Articles | Volume 18, issue 7
https://doi.org/10.5194/gmd-18-2231-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/gmd-18-2231-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Sensitivity studies of a four-dimensional local ensemble transform Kalman filter coupled with WRF-Chem version 3.9.1 for improving particulate matter simulation accuracy
Jianyu Lin
College of Oceanic and Atmospheric Sciences, Ocean University of China, Qingdao, 266100, China
State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, China
State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, China
Lifang Sheng
College of Oceanic and Atmospheric Sciences, Ocean University of China, Qingdao, 266100, China
Weihang Zhang
College of Oceanic and Atmospheric Sciences, Ocean University of China, Qingdao, 266100, China
Shangfei Hai
CMA Earth System Modeling and Prediction Centre, China Meteorological Administration (CMA), Beijing 100081, China
Yawen Kong
State Key Laboratory of Remote Sensing Science, Aerospace Information Research Institute, Chinese Academy of Sciences, Beijing 100101, China
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Yawen Kong, Bo Zheng, and Yuxi Liu
Atmos. Chem. Phys., 25, 5959–5976, https://doi.org/10.5194/acp-25-5959-2025, https://doi.org/10.5194/acp-25-5959-2025, 2025
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Current high-resolution satellite remote sensing technologies provide a unique opportunity to derive timely high-resolution emission data. We developed an emission inversion system to assimilate satellite NO2 data to obtain daily kilometer-scale NOx emission inventories. Our results enhance inventory accuracy, allowing us to capture the effects of pollution control policies on daily emissions (e.g., during COVID-19 lockdowns) and improve fine-scale air quality modeling.
Xiadong An, Wen Chen, Tianjiao Ma, and Lifang Sheng
EGUsphere, https://doi.org/10.5194/egusphere-2025-285, https://doi.org/10.5194/egusphere-2025-285, 2025
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Air pollution in the North China Plain is tends to be influenced by El Niño-Southern Oscillation (ENSO) and stratospheric Quasi-Biennial Oscillation (QBO). During El Niño and easterly QBO, pollution rises, while La Niña and easterly QBO improve air quality through changes in atmospheric circulation and weather conditions.
Yueming Cheng, Tie Dai, Junji Cao, Daisuke Goto, Jianbing Jin, Teruyuki Nakajima, and Guangyu Shi
Atmos. Chem. Phys., 24, 12643–12659, https://doi.org/10.5194/acp-24-12643-2024, https://doi.org/10.5194/acp-24-12643-2024, 2024
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In March 2021, east Asia experienced an outbreak of severe dust storms after an absence of 1.5 decades. Here, we innovatively used the time-lagged ground-based aerosol size information with the fixed-lag ensemble Kalman smoother to optimize dust emission and reproduce the dust storm. This work is valuable for not only the quantification of health damage, aviation risks, and profound impacts on the Earth's system but also revealing the climatic driving force and the process of desertification.
Wenshuai Li, Yuxuan Qi, Yingchen Liu, Guanru Wu, Yanjing Zhang, Jinhui Shi, Wenjun Qu, Lifang Sheng, Wencai Wang, Daizhou Zhang, and Yang Zhou
Atmos. Chem. Phys., 24, 6495–6508, https://doi.org/10.5194/acp-24-6495-2024, https://doi.org/10.5194/acp-24-6495-2024, 2024
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Aerosol particles from mainland can transport to oceans and deposit, providing soluble Fe and affecting phytoplankton growth. Thus, we studied the dissolution process of aerosol Fe and found that photochemistry played a key role in promoting Fe dissolution in clean conditions. RH-dependent reactions were more influential in slightly polluted conditions. These results highlight the distinct roles of two weather-related parameters (radiation and RH) in influencing geochemical cycles related to Fe.
Feifan Yan, Hang Su, Yafang Cheng, Rujin Huang, Hong Liao, Ting Yang, Yuanyuan Zhu, Shaoqing Zhang, Lifang Sheng, Wenbin Kou, Xinran Zeng, Shengnan Xiang, Xiaohong Yao, Huiwang Gao, and Yang Gao
Atmos. Chem. Phys., 24, 2365–2376, https://doi.org/10.5194/acp-24-2365-2024, https://doi.org/10.5194/acp-24-2365-2024, 2024
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PM2.5 pollution is a major air quality issue deteriorating human health, and previous studies mostly focus on regions like the North China Plain and Yangtze River Delta. However, the characteristics of PM2.5 concentrations between these two regions are studied less often. Focusing on the transport corridor region, we identify an interesting seesaw transport phenomenon with stagnant weather conditions, conducive to PM2.5 accumulation over this region, resulting in large health effects.
Min Zhao, Tie Dai, Daisuke Goto, Hao Wang, and Guangyu Shi
Atmos. Chem. Phys., 24, 235–258, https://doi.org/10.5194/acp-24-235-2024, https://doi.org/10.5194/acp-24-235-2024, 2024
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During a springtime pollution input from South Asia to the Tibetan Plateau, we combined atmospheric chemistry modeling and data assimilation methods to assimilate and forecast aerosols from South Asia and the Tibetan Plateau. Assimilation of observations over a whole time window leads to a more reasonable distribution of daily variations in the aerosol forecast field. We also find that aerosol assimilation can improve the surface solar energy forecast in the Tibetan Plateau region.
Chupeng Zhang, Shangfei Hai, Yang Gao, Yuhang Wang, Shaoqing Zhang, Lifang Sheng, Bin Zhao, Shuxiao Wang, Jingkun Jiang, Xin Huang, Xiaojing Shen, Junying Sun, Aura Lupascu, Manish Shrivastava, Jerome D. Fast, Wenxuan Cheng, Xiuwen Guo, Ming Chu, Nan Ma, Juan Hong, Qiaoqiao Wang, Xiaohong Yao, and Huiwang Gao
Atmos. Chem. Phys., 23, 10713–10730, https://doi.org/10.5194/acp-23-10713-2023, https://doi.org/10.5194/acp-23-10713-2023, 2023
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New particle formation is an important source of atmospheric particles, exerting critical influences on global climate. Numerical models are vital tools to understanding atmospheric particle evolution, which, however, suffer from large biases in simulating particle numbers. Here we improve the model chemical processes governing particle sizes and compositions. The improved model reveals substantial contributions of newly formed particles to climate through effects on cloud condensation nuclei.
Qian Liu, Guixing Chen, Lifang Sheng, and Toshiki Iwasaki
Atmos. Chem. Phys., 22, 13371–13388, https://doi.org/10.5194/acp-22-13371-2022, https://doi.org/10.5194/acp-22-13371-2022, 2022
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Air pollution can be cleaned up quickly by a cold air outbreak (CAO) but reappears after a CAO. By quantifying the CAO properties, we find the coldness and depth of the cold air mass are key factors affecting the rapid (slow) reappearance of air pollution through modulating the atmospheric boundary layer height and stability. We also find that the spatial pattern of CAO in high-latitude Eurasia a few days ahead can be recognized as a precursor for the reappearance of air pollution.
Yawen Kong, Bo Zheng, Qiang Zhang, and Kebin He
Atmos. Chem. Phys., 22, 10769–10788, https://doi.org/10.5194/acp-22-10769-2022, https://doi.org/10.5194/acp-22-10769-2022, 2022
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We developed a Bayesian atmospheric inversion system based on the 4D local ensemble transform Kalman filter (4D-LETKF) algorithm coupled with GEOS-Chem from the latest Orbiting Carbon Observatory-2 (OCO-2) V10r XCO2 retrievals. This is the first adaptation of 4D-LETKF to an OCO-2-based global carbon inversion system. We inferred global gridded carbon fluxes and investigated their magnitudes, variations, and partitioning schemes to understand the global and regional carbon budgets for 2015–2020.
Xiadong An, Wen Chen, Peng Hu, Shangfeng Chen, and Lifang Sheng
Atmos. Chem. Phys., 22, 6507–6521, https://doi.org/10.5194/acp-22-6507-2022, https://doi.org/10.5194/acp-22-6507-2022, 2022
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The intraseasonal NAAA usually establishes quickly on day −3 with a life span of 8 days. Further results revealed that the probability of regional PM2.5 pollution related to the NAAA for at least 2 days in the NCP is 80% in NDJ period 2000–2021. Particularly, air quality in the NCP tends to deteriorate on day 2 prior to the peak day of the NAAA and reaches a peak on day −1 with a life cycle of 4 days. The corresponding meteorological conditions support these conclusions.
Xiadong An, Lifang Sheng, Chun Li, Wen Chen, Yulian Tang, and Jingliang Huangfu
Atmos. Chem. Phys., 22, 725–738, https://doi.org/10.5194/acp-22-725-2022, https://doi.org/10.5194/acp-22-725-2022, 2022
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The North China Plain (NCP) suffered many periods of haze in winter during 1985–2015, related to the rainfall-induced diabatic heating over southern China. The haze over the NCP is modulated by an anomalous anticyclone caused by the Rossby wave and a north–south circulation (NSC) induced mainly by diabatic heating. As a Rossby wave source, rainfall-induced diabatic heating supports waves and finally strengthens the anticyclone over the NCP. These changes favor haze over the NCP.
Zhenbin Wang, Bin Zhu, Hanqing Kang, Wen Lu, Shuqi Yan, Delong Zhao, Weihang Zhang, and Jinhui Gao
Atmos. Chem. Phys., 21, 15555–15567, https://doi.org/10.5194/acp-21-15555-2021, https://doi.org/10.5194/acp-21-15555-2021, 2021
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In this paper, by using WRF-Chem with a black carbon (BC) tagging technique, we investigate the formation mechanism and regional sources of a BC peak in the free troposphere observed by aircraft flights. Local sources dominated BC from the surface to about 700 m (78.5 %), while the BC peak in the free troposphere was almost entirely imported from external sources (99.8 %). Our results indicate that cyclone systems can quickly lift BC up to the free troposphere, as well as extend its lifetime.
