Articles | Volume 18, issue 18
https://doi.org/10.5194/gmd-18-6023-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/gmd-18-6023-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Development and technical paper
| 
16 Sep 2025
Development and technical paper |
| 16 Sep 2025
| 16 Sep 2025
REtrieval Method for optical and physical Aerosol Properties in the stratosphere (REMAPv1)
Andrin Jörimann
CORRESPONDING AUTHOR
Physikalisch-Meteorologisches Observatorium Davos/World Radiation Center, Davos, Switzerland
Institute for Particle Physics and Astrophysics, ETH Zürich, Zurich, Switzerland
Timofei Sukhodolov
Physikalisch-Meteorologisches Observatorium Davos/World Radiation Center, Davos, Switzerland
Beiping Luo
Institute for Atmospheric and Climate Science, ETH Zürich, Zurich, Switzerland
Gabriel Chiodo
Institute for Atmospheric and Climate Science, ETH Zürich, Zurich, Switzerland
Instituto de Geociencias, Spanish National Research Council (IGEO-CSIC-UCM), Madrid, Spain
Graham Mann
School of Earth and Environment, University of Leeds, Leeds, UK
UK National Centre for Atmospheric Science, University of Leeds, Leeds, UK
Thomas Peter
Institute for Atmospheric and Climate Science, ETH Zürich, Zurich, Switzerland
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Marina Friedel, Gabriel Chiodo, Timofei Sukhodolov, James Keeble, Thomas Peter, Svenja Seeber, Andrea Stenke, Hideharu Akiyoshi, Eugene Rozanov, David Plummer, Patrick Jöckel, Guang Zeng, Olaf Morgenstern, and Béatrice Josse
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Tatiana Egorova, Jan Sedlacek, Timofei Sukhodolov, Arseniy Karagodin-Doyennel, Franziska Zilker, and Eugene Rozanov
Atmos. Chem. Phys., 23, 5135–5147, https://doi.org/10.5194/acp-23-5135-2023, https://doi.org/10.5194/acp-23-5135-2023, 2023
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This paper describes the climate and atmosphere benefits of the Montreal Protocol, simulated with the state-of-the-art Earth system model SOCOLv4.0. We have added to and confirmed the previous studies by showing that without the Montreal Protocol by the end of the 21st century there would be a dramatic reduction in the ozone layer as well as substantial perturbation of the essential climate variables in the troposphere caused by the warming from increasing ozone-depleting substances.
Daniele Visioni, Ben Kravitz, Alan Robock, Simone Tilmes, Jim Haywood, Olivier Boucher, Mark Lawrence, Peter Irvine, Ulrike Niemeier, Lili Xia, Gabriel Chiodo, Chris Lennard, Shingo Watanabe, John C. Moore, and Helene Muri
Atmos. Chem. Phys., 23, 5149–5176, https://doi.org/10.5194/acp-23-5149-2023, https://doi.org/10.5194/acp-23-5149-2023, 2023
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Anand Kumar, Kristian Klumpp, Chen Barak, Giora Rytwo, Michael Plötze, Thomas Peter, and Claudia Marcolli
Atmos. Chem. Phys., 23, 4881–4902, https://doi.org/10.5194/acp-23-4881-2023, https://doi.org/10.5194/acp-23-4881-2023, 2023
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Smectites are a major class of clay minerals that are ice nucleation (IN) active. They form platelets that swell or even delaminate in water by intercalation of water between their layers. We hypothesize that at least three smectite layers need to be stacked together to host a critical ice embryo on clay mineral edges and that the larger the surface edge area is, the higher the freezing temperature. Edge sites on such clay particles play a crucial role in imparting IN ability to such particles.
Arseniy Karagodin-Doyennel, Eugene Rozanov, Timofei Sukhodolov, Tatiana Egorova, Jan Sedlacek, and Thomas Peter
Atmos. Chem. Phys., 23, 4801–4817, https://doi.org/10.5194/acp-23-4801-2023, https://doi.org/10.5194/acp-23-4801-2023, 2023
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Alexander D. James, Finn Pace, Sebastien N. F. Sikora, Graham W. Mann, John M. C. Plane, and Benjamin J. Murray
Atmos. Chem. Phys., 23, 2215–2233, https://doi.org/10.5194/acp-23-2215-2023, https://doi.org/10.5194/acp-23-2215-2023, 2023
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Kristian Klumpp, Claudia Marcolli, Ana Alonso-Hellweg, Christopher H. Dreimol, and Thomas Peter
Atmos. Chem. Phys., 23, 1579–1598, https://doi.org/10.5194/acp-23-1579-2023, https://doi.org/10.5194/acp-23-1579-2023, 2023
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Ilaria Quaglia, Claudia Timmreck, Ulrike Niemeier, Daniele Visioni, Giovanni Pitari, Christina Brodowsky, Christoph Brühl, Sandip S. Dhomse, Henning Franke, Anton Laakso, Graham W. Mann, Eugene Rozanov, and Timofei Sukhodolov
Atmos. Chem. Phys., 23, 921–948, https://doi.org/10.5194/acp-23-921-2023, https://doi.org/10.5194/acp-23-921-2023, 2023
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The last very large explosive volcanic eruption we have measurements for is the eruption of Mt. Pinatubo in 1991. It is therefore often used as a benchmark for climate models' ability to reproduce these kinds of events. Here, we compare available measurements with the results from multiple experiments conducted with climate models interactively simulating the aerosol cloud formation.
Arseniy Karagodin-Doyennel, Eugene Rozanov, Timofei Sukhodolov, Tatiana Egorova, Jan Sedlacek, William Ball, and Thomas Peter
Atmos. Chem. Phys., 22, 15333–15350, https://doi.org/10.5194/acp-22-15333-2022, https://doi.org/10.5194/acp-22-15333-2022, 2022
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Applying the dynamic linear model, we confirm near-global ozone recovery (55°N–55°S) in the mesosphere, upper and middle stratosphere, and a steady increase in the troposphere. We also show that modern chemistry–climate models (CCMs) like SOCOLv4 may reproduce the observed trend distribution of lower stratospheric ozone, despite exhibiting a lower magnitude and statistical significance. The obtained ozone trend pattern in SOCOLv4 is generally consistent with observations and reanalysis datasets.
Nikou Hamzehpour, Claudia Marcolli, Sara Pashai, Kristian Klumpp, and Thomas Peter
Atmos. Chem. Phys., 22, 14905–14930, https://doi.org/10.5194/acp-22-14905-2022, https://doi.org/10.5194/acp-22-14905-2022, 2022
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Playa surfaces in Iran that emerged through Lake Urmia (LU) desiccation have become a relevant dust source of regional relevance. Here, we identify highly erodible LU playa surfaces and determine their physicochemical properties and mineralogical composition and perform emulsion-freezing experiments with them. We find high ice nucleation activities (up to 250 K) that correlate positively with organic matter and clay content and negatively with pH, salinity, K-feldspars, and quartz.
Nikou Hamzehpour, Claudia Marcolli, Kristian Klumpp, Debora Thöny, and Thomas Peter
Atmos. Chem. Phys., 22, 14931–14956, https://doi.org/10.5194/acp-22-14931-2022, https://doi.org/10.5194/acp-22-14931-2022, 2022
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Dust aerosols from dried lakebeds contain mineral particles, as well as soluble salts and (bio-)organic compounds. Here, we investigate ice nucleation (IN) activity of dust samples from Lake Urmia playa, Iran. We find high IN activity of the untreated samples that decreases after organic matter removal but increases after removing soluble salts and carbonates, evidencing inhibiting effects of soluble salts and carbonates on the IN activity of organic matter and minerals, especially microcline.
