Articles | Volume 14, issue 3
https://doi.org/10.5194/gmd-14-1219-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/gmd-14-1219-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Model evaluation paper
| 
05 Mar 2021
Model evaluation paper |
| 05 Mar 2021
| 05 Mar 2021
Evaluation of the interactive stratospheric ozone (O3v2) module in the E3SM version 1 Earth system model
Lawrence Livermore National Laboratory, Livermore, CA 94550, USA
Michael J. Prather
Departments of Earth System Science, University of California, Irvine, CA 92697, USA
Departments of Earth System Science, University of California, Irvine, CA 92697, USA
Daniel J. Ruiz
Departments of Earth System Science, University of California, Irvine, CA 92697, USA
Philip J. Cameron-Smith
Lawrence Livermore National Laboratory, Livermore, CA 94550, USA
Shaocheng Xie
Lawrence Livermore National Laboratory, Livermore, CA 94550, USA
Jean-Christophe Golaz
Lawrence Livermore National Laboratory, Livermore, CA 94550, USA
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Qi Tang, Stephen A. Klein, Shaocheng Xie, Wuyin Lin, Jean-Christophe Golaz, Erika L. Roesler, Mark A. Taylor, Philip J. Rasch, David C. Bader, Larry K. Berg, Peter Caldwell, Scott E. Giangrande, Richard B. Neale, Yun Qian, Laura D. Riihimaki, Charles S. Zender, Yuying Zhang, and Xue Zheng
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Kai Zhang, Philip J. Rasch, Mark A. Taylor, Hui Wan, Ruby Leung, Po-Lun Ma, Jean-Christophe Golaz, Jon Wolfe, Wuyin Lin, Balwinder Singh, Susannah Burrows, Jin-Ho Yoon, Hailong Wang, Yun Qian, Qi Tang, Peter Caldwell, and Shaocheng Xie
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We evaluated how well we can infer air pollutant levels (ozone, carbon monoxide, and nitrogen oxides) between air quality stations throughout South Korea, finding good representation in most densely measured cities in spite of intense small-scale emission hotspots. Comparing observed air quality with gridded model output is desirable, and so we created gridded datasets over South Korea using air quality station measurements, which agreed with airborne measurements around Seoul.
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Katherine M. Smith, Alice M. Barthel, LeAnn M. Conlon, Luke P. Van Roekel, Anthony Bartoletti, Jean-Christophe Golaz, Chengzhu Zhang, Carolyn Branecky Begeman, James J. Benedict, Gautam Bisht, Yan Feng, Walter Hannah, Bryce E. Harrop, Nicole Jeffery, Wuyin Lin, Po-Lun Ma, Mathew E. Maltrud, Mark R. Petersen, Balwinder Singh, Qi Tang, Teklu Tesfa, Jonathan D. Wolfe, Shaocheng Xie, Xue Zheng, Karthik Balaguru, Oluwayemi Garuba, Peter Gleckler, Aixue Hu, Jiwoo Lee, Ben Moore-Maley, and Ana C. Ordoñez
Geosci. Model Dev., 18, 1613–1633, https://doi.org/10.5194/gmd-18-1613-2025, https://doi.org/10.5194/gmd-18-1613-2025, 2025
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Version 2.1 of the U.S. Department of Energy's Energy Exascale Earth System Model (E3SM) adds the Fox-Kemper et al. (2011) mixed-layer eddy parameterization, which restratifies the ocean surface layer through an overturning streamfunction. Results include surface layer bias reduction in temperature, salinity, and sea ice extent in the North Atlantic; a small strengthening of the Atlantic meridional overturning circulation; and improvements to many atmospheric climatological variables.
Mingxuan Wu, Hailong Wang, Zheng Lu, Xiaohong Liu, Huisheng Bian, David Cohen, Yan Feng, Mian Chin, Didier A. Hauglustaine, Vlassis A. Karydis, Marianne T. Lund, Gunnar Myhre, Andrea Pozzer, Michael Schulz, Ragnhild B. Skeie, Alexandra P. Tsimpidi, Svetlana G. Tsyro, and Shaocheng Xie
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A key challenge in simulating the lifecycle of nitrate aerosol in global climate models is to accurately represent mass size distribution of nitrate aerosol, which lacks sufficient observational constraints. We found that most climate models underestimate the mass fraction of fine-mode nitrate at surface in all regions. Our study highlights the importance of gas-aerosol partitioning parameterization and simulation of dust and sea salt in correctly simulating mass size distribution of nitrate.
Maryam Ramezani Ziarani, Miriam Sinnhuber, Thomas Reddmann, Bernd Funke, Stefan Bender, and Michael Prather
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Preprint under review for GMD
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Our study aims to present a new method for incorporating top-down solar forcing into stratospheric ozone relying on linearized ozone scheme. The addition of geomagnetic forcing led to significant ozone losses in the polar upper stratosphere of both hemispheres due to the catalytic cycles involving NOy. In addition to the particle precipitation effect, accounting for solar UV variability in the ICON-ART model leads to the changes in ozone in the tropical stratosphere.
Peter A. Bogenschutz, Jishi Zhang, Qi Tang, and Philip Cameron-Smith
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Using high-resolution and state-of-the-art modeling techniques we simulate five atmospheric river events for California to test the capability to represent precipitation for these events. We find that our model is able to capture the distribution of precipitation very well but suffers from overestimating the precipitation amounts over high elevation. Increasing the resolution further has no impact on reducing this bias, while increasing the domain size does have modest impacts.
Paul T. Griffiths, Laura J. Wilcox, Robert J. Allen, Vaishali Naik, Fiona M. O'Connor, Michael J. Prather, Alexander T. Archibald, Florence Brown, Makoto Deushi, William Collins, Stephanie Fiedler, Naga Oshima, Lee T. Murray, Christopher J. Smith, Steven T. Turnock, Duncan Watson-Parris, and Paul J. Young
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Analysis of the interaction between the climate and ozone in the stratosphere is complicated by the in-ability climate model in simulating the Quasi-Biennial Oscillation (QBO) – an important climate mode in the stratosphere. We use a set of model simulation that realistically simulate QBO and a novel ozone diagnostic tool to separate the temperature and circulation-driven QBO impact. These are important for diagnosing model-model differences in the QBO-ozone responses for climate projections.
Hanqin Tian, Naiqing Pan, Rona L. Thompson, Josep G. Canadell, Parvadha Suntharalingam, Pierre Regnier, Eric A. Davidson, Michael Prather, Philippe Ciais, Marilena Muntean, Shufen Pan, Wilfried Winiwarter, Sönke Zaehle, Feng Zhou, Robert B. Jackson, Hermann W. Bange, Sarah Berthet, Zihao Bian, Daniele Bianchi, Alexander F. Bouwman, Erik T. Buitenhuis, Geoffrey Dutton, Minpeng Hu, Akihiko Ito, Atul K. Jain, Aurich Jeltsch-Thömmes, Fortunat Joos, Sian Kou-Giesbrecht, Paul B. Krummel, Xin Lan, Angela Landolfi, Ronny Lauerwald, Ya Li, Chaoqun Lu, Taylor Maavara, Manfredi Manizza, Dylan B. Millet, Jens Mühle, Prabir K. Patra, Glen P. Peters, Xiaoyu Qin, Peter Raymond, Laure Resplandy, Judith A. Rosentreter, Hao Shi, Qing Sun, Daniele Tonina, Francesco N. Tubiello, Guido R. van der Werf, Nicolas Vuichard, Junjie Wang, Kelley C. Wells, Luke M. Western, Chris Wilson, Jia Yang, Yuanzhi Yao, Yongfa You, and Qing Zhu
Earth Syst. Sci. Data, 16, 2543–2604, https://doi.org/10.5194/essd-16-2543-2024, https://doi.org/10.5194/essd-16-2543-2024, 2024
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Atmospheric concentrations of nitrous oxide (N2O), a greenhouse gas 273 times more potent than carbon dioxide, have increased by 25 % since the preindustrial period, with the highest observed growth rate in 2020 and 2021. This rapid growth rate has primarily been due to a 40 % increase in anthropogenic emissions since 1980. Observed atmospheric N2O concentrations in recent years have exceeded the worst-case climate scenario, underscoring the importance of reducing anthropogenic N2O emissions.
Ziming Ke, Qi Tang, Jean-Christoophe Golaz, Xiaohong Liu, and Hailong Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-1612, https://doi.org/10.5194/egusphere-2024-1612, 2024
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By treating volcanic emission interactively, model results improve simulated temperature variability, showing better correlations for 1940–1959 and 1960–1979, and reveals how volcanic activity influences cloud behavior and climate.
Jishi Zhang, Peter Bogenschutz, Qi Tang, Philip Cameron-smith, and Chengzhu Zhang
Geosci. Model Dev., 17, 3687–3731, https://doi.org/10.5194/gmd-17-3687-2024, https://doi.org/10.5194/gmd-17-3687-2024, 2024
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We developed a regionally refined climate model that allows resolved convection and performed a 20-year projection to the end of the century. The model has a resolution of 3.25 km in California, which allows us to predict climate with unprecedented accuracy, and a resolution of 100 km for the rest of the globe to achieve efficient, self-consistent simulations. The model produces superior results in reproducing climate patterns over California that typical modern climate models cannot resolve.
John T. Fasullo, Jean-Christophe Golaz, Julie M. Caron, Nan Rosenbloom, Gerald A. Meehl, Warren Strand, Sasha Glanville, Samantha Stevenson, Maria Molina, Christine A. Shields, Chengzhu Zhang, James Benedict, Hailong Wang, and Tony Bartoletti
Earth Syst. Dynam., 15, 367–386, https://doi.org/10.5194/esd-15-367-2024, https://doi.org/10.5194/esd-15-367-2024, 2024
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Climate model large ensembles provide a unique and invaluable means for estimating the climate response to external forcing agents and quantify contrasts in model structure. Here, an overview of the Energy Exascale Earth System Model (E3SM) version 2 large ensemble is given along with comparisons to large ensembles from E3SM version 1 and versions 1 and 2 of the Community Earth System Model. The paper provides broad and important context for users of these ensembles.
Hsiang-He Lee, Qi Tang, and Michael Prather
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2023-203, https://doi.org/10.5194/gmd-2023-203, 2024
Revised manuscript not accepted
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The E3SM Chemistry diagnostics package (ChemDyg) is a software tool, which is designed for the global climate model (E3SM) chemistry development. ChemDyg generates several diagnostic plots and tables for model-to-model and model-to-observation comparison, including 2-dimentional contour mapping plots, diurnal and annual cycle, time-series plots, and comprehensive processing tables. This paper is to introduce the details of each diagnostics set and its required input data formats in ChemDyg.
Yuying Zhang, Shaocheng Xie, Yi Qin, Wuyin Lin, Jean-Christophe Golaz, Xue Zheng, Po-Lun Ma, Yun Qian, Qi Tang, Christopher R. Terai, and Meng Zhang
Geosci. Model Dev., 17, 169–189, https://doi.org/10.5194/gmd-17-169-2024, https://doi.org/10.5194/gmd-17-169-2024, 2024
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We performed systematic evaluation of clouds simulated in the Energy
Exascale Earth System Model (E3SMv2) to document model performance and understand what updates in E3SMv2 have caused changes in clouds from E3SMv1 to E3SMv2. We find that stratocumulus clouds along the subtropical west coast of continents are dramatically improved, primarily due to the retuning done in CLUBB. This study offers additional insights into clouds simulated in E3SMv2 and will benefit future E3SM developments.
Exascale Earth System Model (E3SMv2) to document model performance and understand what updates in E3SMv2 have caused changes in clouds from E3SMv1 to E3SMv2. We find that stratocumulus clouds along the subtropical west coast of continents are dramatically improved, primarily due to the retuning done in CLUBB. This study offers additional insights into clouds simulated in E3SMv2 and will benefit future E3SM developments.
