Articles | Volume 17, issue 7
https://doi.org/10.5194/gmd-17-2617-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/gmd-17-2617-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Decision Support System version 1.0 (DSS v1.0) for air quality management in Delhi, India
Gaurav Govardhan
CORRESPONDING AUTHOR
Indian Institute of Tropical Meteorology, Ministry of Earth Sciences, Pune, Maharashtra, India
National Centre for Medium-Range Weather Forecasting, Ministry of Earth Sciences, Noida, Uttar Pradesh, India
Sachin D. Ghude
CORRESPONDING AUTHOR
Indian Institute of Tropical Meteorology, Ministry of Earth Sciences, Pune, Maharashtra, India
Rajesh Kumar
NSF National Center for Atmospheric Research, Boulder, CO, United States of America
Sumit Sharma
The Energy and Resources Institute, Delhi, India
Preeti Gunwani
India Meteorology Department, Ministry of Earth Sciences, Delhi, India
Chinmay Jena
India Meteorology Department, Ministry of Earth Sciences, Delhi, India
Prafull Yadav
Indian Institute of Tropical Meteorology, Ministry of Earth Sciences, Pune, Maharashtra, India
Department of Atmospheric and Space Sciences, Savitribai Phule Pune University, Pune, Maharashtra, India
Shubhangi Ingle
Indian Institute of Tropical Meteorology, Ministry of Earth Sciences, Pune, Maharashtra, India
Sreyashi Debnath
Indian Institute of Tropical Meteorology, Ministry of Earth Sciences, Pune, Maharashtra, India
Department of Atmospheric and Space Sciences, Savitribai Phule Pune University, Pune, Maharashtra, India
Pooja Pawar
Indian Institute of Tropical Meteorology, Ministry of Earth Sciences, Pune, Maharashtra, India
Department of Chemical Technology, Kalinga Institute of Industrial Technology (KIIT), Bhubaneshwar, India
Prodip Acharja
Indian Institute of Tropical Meteorology, Ministry of Earth Sciences, Pune, Maharashtra, India
Department of Atmospheric and Space Sciences, Savitribai Phule Pune University, Pune, Maharashtra, India
Rajmal Jat
Indian Institute of Tropical Meteorology, Ministry of Earth Sciences, Pune, Maharashtra, India
Gayatry Kalita
Indian Institute of Tropical Meteorology, Ministry of Earth Sciences, Pune, Maharashtra, India
Rupal Ambulkar
Indian Institute of Tropical Meteorology, Ministry of Earth Sciences, Pune, Maharashtra, India
Department of Environmental Sciences, Savitribai Phule Pune University, Pune, India
Santosh Kulkarni
Centre for Development of Advanced Computing, Innovation Park, Pune, Maharashtra, India
Akshara Kaginalkar
Centre for Development of Advanced Computing, Innovation Park, Pune, Maharashtra, India
Vijay K. Soni
India Meteorology Department, Ministry of Earth Sciences, Delhi, India
Ravi S. Nanjundiah
Centre for Atmospheric and Oceanic Sciences, Indian Institute of Science, Bengaluru, India
Divecha Centre for Climate Change, Indian Institute of Science, Bengaluru, India
Madhavan Rajeevan
National Centre for Earth Science Studies, Thiruvananthapuram, Kerala, India
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Atmos. Chem. Phys., 23, 41–59, https://doi.org/10.5194/acp-23-41-2023, https://doi.org/10.5194/acp-23-41-2023, 2023
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In this study, for the first time in South Asia we compare simulated ammonia, ammonium, and total ammonia using the WRF-Chem model and MARGA measurements during winter in the Indo-Gangetic Plain region. Since observations show HCl promotes the fraction of high chlorides in Delhi, we added HCl / Cl emissions to the model. We conducted three sensitivity experiments with changes in HCl emissions, and improvements are reported in accurately simulating ammonia, ammonium, and total ammonia.
