Articles | Volume 13, issue 3
https://doi.org/10.5194/gmd-13-1007-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/gmd-13-1007-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Development and technical paper
| 
10 Mar 2020
Development and technical paper |
| 10 Mar 2020
| 10 Mar 2020
An aerosol climatology for global models based on the tropospheric aerosol scheme in the Integrated Forecasting System of ECMWF
European Centre for Medium-Range Weather Forecasts, Reading, UK
now at: European Organisation for the Exploitation of Meteorological Satellites, Darmstadt, Germany
Angela Benedetti
European Centre for Medium-Range Weather Forecasts, Reading, UK
Johannes Flemming
European Centre for Medium-Range Weather Forecasts, Reading, UK
Zak Kipling
European Centre for Medium-Range Weather Forecasts, Reading, UK
Samuel Rémy
European Centre for Medium-Range Weather Forecasts, Reading, UK
Institute Pierre-Simon Laplace, Sorbonne Université/CNRS, Paris, France
Related authors
Shannon L. Mason, Robin J. Hogan, Alessio Bozzo, and Nicola L. Pounder
Atmos. Meas. Tech., 16, 3459–3486, https://doi.org/10.5194/amt-16-3459-2023, https://doi.org/10.5194/amt-16-3459-2023, 2023
Short summary
Short summary
We present a method for accurately estimating the contents and properties of clouds, snow, rain, and aerosols through the atmosphere, using the combined measurements of the radar, lidar, and radiometer instruments aboard the upcoming EarthCARE satellite, and evaluate the performance of the retrieval, using test scenes simulated from a numerical forecast model. When EarthCARE is in operation, these quantities and their estimated uncertainties will be distributed in a data product called ACM-CAP.
Beatriz M. Monge-Sanz, Alessio Bozzo, Nicholas Byrne, Martyn P. Chipperfield, Michail Diamantakis, Johannes Flemming, Lesley J. Gray, Robin J. Hogan, Luke Jones, Linus Magnusson, Inna Polichtchouk, Theodore G. Shepherd, Nils Wedi, and Antje Weisheimer
Atmos. Chem. Phys., 22, 4277–4302, https://doi.org/10.5194/acp-22-4277-2022, https://doi.org/10.5194/acp-22-4277-2022, 2022
Short summary
Short summary
The stratosphere is emerging as one of the keys to improve tropospheric weather and climate predictions. This study provides evidence of the role the stratospheric ozone layer plays in improving weather predictions at different timescales. Using a new ozone modelling approach suitable for high-resolution global models that provide operational forecasts from days to seasons, we find significant improvements in stratospheric meteorological fields and stratosphere–troposphere coupling.
Samuel Rémy, Zak Kipling, Johannes Flemming, Olivier Boucher, Pierre Nabat, Martine Michou, Alessio Bozzo, Melanie Ades, Vincent Huijnen, Angela Benedetti, Richard Engelen, Vincent-Henri Peuch, and Jean-Jacques Morcrette
Geosci. Model Dev., 12, 4627–4659, https://doi.org/10.5194/gmd-12-4627-2019, https://doi.org/10.5194/gmd-12-4627-2019, 2019
Short summary
Short summary
This article describes the IFS-AER aerosol module used operationally in the Integrated Forecasting System (IFS) cycle 45R1, operated by the ECMWF in the framework of the Copernicus Atmospheric Monitoring Services (CAMS). We describe the different parameterizations for aerosol sources, sinks, and how the aerosols are integrated in the larger atmospheric composition forecasting system. The skill of PM and AOD simulations against observations is improved compared to the older cycle 40R2.
Jeronimo Escribano, Alessio Bozzo, Philippe Dubuisson, Johannes Flemming, Robin J. Hogan, Laurent C.-Labonnote, and Olivier Boucher
Geosci. Model Dev., 12, 805–827, https://doi.org/10.5194/gmd-12-805-2019, https://doi.org/10.5194/gmd-12-805-2019, 2019
Short summary
Short summary
Accurate shortwave radiance computations are becoming increasingly important for some applications in atmospheric composition. In this work we propose a benchmark protocol and dataset to asses the accuracy and computing runtime of radiance calculations of radiative transfer models. It is applied to four models, showing the potential of this benchmark to evaluate the model performance under a variety of atmospheric conditions, viewing geometries, aerosol loading, and optical properties.
Johannes Flemming, Angela Benedetti, Antje Inness, Richard J. Engelen, Luke Jones, Vincent Huijnen, Samuel Remy, Mark Parrington, Martin Suttie, Alessio Bozzo, Vincent-Henri Peuch, Dimitris Akritidis, and Eleni Katragkou
Atmos. Chem. Phys., 17, 1945–1983, https://doi.org/10.5194/acp-17-1945-2017, https://doi.org/10.5194/acp-17-1945-2017, 2017
Short summary
Short summary
We combine satellite observations of carbon monoxide, ozone and aerosols with the results from a model using a technique called data assimilation. The generated global data set (CAMS interim reanalysis) covers the period 2003–2015 at a resolution of about 110 km. The CAMS interim reanalysis can be used to study global air pollution and climate forcing of aerosol and stratospheric ozone. It has been produced by the Copernicus Atmosphere Monitoring Service (http://atmosphere. copernicus.eu).
S. Rémy, A. Benedetti, A. Bozzo, T. Haiden, L. Jones, M. Razinger, J. Flemming, R. J. Engelen, V. H. Peuch, and J. N. Thepaut
Atmos. Chem. Phys., 15, 12909–12933, https://doi.org/10.5194/acp-15-12909-2015, https://doi.org/10.5194/acp-15-12909-2015, 2015
Short summary
Short summary
In this paper we report on the feedbacks between dust and boundary layer meteorology during a dust storm over Egypt and Libya in April 2012, using an atmospheric composition forecasting system. Dust was found to act on atmospheric stability, leading to an increase (night) or a decrease (day) in dust production. Horizontal gradients of temperature were modified by the radiative impact of the dust layer, leading to changes in wind patterns at the edge of the storm due to the thermal wind effect.
Paolo Andreozzi, Mark D. Fielding, Robin J. Hogan, Richard M. Forbes, Samuel Rémy, Birger Bohn, and Ulrich Löhnert
EGUsphere, https://doi.org/10.5194/egusphere-2025-3790, https://doi.org/10.5194/egusphere-2025-3790, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
Aerosols significantly contribute to the Earth’s climate, but models still struggle at representing them. Here we use satellite observations of clouds to improve aerosols in our weather and air-quality model. We show that African wildfires induce too bright simulated clouds and that our model removes too much aerosol from ice-containing clouds. This showcases how our approach effectively targets poorly observed aerosol processes, potentially informing weather forecasting and climate models.
Anam M. Khan, Olivia E. Clifton, Jesse O. Bash, Sam Bland, Nathan Booth, Philip Cheung, Lisa Emberson, Johannes Flemming, Erick Fredj, Stefano Galmarini, Laurens Ganzeveld, Orestis Gazetas, Ignacio Goded, Christian Hogrefe, Christopher D. Holmes, László Horváth, Vincent Huijnen, Qian Li, Paul A. Makar, Ivan Mammarella, Giovanni Manca, J. William Munger, Juan L. Pérez-Camanyo, Jonathan Pleim, Limei Ran, Roberto San Jose, Donna Schwede, Sam J. Silva, Ralf Staebler, Shihan Sun, Amos P. K. Tai, Eran Tas, Timo Vesala, Tamás Weidinger, Zhiyong Wu, Leiming Zhang, and Paul C. Stoy
Atmos. Chem. Phys., 25, 8613–8635, https://doi.org/10.5194/acp-25-8613-2025, https://doi.org/10.5194/acp-25-8613-2025, 2025
Short summary
Short summary
Vegetation removes tropospheric ozone through stomatal uptake, and accurately modeling the stomatal uptake of ozone is important for modeling dry deposition and air quality. We evaluated the stomatal component of ozone dry deposition modeled by atmospheric chemistry models at six sites. We find that models and observation-based estimates agree at times during the growing season at all sites, but some models overestimated the stomatal component during the dry summers at a seasonally dry site.
Simon Chabrillat, Samuel Rémy, Quentin Errera, Vincent Huijnen, Christine Bingen, Jonas Debosscher, François Hendrick, Swen Metzger, Adrien Mora, Daniele Minganti, Marc Op de beek, Léa Reisenfeld, Jason E. Williams, Henk Eskes, and Johannes Flemming
EGUsphere, https://doi.org/10.5194/egusphere-2025-1327, https://doi.org/10.5194/egusphere-2025-1327, 2025
Short summary
Short summary
We document the forecasts of the composition of the stratosphere by the Copernicus Atmosphere Monitoring Service. The model's predictions are compared with satellite measurements over a recent period, during polar ozone depletion events, and after the Mount Pinatubo volcanic eruption. The system performs well for sulfate aerosols, ozone and several other key gases but not as well for several nitrogen-containing gases. Chemical processes in aerosols and polar clouds should be improved.
Konstantinos Rizos, Emmanouil Proestakis, Thanasis Georgiou, Antonis Gkikas, Eleni Marinou, Peristera Paschou, Kalliopi Artemis Voudouri, Athanasios Tsikerdekis, David Donovan, Gerd-Jan van Zadelhoff, Angela Benedetti, Holger Baars, Athena Augusta Floutsi, Nikos Benas, Martin Stengel, Christian Retscher, Edward Malina, and Vassilis Amiridis
EGUsphere, https://doi.org/10.5194/egusphere-2025-1175, https://doi.org/10.5194/egusphere-2025-1175, 2025
This preprint is open for discussion and under review for Atmospheric Measurement Techniques (AMT).
Short summary
Short summary
The Aeolus satellite's lidar system had limitations in detecting certain atmospheric layers and distinguishing between aerosol and cloud types. To improve accuracy, a new dust detection product was developed. By combining data from various sources and validating it with ground-based measurements, this enhanced product performs better than the original. It helps improve dust transport models and weather predictions, making it a valuable tool for atmospheric monitoring and forecasting.
Sini Talvinen, Paul Kim, Emanuele Tovazzi, Eemeli Holopainen, Roxana Cremer, Thomas Kühn, Harri Kokkola, Zak Kipling, David Neubauer, João C. Teixeira, Alistair Sellar, Duncan Watson-Parris, Yang Yang, Jialei Zhu, Srinath Krishnan, Annele Virtanen, and Daniel G. Partridge
EGUsphere, https://doi.org/10.5194/egusphere-2025-721, https://doi.org/10.5194/egusphere-2025-721, 2025
Short summary
Short summary
Climate models struggle to predict how clouds and aerosols interact, affecting Earth’s energy balance. This study compares models to observations to see how they describe effects of clouds and rain on aerosols. While both models show similar overall trends, seasonal differences emerged. These, however, align with differences in key variables participating in cloud formation. The study provides tools to improve the representation of aerosol-cloud interactions in climate models.
Emmanouil Proestakis, Vassilis Amiridis, Carlos Pérez García-Pando, Svetlana Tsyro, Jan Griesfeller, Antonis Gkikas, Thanasis Georgiou, María Gonçalves Ageitos, Jeronimo Escribano, Stelios Myriokefalitakis, Elisa Bergas Masso, Enza Di Tomaso, Sara Basart, Jan-Berend W. Stuut, and Angela Benedetti
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2025-43, https://doi.org/10.5194/essd-2025-43, 2025
Revised manuscript accepted for ESSD
Short summary
Short summary
Quantification of dust deposition into the broader Atlantic Ocean is provided, with the estimates established on the basis of Earth Observations. The dataset is considered unique with respect to a range of applications, including compensating for spatiotemporal gaps of sediment-trap measurements, assessments of model simulations, shedding light into physical processes related to the dust cycle, and to better understand dust biogeochemical impacts on oceanic ecosystems, on weather, and climate.
Mariya Petrenko, Ralph Kahn, Mian Chin, Susanne E. Bauer, Tommi Bergman, Huisheng Bian, Gabriele Curci, Ben Johnson, Johannes W. Kaiser, Zak Kipling, Harri Kokkola, Xiaohong Liu, Keren Mezuman, Tero Mielonen, Gunnar Myhre, Xiaohua Pan, Anna Protonotariou, Samuel Remy, Ragnhild Bieltvedt Skeie, Philip Stier, Toshihiko Takemura, Kostas Tsigaridis, Hailong Wang, Duncan Watson-Parris, and Kai Zhang
Atmos. Chem. Phys., 25, 1545–1567, https://doi.org/10.5194/acp-25-1545-2025, https://doi.org/10.5194/acp-25-1545-2025, 2025
Short summary
Short summary
We compared smoke plume simulations from 11 global models to each other and to satellite smoke amount observations aimed at constraining smoke source strength. In regions where plumes are thick and background aerosol is low, models and satellites compare well. However, the input emission inventory tends to underestimate in many places, and particle property and loss rate assumptions vary enormously among models, causing uncertainties that require systematic in situ measurements to resolve.
Augustin Colette, Gaëlle Collin, François Besson, Etienne Blot, Vincent Guidard, Frederik Meleux, Adrien Royer, Valentin Petiot, Claire Miller, Oihana Fermond, Alizé Jeant, Mario Adani, Joaquim Arteta, Anna Benedictow, Robert Bergström, Dene Bowdalo, Jorgen Brandt, Gino Briganti, Ana C. Carvalho, Jesper Heile Christensen, Florian Couvidat, Ilia D’Elia, Massimo D’Isidoro, Hugo Denier van der Gon, Gaël Descombes, Enza Di Tomaso, John Douros, Jeronimo Escribano, Henk Eskes, Hilde Fagerli, Yalda Fatahi, Johannes Flemming, Elmar Friese, Lise Frohn, Michael Gauss, Camilla Geels, Guido Guarnieri, Marc Guevara, Antoine Guion, Jonathan Guth, Risto Hänninen, Kaj Hansen, Ulas Im, Ruud Janssen, Marine Jeoffrion, Mathieu Joly, Luke Jones, Oriol Jorba, Evgeni Kadantsev, Michael Kahnert, Jacek W. Kaminski, Rostislav Kouznetsov, Richard Kranenburg, Jeroen Kuenen, Anne Caroline Lange, Joachim Langner, Victor Lannuque, Francesca Macchia, Astrid Manders, Mihaela Mircea, Agnes Nyiri, Miriam Olid, Carlos Pérez García-Pando, Yuliia Palamarchuk, Antonio Piersanti, Blandine Raux, Miha Razinger, Lennard Robertson, Arjo Segers, Martijn Schaap, Pilvi Siljamo, David Simpson, Mikhail Sofiev, Anders Stangel, Joanna Struzewska, Carles Tena, Renske Timmermans, Thanos Tsikerdekis, Svetlana Tsyro, Svyatoslav Tyuryakov, Anthony Ung, Andreas Uppstu, Alvaro Valdebenito, Peter van Velthoven, Lina Vitali, Zhuyun Ye, Vincent-Henri Peuch, and Laurence Rouïl
EGUsphere, https://doi.org/10.5194/egusphere-2024-3744, https://doi.org/10.5194/egusphere-2024-3744, 2024
Short summary
Short summary
The Copernicus Atmosphere Monitoring Service – Regional Production delivers daily forecasts, analyses, and reanalyses of air quality in Europe. The Service relies on a distributed modelling production by eleven leading European modelling teams following stringent requirements with an operational design which has no equivalent in the world. All the products are full, free, open and quality assured and disseminated with a high level of reliability.
Jason Williams, Swen Metzer, Samuel Remy, Vincent Huijnen, and Johannes Flemming
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-188, https://doi.org/10.5194/gmd-2024-188, 2024
Revised manuscript under review for GMD
Short summary
Short summary
One of the main constituents of Particulate Matter at the surface are Secondary Inorganic Aerosols (SIA) which are influenced by both anthropogenic emissions and the acidity of clouds and aerosols. This study shows improvements in introduced into the IFS-COMPO simulating the surface concentrations of SIA and the resulting changes in the total wet deposition for Europe, the US and South-East Asia.
Yunqian Zhu, Hideharu Akiyoshi, Valentina Aquila, Elisabeth Asher, Ewa M. Bednarz, Slimane Bekki, Christoph Brühl, Amy H. Butler, Parker Case, Simon Chabrillat, Gabriel Chiodo, Margot Clyne, Lola Falletti, Peter R. Colarco, Eric Fleming, Andrin Jörimann, Mahesh Kovilakam, Gerbrand Koren, Ales Kuchar, Nicolas Lebas, Qing Liang, Cheng-Cheng Liu, Graham Mann, Michael Manyin, Marion Marchand, Olaf Morgenstern, Paul Newman, Luke D. Oman, Freja F. Østerstrøm, Yifeng Peng, David Plummer, Ilaria Quaglia, William Randel, Samuel Rémy, Takashi Sekiya, Stephen Steenrod, Timofei Sukhodolov, Simone Tilmes, Kostas Tsigaridis, Rei Ueyama, Daniele Visioni, Xinyue Wang, Shingo Watanabe, Yousuke Yamashita, Pengfei Yu, Wandi Yu, Jun Zhang, and Zhihong Zhuo
EGUsphere, https://doi.org/10.5194/egusphere-2024-3412, https://doi.org/10.5194/egusphere-2024-3412, 2024
Short summary
Short summary
To understand the climate impact of the 2022 Hunga volcanic eruption, we developed a climate model-observation comparison project. The paper describes the protocols and models that participate in the experiments. We designed several experiments to achieve our goal of this activity: 1. evaluate the climate model performance; 2. understand the Earth system responses to this eruption.
Samuel Rémy, Swen Metzger, Vincent Huijnen, Jason E. Williams, and Johannes Flemming
Geosci. Model Dev., 17, 7539–7567, https://doi.org/10.5194/gmd-17-7539-2024, https://doi.org/10.5194/gmd-17-7539-2024, 2024
Short summary
Short summary
In this paper we describe the development of the future operational cycle 49R1 of the IFS-COMPO system, used for operational forecasts of atmospheric composition in the CAMS project, and focus on the implementation of the thermodynamical model EQSAM4Clim version 12. The implementation of EQSAM4Clim significantly improves the simulated secondary inorganic aerosol surface concentration. The new aerosol and precipitation acidity diagnostics showed good agreement against observational datasets.
Jorge E. Pachón, Mariel A. Opazo, Pablo Lichtig, Nicolas Huneeus, Idir Bouarar, Guy Brasseur, Cathy W. Y. Li, Johannes Flemming, Laurent Menut, Camilo Menares, Laura Gallardo, Michael Gauss, Mikhail Sofiev, Rostislav Kouznetsov, Julia Palamarchuk, Andreas Uppstu, Laura Dawidowski, Nestor Y. Rojas, María de Fátima Andrade, Mario E. Gavidia-Calderón, Alejandro H. Delgado Peralta, and Daniel Schuch
Geosci. Model Dev., 17, 7467–7512, https://doi.org/10.5194/gmd-17-7467-2024, https://doi.org/10.5194/gmd-17-7467-2024, 2024
Short summary
Short summary
Latin America (LAC) has some of the most populated urban areas in the world, with high levels of air pollution. Air quality management in LAC has been traditionally focused on surveillance and building emission inventories. This study performed the first intercomparison and model evaluation in LAC, with interesting and insightful findings for the region. A multiscale modeling ensemble chain was assembled as a first step towards an air quality forecasting system.
Henk Eskes, Athanasios Tsikerdekis, Melanie Ades, Mihai Alexe, Anna Carlin Benedictow, Yasmine Bennouna, Lewis Blake, Idir Bouarar, Simon Chabrillat, Richard Engelen, Quentin Errera, Johannes Flemming, Sebastien Garrigues, Jan Griesfeller, Vincent Huijnen, Luka Ilić, Antje Inness, John Kapsomenakis, Zak Kipling, Bavo Langerock, Augustin Mortier, Mark Parrington, Isabelle Pison, Mikko Pitkänen, Samuel Remy, Andreas Richter, Anja Schoenhardt, Michael Schulz, Valerie Thouret, Thorsten Warneke, Christos Zerefos, and Vincent-Henri Peuch
Atmos. Chem. Phys., 24, 9475–9514, https://doi.org/10.5194/acp-24-9475-2024, https://doi.org/10.5194/acp-24-9475-2024, 2024
Short summary
Short summary
The Copernicus Atmosphere Monitoring Service (CAMS) provides global analyses and forecasts of aerosols and trace gases in the atmosphere. On 27 June 2023 a major upgrade, Cy48R1, became operational. Comparisons with in situ, surface remote sensing, aircraft, and balloon and satellite observations show that the new CAMS system is a significant improvement. The results quantify the skill of CAMS to forecast impactful events, such as wildfires, dust storms and air pollution peaks.
Claire L. Ryder, Clément Bézier, Helen F. Dacre, Rory Clarkson, Vassilis Amiridis, Eleni Marinou, Emmanouil Proestakis, Zak Kipling, Angela Benedetti, Mark Parrington, Samuel Rémy, and Mark Vaughan
Nat. Hazards Earth Syst. Sci., 24, 2263–2284, https://doi.org/10.5194/nhess-24-2263-2024, https://doi.org/10.5194/nhess-24-2263-2024, 2024
Short summary
Short summary
Desert dust poses a hazard to aircraft via degradation of engine components. This has financial implications for the aviation industry and results in increased fuel burn with climate impacts. Here we quantify dust ingestion by aircraft engines at airports worldwide. We find Dubai and Delhi in summer are among the dustiest airports, where substantial engine degradation would occur after 1000 flights. Dust ingestion can be reduced by changing take-off times and the altitude of holding patterns.