Michael J. Prather, Hao Guo, and Xin Zhu
Earth Syst. Sci. Data, 15, 3299–3349, https://doi.org/10.5194/essd-15-3299-2023, https://doi.org/10.5194/essd-15-3299-2023, 2023
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The Atmospheric Tomography Mission (ATom) measured the chemical composition in air parcels from 0–12 km altitude on 2 km horizontal by 80 m vertical scales for four seasons, resolving most scales of chemical heterogeneity. ATom is one of the first missions designed to calculate the chemical evolution of each parcel, providing semi-global diurnal budgets for ozone and methane. Observations covered the remote troposphere: Pacific and Atlantic Ocean basins, Southern Ocean, Arctic basin, Antarctica.
Qi Tang, Jean-Christophe Golaz, Luke P. Van Roekel, Mark A. Taylor, Wuyin Lin, Benjamin R. Hillman, Paul A. Ullrich, Andrew M. Bradley, Oksana Guba, Jonathan D. Wolfe, Tian Zhou, Kai Zhang, Xue Zheng, Yunyan Zhang, Meng Zhang, Mingxuan Wu, Hailong Wang, Cheng Tao, Balwinder Singh, Alan M. Rhoades, Yi Qin, Hong-Yi Li, Yan Feng, Yuying Zhang, Chengzhu Zhang, Charles S. Zender, Shaocheng Xie, Erika L. Roesler, Andrew F. Roberts, Azamat Mametjanov, Mathew E. Maltrud, Noel D. Keen, Robert L. Jacob, Christiane Jablonowski, Owen K. Hughes, Ryan M. Forsyth, Alan V. Di Vittorio, Peter M. Caldwell, Gautam Bisht, Renata B. McCoy, L. Ruby Leung, and David C. Bader
Geosci. Model Dev., 16, 3953–3995, https://doi.org/10.5194/gmd-16-3953-2023, https://doi.org/10.5194/gmd-16-3953-2023, 2023
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High-resolution simulations are superior to low-resolution ones in capturing regional climate changes and climate extremes. However, uniformly reducing the grid size of a global Earth system model is too computationally expensive. We provide an overview of the fully coupled regionally refined model (RRM) of E3SMv2 and document a first-of-its-kind set of climate production simulations using RRM at an economic cost. The key to this success is our innovative hybrid time step method.
Dana L. McGuffin, Philip J. Cameron-Smith, Matthew A. Horsley, Brian J. Bauman, Wim De Vries, Denis Healy, Alex Pertica, Chris Shaffer, and Lance M. Simms
Atmos. Meas. Tech., 16, 2129–2144, https://doi.org/10.5194/amt-16-2129-2023, https://doi.org/10.5194/amt-16-2129-2023, 2023
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This work demonstrates the viability of a remote sensing technique using nanosatellites to measure stratospheric temperature. This measurement technique can probe the stratosphere and mesosphere at a fine vertical scale around the globe unlike other high-altitude measurement techniques, which would provide an opportunity to observe atmospheric gravity waves and turbulence. We analyze observations from two satellite platforms to provide a proof of concept and characterize measurement uncertainty.
Michael J. Prather, Lucien Froidevaux, and Nathaniel J. Livesey
Atmos. Chem. Phys., 23, 843–849, https://doi.org/10.5194/acp-23-843-2023, https://doi.org/10.5194/acp-23-843-2023, 2023
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From satellite data for nitrous oxide (N2O), ozone and temperature, we calculate the monthly loss of N2O and find it is increasing faster than expected, resulting in a shorter lifetime, which reduces the impact of anthropogenic emissions. We identify the cause as enhanced vertical lofting of high-N2O air into the tropical middle stratosphere, where it is destroyed photochemically. Because global warming is due in part to N2O, this finding presents a new negative climate-chemistry feedback.
Peter A. Bogenschutz, Hsiang-He Lee, Qi Tang, and Takanobu Yamaguchi
Geosci. Model Dev., 16, 335–352, https://doi.org/10.5194/gmd-16-335-2023, https://doi.org/10.5194/gmd-16-335-2023, 2023
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Models that are used to simulate and predict climate often have trouble representing specific cloud types, such as stratocumulus, that are particularly thin in the vertical direction. It has been found that increasing the model resolution can help improve this problem. In this paper, we develop a novel framework that increases the horizontal and vertical resolutions only for areas of the globe that contain stratocumulus, hence reducing the model runtime while providing better results.
Hao Guo, Clare M. Flynn, Michael J. Prather, Sarah A. Strode, Stephen D. Steenrod, Louisa Emmons, Forrest Lacey, Jean-Francois Lamarque, Arlene M. Fiore, Gus Correa, Lee T. Murray, Glenn M. Wolfe, Jason M. St. Clair, Michelle Kim, John Crounse, Glenn Diskin, Joshua DiGangi, Bruce C. Daube, Roisin Commane, Kathryn McKain, Jeff Peischl, Thomas B. Ryerson, Chelsea Thompson, Thomas F. Hanisco, Donald Blake, Nicola J. Blake, Eric C. Apel, Rebecca S. Hornbrook, James W. Elkins, Eric J. Hintsa, Fred L. Moore, and Steven C. Wofsy
Atmos. Chem. Phys., 23, 99–117, https://doi.org/10.5194/acp-23-99-2023, https://doi.org/10.5194/acp-23-99-2023, 2023
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We have prepared a unique and unusual result from the recent ATom aircraft mission: a measurement-based derivation of the production and loss rates of ozone and methane over the ocean basins. These are the key products of chemistry models used in assessments but have thus far lacked observational metrics. It also shows the scales of variability of atmospheric chemical rates and provides a major challenge to the atmospheric models.
Chengzhu Zhang, Jean-Christophe Golaz, Ryan Forsyth, Tom Vo, Shaocheng Xie, Zeshawn Shaheen, Gerald L. Potter, Xylar S. Asay-Davis, Charles S. Zender, Wuyin Lin, Chih-Chieh Chen, Chris R. Terai, Salil Mahajan, Tian Zhou, Karthik Balaguru, Qi Tang, Cheng Tao, Yuying Zhang, Todd Emmenegger, Susannah Burrows, and Paul A. Ullrich
Geosci. Model Dev., 15, 9031–9056, https://doi.org/10.5194/gmd-15-9031-2022, https://doi.org/10.5194/gmd-15-9031-2022, 2022
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Earth system model (ESM) developers run automated analysis tools on data from candidate models to inform model development. This paper introduces a new Python package, E3SM Diags, that has been developed to support ESM development and use routinely in the development of DOE's Energy Exascale Earth System Model. This tool covers a set of essential diagnostics to evaluate the mean physical climate from simulations, as well as several process-oriented and phenomenon-based evaluation diagnostics.
Kai Zhang, Wentao Zhang, Hui Wan, Philip J. Rasch, Steven J. Ghan, Richard C. Easter, Xiangjun Shi, Yong Wang, Hailong Wang, Po-Lun Ma, Shixuan Zhang, Jian Sun, Susannah M. Burrows, Manish Shrivastava, Balwinder Singh, Yun Qian, Xiaohong Liu, Jean-Christophe Golaz, Qi Tang, Xue Zheng, Shaocheng Xie, Wuyin Lin, Yan Feng, Minghuai Wang, Jin-Ho Yoon, and L. Ruby Leung
Atmos. Chem. Phys., 22, 9129–9160, https://doi.org/10.5194/acp-22-9129-2022, https://doi.org/10.5194/acp-22-9129-2022, 2022
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Here we analyze the effective aerosol forcing simulated by E3SM version 1 using both century-long free-running and short nudged simulations. The aerosol forcing in E3SMv1 is relatively large compared to other models, mainly due to the large indirect aerosol effect. Aerosol-induced changes in liquid and ice cloud properties in E3SMv1 have a strong correlation. The aerosol forcing estimates in E3SMv1 are sensitive to the parameterization changes in both liquid and ice cloud processes.
Xue Zheng, Qing Li, Tian Zhou, Qi Tang, Luke P. Van Roekel, Jean-Christophe Golaz, Hailong Wang, and Philip Cameron-Smith
Geosci. Model Dev., 15, 3941–3967, https://doi.org/10.5194/gmd-15-3941-2022, https://doi.org/10.5194/gmd-15-3941-2022, 2022
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We document the model experiments for the future climate projection by E3SMv1.0. At the highest future emission scenario, E3SMv1.0 projects a strong surface warming with rapid changes in the atmosphere, ocean, sea ice, and land runoff. Specifically, we detect a significant polar amplification and accelerated warming linked to the unmasking of the aerosol effects. The impact of greenhouse gas forcing is examined in different climate components.
Aurore Voldoire, Romain Roehrig, Hervé Giordani, Robin Waldman, Yunyan Zhang, Shaocheng Xie, and Marie-Nöelle Bouin
Geosci. Model Dev., 15, 3347–3370, https://doi.org/10.5194/gmd-15-3347-2022, https://doi.org/10.5194/gmd-15-3347-2022, 2022
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A single-column version of the global climate model CNRM-CM6-1 has been designed to ease development and validation of the model physics at the air–sea interface in a simplified environment. This model is then used to assess the ability to represent the sea surface temperature diurnal cycle. We conclude that the sea surface temperature diurnal variability is reasonably well represented in CNRM-CM6-1 with a 1 h coupling time step and the upper-ocean model resolution of 1 m.
Po-Lun Ma, Bryce E. Harrop, Vincent E. Larson, Richard B. Neale, Andrew Gettelman, Hugh Morrison, Hailong Wang, Kai Zhang, Stephen A. Klein, Mark D. Zelinka, Yuying Zhang, Yun Qian, Jin-Ho Yoon, Christopher R. Jones, Meng Huang, Sheng-Lun Tai, Balwinder Singh, Peter A. Bogenschutz, Xue Zheng, Wuyin Lin, Johannes Quaas, Hélène Chepfer, Michael A. Brunke, Xubin Zeng, Johannes Mülmenstädt, Samson Hagos, Zhibo Zhang, Hua Song, Xiaohong Liu, Michael S. Pritchard, Hui Wan, Jingyu Wang, Qi Tang, Peter M. Caldwell, Jiwen Fan, Larry K. Berg, Jerome D. Fast, Mark A. Taylor, Jean-Christophe Golaz, Shaocheng Xie, Philip J. Rasch, and L. Ruby Leung
Geosci. Model Dev., 15, 2881–2916, https://doi.org/10.5194/gmd-15-2881-2022, https://doi.org/10.5194/gmd-15-2881-2022, 2022
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An alternative set of parameters for E3SM Atmospheric Model version 1 has been developed based on a tuning strategy that focuses on clouds. When clouds in every regime are improved, other aspects of the model are also improved, even though they are not the direct targets for calibration. The recalibrated model shows a lower sensitivity to anthropogenic aerosols and surface warming, suggesting potential improvements to the simulated climate in the past and future.
Michael J. Prather
Earth Syst. Dynam., 13, 703–709, https://doi.org/10.5194/esd-13-703-2022, https://doi.org/10.5194/esd-13-703-2022, 2022
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Atmospheric CO2 fluctuations point to changes in fossil fuel emissions plus natural and perturbed variations in the natural carbon cycle. One unstudied source of variability is the stratosphere, where the influx of aged CO2-depleted air can cause surface fluctuations. Using modeling and, separately, scaling the observed N2O variability, I find that stratosphere-driven surface variability in CO2 is not a significant uncertainty (at most 10 % of the observed interannual variability).
Daniel J. Ruiz and Michael J. Prather
Atmos. Chem. Phys., 22, 2079–2093, https://doi.org/10.5194/acp-22-2079-2022, https://doi.org/10.5194/acp-22-2079-2022, 2022
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The stratosphere is an important source of tropospheric ozone, which affects climate, chemistry, and air quality, but is extremely difficult to quantify given the large production and loss terms in the troposphere. Here, we use other gases that are well observed and quantified as a reference to test our simulations of ozone transport in the atmosphere. This allows us to better constrain the stratospheric source of ozone and also offers guidance to improve future simulations of ozone transport.