Marina Friedel, Gabriel Chiodo, Andrea Stenke, Daniela I. V. Domeisen, and Thomas Peter
Atmos. Chem. Phys., 22, 13997–14017, https://doi.org/10.5194/acp-22-13997-2022, https://doi.org/10.5194/acp-22-13997-2022, 2022
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In spring, winds the Arctic stratosphere change direction – an event called final stratospheric warming (FSW). Here, we examine whether the interannual variability in Arctic stratospheric ozone impacts the timing of the FSW. We find that Arctic ozone shifts the FSW to earlier and later dates in years with high and low ozone via the absorption of UV light. The modulation of the FSW by ozone has consequences for surface climate in ozone-rich years, which may result in better seasonal predictions.
Nora Bergner, Marina Friedel, Daniela I. V. Domeisen, Darryn Waugh, and Gabriel Chiodo
Atmos. Chem. Phys., 22, 13915–13934, https://doi.org/10.5194/acp-22-13915-2022, https://doi.org/10.5194/acp-22-13915-2022, 2022
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Polar vortex extremes, particularly situations with an unusually weak cyclonic circulation in the stratosphere, can influence the surface climate in the spring–summer time in the Southern Hemisphere. Using chemistry-climate models and observations, we evaluate the robustness of the surface impacts. While models capture the general surface response, they do not show the observed climate patterns in midlatitude regions, which we trace back to biases in the models' circulations.
Juan-Carlos Antuña-Marrero, Graham W. Mann, John Barnes, Abel Calle, Sandip S. Dhomse, Victoria E. Cachorro-Revilla, Terry Deshler, Li Zhengyao, Nimmi Sharma, and Louis Elterman
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2022-272, https://doi.org/10.5194/essd-2022-272, 2022
Revised manuscript not accepted
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Tropospheric and stratospheric aerosol extinction profiles observations from a searchlight at New Mexico, US, were rescued and re-calibrated. Spanning between December 1963 and 1964, they measured the volcanic aerosols from the 1963 Agung eruption. Contemporary and state of the art information were used in the re-calibration. A unique and until the present forgotten/ignored dataset, it contributes current observational and modelling research on the impact of major volcanic eruptions on climate.
Clare E. Singer, Benjamin W. Clouser, Sergey M. Khaykin, Martina Krämer, Francesco Cairo, Thomas Peter, Alexey Lykov, Christian Rolf, Nicole Spelten, Armin Afchine, Simone Brunamonti, and Elisabeth J. Moyer
Atmos. Meas. Tech., 15, 4767–4783, https://doi.org/10.5194/amt-15-4767-2022, https://doi.org/10.5194/amt-15-4767-2022, 2022
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In situ measurements of water vapor in the upper troposphere are necessary to study cloud formation and hydration of the stratosphere but challenging due to cold–dry conditions. We compare measurements from three water vapor instruments from the StratoClim campaign in 2017. In clear sky (clouds), point-by-point differences were <1.5±8 % (<1±8 %). This excellent agreement allows detection of fine-scale structures required to understand the impact of convection on stratospheric water vapor.
Irina Mironova, Miriam Sinnhuber, Galina Bazilevskaya, Mark Clilverd, Bernd Funke, Vladimir Makhmutov, Eugene Rozanov, Michelle L. Santee, Timofei Sukhodolov, and Thomas Ulich
Atmos. Chem. Phys., 22, 6703–6716, https://doi.org/10.5194/acp-22-6703-2022, https://doi.org/10.5194/acp-22-6703-2022, 2022
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From balloon measurements, we detected unprecedented, extremely powerful, electron precipitation over the middle latitudes. The robustness of this event is confirmed by satellite observations of electron fluxes and chemical composition, as well as by ground-based observations of the radio signal propagation. The applied chemistry–climate model shows the almost complete destruction of ozone in the mesosphere over the region where high-energy electrons were observed.
Kristian Klumpp, Claudia Marcolli, and Thomas Peter
Atmos. Chem. Phys., 22, 3655–3673, https://doi.org/10.5194/acp-22-3655-2022, https://doi.org/10.5194/acp-22-3655-2022, 2022
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Surface interactions with solutes can significantly alter the ice nucleation activity of mineral dust. Past studies revealed the sensitivity of microcline, one of the most ice-active types of dust in the atmosphere, to inorganic solutes. This study focuses on the interaction of microcline with bio-organic substances and the resulting effects on its ice nucleation activity. We observe strongly hampered ice nucleation activity due to the presence of carboxylic and amino acids but not for polyols.
Davide Zanchettin, Claudia Timmreck, Myriam Khodri, Anja Schmidt, Matthew Toohey, Manabu Abe, Slimane Bekki, Jason Cole, Shih-Wei Fang, Wuhu Feng, Gabriele Hegerl, Ben Johnson, Nicolas Lebas, Allegra N. LeGrande, Graham W. Mann, Lauren Marshall, Landon Rieger, Alan Robock, Sara Rubinetti, Kostas Tsigaridis, and Helen Weierbach
Geosci. Model Dev., 15, 2265–2292, https://doi.org/10.5194/gmd-15-2265-2022, https://doi.org/10.5194/gmd-15-2265-2022, 2022
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This paper provides metadata and first analyses of the volc-pinatubo-full experiment of CMIP6-VolMIP. Results from six Earth system models reveal significant differences in radiative flux anomalies that trace back to different implementations of volcanic forcing. Surface responses are in contrast overall consistent across models, reflecting the large spread due to internal variability. A second phase of VolMIP shall consider both aspects toward improved protocol for volc-pinatubo-full.
Debra K. Weisenstein, Daniele Visioni, Henning Franke, Ulrike Niemeier, Sandro Vattioni, Gabriel Chiodo, Thomas Peter, and David W. Keith
Atmos. Chem. Phys., 22, 2955–2973, https://doi.org/10.5194/acp-22-2955-2022, https://doi.org/10.5194/acp-22-2955-2022, 2022
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This paper explores a potential method of geoengineering that could be used to slow the rate of change of climate over decadal scales. We use three climate models to explore how injections of accumulation-mode sulfuric acid aerosol change the large-scale stratospheric particle size distribution and radiative forcing response for the chosen scenarios. Radiative forcing per unit sulfur injected and relative to the change in aerosol burden is larger with particulate than with SO2 injections.
Sandip S. Dhomse, Martyn P. Chipperfield, Wuhu Feng, Ryan Hossaini, Graham W. Mann, Michelle L. Santee, and Mark Weber
Atmos. Chem. Phys., 22, 903–916, https://doi.org/10.5194/acp-22-903-2022, https://doi.org/10.5194/acp-22-903-2022, 2022
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Solar flux variations associated with 11-year sunspot cycle is believed to exert important external climate forcing. As largest variations occur at shorter wavelengths such as ultra-violet part of the solar spectrum, associated changes in stratospheric ozone are thought to provide direct evidence for solar climate interaction. Until now, most of the studies reported double-peak structured solar cycle signal (SCS), but relatively new satellite data suggest only single-peak-structured SCS.
Kseniia Golubenko, Eugene Rozanov, Gennady Kovaltsov, Ari-Pekka Leppänen, Timofei Sukhodolov, and Ilya Usoskin
Geosci. Model Dev., 14, 7605–7620, https://doi.org/10.5194/gmd-14-7605-2021, https://doi.org/10.5194/gmd-14-7605-2021, 2021
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A new full 3-D time-dependent model, based on SOCOL-AERv2, of beryllium atmospheric production, transport, and deposition has been developed and validated using directly measured data. The model is recommended to be used in studies related to, e.g., atmospheric dynamical patterns, extreme solar particle storms, long-term solar activity reconstruction from cosmogenic proxy data, and solar–terrestrial relations.