Swen Metzger, Samuel Rémy, Jason E. Williams, Vincent Huijnen, and Johannes Flemming
Geosci. Model Dev., 17, 5009–5021, https://doi.org/10.5194/gmd-17-5009-2024, https://doi.org/10.5194/gmd-17-5009-2024, 2024
Short summary
Short summary
EQSAM4Clim has recently been revised to provide an accurate and efficient method for calculating the acidity of atmospheric particles. It is based on an analytical concept that is sufficiently fast and free of numerical noise, which makes it attractive for air quality forecasting. Version 12 allows the calculation of aerosol composition based on the gas–liquid–solid and the reduced gas–liquid partitioning with the associated water uptake for both cases, including the acidity of the aerosols.
Peng Xian, Jeffrey S. Reid, Melanie Ades, Angela Benedetti, Peter R. Colarco, Arlindo da Silva, Tom F. Eck, Johannes Flemming, Edward J. Hyer, Zak Kipling, Samuel Rémy, Tsuyoshi Thomas Sekiyama, Taichu Tanaka, Keiya Yumimoto, and Jianglong Zhang
Atmos. Chem. Phys., 24, 6385–6411, https://doi.org/10.5194/acp-24-6385-2024, https://doi.org/10.5194/acp-24-6385-2024, 2024
Short summary
Short summary
The study compares and evaluates monthly AOD of four reanalyses (RA) and their consensus (i.e., ensemble mean). The basic verification characteristics of these RA versus both AERONET and MODIS retrievals are presented. The study discusses the strength of each RA and identifies regions where divergence and challenges are prominent. The RA consensus usually performs very well on a global scale in terms of how well it matches the observational data, making it a good choice for various applications.
Sebastien Garrigues, Melanie Ades, Samuel Remy, Johannes Flemming, Zak Kipling, Istvan Laszlo, Mark Parrington, Antje Inness, Roberto Ribas, Luke Jones, Richard Engelen, and Vincent-Henri Peuch
Atmos. Chem. Phys., 23, 10473–10487, https://doi.org/10.5194/acp-23-10473-2023, https://doi.org/10.5194/acp-23-10473-2023, 2023
Short summary
Short summary
The Copernicus Atmosphere Monitoring Service (CAMS) provides global monitoring of aerosols using the ECMWF forecast model constrained by the assimilation of satellite aerosol optical depth (AOD). This work aims at evaluating the assimilation of the NOAA VIIRS AOD product in the ECMWF model. It shows that the introduction of VIIRS in the CAMS data assimilation system enhances the accuracy of the aerosol analysis, particularly over Europe and desert and maritime sites.
Olivia E. Clifton, Donna Schwede, Christian Hogrefe, Jesse O. Bash, Sam Bland, Philip Cheung, Mhairi Coyle, Lisa Emberson, Johannes Flemming, Erick Fredj, Stefano Galmarini, Laurens Ganzeveld, Orestis Gazetas, Ignacio Goded, Christopher D. Holmes, László Horváth, Vincent Huijnen, Qian Li, Paul A. Makar, Ivan Mammarella, Giovanni Manca, J. William Munger, Juan L. Pérez-Camanyo, Jonathan Pleim, Limei Ran, Roberto San Jose, Sam J. Silva, Ralf Staebler, Shihan Sun, Amos P. K. Tai, Eran Tas, Timo Vesala, Tamás Weidinger, Zhiyong Wu, and Leiming Zhang
Atmos. Chem. Phys., 23, 9911–9961, https://doi.org/10.5194/acp-23-9911-2023, https://doi.org/10.5194/acp-23-9911-2023, 2023
Short summary
Short summary
A primary sink of air pollutants is dry deposition. Dry deposition estimates differ across the models used to simulate atmospheric chemistry. Here, we introduce an effort to examine dry deposition schemes from atmospheric chemistry models. We provide our approach’s rationale, document the schemes, and describe datasets used to drive and evaluate the schemes. We also launch the analysis of results by evaluating against observations and identifying the processes leading to model–model differences.
Shannon L. Mason, Robin J. Hogan, Alessio Bozzo, and Nicola L. Pounder
Atmos. Meas. Tech., 16, 3459–3486, https://doi.org/10.5194/amt-16-3459-2023, https://doi.org/10.5194/amt-16-3459-2023, 2023
Short summary
Short summary
We present a method for accurately estimating the contents and properties of clouds, snow, rain, and aerosols through the atmosphere, using the combined measurements of the radar, lidar, and radiometer instruments aboard the upcoming EarthCARE satellite, and evaluate the performance of the retrieval, using test scenes simulated from a numerical forecast model. When EarthCARE is in operation, these quantities and their estimated uncertainties will be distributed in a data product called ACM-CAP.
Pantelis Kiriakidis, Antonis Gkikas, Georgios Papangelis, Theodoros Christoudias, Jonilda Kushta, Emmanouil Proestakis, Anna Kampouri, Eleni Marinou, Eleni Drakaki, Angela Benedetti, Michael Rennie, Christian Retscher, Anne Grete Straume, Alexandru Dandocsi, Jean Sciare, and Vasilis Amiridis
Atmos. Chem. Phys., 23, 4391–4417, https://doi.org/10.5194/acp-23-4391-2023, https://doi.org/10.5194/acp-23-4391-2023, 2023
Short summary
Short summary
With the launch of the Aeolus satellite, higher-accuracy wind products became available. This research was carried out to validate the assimilated wind products by testing their effect on the WRF-Chem model predictive ability of dust processes. This was carried out for the eastern Mediterranean and Middle East region for two 2-month periods in autumn and spring 2020. The use of the assimilated products improved the dust forecasts of the autumn season (both quantitatively and qualitatively).
Anna Agustí-Panareda, Jérôme Barré, Sébastien Massart, Antje Inness, Ilse Aben, Melanie Ades, Bianca C. Baier, Gianpaolo Balsamo, Tobias Borsdorff, Nicolas Bousserez, Souhail Boussetta, Michael Buchwitz, Luca Cantarello, Cyril Crevoisier, Richard Engelen, Henk Eskes, Johannes Flemming, Sébastien Garrigues, Otto Hasekamp, Vincent Huijnen, Luke Jones, Zak Kipling, Bavo Langerock, Joe McNorton, Nicolas Meilhac, Stefan Noël, Mark Parrington, Vincent-Henri Peuch, Michel Ramonet, Miha Razinger, Maximilian Reuter, Roberto Ribas, Martin Suttie, Colm Sweeney, Jérôme Tarniewicz, and Lianghai Wu
Atmos. Chem. Phys., 23, 3829–3859, https://doi.org/10.5194/acp-23-3829-2023, https://doi.org/10.5194/acp-23-3829-2023, 2023
Short summary
Short summary
We present a global dataset of atmospheric CO2 and CH4, the two most important human-made greenhouse gases, which covers almost 2 decades (2003–2020). It is produced by combining satellite data of CO2 and CH4 with a weather and air composition prediction model, and it has been carefully evaluated against independent observations to ensure validity and point out deficiencies to the user. This dataset can be used for scientific studies in the field of climate change and the global carbon cycle.
Stijn Naus, Lucas G. Domingues, Maarten Krol, Ingrid T. Luijkx, Luciana V. Gatti, John B. Miller, Emanuel Gloor, Sourish Basu, Caio Correia, Gerbrand Koren, Helen M. Worden, Johannes Flemming, Gabrielle Pétron, and Wouter Peters
Atmos. Chem. Phys., 22, 14735–14750, https://doi.org/10.5194/acp-22-14735-2022, https://doi.org/10.5194/acp-22-14735-2022, 2022
Short summary
Short summary
We assimilate MOPITT CO satellite data in the TM5-4D-Var inverse modelling framework to estimate Amazon fire CO emissions for 2003–2018. We show that fire emissions have decreased over the analysis period, coincident with a decrease in deforestation rates. However, interannual variations in fire emissions are large, and they correlate strongly with soil moisture. Our results reveal an important role for robust, top-down fire CO emissions in quantifying and attributing Amazon fire intensity.
Sebastien Garrigues, Samuel Remy, Julien Chimot, Melanie Ades, Antje Inness, Johannes Flemming, Zak Kipling, Istvan Laszlo, Angela Benedetti, Roberto Ribas, Soheila Jafariserajehlou, Bertrand Fougnie, Shobha Kondragunta, Richard Engelen, Vincent-Henri Peuch, Mark Parrington, Nicolas Bousserez, Margarita Vazquez Navarro, and Anna Agusti-Panareda
Atmos. Chem. Phys., 22, 14657–14692, https://doi.org/10.5194/acp-22-14657-2022, https://doi.org/10.5194/acp-22-14657-2022, 2022
Short summary
Short summary
The Copernicus Atmosphere Monitoring Service (CAMS) provides global monitoring of aerosols using the ECMWF forecast model constrained by the assimilation of satellite aerosol optical depth (AOD). This work aims at evaluating two new satellite AODs to enhance the CAMS aerosol global forecast. It highlights the spatial and temporal differences between the satellite AOD products at the model spatial resolution, which is essential information to design multi-satellite AOD data assimilation schemes.
Antje Inness, Ilse Aben, Melanie Ades, Tobias Borsdorff, Johannes Flemming, Luke Jones, Jochen Landgraf, Bavo Langerock, Philippe Nedelec, Mark Parrington, and Roberto Ribas
Atmos. Chem. Phys., 22, 14355–14376, https://doi.org/10.5194/acp-22-14355-2022, https://doi.org/10.5194/acp-22-14355-2022, 2022
Short summary
Short summary
The Copernicus Atmosphere Monitoring Service (CAMS) provides daily global air quality forecasts to users worldwide. One of the species of interest is carbon monoxide (CO), an important trace gas in the atmosphere with anthropogenic and natural sources, produced by incomplete combustion, for example, by wildfires. This paper looks at how well CAMS can model CO in the atmosphere and shows that the fields can be improved when blending CO data from the TROPOMI instrument with the CAMS model.
Thomas Drugé, Pierre Nabat, Marc Mallet, Martine Michou, Samuel Rémy, and Oleg Dubovik
Atmos. Chem. Phys., 22, 12167–12205, https://doi.org/10.5194/acp-22-12167-2022, https://doi.org/10.5194/acp-22-12167-2022, 2022
Short summary
Short summary
This study presents the implementation of brown carbon in the atmospheric component of the CNRM global climate model and particularly in its aerosol scheme TACTIC. Several simulations were carried out with this climate model, over the period 2000–2014, to evaluate the model by comparison with different reference datasets (PARASOL-GRASP, OMI-OMAERUVd, MACv2, FMI_SAT, AERONET) and to analyze the brown carbon radiative and climatic effects.
Sini Isokääntä, Paul Kim, Santtu Mikkonen, Thomas Kühn, Harri Kokkola, Taina Yli-Juuti, Liine Heikkinen, Krista Luoma, Tuukka Petäjä, Zak Kipling, Daniel Partridge, and Annele Virtanen
Atmos. Chem. Phys., 22, 11823–11843, https://doi.org/10.5194/acp-22-11823-2022, https://doi.org/10.5194/acp-22-11823-2022, 2022
Short summary
Short summary
This research employs air mass history analysis and observations to study how clouds and precipitation affect atmospheric aerosols during transport to a boreal forest site. The mass concentrations of studied chemical species showed exponential decrease as a function of accumulated rain along the air mass route. Our analysis revealed in-cloud sulfate formation, while no major changes in organic mass were seen. Most of the in-cloud-formed sulfate could be assigned to particle sizes above 200 nm.
Qirui Zhong, Nick Schutgens, Guido van der Werf, Twan van Noije, Kostas Tsigaridis, Susanne E. Bauer, Tero Mielonen, Alf Kirkevåg, Øyvind Seland, Harri Kokkola, Ramiro Checa-Garcia, David Neubauer, Zak Kipling, Hitoshi Matsui, Paul Ginoux, Toshihiko Takemura, Philippe Le Sager, Samuel Rémy, Huisheng Bian, Mian Chin, Kai Zhang, Jialei Zhu, Svetlana G. Tsyro, Gabriele Curci, Anna Protonotariou, Ben Johnson, Joyce E. Penner, Nicolas Bellouin, Ragnhild B. Skeie, and Gunnar Myhre
Atmos. Chem. Phys., 22, 11009–11032, https://doi.org/10.5194/acp-22-11009-2022, https://doi.org/10.5194/acp-22-11009-2022, 2022
Short summary
Short summary
Aerosol optical depth (AOD) errors for biomass burning aerosol (BBA) are evaluated in 18 global models against satellite datasets. Notwithstanding biases in satellite products, they allow model evaluations. We observe large and diverse model biases due to errors in BBA. Further interpretations of AOD diversities suggest large biases exist in key processes for BBA which require better constraining. These results can contribute to further model improvement and development.
Vincent Huijnen, Philippe Le Sager, Marcus O. Köhler, Glenn Carver, Samuel Rémy, Johannes Flemming, Simon Chabrillat, Quentin Errera, and Twan van Noije
Geosci. Model Dev., 15, 6221–6241, https://doi.org/10.5194/gmd-15-6221-2022, https://doi.org/10.5194/gmd-15-6221-2022, 2022
Short summary
Short summary
We report on the first implementation of atmospheric chemistry and aerosol as part of the OpenIFS model, based on the CAMS global model. We give an overview of the model and evaluate two reference model configurations, with and without the stratospheric chemistry extension, against a variety of observational datasets. This OpenIFS version with atmospheric composition components is open to the scientific user community under a standard OpenIFS license.
Peng Xian, Jianglong Zhang, Norm T. O'Neill, Travis D. Toth, Blake Sorenson, Peter R. Colarco, Zak Kipling, Edward J. Hyer, James R. Campbell, Jeffrey S. Reid, and Keyvan Ranjbar
Atmos. Chem. Phys., 22, 9915–9947, https://doi.org/10.5194/acp-22-9915-2022, https://doi.org/10.5194/acp-22-9915-2022, 2022
Short summary
Short summary
The study provides baseline Arctic spring and summertime aerosol optical depth climatology, trend, and extreme event statistics from 2003 to 2019 using a combination of aerosol reanalyses, remote sensing, and ground observations. Biomass burning smoke has an overwhelming contribution to black carbon (an efficient climate forcer) compared to anthropogenic sources. Burning's large interannual variability and increasing summer trend have important implications for the Arctic climate.
Samuel Rémy, Zak Kipling, Vincent Huijnen, Johannes Flemming, Pierre Nabat, Martine Michou, Melanie Ades, Richard Engelen, and Vincent-Henri Peuch
Geosci. Model Dev., 15, 4881–4912, https://doi.org/10.5194/gmd-15-4881-2022, https://doi.org/10.5194/gmd-15-4881-2022, 2022
Short summary
Short summary
This article describes a new version of IFS-AER, the tropospheric aerosol scheme used to provide global aerosol products within the Copernicus Atmosphere Monitoring Service (CAMS) cycle. Several components of the model have been updated, such as the dynamical dust and sea salt aerosol emission schemes. New deposition schemes have also been incorporated but are not yet used operationally. This new version of IFS-AER has been evaluated and shown to have a greater skill than previous versions.
Jason E. Williams, Vincent Huijnen, Idir Bouarar, Mehdi Meziane, Timo Schreurs, Sophie Pelletier, Virginie Marécal, Beatrice Josse, and Johannes Flemming
Geosci. Model Dev., 15, 4657–4687, https://doi.org/10.5194/gmd-15-4657-2022, https://doi.org/10.5194/gmd-15-4657-2022, 2022
Short summary
Short summary
The global CAMS air quality model is used for providing tropospheric ozone information to end users. This paper updates the chemical mechanism employed (CBA) and compares it against two other mechanisms (MOCAGE, MOZART) and a multi-decadal dataset based on a previous version of CBA. We perform extensive validation for the US using multiple surface and aircraft datasets, providing an assessment of biases and the extent of correlation across different seasons during 2014.
Dimitris Akritidis, Andrea Pozzer, Johannes Flemming, Antje Inness, Philippe Nédélec, and Prodromos Zanis
Atmos. Chem. Phys., 22, 6275–6289, https://doi.org/10.5194/acp-22-6275-2022, https://doi.org/10.5194/acp-22-6275-2022, 2022
Short summary
Short summary
We perform a process-oriented evaluation of Copernicus Atmosphere Monitoring Service (CAMS) reanalysis (CAMSRA) O3 over Europe using WOUDC (World Ozone and Ultraviolet Radiation Data Centre) ozonesondes and IAGOS (In-service Aircraft for a Global Observing System) aircraft measurements. Chemical data assimilation assists CAMSRA to reproduce the observed O3 increases in the troposphere during the examined folding events, but it mostly results in O3 overestimation in the upper troposphere.
Joe McNorton, Nicolas Bousserez, Anna Agustí-Panareda, Gianpaolo Balsamo, Luca Cantarello, Richard Engelen, Vincent Huijnen, Antje Inness, Zak Kipling, Mark Parrington, and Roberto Ribas
Atmos. Chem. Phys., 22, 5961–5981, https://doi.org/10.5194/acp-22-5961-2022, https://doi.org/10.5194/acp-22-5961-2022, 2022
Short summary
Short summary
Concentrations of atmospheric methane continue to grow, in recent years at an increasing rate, for unknown reasons. Using newly available satellite observations and a state-of-the-art weather prediction model we perform global estimates of emissions from hotspots at high resolution. Results show that the system can accurately report on biases in national inventories and is used to conclude that the early COVID-19 slowdown period (March–June 2020) had little impact on global methane emissions.
Beatriz M. Monge-Sanz, Alessio Bozzo, Nicholas Byrne, Martyn P. Chipperfield, Michail Diamantakis, Johannes Flemming, Lesley J. Gray, Robin J. Hogan, Luke Jones, Linus Magnusson, Inna Polichtchouk, Theodore G. Shepherd, Nils Wedi, and Antje Weisheimer
Atmos. Chem. Phys., 22, 4277–4302, https://doi.org/10.5194/acp-22-4277-2022, https://doi.org/10.5194/acp-22-4277-2022, 2022
Short summary
Short summary
The stratosphere is emerging as one of the keys to improve tropospheric weather and climate predictions. This study provides evidence of the role the stratospheric ozone layer plays in improving weather predictions at different timescales. Using a new ozone modelling approach suitable for high-resolution global models that provide operational forecasts from days to seasons, we find significant improvements in stratospheric meteorological fields and stratosphere–troposphere coupling.
Antje Inness, Melanie Ades, Dimitris Balis, Dmitry Efremenko, Johannes Flemming, Pascal Hedelt, Maria-Elissavet Koukouli, Diego Loyola, and Roberto Ribas
Geosci. Model Dev., 15, 971–994, https://doi.org/10.5194/gmd-15-971-2022, https://doi.org/10.5194/gmd-15-971-2022, 2022
Short summary
Short summary
This paper describes the way that the Copernicus Atmosphere Monitoring Service (CAMS) produces forecasts of volcanic SO2. These forecasts are provided routinely every day. They are created by blending SO2 data from satellite instruments (TROPOMI and GOME-2) with the CAMS model. We show that the quality of the CAMS SO2 forecasts can be improved if additional information about the height of volcanic plumes is provided in the satellite data.
Maria Sand, Bjørn H. Samset, Gunnar Myhre, Jonas Gliß, Susanne E. Bauer, Huisheng Bian, Mian Chin, Ramiro Checa-Garcia, Paul Ginoux, Zak Kipling, Alf Kirkevåg, Harri Kokkola, Philippe Le Sager, Marianne T. Lund, Hitoshi Matsui, Twan van Noije, Dirk J. L. Olivié, Samuel Remy, Michael Schulz, Philip Stier, Camilla W. Stjern, Toshihiko Takemura, Kostas Tsigaridis, Svetlana G. Tsyro, and Duncan Watson-Parris
Atmos. Chem. Phys., 21, 15929–15947, https://doi.org/10.5194/acp-21-15929-2021, https://doi.org/10.5194/acp-21-15929-2021, 2021
Short summary
Short summary
Absorption of shortwave radiation by aerosols can modify precipitation and clouds but is poorly constrained in models. A total of 15 different aerosol models from AeroCom phase III have reported total aerosol absorption, and for the first time, 11 of these models have reported in a consistent experiment the contributions to absorption from black carbon, dust, and organic aerosol. Here, we document the model diversity in aerosol absorption.
Anthony C. Jones, Adrian Hill, Samuel Remy, N. Luke Abraham, Mohit Dalvi, Catherine Hardacre, Alan J. Hewitt, Ben Johnson, Jane P. Mulcahy, and Steven T. Turnock
Atmos. Chem. Phys., 21, 15901–15927, https://doi.org/10.5194/acp-21-15901-2021, https://doi.org/10.5194/acp-21-15901-2021, 2021
Short summary
Short summary
Ammonium nitrate is hard to model because it forms and evaporates rapidly. One approach is to relate its equilibrium concentration to temperature, humidity, and the amount of nitric acid and ammonia gases. Using this approach, we limit the rate at which equilibrium is reached using various condensation rates in a climate model. We show that ammonium nitrate concentrations are highly sensitive to the condensation rate. Our results will help improve the representation of nitrate in climate models.
Jérôme Barré, Hervé Petetin, Augustin Colette, Marc Guevara, Vincent-Henri Peuch, Laurence Rouil, Richard Engelen, Antje Inness, Johannes Flemming, Carlos Pérez García-Pando, Dene Bowdalo, Frederik Meleux, Camilla Geels, Jesper H. Christensen, Michael Gauss, Anna Benedictow, Svetlana Tsyro, Elmar Friese, Joanna Struzewska, Jacek W. Kaminski, John Douros, Renske Timmermans, Lennart Robertson, Mario Adani, Oriol Jorba, Mathieu Joly, and Rostislav Kouznetsov
Atmos. Chem. Phys., 21, 7373–7394, https://doi.org/10.5194/acp-21-7373-2021, https://doi.org/10.5194/acp-21-7373-2021, 2021
Short summary
Short summary
This study provides a comprehensive assessment of air quality changes across the main European urban areas induced by the COVID-19 lockdown using satellite observations, surface site measurements, and the forecasting system from the Copernicus Atmospheric Monitoring Service (CAMS). We demonstrate the importance of accounting for weather and seasonal variability when calculating such estimates.