Hao Guo, Clare M. Flynn, Michael J. Prather, Sarah A. Strode, Stephen D. Steenrod, Louisa Emmons, Forrest Lacey, Jean-Francois Lamarque, Arlene M. Fiore, Gus Correa, Lee T. Murray, Glenn M. Wolfe, Jason M. St. Clair, Michelle Kim, John Crounse, Glenn Diskin, Joshua DiGangi, Bruce C. Daube, Roisin Commane, Kathryn McKain, Jeff Peischl, Thomas B. Ryerson, Chelsea Thompson, Thomas F. Hanisco, Donald Blake, Nicola J. Blake, Eric C. Apel, Rebecca S. Hornbrook, James W. Elkins, Eric J. Hintsa, Fred L. Moore, and Steven Wofsy
Atmos. Chem. Phys., 21, 13729–13746, https://doi.org/10.5194/acp-21-13729-2021, https://doi.org/10.5194/acp-21-13729-2021, 2021
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The NASA Atmospheric Tomography (ATom) mission built a climatology of the chemical composition of tropospheric air parcels throughout the middle of the Pacific and Atlantic oceans. The level of detail allows us to reconstruct the photochemical budgets of O3 and CH4 over these vast, remote regions. We find that most of the chemical heterogeneity is captured at the resolution used in current global chemistry models and that the majority of reactivity occurs in the
hottest20 % of parcels.
Yongkang Xue, Tandong Yao, Aaron A. Boone, Ismaila Diallo, Ye Liu, Xubin Zeng, William K. M. Lau, Shiori Sugimoto, Qi Tang, Xiaoduo Pan, Peter J. van Oevelen, Daniel Klocke, Myung-Seo Koo, Tomonori Sato, Zhaohui Lin, Yuhei Takaya, Constantin Ardilouze, Stefano Materia, Subodh K. Saha, Retish Senan, Tetsu Nakamura, Hailan Wang, Jing Yang, Hongliang Zhang, Mei Zhao, Xin-Zhong Liang, J. David Neelin, Frederic Vitart, Xin Li, Ping Zhao, Chunxiang Shi, Weidong Guo, Jianping Tang, Miao Yu, Yun Qian, Samuel S. P. Shen, Yang Zhang, Kun Yang, Ruby Leung, Yuan Qiu, Daniele Peano, Xin Qi, Yanling Zhan, Michael A. Brunke, Sin Chan Chou, Michael Ek, Tianyi Fan, Hong Guan, Hai Lin, Shunlin Liang, Helin Wei, Shaocheng Xie, Haoran Xu, Weiping Li, Xueli Shi, Paulo Nobre, Yan Pan, Yi Qin, Jeff Dozier, Craig R. Ferguson, Gianpaolo Balsamo, Qing Bao, Jinming Feng, Jinkyu Hong, Songyou Hong, Huilin Huang, Duoying Ji, Zhenming Ji, Shichang Kang, Yanluan Lin, Weiguang Liu, Ryan Muncaster, Patricia de Rosnay, Hiroshi G. Takahashi, Guiling Wang, Shuyu Wang, Weicai Wang, Xu Zhou, and Yuejian Zhu
Geosci. Model Dev., 14, 4465–4494, https://doi.org/10.5194/gmd-14-4465-2021, https://doi.org/10.5194/gmd-14-4465-2021, 2021
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The subseasonal prediction of extreme hydroclimate events such as droughts/floods has remained stubbornly low for years. This paper presents a new international initiative which, for the first time, introduces spring land surface temperature anomalies over high mountains to improve precipitation prediction through remote effects of land–atmosphere interactions. More than 40 institutions worldwide are participating in this effort. The experimental protocol and preliminary results are presented.
James Keeble, Birgit Hassler, Antara Banerjee, Ramiro Checa-Garcia, Gabriel Chiodo, Sean Davis, Veronika Eyring, Paul T. Griffiths, Olaf Morgenstern, Peer Nowack, Guang Zeng, Jiankai Zhang, Greg Bodeker, Susannah Burrows, Philip Cameron-Smith, David Cugnet, Christopher Danek, Makoto Deushi, Larry W. Horowitz, Anne Kubin, Lijuan Li, Gerrit Lohmann, Martine Michou, Michael J. Mills, Pierre Nabat, Dirk Olivié, Sungsu Park, Øyvind Seland, Jens Stoll, Karl-Hermann Wieners, and Tongwen Wu
Atmos. Chem. Phys., 21, 5015–5061, https://doi.org/10.5194/acp-21-5015-2021, https://doi.org/10.5194/acp-21-5015-2021, 2021
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Stratospheric ozone and water vapour are key components of the Earth system; changes to both have important impacts on global and regional climate. We evaluate changes to these species from 1850 to 2100 in the new generation of CMIP6 models. There is good agreement between the multi-model mean and observations, although there is substantial variation between the individual models. The future evolution of both ozone and water vapour is strongly dependent on the assumed future emissions scenario.
Yong Wang, Guang J. Zhang, Shaocheng Xie, Wuyin Lin, George C. Craig, Qi Tang, and Hsi-Yen Ma
Geosci. Model Dev., 14, 1575–1593, https://doi.org/10.5194/gmd-14-1575-2021, https://doi.org/10.5194/gmd-14-1575-2021, 2021
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A stochastic deep convection parameterization is implemented into the US Department of Energy Energy Exascale Earth System Model Atmosphere Model version 1 (EAMv1). Compared to the default model, the well-known problem of
too much light rain and too little heavy rainis largely alleviated over the tropics with the stochastic scheme. Results from this study provide important insights into the model performance of EAMv1 when stochasticity is included in the deep convective parameterization.
Claudia Tebaldi, Kevin Debeire, Veronika Eyring, Erich Fischer, John Fyfe, Pierre Friedlingstein, Reto Knutti, Jason Lowe, Brian O'Neill, Benjamin Sanderson, Detlef van Vuuren, Keywan Riahi, Malte Meinshausen, Zebedee Nicholls, Katarzyna B. Tokarska, George Hurtt, Elmar Kriegler, Jean-Francois Lamarque, Gerald Meehl, Richard Moss, Susanne E. Bauer, Olivier Boucher, Victor Brovkin, Young-Hwa Byun, Martin Dix, Silvio Gualdi, Huan Guo, Jasmin G. John, Slava Kharin, YoungHo Kim, Tsuyoshi Koshiro, Libin Ma, Dirk Olivié, Swapna Panickal, Fangli Qiao, Xinyao Rong, Nan Rosenbloom, Martin Schupfner, Roland Séférian, Alistair Sellar, Tido Semmler, Xiaoying Shi, Zhenya Song, Christian Steger, Ronald Stouffer, Neil Swart, Kaoru Tachiiri, Qi Tang, Hiroaki Tatebe, Aurore Voldoire, Evgeny Volodin, Klaus Wyser, Xiaoge Xin, Shuting Yang, Yongqiang Yu, and Tilo Ziehn
Earth Syst. Dynam., 12, 253–293, https://doi.org/10.5194/esd-12-253-2021, https://doi.org/10.5194/esd-12-253-2021, 2021
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We present an overview of CMIP6 ScenarioMIP outcomes from up to 38 participating ESMs according to the new SSP-based scenarios. Average temperature and precipitation projections according to a wide range of forcings, spanning a wider range than the CMIP5 projections, are documented as global averages and geographic patterns. Times of crossing various warming levels are computed, together with benefits of mitigation for selected pairs of scenarios. Comparisons with CMIP5 are also discussed.
Hsi-Yen Ma, Chen Zhou, Yunyan Zhang, Stephen A. Klein, Mark D. Zelinka, Xue Zheng, Shaocheng Xie, Wei-Ting Chen, and Chien-Ming Wu
Geosci. Model Dev., 14, 73–90, https://doi.org/10.5194/gmd-14-73-2021, https://doi.org/10.5194/gmd-14-73-2021, 2021
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We propose an experimental design of a suite of multi-year, short-term hindcasts and compare them with corresponding observations or measurements for periods based on different weather and climate phenomena. This atypical way of evaluating model performance is particularly useful and beneficial, as these hindcasts can give scientists a robust picture of modeled precipitation, and cloud and radiation processes from their diurnal variation to year-to-year variability.
Landon A. Rieger, Jason N. S. Cole, John C. Fyfe, Stephen Po-Chedley, Philip J. Cameron-Smith, Paul J. Durack, Nathan P. Gillett, and Qi Tang
Geosci. Model Dev., 13, 4831–4843, https://doi.org/10.5194/gmd-13-4831-2020, https://doi.org/10.5194/gmd-13-4831-2020, 2020
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Recently, the stratospheric aerosol forcing dataset used as an input to the Coupled Model Intercomparison Project phase 6 was updated. This work explores the impact of those changes on the modelled historical climates in the CanESM5 and EAMv1 models. Temperature differences in the stratosphere shortly after the Pinatubo eruption are found to be significant, but surface temperatures and precipitation do not show a significant change.
Peter A. Bogenschutz, Shuaiqi Tang, Peter M. Caldwell, Shaocheng Xie, Wuyin Lin, and Yao-Sheng Chen
Geosci. Model Dev., 13, 4443–4458, https://doi.org/10.5194/gmd-13-4443-2020, https://doi.org/10.5194/gmd-13-4443-2020, 2020
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This paper documents a tool that has been developed that can be used to accelerate the development and understanding of climate models. This version of the model, known as a the single-column model, is much faster to run than the full climate model, and we demonstrate that this tool can be used to quickly exploit model biases that arise due to physical processes. We show examples of how this single-column model can directly benefit the field.
Qi Tang, Stephen A. Klein, Shaocheng Xie, Wuyin Lin, Jean-Christophe Golaz, Erika L. Roesler, Mark A. Taylor, Philip J. Rasch, David C. Bader, Larry K. Berg, Peter Caldwell, Scott E. Giangrande, Richard B. Neale, Yun Qian, Laura D. Riihimaki, Charles S. Zender, Yuying Zhang, and Xue Zheng
Geosci. Model Dev., 12, 2679–2706, https://doi.org/10.5194/gmd-12-2679-2019, https://doi.org/10.5194/gmd-12-2679-2019, 2019
Tao Zhang, Minghua Zhang, Wuyin Lin, Yanluan Lin, Wei Xue, Haiyang Yu, Juanxiong He, Xiaoge Xin, Hsi-Yen Ma, Shaocheng Xie, and Weimin Zheng
Geosci. Model Dev., 11, 5189–5201, https://doi.org/10.5194/gmd-11-5189-2018, https://doi.org/10.5194/gmd-11-5189-2018, 2018
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Tuning of uncertain parameters in global atmospheric general circulation models has extreme computational cost. In this study, we provide an automatic tuning method by combining an auto-optimization algorithm with hindcasts to improve climate simulations in CAM5. The tuning improved the overall performance of a well-calibrated model by about 10 %. The computational cost of the entire auto-tuning procedure is just equivalent to a single 20-year simulation of CAM5.
Samuel R. Hall, Kirk Ullmann, Michael J. Prather, Clare M. Flynn, Lee T. Murray, Arlene M. Fiore, Gustavo Correa, Sarah A. Strode, Stephen D. Steenrod, Jean-Francois Lamarque, Jonathan Guth, Béatrice Josse, Johannes Flemming, Vincent Huijnen, N. Luke Abraham, and Alex T. Archibald
Atmos. Chem. Phys., 18, 16809–16828, https://doi.org/10.5194/acp-18-16809-2018, https://doi.org/10.5194/acp-18-16809-2018, 2018
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Photolysis (J rates) initiates and drives atmospheric chemistry, and Js are perturbed by factors of 2 by clouds. The NASA Atmospheric Tomography (ATom) Mission provides the first comprehensive observations on how clouds perturb Js through the remote Pacific and Atlantic basins. We compare these cloud-perturbation J statistics with those from nine global chemistry models. While basic patterns agree, there is a large spread across models, and all lack some basic features of the observations.
