human health concern for society as a whole. In that regard, this work deals with monitoring and modelling mercury in the environment, improving wherewithal, identifying the strength of the different components at play, and interpreting information to support the efforts that seek to safeguard public health.
Stefano Galmarini, Paul Makar, Olivia E. Clifton, Christian Hogrefe, Jesse O. Bash, Roberto Bellasio, Roberto Bianconi, Johannes Bieser, Tim Butler, Jason Ducker, Johannes Flemming, Alma Hodzic, Christopher D. Holmes, Ioannis Kioutsioukis, Richard Kranenburg, Aurelia Lupascu, Juan Luis Perez-Camanyo, Jonathan Pleim, Young-Hee Ryu, Roberto San Jose, Donna Schwede, Sam Silva, and Ralf Wolke
Atmos. Chem. Phys., 21, 15663–15697, https://doi.org/10.5194/acp-21-15663-2021, https://doi.org/10.5194/acp-21-15663-2021, 2021
Short summary
Short summary
This technical note presents the research protocols for phase 4 of the Air Quality Model Evaluation International Initiative (AQMEII4). This initiative has three goals: (i) to define the state of wet and dry deposition in regional models, (ii) to evaluate how dry deposition influences air concentration and flux predictions, and (iii) to identify the causes for prediction differences. The evaluation compares LULC-specific dry deposition and effective conductances and fluxes.
Johannes Bieser, Hélène Angot, Franz Slemr, and Lynwill Martin
Atmos. Chem. Phys., 20, 10427–10439, https://doi.org/10.5194/acp-20-10427-2020, https://doi.org/10.5194/acp-20-10427-2020, 2020
Short summary
Short summary
We use numerical models to determine the origin of air masses measured for elemental gaseous mercury (GEM) at Cape Point (CPT), South Africa. Our analysis is based on 10 years of hourly GEM measurements at CPT from 2007 to 2016. Based on GEM concentration and the origin of the air mass, we identify source and sink regions at CPT. We find, that the warm Agulhas Current to the south-east is the major Hg source and the continent the major sink.
Danilo Custodio, Ralf Ebinghaus, T. Gerard Spain, and Johannes Bieser
Atmos. Chem. Phys., 20, 7929–7939, https://doi.org/10.5194/acp-20-7929-2020, https://doi.org/10.5194/acp-20-7929-2020, 2020
Short summary
Short summary
Using a stereo algorithm, we reconstructed 99.9 % of the total atmospheric gas mercury and presented a new insight into atmospheric mercury source assessing, which can have great relevance for policy and regulations in light of the Minamata convention.
Franz Slemr, Lynwill Martin, Casper Labuschagne, Thumeka Mkololo, Hélène Angot, Olivier Magand, Aurélien Dommergue, Philippe Garat, Michel Ramonet, and Johannes Bieser
Atmos. Chem. Phys., 20, 7683–7692, https://doi.org/10.5194/acp-20-7683-2020, https://doi.org/10.5194/acp-20-7683-2020, 2020
Short summary
Short summary
Monitoring of atmospheric mercury (Hg) concentrations is an important part of the effectiveness evaluation of the Minamata Convention on Hg. Hg concentrations in 2012–2017 at Cape Point, South Africa, and at Amsterdam Island in the remote Indian Ocean are comparable, and no trend or a slightly downward trend was observed at both stations. Over the 2007–2017 period an upward trend was observed at CPT which was driven mainly by the 2007–2014 data. The trend and its change are discussed.
Martin Otto Paul Ramacher, Matthias Karl, Johannes Bieser, Jukka-Pekka Jalkanen, and Lasse Johansson
Atmos. Chem. Phys., 19, 9153–9179, https://doi.org/10.5194/acp-19-9153-2019, https://doi.org/10.5194/acp-19-9153-2019, 2019
Short summary
Short summary
We simulated the impact of NOx shipping emissions on air quality and exposure in the Baltic Sea harbour cities Rostock (Germany), Riga (Latvia) and Gdańsk–Gdynia (Poland) for 2012. We found that local shipping affects total NO2, with contributions of 22 %, 11 % and 16 % in Rostock, Riga and Gdańsk–Gdynia. Exposure to NO2 from all emission sources was highest at home addresses (54 %–59 %). Emissions from shipping have a high impact on NO2 exposure in the port area (50 %–80 %).
Matthias Karl, Johannes Bieser, Beate Geyer, Volker Matthias, Jukka-Pekka Jalkanen, Lasse Johansson, and Erik Fridell
Atmos. Chem. Phys., 19, 1721–1752, https://doi.org/10.5194/acp-19-1721-2019, https://doi.org/10.5194/acp-19-1721-2019, 2019
Short summary
Short summary
Air emissions of nitrogen oxides from ship traffic in the Baltic Sea are a health concern in coastal areas of the Baltic Sea region. We find that the introduction of the nitrogen emission control area (NECA) is critical for reducing ship emissions of nitrogen oxides to levels that are low enough to sustainably dampen ozone production. The decline of the ship-related nitrogen deposition to the Baltic Sea between 2012 and 2040 varies between 46 % and 78 % in different regulation scenarios.
Gabriele Curci, Ummugulsum Alyuz, Rocio Barò, Roberto Bianconi, Johannes Bieser, Jesper H. Christensen, Augustin Colette, Aidan Farrow, Xavier Francis, Pedro Jiménez-Guerrero, Ulas Im, Peng Liu, Astrid Manders, Laura Palacios-Peña, Marje Prank, Luca Pozzoli, Ranjeet Sokhi, Efisio Solazzo, Paolo Tuccella, Alper Unal, Marta G. Vivanco, Christian Hogrefe, and Stefano Galmarini
Atmos. Chem. Phys., 19, 181–204, https://doi.org/10.5194/acp-19-181-2019, https://doi.org/10.5194/acp-19-181-2019, 2019
Short summary
Short summary
Atmospheric carbonaceous aerosols are able to absorb solar radiation and they continue to contribute some of the largest uncertainties in projected climate change. One important detail is how the chemical species are arranged inside each particle, i.e. the knowledge of their mixing state. We use an ensemble of regional model simulations to test different mixing state assumptions and found that a combination of internal and external mixing may better reproduce sunphotometer observations.
Peng Liu, Christian Hogrefe, Ulas Im, Jesper H. Christensen, Johannes Bieser, Uarporn Nopmongcol, Greg Yarwood, Rohit Mathur, Shawn Roselle, and Tanya Spero
Atmos. Chem. Phys., 18, 17157–17175, https://doi.org/10.5194/acp-18-17157-2018, https://doi.org/10.5194/acp-18-17157-2018, 2018
Short summary
Short summary
This study represents an intercomparison of four regional-scale air quality simulations in order to understand the model similarities and differences in estimating the impact of ozone imported from outside of the US on the surface ozone within the US at process level. Vertical turbulent mixing stands out as a primary contributor to the model differences in inert tracers.
Marina Astitha, Ioannis Kioutsioukis, Ghezae Araya Fisseha, Roberto Bianconi, Johannes Bieser, Jesper H. Christensen, Owen R. Cooper, Stefano Galmarini, Christian Hogrefe, Ulas Im, Bryan Johnson, Peng Liu, Uarporn Nopmongcol, Irina Petropavlovskikh, Efisio Solazzo, David W. Tarasick, and Greg Yarwood
Atmos. Chem. Phys., 18, 13925–13945, https://doi.org/10.5194/acp-18-13925-2018, https://doi.org/10.5194/acp-18-13925-2018, 2018
Short summary
Short summary
This work is unique in the detailed analyses of modeled ozone vertical profiles from sites in North America through the collaboration of four research groups from the US and EU. We assess the air quality models' performance and model inter-comparison for ozone vertical profiles and stratospheric ozone intrusions. Lastly, we designate the important role of lateral boundary conditions in the ozone vertical profiles using chemically inert tracers.
Franz Slemr, Andreas Weigelt, Ralf Ebinghaus, Johannes Bieser, Carl A. M. Brenninkmeijer, Armin Rauthe-Schöch, Markus Hermann, Bengt G. Martinsson, Peter van Velthoven, Harald Bönisch, Marco Neumaier, Andreas Zahn, and Helmut Ziereis
Atmos. Chem. Phys., 18, 12329–12343, https://doi.org/10.5194/acp-18-12329-2018, https://doi.org/10.5194/acp-18-12329-2018, 2018
Short summary
Short summary
Total and elemental mercury were measured in the upper troposphere and lower stratosphere onboard a passenger aircraft. Their concentrations in the upper troposphere were comparable implying low concentrations of oxidized mercury in this region. Large scale seasonally dependent influence of emissions from biomass burning was also observed. Their distributions in the lower stratosphere implies a long stratospheric lifetime, which precludes significant mercury oxidation by ozone.
Marta G. Vivanco, Mark R. Theobald, Héctor García-Gómez, Juan Luis Garrido, Marje Prank, Wenche Aas, Mario Adani, Ummugulsum Alyuz, Camilla Andersson, Roberto Bellasio, Bertrand Bessagnet, Roberto Bianconi, Johannes Bieser, Jørgen Brandt, Gino Briganti, Andrea Cappelletti, Gabriele Curci, Jesper H. Christensen, Augustin Colette, Florian Couvidat, Cornelis Cuvelier, Massimo D'Isidoro, Johannes Flemming, Andrea Fraser, Camilla Geels, Kaj M. Hansen, Christian Hogrefe, Ulas Im, Oriol Jorba, Nutthida Kitwiroon, Astrid Manders, Mihaela Mircea, Noelia Otero, Maria-Teresa Pay, Luca Pozzoli, Efisio Solazzo, Svetlana Tsyro, Alper Unal, Peter Wind, and Stefano Galmarini
Atmos. Chem. Phys., 18, 10199–10218, https://doi.org/10.5194/acp-18-10199-2018, https://doi.org/10.5194/acp-18-10199-2018, 2018
Short summary
Short summary
European wet and dry atmospheric deposition of N and S estimated by 14 air quality models was found to vary substantially. An ensemble of models meeting acceptability criteria was used to estimate the exceedances of the critical loads for N in habitats within the Natura 2000 network, as well as their lower and upper limits. Scenarios with 20 % emission reductions in different regions of the world showed that European emissions are responsible for most of the N and S deposition in Europe.
Ulas Im, Jesper Heile Christensen, Camilla Geels, Kaj Mantzius Hansen, Jørgen Brandt, Efisio Solazzo, Ummugulsum Alyuz, Alessandra Balzarini, Rocio Baro, Roberto Bellasio, Roberto Bianconi, Johannes Bieser, Augustin Colette, Gabriele Curci, Aidan Farrow, Johannes Flemming, Andrea Fraser, Pedro Jimenez-Guerrero, Nutthida Kitwiroon, Peng Liu, Uarporn Nopmongcol, Laura Palacios-Peña, Guido Pirovano, Luca Pozzoli, Marje Prank, Rebecca Rose, Ranjeet Sokhi, Paolo Tuccella, Alper Unal, Marta G. Vivanco, Greg Yarwood, Christian Hogrefe, and Stefano Galmarini
Atmos. Chem. Phys., 18, 8929–8952, https://doi.org/10.5194/acp-18-8929-2018, https://doi.org/10.5194/acp-18-8929-2018, 2018
Short summary
Short summary
We evaluate the impact of global and regional anthropogenic emission reductions on major air pollutant levels over Europe and North America, using a multi-model ensemble of regional chemistry and transport models. Results show that ozone levels are largely driven by long-range transport over both continents while other pollutants such as carbon monoxide or aerosols are mainly controlled by domestic sources. Use of multi-model ensembles can help to reduce the uncertainties in individual models.
Stefano Galmarini, Ioannis Kioutsioukis, Efisio Solazzo, Ummugulsum Alyuz, Alessandra Balzarini, Roberto Bellasio, Anna M. K. Benedictow, Roberto Bianconi, Johannes Bieser, Joergen Brandt, Jesper H. Christensen, Augustin Colette, Gabriele Curci, Yanko Davila, Xinyi Dong, Johannes Flemming, Xavier Francis, Andrea Fraser, Joshua Fu, Daven K. Henze, Christian Hogrefe, Ulas Im, Marta Garcia Vivanco, Pedro Jiménez-Guerrero, Jan Eiof Jonson, Nutthida Kitwiroon, Astrid Manders, Rohit Mathur, Laura Palacios-Peña, Guido Pirovano, Luca Pozzoli, Marie Prank, Martin Schultz, Rajeet S. Sokhi, Kengo Sudo, Paolo Tuccella, Toshihiko Takemura, Takashi Sekiya, and Alper Unal
Atmos. Chem. Phys., 18, 8727–8744, https://doi.org/10.5194/acp-18-8727-2018, https://doi.org/10.5194/acp-18-8727-2018, 2018
Short summary
Short summary
An ensemble of model results relating to ozone concentrations in Europe in 2010 has been produced and studied. The novelty consists in the fact that the ensemble is made of results of models working at two different scales (regional and global), therefore contributing in detail two different parts of the atmospheric spectrum. The ensemble defined as a hybrid has been studied in detail and shown to bring additional value to the assessment of air quality.
Ulas Im, Jørgen Brandt, Camilla Geels, Kaj Mantzius Hansen, Jesper Heile Christensen, Mikael Skou Andersen, Efisio Solazzo, Ioannis Kioutsioukis, Ummugulsum Alyuz, Alessandra Balzarini, Rocio Baro, Roberto Bellasio, Roberto Bianconi, Johannes Bieser, Augustin Colette, Gabriele Curci, Aidan Farrow, Johannes Flemming, Andrea Fraser, Pedro Jimenez-Guerrero, Nutthida Kitwiroon, Ciao-Kai Liang, Uarporn Nopmongcol, Guido Pirovano, Luca Pozzoli, Marje Prank, Rebecca Rose, Ranjeet Sokhi, Paolo Tuccella, Alper Unal, Marta Garcia Vivanco, Jason West, Greg Yarwood, Christian Hogrefe, and Stefano Galmarini
Atmos. Chem. Phys., 18, 5967–5989, https://doi.org/10.5194/acp-18-5967-2018, https://doi.org/10.5194/acp-18-5967-2018, 2018
Short summary
Short summary
The impacts of air pollution on human health and their costs in Europe and the United States for the year 2010 ared modeled by a multi-model ensemble. In Europe, the number of premature deaths is calculated to be 414 000, while in the US it is estimated to be 160 000. Health impacts estimated by individual models can vary up to a factor of 3. Results show that the domestic emissions have the largest impact on premature deaths, compared to foreign sources.
Johannes Bieser, Franz Slemr, Jesse Ambrose, Carl Brenninkmeijer, Steve Brooks, Ashu Dastoor, Francesco DeSimone, Ralf Ebinghaus, Christian N. Gencarelli, Beate Geyer, Lynne E. Gratz, Ian M. Hedgecock, Daniel Jaffe, Paul Kelley, Che-Jen Lin, Lyatt Jaegle, Volker Matthias, Andrei Ryjkov, Noelle E. Selin, Shaojie Song, Oleg Travnikov, Andreas Weigelt, Winston Luke, Xinrong Ren, Andreas Zahn, Xin Yang, Yun Zhu, and Nicola Pirrone
Atmos. Chem. Phys., 17, 6925–6955, https://doi.org/10.5194/acp-17-6925-2017, https://doi.org/10.5194/acp-17-6925-2017, 2017
Short summary
Short summary
We conducted a multi model study to investigate our ability to reproduce the vertical distribution of mercury in the atmosphere. For this, we used observational data from over 40 aircraft flights in EU and US. We compared observations to the results of seven chemistry transport models and found that the models are able to reproduce vertical gradients of total and elemental Hg. Finally, we found that different chemical reactions seem responsible for the oxidation of Hg depending on altitude.
Oleg Travnikov, Hélène Angot, Paulo Artaxo, Mariantonia Bencardino, Johannes Bieser, Francesco D'Amore, Ashu Dastoor, Francesco De Simone, María del Carmen Diéguez, Aurélien Dommergue, Ralf Ebinghaus, Xin Bin Feng, Christian N. Gencarelli, Ian M. Hedgecock, Olivier Magand, Lynwill Martin, Volker Matthias, Nikolay Mashyanov, Nicola Pirrone, Ramesh Ramachandran, Katie Alana Read, Andrei Ryjkov, Noelle E. Selin, Fabrizio Sena, Shaojie Song, Francesca Sprovieri, Dennis Wip, Ingvar Wängberg, and Xin Yang
Atmos. Chem. Phys., 17, 5271–5295, https://doi.org/10.5194/acp-17-5271-2017, https://doi.org/10.5194/acp-17-5271-2017, 2017
Short summary
Short summary
The study provides a complex analysis of processes governing Hg fate in the atmosphere involving both measurement data and simulation results of chemical transport models. Evaluation of the model simulations and numerical experiments against observations allows explaining spatial and temporal variations of Hg concentration in the near-surface atmospheric layer and shows possibility of multiple pathways of Hg oxidation occurring concurrently in various parts of the atmosphere.
Efisio Solazzo, Roberto Bianconi, Christian Hogrefe, Gabriele Curci, Paolo Tuccella, Ummugulsum Alyuz, Alessandra Balzarini, Rocío Baró, Roberto Bellasio, Johannes Bieser, Jørgen Brandt, Jesper H. Christensen, Augistin Colette, Xavier Francis, Andrea Fraser, Marta Garcia Vivanco, Pedro Jiménez-Guerrero, Ulas Im, Astrid Manders, Uarporn Nopmongcol, Nutthida Kitwiroon, Guido Pirovano, Luca Pozzoli, Marje Prank, Ranjeet S. Sokhi, Alper Unal, Greg Yarwood, and Stefano Galmarini
Atmos. Chem. Phys., 17, 3001–3054, https://doi.org/10.5194/acp-17-3001-2017, https://doi.org/10.5194/acp-17-3001-2017, 2017
Short summary
Short summary
As part of the third phase of AQMEII, this study uses timescale analysis to apportion error to the responsible processes, detect causes of model error, and identify the processes and scales that require dedicated investigations. The analysis tackles model performance gauging through measurement-to-model comparison, error decomposition, and time series analysis of model biases for ozone, CO, SO2, NO, NO2, PM10, PM2.5, wind speed, and temperature over Europe and North America.
Christian N. Gencarelli, Johannes Bieser, Francesco Carbone, Francesco De Simone, Ian M. Hedgecock, Volker Matthias, Oleg Travnikov, Xin Yang, and Nicola Pirrone
Atmos. Chem. Phys., 17, 627–643, https://doi.org/10.5194/acp-17-627-2017, https://doi.org/10.5194/acp-17-627-2017, 2017
Short summary
Short summary
Atmospheric deposition is an important pathway by which Hg reaches marine ecosystems, where it can be methylated and enter the base of food chain. High resolution numerical experiments has been performed in order to investigate the contributions (sensitivity) of the Hg anthtropogenic emissions, speciation and atmospherical chemical reactions on Hg depositions over Europe. The comparison of wet deposition fluxes and concentrations measured on 28 monitioring sites were used to support the analysis.
