Oligomer formation in the troposphere: from experimental knowledge to 3-D  modeling

Lemaire, Vincent; Coll, Isabelle; Couvidat, Florian; Mouchel-Vallon, Camille; Seigneur, Christian; Siour, Guillaume

doi:https://doi.org/10.5194/gmd-9-1361-2016

Articles | Volume 9, issue 4

https://doi.org/10.5194/gmd-9-1361-2016

© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

https://doi.org/10.5194/gmd-9-1361-2016

© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Articles | Volume 9, issue 4

Methods for assessment of models

|

11 Apr 2016

Methods for assessment of models |

| 11 Apr 2016

Oligomer formation in the troposphere: from experimental knowledge to 3-D modeling

Vincent Lemaire, Isabelle Coll, Florian Couvidat, Camille Mouchel-Vallon, Christian Seigneur, and Guillaume Siour

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Final revised paper (published on 11 Apr 2016)
Preprint (discussion started on 28 Oct 2015)

Interactive discussion

Status: closed

AC: Author comment | RC: Referee comment | SC: Short comment | EC: Editor comment

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RC C3054: 'Review of paper gmdd-8-9229-2015 by Lemaire et al.', Anonymous Referee #1, 23 Nov 2015
RC C3132: 'Review', Anonymous Referee #2, 01 Dec 2015
RC C3346: 'Referee Comment', Anonymous Referee #3, 15 Dec 2015
AC C4087: 'Author comments', Vincent Lemaire, 01 Mar 2016

Peer-review completion

AR: Author's response | RR: Referee report | ED: Editor decision

AR by Vincent Lemaire on behalf of the Authors (01 Mar 2016) Author's response Manuscript

ED: Publish subject to technical corrections (16 Mar 2016) by Holger Tost

AR by Vincent Lemaire on behalf of the Authors (24 Mar 2016) Manuscript

Short summary

Oligomerization is one of the most important identified processes of secondary organic aerosol evolution. We have simulated the formation of oligomers from biogenic precursors, using two different parameterizations implemented in the air quality model CHIMERE. This study shows that oligomer concentration fields are quite sensitive to the way the competition between local formation, evaporation and transport is restituted. The benefits and disadvantages of each approach are discussed in details.