Tie Dai, Yueming Cheng, Daisuke Goto, Yingruo Li, Xiao Tang, Guangyu Shi, and Teruyuki Nakajima
Atmos. Chem. Phys., 21, 4357–4379, https://doi.org/10.5194/acp-21-4357-2021, https://doi.org/10.5194/acp-21-4357-2021, 2021
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The anthropogenic emission of sulfur dioxide (SO2) over China has significantly declined as a consequence of the clean air actions. We have developed a new emission inversion system to dynamically update the SO2 emission grid by grid over China by assimilating ground-based SO2 observations. The inverted SO2 emission over China in November 2016 on average had declined by 49.4 % since 2010, which is well in agreement with the bottom-up estimation of 48.0 %.
Yueming Cheng, Tie Dai, Jiming Li, and Guangyu Shi
Atmos. Chem. Phys., 20, 15307–15322, https://doi.org/10.5194/acp-20-15307-2020, https://doi.org/10.5194/acp-20-15307-2020, 2020
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In this paper we present the analysis of the aerosol vertical features observed by CATS collected from 2015 to 2017 over three selected regions (North China, the Tibetan Plateau, and the Tarim Basin) over different timescales. This comprehensive information provides insights into the seasonal variations and diurnal cycles of the aerosol vertical features across East Asia.
Xiadong An, Lifang Sheng, Qian Liu, Chun Li, Yang Gao, and Jianping Li
Atmos. Chem. Phys., 20, 4667–4680, https://doi.org/10.5194/acp-20-4667-2020, https://doi.org/10.5194/acp-20-4667-2020, 2020
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Severe haze occurred in the North China Plain (NCP) in November to December 2015. We found that the two Rossby waveguides within the westerly jet originating from the Mediterranean were responsible for the haze formation in the NCP. The weak East Asia winter monsoon and anomalous circulation with ascending motion over southern China and descending motion over the NCP related to the two Rossby waveguides, which modulated haze accumulation and favored the maintenance of severe haze.
Yueming Cheng, Tie Dai, Daisuke Goto, Nick A. J. Schutgens, Guangyu Shi, and Teruyuki Nakajima
Atmos. Chem. Phys., 19, 13445–13467, https://doi.org/10.5194/acp-19-13445-2019, https://doi.org/10.5194/acp-19-13445-2019, 2019
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Aerosol vertical information is critical to quantify the influences of aerosol on the climate and environment; however, large uncertainties still persist in model simulations. Global aerosol vertical distributions are more accurately simulated by assimilating the vertical aerosol extinction coefficients from the Cloud–Aerosol Lidar with Orthogonal Polarization (CALIOP).
Mingchen Ma, Yang Gao, Yuhang Wang, Shaoqing Zhang, L. Ruby Leung, Cheng Liu, Shuxiao Wang, Bin Zhao, Xing Chang, Hang Su, Tianqi Zhang, Lifang Sheng, Xiaohong Yao, and Huiwang Gao
Atmos. Chem. Phys., 19, 12195–12207, https://doi.org/10.5194/acp-19-12195-2019, https://doi.org/10.5194/acp-19-12195-2019, 2019
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Ozone pollution has become severe in China, and extremely high ozone episodes occurred in summer 2017 over the North China Plain. While meteorology impacts are clear, we find that enhanced biogenic emissions, previously ignored by the community, driven by high vapor pressure deficit, land cover change and urban landscape contribute substantially to ozone formation. This study has significant implications for ozone pollution control with more frequent heat waves and urbanization growth in future.
Zongbo Shi, Tuan Vu, Simone Kotthaus, Roy M. Harrison, Sue Grimmond, Siyao Yue, Tong Zhu, James Lee, Yiqun Han, Matthias Demuzere, Rachel E. Dunmore, Lujie Ren, Di Liu, Yuanlin Wang, Oliver Wild, James Allan, W. Joe Acton, Janet Barlow, Benjamin Barratt, David Beddows, William J. Bloss, Giulia Calzolai, David Carruthers, David C. Carslaw, Queenie Chan, Lia Chatzidiakou, Yang Chen, Leigh Crilley, Hugh Coe, Tie Dai, Ruth Doherty, Fengkui Duan, Pingqing Fu, Baozhu Ge, Maofa Ge, Daobo Guan, Jacqueline F. Hamilton, Kebin He, Mathew Heal, Dwayne Heard, C. Nicholas Hewitt, Michael Hollaway, Min Hu, Dongsheng Ji, Xujiang Jiang, Rod Jones, Markus Kalberer, Frank J. Kelly, Louisa Kramer, Ben Langford, Chun Lin, Alastair C. Lewis, Jie Li, Weijun Li, Huan Liu, Junfeng Liu, Miranda Loh, Keding Lu, Franco Lucarelli, Graham Mann, Gordon McFiggans, Mark R. Miller, Graham Mills, Paul Monk, Eiko Nemitz, Fionna O'Connor, Bin Ouyang, Paul I. Palmer, Carl Percival, Olalekan Popoola, Claire Reeves, Andrew R. Rickard, Longyi Shao, Guangyu Shi, Dominick Spracklen, David Stevenson, Yele Sun, Zhiwei Sun, Shu Tao, Shengrui Tong, Qingqing Wang, Wenhua Wang, Xinming Wang, Xuejun Wang, Zifang Wang, Lianfang Wei, Lisa Whalley, Xuefang Wu, Zhijun Wu, Pinhua Xie, Fumo Yang, Qiang Zhang, Yanli Zhang, Yuanhang Zhang, and Mei Zheng
Atmos. Chem. Phys., 19, 7519–7546, https://doi.org/10.5194/acp-19-7519-2019, https://doi.org/10.5194/acp-19-7519-2019, 2019
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APHH-Beijing is a collaborative international research programme to study the sources, processes and health effects of air pollution in Beijing. This introduction to the special issue provides an overview of (i) the APHH-Beijing programme, (ii) the measurement and modelling activities performed as part of it and (iii) the air quality and meteorological conditions during joint intensive field campaigns as a core activity within APHH-Beijing.
D. Goto, T. Dai, M. Satoh, H. Tomita, J. Uchida, S. Misawa, T. Inoue, H. Tsuruta, K. Ueda, C. F. S. Ng, A. Takami, N. Sugimoto, A. Shimizu, T. Ohara, and T. Nakajima
Geosci. Model Dev., 8, 235–259, https://doi.org/10.5194/gmd-8-235-2015, https://doi.org/10.5194/gmd-8-235-2015, 2015
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An aerosol-coupled global non-hydrostatic model with a stretched-grid system has been developed to simulate aerosols on a region scale of 10 km grids. The regional simulation does require either a nesting technique or lateral boundary conditions, as opposed to general regional models. It generally reproduces monthly mean distributions of the observed sulfate and SO2 over East Asia as well as the diurnal and synoptic variations of the observed ones around the main target region, Tokyo/Japan.
Related subject area
Atmospheric sciences
New submodel for emissions from Explosive Volcanic ERuptions (EVER v1.1) within the Modular Earth Submodel System (MESSy, version 2.55.1)
Quantifying the oscillatory evolution of simulated boundary-layer cloud fields using Gaussian process regression
Numerical investigations on the modelling of ultrafine particles in SSH-aerosol-v1.3a: size resolution and redistribution
The third Met Office Unified Model–JULES Regional Atmosphere and Land Configuration, RAL3
The sensitivity of aerosol data assimilation to vertical profiles: case study of dust storm assimilation with LOTOS-EUROS v2.2
Knowledge-inspired fusion strategies for the inference of PM2.5 values with a neural network
Tuning the ICON-A 2.6.4 climate model with machine-learning-based emulators and history matching
A novel method for quantifying the contribution of regional transport to PM2.5 in Beijing (2013–2020): combining machine learning with concentration-weighted trajectory analysis
Quantification of CO2 hotspot emissions from OCO-3 SAM CO2 satellite images using deep learning methods
Diagnosis of winter precipitation types using the spectral bin model (version 1DSBM-19M): comparison of five methods using ICE-POP 2018 field experiment data
Improving winter condition simulations in SURFEX-TEB v9.0 with a multi-layer snow model and ice
UA-ICON with the NWP physics package (version ua-icon-2.1): mean state and variability of the middle atmosphere
Integrated Methane Inversion (IMI) 2.0: an improved research and stakeholder tool for monitoring total methane emissions with high resolution worldwide using TROPOMI satellite observations
HTAP3 Fires: towards a multi-model, multi-pollutant study of fire impacts
Using a data-driven statistical model to better evaluate surface turbulent heat fluxes in weather and climate numerical models: a demonstration study
Pochva: a new hydro-thermal process model in soil, snow, and vegetation for application in atmosphere numerical models
ClimKern v1.2: a new Python package and kernel repository for calculating radiative feedbacks
Accounting for effects of coagulation and model uncertainties in particle number concentration estimates based on measurements from sampling lines – a Bayesian inversion approach with SLIC v1.0
Top-down CO emission estimates using TROPOMI CO data in the TM5-4DVAR (r1258) inverse modeling suit
The Multi-Compartment Hg Modeling and Analysis Project (MCHgMAP): mercury modeling to support international environmental policy
Similarity-based analysis of atmospheric organic compounds for machine learning applications
Porting the Meso-NH atmospheric model on different GPU architectures for the next generation of supercomputers (version MESONH-v55-OpenACC)
Estimation of aerosol and cloud radiative heating rate in the tropical stratosphere using a radiative kernel method
Evaluation of dust emission and land surface schemes in predicting a mega Asian dust storm over South Korea using WRF-Chem
A Bayesian method for predicting background radiation at environmental monitoring stations in local-scale networks
Inclusion of the ECMWF ecRad radiation scheme (v1.5.0) in the MAR (v3.14), regional evaluation for Belgium, and assessment of surface shortwave spectral fluxes at Uccle
Development of a fast radiative transfer model for ground-based microwave radiometers (ARMS-gb v1.0): validation and comparison to RTTOV-gb
Indian Institute of Tropical Meteorology (IITM) High-Resolution Global Forecast Model version 1: an attempt to resolve monsoon prediction deadlock