Benjamin Brown-Steiner, Noelle E. Selin, Ronald Prinn, Simone Tilmes, Louisa Emmons, Jean-François Lamarque, and Philip Cameron-Smith
Geosci. Model Dev., 11, 4155–4174, https://doi.org/10.5194/gmd-11-4155-2018, https://doi.org/10.5194/gmd-11-4155-2018, 2018
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We conduct three simulations of atmospheric chemistry using chemical mechanisms of different levels of complexity and compare their results to observations. We explore situations in which the simplified mechanisms match the output of the most complex mechanism, as well as when they diverge. We investigate how concurrent utilization of chemical mechanisms of different complexities can further our atmospheric-chemistry understanding at various scales and give some strategies for future research.
Sarah A. Strode, Junhua Liu, Leslie Lait, Róisín Commane, Bruce Daube, Steven Wofsy, Austin Conaty, Paul Newman, and Michael Prather
Atmos. Chem. Phys., 18, 10955–10971, https://doi.org/10.5194/acp-18-10955-2018, https://doi.org/10.5194/acp-18-10955-2018, 2018
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The GEOS-5 atmospheric model provided forecasts for the Atmospheric Tomography Mission (ATom). GEOS-5 shows skill in simulating the carbon monoxide (CO) measured in ATom-1. African fires contribute to high CO over the tropical Atlantic, but non-fire sources are the main contributors elsewhere. ATom aims to provide a chemical climatology, so we consider whether ATom-1 occurred during a typical summer month. Satellite observations suggest ATom-1 occurred in a clean but not exceptional month.
Kai Zhang, Philip J. Rasch, Mark A. Taylor, Hui Wan, Ruby Leung, Po-Lun Ma, Jean-Christophe Golaz, Jon Wolfe, Wuyin Lin, Balwinder Singh, Susannah Burrows, Jin-Ho Yoon, Hailong Wang, Yun Qian, Qi Tang, Peter Caldwell, and Shaocheng Xie
Geosci. Model Dev., 11, 1971–1988, https://doi.org/10.5194/gmd-11-1971-2018, https://doi.org/10.5194/gmd-11-1971-2018, 2018
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The conservation of total water is an important numerical feature for global Earth system models. Even small conservation problems in the water budget can lead to systematic errors in century-long simulations for sea level rise projection. This study quantifies and reduces various sources of water conservation error in the atmosphere component of the Energy Exascale Earth System Model.
Michael J. Prather, Clare M. Flynn, Xin Zhu, Stephen D. Steenrod, Sarah A. Strode, Arlene M. Fiore, Gustavo Correa, Lee T. Murray, and Jean-Francois Lamarque
Atmos. Meas. Tech., 11, 2653–2668, https://doi.org/10.5194/amt-11-2653-2018, https://doi.org/10.5194/amt-11-2653-2018, 2018
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A new protocol for merging in situ atmospheric chemistry measurements with 3-D models is developed. This technique can identify the most reactive air parcels in terms of tropospheric production/loss of O3 & CH4. This approach highlights differences in 6 global chemistry models even with composition specified. Thus in situ measurements from, e.g., NASA's ATom mission can be used to develop a chemical climatology of, not only the key species, but also the rates of key reactions in each air parcel.
Scott E. Giangrande, Zhe Feng, Michael P. Jensen, Jennifer M. Comstock, Karen L. Johnson, Tami Toto, Meng Wang, Casey Burleyson, Nitin Bharadwaj, Fan Mei, Luiz A. T. Machado, Antonio O. Manzi, Shaocheng Xie, Shuaiqi Tang, Maria Assuncao F. Silva Dias, Rodrigo A. F de Souza, Courtney Schumacher, and Scot T. Martin
Atmos. Chem. Phys., 17, 14519–14541, https://doi.org/10.5194/acp-17-14519-2017, https://doi.org/10.5194/acp-17-14519-2017, 2017
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The Amazon forest is the largest tropical rain forest on the planet, featuring
prolific and diverse cloud conditions. The Observations and Modeling of the Green Ocean Amazon (GoAmazon2014/5) experiment was motivated by demands to gain a better understanding of aerosol and cloud interactions on climate and the global circulation. The routine DOE ARM observations from this 2-year campaign are summarized to help quantify controls on clouds and precipitation over this undersampled region.
Ruth M. Doherty, Clara Orbe, Guang Zeng, David A. Plummer, Michael J. Prather, Oliver Wild, Meiyun Lin, Drew T. Shindell, and Ian A. Mackenzie
Atmos. Chem. Phys., 17, 14219–14237, https://doi.org/10.5194/acp-17-14219-2017, https://doi.org/10.5194/acp-17-14219-2017, 2017
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We investigate how climate change impacts global air pollution transport. To study transport changes, we use a carbon monoxide (CO) tracer species emitted from global sources. We find robust and consistent changes in CO-tracer distributions in climate change simulations performed by four chemistry–climate models in different seasons. We highlight the importance of the co-location of emission source regions and controlling transport processes in determining future pollution transport.
Donald D. Lucas, Matthew Simpson, Philip Cameron-Smith, and Ronald L. Baskett
Atmos. Chem. Phys., 17, 13521–13543, https://doi.org/10.5194/acp-17-13521-2017, https://doi.org/10.5194/acp-17-13521-2017, 2017
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Monte Carlo ensemble simulations, Bayesian inversion, and machine learning are used to quantify uncertainty in the atmospheric transport and emissions of a controlled tracer released from a nuclear power plant. Uncertainty of different settings in a weather model and source terms in a dispersion model are jointly estimated. The algorithm is validated using model-generated output and field observations and can benefit atmospheric researchers who need to estimate tracer transport uncertainty.
Gavin A. Schmidt, David Bader, Leo J. Donner, Gregory S. Elsaesser, Jean-Christophe Golaz, Cecile Hannay, Andrea Molod, Richard B. Neale, and Suranjana Saha
Geosci. Model Dev., 10, 3207–3223, https://doi.org/10.5194/gmd-10-3207-2017, https://doi.org/10.5194/gmd-10-3207-2017, 2017
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The development of coupled ocean atmosphere climate models is a complex process that inevitably includes multiple calibration steps (sometimes called
tuning). Tuning uses degrees of freedom allowed by uncertainties in model approximations to modify parameters to make the simulation better align with some selected observed target(s). We describe how these tuning targets, parameters, and philosophy vary across six US modeling centers in order to increase the transparency of the practice.
Michael J. Prather, Xin Zhu, Clare M. Flynn, Sarah A. Strode, Jose M. Rodriguez, Stephen D. Steenrod, Junhua Liu, Jean-Francois Lamarque, Arlene M. Fiore, Larry W. Horowitz, Jingqiu Mao, Lee T. Murray, Drew T. Shindell, and Steven C. Wofsy
Atmos. Chem. Phys., 17, 9081–9102, https://doi.org/10.5194/acp-17-9081-2017, https://doi.org/10.5194/acp-17-9081-2017, 2017
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We present a new approach for comparing atmospheric chemistry models with measurements based on what these models are used to do, i.e., calculate changes in ozone and methane, prime greenhouse gases. This method anticipates a new type of measurements from the NASA Atmospheric Tomography (ATom) mission. In comparing the mixture of species within air parcels, we focus on those responsible for key chemical changes and weight these parcels by their chemical reactivity.
James Hansen, Makiko Sato, Pushker Kharecha, Karina von Schuckmann, David J. Beerling, Junji Cao, Shaun Marcott, Valerie Masson-Delmotte, Michael J. Prather, Eelco J. Rohling, Jeremy Shakun, Pete Smith, Andrew Lacis, Gary Russell, and Reto Ruedy
Earth Syst. Dynam., 8, 577–616, https://doi.org/10.5194/esd-8-577-2017, https://doi.org/10.5194/esd-8-577-2017, 2017
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Global temperature now exceeds +1.25 °C relative to 1880–1920, similar to warmth of the Eemian period. Keeping warming less than 1.5 °C or CO2 below 350 ppm now requires extraction of CO2 from the air. If rapid phaseout of fossil fuel emissions begins soon, most extraction can be via improved agricultural and forestry practices. In contrast, continued high emissions places a burden on young people of massive technological CO2 extraction with large risks, high costs and uncertain feasibility.
Juno Hsu, Michael J. Prather, Philip Cameron-Smith, Alex Veidenbaum, and Alex Nicolau
Geosci. Model Dev., 10, 2525–2545, https://doi.org/10.5194/gmd-10-2525-2017, https://doi.org/10.5194/gmd-10-2525-2017, 2017
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Solar-J is a high-fidelity solar radiative transfer Fortran 90 code. It has been developed for consistently calculating both the photolysis rates of important chemical species and the heating rates of the atmosphere and the Earth's surface. Its spectral range spans from 177 nm to 12 microns. It can be easily dropped in as a module in global climate–chemistry models.
Gunnar Myhre, Wenche Aas, Ribu Cherian, William Collins, Greg Faluvegi, Mark Flanner, Piers Forster, Øivind Hodnebrog, Zbigniew Klimont, Marianne T. Lund, Johannes Mülmenstädt, Cathrine Lund Myhre, Dirk Olivié, Michael Prather, Johannes Quaas, Bjørn H. Samset, Jordan L. Schnell, Michael Schulz, Drew Shindell, Ragnhild B. Skeie, Toshihiko Takemura, and Svetlana Tsyro
Atmos. Chem. Phys., 17, 2709–2720, https://doi.org/10.5194/acp-17-2709-2017, https://doi.org/10.5194/acp-17-2709-2017, 2017
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Over the past decades, the geographical distribution of emissions of substances that alter the atmospheric energy balance has changed due to economic growth and pollution regulations. Here, we show the resulting changes to aerosol and ozone abundances and their radiative forcing using recently updated emission data for the period 1990–2015, as simulated by seven global atmospheric composition models. The global mean radiative forcing is more strongly positive than reported in IPCC AR5.
William J. Collins, Jean-François Lamarque, Michael Schulz, Olivier Boucher, Veronika Eyring, Michaela I. Hegglin, Amanda Maycock, Gunnar Myhre, Michael Prather, Drew Shindell, and Steven J. Smith
Geosci. Model Dev., 10, 585–607, https://doi.org/10.5194/gmd-10-585-2017, https://doi.org/10.5194/gmd-10-585-2017, 2017
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We have designed a set of climate model experiments called the Aerosol Chemistry Model Intercomparison Project (AerChemMIP). These are designed to quantify the climate and air quality impacts of aerosols and chemically reactive gases in the climate models that are used to simulate past and future climate. We hope that many climate modelling centres will choose to run these experiments to help understand the contribution of aerosols and chemistry to climate change.
Bojan Sič, Laaziz El Amraoui, Andrea Piacentini, Virginie Marécal, Emanuele Emili, Daniel Cariolle, Michael Prather, and Jean-Luc Attié
Atmos. Meas. Tech., 9, 5535–5554, https://doi.org/10.5194/amt-9-5535-2016, https://doi.org/10.5194/amt-9-5535-2016, 2016
Shuaiqi Tang, Shaocheng Xie, Yunyan Zhang, Minghua Zhang, Courtney Schumacher, Hannah Upton, Michael P. Jensen, Karen L. Johnson, Meng Wang, Maike Ahlgrimm, Zhe Feng, Patrick Minnis, and Mandana Thieman
Atmos. Chem. Phys., 16, 14249–14264, https://doi.org/10.5194/acp-16-14249-2016, https://doi.org/10.5194/acp-16-14249-2016, 2016
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Data observed during the Green Ocean Amazon (GoAmazon2014/5) experiment are used to derive the large-scale fields in this study. The morning propagating convective systems are active during the wet season but rare during the dry season. The afternoon convections are active in both seasons, with heating and moistening in the lower level corresponding to the vertical convergence of eddy fluxes. Case study shows distinguish large-scale environments for three types of convective systems in Amazonia.