Arseniy Karagodin-Doyennel, Eugene Rozanov, Timofei Sukhodolov, Tatiana Egorova, Alfonso Saiz-Lopez, Carlos A. Cuevas, Rafael P. Fernandez, Tomás Sherwen, Rainer Volkamer, Theodore K. Koenig, Tanguy Giroud, and Thomas Peter
Geosci. Model Dev., 14, 6623–6645, https://doi.org/10.5194/gmd-14-6623-2021, https://doi.org/10.5194/gmd-14-6623-2021, 2021
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Here, we present the iodine chemistry module in the SOCOL-AERv2 model. The obtained iodine distribution demonstrated a good agreement when validated against other simulations and available observations. We also estimated the iodine influence on ozone in the case of present-day iodine emissions, the sensitivity of ozone to doubled iodine emissions, and when considering only organic or inorganic iodine sources. The new model can be used as a tool for further studies of iodine effects on ozone.
Juan-Carlos Antuña-Marrero, Graham W. Mann, John Barnes, Albeht Rodríguez-Vega, Sarah Shallcross, Sandip S. Dhomse, Giorgio Fiocco, and Gerald W. Grams
Earth Syst. Sci. Data, 13, 4407–4423, https://doi.org/10.5194/essd-13-4407-2021, https://doi.org/10.5194/essd-13-4407-2021, 2021
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The first multi-year stratospheric aerosol lidar dataset was recovered and recalibrated. The vertical profile dataset, January 1964 to August 1965 at Lexington, MA, and July to August 1964 at Fairbanks, AK, provides info on volcanic forcing after the 1963 Agung eruption. Applying two-way transmittance correction to the original dataset reveals data variations, with corrected stratospheric aerosol optical depth (sAOD) highest in 1965 with the highest 532 nm sAOD peak at 0.07 in March 1965.
Timofei Sukhodolov, Tatiana Egorova, Andrea Stenke, William T. Ball, Christina Brodowsky, Gabriel Chiodo, Aryeh Feinberg, Marina Friedel, Arseniy Karagodin-Doyennel, Thomas Peter, Jan Sedlacek, Sandro Vattioni, and Eugene Rozanov
Geosci. Model Dev., 14, 5525–5560, https://doi.org/10.5194/gmd-14-5525-2021, https://doi.org/10.5194/gmd-14-5525-2021, 2021
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This paper features the new atmosphere–ocean–aerosol–chemistry–climate model SOCOLv4.0 and its validation. The model performance is evaluated against reanalysis products and observations of atmospheric circulation and trace gas distribution, with a focus on stratospheric processes. Although we identified some problems to be addressed in further model upgrades, we demonstrated that SOCOLv4.0 is already well suited for studies related to chemistry–climate–aerosol interactions.
Ralf Weigel, Christoph Mahnke, Manuel Baumgartner, Antonis Dragoneas, Bärbel Vogel, Felix Ploeger, Silvia Viciani, Francesco D'Amato, Silvia Bucci, Bernard Legras, Beiping Luo, and Stephan Borrmann
Atmos. Chem. Phys., 21, 11689–11722, https://doi.org/10.5194/acp-21-11689-2021, https://doi.org/10.5194/acp-21-11689-2021, 2021
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In July and August 2017, eight StratoClim mission flights of the Geophysica reached up to 20 km in the Asian monsoon anticyclone. New particle formation (NPF) was identified in situ by abundant nucleation-mode aerosols (6–15 nm in diameter) with mixing ratios of up to 50 000 mg−1. NPF occurred most frequently at 12–16 km with fractions of non-volatile residues of down to 15 %. Abundance and productivity of observed NPF indicate its ability to promote the Asian tropopause aerosol layer.
Michael Weimer, Jennifer Buchmüller, Lars Hoffmann, Ole Kirner, Beiping Luo, Roland Ruhnke, Michael Steiner, Ines Tritscher, and Peter Braesicke
Atmos. Chem. Phys., 21, 9515–9543, https://doi.org/10.5194/acp-21-9515-2021, https://doi.org/10.5194/acp-21-9515-2021, 2021
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We show that we are able to directly simulate polar stratospheric clouds formed locally in a mountain wave and represent their effect on the ozone chemistry with the global atmospheric chemistry model ICON-ART. Thus, we show the first simulations that close the gap between directly resolved mountain-wave-induced polar stratospheric clouds and their representation at coarse global resolutions.
James Keeble, Birgit Hassler, Antara Banerjee, Ramiro Checa-Garcia, Gabriel Chiodo, Sean Davis, Veronika Eyring, Paul T. Griffiths, Olaf Morgenstern, Peer Nowack, Guang Zeng, Jiankai Zhang, Greg Bodeker, Susannah Burrows, Philip Cameron-Smith, David Cugnet, Christopher Danek, Makoto Deushi, Larry W. Horowitz, Anne Kubin, Lijuan Li, Gerrit Lohmann, Martine Michou, Michael J. Mills, Pierre Nabat, Dirk Olivié, Sungsu Park, Øyvind Seland, Jens Stoll, Karl-Hermann Wieners, and Tongwen Wu
Atmos. Chem. Phys., 21, 5015–5061, https://doi.org/10.5194/acp-21-5015-2021, https://doi.org/10.5194/acp-21-5015-2021, 2021
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Stratospheric ozone and water vapour are key components of the Earth system; changes to both have important impacts on global and regional climate. We evaluate changes to these species from 1850 to 2100 in the new generation of CMIP6 models. There is good agreement between the multi-model mean and observations, although there is substantial variation between the individual models. The future evolution of both ozone and water vapour is strongly dependent on the assumed future emissions scenario.
Margot Clyne, Jean-Francois Lamarque, Michael J. Mills, Myriam Khodri, William Ball, Slimane Bekki, Sandip S. Dhomse, Nicolas Lebas, Graham Mann, Lauren Marshall, Ulrike Niemeier, Virginie Poulain, Alan Robock, Eugene Rozanov, Anja Schmidt, Andrea Stenke, Timofei Sukhodolov, Claudia Timmreck, Matthew Toohey, Fiona Tummon, Davide Zanchettin, Yunqian Zhu, and Owen B. Toon
Atmos. Chem. Phys., 21, 3317–3343, https://doi.org/10.5194/acp-21-3317-2021, https://doi.org/10.5194/acp-21-3317-2021, 2021
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This study finds how and why five state-of-the-art global climate models with interactive stratospheric aerosols differ when simulating the aftermath of large volcanic injections as part of the Model Intercomparison Project on the climatic response to Volcanic forcing (VolMIP). We identify and explain the consequences of significant disparities in the underlying physics and chemistry currently in some of the models, which are problems likely not unique to the models participating in this study.
Manuel Graf, Philipp Scheidegger, André Kupferschmid, Herbert Looser, Thomas Peter, Ruud Dirksen, Lukas Emmenegger, and Béla Tuzson
Atmos. Meas. Tech., 14, 1365–1378, https://doi.org/10.5194/amt-14-1365-2021, https://doi.org/10.5194/amt-14-1365-2021, 2021
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Water vapor is the most important natural greenhouse gas. The accurate and frequent measurement of its abundance, especially in the upper troposphere and lower stratosphere (UTLS), is technically challenging. We developed and characterized a mid-IR absorption spectrometer for highly accurate water vapor measurements in the UTLS. The instrument is sufficiently small and lightweight (3.9 kg) to be carried by meteorological balloons, which enables frequent and cost-effective soundings.
Michael Steiner, Beiping Luo, Thomas Peter, Michael C. Pitts, and Andrea Stenke
Geosci. Model Dev., 14, 935–959, https://doi.org/10.5194/gmd-14-935-2021, https://doi.org/10.5194/gmd-14-935-2021, 2021
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We evaluate polar stratospheric clouds (PSCs) as simulated by the chemistry–climate model (CCM) SOCOLv3.1 in comparison with measurements by the CALIPSO satellite. A cold bias results in an overestimated PSC area and mountain-wave ice is underestimated, but we find overall good temporal and spatial agreement of PSC occurrence and composition. This work confirms previous studies indicating that simplified PSC schemes may also achieve good approximations of the fundamental properties of PSCs.
