Articles | Volume 9, issue 1
https://doi.org/10.5194/gmd-9-111-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/gmd-9-111-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Model description paper
| 
19 Jan 2016
Model description paper |
| 19 Jan 2016
Prediction of cloud condensation nuclei activity for organic compounds using functional group contribution methods
Department of Marine, Earth, and Atmospheric Sciences, North Carolina State University, Raleigh, NC, USA
S. M. Kreidenweis
Department of Atmospheric Sciences, Colorado State University, Fort Collins, CO, USA
P. J. Ziemann
Department of Chemistry and Biochemistry, Colorado University, Boulder, CO, USA
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- Recent advances in understanding secondary organic aerosol: Implications for global climate forcing M. Shrivastava et al. 10.1002/2016RG000540
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- The effect of hydrophobic glassy organic material on the cloud condensation nuclei activity of particles with different morphologies A. Tandon et al. 10.5194/acp-19-3325-2019
- Relative-humidity-dependent organic aerosol thermodynamics via an efficient reduced-complexity model K. Gorkowski et al. 10.5194/acp-19-13383-2019
- Meteorological and aerosol effects on marine cloud microphysical properties K. Sanchez et al. 10.1002/2015JD024595
31 citations as recorded by crossref.
- Aerosol mixing state, new particle formation, and cloud droplet number concentration in an urban environment S. Kasparoglu et al. 10.1016/j.scitotenv.2024.175307
- Hygroscopicity of Organic Compounds as a Function of Carbon Chain Length and Carboxyl, Hydroperoxy, and Carbonyl Functional Groups S. Petters et al. 10.1021/acs.jpca.7b04114
- Cloud droplet activation of secondary organic aerosol is mainly controlled by molecular weight, not water solubility J. Wang et al. 10.5194/acp-19-941-2019
- Evidence of a reduction in cloud condensation nuclei activity of water-soluble aerosols caused by biogenic emissions in a cool-temperate forest A. Müller et al. 10.1038/s41598-017-08112-9
- Characteristics of PM2.5 hygroscopicity and the influences of water-soluble ions during haze events in Beijing S. Ge et al. 10.1016/j.atmosenv.2024.120382
- Laboratory evaluation of species-dependent relative ionization efficiencies in the Aerodyne Aerosol Mass Spectrometer W. Xu et al. 10.1080/02786826.2018.1439570
- A Review on Laboratory Studies and Field Measurements of Atmospheric Organic Aerosol Hygroscopicity and Its Parameterization Based on Oxidation Levels Y. Kuang et al. 10.1007/s40726-020-00164-2
- Recent advances in understanding secondary organic aerosol: Implications for global climate forcing M. Shrivastava et al. 10.1002/2016RG000540
- Temperature‐ and Humidity‐Dependent Phase States of Secondary Organic Aerosols S. Petters et al. 10.1029/2018GL080563
- 100 Years of Progress in Cloud Physics, Aerosols, and Aerosol Chemistry Research S. Kreidenweis et al. 10.1175/AMSMONOGRAPHS-D-18-0024.1
- A Significant Portion of Water-Soluble Organic Matter in Fresh Biomass Burning Particles Does Not Contribute to Hygroscopic Growth: An Application of Polarity Segregation by 1-Octanol–Water Partitioning Method J. Chen et al. 10.1021/acs.est.9b01696
- Why would apparent κ linearly change with O/C? Assessing the role of volatility, solubility, and surface activity of organic aerosols S. Nakao 10.1080/02786826.2017.1352082
- Technical note: The role of evolving surface tension in the formation of cloud droplets J. Davies et al. 10.5194/acp-19-2933-2019
- Modeling of hygroscopicity parameter kappa of organic aerosols using quantitative structure-property relationships J. Markelj et al. 10.1007/s10874-016-9347-3
- Aerosol Properties Observed in the Subtropical North Pacific Boundary Layer T. Royalty et al. 10.1002/2017JD026897
- Water Activity from Equilibrium Molecular Dynamics Simulations and Kirkwood-Buff Theory M. Lbadaoui-Darvas & S. Takahama 10.1021/acs.jpcb.9b06735
- Uncertainty in Predicting CCN Activity of Aged and Primary Aerosols F. Zhang et al. 10.1002/2017JD027058
- Impact of fatty acid coating on the CCN activity of sea salt particles Q. Nguyen et al. 10.1080/16000889.2017.1304064
- Optical properties and cloud condensation nuclei activity of brown carbon containing α–dicarbonyls and reduced nitrogen compounds J. Zhou et al. 10.1016/j.atmosres.2023.106935
- Predicting the influence of particle size on the glass transition temperature and viscosity of secondary organic material M. Petters & S. Kasparoglu 10.1038/s41598-020-71490-0
- Establishing the impact of model surfactants on cloud condensation nuclei activity of sea spray aerosol mimics S. Forestieri et al. 10.5194/acp-18-10985-2018
- Cloud droplet activation of black carbon particles coated with organic compounds of varying solubility M. Dalirian et al. 10.5194/acp-18-12477-2018
- Secondary aerosol formation promotes water uptake by organic-rich wildfire haze particles in equatorial Asia J. Chen et al. 10.5194/acp-18-7781-2018
- Water uptake by fresh Indonesian peat burning particles is limited by water-soluble organic matter J. Chen et al. 10.5194/acp-17-11591-2017
- Chemical Characterization of Cloudwater Collected at Puy de Dôme by FT-ICR MS Reveals the Presence of SOA Components A. Bianco et al. 10.1021/acsearthspacechem.9b00153
- Comment on “The effects of molecular weight and thermal decomposition on the sensitivity of a thermal desorption aerosol mass spectrometer” J. Jimenez et al. 10.1080/02786826.2016.1205728
- Water Solubility Distribution of Organic Matter Accounts for the Discrepancy in Hygroscopicity among Sub- and Supersaturated Humidity Regimes W. Lee et al. 10.1021/acs.est.2c04647
- Influence of organic compound functionality on aerosol hygroscopicity: dicarboxylic acids, alkyl-substituents, sugars and amino acids A. Marsh et al. 10.5194/acp-17-5583-2017
- Characterization of the temperature and humidity-dependent phase diagram of amorphous nanoscale organic aerosols N. Rothfuss & M. Petters 10.1039/C6CP08593H
- The effect of hydrophobic glassy organic material on the cloud condensation nuclei activity of particles with different morphologies A. Tandon et al. 10.5194/acp-19-3325-2019
- Relative-humidity-dependent organic aerosol thermodynamics via an efficient reduced-complexity model K. Gorkowski et al. 10.5194/acp-19-13383-2019
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Saved (preprint)
Latest update: 23 Nov 2024
Short summary
Organic particles suspended in air serve as nucleation seeds for droplets in atmospheric clouds. Over time their chemical composition changes towards more functionalized compounds. This work presents a model that can predict an organic compounds' ability promote the nucleation of cloud drops from its functional group composition. Hydroxyl, carboxyl, aldehyde, hydroperoxide, carbonyl, and ether moieties promote droplet nucleation. Methylene and nitrate moieties inhibit droplet nucleation.
Organic particles suspended in air serve as nucleation seeds for droplets in atmospheric clouds....