Raquel A. Silva, J. Jason West, Jean-François Lamarque, Drew T. Shindell, William J. Collins, Stig Dalsoren, Greg Faluvegi, Gerd Folberth, Larry W. Horowitz, Tatsuya Nagashima, Vaishali Naik, Steven T. Rumbold, Kengo Sudo, Toshihiko Takemura, Daniel Bergmann, Philip Cameron-Smith, Irene Cionni, Ruth M. Doherty, Veronika Eyring, Beatrice Josse, Ian A. MacKenzie, David Plummer, Mattia Righi, David S. Stevenson, Sarah Strode, Sophie Szopa, and Guang Zengast
Atmos. Chem. Phys., 16, 9847–9862, https://doi.org/10.5194/acp-16-9847-2016, https://doi.org/10.5194/acp-16-9847-2016, 2016
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Using ozone and PM2.5 concentrations from the ACCMIP ensemble of chemistry-climate models for the four Representative Concentration Pathway scenarios (RCPs), together with projections of future population and baseline mortality rates, we quantify the human premature mortality impacts of future ambient air pollution in 2030, 2050 and 2100, relative to 2000 concentrations. We also estimate the global mortality burden of ozone and PM2.5 in 2000 and each future period.
D. M. Westervelt, L. W. Horowitz, V. Naik, J.-C. Golaz, and D. L. Mauzerall
Atmos. Chem. Phys., 15, 12681–12703, https://doi.org/10.5194/acp-15-12681-2015, https://doi.org/10.5194/acp-15-12681-2015, 2015
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Decreases in aerosols over the 21st century as projected by the Representative Concentration Pathways (RCPs) lead to increases up to 0.5 - 1 ºC in global temperature and up to 0.05 - 0.1 mm/day in global precipitation, depending strongly on present-day aerosol radiative forcing. In East Asia, future aerosol decreases could be responsible for 10-20% of the total temperature increase (30-40% with strong present-day aerosol forcing), even under the high greenhouse gas emissions scenario (RCP8.5).
J. L. Schnell, M. J. Prather, B. Josse, V. Naik, L. W. Horowitz, P. Cameron-Smith, D. Bergmann, G. Zeng, D. A. Plummer, K. Sudo, T. Nagashima, D. T. Shindell, G. Faluvegi, and S. A. Strode
Atmos. Chem. Phys., 15, 10581–10596, https://doi.org/10.5194/acp-15-10581-2015, https://doi.org/10.5194/acp-15-10581-2015, 2015
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We test global chemistry--climate models in their ability to simulate present-day surface ozone. Models are tested against observed hourly ozone from 4217 stations in North America and Europe that are averaged over 1°x1° grid cells. Using novel metrics, we find most models match the shape but not the amplitude of regional summertime diurnal and annual cycles and match the pattern but not the magnitude of summer ozone enhancement. Most also match the observed distribution of extreme episode sizes
M. J. Prather
Geosci. Model Dev., 8, 2587–2595, https://doi.org/10.5194/gmd-8-2587-2015, https://doi.org/10.5194/gmd-8-2587-2015, 2015
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A new approach for modeling photolysis rates (J values) in atmospheres with fractional cloud cover has been developed and is implemented as Cloud-J – a multi-scattering eight-stream radiative transfer model for solar radiation based on Fast-J. Using observations of the vertical correlation of cloud layers, Cloud-J provides a practical and accurate method for modeling atmospheric chemistry, which can be extended to solar heating rates.
D. D. Lucas, C. Yver Kwok, P. Cameron-Smith, H. Graven, D. Bergmann, T. P. Guilderson, R. Weiss, and R. Keeling
Geosci. Instrum. Method. Data Syst., 4, 121–137, https://doi.org/10.5194/gi-4-121-2015, https://doi.org/10.5194/gi-4-121-2015, 2015
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Multiobjective optimization is used to design Pareto optimal greenhouse gas (GHG) observing networks. A prototype GHG network is designed to optimize scientific performance and measurement costs. The Pareto frontier is convex, showing the trade-offs between performance and cost and the diminishing returns in trading one for the other. Other objectives and constraints that are important in the design of practical GHG monitoring networks can be incorporated into our method.
P. Hess, D. Kinnison, and Q. Tang
Atmos. Chem. Phys., 15, 2341–2365, https://doi.org/10.5194/acp-15-2341-2015, https://doi.org/10.5194/acp-15-2341-2015, 2015
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Using a series of model simulations, we find that at widespread NH extratropical locations, interannual tropospheric ozone variability is largely determined by the transport of ozone from the stratosphere. This has implications in the interpretation of measured tropospheric ozone variability in light of changes in the emissions of ozone precursors and in the response of tropospheric ozone to climate change.
M. P. Jensen, T. Toto, D. Troyan, P. E. Ciesielski, D. Holdridge, J. Kyrouac, J. Schatz, Y. Zhang, and S. Xie
Atmos. Meas. Tech., 8, 421–434, https://doi.org/10.5194/amt-8-421-2015, https://doi.org/10.5194/amt-8-421-2015, 2015
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A major component of the 2011 Midlatitude Continental Convective Clouds Experiment (MC3E) was a six-site radiosonde array designed to capture the large-scale variability of the atmospheric state. This manuscript describes the details of the MC3E radiosonde operations including the instrumentation, data processing and analysis of the impacts of bias correction and algorithm assumptions on the determination of forcing data sets.
J. L. Schnell, C. D. Holmes, A. Jangam, and M. J. Prather
Atmos. Chem. Phys., 14, 7721–7739, https://doi.org/10.5194/acp-14-7721-2014, https://doi.org/10.5194/acp-14-7721-2014, 2014
C. D. Holmes, M. J. Prather, and G. C. M. Vinken
Atmos. Chem. Phys., 14, 6801–6812, https://doi.org/10.5194/acp-14-6801-2014, https://doi.org/10.5194/acp-14-6801-2014, 2014
P. H. Lauritzen, P. A. Ullrich, C. Jablonowski, P. A. Bosler, D. Calhoun, A. J. Conley, T. Enomoto, L. Dong, S. Dubey, O. Guba, A. B. Hansen, E. Kaas, J. Kent, J.-F. Lamarque, M. J. Prather, D. Reinert, V. V. Shashkin, W. C. Skamarock, B. Sørensen, M. A. Taylor, and M. A. Tolstykh
Geosci. Model Dev., 7, 105–145, https://doi.org/10.5194/gmd-7-105-2014, https://doi.org/10.5194/gmd-7-105-2014, 2014
R. Locatelli, P. Bousquet, F. Chevallier, A. Fortems-Cheney, S. Szopa, M. Saunois, A. Agusti-Panareda, D. Bergmann, H. Bian, P. Cameron-Smith, M. P. Chipperfield, E. Gloor, S. Houweling, S. R. Kawa, M. Krol, P. K. Patra, R. G. Prinn, M. Rigby, R. Saito, and C. Wilson
Atmos. Chem. Phys., 13, 9917–9937, https://doi.org/10.5194/acp-13-9917-2013, https://doi.org/10.5194/acp-13-9917-2013, 2013
J.-F. Lamarque, F. Dentener, J. McConnell, C.-U. Ro, M. Shaw, R. Vet, D. Bergmann, P. Cameron-Smith, S. Dalsoren, R. Doherty, G. Faluvegi, S. J. Ghan, B. Josse, Y. H. Lee, I. A. MacKenzie, D. Plummer, D. T. Shindell, R. B. Skeie, D. S. Stevenson, S. Strode, G. Zeng, M. Curran, D. Dahl-Jensen, S. Das, D. Fritzsche, and M. Nolan
Atmos. Chem. Phys., 13, 7997–8018, https://doi.org/10.5194/acp-13-7997-2013, https://doi.org/10.5194/acp-13-7997-2013, 2013
V. Naik, A. Voulgarakis, A. M. Fiore, L. W. Horowitz, J.-F. Lamarque, M. Lin, M. J. Prather, P. J. Young, D. Bergmann, P. J. Cameron-Smith, I. Cionni, W. J. Collins, S. B. Dalsøren, R. Doherty, V. Eyring, G. Faluvegi, G. A. Folberth, B. Josse, Y. H. Lee, I. A. MacKenzie, T. Nagashima, T. P. C. van Noije, D. A. Plummer, M. Righi, S. T. Rumbold, R. Skeie, D. T. Shindell, D. S. Stevenson, S. Strode, K. Sudo, S. Szopa, and G. Zeng
Atmos. Chem. Phys., 13, 5277–5298, https://doi.org/10.5194/acp-13-5277-2013, https://doi.org/10.5194/acp-13-5277-2013, 2013
A. Voulgarakis, V. Naik, J.-F. Lamarque, D. T. Shindell, P. J. Young, M. J. Prather, O. Wild, R. D. Field, D. Bergmann, P. Cameron-Smith, I. Cionni, W. J. Collins, S. B. Dalsøren, R. M. Doherty, V. Eyring, G. Faluvegi, G. A. Folberth, L. W. Horowitz, B. Josse, I. A. MacKenzie, T. Nagashima, D. A. Plummer, M. Righi, S. T. Rumbold, D. S. Stevenson, S. A. Strode, K. Sudo, S. Szopa, and G. Zeng
Atmos. Chem. Phys., 13, 2563–2587, https://doi.org/10.5194/acp-13-2563-2013, https://doi.org/10.5194/acp-13-2563-2013, 2013
J.-F. Lamarque, D. T. Shindell, B. Josse, P. J. Young, I. Cionni, V. Eyring, D. Bergmann, P. Cameron-Smith, W. J. Collins, R. Doherty, S. Dalsoren, G. Faluvegi, G. Folberth, S. J. Ghan, L. W. Horowitz, Y. H. Lee, I. A. MacKenzie, T. Nagashima, V. Naik, D. Plummer, M. Righi, S. T. Rumbold, M. Schulz, R. B. Skeie, D. S. Stevenson, S. Strode, K. Sudo, S. Szopa, A. Voulgarakis, and G. Zeng
Geosci. Model Dev., 6, 179–206, https://doi.org/10.5194/gmd-6-179-2013, https://doi.org/10.5194/gmd-6-179-2013, 2013
D. A. Belikov, S. Maksyutov, M. Krol, A. Fraser, M. Rigby, H. Bian, A. Agusti-Panareda, D. Bergmann, P. Bousquet, P. Cameron-Smith, M. P. Chipperfield, A. Fortems-Cheiney, E. Gloor, K. Haynes, P. Hess, S. Houweling, S. R. Kawa, R. M. Law, Z. Loh, L. Meng, P. I. Palmer, P. K. Patra, R. G. Prinn, R. Saito, and C. Wilson
Atmos. Chem. Phys., 13, 1093–1114, https://doi.org/10.5194/acp-13-1093-2013, https://doi.org/10.5194/acp-13-1093-2013, 2013
C. D. Holmes, M. J. Prather, O. A. Søvde, and G. Myhre
Atmos. Chem. Phys., 13, 285–302, https://doi.org/10.5194/acp-13-285-2013, https://doi.org/10.5194/acp-13-285-2013, 2013
Ø. Hodnebrog, T. K. Berntsen, O. Dessens, M. Gauss, V. Grewe, I. S. A. Isaksen, B. Koffi, G. Myhre, D. Olivié, M. J. Prather, F. Stordal, S. Szopa, Q. Tang, P. van Velthoven, and J. E. Williams
Atmos. Chem. Phys., 12, 12211–12225, https://doi.org/10.5194/acp-12-12211-2012, https://doi.org/10.5194/acp-12-12211-2012, 2012
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Observational operator for fair model evaluation with ground NO2 measurements
Valid time shifting ensemble Kalman filter (VTS-EnKF) for dust storm forecasting
Development of the CMA-GFS-AERO 4D-Var assimilation system v1.0 – Part 1: System description
The third Met Office Unified Model-JULES Regional Atmosphere and Land Configuration, RAL3
Tyler P. Janoski, Ivan Mitevski, Ryan J. Kramer, Michael Previdi, and Lorenzo M. Polvani
Geosci. Model Dev., 18, 3065–3079, https://doi.org/10.5194/gmd-18-3065-2025, https://doi.org/10.5194/gmd-18-3065-2025, 2025
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We developed ClimKern, a Python package and radiative kernel repository, to simplify calculating radiative feedbacks and make climate sensitivity studies more reproducible. Testing of ClimKern with sample climate model data reveals that radiative kernel choice may be more important than previously thought, especially in polar regions. Our work highlights the need for kernel sensitivity analyses to be included in future studies.