Teresa Jorge, Simone Brunamonti, Yann Poltera, Frank G. Wienhold, Bei P. Luo, Peter Oelsner, Sreeharsha Hanumanthu, Bhupendra B. Singh, Susanne Körner, Ruud Dirksen, Manish Naja, Suvarna Fadnavis, and Thomas Peter
Atmos. Meas. Tech., 14, 239–268, https://doi.org/10.5194/amt-14-239-2021, https://doi.org/10.5194/amt-14-239-2021, 2021
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Balloon-borne frost point hygrometers are crucial for the monitoring of water vapour in the upper troposphere and lower stratosphere. We found that when traversing a mixed-phase cloud with big supercooled droplets, the intake tube of the instrument collects on its inner surface a high percentage of these droplets. The newly formed ice layer will sublimate at higher levels and contaminate the measurement. The balloon is also a source of contamination, but only at higher levels during the ascent.
Jing Dou, Peter A. Alpert, Pablo Corral Arroyo, Beiping Luo, Frederic Schneider, Jacinta Xto, Thomas Huthwelker, Camelia N. Borca, Katja D. Henzler, Jörg Raabe, Benjamin Watts, Hartmut Herrmann, Thomas Peter, Markus Ammann, and Ulrich K. Krieger
Atmos. Chem. Phys., 21, 315–338, https://doi.org/10.5194/acp-21-315-2021, https://doi.org/10.5194/acp-21-315-2021, 2021
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Photochemistry of iron(III) complexes plays an important role in aerosol aging, especially in the lower troposphere. Ensuing radical chemistry leads to decarboxylation, and the production of peroxides, and oxygenated volatile compounds, resulting in particle mass loss due to release of the volatile products to the gas phase. We investigated kinetic transport limitations due to high particle viscosity under low relative humidity conditions. For quantification a numerical model was developed.
Arseniy Karagodin-Doyennel, Eugene Rozanov, Ales Kuchar, William Ball, Pavle Arsenovic, Ellis Remsberg, Patrick Jöckel, Markus Kunze, David A. Plummer, Andrea Stenke, Daniel Marsh, Doug Kinnison, and Thomas Peter
Atmos. Chem. Phys., 21, 201–216, https://doi.org/10.5194/acp-21-201-2021, https://doi.org/10.5194/acp-21-201-2021, 2021
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The solar signal in the mesospheric H2O and CO was extracted from the CCMI-1 model simulations and satellite observations using multiple linear regression (MLR) analysis. MLR analysis shows a pronounced and statistically robust solar signal in both H2O and CO. The model results show a general agreement with observations reproducing a negative/positive solar signal in H2O/CO. The pattern of the solar signal varies among the considered models, reflecting some differences in the model setup.
Jane P. Mulcahy, Colin Johnson, Colin G. Jones, Adam C. Povey, Catherine E. Scott, Alistair Sellar, Steven T. Turnock, Matthew T. Woodhouse, Nathan Luke Abraham, Martin B. Andrews, Nicolas Bellouin, Jo Browse, Ken S. Carslaw, Mohit Dalvi, Gerd A. Folberth, Matthew Glover, Daniel P. Grosvenor, Catherine Hardacre, Richard Hill, Ben Johnson, Andy Jones, Zak Kipling, Graham Mann, James Mollard, Fiona M. O'Connor, Julien Palmiéri, Carly Reddington, Steven T. Rumbold, Mark Richardson, Nick A. J. Schutgens, Philip Stier, Marc Stringer, Yongming Tang, Jeremy Walton, Stephanie Woodward, and Andrew Yool
Geosci. Model Dev., 13, 6383–6423, https://doi.org/10.5194/gmd-13-6383-2020, https://doi.org/10.5194/gmd-13-6383-2020, 2020
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Aerosols are an important component of the Earth system. Here, we comprehensively document and evaluate the aerosol schemes as implemented in the physical and Earth system models, HadGEM3-GC3.1 and UKESM1. This study provides a useful characterisation of the aerosol climatology in both models, facilitating the understanding of the numerous aerosol–climate interaction studies that will be conducted for CMIP6 and beyond.
Sreeharsha Hanumanthu, Bärbel Vogel, Rolf Müller, Simone Brunamonti, Suvarna Fadnavis, Dan Li, Peter Ölsner, Manish Naja, Bhupendra Bahadur Singh, Kunchala Ravi Kumar, Sunil Sonbawne, Hannu Jauhiainen, Holger Vömel, Beiping Luo, Teresa Jorge, Frank G. Wienhold, Ruud Dirkson, and Thomas Peter
Atmos. Chem. Phys., 20, 14273–14302, https://doi.org/10.5194/acp-20-14273-2020, https://doi.org/10.5194/acp-20-14273-2020, 2020
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During boreal summer, anthropogenic sources yield the Asian Tropopause Aerosol Layer (ATAL), found in Asia between about 13 and 18 km altitude. Balloon-borne measurements of the ATAL conducted in northern India in 2016 show the strong variability of the ATAL. To explain its observed variability, model simulations are performed to deduce the origin of air masses on the Earth's surface, which is important to develop recommendations for regulations of anthropogenic surface emissions of the ATAL.
Juan-Carlos Antuña-Marrero, Graham W. Mann, Philippe Keckhut, Sergey Avdyushin, Bruno Nardi, and Larry W. Thomason
Earth Syst. Sci. Data, 12, 2843–2851, https://doi.org/10.5194/essd-12-2843-2020, https://doi.org/10.5194/essd-12-2843-2020, 2020
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We report the recovery of lidar measurements of the 1991 Pinatubo eruption. Two Soviet ships crossing the tropical Atlantic in July–September 1991 and January–February 1992 measured the vertical profile of the Pinatubo cloud at different points in its spatio-temporal evolution. The datasets provide valuable new information on the eruption's impacts on climate, with the SAGE-II satellite measurements not able to measure most of the lower half of the Pinatubo cloud in the tropics in this period.
Sandip S. Dhomse, Graham W. Mann, Juan Carlos Antuña Marrero, Sarah E. Shallcross, Martyn P. Chipperfield, Kenneth S. Carslaw, Lauren Marshall, N. Luke Abraham, and Colin E. Johnson
Atmos. Chem. Phys., 20, 13627–13654, https://doi.org/10.5194/acp-20-13627-2020, https://doi.org/10.5194/acp-20-13627-2020, 2020
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We confirm downward adjustment of SO2 emission to simulate the Pinatubo aerosol cloud with aerosol microphysics models. Similar adjustment is also needed to simulate the El Chichón and Agung volcanic cloud, indicating potential missing removal or vertical redistribution process in models. Important inhomogeneities in the CMIP6 forcing datasets after Agung and El Chichón eruptions are difficult to reconcile. Quasi-biennial oscillation plays an important role in modifying stratospheric warming.