Harald Flentje, Ina Mattis, Zak Kipling, Samuel Rémy, and Werner Thomas
Geosci. Model Dev., 14, 1721–1751, https://doi.org/10.5194/gmd-14-1721-2021, https://doi.org/10.5194/gmd-14-1721-2021, 2021
Short summary
Short summary
Atmospheric aerosols crucially impact air quality, climate and weather. Thus, global model forecasts of atmospheric constituents are published daily on the ECMWF website and are regularly verified by the CAMS service team. The IFS-AER model is largely able to reproduce observed 3-D distributions of the important particle types over Germany. The particle concentration is mostly captured within several tens of percent, but quantification of some specific processes still remains a challenge.
Jonas Gliß, Augustin Mortier, Michael Schulz, Elisabeth Andrews, Yves Balkanski, Susanne E. Bauer, Anna M. K. Benedictow, Huisheng Bian, Ramiro Checa-Garcia, Mian Chin, Paul Ginoux, Jan J. Griesfeller, Andreas Heckel, Zak Kipling, Alf Kirkevåg, Harri Kokkola, Paolo Laj, Philippe Le Sager, Marianne Tronstad Lund, Cathrine Lund Myhre, Hitoshi Matsui, Gunnar Myhre, David Neubauer, Twan van Noije, Peter North, Dirk J. L. Olivié, Samuel Rémy, Larisa Sogacheva, Toshihiko Takemura, Kostas Tsigaridis, and Svetlana G. Tsyro
Atmos. Chem. Phys., 21, 87–128, https://doi.org/10.5194/acp-21-87-2021, https://doi.org/10.5194/acp-21-87-2021, 2021
Short summary
Short summary
Simulated aerosol optical properties as well as the aerosol life cycle are investigated for 14 global models participating in the AeroCom initiative. Considerable diversity is found in the simulated aerosol species emissions and lifetimes, also resulting in a large diversity in the simulated aerosol mass, composition, and optical properties. A comparison with observations suggests that, on average, current models underestimate the direct effect of aerosol on the atmosphere radiation budget.
Jane P. Mulcahy, Colin Johnson, Colin G. Jones, Adam C. Povey, Catherine E. Scott, Alistair Sellar, Steven T. Turnock, Matthew T. Woodhouse, Nathan Luke Abraham, Martin B. Andrews, Nicolas Bellouin, Jo Browse, Ken S. Carslaw, Mohit Dalvi, Gerd A. Folberth, Matthew Glover, Daniel P. Grosvenor, Catherine Hardacre, Richard Hill, Ben Johnson, Andy Jones, Zak Kipling, Graham Mann, James Mollard, Fiona M. O'Connor, Julien Palmiéri, Carly Reddington, Steven T. Rumbold, Mark Richardson, Nick A. J. Schutgens, Philip Stier, Marc Stringer, Yongming Tang, Jeremy Walton, Stephanie Woodward, and Andrew Yool
Geosci. Model Dev., 13, 6383–6423, https://doi.org/10.5194/gmd-13-6383-2020, https://doi.org/10.5194/gmd-13-6383-2020, 2020
Short summary
Short summary
Aerosols are an important component of the Earth system. Here, we comprehensively document and evaluate the aerosol schemes as implemented in the physical and Earth system models, HadGEM3-GC3.1 and UKESM1. This study provides a useful characterisation of the aerosol climatology in both models, facilitating the understanding of the numerous aerosol–climate interaction studies that will be conducted for CMIP6 and beyond.
Peng Xian, Philip J. Klotzbach, Jason P. Dunion, Matthew A. Janiga, Jeffrey S. Reid, Peter R. Colarco, and Zak Kipling
Atmos. Chem. Phys., 20, 15357–15378, https://doi.org/10.5194/acp-20-15357-2020, https://doi.org/10.5194/acp-20-15357-2020, 2020
Short summary
Short summary
Using dust AOD (DAOD) data from three aerosol reanalyses, we explored the correlative relationships between DAOD and multiple indices representing seasonal Atlantic TC activities. A robust negative correlation with Caribbean DAOD and Atlantic TC activity was found. We documented for the first time the regional differences of this relationship for over the Caribbean and the tropical North Atlantic. We also evaluated the impacts of potential confounding climate factors in this relationship.
Dimitris Akritidis, Eleni Katragkou, Aristeidis K. Georgoulias, Prodromos Zanis, Stergios Kartsios, Johannes Flemming, Antje Inness, John Douros, and Henk Eskes
Atmos. Chem. Phys., 20, 13557–13578, https://doi.org/10.5194/acp-20-13557-2020, https://doi.org/10.5194/acp-20-13557-2020, 2020
Short summary
Short summary
We assess the Copernicus Atmosphere Monitoring Service (CAMS) global and regional forecasts performance during a complex aerosol transport event over Europe induced by the passage of Storm Ophelia in mid-October 2017. Comparison with satellite observations reveals a satisfactory performance of CAMS global forecast assisted by data assimilation, while comparison with ground-based measurements indicates that the CAMS regional system over-performs compared to the global one in terms of air quality.
Augustin Mortier, Jonas Gliß, Michael Schulz, Wenche Aas, Elisabeth Andrews, Huisheng Bian, Mian Chin, Paul Ginoux, Jenny Hand, Brent Holben, Hua Zhang, Zak Kipling, Alf Kirkevåg, Paolo Laj, Thibault Lurton, Gunnar Myhre, David Neubauer, Dirk Olivié, Knut von Salzen, Ragnhild Bieltvedt Skeie, Toshihiko Takemura, and Simone Tilmes
Atmos. Chem. Phys., 20, 13355–13378, https://doi.org/10.5194/acp-20-13355-2020, https://doi.org/10.5194/acp-20-13355-2020, 2020
Short summary
Short summary
We present a multiparameter analysis of the aerosol trends over the last 2 decades in the different regions of the world. In most of the regions, ground-based observations show a decrease in aerosol content in both the total atmospheric column and at the surface. The use of climate models, assessed against these observations, reveals however an increase in the total aerosol load, which is not seen with the sole use of observation due to partial coverage in space and time.
Debbie O'Sullivan, Franco Marenco, Claire L. Ryder, Yaswant Pradhan, Zak Kipling, Ben Johnson, Angela Benedetti, Melissa Brooks, Matthew McGill, John Yorks, and Patrick Selmer
Atmos. Chem. Phys., 20, 12955–12982, https://doi.org/10.5194/acp-20-12955-2020, https://doi.org/10.5194/acp-20-12955-2020, 2020
Short summary
Short summary
Mineral dust is an important component of the climate system, and we assess how well it is predicted by two operational models. We flew an aircraft in the dust layers in the eastern Atlantic, and we also make use of satellites. We show that models predict the dust layer too low and that it predicts the particles to be too small. We believe that these discrepancies may be overcome if models can be constrained with operational observations of dust vertical and size-resolved distribution.
María A. Burgos, Elisabeth Andrews, Gloria Titos, Angela Benedetti, Huisheng Bian, Virginie Buchard, Gabriele Curci, Zak Kipling, Alf Kirkevåg, Harri Kokkola, Anton Laakso, Julie Letertre-Danczak, Marianne T. Lund, Hitoshi Matsui, Gunnar Myhre, Cynthia Randles, Michael Schulz, Twan van Noije, Kai Zhang, Lucas Alados-Arboledas, Urs Baltensperger, Anne Jefferson, James Sherman, Junying Sun, Ernest Weingartner, and Paul Zieger
Atmos. Chem. Phys., 20, 10231–10258, https://doi.org/10.5194/acp-20-10231-2020, https://doi.org/10.5194/acp-20-10231-2020, 2020
Short summary
Short summary
We investigate how well models represent the enhancement in scattering coefficients due to particle water uptake, and perform an evaluation of several implementation schemes used in ten Earth system models. Our results show the importance of the parameterization of hygroscopicity and model chemistry as drivers of some of the observed diversity amongst model estimates. The definition of dry conditions and the phenomena taking place in this relative humidity range also impact the model evaluation.
Alexander Ukhov, Suleiman Mostamandi, Arlindo da Silva, Johannes Flemming, Yasser Alshehri, Illia Shevchenko, and Georgiy Stenchikov
Atmos. Chem. Phys., 20, 9281–9310, https://doi.org/10.5194/acp-20-9281-2020, https://doi.org/10.5194/acp-20-9281-2020, 2020
Short summary
Short summary
The data assimilation products MERRA2 and CAMS are tested over the Middle East (ME) against in situ and satellite observations. For the first time, we compared the new MODIS aerosol optical depth (AOD) retrieval, MAIAC, with the Deep Blue and Dark Target MODIS AOD. We conducted 2-year high-resolution WRF-Chem simulations with the most accurate OMI-HTAP SO2 emissions to estimate the contribution of natural and anthropogenic aerosols to the PM pollution in the ME.
Joe R. McNorton, Nicolas Bousserez, Anna Agustí-Panareda, Gianpaolo Balsamo, Margarita Choulga, Andrew Dawson, Richard Engelen, Zak Kipling, and Simon Lang
Geosci. Model Dev., 13, 2297–2313, https://doi.org/10.5194/gmd-13-2297-2020, https://doi.org/10.5194/gmd-13-2297-2020, 2020
Short summary
Short summary
To infer carbon emissions from observations using atmospheric models, detailed knowledge of uncertainty is required. The uncertainties associated with models are often estimated because they are difficult to attribute. Here we use a state-of-the-art weather model to assess the impact of uncertainty in the wind fields on atmospheric concentrations of carbon dioxide. These results can be used to help quantify the uncertainty in estimated carbon emissions from atmospheric observations.
Zak Kipling, Laurent Labbouz, and Philip Stier
Atmos. Chem. Phys., 20, 4445–4460, https://doi.org/10.5194/acp-20-4445-2020, https://doi.org/10.5194/acp-20-4445-2020, 2020
Yuting Wang, Yong-Feng Ma, Henk Eskes, Antje Inness, Johannes Flemming, and Guy P. Brasseur
Atmos. Chem. Phys., 20, 4493–4521, https://doi.org/10.5194/acp-20-4493-2020, https://doi.org/10.5194/acp-20-4493-2020, 2020
Short summary
Short summary
The paper presents an evaluation of the CAMS global reanalysis of reactive gases performed for the period 2003–2016. The evaluation is performed by comparing concentrations of chemical species gathered during airborne field campaigns with calculated values. The reanalysis successfully reproduces the observed concentrations of ozone and carbon monoxide but generally underestimates the abundance of hydrocarbons. Large discrepancies exist for fast-reacting radicals such as OH and HO2.
Vincent Huijnen, Kazuyuki Miyazaki, Johannes Flemming, Antje Inness, Takashi Sekiya, and Martin G. Schultz
Geosci. Model Dev., 13, 1513–1544, https://doi.org/10.5194/gmd-13-1513-2020, https://doi.org/10.5194/gmd-13-1513-2020, 2020
Short summary
Short summary
We present the evaluation and intercomparison of global tropospheric ozone reanalyses that have been produced in recent years. Such reanalyses can be used to assess the current state and variability of tropospheric ozone.
The reanalyses show overall good agreements with independent ground and ozone-sonde observations for the diurnal, synoptical, seasonal, and interannual variabilities, with generally improved performances for the updated reanalyses.
Samuel Rémy, Zak Kipling, Johannes Flemming, Olivier Boucher, Pierre Nabat, Martine Michou, Alessio Bozzo, Melanie Ades, Vincent Huijnen, Angela Benedetti, Richard Engelen, Vincent-Henri Peuch, and Jean-Jacques Morcrette
Geosci. Model Dev., 12, 4627–4659, https://doi.org/10.5194/gmd-12-4627-2019, https://doi.org/10.5194/gmd-12-4627-2019, 2019
Short summary
Short summary
This article describes the IFS-AER aerosol module used operationally in the Integrated Forecasting System (IFS) cycle 45R1, operated by the ECMWF in the framework of the Copernicus Atmospheric Monitoring Services (CAMS). We describe the different parameterizations for aerosol sources, sinks, and how the aerosols are integrated in the larger atmospheric composition forecasting system. The skill of PM and AOD simulations against observations is improved compared to the older cycle 40R2.
Vincent Huijnen, Andrea Pozzer, Joaquim Arteta, Guy Brasseur, Idir Bouarar, Simon Chabrillat, Yves Christophe, Thierno Doumbia, Johannes Flemming, Jonathan Guth, Béatrice Josse, Vlassis A. Karydis, Virginie Marécal, and Sophie Pelletier
Geosci. Model Dev., 12, 1725–1752, https://doi.org/10.5194/gmd-12-1725-2019, https://doi.org/10.5194/gmd-12-1725-2019, 2019
Short summary
Short summary
We report on an evaluation of tropospheric ozone and its precursor gases in three atmospheric chemistry versions as implemented in ECMWF’s Integrated Forecasting System (IFS), referred to as IFS(CB05BASCOE), IFS(MOZART) and IFS(MOCAGE). This configuration of having various chemistry versions within IFS provides a quantification of uncertainties in CAMS trace gas products that are induced by chemistry modelling.
Anna Katinka Petersen, Guy P. Brasseur, Idir Bouarar, Johannes Flemming, Michael Gauss, Fei Jiang, Rostislav Kouznetsov, Richard Kranenburg, Bas Mijling, Vincent-Henri Peuch, Matthieu Pommier, Arjo Segers, Mikhail Sofiev, Renske Timmermans, Ronald van der A, Stacy Walters, Ying Xie, Jianming Xu, and Guangqiang Zhou
Geosci. Model Dev., 12, 1241–1266, https://doi.org/10.5194/gmd-12-1241-2019, https://doi.org/10.5194/gmd-12-1241-2019, 2019
Short summary
Short summary
An operational multi-model forecasting system for air quality is providing daily forecasts of ozone, nitrogen oxides, and particulate matter for 37 urban areas of China. The paper presents the evaluation of the different forecasts performed during the first year of operation.
Antje Inness, Melanie Ades, Anna Agustí-Panareda, Jérôme Barré, Anna Benedictow, Anne-Marlene Blechschmidt, Juan Jose Dominguez, Richard Engelen, Henk Eskes, Johannes Flemming, Vincent Huijnen, Luke Jones, Zak Kipling, Sebastien Massart, Mark Parrington, Vincent-Henri Peuch, Miha Razinger, Samuel Remy, Michael Schulz, and Martin Suttie
Atmos. Chem. Phys., 19, 3515–3556, https://doi.org/10.5194/acp-19-3515-2019, https://doi.org/10.5194/acp-19-3515-2019, 2019
Short summary
Short summary
This paper describes a new global dataset of atmospheric composition data for the years 2003-2016 that has been produced by the Copernicus Atmosphere Monitoring Service (CAMS). It is called the CAMS reanalysis and provides information on aerosols and reactive gases. The CAMS reanalysis shows an improved performance compared to our previous atmospheric composition reanalyses; has smaller biases compared to independent O3, CO, NO2 and aerosol observations; and is more consistent in time.
Jeronimo Escribano, Alessio Bozzo, Philippe Dubuisson, Johannes Flemming, Robin J. Hogan, Laurent C.-Labonnote, and Olivier Boucher
Geosci. Model Dev., 12, 805–827, https://doi.org/10.5194/gmd-12-805-2019, https://doi.org/10.5194/gmd-12-805-2019, 2019
Short summary
Short summary
Accurate shortwave radiance computations are becoming increasingly important for some applications in atmospheric composition. In this work we propose a benchmark protocol and dataset to asses the accuracy and computing runtime of radiance calculations of radiative transfer models. It is applied to four models, showing the potential of this benchmark to evaluate the model performance under a variety of atmospheric conditions, viewing geometries, aerosol loading, and optical properties.
Angela Benedetti, Francesca Di Giuseppe, Luke Jones, Vincent-Henri Peuch, Samuel Rémy, and Xiaoye Zhang
Atmos. Chem. Phys., 19, 987–998, https://doi.org/10.5194/acp-19-987-2019, https://doi.org/10.5194/acp-19-987-2019, 2019
Guy P. Brasseur, Ying Xie, Anna Katinka Petersen, Idir Bouarar, Johannes Flemming, Michael Gauss, Fei Jiang, Rostislav Kouznetsov, Richard Kranenburg, Bas Mijling, Vincent-Henri Peuch, Matthieu Pommier, Arjo Segers, Mikhail Sofiev, Renske Timmermans, Ronald van der A, Stacy Walters, Jianming Xu, and Guangqiang Zhou
Geosci. Model Dev., 12, 33–67, https://doi.org/10.5194/gmd-12-33-2019, https://doi.org/10.5194/gmd-12-33-2019, 2019
Short summary
Short summary
An operational multi-model forecasting system for air quality provides daily forecasts of ozone, nitrogen oxides, and particulate matter for 37 urban areas in China. The paper presents an intercomparison of the different forecasts performed during a specific period of time and highlights recurrent differences between the model output. Pathways to improve the forecasts by the multi-model system are suggested.
Samuel R. Hall, Kirk Ullmann, Michael J. Prather, Clare M. Flynn, Lee T. Murray, Arlene M. Fiore, Gustavo Correa, Sarah A. Strode, Stephen D. Steenrod, Jean-Francois Lamarque, Jonathan Guth, Béatrice Josse, Johannes Flemming, Vincent Huijnen, N. Luke Abraham, and Alex T. Archibald
Atmos. Chem. Phys., 18, 16809–16828, https://doi.org/10.5194/acp-18-16809-2018, https://doi.org/10.5194/acp-18-16809-2018, 2018
Short summary
Short summary
Photolysis (J rates) initiates and drives atmospheric chemistry, and Js are perturbed by factors of 2 by clouds. The NASA Atmospheric Tomography (ATom) Mission provides the first comprehensive observations on how clouds perturb Js through the remote Pacific and Atlantic basins. We compare these cloud-perturbation J statistics with those from nine global chemistry models. While basic patterns agree, there is a large spread across models, and all lack some basic features of the observations.
Dimitris Akritidis, Eleni Katragkou, Prodromos Zanis, Ioannis Pytharoulis, Dimitris Melas, Johannes Flemming, Antje Inness, Hannah Clark, Matthieu Plu, and Henk Eskes
Atmos. Chem. Phys., 18, 15515–15534, https://doi.org/10.5194/acp-18-15515-2018, https://doi.org/10.5194/acp-18-15515-2018, 2018
Short summary
Short summary
Analysis and evaluation of the Copernicus Atmosphere Monitoring Service (CAMS) global and regional forecast systems during a deep stratosphere-to-troposphere ozone transport event over Europe in January 2017. Radiosondes, satellite images, ozonesondes and aircraft measurements were used to investigate the folding of the tropopause at several European sites and the induced presence of dry and ozone-rich air in the troposphere.
Jan Eiof Jonson, Michael Schulz, Louisa Emmons, Johannes Flemming, Daven Henze, Kengo Sudo, Marianne Tronstad Lund, Meiyun Lin, Anna Benedictow, Brigitte Koffi, Frank Dentener, Terry Keating, Rigel Kivi, and Yanko Davila
Atmos. Chem. Phys., 18, 13655–13672, https://doi.org/10.5194/acp-18-13655-2018, https://doi.org/10.5194/acp-18-13655-2018, 2018
Short summary
Short summary
Focusing on Europe, this HTAP 2 study computes ozone in several global models when reducing anthropogenic emissions by 20 % in different world regions. The differences in model results are explored
by use of a novel stepwise approach combining a tracer, CO and ozone. For ozone the contributions from the rest of the world are larger than from Europe, with the largest contributions from North America and eastern Asia. Contributions do, however, depend on the choice of ozone metric.
Angela Benedetti, Jeffrey S. Reid, Peter Knippertz, John H. Marsham, Francesca Di Giuseppe, Samuel Rémy, Sara Basart, Olivier Boucher, Ian M. Brooks, Laurent Menut, Lucia Mona, Paolo Laj, Gelsomina Pappalardo, Alfred Wiedensohler, Alexander Baklanov, Malcolm Brooks, Peter R. Colarco, Emilio Cuevas, Arlindo da Silva, Jeronimo Escribano, Johannes Flemming, Nicolas Huneeus, Oriol Jorba, Stelios Kazadzis, Stefan Kinne, Thomas Popp, Patricia K. Quinn, Thomas T. Sekiyama, Taichu Tanaka, and Enric Terradellas
Atmos. Chem. Phys., 18, 10615–10643, https://doi.org/10.5194/acp-18-10615-2018, https://doi.org/10.5194/acp-18-10615-2018, 2018
Short summary
Short summary
Numerical prediction of aerosol particle properties has become an important activity at many research and operational weather centers. This development is due to growing interest from a diverse set of stakeholders, such as air quality regulatory bodies, aviation authorities, solar energy plant managers, climate service providers, and health professionals. This paper describes the advances in the field and sets out requirements for observations for the sustainability of these activities.