Matti Niskanen, Aku Seppänen, Henri Oikarinen, Miska Olin, Panu Karjalainen, Santtu Mikkonen, and Kari Lehtinen
Geosci. Model Dev., 18, 2983–3001, https://doi.org/10.5194/gmd-18-2983-2025, https://doi.org/10.5194/gmd-18-2983-2025, 2025
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Particle size is a key factor determining the properties of aerosol particles which have a major influence on the climate and on human health. When measuring the particle sizes, however, sometimes the sampling lines that transfer the aerosol to the measurement device distort the size distribution, making the measurement unreliable. We propose a method to correct for the distortions and estimate the true particle sizes, improving measurement accuracy.
Johann Rasmus Nüß, Nikos Daskalakis, Fabian Günther Piwowarczyk, Angelos Gkouvousis, Oliver Schneising, Michael Buchwitz, Maria Kanakidou, Maarten C. Krol, and Mihalis Vrekoussis
Geosci. Model Dev., 18, 2861–2890, https://doi.org/10.5194/gmd-18-2861-2025, https://doi.org/10.5194/gmd-18-2861-2025, 2025
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We estimate carbon monoxide emissions through inverse modeling, an approach where measurements of tracers in the atmosphere are fed to a model to calculate backwards in time (inverse) where the tracers came from. We introduce measurements from a new satellite instrument and show that, in most places globally, these on their own sufficiently constrain the emissions. This alleviates the need for additional datasets, which could shorten the delay for future carbon monoxide source estimates.
Ashu Dastoor, Hélène Angot, Johannes Bieser, Flora Brocza, Brock Edwards, Aryeh Feinberg, Xinbin Feng, Benjamin Geyman, Charikleia Gournia, Yipeng He, Ian M. Hedgecock, Ilia Ilyin, Jane Kirk, Che-Jen Lin, Igor Lehnherr, Robert Mason, David McLagan, Marilena Muntean, Peter Rafaj, Eric M. Roy, Andrei Ryjkov, Noelle E. Selin, Francesco De Simone, Anne L. Soerensen, Frits Steenhuisen, Oleg Travnikov, Shuxiao Wang, Xun Wang, Simon Wilson, Rosa Wu, Qingru Wu, Yanxu Zhang, Jun Zhou, Wei Zhu, and Scott Zolkos
Geosci. Model Dev., 18, 2747–2860, https://doi.org/10.5194/gmd-18-2747-2025, https://doi.org/10.5194/gmd-18-2747-2025, 2025
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This paper introduces the Multi-Compartment Mercury (Hg) Modeling and Analysis Project (MCHgMAP) aimed at informing the effectiveness evaluations of two multilateral environmental agreements: the Minamata Convention on Mercury and the Convention on Long-Range Transboundary Air Pollution. The experimental design exploits a variety of models (atmospheric, land, oceanic ,and multimedia mass balance models) to assess the short- and long-term influences of anthropogenic Hg releases into the environment.
Hilda Sandström and Patrick Rinke
Geosci. Model Dev., 18, 2701–2724, https://doi.org/10.5194/gmd-18-2701-2025, https://doi.org/10.5194/gmd-18-2701-2025, 2025
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Machine learning has the potential to aid the identification of organic molecules involved in aerosol formation. Yet, progress is stalled by a lack of curated atmospheric molecular datasets. Here, we compared atmospheric compounds with large molecular datasets used in machine learning and found minimal overlap with similarity algorithms. Our result underlines the need for collaborative efforts to curate atmospheric molecular data to facilitate machine learning models in atmospheric sciences.
Juan Escobar, Philippe Wautelet, Joris Pianezze, Florian Pantillon, Thibaut Dauhut, Christelle Barthe, and Jean-Pierre Chaboureau
Geosci. Model Dev., 18, 2679–2700, https://doi.org/10.5194/gmd-18-2679-2025, https://doi.org/10.5194/gmd-18-2679-2025, 2025
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The Meso-NH weather research code is adapted for GPUs using OpenACC, leading to significant performance and energy efficiency improvements. Called MESONH-v55-OpenACC, it includes enhanced memory management, communication optimizations and a new solver. On the AMD MI250X Adastra platform, it achieved up to 6× speedup and 2.3× energy efficiency gain compared to CPUs. Storm simulations at 100 m resolution show positive results, positioning the code for future use on exascale supercomputers.
Jie Gao, Yi Huang, Jonathon S. Wright, Ke Li, Tao Geng, and Qiurun Yu
Geosci. Model Dev., 18, 2569–2586, https://doi.org/10.5194/gmd-18-2569-2025, https://doi.org/10.5194/gmd-18-2569-2025, 2025
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The aerosol in the upper troposphere and stratosphere is highly variable, and its radiative effect is poorly understood. To estimate this effect, the radiative kernel is constructed and applied. The results show that the kernels can reproduce aerosol radiative effects and are expected to simulate stratospheric aerosol radiative effects. This approach reduces computational expense, is consistent with radiative model calculations, and can be applied to atmospheric models with speed requirements.
Ji Won Yoon, Seungyeon Lee, Ebony Lee, and Seon Ki Park
Geosci. Model Dev., 18, 2303–2328, https://doi.org/10.5194/gmd-18-2303-2025, https://doi.org/10.5194/gmd-18-2303-2025, 2025
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This study evaluates the Weather Research and Forecasting Model (WRF) coupled with Chemistry (WRF-Chem) to predict a mega Asian dust storm (ADS) over South Korea on 28–29 March 2021. We assessed combinations of five dust emission and four land surface schemes by analyzing meteorological and air quality variables. The best scheme combination reduced the root mean square error (RMSE) for particulate matter 10 (PM10) by up to 29.6 %, demonstrating the highest performance.
Jianyu Lin, Tie Dai, Lifang Sheng, Weihang Zhang, Shangfei Hai, and Yawen Kong
Geosci. Model Dev., 18, 2231–2248, https://doi.org/10.5194/gmd-18-2231-2025, https://doi.org/10.5194/gmd-18-2231-2025, 2025
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The effectiveness of this assimilation system and its sensitivity to the ensemble member size and length of the assimilation window are investigated. This study advances our understanding of the selection of basic parameters in the four-dimensional local ensemble transform Kalman filter assimilation system and the performance of ensemble simulation in a particulate-matter-polluted environment.
Jens Peter Karolus Wenceslaus Frankemölle, Johan Camps, Pieter De Meutter, and Johan Meyers
Geosci. Model Dev., 18, 1989–2003, https://doi.org/10.5194/gmd-18-1989-2025, https://doi.org/10.5194/gmd-18-1989-2025, 2025
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To detect anomalous radioactivity in the environment, it is paramount that we understand the natural background level. In this work, we propose a statistical model to describe the most likely background level and the associated uncertainty in a network of dose rate detectors. We train, verify, and validate the model using real environmental data. Using the model, we show that we can correctly predict the background level in a subset of the detector network during a known
anomalous event.
Jean-François Grailet, Robin J. Hogan, Nicolas Ghilain, David Bolsée, Xavier Fettweis, and Marilaure Grégoire
Geosci. Model Dev., 18, 1965–1988, https://doi.org/10.5194/gmd-18-1965-2025, https://doi.org/10.5194/gmd-18-1965-2025, 2025
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The MAR (Modèle Régional Atmosphérique) is a regional climate model used for weather forecasting and studying the climate over various regions. This paper presents an update of MAR thanks to which it can precisely decompose solar radiation, in particular in the UV (ultraviolet) and photosynthesis ranges, both being critical to human health and ecosystems. As a first application of this new capability, this paper presents a method for predicting UV indices with MAR.
Yi-Ning Shi, Jun Yang, Wei Han, Lujie Han, Jiajia Mao, Wanlin Kan, and Fuzhong Weng
Geosci. Model Dev., 18, 1947–1964, https://doi.org/10.5194/gmd-18-1947-2025, https://doi.org/10.5194/gmd-18-1947-2025, 2025
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Direct assimilation of observations from ground-based microwave radiometers (GMRs) holds significant potential for improving forecast accuracy. Radiative transfer models (RTMs) play a crucial role in direct data assimilation. In this study, we introduce a new RTM, the Advanced Radiative Transfer Modeling System – Ground-Based (ARMS-gb), designed to simulate brightness temperatures observed by GMRs along with their Jacobians. Several enhancements have been incorporated to achieve higher accuracy.
R. Phani Murali Krishna, Siddharth Kumar, A. Gopinathan Prajeesh, Peter Bechtold, Nils Wedi, Kumar Roy, Malay Ganai, B. Revanth Reddy, Snehlata Tirkey, Tanmoy Goswami, Radhika Kanase, Sahadat Sarkar, Medha Deshpande, and Parthasarathi Mukhopadhyay
Geosci. Model Dev., 18, 1879–1894, https://doi.org/10.5194/gmd-18-1879-2025, https://doi.org/10.5194/gmd-18-1879-2025, 2025
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The High-Resolution Global Forecast Model (HGFM) is an advanced iteration of the operational Global Forecast System (GFS) model. HGFM can produce forecasts at a spatial scale of ~6 km in tropics. It demonstrates improved accuracy in short- to medium-range weather prediction over the Indian region, with notable success in predicting extreme events. Further, the model will be entrusted to operational forecasting agencies after validation and testing.
Jenna Ritvanen, Seppo Pulkkinen, Dmitri Moisseev, and Daniele Nerini
Geosci. Model Dev., 18, 1851–1878, https://doi.org/10.5194/gmd-18-1851-2025, https://doi.org/10.5194/gmd-18-1851-2025, 2025
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Nowcasting models struggle with the rapid evolution of heavy rain, and common verification methods are unable to describe how accurately the models predict the growth and decay of heavy rain. We propose a framework to assess model performance. In the framework, convective cells are identified and tracked in the forecasts and observations, and the model skill is then evaluated by comparing differences between forecast and observed cells. We demonstrate the framework with four open-source models.
Andrew Geiss and Po-Lun Ma
Geosci. Model Dev., 18, 1809–1827, https://doi.org/10.5194/gmd-18-1809-2025, https://doi.org/10.5194/gmd-18-1809-2025, 2025
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Particles in the Earth's atmosphere strongly impact the planet's energy budget, and atmosphere simulations require accurate representation of their interaction with light. This work introduces two approaches to represent light scattering by small particles. The first is a scattering simulator based on Mie theory implemented in Python. The second is a neural network emulator that is more accurate than existing methods and is fast enough to be used in climate and weather simulations.
Qin Wang, Bo Zeng, Gong Chen, and Yaoting Li
Geosci. Model Dev., 18, 1769–1784, https://doi.org/10.5194/gmd-18-1769-2025, https://doi.org/10.5194/gmd-18-1769-2025, 2025
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This study evaluates the performance of four planetary boundary layer (PBL) schemes in near-surface wind fields over the Sichuan Basin, China. Using 112 sensitivity experiments with the Weather Research and Forecasting (WRF) model and focusing on 28 wind events, it is found that wind direction was less sensitive to the PBL schemes. The quasi-normal scale elimination (QNSE) scheme captured temporal variations best, while the Mellor–Yamada–Janjić (MYJ) scheme had the least error in wind speed.
Tai-Long He, Nikhil Dadheech, Tammy M. Thompson, and Alexander J. Turner
Geosci. Model Dev., 18, 1661–1671, https://doi.org/10.5194/gmd-18-1661-2025, https://doi.org/10.5194/gmd-18-1661-2025, 2025
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It is computationally expensive to infer greenhouse gas (GHG) emissions using atmospheric observations. This is partly due to the detailed model used to represent atmospheric transport. We demonstrate how a machine learning (ML) model can be used to simulate high-resolution atmospheric transport. This type of ML model will help estimate GHG emissions using dense observations, which are becoming increasingly common with the proliferation of urban monitoring networks and geostationary satellites.