Christos I. Efstathiou, Jana Matejovičová, Johannes Bieser, and Gerhard Lammel
Atmos. Chem. Phys., 16, 15327–15345, https://doi.org/10.5194/acp-16-15327-2016, https://doi.org/10.5194/acp-16-15327-2016, 2016
Short summary
Short summary
Gas-particle partitioning is an important process that determines the fate and long-range transport potential of persistent organic pollutants. This work is the first effort to evaluate the behaviour of parameterizations within a regional air quality system adapted for Europe. Results corroborate the significance of the chosen implementation in predicting ambient levels and transport patterns. Implications point to improvements on the side of the emission inventories and aerosol module.
Andreas Weigelt, Franz Slemr, Ralf Ebinghaus, Nicola Pirrone, Johannes Bieser, Jan Bödewadt, Giulio Esposito, and Peter F. J. van Velthoven
Atmos. Chem. Phys., 16, 13653–13668, https://doi.org/10.5194/acp-16-13653-2016, https://doi.org/10.5194/acp-16-13653-2016, 2016
Short summary
Short summary
Hg ∕ SO2, Hg ∕ CO, and NOx ∕ SO2 emission ratios (ERs) in the plume of the coal-fired power plant (CFPP), Lippendorf, near Leipzig in Germany, were determined in August 2013. GOM fraction of mercury emissions was also assessed. Measured Hg ∕ SO2 and Hg ∕ CO ERs were consistent with the ratios calculated from annual emissions in 2013 reported by the CFPP operator. The NOx ∕ SO2 ER was somewhat lower. GOM fractions of ~ 40 % of CFPP mercury emissions in current emission inventories are overestimated.
Bertrand Bessagnet, Guido Pirovano, Mihaela Mircea, Cornelius Cuvelier, Armin Aulinger, Giuseppe Calori, Giancarlo Ciarelli, Astrid Manders, Rainer Stern, Svetlana Tsyro, Marta García Vivanco, Philippe Thunis, Maria-Teresa Pay, Augustin Colette, Florian Couvidat, Frédérik Meleux, Laurence Rouïl, Anthony Ung, Sebnem Aksoyoglu, José María Baldasano, Johannes Bieser, Gino Briganti, Andrea Cappelletti, Massimo D'Isidoro, Sandro Finardi, Richard Kranenburg, Camillo Silibello, Claudio Carnevale, Wenche Aas, Jean-Charles Dupont, Hilde Fagerli, Lucia Gonzalez, Laurent Menut, André S. H. Prévôt, Pete Roberts, and Les White
Atmos. Chem. Phys., 16, 12667–12701, https://doi.org/10.5194/acp-16-12667-2016, https://doi.org/10.5194/acp-16-12667-2016, 2016
Short summary
Short summary
The EURODELTA III exercise allows a very comprehensive intercomparison and evaluation of air quality models' performance. On average, the models provide a rather good picture of the particulate matter (PM) concentrations over Europe even if the highest concentrations are underestimated. The meteorology is responsible for model discrepancies, while the lack of emissions, particularly in winter, is mentioned as the main reason for the underestimations of PM.
Daniel Neumann, Volker Matthias, Johannes Bieser, Armin Aulinger, and Markus Quante
Atmos. Chem. Phys., 16, 9905–9933, https://doi.org/10.5194/acp-16-9905-2016, https://doi.org/10.5194/acp-16-9905-2016, 2016
Short summary
Short summary
Atmospheric sea salt particles provide surface area for the condensation of gaseous substances and, thus, impact these substances' atmospheric residence time and chemical reactions. The number and size of sea salt particles govern the strength of these impacts. Therefore, these parameters should be reflected accurately in chemistry transport models. In this study, three different sea salt emission functions are compared in order to evaluate which one is best suited for the given model setup.
Andreas Weigelt, Ralf Ebinghaus, Nicola Pirrone, Johannes Bieser, Jan Bödewadt, Giulio Esposito, Franz Slemr, Peter F. J. van Velthoven, Andreas Zahn, and Helmut Ziereis
Atmos. Chem. Phys., 16, 4135–4146, https://doi.org/10.5194/acp-16-4135-2016, https://doi.org/10.5194/acp-16-4135-2016, 2016
Short summary
Short summary
We show the first mercury profile measurements over Europe since 1996. Besides gaseous elemental mercury (GEM) and total gaseous mercury (TGM), the gases CO, SO2, NOx, and O3 were measured from aboard a research aircraft over four European locations. Compared to the boundary layer, the concentration of GEM and TGM in the free troposphere was 10–30% lower. Inside the individual layers no vertical gradient was apparent. Combined with CARIBIC data, a unique profile from 0.4 to 10.5 km is provided.
Daniel Neumann, Volker Matthias, Johannes Bieser, Armin Aulinger, and Markus Quante
Atmos. Chem. Phys., 16, 2921–2942, https://doi.org/10.5194/acp-16-2921-2016, https://doi.org/10.5194/acp-16-2921-2016, 2016
Short summary
Short summary
Sea salt emissions were updated to be dependent on salinity which improved sodium predictions in the Baltic Sea region. The impact of sea salt on atmospheric nitrate and ammonium concentrations and on nitrogen deposition in the North and Baltic Sea region is assessed. Sea salt has a low effect on nitrate concentrations but does not improve them. 3 to 7 % of the nitrogen deposition into the North Sea is accounted to the presence of sea salt. In the Baltic Sea, the contribution is negligible.
V. Matthias, A. Aulinger, A. Backes, J. Bieser, B. Geyer, M. Quante, and M. Zeretzke
Atmos. Chem. Phys., 16, 759–776, https://doi.org/10.5194/acp-16-759-2016, https://doi.org/10.5194/acp-16-759-2016, 2016
Short summary
Short summary
Scenarios for future shipping emissions in the North Sea were developed. Compared to today, the contribution of shipping to the nitrogen dioxide and ozone concentrations will increase due to the expected enhanced traffic by more than 20 % and 5 %, respectively, by 2030 if no regulation for further emission reductions is implemented. PM2.5 will decrease slightly because the sulfur content in ship fuels will be reduced.
A. Aulinger, V. Matthias, M. Zeretzke, J. Bieser, M. Quante, and A. Backes
Atmos. Chem. Phys., 16, 739–758, https://doi.org/10.5194/acp-16-739-2016, https://doi.org/10.5194/acp-16-739-2016, 2016
Short summary
Short summary
A multi-model approach consisting of a bottom-up ship emissions model and a chemistry transport model was used to evaluate the impact of shipping on air quality in North Sea bordering countries. As an example, the results of the simulations indicated that the relative contribution of ships to NO2 concentration levels ashore close to the sea can reach up to 25 % in summer and 15 % in winter. Some hundred kilometers away from the sea, the contribution was about 6 % in summer and 4 % in winter.
J. Zhu, T. Wang, J. Bieser, and V. Matthias
Atmos. Chem. Phys., 15, 8767–8779, https://doi.org/10.5194/acp-15-8767-2015, https://doi.org/10.5194/acp-15-8767-2015, 2015
Short summary
Short summary
This study estimated the contributions to mercury concentration and deposition in easter China from seven categories of emission sources by CMAQ-Hg. Also, this study focuses on diagnostic and process analyses for atmospheric mercury pollution formation and on identification of the dominant atmospheric processes for mercury.
Peter Arlinghaus, Corinna Schrum, Ingrid Kröncke, and Wenyan Zhang
Earth Surf. Dynam., 12, 537–558, https://doi.org/10.5194/esurf-12-537-2024, https://doi.org/10.5194/esurf-12-537-2024, 2024
Short summary
Short summary
Benthos is recognized to strongly influence sediment stability, deposition, and erosion. This is well studied on small scales, but large-scale impact on morphological change is largely unknown. We quantify the large-scale impact of benthos by modeling the evolution of a tidal basin. Results indicate a profound impact of benthos by redistributing sediments on large scales. As confirmed by measurements, including benthos significantly improves model results compared to an abiotic scenario.
Lucas Porz, Wenyan Zhang, Nils Gerrit Christiansen, Jan Kossack, Ute Daewel, and Corinna Schrum
EGUsphere, https://doi.org/10.5194/egusphere-2024-399, https://doi.org/10.5194/egusphere-2024-399, 2024
Short summary
Short summary
Seafloor sediments store a large amount of carbon, helping to naturally regulate Earth's climate. If disturbed, some sediment particles can turn into CO2, but this effect is not well understood. Using computer simulations, we found that bottom-contacting fishing gears release about 1 million tons of CO2 per year in the North Sea, one of the most heavily fished regions globally. We show how protecting certain areas could reduce these emissions while also benefitting seafloor-living animals.
Philipp Heinrich, Stefan Hagemann, Ralf Weisse, Corinna Schrum, Ute Daewel, and Lidia Gaslikova
Nat. Hazards Earth Syst. Sci., 23, 1967–1985, https://doi.org/10.5194/nhess-23-1967-2023, https://doi.org/10.5194/nhess-23-1967-2023, 2023
Short summary
Short summary
High seawater levels co-occurring with high river discharges have the potential to cause destructive flooding. For the past decades, the number of such compound events was larger than expected by pure chance for most of the west-facing coasts in Europe. Additionally rivers with smaller catchments showed higher numbers. In most cases, such events were associated with a large-scale weather pattern characterized by westerly winds and strong rainfall.
Veli Çağlar Yumruktepe, Annette Samuelsen, and Ute Daewel
Geosci. Model Dev., 15, 3901–3921, https://doi.org/10.5194/gmd-15-3901-2022, https://doi.org/10.5194/gmd-15-3901-2022, 2022
Short summary
Short summary
We describe the coupled bio-physical model ECOSMO II(CHL), which is used for regional configurations for the North Atlantic and the Arctic hind-casting and operational purposes. The model is consistent with the large-scale climatological nutrient settings and is capable of representing regional and seasonal changes, and model primary production agrees with previous measurements. For the users of this model, this paper provides the underlying science, model evaluation and its development.
Danilo Custódio, Katrine Aspmo Pfaffhuber, T. Gerard Spain, Fidel F. Pankratov, Iana Strigunova, Koketso Molepo, Henrik Skov, Johannes Bieser, and Ralf Ebinghaus
Atmos. Chem. Phys., 22, 3827–3840, https://doi.org/10.5194/acp-22-3827-2022, https://doi.org/10.5194/acp-22-3827-2022, 2022
Short summary
Short summary
As a poison in the air that we breathe and the food that we eat, mercury is a human health concern for society as a whole. In that regard, this work deals with monitoring and modelling mercury in the environment, improving wherewithal, identifying the strength of the different components at play, and interpreting information to support the efforts that seek to safeguard public health.
Stefano Galmarini, Paul Makar, Olivia E. Clifton, Christian Hogrefe, Jesse O. Bash, Roberto Bellasio, Roberto Bianconi, Johannes Bieser, Tim Butler, Jason Ducker, Johannes Flemming, Alma Hodzic, Christopher D. Holmes, Ioannis Kioutsioukis, Richard Kranenburg, Aurelia Lupascu, Juan Luis Perez-Camanyo, Jonathan Pleim, Young-Hee Ryu, Roberto San Jose, Donna Schwede, Sam Silva, and Ralf Wolke
Atmos. Chem. Phys., 21, 15663–15697, https://doi.org/10.5194/acp-21-15663-2021, https://doi.org/10.5194/acp-21-15663-2021, 2021
Short summary
Short summary
This technical note presents the research protocols for phase 4 of the Air Quality Model Evaluation International Initiative (AQMEII4). This initiative has three goals: (i) to define the state of wet and dry deposition in regional models, (ii) to evaluate how dry deposition influences air concentration and flux predictions, and (iii) to identify the causes for prediction differences. The evaluation compares LULC-specific dry deposition and effective conductances and fluxes.
Johannes Bieser, Hélène Angot, Franz Slemr, and Lynwill Martin
Atmos. Chem. Phys., 20, 10427–10439, https://doi.org/10.5194/acp-20-10427-2020, https://doi.org/10.5194/acp-20-10427-2020, 2020
Short summary
Short summary
We use numerical models to determine the origin of air masses measured for elemental gaseous mercury (GEM) at Cape Point (CPT), South Africa. Our analysis is based on 10 years of hourly GEM measurements at CPT from 2007 to 2016. Based on GEM concentration and the origin of the air mass, we identify source and sink regions at CPT. We find, that the warm Agulhas Current to the south-east is the major Hg source and the continent the major sink.
Danilo Custodio, Ralf Ebinghaus, T. Gerard Spain, and Johannes Bieser
Atmos. Chem. Phys., 20, 7929–7939, https://doi.org/10.5194/acp-20-7929-2020, https://doi.org/10.5194/acp-20-7929-2020, 2020
Short summary
Short summary
Using a stereo algorithm, we reconstructed 99.9 % of the total atmospheric gas mercury and presented a new insight into atmospheric mercury source assessing, which can have great relevance for policy and regulations in light of the Minamata convention.
Franz Slemr, Lynwill Martin, Casper Labuschagne, Thumeka Mkololo, Hélène Angot, Olivier Magand, Aurélien Dommergue, Philippe Garat, Michel Ramonet, and Johannes Bieser
Atmos. Chem. Phys., 20, 7683–7692, https://doi.org/10.5194/acp-20-7683-2020, https://doi.org/10.5194/acp-20-7683-2020, 2020
Short summary
Short summary
Monitoring of atmospheric mercury (Hg) concentrations is an important part of the effectiveness evaluation of the Minamata Convention on Hg. Hg concentrations in 2012–2017 at Cape Point, South Africa, and at Amsterdam Island in the remote Indian Ocean are comparable, and no trend or a slightly downward trend was observed at both stations. Over the 2007–2017 period an upward trend was observed at CPT which was driven mainly by the 2007–2014 data. The trend and its change are discussed.
Laurie M. Charrieau, Karl Ljung, Frederik Schenk, Ute Daewel, Emma Kritzberg, and Helena L. Filipsson
Biogeosciences, 16, 3835–3852, https://doi.org/10.5194/bg-16-3835-2019, https://doi.org/10.5194/bg-16-3835-2019, 2019
Short summary
Short summary
We reconstructed environmental changes in the Öresund during the last 200 years, using foraminifera (microfossils), sediment, and climate data. Five zones were identified, reflecting oxygen, salinity, food content, and pollution levels for each period. The largest changes occurred ~ 1950, towards stronger currents. The foraminifera responded quickly (< 10 years) to the changes. Moreover, they did not rebound when the system returned to the previous pattern, but displayed a new equilibrium state.
Martin Otto Paul Ramacher, Matthias Karl, Johannes Bieser, Jukka-Pekka Jalkanen, and Lasse Johansson
Atmos. Chem. Phys., 19, 9153–9179, https://doi.org/10.5194/acp-19-9153-2019, https://doi.org/10.5194/acp-19-9153-2019, 2019
Short summary
Short summary
We simulated the impact of NOx shipping emissions on air quality and exposure in the Baltic Sea harbour cities Rostock (Germany), Riga (Latvia) and Gdańsk–Gdynia (Poland) for 2012. We found that local shipping affects total NO2, with contributions of 22 %, 11 % and 16 % in Rostock, Riga and Gdańsk–Gdynia. Exposure to NO2 from all emission sources was highest at home addresses (54 %–59 %). Emissions from shipping have a high impact on NO2 exposure in the port area (50 %–80 %).
Johannes Pein, Annika Eisele, Richard Hofmeister, Tina Sanders, Ute Daewel, Emil V. Stanev, Justus van Beusekom, Joanna Staneva, and Corinna Schrum
Biogeosciences Discuss., https://doi.org/10.5194/bg-2019-265, https://doi.org/10.5194/bg-2019-265, 2019
Revised manuscript not accepted
Short summary
Short summary
The Elbe estuary is subject to vigorous tidal forcing from the sea side and considerable biological inputs from the land side. Our 3D numerical coupled physical-biogeochemical integrates these forcing signals and provides highly realistic hindcasts of the associated dynamics. Model simulations show that the freshwater part of Elbe estuary is inhabited by plankton. According to simulations these organism play a key role in converting organic inputs into nitrate, the major inorganic nutrient.
Ute Daewel, Corinna Schrum, and Jed I. Macdonald
Geosci. Model Dev., 12, 1765–1789, https://doi.org/10.5194/gmd-12-1765-2019, https://doi.org/10.5194/gmd-12-1765-2019, 2019
Short summary
Short summary
Here we propose a novel modelling approach that includes an extended food web in a functional-group-type marine ecosystem model (ECOSMO E2E) by formulating new groups for macrobenthos and fish. This enables the estimation of the dynamics of the higher-trophic-level production potential and constitutes a more consistent closure term for the lower-trophic-level ecosystem. Thus, the model allows for the study of the control mechanisms for marine ecosystems at a high spatial and temporal resolution.
Changjin Zhao, Ute Daewel, and Corinna Schrum
Earth Syst. Dynam., 10, 287–317, https://doi.org/10.5194/esd-10-287-2019, https://doi.org/10.5194/esd-10-287-2019, 2019
Short summary
Short summary
Our study highlights the importance of tides in controlling the spatial and temporal distributions North Sea primary production based on numerical experiments. We identified two different response chains acting in different regions of the North Sea. (i) In the southern shallow areas, strong tidal mixing dilutes phytoplankton concentrations and increases turbidity, thus decreasing NPP. (ii) In the frontal regions, tidal mixing infuses nutrients into the surface mixed layer, thus increasing NPP.
Matthias Karl, Johannes Bieser, Beate Geyer, Volker Matthias, Jukka-Pekka Jalkanen, Lasse Johansson, and Erik Fridell
Atmos. Chem. Phys., 19, 1721–1752, https://doi.org/10.5194/acp-19-1721-2019, https://doi.org/10.5194/acp-19-1721-2019, 2019
Short summary
Short summary
Air emissions of nitrogen oxides from ship traffic in the Baltic Sea are a health concern in coastal areas of the Baltic Sea region. We find that the introduction of the nitrogen emission control area (NECA) is critical for reducing ship emissions of nitrogen oxides to levels that are low enough to sustainably dampen ozone production. The decline of the ship-related nitrogen deposition to the Baltic Sea between 2012 and 2040 varies between 46 % and 78 % in different regulation scenarios.