Ciao-Kai Liang, J. Jason West, Raquel A. Silva, Huisheng Bian, Mian Chin, Yanko Davila, Frank J. Dentener, Louisa Emmons, Johannes Flemming, Gerd Folberth, Daven Henze, Ulas Im, Jan Eiof Jonson, Terry J. Keating, Tom Kucsera, Allen Lenzen, Meiyun Lin, Marianne Tronstad Lund, Xiaohua Pan, Rokjin J. Park, R. Bradley Pierce, Takashi Sekiya, Kengo Sudo, and Toshihiko Takemura
Atmos. Chem. Phys., 18, 10497–10520, https://doi.org/10.5194/acp-18-10497-2018, https://doi.org/10.5194/acp-18-10497-2018, 2018
Short summary
Short summary
Emissions from one continent affect air quality and health elsewhere. Here we quantify the effects of intercontinental PM2.5 and ozone transport on human health using a new multi-model ensemble, evaluating the health effects of emissions from six world regions and three emission source sectors. Emissions from one region have significant health impacts outside of that source region; similarly, foreign emissions contribute significantly to air-pollution-related deaths in several world regions.
Marta G. Vivanco, Mark R. Theobald, Héctor García-Gómez, Juan Luis Garrido, Marje Prank, Wenche Aas, Mario Adani, Ummugulsum Alyuz, Camilla Andersson, Roberto Bellasio, Bertrand Bessagnet, Roberto Bianconi, Johannes Bieser, Jørgen Brandt, Gino Briganti, Andrea Cappelletti, Gabriele Curci, Jesper H. Christensen, Augustin Colette, Florian Couvidat, Cornelis Cuvelier, Massimo D'Isidoro, Johannes Flemming, Andrea Fraser, Camilla Geels, Kaj M. Hansen, Christian Hogrefe, Ulas Im, Oriol Jorba, Nutthida Kitwiroon, Astrid Manders, Mihaela Mircea, Noelia Otero, Maria-Teresa Pay, Luca Pozzoli, Efisio Solazzo, Svetlana Tsyro, Alper Unal, Peter Wind, and Stefano Galmarini
Atmos. Chem. Phys., 18, 10199–10218, https://doi.org/10.5194/acp-18-10199-2018, https://doi.org/10.5194/acp-18-10199-2018, 2018
Short summary
Short summary
European wet and dry atmospheric deposition of N and S estimated by 14 air quality models was found to vary substantially. An ensemble of models meeting acceptability criteria was used to estimate the exceedances of the critical loads for N in habitats within the Natura 2000 network, as well as their lower and upper limits. Scenarios with 20 % emission reductions in different regions of the world showed that European emissions are responsible for most of the N and S deposition in Europe.
Steven T. Turnock, Oliver Wild, Frank J. Dentener, Yanko Davila, Louisa K. Emmons, Johannes Flemming, Gerd A. Folberth, Daven K. Henze, Jan E. Jonson, Terry J. Keating, Sudo Kengo, Meiyun Lin, Marianne Lund, Simone Tilmes, and Fiona M. O'Connor
Atmos. Chem. Phys., 18, 8953–8978, https://doi.org/10.5194/acp-18-8953-2018, https://doi.org/10.5194/acp-18-8953-2018, 2018
Short summary
Short summary
A simple parameterisation was developed in this study to provide a rapid assessment of the impacts and uncertainties associated with future emission control strategies by predicting changes to surface ozone air quality and near-term climate forcing of ozone. Future emissions scenarios based on currently implemented legislation are shown to worsen surface ozone air quality and enhance near-term climate warming, with changes in methane becoming increasingly important in the future.
Ulas Im, Jesper Heile Christensen, Camilla Geels, Kaj Mantzius Hansen, Jørgen Brandt, Efisio Solazzo, Ummugulsum Alyuz, Alessandra Balzarini, Rocio Baro, Roberto Bellasio, Roberto Bianconi, Johannes Bieser, Augustin Colette, Gabriele Curci, Aidan Farrow, Johannes Flemming, Andrea Fraser, Pedro Jimenez-Guerrero, Nutthida Kitwiroon, Peng Liu, Uarporn Nopmongcol, Laura Palacios-Peña, Guido Pirovano, Luca Pozzoli, Marje Prank, Rebecca Rose, Ranjeet Sokhi, Paolo Tuccella, Alper Unal, Marta G. Vivanco, Greg Yarwood, Christian Hogrefe, and Stefano Galmarini
Atmos. Chem. Phys., 18, 8929–8952, https://doi.org/10.5194/acp-18-8929-2018, https://doi.org/10.5194/acp-18-8929-2018, 2018
Short summary
Short summary
We evaluate the impact of global and regional anthropogenic emission reductions on major air pollutant levels over Europe and North America, using a multi-model ensemble of regional chemistry and transport models. Results show that ozone levels are largely driven by long-range transport over both continents while other pollutants such as carbon monoxide or aerosols are mainly controlled by domestic sources. Use of multi-model ensembles can help to reduce the uncertainties in individual models.
Aristeidis K. Georgoulias, Athanasios Tsikerdekis, Vassilis Amiridis, Eleni Marinou, Angela Benedetti, Prodromos Zanis, Georgia Alexandri, Lucia Mona, Konstantinos A. Kourtidis, and Jos Lelieveld
Atmos. Chem. Phys., 18, 8601–8620, https://doi.org/10.5194/acp-18-8601-2018, https://doi.org/10.5194/acp-18-8601-2018, 2018
Short summary
Short summary
In this work, the MACC reanalysis dust product is evaluated over Europe, Northern Africa and the Middle East using the EARLINET-optimized CALIOP/CALIPSO pure dust satellite-based product LIVAS (2007–2012). As dust plays a determinant role in processes related to weather and climate, human healt, and the economy, it is obvious that adequately simulating the amount of dust and its optical properties is essential. Our results could be used as a reference in future climate model evaluations.
Ulas Im, Jørgen Brandt, Camilla Geels, Kaj Mantzius Hansen, Jesper Heile Christensen, Mikael Skou Andersen, Efisio Solazzo, Ioannis Kioutsioukis, Ummugulsum Alyuz, Alessandra Balzarini, Rocio Baro, Roberto Bellasio, Roberto Bianconi, Johannes Bieser, Augustin Colette, Gabriele Curci, Aidan Farrow, Johannes Flemming, Andrea Fraser, Pedro Jimenez-Guerrero, Nutthida Kitwiroon, Ciao-Kai Liang, Uarporn Nopmongcol, Guido Pirovano, Luca Pozzoli, Marje Prank, Rebecca Rose, Ranjeet Sokhi, Paolo Tuccella, Alper Unal, Marta Garcia Vivanco, Jason West, Greg Yarwood, Christian Hogrefe, and Stefano Galmarini
Atmos. Chem. Phys., 18, 5967–5989, https://doi.org/10.5194/acp-18-5967-2018, https://doi.org/10.5194/acp-18-5967-2018, 2018
Short summary
Short summary
The impacts of air pollution on human health and their costs in Europe and the United States for the year 2010 ared modeled by a multi-model ensemble. In Europe, the number of premature deaths is calculated to be 414 000, while in the US it is estimated to be 160 000. Health impacts estimated by individual models can vary up to a factor of 3. Results show that the domestic emissions have the largest impact on premature deaths, compared to foreign sources.
Francesca Di Giuseppe, Samuel Rémy, Florian Pappenberger, and Fredrik Wetterhall
Atmos. Chem. Phys., 18, 5359–5370, https://doi.org/10.5194/acp-18-5359-2018, https://doi.org/10.5194/acp-18-5359-2018, 2018
Short summary
Short summary
Fire emissions injected into the atmosphere are crucial input for air quality models. This information is available globally using fire radiative power (FRP) observations, converted into smoke constituents. In case of a missing observation after ignition, a practical choice is to assume persistence. As an improvement we propose the use of the Canadian Fire Weather Index (FWI) to predict the FRP evolution. We show that the FWI is able to capture weather-related changes in fire activity well.
Christian Hogrefe, Peng Liu, George Pouliot, Rohit Mathur, Shawn Roselle, Johannes Flemming, Meiyun Lin, and Rokjin J. Park
Atmos. Chem. Phys., 18, 3839–3864, https://doi.org/10.5194/acp-18-3839-2018, https://doi.org/10.5194/acp-18-3839-2018, 2018
Short summary
Short summary
This study quantifies the impacts of different representations of background ozone in state-of-the-science large-scale models on surface and aloft ozone burdens simulated by the CMAQ regional model over the United States. It also compares both the CMAQ simulations and the driving large-scale models to surface and upper air observations.
Albert Ansmann, Franziska Rittmeister, Ronny Engelmann, Sara Basart, Oriol Jorba, Christos Spyrou, Samuel Remy, Annett Skupin, Holger Baars, Patric Seifert, Fabian Senf, and Thomas Kanitz
Atmos. Chem. Phys., 17, 14987–15006, https://doi.org/10.5194/acp-17-14987-2017, https://doi.org/10.5194/acp-17-14987-2017, 2017
Bethan White, Edward Gryspeerdt, Philip Stier, Hugh Morrison, Gregory Thompson, and Zak Kipling
Atmos. Chem. Phys., 17, 12145–12175, https://doi.org/10.5194/acp-17-12145-2017, https://doi.org/10.5194/acp-17-12145-2017, 2017
Short summary
Short summary
Aerosols influence cloud and precipitation by modifying cloud droplet number concentrations (CDNCs). We simulate three different types of convective cloud using two different cloud microphysics parameterisations. The simulated cloud and precipitation depends much more strongly on the choice of microphysics scheme than on CDNC. The uncertainty differs between types of convection. Our results highlight a large uncertainty in cloud and precipitation responses to aerosol in current models.
Min Huang, Gregory R. Carmichael, R. Bradley Pierce, Duseong S. Jo, Rokjin J. Park, Johannes Flemming, Louisa K. Emmons, Kevin W. Bowman, Daven K. Henze, Yanko Davila, Kengo Sudo, Jan Eiof Jonson, Marianne Tronstad Lund, Greet Janssens-Maenhout, Frank J. Dentener, Terry J. Keating, Hilke Oetjen, and Vivienne H. Payne
Atmos. Chem. Phys., 17, 5721–5750, https://doi.org/10.5194/acp-17-5721-2017, https://doi.org/10.5194/acp-17-5721-2017, 2017
Short summary
Short summary
In support of the HTAP phase 2 experiment, we conducted a number of regional-scale Sulfur Transport and dEposition Model base and sensitivity simulations over North America during May–June 2010. The STEM chemical boundary conditions were downscaled from three (GEOS-Chem, RAQMS, and ECMWF C-IFS) global chemical transport models' simulations. Analyses were performed on large spatial–temporal scales relative to HTAP1 and also on subcontinental and event scales including the use of satellite data.
Samuel Rémy, Andreas Veira, Ronan Paugam, Mikhail Sofiev, Johannes W. Kaiser, Franco Marenco, Sharon P. Burton, Angela Benedetti, Richard J. Engelen, Richard Ferrare, and Jonathan W. Hair
Atmos. Chem. Phys., 17, 2921–2942, https://doi.org/10.5194/acp-17-2921-2017, https://doi.org/10.5194/acp-17-2921-2017, 2017
Short summary
Short summary
Biomass burning emission injection heights are an important source of uncertainty in global climate and atmospheric composition modelling. This work provides a global daily data set of injection heights computed by two very different algorithms, which coherently complete a global biomass burning emissions database. The two data sets were compared and validated against observations, and their use was found to improve forecasts of carbonaceous aerosols in two case studies.
Johannes Flemming, Angela Benedetti, Antje Inness, Richard J. Engelen, Luke Jones, Vincent Huijnen, Samuel Remy, Mark Parrington, Martin Suttie, Alessio Bozzo, Vincent-Henri Peuch, Dimitris Akritidis, and Eleni Katragkou
Atmos. Chem. Phys., 17, 1945–1983, https://doi.org/10.5194/acp-17-1945-2017, https://doi.org/10.5194/acp-17-1945-2017, 2017
Short summary
Short summary
We combine satellite observations of carbon monoxide, ozone and aerosols with the results from a model using a technique called data assimilation. The generated global data set (CAMS interim reanalysis) covers the period 2003–2015 at a resolution of about 110 km. The CAMS interim reanalysis can be used to study global air pollution and climate forcing of aerosol and stratospheric ozone. It has been produced by the Copernicus Atmosphere Monitoring Service (http://atmosphere. copernicus.eu).
Zak Kipling, Philip Stier, Laurent Labbouz, and Till Wagner
Atmos. Chem. Phys., 17, 327–342, https://doi.org/10.5194/acp-17-327-2017, https://doi.org/10.5194/acp-17-327-2017, 2017
Short summary
Short summary
We present the first evaluation of the convective cloud field model (CCFM) in the context of a global climate model. CCFM attempts to address some of the shortcomings of commonly used representations of convection, in particular allowing for physically based aerosol effects on different types of convective cloud. We show that the model performs well overall in the context of the climate model and is thus well placed to study aerosol–convection–climate interactions at the global scale.
Ioannis Kioutsioukis, Ulas Im, Efisio Solazzo, Roberto Bianconi, Alba Badia, Alessandra Balzarini, Rocío Baró, Roberto Bellasio, Dominik Brunner, Charles Chemel, Gabriele Curci, Hugo Denier van der Gon, Johannes Flemming, Renate Forkel, Lea Giordano, Pedro Jiménez-Guerrero, Marcus Hirtl, Oriol Jorba, Astrid Manders-Groot, Lucy Neal, Juan L. Pérez, Guidio Pirovano, Roberto San Jose, Nicholas Savage, Wolfram Schroder, Ranjeet S. Sokhi, Dimiter Syrakov, Paolo Tuccella, Johannes Werhahn, Ralf Wolke, Christian Hogrefe, and Stefano Galmarini
Atmos. Chem. Phys., 16, 15629–15652, https://doi.org/10.5194/acp-16-15629-2016, https://doi.org/10.5194/acp-16-15629-2016, 2016
Short summary
Short summary
Four ensemble methods are applied to two annual AQMEII datasets and their performance is compared for O3, NO2 and PM10. The goal of the study is to quantify to what extent we can extract predictable signals from an ensemble with superior skill at each station over the single models and the ensemble mean. The promotion of the right amount of accuracy and diversity within the ensemble results in an average additional skill of up to 31 % compared to using the full ensemble in an unconditional way.
Fernando Chouza, Oliver Reitebuch, Angela Benedetti, and Bernadett Weinzierl
Atmos. Chem. Phys., 16, 11581–11600, https://doi.org/10.5194/acp-16-11581-2016, https://doi.org/10.5194/acp-16-11581-2016, 2016
Duncan Watson-Parris, Nick Schutgens, Nicholas Cook, Zak Kipling, Philip Kershaw, Edward Gryspeerdt, Bryan Lawrence, and Philip Stier
Geosci. Model Dev., 9, 3093–3110, https://doi.org/10.5194/gmd-9-3093-2016, https://doi.org/10.5194/gmd-9-3093-2016, 2016
Short summary
Short summary
In this paper we describe CIS, a new command line tool for the easy visualization, analysis and comparison of a wide variety of gridded and ungridded data sets used in Earth sciences. Users can now use a single tool to not only view plots of satellite, aircraft, station or model data, but also bring them onto the same spatio-temporal sampling. This allows robust, quantitative comparisons to be made easily. CIS is an open-source project and welcomes input from the community.
Vincent Huijnen, Johannes Flemming, Simon Chabrillat, Quentin Errera, Yves Christophe, Anne-Marlene Blechschmidt, Andreas Richter, and Henk Eskes
Geosci. Model Dev., 9, 3071–3091, https://doi.org/10.5194/gmd-9-3071-2016, https://doi.org/10.5194/gmd-9-3071-2016, 2016
Short summary
Short summary
We present a model description and benchmark evaluation of an extension of the tropospheric chemistry module in the ECMWF Integrated Forecasting System (IFS) with stratospheric chemistry. The stratospheric chemistry originates from the one used in the Belgian Assimilation System for Chemical ObsErvations (BASCOE), and is here combined with the modified CB05 chemistry module for the troposphere as currently used operationally in the Copernicus Atmosphere Monitoring Service (CAMS).
Jianglong Zhang, Jeffrey S. Reid, Matthew Christensen, and Angela Benedetti
Atmos. Chem. Phys., 16, 6475–6494, https://doi.org/10.5194/acp-16-6475-2016, https://doi.org/10.5194/acp-16-6475-2016, 2016
Short summary
Short summary
Through analyzing a smoke aerosol event over the Midwestern USA, the potential impacts of aerosol particles on model/weather-station-forecasted surface temperatures are studied, and for the first time, smoke-aerosol-induced surface cooling is investigated as a function of observed aerosol properties and multiple operational models over a large network of ground stations. The potential issues of incorporating aerosol models into weather models for forecasting surface temperatures are explored.
N. Huneeus, S. Basart, S. Fiedler, J.-J. Morcrette, A. Benedetti, J. Mulcahy, E. Terradellas, C. Pérez García-Pando, G. Pejanovic, S. Nickovic, P. Arsenovic, M. Schulz, E. Cuevas, J. M. Baldasano, J. Pey, S. Remy, and B. Cvetkovic
Atmos. Chem. Phys., 16, 4967–4986, https://doi.org/10.5194/acp-16-4967-2016, https://doi.org/10.5194/acp-16-4967-2016, 2016
Short summary
Short summary
Five dust models are evaluated regarding their performance in predicting an intense Saharan dust outbreak affecting western and northern Europe (NE). Models predict the onset and evolution of the event for all analysed lead times. On average, differences among the models are larger than differences in lead times for each model. The models tend to underestimate the long-range transport towards NE. This is partly due to difficulties in simulating the vertical dust distribution and horizontal wind.
Shipeng Zhang, Minghuai Wang, Steven J. Ghan, Aijun Ding, Hailong Wang, Kai Zhang, David Neubauer, Ulrike Lohmann, Sylvaine Ferrachat, Toshihiko Takeamura, Andrew Gettelman, Hugh Morrison, Yunha Lee, Drew T. Shindell, Daniel G. Partridge, Philip Stier, Zak Kipling, and Congbin Fu
Atmos. Chem. Phys., 16, 2765–2783, https://doi.org/10.5194/acp-16-2765-2016, https://doi.org/10.5194/acp-16-2765-2016, 2016
Short summary
Short summary
The variation of aerosol indirect effects (AIE) in several climate models is investigated across different dynamical regimes. Regimes with strong large-scale ascent are shown to be as important as stratocumulus regimes in studying AIE. AIE over regions with high monthly large-scale surface precipitation rate contributes the most to the total aerosol indirect forcing. These results point to the need to reduce the uncertainty in AIE in different dynamical regimes.
Zak Kipling, Philip Stier, Colin E. Johnson, Graham W. Mann, Nicolas Bellouin, Susanne E. Bauer, Tommi Bergman, Mian Chin, Thomas Diehl, Steven J. Ghan, Trond Iversen, Alf Kirkevåg, Harri Kokkola, Xiaohong Liu, Gan Luo, Twan van Noije, Kirsty J. Pringle, Knut von Salzen, Michael Schulz, Øyvind Seland, Ragnhild B. Skeie, Toshihiko Takemura, Kostas Tsigaridis, and Kai Zhang
Atmos. Chem. Phys., 16, 2221–2241, https://doi.org/10.5194/acp-16-2221-2016, https://doi.org/10.5194/acp-16-2221-2016, 2016
Short summary
Short summary
The vertical distribution of atmospheric aerosol is an important factor in its effects on climate. In this study we use a sophisticated model of the many interacting processes affecting aerosol in the atmosphere to show that the vertical distribution is typically dominated by only a few of these processes. Constraining these physical processes may help to reduce the large differences between models. However, the important processes are not always the same for different types of aerosol.
Franco Marenco, Ben Johnson, Justin M. Langridge, Jane Mulcahy, Angela Benedetti, Samuel Remy, Luke Jones, Kate Szpek, Jim Haywood, Karla Longo, and Paulo Artaxo
Atmos. Chem. Phys., 16, 2155–2174, https://doi.org/10.5194/acp-16-2155-2016, https://doi.org/10.5194/acp-16-2155-2016, 2016
Short summary
Short summary
A widespread and persistent smoke layer was observed in the Amazon
region during the biomass burning season, spanning a distance of 2200 km
and a period of 14 days. The larger smoke content was typically found
in elevated layers, from 1–1.5 km to 4–6 km.
Measurements have been compared to model predictions, and the latter
were able to reproduce the general features of the smoke layer, but
with some differences which are analysed and described in the paper.
A. Wagner, A.-M. Blechschmidt, I. Bouarar, E.-G. Brunke, C. Clerbaux, M. Cupeiro, P. Cristofanelli, H. Eskes, J. Flemming, H. Flentje, M. George, S. Gilge, A. Hilboll, A. Inness, J. Kapsomenakis, A. Richter, L. Ries, W. Spangl, O. Stein, R. Weller, and C. Zerefos
Atmos. Chem. Phys., 15, 14005–14030, https://doi.org/10.5194/acp-15-14005-2015, https://doi.org/10.5194/acp-15-14005-2015, 2015
Short summary
Short summary
The Monitoring Atmospheric Composition and Climate project (MACC) operationally produces global analyses and forecasts of reactive gases and aerosol fields. We have investigated the ability of the model to simulate concentrations of reactive gases (carbon monoxide, nitrogen dioxide and ozone) between 2009 and 2012. The model reproduced reactive gas concentrations with consistent quality, however, with a seasonally dependent bias compared to surface and satellite observations.
G. Roberts, M. J. Wooster, W. Xu, P. H. Freeborn, J.-J. Morcrette, L. Jones, A. Benedetti, H. Jiangping, D. Fisher, and J. W. Kaiser
Atmos. Chem. Phys., 15, 13241–13267, https://doi.org/10.5194/acp-15-13241-2015, https://doi.org/10.5194/acp-15-13241-2015, 2015
Short summary
Short summary
Characterising the dynamics of wildfires at high temporal resolution is best achieved using observations from geostationary satellite sensors. The SEVIRI Fire Radiative Power (FRP) products have been developed using such imagery at up to 15-minute temporal frequency. These data are used to estimate wildfire fuel consumption and to the characterise smoke emissions from the 2007 Peloponnese "mega fires" within an atmospheric transport model.