Cited articles
Ammann, C. M., Meehl, G. A., Washington, W. M., and Zender, C. S.: A monthly and latitudinally varying volcanic forcing dataset in simulations of 20th century climate, Geophys. Res. Lett., 30, 1657, https://doi.org/10.1029/2003GL016875, 2003. a
Andersson, S. M., Martinsson, B. G., Vernier, J.-P., Friberg, J., Brenninkmeijer, C. A. M., Hermann, M., van Velthoven, P. F. J., and Zahn, A.: Significant radiative impact of volcanic aerosol in the lowermost stratosphere, Nat. Commun., 6, 7692, https://doi.org/10.1038/ncomms8692, 2015. a
Arfeuille, F., Luo, B. P., Heckendorn, P., Weisenstein, D., Sheng, J. X., Rozanov, E., Schraner, M., Brönnimann, S., Thomason, L. W., and Peter, T.: Modeling the stratospheric warming following the Mt. Pinatubo eruption: uncertainties in aerosol extinctions, Atmos. Chem. Phys., 13, 11221–11234, https://doi.org/10.5194/acp-13-11221-2013, 2013. a, b, c, d, e
Arfeuille, F., Weisenstein, D., Mack, H., Rozanov, E., Peter, T., and Brönnimann, S.: Volcanic forcing for climate modeling: a new microphysics-based data set covering years 1600–present, Clim. Past, 10, 359–375, https://doi.org/10.5194/cp-10-359-2014, 2014. a
Biermann, U. M., Luo, B. P., and Peter, T.: Absorption Spectra and Optical Constants of Binary and Ternary Solutions of H2SO4, HNO3, and H2O in the Mid Infrared at Atmospheric Temperatures, J. Phys. Chem. A, 104, 783–793, https://doi.org/10.1021/jp992349i, 2000. a, b, c
Bingen, C., Vanhellemont, F., and Fussen, D.: A new regularized inversion method for the retrieval of stratospheric aerosol size distributions applied to 16 years of SAGE II data (1984–2000): method, results and validation, Ann. Geophys., 21, 797–804, https://doi.org/10.5194/angeo-21-797-2003, 2003. a
Bohren, C. F. and Huffman, D. R.: Absorption and Scattering of Light by Small Particles, Wiley, https://doi.org/10.1002/9783527618156, 1998. a, b, c
Brodowsky, C. V., Sukhodolov, T., Chiodo, G., Aquila, V., Bekki, S., Dhomse, S. S., Höpfner, M., Laakso, A., Mann, G. W., Niemeier, U., Pitari, G., Quaglia, I., Rozanov, E., Schmidt, A., Sekiya, T., Tilmes, S., Timmreck, C., Vattioni, S., Visioni, D., Yu, P., Zhu, Y., and Peter, T.: Analysis of the global atmospheric background sulfur budget in a multi-model framework, Atmos. Chem. Phys., 24, 5513–5548, https://doi.org/10.5194/acp-24-5513-2024, 2024. a
Carn, S.: Multi-Satellite Volcanic Sulfur Dioxide L4 Long-Term Global Database V4, GES DISC [data set], https://doi.org/10.5067/MEASURES/SO2/DATA405, 2022. a
Carn, S. A., Fioletov, V. E., McLinden, C. A., Li, C., and Krotkov, N. A.: A decade of global volcanic SO2 emissions measured from space, Sci. Rep.-UK, 7, 44095, https://doi.org/10.1038/srep44095, 2017. a
Carslaw, K. S., Luo, B., and Peter, T.: An analytic expression for the composition of aqueous HNO3-H2SO4 stratospheric aerosols including gas phase removal of HNO3, Geophys. Res. Lett., 22, 1877–1880, https://doi.org/10.1029/95GL01668, 1995. a
Chagnon, C. W. and Junge, C. E.: The vertical distribution of sub-micron particles in the stratosphere, J. Atmos. Sci., 18, 746–752, 1961. a
Clyne, M., Lamarque, J.-F., Mills, M. J., Khodri, M., Ball, W., Bekki, S., Dhomse, S. S., Lebas, N., Mann, G., Marshall, L., Niemeier, U., Poulain, V., Robock, A., Rozanov, E., Schmidt, A., Stenke, A., Sukhodolov, T., Timmreck, C., Toohey, M., Tummon, F., Zanchettin, D., Zhu, Y., and Toon, O. B.: Model physics and chemistry causing intermodel disagreement within the VolMIP-Tambora Interactive Stratospheric Aerosol ensemble, Atmos. Chem. Phys., 21, 3317–3343, https://doi.org/10.5194/acp-21-3317-2021, 2021. a
Crameri, F.: Scientific colour maps, Zenodo [data set], https://doi.org/10.5281/zenodo.8409685, 2023. a
Crutzen, P. J.: Albedo Enhancement by Stratospheric Sulfur Injections: A Contribution to Resolve a Policy Dilemma?, Climatic Change, 77, 211, https://doi.org/10.1007/s10584-006-9101-y, 2006. a
Damadeo, R. P., Zawodny, J. M., Thomason, L. W., and Iyer, N.: SAGE version 7.0 algorithm: application to SAGE II, Atmos. Meas. Tech., 6, 3539–3561, https://doi.org/10.5194/amt-6-3539-2013, 2013. a
Delene, D. J. and Deshler, T.: Calibration of a Photometric Cloud Condensation Nucleus Counter Designed for Deployment on a Balloon Package, Journal of Atmospheric and Oceanic Technology, 17, 459–467, https://doi.org/10.1175/1520-0426(2000)017<0459:COAPCC>2.0.CO;2, 2000. a
Deshler, T.: A review of global stratospheric aerosol: Measurements, importance, life cycle, and local stratospheric aerosol, Atmospheric Research, 90, 223–232, https://doi.org/10.1016/j.atmosres.2008.03.016, 2008. a
Deshler, T., Hofmann, D. J., Johnson, B. J., and Rozier, W. R.: Balloonborne measurements of the Pinatubo aerosol size distribution and volatility at Laramie, Wyoming during the summer of 1991, Geophys. Res. Lett., 19, 199–202, https://doi.org/10.1029/91GL02787, 1992. a, b
Deshler, T., Luo, B., Kovilakam, M., Peter, T., and Kalnajs, L. E.: Retrieval of Aerosol Size Distributions From In Situ Particle Counter Measurements: Instrument Counting Efficiency and Comparisons With Satellite Measurements, J. Geophys. Res.-Atmos., 124, 5058–5087, https://doi.org/10.1029/2018JD029558, 2019. a
Eyring, V., Shepherd, T. G., and Waugh, D. W.: SPARC CCMVal Report on the Evaluation of Chemistry-Climate Models, http://www.sparc-climate.org/publications/sparc-reports/ (last access: 4 September 2025), 2010. a
Eyring, V., Lamarque, J.-F., Hess, P., Arfeuille, F., Bowman, K., Chipperfield, M., Duncan, B., Fiore, A. M., Gettelman, A., Giorgetta, M., Granier, C., Hegglin, M., Kinnison, D., Kunze, M., Langematz, U., Luo, B., Martin, R., Matthes, K., Newman, P., and Young, P. J.: Overview of IGAC/SPARC Chemistry-Climate Model Initiative (CCMI) community simulations in support of upcoming ozone and climate assessments, https://www.aparc-climate.org/wp-content/uploads/2017/12/SPARCnewsletter_No40_Jan2013_web.pdf, (last access: 25 July 2024), 2013. a, b
Eyring, V., Bony, S., Meehl, G. A., Senior, C. A., Stevens, B., Stouffer, R. J., and Taylor, K. E.: Overview of the Coupled Model Intercomparison Project Phase 6 (CMIP6) experimental design and organization, Geosci. Model Dev., 9, 1937–1958, https://doi.org/10.5194/gmd-9-1937-2016, 2016. a, b