Cell-tracking-based framework for assessing nowcasting model skill in reproducing growth and decay of convective rainfall
NeuralMie (v1.0): an aerosol optics emulator
A REtrieval Method for optical and physical Aerosol Properties in the stratosphere (REMAPv1)
Simulation performance of planetary boundary layer schemes in WRF v4.3.1 for near-surface wind over the western Sichuan Basin: a single-site assessment
FootNet v1.0: development of a machine learning emulator of atmospheric transport
Updates and evaluation of NOAA's online-coupled air quality model version 7 (AQMv7) within the Unified Forecast System
Quantifying the analysis uncertainty for nowcasting application
Improving the ensemble square root filter (EnSRF) in the Community Inversion Framework: a case study with ICON-ART 2024.01
The MESSy DWARF (based on MESSy v2.55.2)
Generalized local fractions – a method for the calculation of sensitivities to emissions from multiple sources for chemically active species, illustrated using the EMEP MSC-W model (rv5.5)
SanDyPALM v1.0: Static and Dynamic Drivers for the PALM-4U Model to Facilitate Realistic Urban Microclimate Simulations
An enhanced emission module for the PALM model system 23.10 with application for PM10 emission from urban domestic heating
Identifying lightning processes in ERA5 soundings with deep learning
Sensitivity of predicted ultrafine particle size distributions in Europe to different nucleation rate parameterizations using PMCAMx-UF v2.2
Explaining neural networks for detection of tropical cyclones and atmospheric rivers in gridded atmospheric simulation data
Implementation of a dry deposition module (DEPAC v3.11) in a large eddy simulation code (DALES v4.4)
Accurate and fast prediction of radioactive pollution by Kriging coupled with Auto-Associative Models
Mitigating Hail Overforecasting in the 2-Moment Milbrandt-Yau Microphysics Scheme (v2.25.2_beta_04) in WRF (v4.5.1) by Incorporating the Graupel Spongy Wet Growth Process (MY2_GSWG v1.0)
PALACE v1.0: Paranal Airglow Line And Continuum Emission model
Accurate space-based NOx emission estimates with the flux divergence approach require fine-scale model information on local oxidation chemistry and profile shapes
Exploring a high-level programming model for the NWP domain using ECMWF microphysics schemes
Quantifying uncertainties in satellite NO2 superobservations for data assimilation and model evaluation
Matthias Kohl, Christoph Brühl, Jennifer Schallock, Holger Tost, Patrick Jöckel, Adrian Jost, Steffen Beirle, Michael Höpfner, and Andrea Pozzer
Geosci. Model Dev., 18, 3985–4007, https://doi.org/10.5194/gmd-18-3985-2025, https://doi.org/10.5194/gmd-18-3985-2025, 2025
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SO2 from explosive volcanic eruptions reaching the stratosphere can oxidize and form sulfur aerosols, potentially persisting for several years. We developed a new submodel, Explosive Volcanic ERuptions (EVER), that seamlessly includes stratospheric volcanic SO2 emissions in global numerical simulations based on a novel standard historical model setup, successfully evaluated with satellite observations. Sensitivity studies on the Nabro eruption in 2011 evaluate different emission methods.
Gunho Loren Oh and Philip H. Austin
Geosci. Model Dev., 18, 3921–3940, https://doi.org/10.5194/gmd-18-3921-2025, https://doi.org/10.5194/gmd-18-3921-2025, 2025
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It is difficult to study the behaviour of a cloud field due to internal fluctuations and observational noise. We perform a high-resolution simulation of the boundary-layer cloud field and introduce statistical and numerical techniques, including machine-learning models, to study the evolution of the cloud field, which shows a periodic behaviour. We aim to use the numerical techniques to identify the underlying behaviour within noisy observations.
Oscar Jacquot and Karine Sartelet
Geosci. Model Dev., 18, 3965–3984, https://doi.org/10.5194/gmd-18-3965-2025, https://doi.org/10.5194/gmd-18-3965-2025, 2025
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Modelling the size distribution and the number concentration is important to represent ultrafine particles. A new analytic formulation is presented to compute coagulation partition coefficients, allowing us to lower the numerical diffusion associated with the resolution of aerosol dynamics. The significance of this effect is assessed in a 0D box model and over greater Paris with a chemistry transport model, using different size resolutions of the particle distribution.
Mike Bush, David L. A. Flack, Huw W. Lewis, Sylvia I. Bohnenstengel, Chris J. Short, Charmaine Franklin, Adrian P. Lock, Martin Best, Paul Field, Anne McCabe, Kwinten Van Weverberg, Segolene Berthou, Ian Boutle, Jennifer K. Brooke, Seb Cole, Shaun Cooper, Gareth Dow, John Edwards, Anke Finnenkoetter, Kalli Furtado, Kate Halladay, Kirsty Hanley, Margaret A. Hendry, Adrian Hill, Aravindakshan Jayakumar, Richard W. Jones, Humphrey Lean, Joshua C. K. Lee, Andy Malcolm, Marion Mittermaier, Saji Mohandas, Stuart Moore, Cyril Morcrette, Rachel North, Aurore Porson, Susan Rennie, Nigel Roberts, Belinda Roux, Claudio Sanchez, Chun-Hsu Su, Simon Tucker, Simon Vosper, David Walters, James Warner, Stuart Webster, Mark Weeks, Jonathan Wilkinson, Michael Whitall, Keith D. Williams, and Hugh Zhang
Geosci. Model Dev., 18, 3819–3855, https://doi.org/10.5194/gmd-18-3819-2025, https://doi.org/10.5194/gmd-18-3819-2025, 2025
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RAL configurations define settings for the Unified Model atmosphere and Joint UK Land Environment Simulator. The third version of the Regional Atmosphere and Land (RAL3) science configuration for kilometre- and sub-kilometre-scale modelling represents a major advance compared to previous versions (RAL2) by delivering a common science definition for applications in tropical and mid-latitude regions. RAL3 has more realistic precipitation distributions and an improved representation of clouds and visibility.
Mijie Pang, Jianbing Jin, Ting Yang, Xi Chen, Arjo Segers, Batjargal Buyantogtokh, Yixuan Gu, Jiandong Li, Hai Xiang Lin, Hong Liao, and Wei Han
Geosci. Model Dev., 18, 3781–3798, https://doi.org/10.5194/gmd-18-3781-2025, https://doi.org/10.5194/gmd-18-3781-2025, 2025
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Aerosol data assimilation has gained popularity as it combines the advantages of modelling and observation. However, few studies have addressed the challenges in the prior vertical structure. Different observations are assimilated to examine the sensitivity of assimilation to vertical structure. Results show that assimilation can optimize the dust field in general. However, if the prior introduces an incorrect structure, the assimilation can significantly deteriorate the integrity of the aerosol profile.
Matthieu Dabrowski, José Mennesson, Jérôme Riedi, Chaabane Djeraba, and Pierre Nabat
Geosci. Model Dev., 18, 3707–3733, https://doi.org/10.5194/gmd-18-3707-2025, https://doi.org/10.5194/gmd-18-3707-2025, 2025
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This work focuses on the prediction of aerosol concentration values at the ground level, which are a strong indicator of air quality, using artificial neural networks. A study of different variables and their efficiency as inputs for these models is also proposed and reveals that the best results are obtained when using all of them. Comparison between network architectures and information fusion methods allows for the extraction of knowledge on the most efficient methods in the context of this study.
Pauline Bonnet, Lorenzo Pastori, Mierk Schwabe, Marco Giorgetta, Fernando Iglesias-Suarez, and Veronika Eyring
Geosci. Model Dev., 18, 3681–3706, https://doi.org/10.5194/gmd-18-3681-2025, https://doi.org/10.5194/gmd-18-3681-2025, 2025
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Tuning a climate model means adjusting uncertain parameters in the model to best match observations like the global radiation balance and cloud cover. This is usually done by running many simulations of the model with different settings, which can be time-consuming and relies heavily on expert knowledge. To make this process faster and more objective, we developed a machine learning emulator to create a large ensemble and apply a method called history matching to find the best settings.
Kang Hu, Hong Liao, Dantong Liu, Jianbing Jin, Lei Chen, Siyuan Li, Yangzhou Wu, Changhao Wu, Shitong Zhao, Xiaotong Jiang, Ping Tian, Kai Bi, Ye Wang, and Delong Zhao
Geosci. Model Dev., 18, 3623–3634, https://doi.org/10.5194/gmd-18-3623-2025, https://doi.org/10.5194/gmd-18-3623-2025, 2025
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This study combines machine learning with concentration-weighted trajectory analysis to quantify regional transport PM2.5. From 2013–2020, local emissions dominated Beijing's pollution events. The Air Pollution Prevention and Control Action Plan reduced regional transport pollution, but the eastern region showed the smallest decrease. Beijing should prioritize local emission reduction while considering the east region's contributions in future strategies.
Joffrey Dumont Le Brazidec, Pierre Vanderbecken, Alban Farchi, Grégoire Broquet, Gerrit Kuhlmann, and Marc Bocquet
Geosci. Model Dev., 18, 3607–3622, https://doi.org/10.5194/gmd-18-3607-2025, https://doi.org/10.5194/gmd-18-3607-2025, 2025
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We developed a deep learning method to estimate CO2 emissions from power plants using satellite images. Trained and validated on simulated data, our model accurately predicts emissions despite challenges like cloud cover. When applied to real OCO3 satellite images, the results closely match reported emissions. This study shows that neural networks trained on simulations can effectively analyse real satellite data, offering a new way to monitor CO2 emissions from space.
