Articles | Volume 19, issue 10
https://doi.org/10.5194/gmd-19-4137-2026
© Author(s) 2026. This work is distributed under the Creative Commons Attribution 4.0 License.
Operational chemical weather forecasting with the ECCC online Regional Air Quality Deterministic Prediction System version 023 (RAQDPS023) – Part 1: system description
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- Final revised paper (published on 20 May 2026)
- Supplement to the final revised paper
- Preprint (discussion started on 09 Dec 2025)
- Supplement to the preprint
Interactive discussion
Status: closed
Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor
| : Report abuse
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RC1: 'Comment on egusphere-2025-4323', Anonymous Referee #1, 12 Jan 2026
- AC1: 'Reply on RC1', Michael Moran, 12 Feb 2026
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RC2: 'Comment on egusphere-2025-4323', Anonymous Referee #2, 15 Jan 2026
- AC2: 'Reply on RC2', Michael Moran, 12 Feb 2026
Peer review completion
AR – Author's response | RR – Referee report | ED – Editor decision | EF – Editorial file upload
AR by Michael Moran on behalf of the Authors (12 Feb 2026)
Author's response
Author's tracked changes
Manuscript
ED: Referee Nomination & Report Request started (17 Feb 2026) by Emmanouil Flaounas
RR by Anonymous Referee #2 (25 Feb 2026)
RR by Anonymous Referee #1 (25 Feb 2026)
ED: Publish as is (03 Mar 2026) by Emmanouil Flaounas
AR by Michael Moran on behalf of the Authors (17 Mar 2026)
Author's response
Manuscript
The manuscript provides a very comprehensive description of the RAQDPS023 modeling system used by Environment and Climate Change Canada to provide air quality forecasts to the public. As such, it is a rare example of a one-stop technical and scientific documentation that allows the reader to gain an understanding of the many different aspects that go into building such a system. It is also extremely well written and structured so that despite its length it is easy to follow. I commend the authors for the care they took in compiling the references that underly the scientific formulations of RAQDPS023. This extensive list of references in conjunction with the detailed descriptions of all RAQDPS023 science processes creates a rare repository of knowledge not only about RAQDPS023 but also about the tremendous amount of effort it takes to design, implement, and operationalize air quality modeling systems more generally. My specific comments listed below are minor and/or editorial in nature.
Specific Comments:
Page 3: “Schiermeir, 1978” should be “Schiermeier, 1978”. While the doi of the scanned copy available through the ACS legacy archives (https://pubs.acs.org/doi/abs/10.1021/es60142a608) indeed mis-spelled the author’s last name, the actual scanned copy available under that doi correctly shows the last name as “Schiermeier”
Page 7, line 218 and Table 1: Consider using “horizontal domain size” instead of “horizontal grid size” since the latter could potentially be misinterpreted to refer to the size (spacing) of individual grid cells which is identical between RAQDPS023 and RDPS 8.0.0.
Page 8, line 255: Maybe change “included a small number of meteorological tracers” to “included two meteorological tracers (water vapour and cloud water)”
Page 8, line 266: Insert “and” between “meteorological” and “chemical”
Page 14, lines 454 - 456: Please clarify relative to which starting point (e.g., 10 bin GEM-MACH configuration, RAQDPS022) this modification of the numerical solution was implemented.
Page 15, line 476: Consider changing “where” to “whereas”
Page 15, lines 495 – 496: This question reveals my lack of understanding of aerosol schemes, but I was still curious what “partially activated” refers to. If there is a critical particle radius above which all aerosol particles are activated as stated on line 489, and if the two bins each represent aerosols of a discrete size, how does partial activation occur? Does each discrete size bin assume an internal distribution of particle radii, allowing a determination of the fraction of particles in a bin that exceed the critical radius above which aerosols are activated?
Page 16, line 521: Would H2O (water vapour) profiles not be available from GEM?
Page 16, lines 537 – 539: Maybe comment on the implications for SOA formation when omitting emissions of organic acids and approaching the decision of which emissions to retain solely from a reactivity point of view.
Page 26, line 877: typo, change “haf already” to “had already”
Page 27, line 898: Could you elaborate on this additional information and how it was used to adjust the inventories?
Page 28, line 942: Should this be “the usual hourly anthropogenic and biogenic emissions” instead of just “the usual hourly anthropogenic emissions”?
Page 30, lines 995 – 1001: Was there any dependency of soil NO emissions on precipitation to represent the pulsing effect described in the Yienger-Levy framework?
Page 33, line 1111: Please check if “for 900 s” is needed here. With the way the end of the sentence is written (“for 900 s for three shorter 300 s time steps”), I am not sure if the only point of the sentence is to say that a single MACH chemistry execution every 900 s still took four times longer than the combined time it took to execute three GEM 300 s physics time steps, or if there is some additional information being conveyed here.
Page 36, lines 1200 – 1211: It might be good to provide a brief summary of which emission inputs (anthropogenic and natural) were used in these MOZART-4 simulations. Did the anthropogenic emissions represent 2009 conditions? Were aircraft, lightning NO, and soil NO emissions considered? Adding such information could set the stage for the updates to LBC in RAQDPS025 and future versions discussed in later sections of the manuscript.
Pages 45, lines 1493 – 1503: Given the episodic nature of processes affecting large-scale distributions of O3, CO, and PM2.5, why did the LBC updates in RAQDPS025 still adopt an approach based on climatology? Were there any differences in the types of anthropogenic and natural emissions considered in the MOZART-4 vs. CAM-chem simulations?
Page 46, lines 1520 – 1522: Does this update eliminate any dependence on the five broad phenological seasons described in the last paragraph of Section 3.9?