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Atmos. Chem. Phys., 24, 10717–10740, https://doi.org/10.5194/acp-24-10717-2024, https://doi.org/10.5194/acp-24-10717-2024, 2024
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Arpit Awasthi, Baerbel Sinha, Haseeb Hakkim, Sachin Mishra, Varkrishna Mummidivarapu, Gurmanjot Singh, Sachin D. Ghude, Vijay Kumar Soni, Narendra Nigam, Vinayak Sinha, and Madhavan N. Rajeevan
Atmos. Chem. Phys., 24, 10279–10304, https://doi.org/10.5194/acp-24-10279-2024, https://doi.org/10.5194/acp-24-10279-2024, 2024
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Atmos. Chem. Phys., 24, 10363–10384, https://doi.org/10.5194/acp-24-10363-2024, https://doi.org/10.5194/acp-24-10363-2024, 2024
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Andrew O. Langford, Raul J. Alvarez II, Kenneth C. Aikin, Sunil Baidar, W. Alan Brewer, Steven S. Brown, Matthew M. Coggan, Patrick D. Cullis, Jessica Gilman, Georgios I. Gkatzelis, Detlev Helmig, Bryan J. Johnson, K. Emma Knowland, Rajesh Kumar, Aaron D. Lamplugh, Audra McClure-Begley, Brandi J. McCarty, Ann M. Middlebrook, Gabriele Pfister, Jeff Peischl, Irina Petropavlovskikh, Pamela S. Rickley, Andrew W. Rollins, Scott P. Sandberg, Christoph J. Senff, and Carsten Warneke
EGUsphere, https://doi.org/10.5194/egusphere-2024-1938, https://doi.org/10.5194/egusphere-2024-1938, 2024
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High ozone (O3) formed by reactions of nitrogen oxides (NOx) and volatile organic compounds (VOCs) can harm human health and welfare. High O3 is usually associated with hot summer days, but under certain conditions, high O3 can also form under winter conditions. In this study, we describe a high O3 event that occurred in Colorado during the COVID-19 quarantine that was caused in part by the decrease in traffic, and in part by a shallow inversion created by descent of stratospheric air.
Cynthia H. Whaley, Tim Butler, Jose A. Adame, Rupal Ambulkar, Stephen R. Arnold, Rebecca R. Buchholz, Benjamin Gaubert, Douglas S. Hamilton, Min Huang, Hayley Hung, Johannes W. Kaiser, Jacek W. Kaminski, Christophe Knote, Gerbrand Koren, Jean-Luc Kouassi, Meiyun Lin, Tianjia Liu, Jianmin Ma, Kasemsan Manomaiphiboon, Elisa Bergas Masso, Jessica L. McCarty, Mariano Mertens, Mark Parrington, Helene Peiro, Pallavi Saxena, Saurabh Sonwani, Vanisa Surapipith, Damaris Tan, Wenfu Tang, Veerachai Tanpipat, Kostas Tsigaridis, Christine Wiedinmyer, Oliver Wild, Yuanyu Xie, and Paquita Zuidema
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-126, https://doi.org/10.5194/gmd-2024-126, 2024
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Atmos. Chem. Phys., 24, 6635–6662, https://doi.org/10.5194/acp-24-6635-2024, https://doi.org/10.5194/acp-24-6635-2024, 2024
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Revised manuscript under review for ESSD
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Yafang Guo, Chayan Roychoudhury, Mohammad Amin Mirrezaei, Rajesh Kumar, Armin Sorooshian, and Avelino F. Arellano
Geosci. Model Dev., 17, 4331–4353, https://doi.org/10.5194/gmd-17-4331-2024, https://doi.org/10.5194/gmd-17-4331-2024, 2024
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This research focuses on surface ozone (O3) pollution in Arizona, a historically air-quality-challenged arid and semi-arid region in the US. The unique characteristics of this kind of region, e.g., intense heat, minimal moisture, and persistent desert shrubs, play a vital role in comprehending O3 exceedances. Using the WRF-Chem model, we analyzed O3 levels in the pre-monsoon month, revealing the model's skill in capturing diurnal and MDA8 O3 levels.
Leon Kuhn, Steffen Beirle, Vinod Kumar, Sergey Osipov, Andrea Pozzer, Tim Bösch, Rajesh Kumar, and Thomas Wagner
Atmos. Chem. Phys., 24, 185–217, https://doi.org/10.5194/acp-24-185-2024, https://doi.org/10.5194/acp-24-185-2024, 2024
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NO₂ is an important air pollutant. It was observed that the WRF-Chem model shows significant deviations in NO₂ abundance when compared to measurements. We use a 1-month simulation over central Europe to show that these deviations can be mostly resolved by reparameterization of the vertical mixing routine. In order to validate our results, they are compared to in situ, satellite, and MAX-DOAS measurements.