Fahey, D. W., Kawa, S. R., Woodbridge, E. L., Tin, P., Wilson, J. C., Jonsson, H. H., Dye, J. E., Baumgardner, D., Borrmann, S., Toohey, D. W., Avallone, L. M., Proffitt, M. H., Margitan, J., Loewenstein, M., Podolske, J. R., Salawitch, R. J., Wofsy, S. C., Ko, M. K. W., Anderson, D. E., Schoeber, M. R., and Chan, K. R.: In situ measurements constraining the role of sulphate aerosols in mid-latitude ozone depletion, Nature, 363, 509–514, https://doi.org/10.1038/363509a0, 1993. a
Gettelman, A., Hegglin, M. I., Son, S.-W., Kim, J., Fujiwara, M., Birner, T., Kremser, S., Rex, M., Añel, J. A., Akiyoshi, H., Austin, J., Bekki, S., Braesike, P., Brühl, C., Butchart, N., Chipperfield, M., Dameris, M., Dhomse, S., Garny, H., Hardiman, S. C., Jöckel, P., Kinnison, D. E., Lamarque, J. F., Mancini, E., Marchand, M., Michou, M., Morgenstern, O., Pawson, S., Pitari, G., Plummer, D., Pyle, J. A., Rozanov, E., Scinocca, J., Shepherd, T. G., Shibata, K., Smale, D., Teyssèdre, H., and Tian, W.: Multimodel assessment of the upper troposphere and lower stratosphere: Tropics and global trends, J. Geophys. Res., 115, D00M08, https://doi.org/10.1029/2009JD013638, 2010. a
Hanson, D. R., Ravishankara, A. R., and Solomon, S.: Heterogeneous reactions in sulfuric acid aerosols: A framework for model calculations, J. Geophys. Res.-Atmos., 99, 3615–3629, https://doi.org/10.1029/93JD02932, 1994. a, b, c, d
Heckendorn, P., Weisenstein, D., Fueglistaler, S., Luo, B. P., Rozanov, E., Schraner, M., Thomason, L. W., and Peter, T.: The impact of geoengineering aerosols on stratospheric temperature and ozone, Environ. Res. Lett., 4, 045108, https://doi.org/10.1088/1748-9326/4/4/045108, 2009. a
Hegglin, M. I., Lamarque, J.-F., Eyring, V., Hess, P., Young, P. J., Fiore, A. M., Myhre, G., Nagashima, T., Ryerson, T., Shepherd, T. G., and Waugh, D. W.: IGAC/SPARC Chemistry-Climate Model Initiative (CCMI) 2014 Science Workshop, SPARC Newsletter, 43, 32–35, 2014. a
Hervig, M. E., Russell, J. M., Gordley, L. L., Daniels, J., Drayson, S. R., and Park, J. H.: Aerosol effects and corrections in the Halogen Occultation Experiment, J. Geophys. Res.-Atmos., 100, 1067–1079, https://doi.org/10.1029/94JD02143, 1995. a
Hofmann, D. J. and Solomon, S.: Ozone destruction through heterogeneous chemistry following the eruption of El Chichón, J. Geophys. Res.-Atmos., 94, 5029–5041, https://doi.org/10.1029/JD094iD04p05029, 1989. a
Jonasz, M. and Fournier, G.: Light scattering by particles in water: theoretical and experimental foundations, Academic Press, San Diego, https://doi.org/10.1016/B978-0-12-388751-1.X5000-5, 2007. a
Jörimann, A.: REMAP-CCMI-2022-sai: Stratospheric aerosol data for use in the CCMI-2022 stratospheric aerosol injection scenario, ETH Research Collection [data set], https://doi.org/10.3929/ethz-b-000714654, previously distributed through ftp://iacftp.ethz.ch/pub_read/andrinj/CCMI-2022-sai (last access: 8 June 2025), 2023. a, b, c
Jörimann, A.: REMAP-GloSSAC-2023: Stratospheric aerosol data for use in HT-MOC models, ETH Research Collection [data set], https://doi.org/10.3929/ethz-b-000713396, previously distributed through ftp://iacftp.ethz.ch/pub_read/andrinj/HT-MOC (last access: 8 June 2025), 2024. a, b, c
Jörimann, A.: A REtrieval Method for optical and physical Aerosol Properties in the stratosphere (REMAPv1), ETH Research Collection [code], https://doi.org/10.3929/ethz-b-000715168, 2025. a
Junge, C. E., Chagnon, C. W., and Manson, J. E.: STRATOSPHERIC AEROSOLS, J. Atmos. Sci., 18, 81–108, https://doi.org/10.1175/1520-0469(1961)018<0081:SA>2.0.CO;2, 1961. a
Knepp, T. N., Kovilakam, M., Thomason, L., and Miller, S. J.: Characterization of stratospheric particle size distribution uncertainties using SAGE II and SAGE III/ISS extinction spectra, Atmos. Meas. Tech., 17, 2025–2054, https://doi.org/10.5194/amt-17-2025-2024, 2024. a
Kovilakam, M., Thomason, L. W., Ernest, N., Rieger, L., Bourassa, A., and Millán, L.: The Global Space-based Stratospheric Aerosol Climatology (version 2.0): 1979–2018, Earth Syst. Sci. Data, 12, 2607–2634, https://doi.org/10.5194/essd-12-2607-2020, 2020. a, b
Kovilakam, M., Thomason, L., and Knepp, T.: SAGE III/ISS aerosol/cloud categorization and its impact on GloSSAC, Atmos. Meas. Tech., 16, 2709–2731, https://doi.org/10.5194/amt-16-2709-2023, 2023. a, b
Kovilakam, M., Thomason, L., Verkerk, M., Aubry, T., and Knepp, T.: OMPS-LP Aerosol Extinction Coefficients And Their Applicability in GloSSAC, EGUsphere [preprint], https://doi.org/10.5194/egusphere-2024-2409, 2024. a
Kuchar, A., Sukhodolov, T., Chiodo, G., Jörimann, A., Kult-Herdin, J., Rozanov, E., and Rieder, H. H.: Modulation of the northern polar vortex by the Hunga Tonga–Hunga Ha'apai eruption and the associated surface response, Atmos. Chem. Phys., 25, 3623–3634, https://doi.org/10.5194/acp-25-3623-2025, 2025. a
Lambert, A., Grainger, R. G., Rodgers, C. D., Taylor, F. W., Mergenthaler, J. L., Kumer, J. B., and Massie, S. T.: Global evolution of the Mt. Pinatubo volcanic aerosols observed by the infrared limb-sounding instruments CLAES and ISAMS on the Upper Atmosphere Research Satellite, J. Geophys. Res.-Atmos., 102, 1495–1512, https://doi.org/10.1029/96JD00096, 1997. a
Lanzante, J. R. and Free, M.: Comparison of Radiosonde and GCM Vertical Temperature Trend Profiles: Effects of Dataset Choice and Data Homogenization, J. Climate, 21, 5417–5435, https://doi.org/10.1175/2008JCLI2287.1, 2008. a
Leckey, J. P., Damadeo, R., and Hill, C. A.: Stratospheric Aerosol and Gas Experiment (SAGE) from SAGE III on the ISS to a Free Flying SAGE IV Cubesat, Remote Sens.-Basel, 13, 4664, https://doi.org/10.3390/rs13224664, 2021. a
Luo, B.: SAGE-4λv2: Stratospheric aerosol data for use in CCMI models, ETH Research Collection [data set], https://doi.org/10.3929/ethz-b-000714581, previously distributed through ftp://iacftp.ethz.ch/pub_read/luo/ccmi (last access: 8 June 2025), 2013. a, b, c
Luo, B.: SAGE-3λv4: Stratospheric aerosol data for use in CMIP6 models, ETH Research Collection [data set], https://doi.org/10.3929/ethz-b-000715155, previously distributed through ftp://iacftp.ethz.ch/pub_read/luo/CMIP6_SAD_radForcing_v4.0.0 (last access: 8 June 2025), 2017. a, b, c