Wonbae Bang, Jacob T. Carlin, Kwonil Kim, Alexander V. Ryzhkov, Guosheng Liu, and GyuWon Lee
Geosci. Model Dev., 18, 3559–3581, https://doi.org/10.5194/gmd-18-3559-2025, https://doi.org/10.5194/gmd-18-3559-2025, 2025
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Microphysics model-based diagnosis, such as the spectral bin model (SBM), has recently been attempted to diagnose winter precipitation types. In this study, the accuracy of SBM-based precipitation type diagnosis is compared with other traditional methods. SBM has a relatively higher accuracy for dry-snow and wet-snow events, whereas it has lower accuracy for rain events. When the microphysics scheme in the SBM was optimized for the corresponding region, the accuracy for rain events improved.
Gabriel Colas, Valéry Masson, François Bouttier, Ludovic Bouilloud, Laura Pavan, and Virve Karsisto
Geosci. Model Dev., 18, 3453–3472, https://doi.org/10.5194/gmd-18-3453-2025, https://doi.org/10.5194/gmd-18-3453-2025, 2025
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In winter, snow- and ice-covered artificial surfaces are important aspects of the urban climate. They may influence the magnitude of the urban heat island effect, but this is still unclear. In this study, we improved the representation of the snow and ice cover in the Town Energy Balance (TEB) urban climate model. Evaluations have shown that the results are promising for using TEB to study the climate of cold cities.
Markus Kunze, Christoph Zülicke, Tarique A. Siddiqui, Claudia C. Stephan, Yosuke Yamazaki, Claudia Stolle, Sebastian Borchert, and Hauke Schmidt
Geosci. Model Dev., 18, 3359–3385, https://doi.org/10.5194/gmd-18-3359-2025, https://doi.org/10.5194/gmd-18-3359-2025, 2025
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We present the Icosahedral Nonhydrostatic (ICON) general circulation model with an upper-atmospheric extension with the physics package for numerical weather prediction (UA-ICON(NWP)). We optimized the parameters for the gravity wave parameterizations and achieved realistic modeling of the thermal and dynamic states of the mesopause regions. UA-ICON(NWP) now shows a realistic frequency of major sudden stratospheric warmings and well-represented solar tides in temperature.
Lucas A. Estrada, Daniel J. Varon, Melissa Sulprizio, Hannah Nesser, Zichong Chen, Nicholas Balasus, Sarah E. Hancock, Megan He, James D. East, Todd A. Mooring, Alexander Oort Alonso, Joannes D. Maasakkers, Ilse Aben, Sabour Baray, Kevin W. Bowman, John R. Worden, Felipe J. Cardoso-Saldaña, Emily Reidy, and Daniel J. Jacob
Geosci. Model Dev., 18, 3311–3330, https://doi.org/10.5194/gmd-18-3311-2025, https://doi.org/10.5194/gmd-18-3311-2025, 2025
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Reducing emissions of methane, a powerful greenhouse gas, is a top policy concern for mitigating anthropogenic climate change. The Integrated Methane Inversion (IMI) is an advanced, cloud-based software that translates satellite observations into actionable emissions data. Here we present IMI version 2.0 with vastly expanded capabilities. These updates enable a wider range of scientific and stakeholder applications from individual basin to global scales with continuous emissions monitoring.
Cynthia H. Whaley, Tim Butler, Jose A. Adame, Rupal Ambulkar, Steve R. Arnold, Rebecca R. Buchholz, Benjamin Gaubert, Douglas S. Hamilton, Min Huang, Hayley Hung, Johannes W. Kaiser, Jacek W. Kaminski, Christoph Knote, Gerbrand Koren, Jean-Luc Kouassi, Meiyun Lin, Tianjia Liu, Jianmin Ma, Kasemsan Manomaiphiboon, Elisa Bergas Masso, Jessica L. McCarty, Mariano Mertens, Mark Parrington, Helene Peiro, Pallavi Saxena, Saurabh Sonwani, Vanisa Surapipith, Damaris Y. T. Tan, Wenfu Tang, Veerachai Tanpipat, Kostas Tsigaridis, Christine Wiedinmyer, Oliver Wild, Yuanyu Xie, and Paquita Zuidema
Geosci. Model Dev., 18, 3265–3309, https://doi.org/10.5194/gmd-18-3265-2025, https://doi.org/10.5194/gmd-18-3265-2025, 2025
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The multi-model experiment design of the HTAP3 Fires project takes a multi-pollutant approach to improving our understanding of transboundary transport of wildland fire and agricultural burning emissions and their impacts. The experiments are designed with the goal of answering science policy questions related to fires. The options for the multi-model approach, including inputs, outputs, and model setup, are discussed, and the official recommendations for the project are presented.
Maurin Zouzoua, Sophie Bastin, Fabienne Lohou, Marie Lothon, Marjolaine Chiriaco, Mathilde Jome, Cécile Mallet, Laurent Barthes, and Guylaine Canut
Geosci. Model Dev., 18, 3211–3239, https://doi.org/10.5194/gmd-18-3211-2025, https://doi.org/10.5194/gmd-18-3211-2025, 2025
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This study proposes using a statistical model to freeze errors due to differences in environmental forcing when evaluating the surface turbulent heat fluxes from numerical simulations with observations. The statistical model is first built with observations and then applied to the simulated environment to generate possibly observed fluxes. This novel method provides insight into differently evaluating the numerical formulation of turbulent heat fluxes with a long period of observational data.
Oxana Drofa
Geosci. Model Dev., 18, 3175–3209, https://doi.org/10.5194/gmd-18-3175-2025, https://doi.org/10.5194/gmd-18-3175-2025, 2025
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This paper presents the result of many years of effort of the author, who developed an original mathematical numerical model of heat and moisture exchange processes in soil, vegetation, and snow. The author relied on her 30 years of research experience in atmospheric numerical modelling. The presented model is the fruit of the author's research on physical processes at the surface–atmosphere interface and their numerical approximation and aims at improving numerical weather forecasting and climate simulations.
Tyler P. Janoski, Ivan Mitevski, Ryan J. Kramer, Michael Previdi, and Lorenzo M. Polvani
Geosci. Model Dev., 18, 3065–3079, https://doi.org/10.5194/gmd-18-3065-2025, https://doi.org/10.5194/gmd-18-3065-2025, 2025
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We developed ClimKern, a Python package and radiative kernel repository, to simplify calculating radiative feedbacks and make climate sensitivity studies more reproducible. Testing of ClimKern with sample climate model data reveals that radiative kernel choice may be more important than previously thought, especially in polar regions. Our work highlights the need for kernel sensitivity analyses to be included in future studies.
Matti Niskanen, Aku Seppänen, Henri Oikarinen, Miska Olin, Panu Karjalainen, Santtu Mikkonen, and Kari Lehtinen
Geosci. Model Dev., 18, 2983–3001, https://doi.org/10.5194/gmd-18-2983-2025, https://doi.org/10.5194/gmd-18-2983-2025, 2025
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Particle size is a key factor determining the properties of aerosol particles which have a major influence on the climate and on human health. When measuring the particle sizes, however, sometimes the sampling lines that transfer the aerosol to the measurement device distort the size distribution, making the measurement unreliable. We propose a method to correct for the distortions and estimate the true particle sizes, improving measurement accuracy.
Johann Rasmus Nüß, Nikos Daskalakis, Fabian Günther Piwowarczyk, Angelos Gkouvousis, Oliver Schneising, Michael Buchwitz, Maria Kanakidou, Maarten C. Krol, and Mihalis Vrekoussis
Geosci. Model Dev., 18, 2861–2890, https://doi.org/10.5194/gmd-18-2861-2025, https://doi.org/10.5194/gmd-18-2861-2025, 2025
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We estimate carbon monoxide emissions through inverse modeling, an approach where measurements of tracers in the atmosphere are fed to a model to calculate backwards in time (inverse) where the tracers came from. We introduce measurements from a new satellite instrument and show that, in most places globally, these on their own sufficiently constrain the emissions. This alleviates the need for additional datasets, which could shorten the delay for future carbon monoxide source estimates.
Ashu Dastoor, Hélène Angot, Johannes Bieser, Flora Brocza, Brock Edwards, Aryeh Feinberg, Xinbin Feng, Benjamin Geyman, Charikleia Gournia, Yipeng He, Ian M. Hedgecock, Ilia Ilyin, Jane Kirk, Che-Jen Lin, Igor Lehnherr, Robert Mason, David McLagan, Marilena Muntean, Peter Rafaj, Eric M. Roy, Andrei Ryjkov, Noelle E. Selin, Francesco De Simone, Anne L. Soerensen, Frits Steenhuisen, Oleg Travnikov, Shuxiao Wang, Xun Wang, Simon Wilson, Rosa Wu, Qingru Wu, Yanxu Zhang, Jun Zhou, Wei Zhu, and Scott Zolkos
Geosci. Model Dev., 18, 2747–2860, https://doi.org/10.5194/gmd-18-2747-2025, https://doi.org/10.5194/gmd-18-2747-2025, 2025
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This paper introduces the Multi-Compartment Mercury (Hg) Modeling and Analysis Project (MCHgMAP) aimed at informing the effectiveness evaluations of two multilateral environmental agreements: the Minamata Convention on Mercury and the Convention on Long-Range Transboundary Air Pollution. The experimental design exploits a variety of models (atmospheric, land, oceanic ,and multimedia mass balance models) to assess the short- and long-term influences of anthropogenic Hg releases into the environment.
Hilda Sandström and Patrick Rinke
Geosci. Model Dev., 18, 2701–2724, https://doi.org/10.5194/gmd-18-2701-2025, https://doi.org/10.5194/gmd-18-2701-2025, 2025
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Machine learning has the potential to aid the identification of organic molecules involved in aerosol formation. Yet, progress is stalled by a lack of curated atmospheric molecular datasets. Here, we compared atmospheric compounds with large molecular datasets used in machine learning and found minimal overlap with similarity algorithms. Our result underlines the need for collaborative efforts to curate atmospheric molecular data to facilitate machine learning models in atmospheric sciences.