Gabriele Curci, Ummugulsum Alyuz, Rocio Barò, Roberto Bianconi, Johannes Bieser, Jesper H. Christensen, Augustin Colette, Aidan Farrow, Xavier Francis, Pedro Jiménez-Guerrero, Ulas Im, Peng Liu, Astrid Manders, Laura Palacios-Peña, Marje Prank, Luca Pozzoli, Ranjeet Sokhi, Efisio Solazzo, Paolo Tuccella, Alper Unal, Marta G. Vivanco, Christian Hogrefe, and Stefano Galmarini
Atmos. Chem. Phys., 19, 181–204, https://doi.org/10.5194/acp-19-181-2019, https://doi.org/10.5194/acp-19-181-2019, 2019
Short summary
Short summary
Atmospheric carbonaceous aerosols are able to absorb solar radiation and they continue to contribute some of the largest uncertainties in projected climate change. One important detail is how the chemical species are arranged inside each particle, i.e. the knowledge of their mixing state. We use an ensemble of regional model simulations to test different mixing state assumptions and found that a combination of internal and external mixing may better reproduce sunphotometer observations.
Peng Liu, Christian Hogrefe, Ulas Im, Jesper H. Christensen, Johannes Bieser, Uarporn Nopmongcol, Greg Yarwood, Rohit Mathur, Shawn Roselle, and Tanya Spero
Atmos. Chem. Phys., 18, 17157–17175, https://doi.org/10.5194/acp-18-17157-2018, https://doi.org/10.5194/acp-18-17157-2018, 2018
Short summary
Short summary
This study represents an intercomparison of four regional-scale air quality simulations in order to understand the model similarities and differences in estimating the impact of ozone imported from outside of the US on the surface ozone within the US at process level. Vertical turbulent mixing stands out as a primary contributor to the model differences in inert tracers.
Marina Astitha, Ioannis Kioutsioukis, Ghezae Araya Fisseha, Roberto Bianconi, Johannes Bieser, Jesper H. Christensen, Owen R. Cooper, Stefano Galmarini, Christian Hogrefe, Ulas Im, Bryan Johnson, Peng Liu, Uarporn Nopmongcol, Irina Petropavlovskikh, Efisio Solazzo, David W. Tarasick, and Greg Yarwood
Atmos. Chem. Phys., 18, 13925–13945, https://doi.org/10.5194/acp-18-13925-2018, https://doi.org/10.5194/acp-18-13925-2018, 2018
Short summary
Short summary
This work is unique in the detailed analyses of modeled ozone vertical profiles from sites in North America through the collaboration of four research groups from the US and EU. We assess the air quality models' performance and model inter-comparison for ozone vertical profiles and stratospheric ozone intrusions. Lastly, we designate the important role of lateral boundary conditions in the ozone vertical profiles using chemically inert tracers.
Franz Slemr, Andreas Weigelt, Ralf Ebinghaus, Johannes Bieser, Carl A. M. Brenninkmeijer, Armin Rauthe-Schöch, Markus Hermann, Bengt G. Martinsson, Peter van Velthoven, Harald Bönisch, Marco Neumaier, Andreas Zahn, and Helmut Ziereis
Atmos. Chem. Phys., 18, 12329–12343, https://doi.org/10.5194/acp-18-12329-2018, https://doi.org/10.5194/acp-18-12329-2018, 2018
Short summary
Short summary
Total and elemental mercury were measured in the upper troposphere and lower stratosphere onboard a passenger aircraft. Their concentrations in the upper troposphere were comparable implying low concentrations of oxidized mercury in this region. Large scale seasonally dependent influence of emissions from biomass burning was also observed. Their distributions in the lower stratosphere implies a long stratospheric lifetime, which precludes significant mercury oxidation by ozone.
Marta G. Vivanco, Mark R. Theobald, Héctor García-Gómez, Juan Luis Garrido, Marje Prank, Wenche Aas, Mario Adani, Ummugulsum Alyuz, Camilla Andersson, Roberto Bellasio, Bertrand Bessagnet, Roberto Bianconi, Johannes Bieser, Jørgen Brandt, Gino Briganti, Andrea Cappelletti, Gabriele Curci, Jesper H. Christensen, Augustin Colette, Florian Couvidat, Cornelis Cuvelier, Massimo D'Isidoro, Johannes Flemming, Andrea Fraser, Camilla Geels, Kaj M. Hansen, Christian Hogrefe, Ulas Im, Oriol Jorba, Nutthida Kitwiroon, Astrid Manders, Mihaela Mircea, Noelia Otero, Maria-Teresa Pay, Luca Pozzoli, Efisio Solazzo, Svetlana Tsyro, Alper Unal, Peter Wind, and Stefano Galmarini
Atmos. Chem. Phys., 18, 10199–10218, https://doi.org/10.5194/acp-18-10199-2018, https://doi.org/10.5194/acp-18-10199-2018, 2018
Short summary
Short summary
European wet and dry atmospheric deposition of N and S estimated by 14 air quality models was found to vary substantially. An ensemble of models meeting acceptability criteria was used to estimate the exceedances of the critical loads for N in habitats within the Natura 2000 network, as well as their lower and upper limits. Scenarios with 20 % emission reductions in different regions of the world showed that European emissions are responsible for most of the N and S deposition in Europe.
Ulas Im, Jesper Heile Christensen, Camilla Geels, Kaj Mantzius Hansen, Jørgen Brandt, Efisio Solazzo, Ummugulsum Alyuz, Alessandra Balzarini, Rocio Baro, Roberto Bellasio, Roberto Bianconi, Johannes Bieser, Augustin Colette, Gabriele Curci, Aidan Farrow, Johannes Flemming, Andrea Fraser, Pedro Jimenez-Guerrero, Nutthida Kitwiroon, Peng Liu, Uarporn Nopmongcol, Laura Palacios-Peña, Guido Pirovano, Luca Pozzoli, Marje Prank, Rebecca Rose, Ranjeet Sokhi, Paolo Tuccella, Alper Unal, Marta G. Vivanco, Greg Yarwood, Christian Hogrefe, and Stefano Galmarini
Atmos. Chem. Phys., 18, 8929–8952, https://doi.org/10.5194/acp-18-8929-2018, https://doi.org/10.5194/acp-18-8929-2018, 2018
Short summary
Short summary
We evaluate the impact of global and regional anthropogenic emission reductions on major air pollutant levels over Europe and North America, using a multi-model ensemble of regional chemistry and transport models. Results show that ozone levels are largely driven by long-range transport over both continents while other pollutants such as carbon monoxide or aerosols are mainly controlled by domestic sources. Use of multi-model ensembles can help to reduce the uncertainties in individual models.
Stefano Galmarini, Ioannis Kioutsioukis, Efisio Solazzo, Ummugulsum Alyuz, Alessandra Balzarini, Roberto Bellasio, Anna M. K. Benedictow, Roberto Bianconi, Johannes Bieser, Joergen Brandt, Jesper H. Christensen, Augustin Colette, Gabriele Curci, Yanko Davila, Xinyi Dong, Johannes Flemming, Xavier Francis, Andrea Fraser, Joshua Fu, Daven K. Henze, Christian Hogrefe, Ulas Im, Marta Garcia Vivanco, Pedro Jiménez-Guerrero, Jan Eiof Jonson, Nutthida Kitwiroon, Astrid Manders, Rohit Mathur, Laura Palacios-Peña, Guido Pirovano, Luca Pozzoli, Marie Prank, Martin Schultz, Rajeet S. Sokhi, Kengo Sudo, Paolo Tuccella, Toshihiko Takemura, Takashi Sekiya, and Alper Unal
Atmos. Chem. Phys., 18, 8727–8744, https://doi.org/10.5194/acp-18-8727-2018, https://doi.org/10.5194/acp-18-8727-2018, 2018
Short summary
Short summary
An ensemble of model results relating to ozone concentrations in Europe in 2010 has been produced and studied. The novelty consists in the fact that the ensemble is made of results of models working at two different scales (regional and global), therefore contributing in detail two different parts of the atmospheric spectrum. The ensemble defined as a hybrid has been studied in detail and shown to bring additional value to the assessment of air quality.
Ulas Im, Jørgen Brandt, Camilla Geels, Kaj Mantzius Hansen, Jesper Heile Christensen, Mikael Skou Andersen, Efisio Solazzo, Ioannis Kioutsioukis, Ummugulsum Alyuz, Alessandra Balzarini, Rocio Baro, Roberto Bellasio, Roberto Bianconi, Johannes Bieser, Augustin Colette, Gabriele Curci, Aidan Farrow, Johannes Flemming, Andrea Fraser, Pedro Jimenez-Guerrero, Nutthida Kitwiroon, Ciao-Kai Liang, Uarporn Nopmongcol, Guido Pirovano, Luca Pozzoli, Marje Prank, Rebecca Rose, Ranjeet Sokhi, Paolo Tuccella, Alper Unal, Marta Garcia Vivanco, Jason West, Greg Yarwood, Christian Hogrefe, and Stefano Galmarini
Atmos. Chem. Phys., 18, 5967–5989, https://doi.org/10.5194/acp-18-5967-2018, https://doi.org/10.5194/acp-18-5967-2018, 2018
Short summary
Short summary
The impacts of air pollution on human health and their costs in Europe and the United States for the year 2010 ared modeled by a multi-model ensemble. In Europe, the number of premature deaths is calculated to be 414 000, while in the US it is estimated to be 160 000. Health impacts estimated by individual models can vary up to a factor of 3. Results show that the domestic emissions have the largest impact on premature deaths, compared to foreign sources.
Joachim Kuss, Siegfried Krüger, Johann Ruickoldt, and Klaus-Peter Wlost
Atmos. Chem. Phys., 18, 4361–4376, https://doi.org/10.5194/acp-18-4361-2018, https://doi.org/10.5194/acp-18-4361-2018, 2018
Short summary
Short summary
The emission of volatile elemental mercury by the sea is an important source of atmospheric mercury. The light-induced biotic and abiotic transformation of deposited ionic mercury to elemental mercury in surface water is highly variable. On research campaigns in the Baltic Sea a new method was applied to measure elemental mercury at high resolution. The Baltic Sea's mercury emission was subsequently calculated based on the new data and the current knowledge of mercury gas exchange parameters.
Ute Daewel and Corinna Schrum
Earth Syst. Dynam., 8, 801–815, https://doi.org/10.5194/esd-8-801-2017, https://doi.org/10.5194/esd-8-801-2017, 2017
Short summary
Short summary
Processes behind observed long-term variations in marine ecosystems are difficult to be deduced from in situ observations only. By statistically analysing a 61-year model simulation for the North Sea and Baltic Sea and additional model scenarios, we identified major modes of variability in the environmental variables and associated those with changes in primary production. We found that the dominant impact on changes in ecosystem productivity was introduced by modulations of the wind fields.
Johannes Bieser, Franz Slemr, Jesse Ambrose, Carl Brenninkmeijer, Steve Brooks, Ashu Dastoor, Francesco DeSimone, Ralf Ebinghaus, Christian N. Gencarelli, Beate Geyer, Lynne E. Gratz, Ian M. Hedgecock, Daniel Jaffe, Paul Kelley, Che-Jen Lin, Lyatt Jaegle, Volker Matthias, Andrei Ryjkov, Noelle E. Selin, Shaojie Song, Oleg Travnikov, Andreas Weigelt, Winston Luke, Xinrong Ren, Andreas Zahn, Xin Yang, Yun Zhu, and Nicola Pirrone
Atmos. Chem. Phys., 17, 6925–6955, https://doi.org/10.5194/acp-17-6925-2017, https://doi.org/10.5194/acp-17-6925-2017, 2017
Short summary
Short summary
We conducted a multi model study to investigate our ability to reproduce the vertical distribution of mercury in the atmosphere. For this, we used observational data from over 40 aircraft flights in EU and US. We compared observations to the results of seven chemistry transport models and found that the models are able to reproduce vertical gradients of total and elemental Hg. Finally, we found that different chemical reactions seem responsible for the oxidation of Hg depending on altitude.
Oleg Travnikov, Hélène Angot, Paulo Artaxo, Mariantonia Bencardino, Johannes Bieser, Francesco D'Amore, Ashu Dastoor, Francesco De Simone, María del Carmen Diéguez, Aurélien Dommergue, Ralf Ebinghaus, Xin Bin Feng, Christian N. Gencarelli, Ian M. Hedgecock, Olivier Magand, Lynwill Martin, Volker Matthias, Nikolay Mashyanov, Nicola Pirrone, Ramesh Ramachandran, Katie Alana Read, Andrei Ryjkov, Noelle E. Selin, Fabrizio Sena, Shaojie Song, Francesca Sprovieri, Dennis Wip, Ingvar Wängberg, and Xin Yang
Atmos. Chem. Phys., 17, 5271–5295, https://doi.org/10.5194/acp-17-5271-2017, https://doi.org/10.5194/acp-17-5271-2017, 2017
Short summary
Short summary
The study provides a complex analysis of processes governing Hg fate in the atmosphere involving both measurement data and simulation results of chemical transport models. Evaluation of the model simulations and numerical experiments against observations allows explaining spatial and temporal variations of Hg concentration in the near-surface atmospheric layer and shows possibility of multiple pathways of Hg oxidation occurring concurrently in various parts of the atmosphere.
Efisio Solazzo, Roberto Bianconi, Christian Hogrefe, Gabriele Curci, Paolo Tuccella, Ummugulsum Alyuz, Alessandra Balzarini, Rocío Baró, Roberto Bellasio, Johannes Bieser, Jørgen Brandt, Jesper H. Christensen, Augistin Colette, Xavier Francis, Andrea Fraser, Marta Garcia Vivanco, Pedro Jiménez-Guerrero, Ulas Im, Astrid Manders, Uarporn Nopmongcol, Nutthida Kitwiroon, Guido Pirovano, Luca Pozzoli, Marje Prank, Ranjeet S. Sokhi, Alper Unal, Greg Yarwood, and Stefano Galmarini
Atmos. Chem. Phys., 17, 3001–3054, https://doi.org/10.5194/acp-17-3001-2017, https://doi.org/10.5194/acp-17-3001-2017, 2017
Short summary
Short summary
As part of the third phase of AQMEII, this study uses timescale analysis to apportion error to the responsible processes, detect causes of model error, and identify the processes and scales that require dedicated investigations. The analysis tackles model performance gauging through measurement-to-model comparison, error decomposition, and time series analysis of model biases for ozone, CO, SO2, NO, NO2, PM10, PM2.5, wind speed, and temperature over Europe and North America.
Christian N. Gencarelli, Johannes Bieser, Francesco Carbone, Francesco De Simone, Ian M. Hedgecock, Volker Matthias, Oleg Travnikov, Xin Yang, and Nicola Pirrone
Atmos. Chem. Phys., 17, 627–643, https://doi.org/10.5194/acp-17-627-2017, https://doi.org/10.5194/acp-17-627-2017, 2017
Short summary
Short summary
Atmospheric deposition is an important pathway by which Hg reaches marine ecosystems, where it can be methylated and enter the base of food chain. High resolution numerical experiments has been performed in order to investigate the contributions (sensitivity) of the Hg anthtropogenic emissions, speciation and atmospherical chemical reactions on Hg depositions over Europe. The comparison of wet deposition fluxes and concentrations measured on 28 monitioring sites were used to support the analysis.
Christos I. Efstathiou, Jana Matejovičová, Johannes Bieser, and Gerhard Lammel
Atmos. Chem. Phys., 16, 15327–15345, https://doi.org/10.5194/acp-16-15327-2016, https://doi.org/10.5194/acp-16-15327-2016, 2016
Short summary
Short summary
Gas-particle partitioning is an important process that determines the fate and long-range transport potential of persistent organic pollutants. This work is the first effort to evaluate the behaviour of parameterizations within a regional air quality system adapted for Europe. Results corroborate the significance of the chosen implementation in predicting ambient levels and transport patterns. Implications point to improvements on the side of the emission inventories and aerosol module.
Andreas Weigelt, Franz Slemr, Ralf Ebinghaus, Nicola Pirrone, Johannes Bieser, Jan Bödewadt, Giulio Esposito, and Peter F. J. van Velthoven
Atmos. Chem. Phys., 16, 13653–13668, https://doi.org/10.5194/acp-16-13653-2016, https://doi.org/10.5194/acp-16-13653-2016, 2016
Short summary
Short summary
Hg ∕ SO2, Hg ∕ CO, and NOx ∕ SO2 emission ratios (ERs) in the plume of the coal-fired power plant (CFPP), Lippendorf, near Leipzig in Germany, were determined in August 2013. GOM fraction of mercury emissions was also assessed. Measured Hg ∕ SO2 and Hg ∕ CO ERs were consistent with the ratios calculated from annual emissions in 2013 reported by the CFPP operator. The NOx ∕ SO2 ER was somewhat lower. GOM fractions of ~ 40 % of CFPP mercury emissions in current emission inventories are overestimated.
Bertrand Bessagnet, Guido Pirovano, Mihaela Mircea, Cornelius Cuvelier, Armin Aulinger, Giuseppe Calori, Giancarlo Ciarelli, Astrid Manders, Rainer Stern, Svetlana Tsyro, Marta García Vivanco, Philippe Thunis, Maria-Teresa Pay, Augustin Colette, Florian Couvidat, Frédérik Meleux, Laurence Rouïl, Anthony Ung, Sebnem Aksoyoglu, José María Baldasano, Johannes Bieser, Gino Briganti, Andrea Cappelletti, Massimo D'Isidoro, Sandro Finardi, Richard Kranenburg, Camillo Silibello, Claudio Carnevale, Wenche Aas, Jean-Charles Dupont, Hilde Fagerli, Lucia Gonzalez, Laurent Menut, André S. H. Prévôt, Pete Roberts, and Les White
Atmos. Chem. Phys., 16, 12667–12701, https://doi.org/10.5194/acp-16-12667-2016, https://doi.org/10.5194/acp-16-12667-2016, 2016
Short summary
Short summary
The EURODELTA III exercise allows a very comprehensive intercomparison and evaluation of air quality models' performance. On average, the models provide a rather good picture of the particulate matter (PM) concentrations over Europe even if the highest concentrations are underestimated. The meteorology is responsible for model discrepancies, while the lack of emissions, particularly in winter, is mentioned as the main reason for the underestimations of PM.
Daniel Neumann, Volker Matthias, Johannes Bieser, Armin Aulinger, and Markus Quante
Atmos. Chem. Phys., 16, 9905–9933, https://doi.org/10.5194/acp-16-9905-2016, https://doi.org/10.5194/acp-16-9905-2016, 2016
Short summary
Short summary
Atmospheric sea salt particles provide surface area for the condensation of gaseous substances and, thus, impact these substances' atmospheric residence time and chemical reactions. The number and size of sea salt particles govern the strength of these impacts. Therefore, these parameters should be reflected accurately in chemistry transport models. In this study, three different sea salt emission functions are compared in order to evaluate which one is best suited for the given model setup.