Wei Li, Beiming Tang, Patrick C. Campbell, Youhua Tang, Barry Baker, Zachary Moon, Daniel Tong, Jianping Huang, Kai Wang, Ivanka Stajner, and Raffaele Montuoro
Geosci. Model Dev., 18, 1635–1660, https://doi.org/10.5194/gmd-18-1635-2025, https://doi.org/10.5194/gmd-18-1635-2025, 2025
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The study describes the updates of NOAA's current UFS-AQMv7 air quality forecast model by incorporating the latest scientific and structural changes in CMAQv5.4. An evaluation during the summer of 2023 shows that the updated model overall improves the simulation of MDA8 O3 by reducing the bias by 8%–12% in the contiguous US. PM2.5 predictions have mixed results due to wildfire, highlighting the need for future refinements.
Yanwei Zhu, Aitor Atencia, Markus Dabernig, and Yong Wang
Geosci. Model Dev., 18, 1545–1559, https://doi.org/10.5194/gmd-18-1545-2025, https://doi.org/10.5194/gmd-18-1545-2025, 2025
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Most works have delved into convective weather nowcasting, and only a few works have discussed the nowcasting uncertainty for variables at the surface level. Hence, we proposed a method to estimate uncertainty. Generating appropriate noises associated with the characteristic of the error in analysis can simulate the uncertainty of nowcasting. This method can contribute to the estimation of near–surface analysis uncertainty in both nowcasting applications and ensemble nowcasting development.
Joël Thanwerdas, Antoine Berchet, Lionel Constantin, Aki Tsuruta, Michael Steiner, Friedemann Reum, Stephan Henne, and Dominik Brunner
Geosci. Model Dev., 18, 1505–1544, https://doi.org/10.5194/gmd-18-1505-2025, https://doi.org/10.5194/gmd-18-1505-2025, 2025
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The Community Inversion Framework (CIF) brings together methods for estimating greenhouse gas fluxes from atmospheric observations. The initial ensemble method implemented in CIF was found to be incomplete and could hardly be compared to other ensemble methods employed in the inversion community. In this paper, we present and evaluate a new implementation of the ensemble mode, building upon the initial developments.
Astrid Kerkweg, Timo Kirfel, Duong H. Do, Sabine Griessbach, Patrick Jöckel, and Domenico Taraborrelli
Geosci. Model Dev., 18, 1265–1286, https://doi.org/10.5194/gmd-18-1265-2025, https://doi.org/10.5194/gmd-18-1265-2025, 2025
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Normally, the Modular Earth Submodel System (MESSy) is linked to complete dynamic models to create chemical climate models. However, the modular concept of MESSy and the newly developed DWARF component presented here make it possible to create simplified models that contain only one or a few process descriptions. This is very useful for technical optimisation, such as porting to GPUs, and can be used to create less complex models, such as a chemical box model.
Edward C. Chan, Ilona J. Jäkel, Basit Khan, Martijn Schaap, Timothy M. Butler, Renate Forkel, and Sabine Banzhaf
Geosci. Model Dev., 18, 1119–1139, https://doi.org/10.5194/gmd-18-1119-2025, https://doi.org/10.5194/gmd-18-1119-2025, 2025
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An enhanced emission module has been developed for the PALM model system, improving flexibility and scalability of emission source representation across different sectors. A model for parametrized domestic emissions has also been included, for which an idealized model run is conducted for particulate matter (PM10). The results show that, in addition to individual sources and diurnal variations in energy consumption, vertical transport and urban topology play a role in concentration distribution.
Gregor Ehrensperger, Thorsten Simon, Georg J. Mayr, and Tobias Hell
Geosci. Model Dev., 18, 1141–1153, https://doi.org/10.5194/gmd-18-1141-2025, https://doi.org/10.5194/gmd-18-1141-2025, 2025
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As lightning is a brief and localized event, it is not explicitly resolved in atmospheric models. Instead, expert-based auxiliary descriptions are used to assess it. This study explores how AI can improve our understanding of lightning without relying on traditional expert knowledge. We reveal that AI independently identified the key factors known to experts as essential for lightning in the Alps region. This shows how knowledge discovery could be sped up in areas with limited expert knowledge.
David Patoulias, Kalliopi Florou, and Spyros N. Pandis
Geosci. Model Dev., 18, 1103–1118, https://doi.org/10.5194/gmd-18-1103-2025, https://doi.org/10.5194/gmd-18-1103-2025, 2025
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The effect of the assumed atmospheric nucleation mechanism on particle number concentrations and size distribution was investigated. Two quite different mechanisms involving sulfuric acid and ammonia or a biogenic organic vapor gave quite similar results which were consistent with measurements at 26 measurement stations across Europe. The number of larger particles that serve as cloud condensation nuclei showed little sensitivity to the assumed nucleation mechanism.
Tim Radke, Susanne Fuchs, Christian Wilms, Iuliia Polkova, and Marc Rautenhaus
Geosci. Model Dev., 18, 1017–1039, https://doi.org/10.5194/gmd-18-1017-2025, https://doi.org/10.5194/gmd-18-1017-2025, 2025
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In our study, we built upon previous work to investigate the patterns artificial intelligence (AI) learns to detect atmospheric features like tropical cyclones (TCs) and atmospheric rivers (ARs). As primary objective, we adopt a method to explain the AI used and investigate the plausibility of learned patterns. We find that plausible patterns are learned for both TCs and ARs. Hence, the chosen method is very useful for gaining confidence in the AI-based detection of atmospheric features.
Stefan Noll, Carsten Schmidt, Patrick Hannawald, Wolfgang Kausch, and Stefan Kimeswenger
EGUsphere, https://doi.org/10.5194/egusphere-2024-3512, https://doi.org/10.5194/egusphere-2024-3512, 2025
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Non-thermal emission from chemical reactions in the Earth's middle und upper atmosphere strongly contributes to the brightness of the night sky below about 2.3 µm. The new Paranal Airglow Line and Continuum Emission model calculates the emission spectrum and its variability with an unprecedented accuracy. Relying on a large spectroscopic data set from astronomical spectrographs and theoretical molecular/atomic data, it is valuable for airglow research and astronomical observatories.
Felipe Cifuentes, Henk Eskes, Enrico Dammers, Charlotte Bryan, and Folkert Boersma
Geosci. Model Dev., 18, 621–649, https://doi.org/10.5194/gmd-18-621-2025, https://doi.org/10.5194/gmd-18-621-2025, 2025
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We tested the capability of the flux divergence approach (FDA) to reproduce known NOx emissions using synthetic NO2 satellite column retrievals from high-resolution model simulations. The FDA accurately reproduced NOx emissions when column observations were limited to the boundary layer and when the variability of the NO2 lifetime, the NOx : NO2 ratio, and NO2 profile shapes were correctly modeled. This introduces strong model dependency, reducing the simplicity of the original FDA formulation.
Stefano Ubbiali, Christian Kühnlein, Christoph Schär, Linda Schlemmer, Thomas C. Schulthess, Michael Staneker, and Heini Wernli
Geosci. Model Dev., 18, 529–546, https://doi.org/10.5194/gmd-18-529-2025, https://doi.org/10.5194/gmd-18-529-2025, 2025
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We explore a high-level programming model for porting numerical weather prediction (NWP) model codes to graphics processing units (GPUs). We present a Python rewrite with the domain-specific library GT4Py (GridTools for Python) of two renowned cloud microphysics schemes and the associated tangent-linear and adjoint algorithms. We find excellent portability, competitive GPU performance, robust execution on diverse computing architectures, and enhanced code maintainability and user productivity.
Pieter Rijsdijk, Henk Eskes, Arlene Dingemans, K. Folkert Boersma, Takashi Sekiya, Kazuyuki Miyazaki, and Sander Houweling
Geosci. Model Dev., 18, 483–509, https://doi.org/10.5194/gmd-18-483-2025, https://doi.org/10.5194/gmd-18-483-2025, 2025
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Clustering high-resolution satellite observations into superobservations improves model validation and data assimilation applications. In our paper, we derive quantitative uncertainties for satellite NO2 column observations based on knowledge of the retrievals, including a detailed analysis of spatial error correlations and representativity errors. The superobservations and uncertainty estimates are tested in a global chemical data assimilation system and are found to improve the forecasts.
Dario Di Santo, Cenlin He, Fei Chen, and Lorenzo Giovannini
Geosci. Model Dev., 18, 433–459, https://doi.org/10.5194/gmd-18-433-2025, https://doi.org/10.5194/gmd-18-433-2025, 2025
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This paper presents the Machine Learning-based Automated Multi-method Parameter Sensitivity and Importance analysis Tool (ML-AMPSIT), a computationally efficient tool that uses machine learning algorithms for sensitivity analysis in atmospheric models. It is tested with the Weather Research and Forecasting (WRF) model coupled with the Noah-Multiparameterization (Noah-MP) land surface model to investigate sea breeze circulation sensitivity to vegetation-related parameters.
Robert Schoetter, Robin James Hogan, Cyril Caliot, and Valéry Masson
Geosci. Model Dev., 18, 405–431, https://doi.org/10.5194/gmd-18-405-2025, https://doi.org/10.5194/gmd-18-405-2025, 2025
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Radiation is relevant to the atmospheric impact on people and infrastructure in cities as it can influence the urban heat island, building energy consumption, and human thermal comfort. A new urban radiation model, assuming a more realistic form of urban morphology, is coupled to the urban climate model Town Energy Balance (TEB). The new TEB is evaluated with a reference radiation model for a variety of urban morphologies, and an improvement in the simulated radiative observables is found.
Zebediah Engberg, Roger Teoh, Tristan Abbott, Thomas Dean, Marc E. J. Stettler, and Marc L. Shapiro
Geosci. Model Dev., 18, 253–286, https://doi.org/10.5194/gmd-18-253-2025, https://doi.org/10.5194/gmd-18-253-2025, 2025
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Contrails forming in some atmospheric conditions may persist and become strongly warming cirrus, while in other conditions may be neutral or cooling. We develop a contrail forecast model to predict contrail climate forcing for any arbitrary point in space and time and explore integration into flight planning and air traffic management. This approach enables contrail interventions to target high-probability high-climate-impact regions and reduce unintended consequences of contrail management.
Nils Eingrüber, Alina Domm, Wolfgang Korres, and Karl Schneider
Geosci. Model Dev., 18, 141–160, https://doi.org/10.5194/gmd-18-141-2025, https://doi.org/10.5194/gmd-18-141-2025, 2025
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Climate change adaptation measures like unsealings can reduce urban heat stress. As grass grid pavers have never been parameterized for microclimate model simulations with ENVI-met, a new parameterization was developed based on field measurements. To analyse the cooling potential, scenario analyses were performed for a densely developed area in Cologne. Statistically significant average cooling effects of up to −11.1 K were found for surface temperature and up to −2.9 K for 1 m air temperature.
Xuan Wang, Lei Bi, Hong Wang, Yaqiang Wang, Wei Han, Xueshun Shen, and Xiaoye Zhang
Geosci. Model Dev., 18, 117–139, https://doi.org/10.5194/gmd-18-117-2025, https://doi.org/10.5194/gmd-18-117-2025, 2025
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The Artificial-Intelligence-based Nonspherical Aerosol Optical Scheme (AI-NAOS) was developed to improve the estimation of the aerosol direct radiation effect and was coupled online with a chemical weather model. The AI-NAOS scheme considers black carbon as fractal aggregates and soil dust as super-spheroids, encapsulated with hygroscopic aerosols. Real-case simulations emphasize the necessity of accurately representing nonspherical and inhomogeneous aerosols in chemical weather models.