Juan Escobar, Philippe Wautelet, Joris Pianezze, Florian Pantillon, Thibaut Dauhut, Christelle Barthe, and Jean-Pierre Chaboureau
Geosci. Model Dev., 18, 2679–2700, https://doi.org/10.5194/gmd-18-2679-2025, https://doi.org/10.5194/gmd-18-2679-2025, 2025
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The Meso-NH weather research code is adapted for GPUs using OpenACC, leading to significant performance and energy efficiency improvements. Called MESONH-v55-OpenACC, it includes enhanced memory management, communication optimizations and a new solver. On the AMD MI250X Adastra platform, it achieved up to 6× speedup and 2.3× energy efficiency gain compared to CPUs. Storm simulations at 100 m resolution show positive results, positioning the code for future use on exascale supercomputers.
Jie Gao, Yi Huang, Jonathon S. Wright, Ke Li, Tao Geng, and Qiurun Yu
Geosci. Model Dev., 18, 2569–2586, https://doi.org/10.5194/gmd-18-2569-2025, https://doi.org/10.5194/gmd-18-2569-2025, 2025
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The aerosol in the upper troposphere and stratosphere is highly variable, and its radiative effect is poorly understood. To estimate this effect, the radiative kernel is constructed and applied. The results show that the kernels can reproduce aerosol radiative effects and are expected to simulate stratospheric aerosol radiative effects. This approach reduces computational expense, is consistent with radiative model calculations, and can be applied to atmospheric models with speed requirements.
Ji Won Yoon, Seungyeon Lee, Ebony Lee, and Seon Ki Park
Geosci. Model Dev., 18, 2303–2328, https://doi.org/10.5194/gmd-18-2303-2025, https://doi.org/10.5194/gmd-18-2303-2025, 2025
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This study evaluates the Weather Research and Forecasting Model (WRF) coupled with Chemistry (WRF-Chem) to predict a mega Asian dust storm (ADS) over South Korea on 28–29 March 2021. We assessed combinations of five dust emission and four land surface schemes by analyzing meteorological and air quality variables. The best scheme combination reduced the root mean square error (RMSE) for particulate matter 10 (PM10) by up to 29.6 %, demonstrating the highest performance.
Jens Peter Karolus Wenceslaus Frankemölle, Johan Camps, Pieter De Meutter, and Johan Meyers
Geosci. Model Dev., 18, 1989–2003, https://doi.org/10.5194/gmd-18-1989-2025, https://doi.org/10.5194/gmd-18-1989-2025, 2025
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To detect anomalous radioactivity in the environment, it is paramount that we understand the natural background level. In this work, we propose a statistical model to describe the most likely background level and the associated uncertainty in a network of dose rate detectors. We train, verify, and validate the model using real environmental data. Using the model, we show that we can correctly predict the background level in a subset of the detector network during a known
anomalous event.
Jean-François Grailet, Robin J. Hogan, Nicolas Ghilain, David Bolsée, Xavier Fettweis, and Marilaure Grégoire
Geosci. Model Dev., 18, 1965–1988, https://doi.org/10.5194/gmd-18-1965-2025, https://doi.org/10.5194/gmd-18-1965-2025, 2025
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The MAR (Modèle Régional Atmosphérique) is a regional climate model used for weather forecasting and studying the climate over various regions. This paper presents an update of MAR thanks to which it can precisely decompose solar radiation, in particular in the UV (ultraviolet) and photosynthesis ranges, both being critical to human health and ecosystems. As a first application of this new capability, this paper presents a method for predicting UV indices with MAR.
Yi-Ning Shi, Jun Yang, Wei Han, Lujie Han, Jiajia Mao, Wanlin Kan, and Fuzhong Weng
Geosci. Model Dev., 18, 1947–1964, https://doi.org/10.5194/gmd-18-1947-2025, https://doi.org/10.5194/gmd-18-1947-2025, 2025
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Direct assimilation of observations from ground-based microwave radiometers (GMRs) holds significant potential for improving forecast accuracy. Radiative transfer models (RTMs) play a crucial role in direct data assimilation. In this study, we introduce a new RTM, the Advanced Radiative Transfer Modeling System – Ground-Based (ARMS-gb), designed to simulate brightness temperatures observed by GMRs along with their Jacobians. Several enhancements have been incorporated to achieve higher accuracy.
R. Phani Murali Krishna, Siddharth Kumar, A. Gopinathan Prajeesh, Peter Bechtold, Nils Wedi, Kumar Roy, Malay Ganai, B. Revanth Reddy, Snehlata Tirkey, Tanmoy Goswami, Radhika Kanase, Sahadat Sarkar, Medha Deshpande, and Parthasarathi Mukhopadhyay
Geosci. Model Dev., 18, 1879–1894, https://doi.org/10.5194/gmd-18-1879-2025, https://doi.org/10.5194/gmd-18-1879-2025, 2025
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The High-Resolution Global Forecast Model (HGFM) is an advanced iteration of the operational Global Forecast System (GFS) model. HGFM can produce forecasts at a spatial scale of ~6 km in tropics. It demonstrates improved accuracy in short- to medium-range weather prediction over the Indian region, with notable success in predicting extreme events. Further, the model will be entrusted to operational forecasting agencies after validation and testing.
Jenna Ritvanen, Seppo Pulkkinen, Dmitri Moisseev, and Daniele Nerini
Geosci. Model Dev., 18, 1851–1878, https://doi.org/10.5194/gmd-18-1851-2025, https://doi.org/10.5194/gmd-18-1851-2025, 2025
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Nowcasting models struggle with the rapid evolution of heavy rain, and common verification methods are unable to describe how accurately the models predict the growth and decay of heavy rain. We propose a framework to assess model performance. In the framework, convective cells are identified and tracked in the forecasts and observations, and the model skill is then evaluated by comparing differences between forecast and observed cells. We demonstrate the framework with four open-source models.
Andrew Geiss and Po-Lun Ma
Geosci. Model Dev., 18, 1809–1827, https://doi.org/10.5194/gmd-18-1809-2025, https://doi.org/10.5194/gmd-18-1809-2025, 2025
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Particles in the Earth's atmosphere strongly impact the planet's energy budget, and atmosphere simulations require accurate representation of their interaction with light. This work introduces two approaches to represent light scattering by small particles. The first is a scattering simulator based on Mie theory implemented in Python. The second is a neural network emulator that is more accurate than existing methods and is fast enough to be used in climate and weather simulations.
Andrin Jörimann, Timofei Sukhodolov, Beiping Luo, Gabriel Chiodo, Graham Mann, and Thomas Peter
EGUsphere, https://doi.org/10.5194/egusphere-2025-145, https://doi.org/10.5194/egusphere-2025-145, 2025
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Aerosol particles in the stratosphere affect our climate. Climate models therefore need an accurate description of their properties and evolution. Satellites measure how strongly aerosol particles extinguish light passing through the stratosphere. We describe a method to use such aerosol extinction data to retrieve the number and sizes of the aerosol particles and calculate their optical effects. The resulting data sets for models are validated against ground-based and balloon observations.
Qin Wang, Bo Zeng, Gong Chen, and Yaoting Li
Geosci. Model Dev., 18, 1769–1784, https://doi.org/10.5194/gmd-18-1769-2025, https://doi.org/10.5194/gmd-18-1769-2025, 2025
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This study evaluates the performance of four planetary boundary layer (PBL) schemes in near-surface wind fields over the Sichuan Basin, China. Using 112 sensitivity experiments with the Weather Research and Forecasting (WRF) model and focusing on 28 wind events, it is found that wind direction was less sensitive to the PBL schemes. The quasi-normal scale elimination (QNSE) scheme captured temporal variations best, while the Mellor–Yamada–Janjić (MYJ) scheme had the least error in wind speed.
Tai-Long He, Nikhil Dadheech, Tammy M. Thompson, and Alexander J. Turner
Geosci. Model Dev., 18, 1661–1671, https://doi.org/10.5194/gmd-18-1661-2025, https://doi.org/10.5194/gmd-18-1661-2025, 2025
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It is computationally expensive to infer greenhouse gas (GHG) emissions using atmospheric observations. This is partly due to the detailed model used to represent atmospheric transport. We demonstrate how a machine learning (ML) model can be used to simulate high-resolution atmospheric transport. This type of ML model will help estimate GHG emissions using dense observations, which are becoming increasingly common with the proliferation of urban monitoring networks and geostationary satellites.
Wei Li, Beiming Tang, Patrick C. Campbell, Youhua Tang, Barry Baker, Zachary Moon, Daniel Tong, Jianping Huang, Kai Wang, Ivanka Stajner, and Raffaele Montuoro
Geosci. Model Dev., 18, 1635–1660, https://doi.org/10.5194/gmd-18-1635-2025, https://doi.org/10.5194/gmd-18-1635-2025, 2025
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The study describes the updates of NOAA's current UFS-AQMv7 air quality forecast model by incorporating the latest scientific and structural changes in CMAQv5.4. An evaluation during the summer of 2023 shows that the updated model overall improves the simulation of MDA8 O3 by reducing the bias by 8%–12% in the contiguous US. PM2.5 predictions have mixed results due to wildfire, highlighting the need for future refinements.
Yanwei Zhu, Aitor Atencia, Markus Dabernig, and Yong Wang
Geosci. Model Dev., 18, 1545–1559, https://doi.org/10.5194/gmd-18-1545-2025, https://doi.org/10.5194/gmd-18-1545-2025, 2025
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Most works have delved into convective weather nowcasting, and only a few works have discussed the nowcasting uncertainty for variables at the surface level. Hence, we proposed a method to estimate uncertainty. Generating appropriate noises associated with the characteristic of the error in analysis can simulate the uncertainty of nowcasting. This method can contribute to the estimation of near–surface analysis uncertainty in both nowcasting applications and ensemble nowcasting development.
Joël Thanwerdas, Antoine Berchet, Lionel Constantin, Aki Tsuruta, Michael Steiner, Friedemann Reum, Stephan Henne, and Dominik Brunner
Geosci. Model Dev., 18, 1505–1544, https://doi.org/10.5194/gmd-18-1505-2025, https://doi.org/10.5194/gmd-18-1505-2025, 2025
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The Community Inversion Framework (CIF) brings together methods for estimating greenhouse gas fluxes from atmospheric observations. The initial ensemble method implemented in CIF was found to be incomplete and could hardly be compared to other ensemble methods employed in the inversion community. In this paper, we present and evaluate a new implementation of the ensemble mode, building upon the initial developments.