Andreas Weigelt, Ralf Ebinghaus, Nicola Pirrone, Johannes Bieser, Jan Bödewadt, Giulio Esposito, Franz Slemr, Peter F. J. van Velthoven, Andreas Zahn, and Helmut Ziereis
Atmos. Chem. Phys., 16, 4135–4146, https://doi.org/10.5194/acp-16-4135-2016, https://doi.org/10.5194/acp-16-4135-2016, 2016
Short summary
Short summary
We show the first mercury profile measurements over Europe since 1996. Besides gaseous elemental mercury (GEM) and total gaseous mercury (TGM), the gases CO, SO2, NOx, and O3 were measured from aboard a research aircraft over four European locations. Compared to the boundary layer, the concentration of GEM and TGM in the free troposphere was 10–30% lower. Inside the individual layers no vertical gradient was apparent. Combined with CARIBIC data, a unique profile from 0.4 to 10.5 km is provided.
Daniel Neumann, Volker Matthias, Johannes Bieser, Armin Aulinger, and Markus Quante
Atmos. Chem. Phys., 16, 2921–2942, https://doi.org/10.5194/acp-16-2921-2016, https://doi.org/10.5194/acp-16-2921-2016, 2016
Short summary
Short summary
Sea salt emissions were updated to be dependent on salinity which improved sodium predictions in the Baltic Sea region. The impact of sea salt on atmospheric nitrate and ammonium concentrations and on nitrogen deposition in the North and Baltic Sea region is assessed. Sea salt has a low effect on nitrate concentrations but does not improve them. 3 to 7 % of the nitrogen deposition into the North Sea is accounted to the presence of sea salt. In the Baltic Sea, the contribution is negligible.
V. Matthias, A. Aulinger, A. Backes, J. Bieser, B. Geyer, M. Quante, and M. Zeretzke
Atmos. Chem. Phys., 16, 759–776, https://doi.org/10.5194/acp-16-759-2016, https://doi.org/10.5194/acp-16-759-2016, 2016
Short summary
Short summary
Scenarios for future shipping emissions in the North Sea were developed. Compared to today, the contribution of shipping to the nitrogen dioxide and ozone concentrations will increase due to the expected enhanced traffic by more than 20 % and 5 %, respectively, by 2030 if no regulation for further emission reductions is implemented. PM2.5 will decrease slightly because the sulfur content in ship fuels will be reduced.
A. Aulinger, V. Matthias, M. Zeretzke, J. Bieser, M. Quante, and A. Backes
Atmos. Chem. Phys., 16, 739–758, https://doi.org/10.5194/acp-16-739-2016, https://doi.org/10.5194/acp-16-739-2016, 2016
Short summary
Short summary
A multi-model approach consisting of a bottom-up ship emissions model and a chemistry transport model was used to evaluate the impact of shipping on air quality in North Sea bordering countries. As an example, the results of the simulations indicated that the relative contribution of ships to NO2 concentration levels ashore close to the sea can reach up to 25 % in summer and 15 % in winter. Some hundred kilometers away from the sea, the contribution was about 6 % in summer and 4 % in winter.
J. Zhu, T. Wang, J. Bieser, and V. Matthias
Atmos. Chem. Phys., 15, 8767–8779, https://doi.org/10.5194/acp-15-8767-2015, https://doi.org/10.5194/acp-15-8767-2015, 2015
Short summary
Short summary
This study estimated the contributions to mercury concentration and deposition in easter China from seven categories of emission sources by CMAQ-Hg. Also, this study focuses on diagnostic and process analyses for atmospheric mercury pollution formation and on identification of the dominant atmospheric processes for mercury.
F. Ziska, B. Quack, K. Abrahamsson, S. D. Archer, E. Atlas, T. Bell, J. H. Butler, L. J. Carpenter, C. E. Jones, N. R. P. Harris, H. Hepach, K. G. Heumann, C. Hughes, J. Kuss, K. Krüger, P. Liss, R. M. Moore, A. Orlikowska, S. Raimund, C. E. Reeves, W. Reifenhäuser, A. D. Robinson, C. Schall, T. Tanhua, S. Tegtmeier, S. Turner, L. Wang, D. Wallace, J. Williams, H. Yamamoto, S. Yvon-Lewis, and Y. Yokouchi
Atmos. Chem. Phys., 13, 8915–8934, https://doi.org/10.5194/acp-13-8915-2013, https://doi.org/10.5194/acp-13-8915-2013, 2013
Related subject area
Oceanography
Implementation of additional spectral wave field exchanges in a three-dimensional wave–current coupled WAVEWATCH-III (version 6.07) and CROCO (version 1.2) configuration: assessment of their implications for macro-tidal coastal hydrodynamics
Comparison of 4-dimensional variational and ensemble optimal interpolation data assimilation systems using a Regional Ocean Modeling System (v3.4) configuration of the eddy-dominated East Australian Current system
LOCATE v1.0: numerical modelling of floating marine debris dispersion in coastal regions using Parcels v2.4.2
New insights into the South China Sea throughflow and water budget seasonal cycle: evaluation and analysis of a high-resolution configuration of the ocean model SYMPHONIE version 2.4
MQGeometry-1.0: a multi-layer quasi-geostrophic solver on non-rectangular geometries
Parameter estimation for ocean background vertical diffusivity coefficients in the Community Earth System Model (v1.2.1) and its impact on El Niño–Southern Oscillation forecasts
Great Lakes wave forecast system on high-resolution unstructured meshes
Impact of increased resolution on Arctic Ocean simulations in Ocean Model Intercomparison Project phase 2 (OMIP-2)
StraitFlux – Precise computations of Water Strait fluxes on various Modelling Grids
A high-resolution physical–biogeochemical model for marine resource applications in the northwest Atlantic (MOM6-COBALT-NWA12 v1.0)
A flexible z-layers approach for the accurate representation of free surface flows in a coastal ocean model (SHYFEM v. 7_5_71)
Implementation and assessment of a model including mixotrophs and the carbonate cycle (Eco3M_MIX-CarbOx v1.0) in a highly dynamic Mediterranean coastal environment (Bay of Marseille, France) – Part 1: Evolution of ecosystem composition under limited light and nutrient conditions
Ocean wave tracing v.1: a numerical solver of the wave ray equations for ocean waves on variable currents at arbitrary depths
Design and evaluation of an efficient high-precision ocean surface wave model with a multiscale grid system (MSG_Wav1.0)
Evaluation of the CMCC global eddying ocean model for the Ocean Model Intercomparison Project (OMIP2)
CAR36, a regional high-resolution ocean forecasting system for improving drift and beaching of Sargassum in the Caribbean Archipelago
Barents-2.5km v2.0: an operational data-assimilative coupled ocean and sea ice ensemble prediction model for the Barents Sea and Svalbard
Open-ocean tides simulated by ICON-O, version icon-2.6.6
Comparison of the Coastal and Regional Ocean Community Model (CROCO) and NCAR-LES in Non-hydrostatic Simulations
Using Probability Density Functions to Evaluate Models (PDFEM, v1.0) to compare a biogeochemical model with satellite-derived chlorophyll
Data assimilation sensitivity experiments in the East Auckland Current system using 4D-Var
Using the COAsT Python package to develop a standardised validation workflow for ocean physics models
Improving Antarctic Bottom Water precursors in NEMO for climate applications
Formulation, optimization, and sensitivity of NitrOMZv1.0, a biogeochemical model of the nitrogen cycle in oceanic oxygen minimum zones
Waves in SKRIPS: WAVEWATCH III coupling implementation and a case study of Tropical Cyclone Mekunu
Adding sea ice effects to a global operational model (NEMO v3.6) for forecasting total water level: approach and impact
DELWAVE 1.0: Deep-learning surrogate model of surface wave climate in the Adriatic Basin
Enhanced ocean wave modeling by including effect of breaking under both deep- and shallow-water conditions
An internal solitary wave forecasting model in the northern South China Sea (ISWFM-NSCS)
Intercomparisons of five ocean particle tracking software packages
Global seamless tidal simulation using a 3D unstructured-grid model (SCHISM v5.10.0)
Arctic Ocean simulations in the CMIP6 Ocean Model Intercomparison Project (OMIP)
ChemicalDrift 1.0: an open-source Lagrangian chemical-fate and transport model for organic aquatic pollutants
The Met Office operational wave forecasting system: the evolution of the regional and global models
4DVarNet-SSH: end-to-end learning of variational interpolation schemes for nadir and wide-swath satellite altimetry
Development and validation of a global 1∕32° surface-wave–tide–circulation coupled ocean model: FIO-COM32
Reproducible and relocatable regional ocean modelling: fundamentals and practices
Barotropic tides in MPAS-Ocean (E3SM V2): impact of ice shelf cavities
Using the two-way nesting technique AGRIF with MARS3D V11.2 to improve hydrodynamics and estimate environmental indicators
Multidecadal and climatological surface current simulations for the southwestern Indian Ocean at 1∕50° resolution
The tidal effects in the Finite-volumE Sea ice–Ocean Model (FESOM2.1): a comparison between parameterised tidal mixing and explicit tidal forcing
HIDRA2: deep-learning ensemble sea level and storm tide forecasting in the presence of seiches – the case of the northern Adriatic
Moana Ocean Hindcast – a > 25-year simulation for New Zealand waters using the Regional Ocean Modeling System (ROMS) v3.9 model
A nonhydrostatic oceanic regional model, ORCTM v1, for internal solitary wave simulation
How does 4DVar data assimilation affect the vertical representation of mesoscale eddies? A case study with observing system simulation experiments (OSSEs) using ROMS v3.9
An ensemble Kalman filter-based ocean data assimilation system improved by adaptive observation error inflation (AOEI)
GULF18, a high-resolution NEMO-based tidal ocean model of the Arabian/Persian Gulf
The Baltic Sea Model Intercomparison Project (BMIP) – a platform for model development, evaluation, and uncertainty assessment
An ensemble Kalman filter system with the Stony Brook Parallel Ocean Model v1.0
Wind work at the air-sea interface: a modeling study in anticipation of future space missions
Gaetano Porcile, Anne-Claire Bennis, Martial Boutet, Sophie Le Bot, Franck Dumas, and Swen Jullien
Geosci. Model Dev., 17, 2829–2853, https://doi.org/10.5194/gmd-17-2829-2024, https://doi.org/10.5194/gmd-17-2829-2024, 2024
Short summary
Short summary
Here a new method of modelling the interaction between ocean currents and waves is presented. We developed an advanced coupling of two models, one for ocean currents and one for waves. In previous couplings, some wave-related calculations were based on simplified assumptions. Our method uses more complex calculations to better represent wave–current interactions. We tested it in a macro-tidal coastal area and found that it significantly improves the model accuracy, especially during storms.
Colette Gabrielle Kerry, Moninya Roughan, Shane Keating, David Gwyther, Gary Brassington, Adil Siripatana, and Joao Marcos A. C. Souza
Geosci. Model Dev., 17, 2359–2386, https://doi.org/10.5194/gmd-17-2359-2024, https://doi.org/10.5194/gmd-17-2359-2024, 2024
Short summary
Short summary
Ocean forecasting relies on the combination of numerical models and ocean observations through data assimilation (DA). Here we assess the performance of two DA systems in a dynamic western boundary current, the East Australian Current, across a common modelling and observational framework. We show that the more advanced, time-dependent method outperforms the time-independent method for forecast horizons of 5 d. This advocates the use of advanced methods for highly variable oceanic regions.
Ivan Hernandez, Leidy M. Castro-Rosero, Manuel Espino, and Jose M. Alsina Torrent
Geosci. Model Dev., 17, 2221–2245, https://doi.org/10.5194/gmd-17-2221-2024, https://doi.org/10.5194/gmd-17-2221-2024, 2024
Short summary
Short summary
The LOCATE numerical model was developed to conduct Lagrangian simulations of the transport and dispersion of marine debris at coastal scales. High-resolution hydrodynamic data and a beaching module that used particle distance to the shore for land–water boundary detection were used on a realistic debris discharge scenario comparing hydrodynamic data at various resolutions. Coastal processes and complex geometric structures were resolved when using nested grids and distance-to-shore beaching.
Ngoc B. Trinh, Marine Herrmann, Caroline Ulses, Patrick Marsaleix, Thomas Duhaut, Thai To Duy, Claude Estournel, and R. Kipp Shearman
Geosci. Model Dev., 17, 1831–1867, https://doi.org/10.5194/gmd-17-1831-2024, https://doi.org/10.5194/gmd-17-1831-2024, 2024
Short summary
Short summary
A high-resolution model was built to study the South China Sea (SCS) water, heat, and salt budgets. Model performance is demonstrated by comparison with observations and simulations. Important discards are observed if calculating offline, instead of online, lateral inflows and outflows of water, heat, and salt. The SCS mainly receives water from the Luzon Strait and releases it through the Mindoro, Taiwan, and Karimata straits. SCS surface interocean water exchanges are driven by monsoon winds.
Louis Thiry, Long Li, Guillaume Roullet, and Etienne Mémin
Geosci. Model Dev., 17, 1749–1764, https://doi.org/10.5194/gmd-17-1749-2024, https://doi.org/10.5194/gmd-17-1749-2024, 2024
Short summary
Short summary
We present a new way of solving the quasi-geostrophic (QG) equations, a simple set of equations describing ocean dynamics. Our method is solely based on the numerical methods used to solve the equations and requires no parameter tuning. Moreover, it can handle non-rectangular geometries, opening the way to study QG equations on realistic domains. We release a PyTorch implementation to ease future machine-learning developments on top of the presented method.
Zheqi Shen, Yihao Chen, Xiaojing Li, and Xunshu Song
Geosci. Model Dev., 17, 1651–1665, https://doi.org/10.5194/gmd-17-1651-2024, https://doi.org/10.5194/gmd-17-1651-2024, 2024
Short summary
Short summary
Parameter estimation is the process that optimizes model parameters using observations, which could reduce model errors and improve forecasting. In this study, we conducted parameter estimation experiments using the CESM and the ensemble adjustment Kalman filter. The obtained initial conditions and parameters are used to perform ensemble forecast experiments for ENSO forecasting. The results revealed that parameter estimation could reduce analysis errors and improve ENSO forecast skills.
Ali Abdolali, Saeideh Banihashemi, Jose Henrique Alves, Aron Roland, Tyler J. Hesser, Mary Anderson Bryant, and Jane McKee Smith
Geosci. Model Dev., 17, 1023–1039, https://doi.org/10.5194/gmd-17-1023-2024, https://doi.org/10.5194/gmd-17-1023-2024, 2024
Short summary
Short summary
This article presents an overview of the development and implementation of Great Lake Wave Unstructured (GLWUv2.0), including the core model and workflow design and development. The validation was conducted against in situ data for the re-forecasted duration for summer and wintertime (ice season). The article describes the limitations and challenges encountered in the operational environment and the path forward for the next generation of wave forecast systems in enclosed basins like the GL.
Qiang Wang, Qi Shu, Alexandra Bozec, Eric P. Chassignet, Pier Giuseppe Fogli, Baylor Fox-Kemper, Andy McC. Hogg, Doroteaciro Iovino, Andrew E. Kiss, Nikolay Koldunov, Julien Le Sommer, Yiwen Li, Pengfei Lin, Hailong Liu, Igor Polyakov, Patrick Scholz, Dmitry Sidorenko, Shizhu Wang, and Xiaobiao Xu
Geosci. Model Dev., 17, 347–379, https://doi.org/10.5194/gmd-17-347-2024, https://doi.org/10.5194/gmd-17-347-2024, 2024
Short summary
Short summary
Increasing resolution improves model skills in simulating the Arctic Ocean, but other factors such as parameterizations and numerics are at least of the same importance for obtaining reliable simulations.
Susanna Winkelbauer, Michael Mayer, and Leopold Haimberger
EGUsphere, https://doi.org/10.5194/egusphere-2023-2883, https://doi.org/10.5194/egusphere-2023-2883, 2024
Short summary
Short summary
Oceanic transports shape the global climate, but the evaluation and validation of this key quantity based on reanalysis and model data is complicated by the distortion of the used modelling grids and the large number of different grid-types. We present two new methods that allow to calculate oceanic fluxes of volume, heat, salinity and ice through almost arbitrary sections for various models and reanalyses, independent of the used modelling grids.
Andrew C. Ross, Charles A. Stock, Alistair Adcroft, Enrique Curchitser, Robert Hallberg, Matthew J. Harrison, Katherine Hedstrom, Niki Zadeh, Michael Alexander, Wenhao Chen, Elizabeth J. Drenkard, Hubert du Pontavice, Raphael Dussin, Fabian Gomez, Jasmin G. John, Dujuan Kang, Diane Lavoie, Laure Resplandy, Alizée Roobaert, Vincent Saba, Sang-Ik Shin, Samantha Siedlecki, and James Simkins
Geosci. Model Dev., 16, 6943–6985, https://doi.org/10.5194/gmd-16-6943-2023, https://doi.org/10.5194/gmd-16-6943-2023, 2023
Short summary
Short summary
We evaluate a model for northwest Atlantic Ocean dynamics and biogeochemistry that balances high resolution with computational economy by building on the new regional features in the MOM6 ocean model and COBALT biogeochemical model. We test the model's ability to simulate impactful historical variability and find that the model simulates the mean state and variability of most features well, which suggests the model can provide information to inform living-marine-resource applications.
Luca Arpaia, Christian Ferrarin, Marco Bajo, and Georg Umgiesser
Geosci. Model Dev., 16, 6899–6919, https://doi.org/10.5194/gmd-16-6899-2023, https://doi.org/10.5194/gmd-16-6899-2023, 2023
Short summary
Short summary
We propose a discrete multilayer shallow water model based on z-layers which, thanks to the insertion and removal of surface layers, can deal with an arbitrarily large tidal oscillation independently of the vertical resolution. The algorithm is based on a two-step procedure used in numerical simulations with moving boundaries (grid movement followed by a grid topology change, that is, the insertion/removal of surface layers), which avoids the appearance of very thin surface layers.
Lucille Barré, Frédéric Diaz, Thibaut Wagener, France Van Wambeke, Camille Mazoyer, Christophe Yohia, and Christel Pinazo
Geosci. Model Dev., 16, 6701–6739, https://doi.org/10.5194/gmd-16-6701-2023, https://doi.org/10.5194/gmd-16-6701-2023, 2023
Short summary
Short summary
While several studies have shown that mixotrophs play a crucial role in the carbon cycle, the impact of environmental forcings on their dynamics remains poorly investigated. Using a biogeochemical model that considers mixotrophs, we study the impact of light and nutrient concentration on the ecosystem composition in a highly dynamic Mediterranean coastal area: the Bay of Marseille. We show that mixotrophs cope better with oligotrophic conditions compared to strict auto- and heterotrophs.