Luo, B.: REMAP-CCMI-2022-ref: Stratospheric aerosol data for use in the CCMI-2022 historical period, ETH Research Collection [data set], https://doi.org/10.3929/ethz-b-000715176, previously distributed through ftp://iacftp.ethz.ch/pub_read/luo/CMIP6_SAD_radForcing_v4.0.0_1850-2018 (last access: 8 June 2025), 2020. a, b, c
Luo, B., Carslaw, K. S., Peter, T., and Clegg, S. L.: vapour pressures of H2SO4/HNO3/HCl/HBr/H2O solutions to low stratospheric temperatures, Geophys. Res. Lett., 22, 247–250, https://doi.org/10.1029/94GL02988, 1995. a
Luo, B., Krieger, U. K., and Peter, T.: Densities and refractive indices of H2SO4/HNO3/H2O solutions to stratospheric temperatures, Geophys. Res. Lett., 23, 3707–3710, https://doi.org/10.1029/96GL03581, 1996. a, b, c
Madhavan, B. L., Kudo, R., Ratnam, M. V., Kloss, C., Berthet, G., and Sellitto, P.: Stratospheric Aerosol Characteristics from the 2017–2019 Volcanic Eruptions Using the SAGE III/ISS Observations, Remote Sens.-Basel, 15, 29, https://doi.org/10.3390/rs15010029, 2022. a
Morgenstern, O., Hegglin, M. I., Rozanov, E., O'Connor, F. M., Abraham, N. L., Akiyoshi, H., Archibald, A. T., Bekki, S., Butchart, N., Chipperfield, M. P., Deushi, M., Dhomse, S. S., Garcia, R. R., Hardiman, S. C., Horowitz, L. W., Jöckel, P., Josse, B., Kinnison, D., Lin, M., Mancini, E., Manyin, M. E., Marchand, M., Marécal, V., Michou, M., Oman, L. D., Pitari, G., Plummer, D. A., Revell, L. E., Saint-Martin, D., Schofield, R., Stenke, A., Stone, K., Sudo, K., Tanaka, T. Y., Tilmes, S., Yamashita, Y., Yoshida, K., and Zeng, G.: Review of the global models used within phase 1 of the Chemistry–Climate Model Initiative (CCMI), Geosci. Model Dev., 10, 639–671, https://doi.org/10.5194/gmd-10-639-2017, 2017. a
Plummer, D., Nagashima, T., Tilmes, S., Archibald, A., Chiodo, G., Fadnavis, S., Garny, H., Josse, B., Kim, J., Lamarque, J.-F., Morgenstern, O., Murray, L., Orbe, C., Tai, A., Chipperfield, M., Funke, B., Juckes, M., Kinnison, D., Kunze, M., Luo, B., Matthes, K., Newman, P. A., Pascoe, C., Peter, T.: CCMI-2022: A new set of Chemistry-Climate Model Initiative (CCMI) community simulations to update the assessment of models and support upcoming ozone assessment activities, SPARC Newsletter, 57, 22–30, https://www.aparc-climate.org/wp-content/uploads/2021/07/SPARCnewsletter_Jul2021_web.pdf#p
age=22 (last access: 8 June 2025), 2021. a, b, c, d
age=22 (last access: 8 June 2025), 2021. a, b, c, d
Pusechel, R. F., Blake, D. F., Snetsinger, K. G., Hansen, A. D. A., Verma, S., and Kato, K.: Black carbon (soot) aerosol in the lower stratosphere and upper troposphere, Geophys. Res. Lett., 19, 1659–1662, https://doi.org/10.1029/92GL01801, 1992. a
Quaglia, I., Timmreck, C., Niemeier, U., Visioni, D., Pitari, G., Brodowsky, C., Brühl, C., Dhomse, S. S., Franke, H., Laakso, A., Mann, G. W., Rozanov, E., and Sukhodolov, T.: Interactive stratospheric aerosol models' response to different amounts and altitudes of SO2 injection during the 1991 Pinatubo eruption, Atmos. Chem. Phys., 23, 921–948, https://doi.org/10.5194/acp-23-921-2023, 2023. a, b
Revell, L. E., Stenke, A., Luo, B., Kremser, S., Rozanov, E., Sukhodolov, T., and Peter, T.: Impacts of Mt Pinatubo volcanic aerosol on the tropical stratosphere in chemistry–climate model simulations using CCMI and CMIP6 stratospheric aerosol data, Atmos. Chem. Phys., 17, 13139–13150, https://doi.org/10.5194/acp-17-13139-2017, 2017. a
Robinson, G. N., Worsnop, D. R., Jayne, J. T., Kolb, C. E., and Davidovits, P.: Heterogeneous uptake of ClONO2 and N2O5 by sulfuric acid solutions, J. Geophys. Res.-Atmos., 102, 3583–3601, 1997. a
Rosen, J. M. and Kjome, N. T.: Backscattersonde: a new instrument for atmospheric aerosol research, Appl. Optics, 30, 1552–1561, 1991. a
Russell, P. B., Livingston, J. M., Dutton, E. G., Pueschel, R. F., Reagan, J. A., DeFoor, T. E., Box, M. A., Allen, D., Pilewskie, P., Herman, B. M., Kinne, S. A., and Hofmann, D. J.: Pinatubo and pre-Pinatubo optical-depth spectra: Mauna Loa measurements, comparisons, inferred particle size distributions, radiative effects, and relationship to lidar data, J. Geophys. Res.-Atmos., 98, 22969–22985, https://doi.org/10.1029/93JD02308, 1993. a
Russell, P. B., Livingston, J. M., Pueschel, R. F., Bauman, J. J., Pollack, J. B., Brooks, S. L., Hamill, P., Thomason, L. W., Stowe, L. L., and Deshler, T.: Global to microscale evolution of the Pinatubo volcanic aerosol derived from diverse measurements and analyses, J. Geophys. Res.-Atmos., 101, 18745–18763, 1996. a
Santer, B. D., Bonfils, C., Painter, J. F., Zelinka, M. D., Mears, C., Solomon, S., Schmidt, G. A., Fyfe, J. C., Cole, J. N. S., Nazarenko, L., Taylor, K. E., and Wentz, F. J.: Volcanic contribution to decadal changes in tropospheric temperature, Nat. Geosci., 7, 185–189, https://doi.org/10.1038/ngeo2098, 2014. a, b, c, d
Sato, M., Hansen, J. E., McCormick, M. P., and Pollack, J. B.: Stratospheric aerosol optical depths, 1850–1990, J. Geophys. Res.-Atmos., 98, 22987–22994, 1993. a
Sheng, J.-X., Weisenstein, D. K., Luo, B.-P., Rozanov, E., Arfeuille, F., and Peter, T.: A perturbed parameter model ensemble to investigate Mt. Pinatubo's 1991 initial sulfur mass emission, Atmos. Chem. Phys., 15, 11501–11512, https://doi.org/10.5194/acp-15-11501-2015, 2015. a
Sofieva, V. F., Rozanov, A., Szelag, M., Burrows, J. P., Retscher, C., Damadeo, R., Degenstein, D., Rieger, L. A., and Bourassa, A.: CREST: a Climate Data Record of Stratospheric Aerosols, Earth Syst. Sci. Data, 16, 5227–5241, https://doi.org/10.5194/essd-16-5227-2024, 2024. a
Solomon, S., Daniel, J. S., Neely, R. R., Vernier, J.-P., Dutton, E. G., and Thomason, L. W.: The Persistently Variable “Background” Stratospheric Aerosol Layer and Global Climate Change, Science, 333, 866–870, https://doi.org/10.1126/science.1206027, 2011. a, b, c
SPARC: SPARC Assessment of Stratospheric Aerosol Properties (ASAP), edited by: Thomason, L. and Peter, T., SPARC Report No. 4, WCRP-124, WMO/TD – No. 1295, 14–16, http://www.aparc-climate.org/publications/sparc-reports/ (last access: 4 September 2025), 2006. a
Stothers, R. B.: Major optical depth perturbations to the stratosphere from volcanic eruptions, J. Geophys. Res.-Atmos., 106, 2993–3003, 2001. a