S. Rémy, A. Benedetti, A. Bozzo, T. Haiden, L. Jones, M. Razinger, J. Flemming, R. J. Engelen, V. H. Peuch, and J. N. Thepaut
Atmos. Chem. Phys., 15, 12909–12933, https://doi.org/10.5194/acp-15-12909-2015, https://doi.org/10.5194/acp-15-12909-2015, 2015
Short summary
Short summary
In this paper we report on the feedbacks between dust and boundary layer meteorology during a dust storm over Egypt and Libya in April 2012, using an atmospheric composition forecasting system. Dust was found to act on atmospheric stability, leading to an increase (night) or a decrease (day) in dust production. Horizontal gradients of temperature were modified by the radiative impact of the dust layer, leading to changes in wind patterns at the edge of the storm due to the thermal wind effect.
A. Inness, A. Benedetti, J. Flemming, V. Huijnen, J. W. Kaiser, M. Parrington, and S. Remy
Atmos. Chem. Phys., 15, 9083–9097, https://doi.org/10.5194/acp-15-9083-2015, https://doi.org/10.5194/acp-15-9083-2015, 2015
E. Katragkou, P. Zanis, A. Tsikerdekis, J. Kapsomenakis, D. Melas, H. Eskes, J. Flemming, V. Huijnen, A. Inness, M. G. Schultz, O. Stein, and C. S. Zerefos
Geosci. Model Dev., 8, 2299–2314, https://doi.org/10.5194/gmd-8-2299-2015, https://doi.org/10.5194/gmd-8-2299-2015, 2015
Short summary
Short summary
This work is an extended evaluation of near-surface ozone as part of the global reanalysis of atmospheric composition, produced within the European-funded project MACC (Monitoring Atmospheric Composition and Climate). It includes an evaluation over the period 2003-2012 and provides an overall assessment of the modelling system performance with respect to near surface ozone for specific European subregions.
E. Gryspeerdt, P. Stier, B. A. White, and Z. Kipling
Atmos. Chem. Phys., 15, 7557–7570, https://doi.org/10.5194/acp-15-7557-2015, https://doi.org/10.5194/acp-15-7557-2015, 2015
Short summary
Short summary
Wet scavenging generates differences between the aerosol properties in clear-sky scenes (observed by satellites) and cloudy scenes, leading to different
aerosol-precipitation relationships in satellite data and global models. Convective systems usually draw in air from clear-sky regions, but global models have difficulty separating this aerosol from the aerosol in cloudy scenes within a model gridbox. This may prevent models from reproducing the observed aerosol-precipitation relationships.
L. K. Emmons, S. R. Arnold, S. A. Monks, V. Huijnen, S. Tilmes, K. S. Law, J. L. Thomas, J.-C. Raut, I. Bouarar, S. Turquety, Y. Long, B. Duncan, S. Steenrod, S. Strode, J. Flemming, J. Mao, J. Langner, A. M. Thompson, D. Tarasick, E. C. Apel, D. R. Blake, R. C. Cohen, J. Dibb, G. S. Diskin, A. Fried, S. R. Hall, L. G. Huey, A. J. Weinheimer, A. Wisthaler, T. Mikoviny, J. Nowak, J. Peischl, J. M. Roberts, T. Ryerson, C. Warneke, and D. Helmig
Atmos. Chem. Phys., 15, 6721–6744, https://doi.org/10.5194/acp-15-6721-2015, https://doi.org/10.5194/acp-15-6721-2015, 2015
Short summary
Short summary
Eleven 3-D tropospheric chemistry models have been compared and evaluated with observations in the Arctic during the International Polar Year (IPY 2008). Large differences are seen among the models, particularly related to the model chemistry of volatile organic compounds (VOCs) and reactive nitrogen (NOx, PAN, HNO3) partitioning. Consistency among the models in the underestimation of CO, ethane and propane indicates the emission inventory is too low for these compounds.
S. R. Arnold, L. K. Emmons, S. A. Monks, K. S. Law, D. A. Ridley, S. Turquety, S. Tilmes, J. L. Thomas, I. Bouarar, J. Flemming, V. Huijnen, J. Mao, B. N. Duncan, S. Steenrod, Y. Yoshida, J. Langner, and Y. Long
Atmos. Chem. Phys., 15, 6047–6068, https://doi.org/10.5194/acp-15-6047-2015, https://doi.org/10.5194/acp-15-6047-2015, 2015
Short summary
Short summary
The extent to which forest fires produce the air pollutant and greenhouse gas ozone (O3) in the atmosphere at high latitudes in not well understood. We have compared how fire emissions produce O3 and its precursors in several models of atmospheric chemistry. We find enhancements in O3 in air dominated by fires in all models, which increase on average as fire emissions age. We also find that in situ O3 production in the Arctic is sensitive to details of organic chemistry and vertical lifting.
M. Bocquet, H. Elbern, H. Eskes, M. Hirtl, R. Žabkar, G. R. Carmichael, J. Flemming, A. Inness, M. Pagowski, J. L. Pérez Camaño, P. E. Saide, R. San Jose, M. Sofiev, J. Vira, A. Baklanov, C. Carnevale, G. Grell, and C. Seigneur
Atmos. Chem. Phys., 15, 5325–5358, https://doi.org/10.5194/acp-15-5325-2015, https://doi.org/10.5194/acp-15-5325-2015, 2015
Short summary
Short summary
Data assimilation is used in atmospheric chemistry models to improve air quality forecasts, construct re-analyses of concentrations, and perform inverse modeling. Coupled chemistry meteorology models (CCMM) are atmospheric chemistry models that simulate meteorological processes and chemical transformations jointly. We review here the current status of data assimilation in atmospheric chemistry models, with a particular focus on future prospects for data assimilation in CCMM.
A. Inness, A.-M. Blechschmidt, I. Bouarar, S. Chabrillat, M. Crepulja, R. J. Engelen, H. Eskes, J. Flemming, A. Gaudel, F. Hendrick, V. Huijnen, L. Jones, J. Kapsomenakis, E. Katragkou, A. Keppens, B. Langerock, M. de Mazière, D. Melas, M. Parrington, V. H. Peuch, M. Razinger, A. Richter, M. G. Schultz, M. Suttie, V. Thouret, M. Vrekoussis, A. Wagner, and C. Zerefos
Atmos. Chem. Phys., 15, 5275–5303, https://doi.org/10.5194/acp-15-5275-2015, https://doi.org/10.5194/acp-15-5275-2015, 2015
Short summary
Short summary
The paper presents results from data assimilation studies with the new Composition-IFS model developed in the MACC project. This system was used in MACC to produce daily analyses and 5-day forecasts of atmospheric composition and is now run daily in the EU’s Copernicus Atmosphere Monitoring Service. The paper looks at the quality of the CO, O3 and NO2 analysis fields obtained with this system, comparing them against observations, a control run and an older version of the model.
E. Cuevas, C. Camino, A. Benedetti, S. Basart, E. Terradellas, J. M. Baldasano, J. J. Morcrette, B. Marticorena, P. Goloub, A. Mortier, A. Berjón, Y. Hernández, M. Gil-Ojeda, and M. Schulz
Atmos. Chem. Phys., 15, 3991–4024, https://doi.org/10.5194/acp-15-3991-2015, https://doi.org/10.5194/acp-15-3991-2015, 2015
Short summary
Short summary
Atmospheric mineral dust from a MACC-II short reanalysis (2007-2008) has been evaluated over northern Africa and the Middle East using satellite aerosol products, AERONET data, in situ PM10 concentrations, and extinction vertical profiles. The MACC-II AOD spatial and temporal variability shows good agreement with satellite sensors and AERONET. We find a good agreement in averaged extinction vertical profiles between MACC-II and lidars. MACC correctly reproduces daily to interannual PM10.
S. A. Monks, S. R. Arnold, L. K. Emmons, K. S. Law, S. Turquety, B. N. Duncan, J. Flemming, V. Huijnen, S. Tilmes, J. Langner, J. Mao, Y. Long, J. L. Thomas, S. D. Steenrod, J. C. Raut, C. Wilson, M. P. Chipperfield, G. S. Diskin, A. Weinheimer, H. Schlager, and G. Ancellet
Atmos. Chem. Phys., 15, 3575–3603, https://doi.org/10.5194/acp-15-3575-2015, https://doi.org/10.5194/acp-15-3575-2015, 2015
Short summary
Short summary
Multi-model simulations of Arctic CO, O3 and OH are evaluated using observations. Models show highly variable concentrations but the relative importance of emission regions and types is robust across the models, demonstrating the importance of biomass burning as a source. Idealised tracer experiments suggest that some of the model spread is due to variations in simulated transport from Europe in winter and from Asia throughout the year.
K. Lefever, R. van der A, F. Baier, Y. Christophe, Q. Errera, H. Eskes, J. Flemming, A. Inness, L. Jones, J.-C. Lambert, B. Langerock, M. G. Schultz, O. Stein, A. Wagner, and S. Chabrillat
Atmos. Chem. Phys., 15, 2269–2293, https://doi.org/10.5194/acp-15-2269-2015, https://doi.org/10.5194/acp-15-2269-2015, 2015
Short summary
Short summary
We validate and discuss the analyses of stratospheric ozone delivered in near-real time between 2009 and 2012 by four different data assimilation systems: IFS-MOZART, BASCOE, SACADA and TM3DAM. It is shown that the characteristics of the assimilation systems are much less important than those of the assimilated data sets. A correct representation of the vertical distribution of ozone requires satellite observations which are well resolved vertically and extend into the lowermost stratosphere.
W. R. Sessions, J. S. Reid, A. Benedetti, P. R. Colarco, A. da Silva, S. Lu, T. Sekiyama, T. Y. Tanaka, J. M. Baldasano, S. Basart, M. E. Brooks, T. F. Eck, M. Iredell, J. A. Hansen, O. C. Jorba, H.-M. H. Juang, P. Lynch, J.-J. Morcrette, S. Moorthi, J. Mulcahy, Y. Pradhan, M. Razinger, C. B. Sampson, J. Wang, and D. L. Westphal
Atmos. Chem. Phys., 15, 335–362, https://doi.org/10.5194/acp-15-335-2015, https://doi.org/10.5194/acp-15-335-2015, 2015
Short summary
S. Remy and J. W. Kaiser
Atmos. Chem. Phys., 14, 13377–13390, https://doi.org/10.5194/acp-14-13377-2014, https://doi.org/10.5194/acp-14-13377-2014, 2014
Short summary
Short summary
This paper describes a method to correct the bias in daily fire radiative power (FRP) observations from any low Earth orbit satellite, so that that the budget of daily smoke emissions remains independent of the number of satellites from which FRP observations are taken into account. This ensures the possibility of running a system assimilating observations from several sensors, e.g. the Global Fire Assimilation System (GFAS), in case of failure of one of the MODIS instruments.
K. Tsigaridis, N. Daskalakis, M. Kanakidou, P. J. Adams, P. Artaxo, R. Bahadur, Y. Balkanski, S. E. Bauer, N. Bellouin, A. Benedetti, T. Bergman, T. K. Berntsen, J. P. Beukes, H. Bian, K. S. Carslaw, M. Chin, G. Curci, T. Diehl, R. C. Easter, S. J. Ghan, S. L. Gong, A. Hodzic, C. R. Hoyle, T. Iversen, S. Jathar, J. L. Jimenez, J. W. Kaiser, A. Kirkevåg, D. Koch, H. Kokkola, Y. H Lee, G. Lin, X. Liu, G. Luo, X. Ma, G. W. Mann, N. Mihalopoulos, J.-J. Morcrette, J.-F. Müller, G. Myhre, S. Myriokefalitakis, N. L. Ng, D. O'Donnell, J. E. Penner, L. Pozzoli, K. J. Pringle, L. M. Russell, M. Schulz, J. Sciare, Ø. Seland, D. T. Shindell, S. Sillman, R. B. Skeie, D. Spracklen, T. Stavrakou, S. D. Steenrod, T. Takemura, P. Tiitta, S. Tilmes, H. Tost, T. van Noije, P. G. van Zyl, K. von Salzen, F. Yu, Z. Wang, Z. Wang, R. A. Zaveri, H. Zhang, K. Zhang, Q. Zhang, and X. Zhang
Atmos. Chem. Phys., 14, 10845–10895, https://doi.org/10.5194/acp-14-10845-2014, https://doi.org/10.5194/acp-14-10845-2014, 2014
R. E. L. West, P. Stier, A. Jones, C. E. Johnson, G. W. Mann, N. Bellouin, D. G. Partridge, and Z. Kipling
Atmos. Chem. Phys., 14, 6369–6393, https://doi.org/10.5194/acp-14-6369-2014, https://doi.org/10.5194/acp-14-6369-2014, 2014
M. Diamantakis and J. Flemming
Geosci. Model Dev., 7, 965–979, https://doi.org/10.5194/gmd-7-965-2014, https://doi.org/10.5194/gmd-7-965-2014, 2014
V. Huijnen, J. E. Williams, and J. Flemming
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-14-8575-2014, https://doi.org/10.5194/acpd-14-8575-2014, 2014
Revised manuscript not accepted
A. Baklanov, K. Schlünzen, P. Suppan, J. Baldasano, D. Brunner, S. Aksoyoglu, G. Carmichael, J. Douros, J. Flemming, R. Forkel, S. Galmarini, M. Gauss, G. Grell, M. Hirtl, S. Joffre, O. Jorba, E. Kaas, M. Kaasik, G. Kallos, X. Kong, U. Korsholm, A. Kurganskiy, J. Kushta, U. Lohmann, A. Mahura, A. Manders-Groot, A. Maurizi, N. Moussiopoulos, S. T. Rao, N. Savage, C. Seigneur, R. S. Sokhi, E. Solazzo, S. Solomos, B. Sørensen, G. Tsegas, E. Vignati, B. Vogel, and Y. Zhang
Atmos. Chem. Phys., 14, 317–398, https://doi.org/10.5194/acp-14-317-2014, https://doi.org/10.5194/acp-14-317-2014, 2014
M. Lefèvre, A. Oumbe, P. Blanc, B. Espinar, B. Gschwind, Z. Qu, L. Wald, M. Schroedter-Homscheidt, C. Hoyer-Klick, A. Arola, A. Benedetti, J. W. Kaiser, and J.-J. Morcrette
Atmos. Meas. Tech., 6, 2403–2418, https://doi.org/10.5194/amt-6-2403-2013, https://doi.org/10.5194/amt-6-2403-2013, 2013
Z. Kipling, P. Stier, J. P. Schwarz, A. E. Perring, J. R. Spackman, G. W. Mann, C. E. Johnson, and P. J. Telford
Atmos. Chem. Phys., 13, 5969–5986, https://doi.org/10.5194/acp-13-5969-2013, https://doi.org/10.5194/acp-13-5969-2013, 2013
Related subject area
Climate and Earth system modeling
SASIEv.1: a framework for seasonal and multi-centennial Arctic sea ice emulation
COSP-RTTOV-1.0: flexible radiation diagnostics to enable new science applications in model evaluation, climate change detection, and satellite mission design
Assessing modifications to the Abdul-Razzak and Ghan aerosol activation parameterization (version ARG2000) to improve simulated aerosol–cloud radiative effects in the UK Met Office Unified Model (UM version 13.0)
Correction of sea surface biases in the NEMO ocean general circulation model using neural networks
Representing lateral groundwater flow from land to river in Earth system models
FINAM is not a model (v1.0): a new Python-based model coupling framework
The Detection and Attribution Model Intercomparison Project (DAMIP v2.0) contribution to CMIP7
Enhancing winter climate simulations of the Great Lakes: insights from a new coupled lake–ice–atmosphere (CLIAv1) system on the importance of integrating 3D hydrodynamics with a regional climate model
Modelling emission and transport of key components of primary marine organic aerosol using the global aerosol–climate model ECHAM6.3–HAM2.3
Assessing the climate impact of an improved volcanic sulfate aerosol representation in E3SM
Advanced climate model evaluation with ESMValTool v2.11.0 using parallel, out-of-core, and distributed computing
ICON-HAM-lite 1.0: simulating the Earth system with interactive aerosols at kilometer scales
Process-based modeling framework for sustainable irrigation management at the regional scale: integrating rice production, water use, and greenhouse gas emissions
Implementing deep soil and dynamic root uptake in Noah-MP (v4.5): impact on Amazon dry-season transpiration
Reducing time and computing costs in EC-Earth: an automatic load-balancing approach for coupled Earth system models
FLAME 1.0: a novel approach for modelling burned area in the Brazilian biomes using the maximum entropy concept
SURFER v3.0: a fast model with ice sheet tipping points and carbon cycle feedbacks for short- and long-term climate scenarios
NMH-CS 3.0: a C# programming language and Windows-system-based ecohydrological model derived from Noah-MP
A method for quantifying uncertainty in spatially interpolated meteorological data with application to daily maximum air temperature
Baseline Climate Variables for Earth System Modelling
PaleoSTeHM v1.0: a modern, scalable spatiotemporal hierarchical modeling framework for paleo-environmental data
The Tropical Basin Interaction Model Intercomparison Project (TBIMIP)
ZEMBA v1.0: an energy and moisture balance climate model to investigate Quaternary climate
Development and evaluation of a new 4DEnVar-based weakly coupled ocean data assimilation system in E3SMv2
TemDeep: a self-supervised framework for temporal downscaling of atmospheric fields at arbitrary time resolutions
The ensemble consistency test: from CESM to MPAS and beyond
Linear Meta-Model optimization for regional climate models (LiMMo version 1.0)
An example of how data quality hinders progress: translating the latest findings on the regulation of leaf senescence timing in trees into the DP3 model (v1.0)
Presentation, calibration and testing of the DCESS II Earth system model of intermediate complexity (version 1.0)
Synthesizing global carbon–nitrogen coupling effects – the MAGICC coupled carbon–nitrogen cycle model v1.0
Historical trends and controlling factors of isoprene emissions in CMIP6 Earth system models
Investigating carbon and nitrogen conservation in reported CMIP6 Earth system model data
OpenBench: a land models evaluation system
From weather data to river runoff: using spatiotemporal convolutional networks for discharge forecasting
A Fortran–Python interface for integrating machine learning parameterization into earth system models
ROCKE-3D 2.0: An updated general circulation model for simulating the climates of rocky planets
A rapid-application emissions-to-impacts tool for scenario assessment: Probabilistic Regional Impacts from Model patterns and Emissions (PRIME)
The sensitivity of EC-Earth3 decadal predictions to the choice of volcanic forcing dataset: Insights for the next major eruption
A first calibration of the JULES-crop version 7.4 for rice using the novel O3-FACE experiment in China
The DOE E3SM version 2.1: overview and assessment of the impacts of parameterized ocean submesoscales
WRF-ELM v1.0: a regional climate model to study land–atmosphere interactions over heterogeneous land use regions
Modeling commercial-scale CO2 storage in the gas hydrate stability zone with PFLOTRAN v6.0
DiuSST: a conceptual model of diurnal warm layers for idealized atmospheric simulations with interactive sea surface temperature
High-Resolution Model Intercomparison Project phase 2 (HighResMIP2) towards CMIP7
T&C-CROP: representing mechanistic crop growth with a terrestrial biosphere model (T&C, v1.5) – model formulation and validation
An updated non-intrusive, multi-scale, and flexible coupling interface in WRF 4.6.0
Monitoring and benchmarking Earth system model simulations with ESMValTool v2.12.0
The Earth Science Box Modeling Toolkit (ESBMTK 0.14.0.11): a Python library for research and teaching
CropSuite v1.0 – a comprehensive open-source crop suitability model considering climate variability for climate impact assessment
ICON ComIn – the ICON Community Interface (ComIn version 0.1.0, with ICON version 2024.01-01)
Sian Megan Chilcott, Malte Meinshausen, and Dirk Notz
Geosci. Model Dev., 18, 4965–4982, https://doi.org/10.5194/gmd-18-4965-2025, https://doi.org/10.5194/gmd-18-4965-2025, 2025
Short summary
Short summary
Climate models are expensive to run and often underestimate how sensitive Arctic sea ice is to climate change. To address this, we developed a simple model that emulates the response of sea ice to global warming. We find that the remaining carbon dioxide (CO2) emissions that will avoid a seasonally ice-free Arctic Ocean are lower than previous estimates of 821 Gt of CO2. Our model also provides insights into the future of winter sea ice, examining a larger ensemble than previously possible.
Jonah K. Shaw, Dustin J. Swales, Sergio DeSouza-Machado, David D. Turner, Jennifer E. Kay, and David P. Schneider
Geosci. Model Dev., 18, 4935–4950, https://doi.org/10.5194/gmd-18-4935-2025, https://doi.org/10.5194/gmd-18-4935-2025, 2025
Short summary
Short summary
Satellites have observed Earth's emissions of infrared radiation since the 1970s. Because infrared wavelengths interact with the atmosphere in distinct ways, these observations contain information about Earth and the atmosphere. We present a tool that runs within Earth system models and produces output that can be directly compared with satellite measurements of infrared radiation. We then use this tool for climate model evaluation, climate change detection, and satellite mission design.