Astrid Kerkweg, Timo Kirfel, Duong H. Do, Sabine Griessbach, Patrick Jöckel, and Domenico Taraborrelli
Geosci. Model Dev., 18, 1265–1286, https://doi.org/10.5194/gmd-18-1265-2025, https://doi.org/10.5194/gmd-18-1265-2025, 2025
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Normally, the Modular Earth Submodel System (MESSy) is linked to complete dynamic models to create chemical climate models. However, the modular concept of MESSy and the newly developed DWARF component presented here make it possible to create simplified models that contain only one or a few process descriptions. This is very useful for technical optimisation, such as porting to GPUs, and can be used to create less complex models, such as a chemical box model.
Peter Wind and Willem van Caspel
EGUsphere, https://doi.org/10.5194/egusphere-2024-3571, https://doi.org/10.5194/egusphere-2024-3571, 2025
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This paper presents a numerical method to assess the origin of air pollution. Combined with a numerical air pollution transport and chemistry model, it can follow the contributions from a large number of emission sources. The result is a series of maps that give the relative contributions from for example all European countries at each point.
Julian Vogel, Sebastian Stadler, Ganesh Chockalingam, Afshin Afshari, Johanna Henning, and Matthias Winkler
EGUsphere, https://doi.org/10.5194/egusphere-2025-144, https://doi.org/10.5194/egusphere-2025-144, 2025
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This study presents a toolkit to simplify input data creation for the urban microclimate model PALM-4U. It introduces novel methods to automate the use of open data sources. Our analysis of four test cases created from different geographic data sources shows variations in temperature, humidity, and wind speed, influenced by data quality. Validation indicates that the automated methods yield results comparable to expert-driven approaches, facilitating user-friendly urban climate modeling.
Edward C. Chan, Ilona J. Jäkel, Basit Khan, Martijn Schaap, Timothy M. Butler, Renate Forkel, and Sabine Banzhaf
Geosci. Model Dev., 18, 1119–1139, https://doi.org/10.5194/gmd-18-1119-2025, https://doi.org/10.5194/gmd-18-1119-2025, 2025
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An enhanced emission module has been developed for the PALM model system, improving flexibility and scalability of emission source representation across different sectors. A model for parametrized domestic emissions has also been included, for which an idealized model run is conducted for particulate matter (PM10). The results show that, in addition to individual sources and diurnal variations in energy consumption, vertical transport and urban topology play a role in concentration distribution.
Gregor Ehrensperger, Thorsten Simon, Georg J. Mayr, and Tobias Hell
Geosci. Model Dev., 18, 1141–1153, https://doi.org/10.5194/gmd-18-1141-2025, https://doi.org/10.5194/gmd-18-1141-2025, 2025
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As lightning is a brief and localized event, it is not explicitly resolved in atmospheric models. Instead, expert-based auxiliary descriptions are used to assess it. This study explores how AI can improve our understanding of lightning without relying on traditional expert knowledge. We reveal that AI independently identified the key factors known to experts as essential for lightning in the Alps region. This shows how knowledge discovery could be sped up in areas with limited expert knowledge.
David Patoulias, Kalliopi Florou, and Spyros N. Pandis
Geosci. Model Dev., 18, 1103–1118, https://doi.org/10.5194/gmd-18-1103-2025, https://doi.org/10.5194/gmd-18-1103-2025, 2025
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The effect of the assumed atmospheric nucleation mechanism on particle number concentrations and size distribution was investigated. Two quite different mechanisms involving sulfuric acid and ammonia or a biogenic organic vapor gave quite similar results which were consistent with measurements at 26 measurement stations across Europe. The number of larger particles that serve as cloud condensation nuclei showed little sensitivity to the assumed nucleation mechanism.
Tim Radke, Susanne Fuchs, Christian Wilms, Iuliia Polkova, and Marc Rautenhaus
Geosci. Model Dev., 18, 1017–1039, https://doi.org/10.5194/gmd-18-1017-2025, https://doi.org/10.5194/gmd-18-1017-2025, 2025
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In our study, we built upon previous work to investigate the patterns artificial intelligence (AI) learns to detect atmospheric features like tropical cyclones (TCs) and atmospheric rivers (ARs). As primary objective, we adopt a method to explain the AI used and investigate the plausibility of learned patterns. We find that plausible patterns are learned for both TCs and ARs. Hence, the chosen method is very useful for gaining confidence in the AI-based detection of atmospheric features.
Leon Geers, Ruud Janssen, Gudrun Thorkelsdottir, Jordi Vilà-Guerau de Arellano, and Martijn Schaap
EGUsphere, https://doi.org/10.5194/egusphere-2025-426, https://doi.org/10.5194/egusphere-2025-426, 2025
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High-resolution data on reactive nitrogen deposition are needed to inform cost-effective policies. Here, we describe the implementation of a dry deposition module into a large eddy simulation code. With this model, we are able to represent the turbulent exchange of tracers at the hectometer resolution. The model calculates the dispersion and deposition of NOx and NH3 in great spatial detail, clearly showing the influence of local land use patterns.
Raphaël Périllat, Sylvain Girard, and Irène Korsakissok
EGUsphere, https://doi.org/10.5194/egusphere-2024-3838, https://doi.org/10.5194/egusphere-2024-3838, 2025
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We developed a method to improve decision-making during nuclear crises by predicting the spread of radiation more efficiently. Existing approaches are often too slow, especially when analyzing complex data like radiation maps. Our method combines techniques to simplify these maps and predict them quickly using statistical tools. This approach could help authorities respond faster and more accurately in emergencies, reducing risks to the population and the environment.
Shaofeng Hua, Gang Chen, Baojun Chen, Mingshan Li, and Xin Xu
EGUsphere, https://doi.org/10.5194/egusphere-2024-3834, https://doi.org/10.5194/egusphere-2024-3834, 2025
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Hail forecasting using numerical models remains a challenge. In this study, we found that the commonly used graupel-to-hail conversion parameterization method led to hail overforecasting in heavy rainfall cases where no hail was observed. By incorporating the spongy wet growth process, we successfully mitigated hail overforecasting. The modified scheme also produced hail in real hail events. This research contributes to a better understanding of hail formation.
Stefan Noll, Carsten Schmidt, Patrick Hannawald, Wolfgang Kausch, and Stefan Kimeswenger
EGUsphere, https://doi.org/10.5194/egusphere-2024-3512, https://doi.org/10.5194/egusphere-2024-3512, 2025
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Non-thermal emission from chemical reactions in the Earth's middle und upper atmosphere strongly contributes to the brightness of the night sky below about 2.3 µm. The new Paranal Airglow Line and Continuum Emission model calculates the emission spectrum and its variability with an unprecedented accuracy. Relying on a large spectroscopic data set from astronomical spectrographs and theoretical molecular/atomic data, it is valuable for airglow research and astronomical observatories.
Felipe Cifuentes, Henk Eskes, Enrico Dammers, Charlotte Bryan, and Folkert Boersma
Geosci. Model Dev., 18, 621–649, https://doi.org/10.5194/gmd-18-621-2025, https://doi.org/10.5194/gmd-18-621-2025, 2025
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We tested the capability of the flux divergence approach (FDA) to reproduce known NOx emissions using synthetic NO2 satellite column retrievals from high-resolution model simulations. The FDA accurately reproduced NOx emissions when column observations were limited to the boundary layer and when the variability of the NO2 lifetime, the NOx : NO2 ratio, and NO2 profile shapes were correctly modeled. This introduces strong model dependency, reducing the simplicity of the original FDA formulation.
Stefano Ubbiali, Christian Kühnlein, Christoph Schär, Linda Schlemmer, Thomas C. Schulthess, Michael Staneker, and Heini Wernli
Geosci. Model Dev., 18, 529–546, https://doi.org/10.5194/gmd-18-529-2025, https://doi.org/10.5194/gmd-18-529-2025, 2025
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We explore a high-level programming model for porting numerical weather prediction (NWP) model codes to graphics processing units (GPUs). We present a Python rewrite with the domain-specific library GT4Py (GridTools for Python) of two renowned cloud microphysics schemes and the associated tangent-linear and adjoint algorithms. We find excellent portability, competitive GPU performance, robust execution on diverse computing architectures, and enhanced code maintainability and user productivity.
Pieter Rijsdijk, Henk Eskes, Arlene Dingemans, K. Folkert Boersma, Takashi Sekiya, Kazuyuki Miyazaki, and Sander Houweling
Geosci. Model Dev., 18, 483–509, https://doi.org/10.5194/gmd-18-483-2025, https://doi.org/10.5194/gmd-18-483-2025, 2025
Short summary
Short summary
Clustering high-resolution satellite observations into superobservations improves model validation and data assimilation applications. In our paper, we derive quantitative uncertainties for satellite NO2 column observations based on knowledge of the retrievals, including a detailed analysis of spatial error correlations and representativity errors. The superobservations and uncertainty estimates are tested in a global chemical data assimilation system and are found to improve the forecasts.
Cited articles
Anderson, J. L.: An adaptive covariance inflation error correction algorithm for ensemble filters, Tellus A, 59, 210–224, https://doi.org/10.1111/j.1600-0870.2006.00216.x, 2007.
Anderson, J. L. and Anderson, S. L.: A Monte Carlo implementation of the nonlinear filtering problem to produce ensemble assimilations and forecasts, Mon. Weather Rev., 127, 2741–2758, 1999.
Bao, J., Yang, X., Zhao, Z., Wang, Z., Yu, C., and Li, X.: The spatial-temporal characteristics of air pollution in China from 2001–2014, Int. J. Environ. Res. Publ. Health, 12, 15875e15887, https://doi.org/10.3390/ijerph121215029, 2015.