Trygve Halsne, Kai Håkon Christensen, Gaute Hope, and Øyvind Breivik
Geosci. Model Dev., 16, 6515–6530, https://doi.org/10.5194/gmd-16-6515-2023, https://doi.org/10.5194/gmd-16-6515-2023, 2023
Short summary
Short summary
Surface waves that propagate in oceanic or coastal environments get influenced by their surroundings. Changes in the ambient current or the depth profile affect the wave propagation path, and the change in wave direction is called refraction. Some analytical solutions to the governing equations exist under ideal conditions, but for realistic situations, the equations must be solved numerically. Here we present such a numerical solver under an open-source license.
Jiangyu Li, Shaoqing Zhang, Qingxiang Liu, Xiaolin Yu, and Zhiwei Zhang
Geosci. Model Dev., 16, 6393–6412, https://doi.org/10.5194/gmd-16-6393-2023, https://doi.org/10.5194/gmd-16-6393-2023, 2023
Short summary
Short summary
Ocean surface waves play an important role in the air–sea interface but are rarely activated in high-resolution Earth system simulations due to their expensive computational costs. To alleviate this situation, this paper designs a new wave modeling framework with a multiscale grid system. Evaluations of a series of numerical experiments show that it has good feasibility and applicability in the WAVEWATCH III model, WW3, and can achieve the goals of efficient and high-precision wave simulation.
Doroteaciro Iovino, Pier Giuseppe Fogli, and Simona Masina
Geosci. Model Dev., 16, 6127–6159, https://doi.org/10.5194/gmd-16-6127-2023, https://doi.org/10.5194/gmd-16-6127-2023, 2023
Short summary
Short summary
This paper describes the model performance of three global ocean–sea ice configurations, from non-eddying (1°) to eddy-rich (1/16°) resolutions. Model simulations are obtained following the Ocean Model Intercomparison Project phase 2 (OMIP2) protocol. We compare key global climate variables across the three models and against observations, emphasizing the relative advantages and disadvantages of running forced ocean–sea ice models at higher resolution.
Sylvain Cailleau, Laurent Bessières, Léonel Chiendje, Flavie Dubost, Guillaume Reffray, Jean-Michel Lellouche, Simon van Gennip, Charly Régnier, Marie Drevillon, Marc Tressol, Matthieu Clavier, Julien Temple-Boyer, and Léo Berline
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2023-183, https://doi.org/10.5194/gmd-2023-183, 2023
Revised manuscript accepted for GMD
Short summary
Short summary
In order to improve the Sargassum drift forecasting in the Caribbean area, drift models can be forced by higher resolution ocean currents. To this goal a 3-km resolution regional ocean model has been developed. its assessment is presented with a particular focus on the reproduction of fine structures representing key features of the Caribbean region dynamics and Sargassum transport. The simulated propagation of a North Brazil Current eddy and its dissipation were found to be quite realistic.
Johannes Röhrs, Yvonne Gusdal, Edel S. U. Rikardsen, Marina Durán Moro, Jostein Brændshøi, Nils Melsom Kristensen, Sindre Fritzner, Keguang Wang, Ann Kristin Sperrevik, Martina Idžanović, Thomas Lavergne, Jens Boldingh Debernard, and Kai H. Christensen
Geosci. Model Dev., 16, 5401–5426, https://doi.org/10.5194/gmd-16-5401-2023, https://doi.org/10.5194/gmd-16-5401-2023, 2023
Short summary
Short summary
A model to predict ocean currents, temperature, and sea ice is presented, covering the Barents Sea and northern Norway. To quantify forecast uncertainties, the model calculates ensemble forecasts with 24 realizations of ocean and ice conditions. Observations from satellites, buoys, and ships are ingested by the model. The model forecasts are compared with observations, and we show that the ocean model has skill in predicting sea surface temperatures.
Jin-Song von Storch, Eileen Hertwig, Veit Lüschow, Nils Brüggemann, Helmuth Haak, Peter Korn, and Vikram Singh
Geosci. Model Dev., 16, 5179–5196, https://doi.org/10.5194/gmd-16-5179-2023, https://doi.org/10.5194/gmd-16-5179-2023, 2023
Short summary
Short summary
The new ocean general circulation model ICON-O is developed for running experiments at kilometer scales and beyond. One targeted application is to simulate internal tides crucial for ocean mixing. To ensure their realism, which is difficult to assess, we evaluate the barotropic tides that generate internal tides. We show that ICON-O is able to realistically simulate the major aspects of the observed barotropic tides and discuss the aspects that impact the quality of the simulated tides.
Xiaoyu Fan, Baylor Fox-Kemper, Nobuhiro Suzuki, Qing Li, Patrick Marchesiello, Francis Auclair, Peter P. Sullivan, and Paul S. Hall
EGUsphere, https://doi.org/10.5194/egusphere-2023-1657, https://doi.org/10.5194/egusphere-2023-1657, 2023
Short summary
Short summary
Simulations of the oceanic turbulent boundary layer using the nonhydrostatic CROCO ROMS and NCAR-LES models are compared. CROCO and the NCAR-LES are similarly accurate, but CROCO’s additional features (e.g., nesting and realism) and its compressible turbulence formulation carry additional costs.
Bror F. Jönsson, Christopher L. Follett, Jacob Bien, Stephanie Dutkiewicz, Sangwon Hyun, Gemma Kulk, Gael L. Forget, Christian Müller, Marie-Fanny Racault, Christopher N. Hill, Thomas Jackson, and Shubha Sathyendranath
Geosci. Model Dev., 16, 4639–4657, https://doi.org/10.5194/gmd-16-4639-2023, https://doi.org/10.5194/gmd-16-4639-2023, 2023
Short summary
Short summary
While biogeochemical models and satellite-derived ocean color data provide unprecedented information, it is problematic to compare them. Here, we present a new approach based on comparing probability density distributions of model and satellite properties to assess model skills. We also introduce Earth mover's distances as a novel and powerful metric to quantify the misfit between models and observations. We find that how 3D chlorophyll fields are aggregated can be a significant source of error.
Rafael Santana, Helen Macdonald, Joanne O'Callaghan, Brian Powell, Sarah Wakes, and Sutara H. Suanda
Geosci. Model Dev., 16, 3675–3698, https://doi.org/10.5194/gmd-16-3675-2023, https://doi.org/10.5194/gmd-16-3675-2023, 2023
Short summary
Short summary
We show the importance of assimilating subsurface temperature and velocity data in a model of the East Auckland Current. Assimilation of velocity increased the representation of large oceanic vortexes. Assimilation of temperature is needed to correctly simulate temperatures around 100 m depth, which is the most difficult region to simulate in ocean models. Our simulations showed improved results in comparison to the US Navy global model and highlight the importance of regional models.
David Byrne, Jeff Polton, Enda O'Dea, and Joanne Williams
Geosci. Model Dev., 16, 3749–3764, https://doi.org/10.5194/gmd-16-3749-2023, https://doi.org/10.5194/gmd-16-3749-2023, 2023
Short summary
Short summary
Validation is a crucial step during the development of models for ocean simulation. The purpose of validation is to assess how accurate a model is. It is most commonly done by comparing output from a model to actual observations. In this paper, we introduce and demonstrate usage of the COAsT Python package to standardise the validation process for physical ocean models. We also discuss our five guiding principles for standardised validation.
Katherine Hutchinson, Julie Deshayes, Christian Éthé, Clément Rousset, Casimir de Lavergne, Martin Vancoppenolle, Nicolas C. Jourdain, and Pierre Mathiot
Geosci. Model Dev., 16, 3629–3650, https://doi.org/10.5194/gmd-16-3629-2023, https://doi.org/10.5194/gmd-16-3629-2023, 2023
Short summary
Short summary
Bottom Water constitutes the lower half of the ocean’s overturning system and is primarily formed in the Weddell and Ross Sea in the Antarctic due to interactions between the atmosphere, ocean, sea ice and ice shelves. Here we use a global ocean 1° resolution model with explicit representation of the three large ice shelves important for the formation of the parent waters of Bottom Water. We find doing so reduces salt biases, improves water mass realism and gives realistic ice shelf melt rates.
Daniele Bianchi, Daniel McCoy, and Simon Yang
Geosci. Model Dev., 16, 3581–3609, https://doi.org/10.5194/gmd-16-3581-2023, https://doi.org/10.5194/gmd-16-3581-2023, 2023
Short summary
Short summary
We present NitrOMZ, a new model of the oceanic nitrogen cycle that simulates chemical transformations within oxygen minimum zones (OMZs). We describe the model formulation and its implementation in a one-dimensional representation of the water column before evaluating its ability to reproduce observations in the eastern tropical South Pacific. We conclude by describing the model sensitivity to parameter choices and environmental factors and its application to nitrogen cycling in the ocean.
Rui Sun, Alison Cobb, Ana B. Villas Bôas, Sabique Langodan, Aneesh C. Subramanian, Matthew R. Mazloff, Bruce D. Cornuelle, Arthur J. Miller, Raju Pathak, and Ibrahim Hoteit
Geosci. Model Dev., 16, 3435–3458, https://doi.org/10.5194/gmd-16-3435-2023, https://doi.org/10.5194/gmd-16-3435-2023, 2023
Short summary
Short summary
In this work, we integrated the WAVEWATCH III model into the regional coupled model SKRIPS. We then performed a case study using the newly implemented model to study Tropical Cyclone Mekunu, which occurred in the Arabian Sea. We found that the coupled model better simulates the cyclone than the uncoupled model, but the impact of waves on the cyclone is not significant. However, the waves change the sea surface temperature and mixed layer, especially in the cold waves produced due to the cyclone.
Pengcheng Wang and Natacha B. Bernier
Geosci. Model Dev., 16, 3335–3354, https://doi.org/10.5194/gmd-16-3335-2023, https://doi.org/10.5194/gmd-16-3335-2023, 2023
Short summary
Short summary
Effects of sea ice are typically neglected in operational flood forecast systems. In this work, we capture these effects via the addition of a parameterized ice–ocean stress. The parameterization takes advantage of forecast fields from an advanced ice–ocean model and features a novel, consistent representation of the tidal relative ice–ocean velocity. The new parameterization leads to improved forecasts of tides and storm surges in polar regions. Associated physical processes are discussed.
Peter Mlakar, Antonio Ricchi, Sandro Carniel, Davide Bonaldo, and Matjaž Ličer
EGUsphere, https://doi.org/10.5194/egusphere-2023-718, https://doi.org/10.5194/egusphere-2023-718, 2023
Short summary
Short summary
We propose a new point-prediction DEep Learning WAVe Emulating model (DELWAVE) which successfully emulates the ocean wave model (SWAN) over synoptic to climate timescales. Compared to control climatology over all wind directions, the mismatch between DELWAVE and SWAN is generally small compared to the difference between scenario and control conditions, suggesting that the noise introduced by surrogate modeling is substantially weaker than the climate change signal.
Yue Xu and Xiping Yu
Geosci. Model Dev., 16, 2811–2831, https://doi.org/10.5194/gmd-16-2811-2023, https://doi.org/10.5194/gmd-16-2811-2023, 2023
Short summary
Short summary
An accurate description of the wind energy input into ocean waves is crucial to ocean wave modeling, and a physics-based consideration of the effect of wave breaking is absolutely necessary to obtain such an accurate description, particularly under extreme conditions. This study evaluates the performance of a recently improved formula, taking into account not only the effect of breaking but also the effect of airflow separation on the leeside of steep wave crests in a reasonably consistent way.
Yankun Gong, Xueen Chen, Jiexin Xu, Jieshuo Xie, Zhiwu Chen, Yinghui He, and Shuqun Cai
Geosci. Model Dev., 16, 2851–2871, https://doi.org/10.5194/gmd-16-2851-2023, https://doi.org/10.5194/gmd-16-2851-2023, 2023
Short summary
Short summary
Internal solitary waves (ISWs) play crucial roles in mass transport and ocean mixing in the northern South China Sea. Massive numerical investigations have been conducted in this region, but there was no systematic evaluation of a three-dimensional model about precisely simulating ISWs. Here, an ISW forecasting model is employed to evaluate the roles of resolution, tidal forcing and stratification in accurately reproducing wave properties via comparison to field and remote-sensing observations.
Jilian Xiong and Parker MacCready
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2023-45, https://doi.org/10.5194/gmd-2023-45, 2023
Revised manuscript accepted for GMD
Short summary
Short summary
A new offline particle tracking model, Tracker, was introduced to work with the Regional Ocean Modeling System (ROMS). Its performance was compared with four other particle tracking models and passive dye, which span a representative range of tracking algorithms. All tracking models perform similarly, especially for the first day. The comparison of multiple tracking codes in the same circulation model establishes confidence in all, and allows comparison of performance and ease of use.
Y. Joseph Zhang, Tomas Fernandez-Montblanc, William Pringle, Hao-Cheng Yu, Linlin Cui, and Saeed Moghimi
Geosci. Model Dev., 16, 2565–2581, https://doi.org/10.5194/gmd-16-2565-2023, https://doi.org/10.5194/gmd-16-2565-2023, 2023
Short summary
Short summary
Simulating global ocean from deep basins to coastal areas is a daunting task but is important for disaster mitigation efforts. We present a new 3D global ocean model on flexible mesh to study both tidal and nontidal processes and total water prediction. We demonstrate the potential for
seamlesssimulation, on a single mesh, from the global ocean to a few estuaries along the US West Coast. The model can serve as the backbone of a global tide surge and compound flooding forecasting framework.
Qi Shu, Qiang Wang, Chuncheng Guo, Zhenya Song, Shizhu Wang, Yan He, and Fangli Qiao
Geosci. Model Dev., 16, 2539–2563, https://doi.org/10.5194/gmd-16-2539-2023, https://doi.org/10.5194/gmd-16-2539-2023, 2023
Short summary
Short summary
Ocean models are often used for scientific studies on the Arctic Ocean. Here the Arctic Ocean simulations by state-of-the-art global ocean–sea-ice models participating in the Ocean Model Intercomparison Project (OMIP) were evaluated. The simulations on Arctic Ocean hydrography, freshwater content, stratification, sea surface height, and gateway transports were assessed and the common biases were detected. The simulations forced by different atmospheric forcing were also evaluated.
Manuel Aghito, Loris Calgaro, Knut-Frode Dagestad, Christian Ferrarin, Antonio Marcomini, Øyvind Breivik, and Lars Robert Hole
Geosci. Model Dev., 16, 2477–2494, https://doi.org/10.5194/gmd-16-2477-2023, https://doi.org/10.5194/gmd-16-2477-2023, 2023
Short summary
Short summary
The newly developed ChemicalDrift model can simulate the transport and fate of chemicals in the ocean and in coastal regions. The model combines ocean physics, including transport due to currents, turbulence due to surface winds and the sinking of particles to the sea floor, with ocean chemistry, such as the partitioning, the degradation and the evaporation of chemicals. The model will be utilized for risk assessment of ocean and sea-floor contamination from pollutants emitted from shipping.
Nieves G. Valiente, Andrew Saulter, Breogan Gomez, Christopher Bunney, Jian-Guo Li, Tamzin Palmer, and Christine Pequignet
Geosci. Model Dev., 16, 2515–2538, https://doi.org/10.5194/gmd-16-2515-2023, https://doi.org/10.5194/gmd-16-2515-2023, 2023
Short summary
Short summary
We document the Met Office operational global and regional wave models which provide wave forecasts up to 7 d ahead. Our models present coarser resolution offshore to higher resolution near the coastline. The increased resolution led to replication of the extremes but to some overestimation during modal conditions. If currents are included, wave directions and long period swells near the coast are significantly improved. New developments focus on the optimisation of the models with resolution.
Maxime Beauchamp, Quentin Febvre, Hugo Georgenthum, and Ronan Fablet
Geosci. Model Dev., 16, 2119–2147, https://doi.org/10.5194/gmd-16-2119-2023, https://doi.org/10.5194/gmd-16-2119-2023, 2023
Short summary
Short summary
4DVarNet is a learning-based method based on traditional data assimilation (DA). This new class of algorithms can be used to provide efficient reconstructions of a dynamical system based on single observations. We provide a 4DVarNet application to sea surface height reconstructions based on nadir and future Surface Water and Ocean and Topography data. It outperforms other methods, from optimal interpolation to sophisticated DA algorithms. This work is part of on-going AI Chair Oceanix projects.
Bin Xiao, Fangli Qiao, Qi Shu, Xunqiang Yin, Guansuo Wang, and Shihong Wang
Geosci. Model Dev., 16, 1755–1777, https://doi.org/10.5194/gmd-16-1755-2023, https://doi.org/10.5194/gmd-16-1755-2023, 2023
Short summary
Short summary
A new global surface-wave–tide–circulation coupled ocean model (FIO-COM32) with a resolution of 1/32° × 1/32° is developed and validated. Both the promotion of the horizontal resolution and included physical processes are shown to be important contributors to the significant improvements in FIO-COM32 simulations. It is time to merge these separated model components (surface waves, tidal currents and ocean circulation) and start a new generation of ocean model development.
Jeff Polton, James Harle, Jason Holt, Anna Katavouta, Dale Partridge, Jenny Jardine, Sarah Wakelin, Julia Rulent, Anthony Wise, Katherine Hutchinson, David Byrne, Diego Bruciaferri, Enda O'Dea, Michela De Dominicis, Pierre Mathiot, Andrew Coward, Andrew Yool, Julien Palmiéri, Gennadi Lessin, Claudia Gabriela Mayorga-Adame, Valérie Le Guennec, Alex Arnold, and Clément Rousset
Geosci. Model Dev., 16, 1481–1510, https://doi.org/10.5194/gmd-16-1481-2023, https://doi.org/10.5194/gmd-16-1481-2023, 2023
Short summary
Short summary
The aim is to increase the capacity of the modelling community to respond to societally important questions that require ocean modelling. The concept of reproducibility for regional ocean modelling is developed: advocating methods for reproducible workflows and standardised methods of assessment. Then, targeting the NEMO framework, we give practical advice and worked examples, highlighting key considerations that will the expedite development cycle and upskill the user community.
Nairita Pal, Kristin N. Barton, Mark R. Petersen, Steven R. Brus, Darren Engwirda, Brian K. Arbic, Andrew F. Roberts, Joannes J. Westerink, and Damrongsak Wirasaet
Geosci. Model Dev., 16, 1297–1314, https://doi.org/10.5194/gmd-16-1297-2023, https://doi.org/10.5194/gmd-16-1297-2023, 2023
Short summary
Short summary
Understanding tides is essential to accurately predict ocean currents. Over the next several decades coastal processes such as flooding and erosion will be severely impacted due to climate change. Tides affect currents along the coastal regions the most. In this paper we show the results of implementing tides in a global ocean model known as MPAS–Ocean. We also show how Antarctic ice shelf cavities affect global tides. Our work points towards future research with tide–ice interactions.