Pratapaditya Ghosh, Katherine J. Evans, Daniel P. Grosvenor, Hyun-Gyu Kang, Salil Mahajan, Min Xu, Wei Zhang, and Hamish Gordon
Geosci. Model Dev., 18, 4899–4913, https://doi.org/10.5194/gmd-18-4899-2025, https://doi.org/10.5194/gmd-18-4899-2025, 2025
Short summary
Short summary
The most popular algorithm for calculating cloud droplet number concentrations in climate models is sensitive to parameters that control simulated aerosol particle number concentrations at different sizes. We recommend small modifications to functions in the algorithm to improve its performance. Implementing the changes in the UK Met Office climate model reduced average bias in simulated global droplet number concentrations, leading to more reflected solar radiation and a net cooling effect.
Andrea Storto, Sergey Frolov, Laura Slivinski, and Chunxue Yang
Geosci. Model Dev., 18, 4789–4804, https://doi.org/10.5194/gmd-18-4789-2025, https://doi.org/10.5194/gmd-18-4789-2025, 2025
Short summary
Short summary
Inaccuracies in air–sea heat fluxes severely degrade the accuracy of ocean numerical simulations. Here, we use artificial neural networks to correct air–sea heat fluxes as a function of oceanic and atmospheric state predictors. The correction successfully improves surface and subsurface ocean temperatures beyond the training period and in prediction experiments.
Chang Liao, L. Ruby Leung, Yilin Fang, Teklu Tesfa, and Robinson Negron-Juarez
Geosci. Model Dev., 18, 4601–4624, https://doi.org/10.5194/gmd-18-4601-2025, https://doi.org/10.5194/gmd-18-4601-2025, 2025
Short summary
Short summary
Understanding horizontal groundwater flow is important for understanding how water moves through the ground. Current climate models often simplify this process because they do not have information about the land surface that is detailed enough. Our study developed a new model that divides the land surface into hillslopes to better represent how groundwater flows. This model can help improve predictions of water availability and how it affects ecosystems.
Sebastian Müller, Martin Lange, Thomas Fischer, Sara König, Matthias Kelbling, Jeisson Javier Leal Rojas, and Stephan Thober
Geosci. Model Dev., 18, 4483–4498, https://doi.org/10.5194/gmd-18-4483-2025, https://doi.org/10.5194/gmd-18-4483-2025, 2025
Short summary
Short summary
This study presents FINAM (
FINAM is not a model), a new coupling framework written in Python to dynamically connect independently developed models. Python, as the ultimate glue language, enables the use of codes from nearly any programming language like Fortran, C++, Rust, and others. FINAM is designed to simplify the integration of various models with minimal effort, as demonstrated through various examples ranging from simple to complex systems.
Nathan P. Gillett, Isla R. Simpson, Gabi Hegerl, Reto Knutti, Dann Mitchell, Aurélien Ribes, Hideo Shiogama, Dáithí Stone, Claudia Tebaldi, Piotr Wolski, Wenxia Zhang, and Vivek K. Arora
Geosci. Model Dev., 18, 4399–4416, https://doi.org/10.5194/gmd-18-4399-2025, https://doi.org/10.5194/gmd-18-4399-2025, 2025
Short summary
Short summary
Climate model simulations of the response to human and natural influences together, natural climate influences alone and greenhouse gases alone are key to quantifying human influence on the climate. The last set of such coordinated simulations underpinned key findings in the last Intergovernmental Panel on Climate Change (IPCC) report. Here we propose a new set of such simulations to be used in the next generation of attribution studies and to underpin the next IPCC report.
Pengfei Xue, Chenfu Huang, Yafang Zhong, Michael Notaro, Miraj B. Kayastha, Xing Zhou, Chuyan Zhao, Christa Peters-Lidard, Carlos Cruz, and Eric Kemp
Geosci. Model Dev., 18, 4293–4316, https://doi.org/10.5194/gmd-18-4293-2025, https://doi.org/10.5194/gmd-18-4293-2025, 2025
Short summary
Short summary
This study introduces a new 3D lake–ice–atmosphere coupled model that significantly improves winter climate simulations for the Great Lakes compared to traditional 1D lake model coupling. The key contribution is the identification of critical hydrodynamic processes – ice transport, heat advection, and shear-driven turbulence production – that influence lake thermal structure and ice cover and explain the superior performance of 3D lake models to their 1D counterparts.
Anisbel Leon-Marcos, Moritz Zeising, Manuela van Pinxteren, Sebastian Zeppenfeld, Astrid Bracher, Elena Barbaro, Anja Engel, Matteo Feltracco, Ina Tegen, and Bernd Heinold
Geosci. Model Dev., 18, 4183–4213, https://doi.org/10.5194/gmd-18-4183-2025, https://doi.org/10.5194/gmd-18-4183-2025, 2025
Short summary
Short summary
This study represents the primary marine organic aerosol (PMOA) emissions, focusing on their sea–atmosphere transfer. Using the FESOM2.1–REcoM3 model, concentrations of key organic biomolecules were estimated and integrated into the ECHAM6.3–HAM2.3 aerosol–climate model. Results highlight the influence of marine biological activity and surface winds on PMOA emissions, with reasonably good agreement with observations improving aerosol representation in the southern oceans.
Ziming Ke, Qi Tang, Jean-Christophe Golaz, Xiaohong Liu, and Hailong Wang
Geosci. Model Dev., 18, 4137–4153, https://doi.org/10.5194/gmd-18-4137-2025, https://doi.org/10.5194/gmd-18-4137-2025, 2025
Short summary
Short summary
This study assesses volcanic aerosol representation in E3SM (Energy Exascale Earth System Model), showing that an emission-based approach moderately improves temperature variability and cloud responses compared to a prescribed forcing approach, yet significant bias persists.
Manuel Schlund, Bouwe Andela, Jörg Benke, Ruth Comer, Birgit Hassler, Emma Hogan, Peter Kalverla, Axel Lauer, Bill Little, Saskia Loosveldt Tomas, Francesco Nattino, Patrick Peglar, Valeriu Predoi, Stef Smeets, Stephen Worsley, Martin Yeo, and Klaus Zimmermann
Geosci. Model Dev., 18, 4009–4021, https://doi.org/10.5194/gmd-18-4009-2025, https://doi.org/10.5194/gmd-18-4009-2025, 2025
Short summary
Short summary
The Earth System Model Evaluation Tool (ESMValTool) is a community diagnostics and performance metrics tool for the evaluation of Earth system models. Here, we describe recent significant improvements of ESMValTool’s computational efficiency including parallel, out-of-core, and distributed computing. Evaluations with the enhanced version of ESMValTool are faster, use less computational resources, and can handle input data larger than the available memory.
Philipp Weiss, Ross Herbert, and Philip Stier
Geosci. Model Dev., 18, 3877–3894, https://doi.org/10.5194/gmd-18-3877-2025, https://doi.org/10.5194/gmd-18-3877-2025, 2025
Short summary
Short summary
Aerosols strongly influence Earth's climate as they interact with radiation and clouds. New Earth system models run at resolutions of a few kilometers. To simulate the Earth system with interactive aerosols, we developed a new aerosol module. It represents aerosols as an ensemble of lognormal modes with given sizes and compositions. We present a year-long simulation with four modes at a resolution of 5 km. It captures key processes like the formation of dust storms in the Sahara.
Yan Bo, Hao Liang, Tao Li, and Feng Zhou
Geosci. Model Dev., 18, 3799–3817, https://doi.org/10.5194/gmd-18-3799-2025, https://doi.org/10.5194/gmd-18-3799-2025, 2025
Short summary
Short summary
This study proposed an advancing framework for modeling regional rice production, water use, and greenhouse gas emissions. The framework integrated a process-based soil-crop model with vital physiological effects, a novel model upscaling method, and the NSGA-II multi-objective optimization algorithm at a parallel computing platform. The framework provides a valuable tool for multi-objective optimization of rice irrigation schemes at a large scale.
Carolina A. Bieri, Francina Dominguez, Gonzalo Miguez-Macho, and Ying Fan
Geosci. Model Dev., 18, 3755–3779, https://doi.org/10.5194/gmd-18-3755-2025, https://doi.org/10.5194/gmd-18-3755-2025, 2025
Short summary
Short summary
Access to deep moisture below the Earth's surface is important for vegetation in areas of the Amazon where there is little precipitation for part of the year. Most existing numerical models of the Earth system do not adequately capture where and when deep root water uptake occurs. We address this by adding deep soil layers and a root water uptake feature to an existing model. Out modifications lead to increased dry-month transpiration and improved simulation of the annual transpiration cycle.
Sergi Palomas, Mario C. Acosta, Gladys Utrera, and Etienne Tourigny
Geosci. Model Dev., 18, 3661–3679, https://doi.org/10.5194/gmd-18-3661-2025, https://doi.org/10.5194/gmd-18-3661-2025, 2025
Short summary
Short summary
We present an automatic tool that optimizes resource distribution in coupled climate models, enhancing speed and reducing computational costs without requiring expert knowledge. Users can set energy/time criteria or limit resource usage. Tested on various European Community Earth System Model (EC-Earth) configurations and high-performance computing (HPC) platforms, it achieved up to 34 % faster simulations with fewer resources.
Maria Lucia Ferreira Barbosa, Douglas I. Kelley, Chantelle A. Burton, Igor J. M. Ferreira, Renata Moura da Veiga, Anna Bradley, Paulo Guilherme Molin, and Liana O. Anderson
Geosci. Model Dev., 18, 3533–3557, https://doi.org/10.5194/gmd-18-3533-2025, https://doi.org/10.5194/gmd-18-3533-2025, 2025
Short summary
Short summary
As fire seasons in Brazil become increasingly severe, confidently understanding the factors driving fires is more critical than ever. To address this challenge, we developed FLAME (Fire Landscape Analysis using Maximum Entropy), a new model designed to predict fires and to analyse the spatial influence of both environmental and human factors while accounting for uncertainties. By adapting the model to different regions, we can enhance fire management strategies, making FLAME a powerful tool for protecting landscapes in Brazil and beyond.
Victor Couplet, Marina Martínez Montero, and Michel Crucifix
Geosci. Model Dev., 18, 3081–3129, https://doi.org/10.5194/gmd-18-3081-2025, https://doi.org/10.5194/gmd-18-3081-2025, 2025
Short summary
Short summary
We present SURFER v3.0, a simple climate model designed to estimate the impact of CO2 and CH4 emissions on global temperatures, sea levels, and ocean pH. We added new carbon cycle processes and calibrated the model to observations and results from more complex models, enabling use over timescales ranging from decades to millions of years. SURFER v3.0 is fast, transparent, and easy to use, making it an ideal tool for policy assessments and suitable for educational purposes.
Yong-He Liu and Zong-Liang Yang
Geosci. Model Dev., 18, 3157–3174, https://doi.org/10.5194/gmd-18-3157-2025, https://doi.org/10.5194/gmd-18-3157-2025, 2025
Short summary
Short summary
NMH-CS 3.0 is a C#-based ecohydrological model reconstructed from the WRF-Hydro/Noah-MP model by translating the Fortran code of WRF-Hydro 3.0 and integrating a parallel river routing module. It enables efficient execution on multi-core personal computers. Simulations in the Yellow River basin demonstrate its consistency with WRF-Hydro outputs, providing a reliable alternative to the original Noah-MP model.
Conor T. Doherty, Weile Wang, Hirofumi Hashimoto, and Ian G. Brosnan
Geosci. Model Dev., 18, 3003–3016, https://doi.org/10.5194/gmd-18-3003-2025, https://doi.org/10.5194/gmd-18-3003-2025, 2025
Short summary
Short summary
We present, analyze, and validate a methodology for quantifying uncertainty in gridded meteorological data products produced by spatial interpolation. In a validation case study using daily maximum near-surface air temperature (Tmax), the method works well and produces predictive distributions with closely matching theoretical versus actual coverage levels. Application of the method reveals that the magnitude of uncertainty in interpolated Tmax varies significantly in both space and time.
Martin Juckes, Karl E. Taylor, Fabrizio Antonio, David Brayshaw, Carlo Buontempo, Jian Cao, Paul J. Durack, Michio Kawamiya, Hyungjun Kim, Tomas Lovato, Chloe Mackallah, Matthew Mizielinski, Alessandra Nuzzo, Martina Stockhause, Daniele Visioni, Jeremy Walton, Briony Turner, Eleanor O'Rourke, and Beth Dingley
Geosci. Model Dev., 18, 2639–2663, https://doi.org/10.5194/gmd-18-2639-2025, https://doi.org/10.5194/gmd-18-2639-2025, 2025
Short summary
Short summary
The Baseline Climate Variables for Earth System Modelling (ESM-BCVs) are defined as a list of 135 variables which have high utility for the evaluation and exploitation of climate simulations. The list reflects the most frequently used variables from Earth system models based on an assessment of data publication and download records from the largest archive of global climate projects.
Yucheng Lin, Robert E. Kopp, Alexander Reedy, Matteo Turilli, Shantenu Jha, and Erica L. Ashe
Geosci. Model Dev., 18, 2609–2637, https://doi.org/10.5194/gmd-18-2609-2025, https://doi.org/10.5194/gmd-18-2609-2025, 2025
Short summary
Short summary
PaleoSTeHM v1.0 is a state-of-the-art framework designed to reconstruct past environmental conditions using geological data. Built on modern machine learning techniques, it efficiently handles the sparse and noisy nature of paleo-records, allowing scientists to make accurate and scalable inferences about past environmental change. By using flexible statistical models, PaleoSTeHM separates different sources of uncertainty, improving the precision of historical climate reconstructions.
Ingo Richter, Ping Chang, Ping-Gin Chiu, Gokhan Danabasoglu, Takeshi Doi, Dietmar Dommenget, Guillaume Gastineau, Zoe E. Gillett, Aixue Hu, Takahito Kataoka, Noel S. Keenlyside, Fred Kucharski, Yuko M. Okumura, Wonsun Park, Malte F. Stuecker, Andréa S. Taschetto, Chunzai Wang, Stephen G. Yeager, and Sang-Wook Yeh
Geosci. Model Dev., 18, 2587–2608, https://doi.org/10.5194/gmd-18-2587-2025, https://doi.org/10.5194/gmd-18-2587-2025, 2025
Short summary
Short summary
Tropical ocean basins influence each other through multiple pathways and mechanisms, referred to here as tropical basin interaction (TBI). Many researchers have examined TBI using comprehensive climate models but have obtained conflicting results. This may be partly due to differences in experiment protocols and partly due to systematic model errors. The Tropical Basin Interaction Model Intercomparison Project (TBIMIP) aims to address this problem by designing a set of TBI experiments that will be performed by multiple models.
Daniel F. J. Gunning, Kerim H. Nisancioglu, Emilie Capron, and Roderik S. W. van de Wal
Geosci. Model Dev., 18, 2479–2508, https://doi.org/10.5194/gmd-18-2479-2025, https://doi.org/10.5194/gmd-18-2479-2025, 2025
Short summary
Short summary
This work documents the first results from ZEMBA: an energy balance model of the climate system. The model is a computationally efficient tool designed to study the response of climate to changes in the Earth's orbit. We demonstrate that ZEMBA reproduces many features of the Earth's climate for both the pre-industrial period and the Earth's most recent cold extreme – the Last Glacial Maximum. We intend to develop ZEMBA further and investigate the glacial cycles of the last 2.5 million years.
Pengfei Shi, L. Ruby Leung, and Bin Wang
Geosci. Model Dev., 18, 2443–2460, https://doi.org/10.5194/gmd-18-2443-2025, https://doi.org/10.5194/gmd-18-2443-2025, 2025
Short summary
Short summary
Improving climate predictions has significant socio-economic impacts. In this study, we develop and apply a new weakly coupled ocean data assimilation (WCODA) system to a coupled climate model. The WCODA system improves simulations of ocean temperature and salinity across many global regions. This system is meant to advance our understanding of the ocean's role in climate predictability.
Liwen Wang, Qian Li, Qi Lv, Xuan Peng, and Wei You
Geosci. Model Dev., 18, 2427–2442, https://doi.org/10.5194/gmd-18-2427-2025, https://doi.org/10.5194/gmd-18-2427-2025, 2025
Short summary
Short summary
Our research presents a novel deep learning approach called "TemDeep" for downscaling atmospheric variables at arbitrary time resolutions based on temporal coherence. Results show that our method can accurately recover evolution details superior to other methods, reaching 53.7 % in the restoration rate. Our findings are important for advancing weather forecasting models and enabling more precise and reliable predictions to support disaster preparedness, agriculture, and sustainable development.
Teo Price-Broncucia, Allison Baker, Dorit Hammerling, Michael Duda, and Rebecca Morrison
Geosci. Model Dev., 18, 2349–2372, https://doi.org/10.5194/gmd-18-2349-2025, https://doi.org/10.5194/gmd-18-2349-2025, 2025
Short summary
Short summary
The ensemble consistency test (ECT) and its ultrafast variant (UF-ECT) have become powerful tools in the development community for the identification of unwanted changes in the Community Earth System Model (CESM). We develop a generalized setup framework to enable easy adoption of the ECT approach for other model developers and communities. This framework specifies test parameters to accurately characterize model variability and balance test sensitivity and computational cost.
Sergei Petrov, Andreas Will, and Beate Geyer
EGUsphere, https://doi.org/10.5194/egusphere-2025-710, https://doi.org/10.5194/egusphere-2025-710, 2025
Short summary
Short summary
This study introduces a new method that helps improve the accuracy of climate models by automatically selecting the best parameters to match real-world observations. Instead of manually adjusting many parameters, the method uses a mathematical tool to find the most appropriate settings for the model. It can be especially helpful for researchers who introduce new physical parameters into climate models to assess their impact on model results and optimize them along with the old ones.
Michael Meier, Christof Bigler, and Isabelle Chuine
EGUsphere, https://doi.org/10.5194/egusphere-2025-460, https://doi.org/10.5194/egusphere-2025-460, 2025
Short summary
Short summary
Formulated according to the leaf development process, the DP3 model of leaf coloring considerably contrasts previous models and allows to set up new hypotheses, e.g. on aging versus stress caused color changes. The DP3 model was as accurate as previous models and a comparison to the constant simulation of the mean date of leaf coloring indicated that noisy leaf coloring data forced the models to resort to this mean, which hinders model evaluation.
Esteban Fernández Villanueva and Gary Shaffer
Geosci. Model Dev., 18, 2161–2192, https://doi.org/10.5194/gmd-18-2161-2025, https://doi.org/10.5194/gmd-18-2161-2025, 2025
Short summary
Short summary
We describe, calibrate and test the Danish Center for Earth System Science (DCESS) II model, a new, broad, adaptable and fast Earth system model. DCESS II is designed for global simulations over timescales of years to millions of years using limited computer resources like a personal computer. With its flexibility and comprehensive treatment of the global carbon cycle, DCESS II is a useful, computationally friendly tool for simulations of past climates as well as for future Earth system projections.
Gang Tang, Zebedee Nicholls, Alexander Norton, Sönke Zaehle, and Malte Meinshausen
Geosci. Model Dev., 18, 2193–2230, https://doi.org/10.5194/gmd-18-2193-2025, https://doi.org/10.5194/gmd-18-2193-2025, 2025
Short summary
Short summary
We studied carbon–nitrogen coupling in Earth system models by developing a global carbon–nitrogen cycle model (CNit v1.0) within the widely used emulator MAGICC. CNit effectively reproduced the global carbon–nitrogen cycle dynamics observed in complex models. Our results show persistent nitrogen limitations on plant growth (net primary production) from 1850 to 2100, suggesting that nitrogen deficiency may constrain future land carbon sequestration.
Ngoc Thi Nhu Do, Kengo Sudo, Akihiko Ito, Louisa K. Emmons, Vaishali Naik, Kostas Tsigaridis, Øyvind Seland, Gerd A. Folberth, and Douglas I. Kelley
Geosci. Model Dev., 18, 2079–2109, https://doi.org/10.5194/gmd-18-2079-2025, https://doi.org/10.5194/gmd-18-2079-2025, 2025
Short summary
Short summary
Understanding historical isoprene emission changes is important for predicting future climate, but trends and their controlling factors remain uncertain. This study shows that long-term isoprene trends vary among Earth system models mainly due to partially incorporating CO2 effects and land cover changes rather than to climate. Future models that refine these factors’ effects on isoprene emissions, along with long-term observations, are essential for better understanding plant–climate interactions.
Gang Tang, Zebedee Nicholls, Chris Jones, Thomas Gasser, Alexander Norton, Tilo Ziehn, Alejandro Romero-Prieto, and Malte Meinshausen
Geosci. Model Dev., 18, 2111–2136, https://doi.org/10.5194/gmd-18-2111-2025, https://doi.org/10.5194/gmd-18-2111-2025, 2025
Short summary
Short summary
We analyzed carbon and nitrogen mass conservation in data from various Earth system models. Our findings reveal significant discrepancies between flux and pool size data, where cumulative imbalances can reach hundreds of gigatons of carbon or nitrogen. These imbalances appear primarily due to missing or inconsistently reported fluxes – especially for land-use and fire emissions. To enhance data quality, we recommend that future climate data protocols address this issue at the reporting stage.
Zhongwang Wei, Qingchen Xu, Fan Bai, Xionghui Xu, Zixin Wei, Wenzong Dong, Hongbin Liang, Nan Wei, Xingjie Lu, Lu Li, Shupeng Zhang, Hua Yuan, Laibo Liu, and Yongjiu Dai
EGUsphere, https://doi.org/10.5194/egusphere-2025-1380, https://doi.org/10.5194/egusphere-2025-1380, 2025
Short summary
Short summary
Land surface models are used for simulating earth's surface interacts with the atmosphere. As models grow more complex and detailed, researchers need better tools to evaluate their performance. OpenBench, a new software system that makes evaluation process more comprehensive and efficient. It stands out by incorporating various factors and working with data at any scale which enabling scientists to incorporate new types of models and measurements as our understanding of Earth’s systems evolves.