Taha, G., Loughman, R., Zhu, T., Thomason, L., Kar, J., Rieger, L., and Bourassa, A.: OMPS LP Version 2.0 multi-wavelength aerosol extinction coefficient retrieval algorithm, Atmos. Meas. Tech., 14, 1015–1036, https://doi.org/10.5194/amt-14-1015-2021, 2021. a, b
Thomason, L. W., Burton, S. P., Luo, B.-P., and Peter, T.: SAGE II measurements of stratospheric aerosol properties at non-volcanic levels, Atmos. Chem. Phys., 8, 983–995, https://doi.org/10.5194/acp-8-983-2008, 2008. a, b
Thomason, L. W., Ernest, N., Millán, L., Rieger, L., Bourassa, A., Vernier, J.-P., Manney, G., Luo, B., Arfeuille, F., and Peter, T.: A global space-based stratospheric aerosol climatology: 1979–2016, Earth Syst. Sci. Data, 10, 469–492, https://doi.org/10.5194/essd-10-469-2018, 2018. a
Tilmes, S., Müller, R., and Salawitch, R.: The Sensitivity of Polar Ozone Depletion to Proposed Geoengineering Schemes, Science, 320, 1201–1204, https://doi.org/10.1126/science.1153966, 2008. a, b
Timmreck, C., Mann, G. W., Aquila, V., Hommel, R., Lee, L. A., Schmidt, A., Brühl, C., Carn, S., Chin, M., Dhomse, S. S., Diehl, T., English, J. M., Mills, M. J., Neely, R., Sheng, J., Toohey, M., and Weisenstein, D.: The Interactive Stratospheric Aerosol Model Intercomparison Project (ISA-MIP): motivation and experimental design, Geosci. Model Dev., 11, 2581–2608, https://doi.org/10.5194/gmd-11-2581-2018, 2018. a
Todt, M. A., Asher, E., Hall, E., Cullis, P., Jordan, A., Xiong, K., Hurst, D. F., and Thornberry, T.: Baseline Balloon Stratospheric Aerosol Profiles (B2SAP)—Systematic Measurements of Aerosol Number Density and Size, J. Geophys. Res.-Atmos., 128, e2022JD038041, https://doi.org/10.1029/2022JD038041, 2023. a
Trickl, T., Vogelmann, H., Giehl, H., Jäger, H., and Perfahl, M.: Stratospheric Aerosol: 45 Years of Lidar Measurements at Garmisch-Partenkirchen, in: Proceedings of the 30th International Laser Radar Conference, Springer International Publishing, 885–891, https://doi.org/10.1007/978-3-031-37818-8_113, 2023. a, b, c
Vernier, J.-P., Thomason, L. W., Pommereau, J.-P., Bourassa, A., Pelon, J., Garnier, A., Hauchecorne, A., Blanot, L., Trepte, C., Degenstein, D., and Vargas, F.: Major influence of tropical volcanic eruptions on the stratospheric aerosol layer during the last decade, Geophys. Res. Lett., 38, L12807, https://doi.org/10.1029/2011GL047563, 2011. a, b
Vömel, H., Evan, S., and Tully, M.: Water vapor injection into the stratosphere by Hunga Tonga-Hunga Ha'apai, Science, 377, 1444–1447, https://doi.org/10.1126/science.abq2299, 2022. a
von Savigny, C. and Hoffmann, C. G.: Issues related to the retrieval of stratospheric-aerosol particle size information based on optical measurements, Atmos. Meas. Tech., 13, 1909–1920, https://doi.org/10.5194/amt-13-1909-2020, 2020. a
Weisenstein, D. K., Visioni, D., Franke, H., Niemeier, U., Vattioni, S., Chiodo, G., Peter, T., and Keith, D. W.: An interactive stratospheric aerosol model intercomparison of solar geoengineering by stratospheric injection of SO2 or accumulation-mode sulfuric acid aerosols, Atmos. Chem. Phys., 22, 2955–2973, https://doi.org/10.5194/acp-22-2955-2022, 2022. a
Wrana, F., von Savigny, C., Zalach, J., and Thomason, L. W.: Retrieval of stratospheric aerosol size distribution parameters using satellite solar occultation measurements at three wavelengths, Atmos. Meas. Tech., 14, 2345–2357, https://doi.org/10.5194/amt-14-2345-2021, 2021. a
Wurl, D., Grainger, R. G., McDonald, A. J., and Deshler, T.: Optimal estimation retrieval of aerosol microphysical properties from SAGE II satellite observations in the volcanically unperturbed lower stratosphere, Atmos. Chem. Phys., 10, 4295–4317, https://doi.org/10.5194/acp-10-4295-2010, 2010. a
Yue, G. K.: Wavelength Dependence of Aerosol Extinction Coefficient for Stratospheric Aerosols, J. Clim. Appl. Meteorol., 25, 1775–1779, https://doi.org/10.1175/1520-0450(1986)025<1775:WDOAEC>2.0.CO;2, 1986. a
Yue, G. K., McCormick, M. P., and Chu, W. P.: Retrieval of Composition and Size Distribution of Stratospheric Aerosols with the SAGE II Satellite Experiment, J. Atmos. Ocean. Tech., 3, 371–380, https://doi.org/10.1175/1520-0426(1986)003<0371:ROCASD>2.0.CO;2, 1986. a
Zanchettin, D., Khodri, M., Timmreck, C., Toohey, M., Schmidt, A., Gerber, E. P., Hegerl, G., Robock, A., Pausata, F. S. R., Ball, W. T., Bauer, S. E., Bekki, S., Dhomse, S. S., LeGrande, A. N., Mann, G. W., Marshall, L., Mills, M., Marchand, M., Niemeier, U., Poulain, V., Rozanov, E., Rubino, A., Stenke, A., Tsigaridis, K., and Tummon, F.: The Model Intercomparison Project on the climatic response to Volcanic forcing (VolMIP): experimental design and forcing input data for CMIP6, Geosci. Model Dev., 9, 2701–2719, https://doi.org/10.5194/gmd-9-2701-2016, 2016. a
Zhu, Y., Akiyoshi, H., Aquila, V., Asher, E., Bednarz, E. M., Bekki, S., Brühl, C., Butler, A. H., Case, P., Chabrillat, S., Chiodo, G., Clyne, M., Falletti, L., Colarco, P. R., Fleming, E., Jörimann, A., Kovilakam, M., Koren, G., Kuchar, A., Lebas, N., Liang, Q., Liu, C.-C., Mann, G., Manyin, M., Marchand, M., Morgenstern, O., Newman, P., Oman, L. D., Østerstrøm, F. F., Peng, Y., Plummer, D., Quaglia, I., Randel, W., Rémy, S., Sekiya, T., Steenrod, S., Sukhodolov, T., Tilmes, S., Tsigaridis, K., Ueyama, R., Visioni, D., Wang, X., Watanabe, S., Yamashita, Y., Yu, P., Yu, W., Zhang, J., and Zhuo, Z.: Hunga Tonga-Hunga Ha'apai Volcano Impact Model Observation Comparison (HTHH-MOC) Project: Experiment Protocol and Model Descriptions, EGUsphere [preprint], https://doi.org/10.5194/egusphere-2024-3412, 2024. a, b
Short summary
Aerosol particles in the stratosphere affect our climate. Climate models therefore need an accurate description of their properties and evolution. Satellites measure how strongly aerosol particles extinguish light passing through the stratosphere. We describe a method to use such aerosol extinction data to retrieve the number and sizes of the aerosol particles and calculate their optical effects. The resulting data sets for models are validated against ground-based and balloon observations.
Aerosol particles in the stratosphere affect our climate. Climate models therefore need an...
