Articles | Volume 17, issue 21
https://doi.org/10.5194/gmd-17-7539-2024
https://doi.org/10.5194/gmd-17-7539-2024
Model evaluation paper
 | 
30 Oct 2024
Model evaluation paper |  | 30 Oct 2024

An improved representation of aerosol in the ECMWF IFS-COMPO 49R1 through the integration of EQSAM4Climv12 – a first attempt at simulating aerosol acidity

Samuel Rémy, Swen Metzger, Vincent Huijnen, Jason E. Williams, and Johannes Flemming

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Cited articles

Agusti-Panareda, A., Diamantakis, M., Bayona, V., Klappenbach, F., and Butz, A.: Improving the inter-hemispheric gradient of total column atmospheric CO2 and CH4 in simulations with the ECMWF semi-Lagrangian atmospheric global model, Geosci. Model Dev., 10, 1–18, https://doi.org/10.5194/gmd-10-1-2017, 2017. a
Albert, M. F. M. A., Anguelova, M. D., Manders, A. M. M., Schaap, M., and de Leeuw, G.: Parameterization of oceanic whitecap fraction based on satellite observations, Atmos. Chem. Phys., 16, 13725–13751, https://doi.org/10.5194/acp-16-13725-2016, 2016. a
Angle, K., Neal, E., and Grassian, V.: Enhanced Rates of Transition-Metal-Ion-Catalyzed Oxidation of S(IV) in Aqueous Aerosols: Insights into Sulfate Aerosol Formation in the Atmosphere, Environ. Sci. Technol., 55, 10291–10299, 2021. a
Anguelova, M. D. and Webster, F.: Whitecap coverage from satellite measurements: A first step toward modeling the variability of oceanic whitecaps, J. Geophys. Res., 111, C03017, https://doi.org/10.1029/2005JC003158, 2006. a
Ault, A. P.: Aerosol Acidity: Novel Measurements and Implications for Atmospheric Chemistry, Accounts Chem. Res., 53, 1703–1714, 2020. a
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Short summary
In this paper we describe the development of the future operational cycle 49R1 of the IFS-COMPO system, used for operational forecasts of atmospheric composition in the CAMS project, and focus on the implementation of the thermodynamical model EQSAM4Clim version 12. The implementation of EQSAM4Clim significantly improves the simulated secondary inorganic aerosol surface concentration. The new aerosol and precipitation acidity diagnostics showed good agreement against observational datasets.
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