Florian Börgel, Sven Karsten, Karoline Rummel, and Ulf Gräwe
Geosci. Model Dev., 18, 2005–2019, https://doi.org/10.5194/gmd-18-2005-2025, https://doi.org/10.5194/gmd-18-2005-2025, 2025
Short summary
Short summary
Forecasting river runoff, which is crucial for managing water resources and understanding climate impacts, can be challenging. This study introduces a new method using convolutional long short-term memory (ConvLSTM) networks, a machine learning model that processes spatial and temporal data. Focusing on the Baltic Sea region, our model uses weather data as input to predict daily river runoff for 97 rivers.
Tao Zhang, Cyril Morcrette, Meng Zhang, Wuyin Lin, Shaocheng Xie, Ye Liu, Kwinten Van Weverberg, and Joana Rodrigues
Geosci. Model Dev., 18, 1917–1928, https://doi.org/10.5194/gmd-18-1917-2025, https://doi.org/10.5194/gmd-18-1917-2025, 2025
Short summary
Short summary
Earth system models (ESMs) struggle with the uncertainties associated with parameterizing subgrid physics. Machine learning (ML) algorithms offer a solution by learning the important relationships and features from high-resolution models. To incorporate ML parameterizations into ESMs, we develop a Fortran–Python interface that allows for calling Python functions within Fortran-based ESMs. Through two case studies, this interface demonstrates its feasibility, modularity, and effectiveness.
Kostas Tsigaridis, Andrew S. Ackerman, Igor Aleinov, Mark A. Chandler, Thomas L. Clune, Christopher M. Colose, Anthony D. Del Genio, Maxwell Kelley, Nancy Y. Kiang, Anthony Leboissetier, Jan P. Perlwitz, Reto A. Ruedy, Gary L. Russell, Linda E. Sohl, Michael J. Way, and Eric T. Wolf
EGUsphere, https://doi.org/10.5194/egusphere-2025-925, https://doi.org/10.5194/egusphere-2025-925, 2025
Short summary
Short summary
We present the second generation of ROCKE-3D, a generalized 3-dimensional model for use in Solar System and exoplanetary simulations of rocky planet climates. We quantify how the different component choices affect model results, and discuss strengths and limitations of using each component, together with how one can select which component to use. ROCKE-3D is publicly available and tutorial sessions are available for the community, greatly facilitating its use by any interested group.
Camilla Mathison, Eleanor J. Burke, Gregory Munday, Chris D. Jones, Chris J. Smith, Norman J. Steinert, Andy J. Wiltshire, Chris Huntingford, Eszter Kovacs, Laila K. Gohar, Rebecca M. Varney, and Douglas McNeall
Geosci. Model Dev., 18, 1785–1808, https://doi.org/10.5194/gmd-18-1785-2025, https://doi.org/10.5194/gmd-18-1785-2025, 2025
Short summary
Short summary
We present PRIME (Probabilistic Regional Impacts from Model patterns and Emissions), which is designed to take new emissions scenarios and rapidly provide regional impact information. PRIME allows large ensembles to be run on multi-centennial timescales, including the analysis of many important variables for impact assessments. Our evaluation shows that PRIME reproduces the climate response for known scenarios, providing confidence in using PRIME for novel scenarios.
Roberto Bilbao, Thomas J. Aubry, Matthew Toohey, and Pablo Ortega
EGUsphere, https://doi.org/10.5194/egusphere-2025-609, https://doi.org/10.5194/egusphere-2025-609, 2025
Short summary
Short summary
Large volcanic eruptions are unpredictable and can have significant climatic impacts. If one occurs, operational decadal forecasts will become invalid and must be rerun including the volcanic forcing. By analyzing the climate response in EC-Earth3 retrospective predictions, we show that idealised forcings produced with two simple models could be used in operational decadal forecasts to account for the radiative impacts of the next major volcanic eruption.
Beiyao Xu, Steven Dobbie, Huiyi Yang, Lianxin Yang, Yu Jiang, Andrew Challinor, Karina Williams, Yunxia Wang, and Tijian Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-4077, https://doi.org/10.5194/egusphere-2024-4077, 2025
Short summary
Short summary
Ozone (O3) pollution harms rice production and threatens food security. To understand these impacts, we calibrated a crop model using unique data from experiments where rice was grown in open fields under controlled O3 exposure (free air). This is the first time such data has been used to improve a model’s ability to predict how rice responds to O3 pollution. Our work provides a more accurate tool to study O3’s effects and guide strategies to protect agriculture.
Katherine M. Smith, Alice M. Barthel, LeAnn M. Conlon, Luke P. Van Roekel, Anthony Bartoletti, Jean-Christophe Golaz, Chengzhu Zhang, Carolyn Branecky Begeman, James J. Benedict, Gautam Bisht, Yan Feng, Walter Hannah, Bryce E. Harrop, Nicole Jeffery, Wuyin Lin, Po-Lun Ma, Mathew E. Maltrud, Mark R. Petersen, Balwinder Singh, Qi Tang, Teklu Tesfa, Jonathan D. Wolfe, Shaocheng Xie, Xue Zheng, Karthik Balaguru, Oluwayemi Garuba, Peter Gleckler, Aixue Hu, Jiwoo Lee, Ben Moore-Maley, and Ana C. Ordoñez
Geosci. Model Dev., 18, 1613–1633, https://doi.org/10.5194/gmd-18-1613-2025, https://doi.org/10.5194/gmd-18-1613-2025, 2025
Short summary
Short summary
Version 2.1 of the U.S. Department of Energy's Energy Exascale Earth System Model (E3SM) adds the Fox-Kemper et al. (2011) mixed-layer eddy parameterization, which restratifies the ocean surface layer through an overturning streamfunction. Results include surface layer bias reduction in temperature, salinity, and sea ice extent in the North Atlantic; a small strengthening of the Atlantic meridional overturning circulation; and improvements to many atmospheric climatological variables.
Huilin Huang, Yun Qian, Gautam Bisht, Jiali Wang, Tirthankar Chakraborty, Dalei Hao, Jianfeng Li, Travis Thurber, Balwinder Singh, Zhao Yang, Ye Liu, Pengfei Xue, William J. Sacks, Ethan Coon, and Robert Hetland
Geosci. Model Dev., 18, 1427–1443, https://doi.org/10.5194/gmd-18-1427-2025, https://doi.org/10.5194/gmd-18-1427-2025, 2025
Short summary
Short summary
We integrate the E3SM Land Model (ELM) with the WRF model through the Lightweight Infrastructure for Land Atmosphere Coupling (LILAC) Earth System Modeling Framework (ESMF). This framework includes a top-level driver, LILAC, for variable communication between WRF and ELM and ESMF caps for ELM initialization, execution, and finalization. The LILAC–ESMF framework maintains the integrity of the ELM's source code structure and facilitates the transfer of future ELM model developments to WRF-ELM.
Michael Nole, Jonah Bartrand, Fawz Naim, and Glenn Hammond
Geosci. Model Dev., 18, 1413–1425, https://doi.org/10.5194/gmd-18-1413-2025, https://doi.org/10.5194/gmd-18-1413-2025, 2025
Short summary
Short summary
Safe carbon dioxide (CO2) storage is likely to be critical for mitigating some of the most severe effects of climate change. We present a simulation framework for modeling CO2 storage beneath the seafloor, where CO2 can form a solid. This can aid in permanent CO2 storage for long periods of time. Our models show what a commercial-scale CO2 injection would look like in a marine environment. We discuss what would need to be considered when designing a subsea CO2 injection.
Reyk Börner, Jan O. Haerter, and Romain Fiévet
Geosci. Model Dev., 18, 1333–1356, https://doi.org/10.5194/gmd-18-1333-2025, https://doi.org/10.5194/gmd-18-1333-2025, 2025
Short summary
Short summary
The daily cycle of sea surface temperature (SST) impacts clouds above the ocean and could influence the clustering of thunderstorms linked to extreme rainfall and hurricanes. However, daily SST variability is often poorly represented in modeling studies of how clouds cluster. We present a simple, wind-responsive model of upper-ocean temperature for use in atmospheric simulations. Evaluating the model against observations, we show that it performs significantly better than common slab models.
Malcolm J. Roberts, Kevin A. Reed, Qing Bao, Joseph J. Barsugli, Suzana J. Camargo, Louis-Philippe Caron, Ping Chang, Cheng-Ta Chen, Hannah M. Christensen, Gokhan Danabasoglu, Ivy Frenger, Neven S. Fučkar, Shabeh ul Hasson, Helene T. Hewitt, Huanping Huang, Daehyun Kim, Chihiro Kodama, Michael Lai, Lai-Yung Ruby Leung, Ryo Mizuta, Paulo Nobre, Pablo Ortega, Dominique Paquin, Christopher D. Roberts, Enrico Scoccimarro, Jon Seddon, Anne Marie Treguier, Chia-Ying Tu, Paul A. Ullrich, Pier Luigi Vidale, Michael F. Wehner, Colin M. Zarzycki, Bosong Zhang, Wei Zhang, and Ming Zhao
Geosci. Model Dev., 18, 1307–1332, https://doi.org/10.5194/gmd-18-1307-2025, https://doi.org/10.5194/gmd-18-1307-2025, 2025
Short summary
Short summary
HighResMIP2 is a model intercomparison project focusing on high-resolution global climate models, that is, those with grid spacings of 25 km or less in the atmosphere and ocean, using simulations of decades to a century in length. We are proposing an update of our simulation protocol to make the models more applicable to key questions for climate variability and hazard in present-day and future projections and to build links with other communities to provide more robust climate information.
Jordi Buckley Paules, Simone Fatichi, Bonnie Warring, and Athanasios Paschalis
Geosci. Model Dev., 18, 1287–1305, https://doi.org/10.5194/gmd-18-1287-2025, https://doi.org/10.5194/gmd-18-1287-2025, 2025
Short summary
Short summary
We present and validate enhancements to the process-based T&C model aimed at improving its representation of crop growth and management practices. The updated model, T&C-CROP, enables applications such as analysing the hydrological and carbon storage impacts of land use transitions (e.g. conversions between crops, forests, and pastures) and optimizing irrigation and fertilization strategies in response to climate change.
Sébastien Masson, Swen Jullien, Eric Maisonnave, David Gill, Guillaume Samson, Mathieu Le Corre, and Lionel Renault
Geosci. Model Dev., 18, 1241–1263, https://doi.org/10.5194/gmd-18-1241-2025, https://doi.org/10.5194/gmd-18-1241-2025, 2025
Short summary
Short summary
This article details a new feature we implemented in the popular regional atmospheric model WRF. This feature allows for data exchange between WRF and any other model (e.g. an ocean model) using the coupling library Ocean–Atmosphere–Sea–Ice–Soil Model Coupling Toolkit (OASIS3-MCT). This coupling interface is designed to be non-intrusive, flexible and modular. It also offers the possibility of taking into account the nested zooms used in WRF or in the models with which it is coupled.
Axel Lauer, Lisa Bock, Birgit Hassler, Patrick Jöckel, Lukas Ruhe, and Manuel Schlund
Geosci. Model Dev., 18, 1169–1188, https://doi.org/10.5194/gmd-18-1169-2025, https://doi.org/10.5194/gmd-18-1169-2025, 2025
Short summary
Short summary
Earth system models are important tools to improve our understanding of current climate and to project climate change. Thus, it is crucial to understand possible shortcomings in the models. New features of the ESMValTool software package allow one to compare and visualize a model's performance with respect to reproducing observations in the context of other climate models in an easy and user-friendly way. We aim to help model developers assess and monitor climate simulations more efficiently.
Ulrich G. Wortmann, Tina Tsan, Mahrukh Niazi, Irene A. Ma, Ruben Navasardyan, Magnus-Roland Marun, Bernardo S. Chede, Jingwen Zhong, and Morgan Wolfe
Geosci. Model Dev., 18, 1155–1167, https://doi.org/10.5194/gmd-18-1155-2025, https://doi.org/10.5194/gmd-18-1155-2025, 2025
Short summary
Short summary
The Earth Science Box Modeling Toolkit (ESBMTK) is a user-friendly Python library that simplifies the creation of models to study earth system processes, such as the carbon cycle and ocean chemistry. It enhances learning by emphasizing concepts over programming and is accessible to students and researchers alike. By automating complex calculations and promoting code clarity, ESBMTK accelerates model development while improving reproducibility and the usability of scientific research.
Florian Zabel, Matthias Knüttel, and Benjamin Poschlod
Geosci. Model Dev., 18, 1067–1087, https://doi.org/10.5194/gmd-18-1067-2025, https://doi.org/10.5194/gmd-18-1067-2025, 2025
Short summary
Short summary
CropSuite is a new open-source crop suitability model. It provides a GUI and a wide range of options, including a spatial downscaling of climate data. We apply CropSuite to 48 staple and opportunity crops at a 1 km spatial resolution in Africa. We find that climate variability significantly impacts suitable areas but also affects optimal sowing dates and multiple cropping potential. The results provide valuable information for climate impact assessments, adaptation, and land-use planning.
Kerstin Hartung, Bastian Kern, Nils-Arne Dreier, Jörn Geisbüsch, Mahnoosh Haghighatnasab, Patrick Jöckel, Astrid Kerkweg, Wilton Jaciel Loch, Florian Prill, and Daniel Rieger
Geosci. Model Dev., 18, 1001–1015, https://doi.org/10.5194/gmd-18-1001-2025, https://doi.org/10.5194/gmd-18-1001-2025, 2025
Short summary
Short summary
The ICOsahedral Non-hydrostatic (ICON) model system Community Interface (ComIn) library supports connecting third-party modules to the ICON model. Third-party modules can range from simple diagnostic Python scripts to full chemistry models. ComIn offers a low barrier for code extensions to ICON, provides multi-language support (Fortran, C/C++, and Python), and reduces the migration effort in response to new ICON releases. This paper presents the ComIn design principles and a range of use cases.
Cited articles
Ahlgrimm, M., Forbes, R., Hogan, R. J., and Sandu, I.: Understanding global model systematic shortwave radiation errors in subtropical marine boundary layer cloud regimes. J. Adv. Model. Earth Sy., 10, 2042–2060, https://doi.org/10.1029/2018MS001346, 2018. a
Andersson, A., Fennig, K., Klepp, C., Bakan, S., Graßl, H., and Schulz, J.: The Hamburg Ocean Atmosphere Parameters and Fluxes from Satellite Data – HOAPS-3, Earth Syst. Sci. Data, 2, 215–234, https://doi.org/10.5194/essd-2-215-2010, 2010. a
Baklanov, A., Schlünzen, K., Suppan, P., Baldasano, J., Brunner, D., Aksoyoglu, S., Carmichael, G., Douros, J., Flemming, J., Forkel, R., Galmarini, S., Gauss, M., Grell, G., Hirtl, M., Joffre, S., Jorba, O., Kaas, E., Kaasik, M., Kallos, G., Kong, X., Korsholm, U., Kurganskiy, A., Kushta, J., Lohmann, U., Mahura, A., Manders-Groot, A., Maurizi, A., Moussiopoulos, N., Rao, S. T., Savage, N., Seigneur, C., Sokhi, R. S., Solazzo, E., Solomos, S., Sørensen, B., Tsegas, G., Vignati, E., Vogel, B., and Zhang, Y.: Online coupled regional meteorology chemistry models in Europe: current status and prospects, Atmos. Chem. Phys., 14, 317–398, https://doi.org/10.5194/acp-14-317-2014, 2014. a
Baklanov, A., Brunner, D., Carmichael, G., Flemming, J., Freitas, S., Gauss, M., Hov, Mathur, R., Schlünzen, K., Seigneur, C., and Vogel, B.: Key Issues for Seamless Integrated Chemistry-Meteorology Modeling, B. Am. Meteorol. Soc., 98, 2285–2292, https://doi.org/10.1175/BAMS-D-15-00166.1., 2018. a
Balkanski, Y., Schulz, M., Claquin, T., and Guibert, S.: Reevaluation of Mineral aerosol radiative forcings suggests a better agreement with satellite and AERONET data, Atmos. Chem. Phys., 7, 81–95, https://doi.org/10.5194/acp-7-81-2007, 2007.
Benedetti, A. and Fisher, M.: Background error statistics for aerosols, Q. J. R. Meteor. Soc., 133, 391–405, 2007. a
Benedetti, A., Morcrette, J.-J., Boucher, O., Dethof, A., Engelen, R. J., Fisher, M., Flentje, H., Huneeus, N., Jones, L., Kaiser, J. W., Kinne, S., Mangold, A., Razinger, M., Simmons, A. J., and Suttie, M.: Aerosol analysis and forecast in the European Centre for Medium-Range Weather Forecasts Integrated Forecast System. Part 2: Data assimilation, J. Geophys. Res.-Atmos., 114, D13205, https://doi.org/10.1020/2008JD011115, 2009. a, b, c, d
Benkovitz, C. M., Scholtz, M. T., Pacyna, J., Tarrasón, L., Dignon, J., Voldner, E. C., Spiro, P. A., Logan, J. A., and Graedel, T. E.: Global gridded inventories of anthropogenic emissions of sulfur and nitrogen, J. Geophys. Res., 101, 29239–29253, https://doi.org/10.1029/96JD00126, 1996. a
Bellouin, N., Boucher, O., Haywood, J., and Reddy, M. S.: Global estimate of aerosol direct radiative forcing from satellite mea-surements, Nature, 438, 1138–1141, 2005. a
Bellouin, N., Rae, J., Jones, A., Johnson, C., Haywood, J., and Boucher, O.: Aerosol forcing in the Climate Model Intercomparison Project (CMIP5) simulations by HadGEM2-ES and the role of ammonium nitrate, J. Geophys. Res., 116, D20206, https://doi.org/10.1029/2011JD016074, 2011. a
Bollasina, M., Ming, Y., and Ramaswamy, V.: Anthropogenic aerosols and the weakening of the South Asian summer Monsoon, Science, 334, 502–505, 2011. a
Bond, T. C., Doherty, S. J., Fahey, D. W., Forster, P. M., Berntsen, T., DeAngelo, B. J., Flanner, M. G., Ghan, S., Kärcher, B., Koch, D., Kinne, S., Kondo, Y., Quinn, P. K., Sarofim, M. C., Schultz, M. G., Schulz, M., Venkataraman, C., Zhang, H., Zhang, S., Bellouin, N., Guttikunda, S. K., Hopke, P. K., Jacobson, M. Z., Kaiser, J. W., Klimont, Z., Lohmann, U., Schwarz, J. P., Shindell, D., Storelvmo, T., Warren, S. G., and Zender, C. S.: Bounding the role of black carbon in the climate system: A scientific assessment, J. Geophys. Res.-Atmos., 118, 5380–5552, https://doi.org/10.1002/jgrd.50171, 2013. a
Boucher, O., Pham, M., and Venkataraman, C.: Simulation of the atmospheric sulfur cycle in the Laboratoire de Meteorologie Dynamique general circulation model: Model description, model evaluation, and global and European budgets, Note Sci. IPSL 23, 27 pp., Inst. Pierre Simon Laplace, Paris, 2002. a
Boucher, O., Randall, D., Artaxo, P., Bretherton, C., Feingold, G., Forster, P., Kerminen, V.-M., Kondo, Y., Liao, H., Lohmann, U., Rasch, P., Satheesh, S.K., Sherwood, S., Stevens, B., and Zhang, X. Y.: Clouds and Aerosols. In: Climate Change 2013: The Physical Science Basis, Contribution of Working Group I to the Fifth Assessment Report of the Intergovernmental Panel on Climate Change, edited by: Stocker, T. F., Qin, D., Plattner, G.-K., Tignor, M., Allen, S. K., Boschung, J., Nauels, A., Xia, Y., Bex, V., and Midgley, P. M., Cambridge University Press, Cambridge, UK, New York, NY, USA, 571–658, https://doi.org/10.1017/CBO9781107415324.016, 2013. a
Bourassa, A. E., Robock, A., Randel, W. J., Deshler, T., Rieger, L. A., Lloyd, N. D., Llewellyn, E. J. (Ted), and Degenstein, D. A.: Large volcanic aerosol load in the stratosphere linked to Asian Monsoon transport, Science, 337, 78–81, https://doi.org/10.1126/science.1219371, 2012.
Bozzo, A., Benedetti, A., Flemming, J., Kipling, Z., and Remy S.: An aerosol climatology for global models based on the tropospheric
aerosol scheme in the Integrated Forecasting System of ECMWF, https://doi.org/10.24380/jgs8-sc58, 2020a. a
Bozzo, A., Benedetti, A., Flemming, J., Kipling, Z., and Remy S.: CAMS Monthly Mean Aerosol CLimatology for global models, available at:
https://confluence.ecmwf.int/display/CKB/CAMS+Monthly+Mean+Aerosol+Climatology+for+global+models, last access: 4 March 2020b. a
Clough, S. A., Shephard, M. W., Mlawer, E. J., Delamere, J. S., Iacono, M. J., Cady-Pereira, K., Boukabara, S., and Brown, P. D.: Atmospheric radiative transfer modeling: a summary of the AER codes, J. Quant. Spectrosc. Ra., 91, 233–244, 2005. a
Colarco, P. R., Nowottnick, E. P., Randles, C. A., Yi, B., Yang, P., Kim, K.-M., Smith, J. A., and Bardeen, C. G.: Impact of radiatively interactive dust aerosols in the NASA GEOS-5 climate model: Sensitivity to dust particle shape and refractive index, J. Geophys. Res.-Atmos., 119, 753–786, https://doi.org/10.1002/2013JD020046, 2014. a
Dee, D., and Uppala, S.: Variational bias correction in ERA-Interim, ECMWF, Technical Memorandum 575, p. 26, available at: http://www.ecmwf.int/publications/library/do/references/show?id=88715 (last access: 4 March 2020), 2008. a
Dentener, F., Kinne, S., Bond, T., Boucher, O., Cofala, J., Generoso, S., Ginoux, P., Gong, S., Hoelzemann, J. J., Ito, A., Marelli, L., Penner, J. E., Putaud, J.-P., Textor, C., Schulz, M., van der Werf, G. R., and Wilson, J.: Emissions of primary aerosol and precursor gases in the years 2000 and 1750 prescribed data-sets for AeroCom, Atmos. Chem. Phys., 6, 4321–4344, https://doi.org/10.5194/acp-6-4321-2006, 2006.