Barbu, A. L., Segers, A. J., Schaap, M., Heemink, A. W., and Builtjes, P. J. H.: A multi-component data assimilation experiment directed to sulphur dioxide and sulphate over Europe, Atmos. Environ., 43, 1622–1631, https://doi.org/10.1016/j.atmosenv.2008.12.005, 2009.
Benedetti, A., Morcrette, J., Boucher, O., Dethof, A., Engelen, R. J., Fisher, M., Flentje, H., Huneeus, N., Jones, L., Kaiser, J. W., Kinne, S., Mangold, A., Razinger, M., Simmons, A. J., and Suttie, M.: Aerosol analysis and forecast in the European Centre for Medium-Range Weather Forecasts Integrated Forecast System: 2. Data assimilation, J. Geophys. Res., 114, D13205, https://doi.org/10.1029/2008JD011115, 2009.
Cheng, Y., Dai, T., Goto, D., Schutgens, N. A. J., Shi, G., and Nakajima, T.: Investigating the assimilation of CALIPSO global aerosol vertical observations using a four-dimensional ensemble Kalman filter, Atmos. Chem. Phys., 19, 13445–13467, https://doi.org/10.5194/acp-19-13445-2019, 2019.
Chen, D., Liu, Z., Ban, J., and Chen, M.: The 2015 and 2016 wintertime air pollution in China: SO2 emission changes derived from a WRF-Chem/EnKF coupled data assimilation system , Atmos. Chem. Phys., 19, 8619–8650, https://doi.org/10.5194/acp-19-8619-2019, 2019a.
Chen, D., Liu, Z., Ban, J., Zhao, P., and Chen, M.: Retrospective analysis of 2015–2017 wintertime PM2.5 in China: response to emission regulations and the role of meteorology, Atmos. Chem. Phys., 19, 7409–7427, https://doi.org/10.5194/acp-19-7409-2019, 2019b.
CNEMC: China National Environmental Monitoring Center, https://www.cnemc.cn (last access: 31 December 2024), 2024.
Dai, T., Cheng, Y., Suzuki, K., Goto, D., Kikuchi, M., Schutgens, N. A. J., Yoshida, M., Zhang, P., Husi, L., Shi, G., and Nakajima, T.: Hourly Aerosol Assimilation of Himawari-8 AOT Using the Four-Dimensional Local Ensemble Transform Kalman Filter, J. Adv. Model. Earth Sy., 11, 680–711, https://doi.org/10.1029/2018MS001475, 2019.
Dai, T., Cheng, Y., Goto, D., Li, Y., Tang, X., Shi, G., and Nakajima, T.: Revealing the sulfur dioxide emission reductions in China by assimilating surface observations in WRF-Chem, Atmos. Chem. Phys., 21, 4357–4379, https://doi.org/10.5194/acp-21-4357-2021, 2021.
Elbern, H., Strunk, A., Schmidt, H., and Talagrand, O.: Emission rate and chemical state estimation by 4-dimensional variational inversion, Atmos. Chem. Phys., 7, 3749–3769, https://doi.org/10.5194/acp-7-3749-2007, 2007.
Evensen, G.: Sequential data assimilation with a nonlinear quasi-geostrophic model using Monte Carlo methods to forecast error statistics, J. Geophys. Res.-Oceans, 99, 10143–10162, https://doi.org/10.1029/94JC00572, 1994.
Evensen, G.: The Ensemble Kalman Filter: theoretical formulation and practical implementation, Ocean Dynam., 53, 343–367, https://doi.org/10.1007/s10236-003-0036-9, 2003.
Feng, S., Jiang, F., Jiang, Z., Wang, H., Cai, Z., and Zhang, L.: Impact of 3DVAR assimilation of surface PM2.5 observations on PM2.5 forecasts over China during wintertime, Atmos. Environ., 187, 34–49, https://doi.org/10.1016/j.atmosenv.2018.05.049, 2018.
Feng, S., Jiang, F., Wang, H., Wang, H., Ju, W., Shen, Y., Zheng, Y., Wu, Z., and Ding, A.: NOx emission changes over China during the COVID-19 epidemic inferred from surface NO2 observations, Geophys. Res. Lett., 47, e2020GL090080, https://doi.org/10.1029/2020GL090080, 2020a.
Feng, S., Jiang, F., Wu, Z., Wang, H., Ju, W., and Wang, H.: CO emissions inferred from surface CO observations over China in December 2013 and 2017, J. Geophys. Res.-Atmos., 125, e2019JD031808, https://doi.org/10.1029/2019JD031808, 2020b.
Feng, S., Jiang, F., Wu, Z., Wang, H., He, W., Shen, Y., Zhang, L., Zheng, Y., Lou, C., Jiang, Z., and Ju, W.: A Regional multi-Air Pollutant Assimilation System (RAPAS v1.0) for emission estimates: system development and application, Geosci. Model Dev., 16, 5949–5977, https://doi.org/10.5194/gmd-16-5949-2023, 2023.
Gao, M., Saide, P. E., Xin, J., Wang, Y., Liu, Z., Wang, Y., Wang, Z., Pagowski, M., Guttikunda, S. K., and Carmichael, G. R.: Estimates of Health Impacts and Radiative Forcing in Winter Haze in Eastern China through Constraints of Surface PM2.5 Predictions, Environ. Sci. Technol., 51, 2178–2185, https://doi.org/10.1021/acs.est.6b03745, 2017.
Grell, G., Peckham, S. E., Schmitz, R., McKeen, S. A., Frost, G., Skamarock, W. C., and Eder, B.: Fully coupled “online” chemistry within the WRF model, Atmos. Environ, 39, 6957–6975, https://doi.org/10.1016/j.atmosenv.2005.04.027, 2005.
Grell, G. A.: Prognostic Evaluation of Assumptions Used by Cumulus Parameterizations, Mon. Weather Rev., 121, 764–787, https://doi.org/10.1175/1520-0493(1993)121<0764:PEOAUB>2.0.CO;2, 1993.
Guenther, A., Hewitt, C. N., Erickson, D., Fall, R., Geron, C., Graedel, T., Harley, P., Klinger, L., Lerdau, M., Mckay, W. A., Pierce, T., Scholes, B., Steinbrecher, R., Tallamraju, R., Taylor, J., and Zimmerman, P.: A global model of natural volatile organic compound emissions, J. Geophys. Res.-Atmos., 100, 8873–8892, https://doi.org/10.1029/94JD02950, 1995.
Hong, S., Noh, Y., and Dudhia, J.: A new vertical diffusion package with an explicit treatment of entrainment processes, Mon. Weather Rev., 134, 2318–2341, https://doi.org/10.1175/MWR3199.1, 2006.
Huang, X. Y., Xiao, Q., Barker, D. M., Zhang, X., Michalakes, J., Huang, W., Henderson, T., Bray, J., Chen, Y., Ma, Z., Dudhia, J., Guo, Y., Zhang, X., Won, D., Lin, H., and Kuo, Y.: Four-dimensional variational data assimilation for WRF: Formulation and preliminary results, Mon. Weather Rev., 137, 299–314, https://doi.org/10.1175/2008MWR2577.1, 2009.
Hunt, B. R., Kalnay, E., Kostelich, E. J., Ott, E., Patil, D. J., Sauer, T., Szunyogh, I., Yorke, J. A., and Zimin, A. V.: Four-dimensional ensemble Kalman filtering, Tellus A, 56, 273–277, https://doi.org/10.3402/tellusa.v56i4.14424, 2004.
Hunt, B. R., Kostelich, E. J., and Szunyogh, I.: Efficient data assimilation for spatiotemporal chaos: a local ensemble transform Kalman filter, Physica D, 230, 112–126, https://doi.org/10.1016/j.physd.2006.11.008, 2007.
Iacono, M. J., Delamere, J. S., Mlawer, E. J., Shephard, M. W., Clough, S. A., and Collins, W. D.: Radiative forcing by long–lived greenhouse gases: Calculations with the AER radiative transfer models, J. Geophys. Res., 113, D13103, https://doi.org/10.1029/2008JD009944, 2008.
Jin, J., Pang, M., Segers, A., Han, W., Fang, L., Li, B., Feng, H., Lin, H. X., and Liao, H.: Inverse modeling of the 2021 spring super dust storms in East Asia, Atmos. Chem. Phys., 22, 6393–6410, https://doi.org/10.5194/acp-22-6393-2022, 2022.
Kong, L., Tang, X., Zhu, J., Wang, Z., Sun, Y., Fu, P., Gao, M., Wu, H., Lu, M., Wu, Q., Huang, S., Sui, W., Li, J., Pan, X., Wu, L., Akimoto, H., and Carmichael, G. R.: Unbalanced emission reductions of different species and sectors in China during COVID-19 lockdown derived by multi-species surface observation assimilation, Atmos. Chem. Phys., 23, 6217–6240, https://doi.org/10.5194/acp-23-6217-2023, 2023.
Kong, Y., Sheng, L., Li, Y., Zhang, W., Zhou, Y., Wang, W., and Zhao, Y.: Improving PM2.5 forecast during haze episodes over China based on a coupled 4D-LETKF and WRF-Chem system, Atmos. Res., 249, 105366, https://doi.org/10.1016/j.atmosres.2020.105366, 2021.
Lin, J.: LETKF-WRF-Chem, Zenodo [code, data set], https://doi.org/10.5281/zenodo.14010521, 2024.
Lin, J.: Observation, Zenodo [data set], https://doi.org/10.5281/zenodo.14835237, 2025.
Lorenc, A. C.: Analysis methods for numerical weather prediction, Q. J. Roy. Meteor. Soc., 112, 1177–1194, https://doi.org/10.1002/qj.49711247414, 1986.
Luo, X., Tang, X., Wang, H., Kong, L., Wu, H., Wang, W., SONG, Y., Luo, H., Wang, Y., Zhu, J., and Wang, Z.: Investigating the Changes in Air Pollutant Emissions over the Beijing-Tianjin-Hebei Region in February from 2014 to 2019 through an Inverse Emission Method, Adv. Atmos. Sci. 40, 601–618, https://doi.org/10.1007/s00376-022-2039-9, 2023.