Lukas Pfitzenmaier, Pavlos Kollias, Nils Risse, Imke Schirmacher, Bernat Puigdomenech Treserras, and Katia Lamer
Geosci. Model Dev., 18, 101–115, https://doi.org/10.5194/gmd-18-101-2025, https://doi.org/10.5194/gmd-18-101-2025, 2025
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The Python tool Orbital-Radar transfers suborbital radar data (ground-based, airborne, and forward-simulated numerical weather prediction model) into synthetic spaceborne cloud profiling radar data, mimicking platform-specific instrument characteristics, e.g. EarthCARE or CloudSat. The tool's novelty lies in simulating characteristic errors and instrument noise. Thus, existing data sets are transferred into synthetic observations and can be used for satellite calibration–validation studies.
Aurélien Mirebeau, Cécile de Munck, Bertrand Bonan, Christine Delire, Aude Lemonsu, Valéry Masson, and Stephan Weber
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-233, https://doi.org/10.5194/gmd-2024-233, 2025
Revised manuscript accepted for GMD
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The greening of cities is recommended to limit the effects of climate change. In particular, green roofs can provide numerous environmental benefits, such as urban cooling, water retention and carbon sequestration. The aim of this research is to develop a new module for calculating green roof CO2 fluxes within a model that can already simulate hydrological and thermal processes of such roofs. The calibration and evaluation of this module take advantage of long term experimental data.
Mark Buehner, Jean-Francois Caron, Ervig Lapalme, Alain Caya, Ping Du, Yves Rochon, Sergey Skachko, Maziar Bani Shahabadi, Sylvain Heilliette, Martin Deshaies-Jacques, Weiguang Chang, and Michael Sitwell
Geosci. Model Dev., 18, 1–18, https://doi.org/10.5194/gmd-18-1-2025, https://doi.org/10.5194/gmd-18-1-2025, 2025
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The Modular and Integrated Data Assimilation System (MIDAS) software is described. The flexible design of MIDAS enables both deterministic and ensemble prediction applications for the atmosphere and several other Earth system components. It is currently used for all main operational weather prediction systems in Canada and also for sea ice and sea surface temperature analysis. The use of MIDAS for multiple Earth system components will facilitate future research on coupled data assimilation.
Alexander de Meij, Cornelis Cuvelier, Philippe Thunis, and Enrico Pisoni
EGUsphere, https://doi.org/10.5194/egusphere-2024-3690, https://doi.org/10.5194/egusphere-2024-3690, 2025
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We assess the relevance and utility indicators developed within FAIRMODE by evaluating 9 CAMS models in calculated air pollutant values. For NO2, the results highlight difficulties at traffic stations. For PM2.5 and PM10 the bias and Winter-Summer gradients reveal issues. O3 evaluation shows that e.g. seasonal gradients are useful. Overall, the indicators provide valuable insights into model limitations, yet there is a need to reconsider the strictness of some indicators for certain pollutants.
Zichen Wu, Xueshun Chen, Zifa Wang, Huansheng Chen, Zhe Wang, Qing Mu, Lin Wu, Wending Wang, Xiao Tang, Jie Li, Ying Li, Qizhong Wu, Yang Wang, Zhiyin Zou, and Zijian Jiang
Geosci. Model Dev., 17, 8885–8907, https://doi.org/10.5194/gmd-17-8885-2024, https://doi.org/10.5194/gmd-17-8885-2024, 2024
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We developed a model to simulate polycyclic aromatic hydrocarbons (PAHs) from global to regional scales. The model can reproduce PAH distribution well. The concentration of BaP (indicator species for PAHs) could exceed the target values of 1 ng m-3 over some areas (e.g., in central Europe, India, and eastern China). The change in BaP is lower than that in PM2.5 from 2013 to 2018. China still faces significant potential health risks posed by BaP although the Action Plan has been implemented.
Marie Taufour, Jean-Pierre Pinty, Christelle Barthe, Benoît Vié, and Chien Wang
Geosci. Model Dev., 17, 8773–8798, https://doi.org/10.5194/gmd-17-8773-2024, https://doi.org/10.5194/gmd-17-8773-2024, 2024
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We have developed a complete two-moment version of the LIMA (Liquid Ice Multiple Aerosols) microphysics scheme. We have focused on collection processes, where the hydrometeor number transfer is often estimated in proportion to the mass transfer. The impact of these parameterizations on a convective system and the prospects for more realistic estimates of secondary parameters (reflectivity, hydrometeor size) are shown in a first test on an idealized case.
Jize Jiang, David S. Stevenson, Aimable Uwizeye, Giuseppe Tempio, Alessandra Falcucci, Flavia Casu, and Mark A. Sutton
EGUsphere, https://doi.org/10.5194/egusphere-2024-3803, https://doi.org/10.5194/egusphere-2024-3803, 2024
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A special model called AMmonia–CLIMate (AMCLIM) has been developed to understand and calculate NH3 emissions from livestock farming. It is estimated that about 30 % of excreted N from livestock was lost due to NH3 emissions from housing, manure management and land application of manure. High NH3 volatilization often occurred in hot regions, while poor management practices also result in significant N losses through NH3 emissions.
Maksym Vasiuta, Angel Navarro Trastoy, Sanam Motlaghzadeh, Lauri Tuppi, Torsten Mayer-Gürr, and Heikki Järvinen
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-136, https://doi.org/10.5194/gmd-2024-136, 2024
Revised manuscript accepted for GMD
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Propagation of electromagnetic signals in the Earth's neutral atmosphere inflicts errors in space geodetic observations. To model these errors as accurately as possible, it is necessary to use a signal ray tracing algorithm which is informed of the state of the atmosphere. We developed such algorithm and tested it by modelling errors in GNSS network observations. Our algorithm's main advantage is loss-less utilization of atmospheric information provided by numerical weather prediction models.
Yuya Takane, Yukihiro Kikegawa, Ko Nakajima, and Hiroyuki Kusaka
Geosci. Model Dev., 17, 8639–8664, https://doi.org/10.5194/gmd-17-8639-2024, https://doi.org/10.5194/gmd-17-8639-2024, 2024
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A new parameterisation for dynamic anthropogenic heat and electricity consumption is described. The model reproduced the temporal variation in and spatial distributions of electricity consumption and temperature well in summer and winter. The partial air conditioning was the most critical factor, significantly affecting the value of anthropogenic heat emission.
Arseniy Karagodin-Doyennel, Fredrik Jansson, Bart van Stratum, Hugo Denier van der Gon, Jordi Vilà-Guerau de Arellano, and Sander Houweling
EGUsphere, https://doi.org/10.5194/egusphere-2024-3721, https://doi.org/10.5194/egusphere-2024-3721, 2024
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We introduce a new simulation platform based on the Dutch Large-Eddy Simulation (DALES) to simulate carbon dioxide (CO2) emissions and their dispersion in the turbulent environments with hectometer resolution. This model incorporates both anthropogenic emission inventory and ecosystem exchanges. Simulation results for the main urban area in the Netherlands demonstrate a strong potential of DALES to enhance CO2 emission modeling, which is important for refining their reduction strategies.
Hongyi Li, Ting Yang, Lars Nerger, Dawei Zhang, Di Zhang, Guigang Tang, Haibo Wang, Yele Sun, Pingqing Fu, Hang Su, and Zifa Wang
Geosci. Model Dev., 17, 8495–8519, https://doi.org/10.5194/gmd-17-8495-2024, https://doi.org/10.5194/gmd-17-8495-2024, 2024
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To accurately characterize the spatiotemporal distribution of particulate matter <2.5 µm chemical components, we developed the Nested Air Quality Prediction Model System with the Parallel Data Assimilation Framework (NAQPMS-PDAF) v2.0 for chemical components with non-Gaussian and nonlinear properties. NAQPMS-PDAF v2.0 has better computing efficiency, excels when used with a small ensemble size, and can significantly improve the simulation performance of chemical components.
T. Nash Skipper, Christian Hogrefe, Barron H. Henderson, Rohit Mathur, Kristen M. Foley, and Armistead G. Russell
Geosci. Model Dev., 17, 8373–8397, https://doi.org/10.5194/gmd-17-8373-2024, https://doi.org/10.5194/gmd-17-8373-2024, 2024
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Chemical transport model simulations are combined with ozone observations to estimate the bias in ozone attributable to US anthropogenic sources and individual sources of US background ozone: natural sources, non-US anthropogenic sources, and stratospheric ozone. Results indicate a positive bias correlated with US anthropogenic emissions during summer in the eastern US and a negative bias correlated with stratospheric ozone during spring.
Li Fang, Jianbing Jin, Arjo Segers, Ke Li, Ji Xia, Wei Han, Baojie Li, Hai Xiang Lin, Lei Zhu, Song Liu, and Hong Liao
Geosci. Model Dev., 17, 8267–8282, https://doi.org/10.5194/gmd-17-8267-2024, https://doi.org/10.5194/gmd-17-8267-2024, 2024
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Model evaluations against ground observations are usually unfair. The former simulates mean status over coarse grids and the latter the surrounding atmosphere. To solve this, we proposed the new land-use-based representative (LUBR) operator that considers intra-grid variance. The LUBR operator is validated to provide insights that align with satellite measurements. The results highlight the importance of considering fine-scale urban–rural differences when comparing models and observation.
Mijie Pang, Jianbing Jin, Arjo Segers, Huiya Jiang, Wei Han, Batjargal Buyantogtokh, Ji Xia, Li Fang, Jiandong Li, Hai Xiang Lin, and Hong Liao
Geosci. Model Dev., 17, 8223–8242, https://doi.org/10.5194/gmd-17-8223-2024, https://doi.org/10.5194/gmd-17-8223-2024, 2024
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The ensemble Kalman filter (EnKF) improves dust storm forecasts but faces challenges with position errors. The valid time shifting EnKF (VTS-EnKF) addresses this by adjusting for position errors, enhancing accuracy in forecasting dust storms, as proven in tests on 2021 events, even with smaller ensembles and time intervals.
Yongzhu Liu, Xiaoye Zhang, Wei Han, Chao Wang, Wenxing Jia, Deying Wang, Zhaorong Zhuang, and Xueshun Shen
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-148, https://doi.org/10.5194/gmd-2024-148, 2024
Revised manuscript accepted for GMD
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In order to investigate the feedbacks of chemical data assimilation on meteorological forecasts, we developed a strongly coupled chemistry meteorology four-dimensional variational (4D-Var) assimilation system, CMA-GFS-AERO 4D-Var, based on the framework of the incremental analysis scheme of the CMA-GFS operational global numerical weather model. The results show that assimilating BC observations can generate analysis increments not only for BC but also for atmospheric variables.
Mike Bush, David L. A. Flack, Huw W. Lewis, Sylvia I. Bohnenstengel, Chris J. Short, Charmaine Franklin, Adrian P. Lock, Martin Best, Paul Field, Anne McCabe, Kwinten Van Weverberg, Segolene Berthou, Ian Boutle, Jennifer K. Brooke, Seb Cole, Shaun Cooper, Gareth Dow, John Edwards, Anke Finnenkoetter, Kalli Furtado, Kate Halladay, Kirsty Hanley, Margaret A. Hendry, Adrian Hill, Aravindakshan Jayakumar, Richard W. Jones, Humphrey Lean, Joshua C. K. Lee, Andy Malcolm, Marion Mittermaier, Saji Mohandas, Stuart Moore, Cyril Morcrette, Rachel North, Aurore Porson, Susan Rennie, Nigel Roberts, Belinda Roux, Claudio Sanchez, Chun-Hsu Su, Simon Tucker, Simon Vosper, David Walters, James Warner, Stuart Webster, Mark Weeks, Jonathan Wilkinson, Michael Whitall, Keith D. Williams, and Hugh Zhang
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-201, https://doi.org/10.5194/gmd-2024-201, 2024
Revised manuscript accepted for GMD
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RAL configurations define settings for the Unified Model atmosphere and Joint UK Land Environment Simulator. The third version of the Regional Atmosphere and Land (RAL3) science configuration for kilometre and sub-km scale modelling represents a major advance compared to previous versions (RAL2) by delivering a common science definition for applications in tropical and mid-latitude regions. RAL3 has more realistic precipitation distributions and improved representation of clouds and visibility.
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