Donner, L., Wyman, B., Hemler, R., Horowitz, L., Ming, Y., Zhao, M., Golaz, J., Ginoux, P., Lin, S., Schwarzkopf, M., Austin, J., Alaka, G., Cooke, W., Delworth, T., Freidenreich, S., Gordon, C., Griffies, S., Held, I., Hurlin, W., Klein, S., Knutson, T., Langenhorst, A., Lee, H., Lin, Y., Magi, B., Malyshev, S., Milly, P., Naik, V., Nath, M., Pincus, R., Ploshay, J., Ramaswamy, V., Seman, C., Shevliakova, E., Sirutis, J., Stern, W., Stouffer, R., Wilson, R., Winton, M., Wittenberg, A., and Zeng, F.: The Dynamical Core, Physical Parameterizations, and Basic Simulation Characteristics of the Atmospheric Component AM3 of the GFDL Global Coupled Model CM3, J. Climate, 24, 3484–3519, https://doi.org/10.1175/2011JCLI3955.1, 2011. a
Dubovik, O., Holben, B., Eck, T., Smirnov, A., Kaufman, Y., King, M., Tanré, D., and Slutsker, I.: Variability of Absorption and Optical Properties of Key Aerosol Types Observed in Worldwide Locations, J. Atmos. Sci., 59, 590–608, https://doi.org/10.1175/1520-0469(2002)059<0590:VOAAOP>2.0.CO;2, 2002. a, b, c, d, e, f
Flemming, J., Huijnen, V., Arteta, J., Bechtold, P., Beljaars, A., Blechschmidt, A.-M., Diamantakis, M., Engelen, R. J., Gaudel, A., Inness, A., Jones, L., Josse, B., Katragkou, E., Marecal, V., Peuch, V.-H., Richter, A., Schultz, M. G., Stein, O., and Tsikerdekis, A.: Tropospheric chemistry in the Integrated Forecasting System of ECMWF, Geosci. Model Dev., 8, 975–1003, https://doi.org/10.5194/gmd-8-975-2015, 2015. a, b
Flemming, J., Benedetti, A., Inness, A., Engelen, R. J., Jones, L., Huijnen, V., Remy, S., Parrington, M., Suttie, M., Bozzo, A., Peuch, V.-H., Akritidis, D., and Katragkou, E.: The CAMS interim Reanalysis of Carbon Monoxide, Ozone and Aerosol for 2003–2015, Atmos. Chem. Phys., 17, 1945–1983, https://doi.org/10.5194/acp-17-1945-2017, 2017. a, b, c, d
Fouquart, Y., Bonnel, B., Brogniez, G., Buriez, J., Smith, L., Morcrette, J., and Cerf, A.: Observations of Saharan aerosols: Results of ECLATS field experiment. Part II: Broadband radiative characteristics of the aerosols and vertical radiative flux divergence, J. Climate Appl. Meteor., 26, 38–52, 1987. a, b
Geer, A. J.: Significance of changes in medium-range forecast scores, Tellus A, 68, 30229, https://doi.org/10.3402/tellusa.v68.30229, 2016. a
Giles, D. M., Holben, B. N. , Eck, T. F. , Sinyuk, A. , Smirnov, A. , Slutsker, I., Dickerson, R. R. , Thompson, A. M., and Schafer, J. S.: An analysis of AERONET aerosol absorption properties and classifications representative of aerosol source regions, J. Geophys. Res., 117, D17203, https://doi.org/10.1029/2012JD018127, 2012.
Guelle, W., Schulz, M., Balkanski, Y., and Dentener, F.: Influence of the source formulation on modeling the atmospheric global distribution of the sea salt aerosol, J. Geophys. Res., 106, 27509–27524, 2001.
Granier, C., Bessagnet, B., Bond, T., D'angiola, A., van der Gon, H. D., Frost, G. J., Heil, A., Kaiser, J. W., Kinne, S., Klimont, Z., Kloster, S., Lamarque, J.-F., Liousse, C., Masui, T., Meleux, F., Mieville, A., Ohara, T., Raut, J.-C., Riahi, K., Schultz, M. G., Smith, S. J., Thompson, A., van Aardenne, J., van der Werf, G. R., and van Vuuren, D. P.: Evolution of anthropogenic and biomass burning emissions of air pollutants at global and regional scales during the 1980–2010 period, Clim. Change, 109, 163, https://doi.org/10.1007/s10584-011-0154-1, 2011. a
Haywood, J. and Boucher, O.: Estimates of the direct and indirect radiative forcing due to tropospheric aerosols: A review, Rev. Geophys., 38, 513–543, 2000. a
Haywood, J., Francis, P., Osborne, S., Glew, M., Loeb, N., Highwood, E., Tanré, D., Myhre, G., Formenti, P., and Hirst, E.: Radiative properties and direct radiative effect of Saharan dust measured by the C-130 aircraft during SHADE: 1. Solar spectrum, J. Geophys. Res., 108, 8577, https://doi.org/10.1029/2002JD002687, 2003.
Holben, B. N., Eck, T. F., Slutsker, I., Tanré, D., Buis, J. P., Setzer, A., Vermote, E., Reagan, J. A., Kaufman, Y. J., Nakajima, T., Lavenu, F., Jankowiak, I., Smirnov, A.: AERONET-A Federated Instrument Network and Data Archive for Aerosol Characterization, Remote Sens. Environ., 66, 1–16 , https://doi.org/10.1016/S0034-4257(98)00031-5, 1998. a, b
Holben, B. N., Tanré, D., Smirnov, A., Eck, T. F., Slutsker, I., Abuhassan, N., Newcomb, W. W., Schafer, J. S., Chatenet, B., Lavenu, F., Kaufman, Y. J., Vande Castle, J., Setzer, A., Markham, B., Clark, D., Frouin, R., Halthore, R., Karneli, A., O'Neill, N. T., Pietras, C., Pinker, R. T., Voss, K., and Zibordi, G.: An emerging ground‐based aerosol climatology: Aerosol optical depth from AERONET, J. Geophys. Res., 106, 12067–12097, https://doi.org/10.1029/2001JD900014, 2001. a, b
Holben, B. N., Eck, T. F., Slutsker, I., Smirnov, A., Sinyuk, A., Schafer, J., Giles, D. and Dubovik, O., AERONET’s Version 2.0 quality assurance criteria, in Remote Sensing of the Atmosphere and Clouds, Proc. SPIE, 64080Q, https://doi.org/10.1117/12.706524, 2006. a, b
Hollingsworth A., Engelen, R. J., Benedetti, A., Dethof, A., Flemming, J., Kaiser, J. W., Morcrette, J.-J., Simmons, A. J., Textor, C., Boucher, O., Chevallier, F., Rayner, P., Elbern, H., Eskes, H., Granier, C., Peuch, V. H., Rouil, L., Schultz, M. G., and the GEMS consortium: Toward a Monitoring and Forecasting System For Atmospheric Composition: The GEMS Project, B. Am. Meteorol. Soc., 89, 1147–1164, https://doi.org/10.1175/2008BAMS2355.1, 2008. a
Huffman, G. J., Adler, R. F., Bolvin, D. T., Gu, G., Nelkin, E. J., Bowman, K. P., Hong, Y., Stocker, E. F., Wolff, D.B.: The TRMM Multi-satellite Precipitation Analysis: Quasi-Global, Multi-Year, Combined-Sensor Precipitation Estimates at Fine Scale, J. Hydrometeor., 8, 38–55, 2007. a
Huffman, G. J., Adler, R. F., Bolvin, D. T., and Nelkin, E. J.: The TRMM Multi-satellite Precipitation Analysis (TMPA), chap. 1, in: Satellite Rainfall Applications for Surface Hydrology, edited by: Hossain, F. and Gebremichael, M., Springer Verlag, 3–22, ISBN: 978-90-481-2914-0, 2010. a
Huffman, G. J., Bolvin, D. T., Nelkin, E. J., and Adler, R. F.: GPCP Version 2.2 Combined Precipitation Data Set, Research Data Archive at the National Center for Atmospheric Research, Computational and Information Systems Laboratory, https://doi.org/10.5065/D6R78C9S, 2015. a
Inness, A., Baier, F., Benedetti, A., Bouarar, I., Chabrillat, S., Clark, H., Clerbaux, C., Coheur, P., Engelen, R. J., Errera, Q., Flemming, J., George, M., Granier, C., Hadji-Lazaro, J., Huijnen, V., Hurtmans, D., Jones, L., Kaiser, J. W., Kapsomenakis, J., Lefever, K., Leitão, J., Razinger, M., Richter, A., Schultz, M. G., Simmons, A. J., Suttie, M., Stein, O., Thépaut, J.-N., Thouret, V., Vrekoussis, M., Zerefos, C., and the MACC team: The MACC reanalysis: an 8 yr data set of atmospheric composition, Atmos. Chem. Phys., 13, 4073–4109, https://doi.org/10.5194/acp-13-4073-2013, 2013. a
Inness, A., Ades, M., Agustí-Panareda, A., Barré, J., Benedictow, A., Blechschmidt, A.-M., Dominguez, J. J., Engelen, R., Eskes, H., Flemming, J., Huijnen, V., Jones, L., Kipling, Z., Massart, S., Parrington, M., Peuch, V.-H., Razinger, M., Remy, S., Schulz, M., and Suttie, M.: The CAMS reanalysis of atmospheric composition, Atmos. Chem. Phys., 19, 3515–3556, https://doi.org/10.5194/acp-19-3515-2019, 2019. a, b
Jin, Q., Wei, J., Yang, Z.-L., Pu, B., and Huang, J.: Consistent response of Indian summer monsoon to Middle East dust in observations and simulations, Atmos. Chem. Phys., 15, 9897–9915, https://doi.org/10.5194/acp-15-9897-2015, 2015. a, b
Jin, Q., Yang, Z.-L., and Wei, J.: High sensitivity of Indian summer monsoon to Middle East dust absorptive properties, Sci. Rep., 6, 30690, https://doi.org/10.1038/srep30690, 2016. a, b
Kaiser, J. W., Heil, A., Andreae, M. O., Benedetti, A., Chubarova, N., Jones, L., Morcrette, J.-J., Razinger, M., Schultz, M. G., Suttie, M., and van der Werf, G. R.: Biomass burning emissions estimated with a global fire assimilation system based on observed fire radiative power, Biogeosciences, 9, 527–554, https://doi.org/10.5194/bg-9-527-2012, 2012. a
Kinne, S., O'Donnel, D., Stier, P., Kloster, S., Zhang, K., Schmidt, H., Rast, S., Giorgetta, M., Eck, T. F., and Stevens, B.: MAC-v1: A new global aerosol climatology for climate studies, J. Adv. Model. Earth Syst., 5, 704–740, https://doi.org/10.1002/jame.20035, 2013. a
Kim, D., Chin, M., Yu, H., Eck, T. F., Sinyuk, A., Smirnov, A., and Holben, B. N.: Dust optical properties over North Africa and Arabian Peninsula derived from the AERONET dataset, Atmos. Chem. Phys., 11, 10733–10741, https://doi.org/10.5194/acp-11-10733-2011, 2011.
Koepke, P., Hess, M., Schult, I., and Shettle, E. P.: Global Aerosol Data Set, Report No. 243, Max-Planck-Institut für Meteorologie, Hamburg, ISSN: 0937-1060, 1997. a
Lau, K. M. and Kim, K. M.: Observational relationships between aerosol and Asian monsoon rainfall, and circulation, Geophys. Res. Lett., 33, L21810, https://doi.org/10.1029/2006GL027546, 2006. a
Levy, R. C., Remer, L. A., Kleidman, R. G., Mattoo, S., Ichoku, C., Kahn, R., and Eck, T. F.: Global evaluation of the Collection 5 MODIS dark-target aerosol products over land, Atmos. Chem. Phys., 10, 10399–10420, https://doi.org/10.5194/acp-10-10399-2010, 2010.
Liu, H., Pinker, R. T., and Holben, B. N.:, A global view of aerosols from merged transport models, satellite, and ground observations, J. Geophys. Res., 110, D10S15, https://doi.org/10.1029/2004JD004695, 2005. a
Menon, S., Del Genio, A. D., Koch, D., and Tselioudis, G.: GCM simulations of the aerosol indirect effect: Sensitivity to cloud parameterization and aerosol burden. J. Atmos. Sci., 59, 692–713, https://doi.org/10.1175/1520-0469(2002)059, 2002. a
Monahan, E. C., Spiel, D. C., and Davidson, K. L.: A model of marine aerosol generation via whitecaps and wave disruption, in: Oceanic Whitecaps, edited by: Monahan, E. C. and Mac Niocaill, G., D. Reidel, Norwell, Massachusetts, 167–174, 1986. a
Morcrette, J.-J., Barker, H. W., Cole, J. N. S., Iacono, M. J., and Pincus, R.: Impact of a new radiationpackage, McRad, in the ECMWF Integrated Forecasting System, Mon. Weather Rev., 136, 4773–4798, 2008a. a
Morcrette, J.-J., Beljaars, A., Benedetti, A., Jones, L., and Boucher, O.: Sea-salt and dust aerosols in the ECMWF IFS model, Geophys. Res. Lett., 35, L24813, https://doi.org/10.1029/2008GL036041, 2008b. a
Morcrette, J.-J., Boucher, O. , Jones, L., Salmond, D., Bechtold, P., Beljaars, A., Benedetti, A., Boner, A., Kaiser, J. W., Razinger, M., Schulz, M., Serrar, S., Simmons, A. J., Sofiev, M., Suttie, M., Tompkins, A. M., and Untch, A.: Aerosol analysis and forecast in the European Centre for Medium-Range Weather Forecasts Integrated Forecast System. Part 1: Forward modelling, J. Geophys. Res.-Atmos., 114, D06206, https://doi.org/10.1029/2008JD011235, 2009. a, b, c
Mulcahy, J. P., Walters, D. N., Bellouin, N., and Milton, S. F.: Impacts of increasing the aerosol complexity in the Met Office global numerical weather prediction model, Atmos. Chem. Phys., 14, 4749–4778, https://doi.org/10.5194/acp-14-4749-2014, 2014. a, b, c, d
Parrish, D. F. and Derber, J. C.: The National Meteorological Center's spectral statistical-interpolation analysis system, Mon. Weather Rev., 120, 1747–1763, 1992.
Reale, O., Lau, K. M., and Da Silva, A.: Impact of an Interactive Aerosol on the African Easterly Jet in the NASA GEOS-5 Global Forecasting System, Weather Forecast., 26, 504–519, 2011. a
Reddy, M. S., Boucher, O., Bellouin, N., Schulz, M., Balkanski, Y., Dufresne, J.-L., and Pham, M.: Estimates of global multicomponent aerosol optical depth and direct radiative perturbation in the Laboratoire de Meteorologie Dynamique general circulation model, J. Geophys. Res.-Atmos., 110, D10S16, https://doi.org/10.1029/2004JD004757, 2005. a, b, c
Rémy, S., Benedetti, A., Bozzo, A., Haiden, T., Jones, L., Razinger, M., Flemming, J., Engelen, R. J., Peuch, V. H., and Thepaut, J. N.: Feedbacks of dust and boundary layer meteorology during a dust storm in the eastern Mediterranean, Atmos. Chem. Phys., 15, 12909–12933, https://doi.org/10.5194/acp-15-12909-2015, 2015. a, b
Rémy, S., Kipling, Z., Flemming, J., Boucher, O., Nabat, P., Michou, M., Bozzo, A., Ades, M., Huijnen, V., Benedetti, A., Engelen, R., Peuch, V.-H., and Morcrette, J.-J.: Description and evaluation of the tropospheric aerosol scheme in the European Centre for Medium-Range Weather Forecasts (ECMWF) Integrated Forecasting System (IFS-AER, cycle 45R1), Geosci. Model Dev., 12, 4627–4659, https://doi.org/10.5194/gmd-12-4627-2019, 2019. a, b, c, d, e, f, g
Rodwell, M. J. and Jung, T.: Understanding the local and global impacts of model physics changes: an aerosol example, Q. J. Roy. Meteor. Soc., 134, 1479–1497, https://doi.org/10.1002/qj.298, 2008. a, b
Schulz, M., de Leeuw, G., and Balkanski, Y.: Sea-salt aerosol source functions and emissions, in: Emission of Atmospheric Trace Compounds, edited by: Granier, C., Artaxo, P., and Reeves, C. E., Kluwer Acad., Norwell, Mass, 333–354, 2004.
Simmons, A. J.: Monitoring Atmospheric Composition and Climate, ECMWF Newsletter, 123, 10–13, 2010. a
Solomon, S., Daniel, J. S., Neely III, R. R., Vernier, J. P., Dutton, E. G., and Thomason, L. W.: The persistently variable “background” stratospheric aerosol layer and global climate change, Science, 12, 866–870, https://doi.org/10.1126/science, 2011.
Stier, P., Feichter, J., Kinne, S., Kloster, S., Vignati, E., Wilson, J., Ganzeveld, L., Tegen, I., Werner, M., Balkanski, Y., Schulz, M., Boucher, O., Minikin, A., and Petzold, A.: The aerosol-climate model ECHAM5-HAM, Atmos. Chem. Phys., 5, 1125–1156, https://doi.org/10.5194/acp-5-1125-2005, 2005. a
Toll, V., Reis, K., Ots, R., Kaasik, M., Männik, A., Prank, M., and Sofiev, M.: SILAM and MACC reanalysis aerosol data used for simulating the aerosol direct radiative effect with the NWP model HARMONIE for summer 2010 wildfire case in Russia, Atmos. Environ., 121, 75–85, https://doi.org/10.1016/j.atmosenv.2015.06.007, 2015. a, b
Toll, V., Gleeson, E., Nielsen, K. P., Männik, A., Mas̈ek, J., Rontu, L., and Post, P.: Impacts of the direct radiative effect of aerosols in numerical weather prediction over Europe using the ALADIN-HIRLAM NWP system, Atmos. Res., 172–173, 163–173, https://doi.org/10.1016/j.atmosres.2016.01.003, 2016. a, b
Tompkins, A. M., Cardinali, C., Morcrette, J.-J., and Rodwell, M.: Influence of aerosol climatology on forecasts of the African Easterly Jet, Geophys. Res. Lett., 32, L10801, https://doi.org/10.1029/2004GL022189, 2005. a
Vinoj, V., Rasch, P. J., Wang, H., Yoon, J.-H., Ma, P.-L., Landu, K., and Singh, B.: Short-term modulation of Indian summer monsoon rainfall by West Asian dust, Nat. Geosci., 7, 308–313, https://doi.org/10.1038/ngeo2107, 2014. a, b, c
Yu, H., Chin, M., Winker, D. M., Omar, A. H., Liu, Z., Kittaka, C., and Diehl, T.: Global view of aerosol vertical distributions from CALIPSO lidar measurements and GOCART simulations: Regional and seasonal variations, J. Geophys. Res., 115, D00H30, https://doi.org/10.1029/2009JD013364, 2010.
Wang, C., Kim, D., Ekman, A. M. L., Barth, M. C., and Rasch, P. J.: Impact of anthropogenic aerosols on Indian summer monsoon, Geophys. Res. Lett., 36, L21704, https://doi.org/10.1029/2009GL040114, 2009. a
Wentz, F. J., Hilburn, K. A., and Smith, D. K.: Remote Sensing Systems DMSP [SSM/I] [Monthly] Environmental Suite on 0.25 deg grid, Version 7, Remote Sensing Systems, Santa Rosa, CA, available at: http://www.remss.com/missions/ssmi/ (last access: 31 October 2019), 2012. a
Winker, D. M., Tackett, J. L., Getzewich, B. J., Liu, Z., Vaughan, M. A., and Rogers, R. R.: The global 3-D distribution of tropospheric aerosols as characterized by CALIOP, Atmos. Chem. Phys., 13, 3345–3361, https://doi.org/10.5194/acp-13-3345-2013, 2013.
Woodward, S.: Modeling the atmospheric life cycle and radiative impact of mineral dust in the Hadley Centre climate model, J. Geophys. Res., 106, 18155–18166, https://doi.org/10.1029/2000JD900795, 2001. a, b, c, d
Zhang, J., Reid, J. S., Christensen, M., and Benedetti, A.: An evaluation of the impact of aerosol particles on weather forecasts from a biomass burning aerosol event over the Midwestern United States: observational-based analysis of surface temperature, Atmos. Chem. Phys., 16, 6475–6494, https://doi.org/10.5194/acp-16-6475-2016, 2016. a
Short summary
Aerosols are tiny particles of natural and anthropogenic origin transported by the winds in the Earth's atmosphere. These particles play a key role in the energy budget of our planet. In numerical models of the Earth's atmosphere, aerosols spatial distribution are often represented by conditions averaged over several years. We prepared a new aerosol climatology and used it in a numerical weather model. We show that in certain regions aerosols can affect the quality of numerical weather forecast.
Aerosols are tiny particles of natural and anthropogenic origin transported by the winds in the...