Sébastien Petton, Valérie Garnier, Matthieu Caillaud, Laurent Debreu, and Franck Dumas
Geosci. Model Dev., 16, 1191–1211, https://doi.org/10.5194/gmd-16-1191-2023, https://doi.org/10.5194/gmd-16-1191-2023, 2023
Short summary
Short summary
The nesting AGRIF library is implemented in the MARS3D hydrodynamic model, a semi-implicit, free-surface numerical model which uses a time scheme as an alternating-direction implicit (ADI) algorithm. Two applications at the regional and coastal scale are introduced. We compare the two-nesting approach to the classic offline one-way approach, based on an in situ dataset. This method is an efficient means to significantly improve the physical hydrodynamics and unravel ecological challenges.
Noam S. Vogt-Vincent and Helen L. Johnson
Geosci. Model Dev., 16, 1163–1178, https://doi.org/10.5194/gmd-16-1163-2023, https://doi.org/10.5194/gmd-16-1163-2023, 2023
Short summary
Short summary
Ocean currents transport things over large distances across the ocean surface. Predicting this transport is key for tackling many environmental problems, such as marine plastic pollution and coral reef resilience. However, doing this requires a good understanding ocean currents, which is currently lacking. Here, we present and validate state-of-the-art simulations for surface currents in the southwestern Indian Ocean, which will support future marine dispersal studies across this region.
Pengyang Song, Dmitry Sidorenko, Patrick Scholz, Maik Thomas, and Gerrit Lohmann
Geosci. Model Dev., 16, 383–405, https://doi.org/10.5194/gmd-16-383-2023, https://doi.org/10.5194/gmd-16-383-2023, 2023
Short summary
Short summary
Tides have essential effects on the ocean and climate. Most previous research applies parameterised tidal mixing to discuss their effects in models. By comparing the effect of a tidal mixing parameterisation and tidal forcing on the ocean state, we assess the advantages and disadvantages of the two methods. Our results show that tidal mixing in the North Pacific Ocean strongly affects the global thermohaline circulation. We also list some effects that are not considered in the parameterisation.
Marko Rus, Anja Fettich, Matej Kristan, and Matjaž Ličer
Geosci. Model Dev., 16, 271–288, https://doi.org/10.5194/gmd-16-271-2023, https://doi.org/10.5194/gmd-16-271-2023, 2023
Short summary
Short summary
We propose a new fast and reliable deep-learning architecture HIDRA2 for sea level and storm surge modeling. HIDRA2 features new feature encoders and a fusion-regression block. We test HIDRA2 on Adriatic storm surges, which depend on an interaction between tides and seiches. We demonstrate that HIDRA2 learns to effectively mimic the timing and amplitude of Adriatic seiches. This is essential for reliable HIDRA2 predictions of total storm surge sea levels.
Joao Marcos Azevedo Correia de Souza, Sutara H. Suanda, Phellipe P. Couto, Robert O. Smith, Colette Kerry, and Moninya Roughan
Geosci. Model Dev., 16, 211–231, https://doi.org/10.5194/gmd-16-211-2023, https://doi.org/10.5194/gmd-16-211-2023, 2023
Short summary
Short summary
The current paper describes the configuration and evaluation of the Moana Ocean Hindcast, a > 25-year simulation of the ocean state around New Zealand using the Regional Ocean Modeling System v3.9. This is the first open-access, long-term, continuous, realistic ocean simulation for this region and provides information for improving the understanding of the ocean processes that affect the New Zealand exclusive economic zone.
Hao Huang, Pengyang Song, Shi Qiu, Jiaqi Guo, and Xueen Chen
Geosci. Model Dev., 16, 109–133, https://doi.org/10.5194/gmd-16-109-2023, https://doi.org/10.5194/gmd-16-109-2023, 2023
Short summary
Short summary
The Oceanic Regional Circulation and Tide Model (ORCTM) is developed to reproduce internal solitary wave dynamics. The three-dimensional nonlinear momentum equations are involved with the nonhydrostatic pressure obtained via solving the Poisson equation. The validation experimental results agree with the internal wave theories and observations, demonstrating that the ORCTM can successfully describe the life cycle of nonlinear internal solitary waves under different oceanic environments.
David E. Gwyther, Shane R. Keating, Colette Kerry, and Moninya Roughan
Geosci. Model Dev., 16, 157–178, https://doi.org/10.5194/gmd-16-157-2023, https://doi.org/10.5194/gmd-16-157-2023, 2023
Short summary
Short summary
Ocean eddies are important for weather, climate, biology, navigation, and search and rescue. Since eddies change rapidly, models that incorporate or assimilate observations are required to produce accurate eddy timings and locations, yet the model accuracy is rarely assessed below the surface. We use a unique type of ocean model experiment to assess three-dimensional eddy structure in the East Australian Current and explore two pathways in which this subsurface structure is being degraded.
Shun Ohishi, Takemasa Miyoshi, and Misako Kachi
Geosci. Model Dev., 15, 9057–9073, https://doi.org/10.5194/gmd-15-9057-2022, https://doi.org/10.5194/gmd-15-9057-2022, 2022
Short summary
Short summary
An adaptive observation error inflation (AOEI) method was proposed for atmospheric data assimilation to mitigate erroneous analysis updates caused by large observation-minus-forecast differences for satellite brightness temperature around clear- and cloudy-sky boundaries. This study implemented the AOEI with an ocean data assimilation system, leading to an improvement of analysis accuracy and dynamical balance around the frontal regions with large meridional temperature differences.
Diego Bruciaferri, Marina Tonani, Isabella Ascione, Fahad Al Senafi, Enda O'Dea, Helene T. Hewitt, and Andrew Saulter
Geosci. Model Dev., 15, 8705–8730, https://doi.org/10.5194/gmd-15-8705-2022, https://doi.org/10.5194/gmd-15-8705-2022, 2022
Short summary
Short summary
More accurate predictions of the Gulf's ocean dynamics are needed. We investigate the impact on the predictive skills of a numerical shelf sea model of the Gulf after changing a few key aspects. Increasing the lateral and vertical resolution and optimising the vertical coordinate system to best represent the leading physical processes at stake significantly improve the accuracy of the simulated dynamics. Additional work may be needed to get real benefit from using a more realistic bathymetry.
Matthias Gröger, Manja Placke, H. E. Markus Meier, Florian Börgel, Sandra-Esther Brunnabend, Cyril Dutheil, Ulf Gräwe, Magnus Hieronymus, Thomas Neumann, Hagen Radtke, Semjon Schimanke, Jian Su, and Germo Väli
Geosci. Model Dev., 15, 8613–8638, https://doi.org/10.5194/gmd-15-8613-2022, https://doi.org/10.5194/gmd-15-8613-2022, 2022
Short summary
Short summary
Comparisons of oceanographic climate data from different models often suffer from different model setups, forcing fields, and output of variables. This paper provides a protocol to harmonize these elements to set up multidecadal simulations for the Baltic Sea, a marginal sea in Europe. First results are shown from six different model simulations from four different model platforms. Topical studies for upwelling, marine heat waves, and stratification are also assessed.
Shun Ohishi, Tsutomu Hihara, Hidenori Aiki, Joji Ishizaka, Yasumasa Miyazawa, Misako Kachi, and Takemasa Miyoshi
Geosci. Model Dev., 15, 8395–8410, https://doi.org/10.5194/gmd-15-8395-2022, https://doi.org/10.5194/gmd-15-8395-2022, 2022
Short summary
Short summary
We develop an ensemble-Kalman-filter-based regional ocean data assimilation system in which satellite and in situ observations are assimilated at a daily frequency. We find the best setting for dynamical balance and accuracy based on sensitivity experiments focused on how to inflate the ensemble spread and how to apply the analysis update to the model evolution. This study has a broader impact on more general data assimilation systems in which the initial shocks are a significant issue.
Hector S. Torres, Patrice Klein, Jinbo Wang, Alexander Wineteer, Bo Qiu, Andrew F. Thompson, Lionel Renault, Ernesto Rodriguez, Dimitris Menemenlis, Andrea Molod, Christopher N. Hill, Ehud Strobach, Hong Zhang, Mar Flexas, and Dragana Perkovic-Martin
Geosci. Model Dev., 15, 8041–8058, https://doi.org/10.5194/gmd-15-8041-2022, https://doi.org/10.5194/gmd-15-8041-2022, 2022
Short summary
Short summary
Wind work at the air-sea interface is the scalar product of winds and currents and is the transfer of kinetic energy between the ocean and the atmosphere. Using a new global coupled ocean-atmosphere simulation performed at kilometer resolution, we show that all scales of winds and currents impact the ocean dynamics at spatial and temporal scales. The consequential interplay of surface winds and currents in the numerical simulation motivates the need for a winds and currents satellite mission.
Cited articles
Allison, J. D. and Allision, T. L.: PARTITION COEFFICIENTS FOR METALS IN SURFACE
WATER, SOIL, AND WASTE, EPA/600/R-05/074 U.S. Environmental Protection Agency, Washington,
DC, https://cfpub.epa.gov/si/si_public_record_report.cfm?Lab=NERL&dirEntryId=135783 (last access:
7 April 2023), 2005.
AMAP/EMEP: Global Mercury Assessment 2013: Sources, Emissions,
Releases and Environmental Transport, UNEP Chemicals Branch, Geneva, 2013.
AMAP/EMEP: Global Mercury Assessment 2018, UN Environment Programme
Chemicals and Health Branch Geneva Switzerland, ISBN 978-92-807-3744-8, 2019a.
AMAP/EMEP: Technical Background Report for the Global Mercury
Assessment 2018, Arctic Monitoring and Assessment Programme, Oslo, Norway/UN
Environment Programme, Chemicals and Health Branch, Geneva, Switzerland,
viii + 426 pp. including E-Annexes, 2019b.
Amos, H. M., Jacob, D. J., Holmes, C. D., Fisher, J. A., Wang, Q., Yantosca, R. M., Corbitt, E. S., Galarneau, E., Rutter, A. P., Gustin, M. S., Steffen, A., Schauer, J. J., Graydon, J. A., Louis, V. L. St., Talbot, R. W., Edgerton, E. S., Zhang, Y., and Sunderland, E. M.: Gas-particle partitioning of atmospheric Hg(II) and its effect on global mercury deposition, Atmos. Chem. Phys., 12, 591–603, https://doi.org/10.5194/acp-12-591-2012, 2012.
Amos, H. M., Jacob, D. J., Streets, D. G., and Sunderland, E. M.: Legacy impacts of
all-time anthropogenic emissions in the global mercury cycle, Global
Biogeochem. Cycles, 27, 410–421, 2013.
Amptmeijer, D. J., Mikheeva, E., Daewel, U., Bieser, J., and Schrum, C.: The
impact of ecosystem interactions on marine mercury and methylmercury
concentrations in the North-and Baltic Seas, in preparation, 2023.
Backhaus, J. O.: A semi-implicit scheme for the shallow water equations
for application to shelf sea modelling, Cont. Shelf Res., 2, 243–254,
https://doi.org/10.1016/0278-4343(82)90020-6, 1983.
Andersson, M. E., Sommar, J., Gårdfeldt, K., and Lindqvist, O.:
Enhanced concentrations of dissolved gaseous mercury in the surface waters
of the Arctic Ocean, Mar. Chem., 110, 190–194, 2008.
Bash, J. O.: Description and initial simulation of a dynamic bidirectional air-surface exchange model for
mercury in Community Multicale Air Quality (CMAQ) model, J. Geophys. Res.-Atmos., 115, 2156–2202,
https://doi.org/10.1029/2009JD012834, 2010.
Batrakova, N., Travnikov, O., and Rozovskaya, O.: Chemical and physical transformations of mercury in the ocean: a review, Ocean Sci., 10, 1047–1063, https://doi.org/10.5194/os-10-1047-2014, 2014.
Bergan, T., Gallardo, L., and Rodhe, H.: Mercury in the global troposphere: a three dimensional model study,
Atmos. Environ., 33, 1575–1585, https://doi.org/10.1016/S1352-2310(98)00370-7, 1999.
Berrisford, P., Kallberg, P., Kobayashi, S., Dee, D., Uppala, S., Simmons, A. J., Poli, P., and Sato, H.:
Atmospheric conservation properties in ERA-Interim, Q. J. Roy.
Meteor. Soc., 137, 1381–1399, https://doi.org/10.1002/qj.864, 2011.
Bieser, J.: MERCY v2.0 (2.0), Zenodo [code], https://doi.org/10.5281/zenodo.7101217, 2022.
Bieser, J. and Schrum, C.: Impact of marine mercury cycling on coastal
atmospheric mercury concentrations in the North and Baltic Sea region,
Elementa, 000111, https://doi.org/10.12952/journal.elementa.000111, 2016.
Bieser, J., Aulinger, A., Matthias, V., Quante, M., and Builtjes, P.: SMOKE for Europe – adaptation, modification and evaluation of a comprehensive emission model for Europe, Geosci. Model Dev., 4, 47–68, https://doi.org/10.5194/gmd-4-47-2011, 2011.
Bieser, J., Matthias, V., Travnikov, O., Hedgecock, I. M., Gencarelli, C., De
Simone, F., Weigelt, A., and Zhu, J.: Diagnostic evaluation of bromine reactions
on mercury chemistry. In Steyn, D., Chaumerliac, N., Air pollution modeling
and its application XXIV, Springer Proceedings in Complexity, 519–523,
2016.
Bieser, J., Slemr, F., Ambrose, J., Brenninkmeijer, C., Brooks, S., Dastoor, A., DeSimone, F., Ebinghaus, R., Gencarelli, C. N., Geyer, B., Gratz, L. E., Hedgecock, I. M., Jaffe, D., Kelley, P., Lin, C.-J., Jaegle, L., Matthias, V., Ryjkov, A., Selin, N. E., Song, S., Travnikov, O., Weigelt, A., Luke, W., Ren, X., Zahn, A., Yang, X., Zhu, Y., and Pirrone, N.: Multi-model study of mercury dispersion in the atmosphere: vertical and interhemispheric distribution of mercury species, Atmos. Chem. Phys., 17, 6925–6955, https://doi.org/10.5194/acp-17-6925-2017, 2017.
Bowman, K. L., Lamborg, C. H., and Agather, A. M.: A global perspective on
mercury cycling in the ocean, Sci. Total Environ., 710, 136–166, 2020.
Bullock, O. R. and Brehme, K. A.: Atmospheric mercury simulaˇtions using the CMAQ model: Formulation
description and analysis of wet deposition results, Atmos. Environ., 36, 2135–2146, 2002.
Bullock, O. R., Atkinson, D., Braverman, T., Civerolo, K., Dastoor, A., Davignon, D., Ku, J.-Y., Lohman,
K., Myers, T. C., Park, R. J., Seigneur, C., Selin, N. E., Sistla, G., and Vjayaraghavan, K.: The North
American Mercury Model Inter comparison Study (NAMMIS): Study description and model-to-model
comparisons, J. Geophys. Res., 113, D17310, https://doi.org/10.1029/2008JD009803, 2008.
Byun, D. W. and Schere, K. L.: Review of the governing equations, computational algorithms, and other
components of the Models Community Multiscale Air Quality (CMAQ) modeling system, Appl. Mech.
Rev., 59, 147–164, 2006.
Capo, E., Bravo, A. G., Soerensen, A. L., Bertilsson, S., Pinhassi, J., Feng, C., Andersson,
A. F., Buck, M., and Björn, E.: Deltaproteobacteriaand Spirochaetes-Like
Bacteria AreAbundant Putative MercuryMethylators in Oxygen-DeficientWater
and Marine Particlesin the Baltic Sea, Front. Microbiol., 11, 574080, https://doi.org/10.3389/fmicb.2020.574080, 2020.
Capo, E., Feng, C., Bravo, A. G., Bertilsson, S., Soerensen, A. L., Pinhassi, J.,
Buck, M., Karlsson, C., Hawkes, J., and Björn, E.: Expression Levels of hgcAB Genes and
Mercury Availability Jointly Explain Methylmercury Formation in Stratified Brackish Waters, Environ.
Sci. Technol., 56, 13119–13130, https://doi.org/10.1021/acs.est.2c03784, 2022.
Carnevale, C., Finzi, G., Pederzoli, A., Pisoni, E., Thunis, P., Turrini, E., and Volta, M.: Applying the delta
tool to support the Air Quality Directive: evaluation of the TCAM chemical
transport model, Air Qual. Atmos. Health, 7, 335–346,
https://doi.org/10.1007/s11869-014-0240-4, 2014.
Chen, C. Y., Driscoll, C. T., Lambert, K. F., Mason, R. P., Rardin, L. R., Serrell,
N., and Sunderland, E. M.: Marine mercury fate: From sources to seafood consumers,
Environ. Res., 119, 1–2, https://doi.org/10.1016/j.envres.2012.10.001, 2012.
Christensen, J. H., Brandt, J., Frohn, L. M., and Skov, H.: Modelling of Mercury in the Arctic with the Danish Eulerian Hemispheric Model, Atmos. Chem. Phys., 4, 2251–2257, https://doi.org/10.5194/acp-4-2251-2004, 2004.
Clarkson, T. W.: Mercury – An Element of Mystery, N. Engl. J. Med., 323, 1137–1139, https://doi.org/10.1056/NEJM199010183231610, 1990.
Cohen, M., Draxler, R. R., Artz, R. S., Blanchard, P., Gustin, M. S., Han,
Y.-J., Holden, T. M., Jaffe, D. A., Kelley, P., Lei, H., Loughner, C. P., Luke,
W. T., Lyman, S. N., Niemi, D., Pacyna, J. M., Pilote, M., Poissant, L., Ratte,
D., Ren, X., Steenhuisen, F., Steffen, A., Tordon, R., and Wilson, S. J.:
Modeling the global atmospheric transport and deposition of mercury to the
Great Lakes, Elementa, 4, 000118, https://doi.org/10.12952/journal.elementa.000118, 2016.
Cossa, D., Heimbürger, L.-E., Pérez, F. F., García-Ibáñez, M. I., Sonke, J. E., Planquette, H., Lherminier, P., Boutorh, J., Cheize, M., Menzel Barraqueta, J. L., Shelley, R., and Sarthou, G.: Mercury distribution and transport in the North Atlantic Ocean along the GEOTRACES-GA01 transect, Biogeosciences, 15, 2309–2323, https://doi.org/10.5194/bg-15-2309-2018, 2018.
Cressie, N.: The origins of kriging, Math. Geol., 22, 239–252,
https://doi.org/10.1007/BF00889887, 1990.