Ma, C., Wang, T., Jiang, Z., Wu, H., Zhao, M., Zhuang, B., Li, S., Xie, M., Li, M., Liu, J., and Wu, R.: Importance of bias correction in data assimilation of multiple observations over eastern China using WRF-Chem/DART, J. Geophys. Res.-Atmos., 125, e2019JD031465, https://doi.org/10.1029/2019JD031465, 2020.
MEIC: Multi-resolution Emission Inventory for China, http://www.meicmodel.org/ (last access: 31 December 2024), 2024.
Miyoshi, T., Yamane, S., and Enomoto, T.: Localizing the Error Covariance by Physical Distances within a Local Ensemble Transform Kalman Filter (LETKF), Scient. Online Lett. Atmos., 3, 89–92, https://doi.org/10.2151/sola.2007-023, 2007.
Morrison, H., Thompson, G., and Tatarskii, V.: Impact of Cloud Microphysics on the Development of Trailing Stratiform Precipitation in a Simulated Squall Line: Comparison of One– and Two–Moment Schemes, Mon. Weather Rev., 137, 991–1007, https://doi.org/10.1175/2008MWR2556.1, 2009.
Miyazaki, K., Eskes, H. J., and Sudo, K.: Global NOx emission estimates derived from an assimilation of OMI tropospheric NO2 columns, Atmos. Chem. Phys., 12, 2263–2288, https://doi.org/10.5194/acp-12-2263-2012, 2012a.
Miyazaki, K., Eskes, H. J., Sudo, K., Takigawa, M., van Weele, M., and Boersma, K. F.: Simultaneous assimilation of satellite NO2, O3, CO, and HNO3 data for the analysis of tropospheric chemical composition and emissions, Atmos. Chem. Phys., 12, 9545–9579, https://doi.org/10.5194/acp-12-9545-2012, 2012b.
Miyoshi, T.: LETKF source codes, GitHub, https://github.com/takemasa-miyoshi/letkf, last access: 1 January 2024.
NCDC: National Climatic Data Center, https://www.ncei.noaa.gov (last access: 31 December 2024), 2024.
Ott, E., Hunt, B. R., Szunyogh, I., Zimin, A. V., Kostelich, E. J., Corazza, M., Kalnay, E., Patil, D. J., and Yorke, J. A.: A local ensemble Kalman filter for atmospheric data assimilation, Tellus A, 56, 415–428, https://doi.org/10.1111/j.1600-0870.2004.00076.x, 2004.
Pagowski, M. and Grell, G. A.: Experiments with the assimilation of fine aerosols using an ensemble Kalman filter, J. Geophys. Res., 117, D21302, https://doi.org/10.1029/2012JD018333, 2012.
Parrish, D. F. and Derber, J. C.: The National Meteorological Center's Spectral Statistical-Interpolation Analysis System, Mon. Weather Rev., 120, 1747–1763, https://doi.org/10.1175/1520-0493(1992)120<1747:TNMCSS>2.0.CO;2, 1992.
Peng, Z., Liu, Z., Chen, D., and Ban, J.: Improving PM2.5 forecast over China by the joint adjustment of initial conditions and source emissions with an ensemble Kalman filter, Atmos. Chem. Phys., 17, 4837–4855, https://doi.org/10.5194/acp-17-4837-2017, 2017.
Peng, Z., Lei, L., Liu, Z., Sun, J., Ding, A., Ban, J., Chen, D., Kou, X., and Chu, K.: The impact of multi-species surface chemical observation assimilation on air quality forecasts in China, Atmos. Chem. Phys., 18, 17387–17404, https://doi.org/10.5194/acp-18-17387-2018, 2018.
Rubin, J. I., Reid, J. S., Hansen, J. A., Anderson, J. L., Collins, N., Hoar, T. J., Hogan, T., Lynch, P., McLay, J., Reynolds, C. A., Sessions, W. R., Westphal, D. L., and Zhang, J.: Development of the Ensemble Navy Aerosol Analysis Prediction System (ENAAPS) and its application of the Data Assimilation Research Testbed (DART) in support of aerosol forecasting, Atmos. Chem. Phys., 16, 3927–3951, https://doi.org/10.5194/acp-16-3927-2016, 2016.
Schutgens, N. A. J., Miyoshi, T., Takemura, T., and Nakajima, T.: Sensitivity tests for an ensemble Kalman filter for aerosol assimilation, Atmos. Chem. Phys., 10, 6583–6600, https://doi.org/10.5194/acp-10-6583-2010, 2010.
Sekiyama, T. T., Tanaka, T. Y., Shimizu, A., and Miyoshi, T.: Data assimilation of CALIPSO aerosol observations, Atmos. Chem. Phys., 10, 39–49, https://doi.org/10.5194/acp-10-39-2010, 2010.
Sun, W., Liu, Z., Chen, D., Zhao, P., and Chen, M.: Development and application of the WRFDA-Chem three-dimensional variational (3DVAR) system: aiming to improve air quality forecasting and diagnose model deficiencies, Atmos. Chem. Phys., 20, 9311–9329, https://doi.org/10.5194/acp-20-9311-2020, 2020.
Schwartz, C. S., Liu, Z., Lin, H. C., and McKeen, S. A.: Simultaneous three-dimensional variational assimilation of surface fine particulate matter and MODIS aerosol optical depth, J. Geophys. Res., 117, D13202, https://doi.org/10.1029/2011JD017383, 2012.
Stockwell, W. R., Kirchner, F., Kuhn, M., and Seefeld, S.: A new mechanism for regional atmospheric chemistry modeling, J. Geophys. Res., 102, 25847–25879, https://doi.org/10.1029/97JD00849, 1997.
Tewari, M., Chen, F., Wang, W., Dudhia, J., LeMone, M. A., Mitchell, K., Ek, M., Gayno, G., Wegiel, J., and Cuenca, R. H.: Implementation and verification of the unified NOAH land surface model in the WRF model, 20th conference on weather analysis and forecasting/16th conference on numerical weather prediction, 11–15, 12–16 January 2004, Seattle, WA, USA, https://ams.confex.com/ams/84Annual/techprogram/paper_69061.htm (last access: 4 April 2025), 2004.
van Donkelaar, A., Martin, R. V., Brauer, M., Hsu, N. C., Kahn, R. A., Levy, R. C., Lyapustin, A., Sayer, A. M., and Winker, D. M.: Global estimates of fine particulate matter using a combined geophysical-statistical method with information from satellites, models, and monitors, Environ. Sci. Technol, 50, 3762–3772, https://doi.org/10.1021/acs.est.5b05833, 2016.
Wang, Z., Li, J., Wang, Z., Yang, W., Tang, X., Ge, B., Yan, P., Zhu, L., Chen, X., and Chen, H.: Modeling study of regional severe hazes over mid-eastern China in January 2013 and its implications on pollution prevention and control, Sci. China-Earth Sci., 57, 3–13, https://doi.org/10.1007/s11430-013-4793-0, 2014.
Whitaker, J. S. and Hamill, T. M.: Ensemble data assimilation without perturbed observations, Mon. Weather Rev., 130, 1913–1924, https://doi.org/10.1175/1520-0493(2002)130<1913:EDAWPO>2.0.CO;2, 2002.
Yan, S., Cao, H., Chen, Y., Wu, C., and Fan, H.: Spatial and temporal characteristics of air quality and air pollutants in 2013 in Beijing, Environ. Sci. Pollut Res., 23, 13996–14007, https://doi.org/10.1007/s11356-016-6518-3, 2016.
Yumimoto, K. and Takemura, T.: Direct radiative effect of aerosols estimated using ensemble-based data assimilation in a global aerosol climate model, Geophys. Res. Lett., 38, L21802, https://doi.org/10.1029/2011GL049258, 2011.
Zhan, D., Kwan, M., Zhang, W., Yu, X., Meng, B., and Liu, Q.: The driving factors of air quality index in China, J. Clean. Prod., 197, 1, 1342–1351, https://doi.org/10.1016/j.jclepro.2018.06.108, 2018.
Zhang, Q., Streets, D. G., Carmichael, G. R., He, K. B., Huo, H., Kannari, A., Klimont, Z., Park, I. S., Reddy, S., Fu, J. S., Chen, D., Duan, L., Lei, Y., Wang, L. T., and Yao, Z. L.: Asian emissions in 2006 for the NASA INTEX-B mission, Atmos. Chem. Phys., 9, 5131–5153, https://doi.org/10.5194/acp-9-5131-2009, 2009.
Zhang, Q., Ma, Q., Zhao, B., Liu, X., Wang, Y., Jia, B., and Zhang, X.: Winter haze over North China Plain from 2009 to 2016: Influence of emission and meteorology, Environ. Pollut., 242, 1308–1318, https://doi.org/10.1016/j.envpol.2018.08.019, 2018.
Zhao, Y., Greybush, S. J., Wilson, R. J., Hoffman, R. N., and Kalnay, E.: Impact of assimilation window length on diurnal features in a Mars atmospheric analysis, Tellus A, 67, 26042, https://doi.org/10.3402/tellusa.v67.26042, 2015.
Zheng, B., Cheng, J., Geng, G., Wang, X., Li, M., Shi, Q., Qi, J., Lei, Y., Zhang, Q., and He, K.: Mapping anthropogenic emissions in China at 1 km spatial resolution and its application in air quality modeling, Sci. Bull., 66, 612–620, https://doi.org/10.1016/j.scib.2020.12.008, 2021.
Short summary
The effectiveness of this assimilation system and its sensitivity to the ensemble member size and length of the assimilation window are investigated. This study advances our understanding of the selection of basic parameters in the four-dimensional local ensemble transform Kalman filter assimilation system and the performance of ensemble simulation in a particulate-matter-polluted environment.
The effectiveness of this assimilation system and its sensitivity to the ensemble member size...