Cushing, D. H.: The estimation of carbon in phytoplankton. In: Rappt.
Proces-Verbaux Reunions, Conseil Perm. Intern. Exploration Mer, 144,
32–33, 1958.
Daewel, U.: hamsom_ecosmo_2e2 v1.0 (v1.0), Zenodo [code], https://doi.org/10.5281/zenodo.7587005, 2023.
Daewel, U. and Schrum, C.: Simulating long-term dynamics of the coupled North Sea and Baltic Sea
ecosystem with ECOSMO II: Model description and validation, J. Mar. Syst., 119–120, 30–49,
https://doi.org/10.1016/j.jmarsys.2013.03.008, 2013.
Daewel, U., Schrum, C., and Macdonald, J. I.: Towards end-to-end (E2E) modelling in a consistent NPZD-F modelling framework (ECOSMO E2E_v1.0): application to the North Sea and Baltic Sea, Geosci. Model Dev., 12, 1765–1789, https://doi.org/10.5194/gmd-12-1765-2019, 2019.
Dastoor, A., Ryzhkov, A., Durnford, D., Lehnherr, I., Steffen, A., and
Morrison, H.: Atmospheric mercury in the Canadian Arctic.Part II: Insight
from modeling, Sci. Total Environ., 509–510, 16–27,
https://doi.org/10.1016/j.scitotenv.2014.10.112, 2015.
Dee, D. P., Uppala, S. M., Simmons, A. J., Berrisford, P., Poli, P., Kobayashi, S., Andrae,
U., Balmaseda, M. A., Balsamo, G., Bauer, P., Bechtold, P.,
Beljaars, A. C. M., van de Berg, L., Bidlot, J., Bormann, N., Delsol, C., Dragani, R.,
Fuentes, M., Geer, A. J., Haimberger, L., Healy, S. B., Hersbach, H., Hólm, E. V., Isaksen,
L., Kållberg, P., Köhler, M., Matricardi, M., McNally, A. P.,
Monge-Sanz, B. M., Morcrette, J.-J., Park, B.-K., Peubey, C., de Rosnay, P.,
Tavolato, C., Thépaut, J.-N., and Vitart, F.: The ERA-Interim reanalysis: configuration and performance of the data assimilation
system, Q. J. Roy. Meteor. Soc., 137, 553–597, 2011.
Derwent, D., Fraser, A., Abbott, J., Willis, P., and Murrells, T.: Evaluating the
performance of air quality models, Department for Environment
and Rural Affairs, issue 3, 2010.
De Simone, F., Gencarelli, C. N., Hedgecock, I. M., and Pirrone, N.: Global
atmospheric cycle of mercury: a model study on the impact of oxidation
mechanisms, Environ. Sci. Pollut. R., 21, 4110–4123, 2014.
Driscoll, C. T., Mason, R. P., Chan, H. M., Jacob, D. J., and Pirrone, N.:
Environ. Sci. Technol., 47, 4967–4983, https://doi.org/10.1021/es305071v, 2013.
Duran, R., Ranchou-Peyruse, M., Menuet, V., Monperrus, M., Bareille, G., Goni, M. S., Salvado, J. C.,
Amouroux, D., Guyoneaud, R., Donard, O. F. X., and Caumette, P.: Mercury methylation by a microbial
community from sediments of the Adour Estuary (Bay of Biscay, France), Environ. Pollut., 156,
951–958, https://doi.org/10.1016/j.envpol.2008.05.007, 2008.
Durnford, D., Dastoor, A., Ryzhkov, A., Poissant, L., Pilote, M., and Figueras-Nieto, D.: How relevant is the deposition of mercury onto snowpacks? – Part 2: A modeling study, Atmos. Chem. Phys., 12, 9251–9274, https://doi.org/10.5194/acp-12-9251-2012, 2012.
Fischer, H. and Matthäus, W.: The importance of the Drogden Sill in the
Sound for major Baltic inflows, J. Mar. Sys., 9, 137–157, 1996.
Fitzgerald, W. F. and Kim, J. P.: Sea-Air Partitioning of Mercury in the Equatorial Pacific Ocean,
Science, 231, 1131–1133, https://doi.org/10.1126/science.231.4742.1131, 1986.
Fitzgerald, W. F., Gill, G. A., and Kim, J. P.: An Equatorial Pacific Ocean Source of Atmospheric Mercury,
Science, 224, 597–599, https://doi.org/10.1126/science.224.4649.597, 1984.
GEBCO Bathymetric Compilation Group: The GEBCO_2022 Grid – a continuous terrain model of the global oceans and land, NERC EDS British Oceanographic Data Centre NOC [data set], https://doi.org/10.5285/e0f0bb80-ab44-2739-e053-6c86abc0289c, 2022.
Gencarelli, C. N., Bieser, J., Carbone, F., De Simone, F., Hedgecock, I. M., Matthias, V., Travnikov, O., Yang, X., and Pirrone, N.: Sensitivity model study of regional mercury dispersion in the atmosphere, Atmos. Chem. Phys., 17, 627–643, https://doi.org/10.5194/acp-17-627-2017, 2017.
Green, N. W., Heldal, H. E., Måge, A., Aas, W., Gäfvert, T., Schrum, C., Boitsov, S., Breivik, K., Iosjpe,
M., Yakushev, E., Skogen, M., Høgåsen, T., Eckhardt, S., Christiansen, A. B., Daae, K. L., Durand, D., and
Debloskaya, E.:
Tilførselsprogrammet 2010, Overvåking av tilførsler og
miljøtilstand i Nordsjøen, NIVA rapport 6187-2011, Klima-og
forurensningsdirektoratet (Klif), Rapport TA 2810/2011, IPCS 1992, ISBN
978-82-577-577-5992-3, 2011.
Heimbürger, L.-E., Sonke, J. E., Cossa, D., Point, D., Lagne, C.,
Laffont, L., Galfond, B. T., Nicolaus, M., Rabe, B., and Rutgers van der Loeff,
M.: Shallow methylmercury production in the marginal sea ice zone of the
central Arctic Ocean, Sci. Rep., 5, 10318, https://doi.org/10.1038/srep10318, 2015.
HELCOM: Heavy Metal Pollution to the Baltic Sea in 2004. Baltic Sea
Environment Proceedings, 108, 33 pp., 2007.
HELCOM: Fifth Baltic Sea Pollution Load Compilation. Baltic Sea
Environment Proceedings, 128, 56 pp., 2011.
Hersbach, H., Bell, B., Berrisford, P., Hirahara, S., Horányi, A., Muñoz-Sabater, J., Nicolas, J., Peubey, C., Radu,
R., Schepers, D., Simmons, A., Soci, C., Abdalla, S., Abellan, X., Balsamo, G., Bechtold, P.,
Biavati, G., Bidlot, J., Bonavita, M., De Chiara, G., Dahlgren, P., Dee, D., Diamantakis, M., Dragani, R., Flemming,
J., Forbes, R., Fuentes, M., Geer, A., Haimberger, L., Healy, S., Hogan, R. J., Hólm, E.,
Janisková, M., Keeley, S., Laloyaux, P., Lopez, P., Radnoti, G., de Rosnay, P., Rozum, I., Vamborg, F.,
Villaume, S., and Thépaut, J.-N.: The ERA5 Global Reanalysis, Q. J. Roy. Meteor.
Soc., 52, 238–249, https://doi.org/10.1002/gj.3003, 2020 (data available at: https://apps.ecmwf.int/datasets/data/interim-full-daily, last access: 7 April 2023).
Hohlfeld, M
and Wolff, J.-O.: Distributed Information Services in Marine Science: MareNet – The
Network of Marine Research Institutions and Documents, Oceanography, 15, 109–111, https://doi.org/10.5670/oceanog.2002.41, 2015 (data available at: https://www.bsh.de/DE/DATEN/Meeresumweltmessnetz/meeresumweltmessnetz_node.html, last access:
7 April 2023).
Holmes, C. D., Jacob, D. J., Corbitt, E. S., Mao, J., Yang, X., Talbot, R., and Slemr, F.: Global atmospheric model for mercury including oxidation by bromine atoms, Atmos. Chem. Phys., 10, 12037–12057, https://doi.org/10.5194/acp-10-12037-2010, 2010.
Horowitz, L. W., Walters, S., Mauzerall, D. L., Emmons, L. K., Rasch, P. J., Granier, C., Tie, X., Lamarque, J.-F., Schultz, M. G., Tyndall, G. S.,
Orlando, J. J., and Brasseur, G. P.: A global simulation of tropospheric ozone and
related tracers: Description and evaluation of MOZART, version 2, J.
Geophys. Res., 108, 4784–4784, 2001.
Horowitz, H. M., Jacob, D. J., Zhang, Y., Dibble, T. S., Slemr, F., Amos, H. M., Schmidt, J. A., Corbitt, E. S., Marais, E. A., and Sunderland, E. M.: A new mechanism for atmospheric mercury redox chemistry: implications for the global mercury budget, Atmos. Chem. Phys., 17, 6353–6371, https://doi.org/10.5194/acp-17-6353-2017, 2017.
Jacovides, C. P., Tymvios, F., Papaioannou, G., Asimakopoulos, D. N.,
and Theofilou, C. M.: Ratio of PAR to broadband solar radiation measured
in Cyprus, Agric. Forest Meteorol., 121, 135–140, 2004.
Jiang, P., Li, Y., Yang, G., Lagos, L., Yin, Y., Gu, B., Jiang, G., and Cai, Y.: Evaluating the role of readsorption
of dissolved Hg2+ during cinnabar dissolution using isotope tracer technique, J.
Hazard. Mater., 317, 466–475, https://doi.org/10.1016/j.jhazmat.2016.05.084, 2016.
Jiskra, M., Sonke, J. E., Obrist, D., Bieser, J., Ebinghaus, R., Myhre, C. L.,
Pfaffhuber, K. A., Wängberg, I., Kyllönen, K., Worthy, D., Martin,
L. G., Labuschagne, C., Mkololo, T., Ramonet, M., Magand, O., and Dommergue,
A.: A vegetation control on seasonal variations in global atmospheric
mercury concentrations, Nat. Geosci., 11, 224–250, 2018.
Jung, G., Hedgecock, I. M., and Pirrone, N.: ECHMERIT V1.0 – a new global fully coupled mercury-chemistry and transport model, Geosci. Model Dev., 2, 175–195, https://doi.org/10.5194/gmd-2-175-2009, 2009.
Kawai, T., Sakurai, T., and Suzuki, N.: Application of a new dynamic 3-D model to investigate human
impacts on the fate of mercury in the global ocean, Environ. Model. Softw., 124, 104599,
https://doi.org/10.1016/j.envsoft.2019.104599, 2020.
Kuss, J.: Water–air gas exchange of elemental mercury: An experimentally
determined mercury diffusion coefficient for Hg0 water–air flux
calculations, Limnol. Oceanogr., 59, 1461–1467,
https://doi.org/10.4319/lo.2014.59.5.1461, 2014.
Kuss, J., Holzmann, J., and Ludwig, R.: An Elemental Mercury Diffusion Coefficient for Natural Waters
Determined by Molecular Dynamics Simulation, Environ. Sci. Technol., 43, 3183–3186,
https://doi.org/10.1021/es8034889, 2009.
Kuss, J., Wasmund, N., Nausch, G., and Labrenz, M.: Mercury emission by the
Baltic Sea: A consequence of cyanobacterial activity, photochemistry, and
low-light mercury transformation, Environ. Sci. Technol., 49,
11449–11457, https://doi.org/10.1021/acs.est.5b02204, 2015.
Kuss, J., Cordes, F., Mohrholz, V., Nausch, G., Naumann, M., Krüger, S.,
and Schulz-Bull, D. E.: The impact of the major Baltic inflow of December
2014 on the mercury species distribution in the Baltic Sea, Environ. Sci.
Technol., 51, 11692–11700, https://doi.org/10.1021/acs.est.7b03011, 2017.
Kuss, J., Krüger, S., Ruickoldt, J., and Wlost, K.-P.: High-resolution measurements of elemental mercury in surface water for an improved quantitative understanding of the Baltic Sea as a source of atmospheric mercury, Atmos. Chem. Phys., 18, 4361–4376, https://doi.org/10.5194/acp-18-4361-2018, 2018.
Kos, G., Ryzhkov, A., Dastoor, A., Narayan, J., Steffen, A., Ariya, P. A., and Zhang, L.: Evaluation of discrepancy between measured and modelled oxidized mercury species, Atmos. Chem. Phys., 13, 4839–4863, https://doi.org/10.5194/acp-13-4839-2013, 2013.
Lee, D. S., Nemitz, E., Fowler, D., and Kingdon, R. D.: Modeling atmospheric transport and deposition
across Europe and the UK, Atmos. Environ., 35, 5455–5466, https://doi.org/10.1016/S1352-2310(01)00284-9, 2001.
Leermakers, M., Galetti, S., Galan, Da Sandra, Brion, N., and Baeyens, W.: Mercury in the Southern North Sea and Scheldt estuary, Marine
Chem., 75, 229–248,
2001.
Lehmann, A. and Post, P.: Variability of atmospheric circulation patterns
associated with large volume changes of the Baltic Sea, Adv. Sci.
Res., 12, 219–225, 2015.
Lehnherr, I.: Methylmercury biogeochemistry: A review with special reference
to Arctic aquatic ecosystems, Environ. Rev., 22, 229–243, 2014.
Lehnherr, I., St. Louis, V. L., Hintelmann, H., and Kirk, J. L.: Methylation of inorganic mercury in polar
marine waters, Nat. Geosci., 4, 298–302, https://doi.org/10.1038/ngeo1134, 2011.
Lyon, B. F., Ambrose, R., Rice, G., and Maxwell, C. J.: Calculation of soil-water and benthic sediment partition coefficients for mercury, Chemosphere, 35, 791–808, https://doi.org/10.1016/s0045-6535(97)00200-2, 1997.
MARENET: Messnetz MARNET,
https://www.bsh.de/DE/DATEN/Klima-und-Meer/Meeresumweltmessnetz/messnetz-marnet_node.html (last access: 7 April 2023), 2020.
Mason, R. P., Reinfelder, J. R., and Morel, F. M. M.: Bioaccumulation of mercury and
methylmercury, Water Air Soil Pollut., 80, 915–921, 1995.
Mason, R. P., Reinfelder, J. R., and Morel, F. M.: Uptake, toxicity, and
trophic transfer of mercury in a coastal diatom, Environ. Sci. Technol.,
30, 1835–1845, 1996.
Mason, R. P., Choi, A. L., Fitzgerald, W. F., Hammerschmidt, C. R., Lamborg,
C. H., Soerensen, A. L., and Sunderland, E. M.: Mercury biogeochemical cycling
in the ocean and policy implications, Environ. Res., 119, 101–117, 2012.
McClelland, J. W., Holmes, R. M., Peterson, B. J., Raymond, P. A., Striegl, R.,
Zhulidov, A. V., Zimov, S., Zimov, N., Tank, S. E., and Spencer, R. G.:
Particulate organic carbon and nitrogen export from major Arctic rivers,
Global Biogeochem. Cycles, 30, 629e643, https://doi.org/10.1007/s12237-011-9386-6, 2016.
McCree, K. J.: Test of current definitions of photosynthetically active radiation against leaf
photosynthesis data, Agric. Meteorol., 10, 443–453, https://doi.org/10.1016/0002-1571(72)90045-3, 1972.
Menden-Deuer, S. and Lessard, E. J.: Carbon to volume relationships for
dinoflagellates, diatoms, and other protist plankton, Limnol. Oceanogr.,
45, 569–579, 2000.
Mohrholz, V., Naumann, M., Nausch, G., Krüger, S., and Gräwe, U.:
Fresh oxygen for the Baltic Sea – An exceptional saline inflow after a
decade of stagnation, J. Mar. Sys., 148, 152–166, 2015.
Monperrus, M., Tessier, E., Amouroux, D., Leynaert, A., Huonnic, P., and Donard, O. F. X.: Mercury
methylation, demethylation and reduction rates in coastal and marine surface waters of the Mediterranean
Sea, Marine Chem., 107, 49–63, https://doi.org/10.1016/j.marchem.2007.01.018, 2007.
Neumann, T.: Towards a 3D-ecosystem model of the Baltic Sea, J.
Marine Sys., 25, 405–419, 2000.
Nfon, E., Cousins, I. T., Järvinen, O., Mukherjee, A. B.,
Verta, M., and Broman, D.: Trophodynamics of mercury and other trace elements in a pelagic food chain from
the Baltic Sea, Sci. Total Environ., 407, 6267–6274,
https://doi.org/10.1016/j.scitotenv.2009.08.032, 2009.
Nightingale, P. D., Malin, G., Law, C. S., Watson, A. J., Liss, P. S., Liddicoat, M. I., Boutin,
J., and Upstill-Goddard, R. C.: In-situ
evaluation of air-sea gas exchange parameterizations using novel
conservative and volatile tracers, Global Biogeochem. Cy., 14, 373–387, 2000.
Niki, H., Maker, P. D., Savage, C. M., and Breitenbach L. P.: A long-path
Fourier transform infrared study of the kinetics and mechanism for the
hydroxyl radical-initiated oxidation of dimethylmercury, J. Phys. Chem., 87, 3722–3724, 1983.
Obrist, D., Kirk, J. L., Zhang, L., Sunderland, E. M., Jiskra, M., and Selin,
N. E.: A review of global environmental mercury processes in response to
human and natural perturbations: Changes of emissions, climate, and land
use, Ambio, 47, 116–140, https://doi.org/10.1007/s13280-017-1004-9, 2018.
Olenina, I., Hajdu, S., Edler, L., Andersson, A.,
Wasmund, N., Busch, S., Göbel, J., Gromisz, S.,
Huseby, S., Huttunen, M., Jaanus, A., Kokkonen, P., Ledaine, I., and Niemkiewicz,
E.: Biovolumes and size-classes of phytoplankton in the Baltic Sea, Helsinki,
HELCOM Balt. Sea Environ. Proc. No. 106, 144 pp., 2003.
Olsen, T. A., Muller, K. A., Painter, S. L., and Brooks, S. C.: Kinetics of Methylmercury Production
Revisited, Environ. Sci. Technol., 52, 2063–2070,
https://doi.org/10.1021/acs.est.7b05152, 2018.
OSPAR Commission, McHugh, B. B., Farmer, R., Fryer, E., Green, R., Larsen, N., Webster, M. M.,
Lepom, L., McGovern, P., Maes, E., Verbruggen, T., and ICES Marine Chemistry Working Group, E.:
Mercury assessment in the marine environment Assessment criteria comparison (EAC/EQS) for mercury,
http://hdl.handle.net/10793/1204, 2016.
Pakhomova, S., Yakushev, E., Protsenko, E., Rigaud, S., Cossa, D., Knoery,
J., Couture, R. L.-M., Radakovitch, O., Yakubov, S., Krzeminska, D., and
Newton, A.: Modeling the influence of eutrophication and redox conditions on
mercury cycling at the sediment-water interface in the Berre Lagoon,
Front. Marine Sci., 5, 291, https://doi.org/10.3389/fmars.2018.00291, 2018.
Paquette, K. and Helz, G.: Solubility of cinnabar (red HgS) and implications for mercury speciation in sulfidic
waters, Water Air Soil Pollut., 80, 1053–1056, https://doi.org/10.1007/BF01189765, 1995.
Parks, J. M., Johs, A., Podar, M., Bridou, R., Hurt, R. A., Smith, S. D.,
Tomanicek, S. J., Qian, Y., Brown, S. D., Brandt, C. C., Palumbo, A. V., Smith,
J. C., Wall, J. D., Elias, D. A., and Liang, L.: The genetic basis for bacterial mercury methylation, Science, 339, 1332–1335,
2013.
Pauly, D., Christensen, V., Guénette, S., Pitcher, T. J., Rashid Sumaila, U., Walters, C. J., Watson, R. and Zeller, D.: Towards sustainability in world fisheries, Nature, 418, 689–695, https://doi.org/10.1038/nature01017, 2002.
Petersen, G., Bloxan, R., Wong, S., Munthe, J., Krüger, O., Schmolcke, S. R., and Kumar, A. V.: A
comprehensive Eulerian modeling framework for airborne mercury species: model development and
application in Europe, Atmos. Environ., 35, 3063–3074, https://doi.org/10.1016/S1352-2310(01)00110-8,
2001.
Pickhardt, P. C. and Fisher, N. S.: Accumulation of inorganic and
methylmercury by freshwater phytoplankton in two contrasting water bodies,
Environ. Sci. Technol., 41, 125–131, https://doi.org/10.1021/es060966w, 2007.
Pickhardt, P. C., Stepanova, M., and Fisher, N. S.: Contrasting uptake routes and tissue
distributions of inorganic and methylmercury in mosquitofish (Gambusia affinis) and redear sunfish
(Lepomis microlophus), Environ. Toxicol. Chem., 25.8, 2132–2142,
https://doi.org/10.1021/es060966w, 2006.
Pirrone, N., Cinnirella, S., Feng, X., Finkelman, R. B., Friedli, H. R., Leaner, J., Mason, R., Mukherjee, A. B., Stracher, G. B., Streets, D. G., and Telmer, K.: Global mercury emissions to the atmosphere from anthropogenic and natural sources, Atmos. Chem. Phys., 10, 5951–5964, https://doi.org/10.5194/acp-10-5951-2010, 2010.
Puty, B., Reis Leão, L. K., Crespo-Lopez, M. E., Costa Ponte Sousa Carvalho
Almeida, A. P., Fernandes Fagundes, N. C., Cople Maia, L., and Rodrigues Lima, R.:
Association between methylmercury environmental exposure and neurological disorders: A systematic
review, J. Trace Elem. Med. Bio., 52, 100–110, https://doi.org/10.1016/j.jtemb.2018.12.001, 2019.
Qureshi, A., MacLeod, M., Scheringer, M., and Hungerbuehler, K.: Mercury cycling and speices mass
balances in four North American lakes, Environ. Pollut., 157, 452–462,
https://doi.org/10.1016/j.envpol.2008.09.023, 2009.
Ricciardi, A. and Bourget, E.: Weight-to-weight conversion factors for
marine benthic macroinvertebrates, Mar. Ecol. Prog. Ser., 163,
245–251, 1998.
Rockel, B.: COSMO-CLM Starter Package (4.0), Zenodo [code], https://doi.org/10.5281/zenodo.5939757, 2022.
Rockel, B., Will, A., and Hense, A.: The Regional Climate Model COSMOCLM
(CCLM), Meteorol. Z., 17, 347–248, 2008.
Rosati, G., Canu, D., Lazzari, P., and Solidoro, C.: Assessing the spatial and temporal variability of methylmercury biogeochemistry and bioaccumulation in the Mediterranean Sea with a coupled 3D model, Biogeosciences, 19, 3663–3682, https://doi.org/10.5194/bg-19-3663-2022, 2022.
Ryaboshapko, A., Bullock, R., Ebinghaus, R., Ilyin, I., Lohman, K., Munthe, J., Petersen, G., Seigneur, I.,
and Wängberg, I.: Comparison of mercury chemistry models, Atmos. Environ., 36, 3881–3898,
https://doi.org/10.1016/S1352-2310(02)00351-5, 2002.
Schartup, A. T., Qureshi, A., Dassuncao, C., Thackray, C. P., Harding, G.,
and Sunderland, E. M.: A model for methylmercury uptake and trophic transfer by marine
plankton, Environ. Sci. Technol., 52, 654–662, https://doi.org/10.1021/acs.est.7b03821, 2018.
Schrum, C. and Backhaus, J. O.: Sensitivity of atmosphere-ocean heat exchange and heat content in the
North Sea and the Baltic Sea, Tellus A, 51, 526–549, https://doi.org/10.1034/j.1600-0870.1992.00006.x,
1999.
Schrum, C., Alekseeva, I., and St. John, M.: Development of a coupled physical–biological ecosystem
model ECOSMO, J. Mar. Syst., 61, 79–99, https://doi.org/10.1016/j.jmarsys.2006.01.005, 2006.
Schutgens, N. A. J., Gryspeerdt, E., Weigum, N., Tsyro, S., Goto, D., Schulz, M., and Stier, P.: Will a perfect model agree with perfect observations? The impact of spatial sampling, Atmos. Chem. Phys., 16, 6335–6353, https://doi.org/10.5194/acp-16-6335-2016, 2016.
Schwarzenbach, R. P., Gschwend, P. M., and Imboden, D. M.: Air-water exchange, Environ.
Org. Chem., 2, 889–890, 2003.
Seigneur, C., Laramchandani, P., Lohman, K., and Vijayaraghavan, K.: Multiscal modeling of the
atmospheric fate and transport of mercury, J. Geophys. Res., 106, 27795–27809,
https://doi.org/10.1029/2000JD000273, 2001.
Selin, N. E., Jacob, D. J., Yantosca, R. M., Strode, S., Jaeglé, L., and
Sunderland, E. M.: Global 3-D land-ocean-atmosphere model for mercury:
present-day versus preindustrial cycles and anthropogenic enrichment factors
for deposition, Global Biogeochem. Cycles, 22, GB2011, https://doi.org/10.1029/2007GB003040, 2008.
Semeniuk, K. and Dastoor, A.: Development of a global ocean mercury model
with a methylation cycle: outstanding issues, Global Biogeochem. Cycles, 31,
400–433, 2017.
Sharif, A., Monperrus, M., Tessier, E., Bouchet, S., Pinaly, H.,
Rodriguez-Gonzalez, P., Maron, P., Amouroux, D.: Fate of mercury species in the coastal
plume of the Adour River estuary (Bay of Biscay, SW France), Sci. Total Environ., 496,
701–713, https://doi.org/10.1016/j.scitotenv.2014.06.116, 2014.
Sicko-Goad, L. M., Schelske, C. L., and Stoermer, E. F.:
Estimation of intracellular carbon
and silica content of diatoms from natural assemblages using morphometric
techniques, Limnol.
Oceanogr., 29, 1170–178, 1984.
Slemr, F., Weigelt, A., Ebinghaus, R., Bieser, J., Brenninkmeijer, C. A. M., Rauthe-Schöch, A., Hermann, M., Martinsson, B. G., van Velthoven, P., Bönisch, H., Neumaier, M., Zahn, A., and Ziereis, H.: Mercury distribution in the upper troposphere and lowermost stratosphere according to measurements by the IAGOS-CARIBIC observatory: 2014–2016, Atmos. Chem. Phys., 18, 12329–12343, https://doi.org/10.5194/acp-18-12329-2018, 2018.
Slowey, A. J.: Rate of formation and dissolution of mercury sulfide nanoparticles: The dual role of
natural organic matter, Geochim. Cosmochim. Ac., 74, 4693–4708,
https://doi.org/10.1016/j.gca.2010.05.012, 2010.
Soerensen, A. L. and Faxneld, S.: The Swedish National Monitoring
Programme for Contaminants in Marine Biota (until 2019 year's data) –
Temporal trends and spatial variations, Stockholm, Överenskommelse: 2213-16-003, Geological Survey of Sweden [data set], https://www.sgu.se/produkter-och-tjanster/nationella-datavardskap/datavardskap-for-miljogifter/biota/
(last access: 1 March 2023), 2020.
Soerensen, A. L., Sunderland, E., Holmes, C. D., Jacob, D. J., Yantosca, R. M.,
Skov, H., Christensen, J. H., Strode, S. A., and Mason, R. P.: An improved
global model for air-sea exchange of mercury: High concentrations over the
North Atlantic, Environ. Sci. Technol., 44, 8574–8580, 2010.
Soerensen, A. L., Jacob, D. J., Schartup, A. T., Fisher, J. A., Lehnherr, I.,
St. Louis, V. L., Heimbürger, L.-E., Sonke, J. E., Krabbenhoft, D. P., and
Sunderland, E. M.: A mass budget for mercury and methylmercury in the Arctic
Ocean, Global Biogeochem. Cycles, 30, 560–575, 2016a.
Soerensen, A. L., Schartup, A. T., Gustafsson, E., Gustafsson, B. G., Undeman,
E., and Erik Björn, E.: Eutrophication increases phytoplankton
methylmercury concentrations in a coastal sea – A Baltic Sea case study,
Environ. Sci. Technol., 50, 11787–11796, 2016b.
Soerensen, A. L., Schartup, A. T., Skrobonja, A., and Björn, E.: Organic
matter drives high interannual variability in methylmercury concentrations
in a subarctic coastal sea, Environ. Pollut., 299, 531–538, 2017.
Soerensen, A. L., Schartup, A. T., Skrobonja, A., Bouchet, S., Amouroux, D.,
Liem-Nguyen, V., and Björn, E.: Deciphering the role of water column
redoxclines on methylmercury cycling using speciation modeling and
observations from the Baltic Sea, Global Biogeochem. Cycles, 32, 11787–11796, 2018.
Song, S., Selin, N. E., Soerensen, A. L., Angot, H., Artz, R., Brooks, S., Brunke, E.-G., Conley, G., Dommergue, A., Ebinghaus, R., Holsen, T. M., Jaffe, D. A., Kang, S., Kelley, P., Luke, W. T., Magand, O., Marumoto, K., Pfaffhuber, K. A., Ren, X., Sheu, G.-R., Slemr, F., Warneke, T., Weigelt, A., Weiss-Penzias, P., Wip, D. C., and Zhang, Q.: Top-down constraints on atmospheric mercury emissions and implications for global biogeochemical cycling, Atmos. Chem. Phys., 15, 7103–7125, https://doi.org/10.5194/acp-15-7103-2015, 2015.
Sørland, S. L., Brogli, R., Pothapakula, P. K., Russo, E., Van de Walle, J., Ahrens, B., Anders, I., Bucchignani, E., Davin, E. L., Demory, M.-E., Dosio, A., Feldmann, H., Früh, B., Geyer, B., Keuler, K., Lee, D., Li, D., van Lipzig, N. P. M., Min, S.-K., Panitz, H.-J., Rockel, B., Schär, C., Steger, C., and Thiery, W.: COSMO-CLM regional climate simulations in the Coordinated Regional Climate Downscaling Experiment (CORDEX) framework: a review, Geosci. Model Dev., 14, 5125–5154, https://doi.org/10.5194/gmd-14-5125-2021, 2021.
Streets, D. G., Horowitz, H. M., Lu, Z., Levin, L., Thackray, C. P., and
Sunderland, E. M.: Five hundred years of anthropogenic mercury: spatial and
temporal release profiles, Environ. Res. Lett., 14, 084004, https://doi.org/10.1088/1748-9326/ab281f, 2019.
Strode, S., Jaeglé, L., Selin, N. E., Jacob, D. J., Park, R. J., Yantosca,
R. M., Mason, R. P., and Slemr, F.: Air-sea exchange in the global mercury
cycle, Global Biogeochem. Cycles, 21, GB1017, https://doi.org/10.1029/2006GB002766, 2007.
Sunderland, E. M. and Mason, R. P.: Human impacts on open ocean mercury
concentrations, Global Biogeochem. Cycles, 21, GB4022, https://doi.org/10.1029/2006GB002876, 2007.
Sunderland, E. M., Krabbenhoft, D. P., Moreau, J. W., Strode, S. A., and
Landing, W. M.: Mercury sources, distribution, and bioavailability in the
North Pacific Ocean: insights from data and models, Global Biogeochem.
Cycles, 23, GB2010, https://doi.org/10.1029/2008GB003425, 2009.
Sunderland, E. M., Li, M., and Bullard, K.: Decadal changes in the edible supply of seafood and
methylmercury exposure in the United States, Environ. Health
Persp., 126, 017006, https://doi.org/10.1289/EHP2644, 2018.
Tesán Onrubia, J. A., Petrova, M. V., Puigcorbé, V., Black, E. E.,
Valk, O., Dufour, A., Hamelin, B., Buesseler, K. O., Masqué, P., Le Moigne, F. A. C., Sonke, J. E.,
Rutgers Van Der Loeff, M., and Heimbürger-Boavida, L. E.: Mercury Export Flux in the Arctic Ocean
Estimated from 234Th
Thunis, P., Pederzoli, A., and Pernigotti, D.: Performance criteria to
evaluate air
quality modeling applications, Atmos. Environ., 59, 476e482, https://doi.org/10.1016/j.atmosenv.2012.05.043, 2012.
Thunis, P., Pernigotti, D., and Gerboles, M.: Model quality objectives based
on measurement uncertainty. Part I: Ozone, Atmos. Environ., 79, 861–868,
https://doi.org/10.1016/j.atmosenv.2013.05, 2013.
Travnikov, O. and Ilyin, I.: The EMEP/MSC-E Mercury ModelingSystem, in:
Mercury Fate and Transport in the Global Atmosphere: Emissions,
Measurements, and Models, edited by: Pirrone, N. and Mason, R. P., Springer,
US, 571–587, 2009.
Travnikov, O., Jonson, J. E., Andersen, A. S., Gauss, M., Gusev, A.,
Rozovskaya, O., Simpson, D., Sokovyh, V., Valiyaveetil, S., and Wind, P.:
Development of the EMEP global modellingframework, Progress report,
EMEP/MSC-E Technical Report7/2009, Meteorological Synthesizing Centre –
East of EMEP, Moscow, 44 pp., http://www.msceast.org/index.php/publications/reports (last access: June 2017), 2009.
Travnikov, O., Angot, H., Artaxo, P., Bencardino, M., Bieser, J., D'Amore, F., Dastoor, A., De Simone, F., Diéguez, M. D. C., Dommergue, A., Ebinghaus, R., Feng, X. B., Gencarelli, C. N., Hedgecock, I. M., Magand, O., Martin, L., Matthias, V., Mashyanov, N., Pirrone, N., Ramachandran, R., Read, K. A., Ryjkov, A., Selin, N. E., Sena, F., Song, S., Sprovieri, F., Wip, D., Wängberg, I., and Yang, X.: Multi-model study of mercury dispersion in the atmosphere: atmospheric processes and model evaluation, Atmos. Chem. Phys., 17, 5271–5295, https://doi.org/10.5194/acp-17-5271-2017, 2017.
Tsui, M. T. K. and Wang, W. X.: Uptake and elimination routes of inorganic
mercuryand methylmercury in Daphnia magna, Environ. Sci. Technol., 38,
808–816, 2004.
US EPA Office of Research and Development: CMAQv4.7.1 (4.7.1), Zenodo [code], https://doi.org/10.5281/zenodo.1079879, 2010.
Walve, J. and Larsson, U.: Carbon, nitrogen and phosphorus stoichiometry of crustacean zooplankton in
the Baltic Sea: implications for nutrient recycling, J. Plankton Res., 21, 2309–2321, https://doi.org/10.1093/plankt/21.12.2309, 1999.
Wang, W.-X. and Wong, R. S. K.: Bioaccumulation kinetics and exposure pathways of
inorganic mercury and methylmercury in a marine fish, the sweetlips Plectorhinchus gibbosus, Marine
Ecol. Prog. Ser., 261, 257–268, https://doi.org/10.3354/meps261257, 2003.
Xu, X., Yang, X., Miller, D. R., Helble, J. J., and Carley, R. J.: A regional scale modeling study of
atmospheric transport and transformation of mercury. I. Model development and evaluation, Atmos.
Envrion., 24 4933–4944, https://doi.org/10.1016/S1352-2310(00)00228-4, 2000.
Zhang, Y., Jaegle, L., and Thompson, L.: Natural biogeochemical cycle of
mercury in a global three-dimensional ocean tracer model, Global Biogeochem.
Cycles, 28, 553–570, 2014a.
Zhang, Y., Jaegle, L., Thompson, L., and Streets, D.G.: Six centuries of
changing oceanic mercury, Global. Biogeochem. Cycles, 28, 1251–1261, 2014b.
Zhang, Y., Horowitz, H., Wang, J., Xie, Z., Kuss, J., and Soerensen, A. L.: A
coupled global atmosphere-ocean model for air-sea exchange of mercury:
insights into wet deposition and atmospheric redox chemistry, Environ. Sci.
Technol., 53, 5052–5061, 2019.
Zhang, Y., Soerensen, A. L., Schartup, A. T., and Sunderland, E. M.: A Global Model for Methylmercury
Formation and Uptake at the Base of Marine Food Webs, Global Biogeochem. Cycles, 34,
e2019GB006348, https://doi.org/10.1029/2019GB006348, 2020.
Zhu, J., Wang, T., Bieser, J., and Matthias, V.: Source attribution and process analysis for atmospheric mercury in eastern China simulated by CMAQ-Hg, Atmos. Chem. Phys., 15, 8767–8779, https://doi.org/10.5194/acp-15-8767-2015, 2015.
Short summary
MERCY is a 3D model to study mercury (Hg) cycling in the ocean. Hg is a highly harmful pollutant regulated by the UN Minamata Convention on Mercury due to widespread human emissions. These emissions eventually reach the oceans, where Hg transforms into the even more toxic and bioaccumulative pollutant methylmercury. MERCY predicts the fate of Hg in the ocean and its buildup in the food chain. It is the first model to consider Hg accumulation in fish, a major source of Hg exposure for humans.
MERCY is a 3D model to study mercury (Hg) cycling in the ocean. Hg is a highly harmful pollutant...