Wenfu Tang, Louisa K. Emmons, Helen M. Worden, Rajesh Kumar, Cenlin He, Benjamin Gaubert, Zhonghua Zheng, Simone Tilmes, Rebecca R. Buchholz, Sara-Eva Martinez-Alonso, Claire Granier, Antonin Soulie, Kathryn McKain, Bruce C. Daube, Jeff Peischl, Chelsea Thompson, and Pieternel Levelt
Geosci. Model Dev., 16, 6001–6028, https://doi.org/10.5194/gmd-16-6001-2023, https://doi.org/10.5194/gmd-16-6001-2023, 2023
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The new MUSICAv0 model enables the study of atmospheric chemistry across all relevant scales. We develop a MUSICAv0 grid for Africa. We evaluate MUSICAv0 with observations and compare it with a previously used model – WRF-Chem. Overall, the performance of MUSICAv0 is comparable to WRF-Chem. Based on model–satellite discrepancies, we find that future field campaigns in an eastern African region (30°E–45°E, 5°S–5°N) could substantially improve the predictive skill of air quality models.
Manu Goudar, Juliëtte C. S. Anema, Rajesh Kumar, Tobias Borsdorff, and Jochen Landgraf
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A framework was developed to automatically detect plumes and compute emission estimates with cross-sectional flux method (CFM) for biomass burning events in TROPOMI CO datasets using Visible Infrared Imaging Radiometer Suite active fire data. The emissions were more reliable when changing plume height in downwind direction was used instead of constant injection height. The CFM had uncertainty even when the meteorological conditions were accurate; thus there is a need for better inversion models.
Matthew S. Johnson, Amir H. Souri, Sajeev Philip, Rajesh Kumar, Aaron Naeger, Jeffrey Geddes, Laura Judd, Scott Janz, Heesung Chong, and John Sullivan
Atmos. Meas. Tech., 16, 2431–2454, https://doi.org/10.5194/amt-16-2431-2023, https://doi.org/10.5194/amt-16-2431-2023, 2023
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Satellites provide vital information for studying the processes controlling ozone formation. Based on the abundance of particular gases in the atmosphere, ozone formation is sensitive to specific human-induced and natural emission sources. However, errors and biases in satellite retrievals hinder this data source’s application for studying ozone formation sensitivity. We conducted a thorough statistical evaluation of two commonly applied satellites for investigating ozone formation sensitivity.
Tuuli Miinalainen, Harri Kokkola, Antti Lipponen, Antti-Pekka Hyvärinen, Vijay Kumar Soni, Kari E. J. Lehtinen, and Thomas Kühn
Atmos. Chem. Phys., 23, 3471–3491, https://doi.org/10.5194/acp-23-3471-2023, https://doi.org/10.5194/acp-23-3471-2023, 2023
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We simulated the effects of aerosol emission mitigation on both global and regional radiative forcing and city-level air quality with a global-scale climate model. We used a machine learning downscaling approach to bias-correct the PM2.5 values obtained from the global model for the Indian megacity New Delhi. Our results indicate that aerosol mitigation could result in both improved air quality and less radiative heating for India.
Prajjwal Rawat, Manish Naja, Evan Fishbein, Pradeep K. Thapliyal, Rajesh Kumar, Piyush Bhardwaj, Aditya Jaiswal, Sugriva N. Tiwari, Sethuraman Venkataramani, and Shyam Lal
Atmos. Meas. Tech., 16, 889–909, https://doi.org/10.5194/amt-16-889-2023, https://doi.org/10.5194/amt-16-889-2023, 2023
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Pooja V. Pawar, Sachin D. Ghude, Gaurav Govardhan, Prodip Acharja, Rachana Kulkarni, Rajesh Kumar, Baerbel Sinha, Vinayak Sinha, Chinmay Jena, Preeti Gunwani, Tapan Kumar Adhya, Eiko Nemitz, and Mark A. Sutton
Atmos. Chem. Phys., 23, 41–59, https://doi.org/10.5194/acp-23-41-2023, https://doi.org/10.5194/acp-23-41-2023, 2023
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In this study, for the first time in South Asia we compare simulated ammonia, ammonium, and total ammonia using the WRF-Chem model and MARGA measurements during winter in the Indo-Gangetic Plain region. Since observations show HCl promotes the fraction of high chlorides in Delhi, we added HCl / Cl emissions to the model. We conducted three sensitivity experiments with changes in HCl emissions, and improvements are reported in accurately simulating ammonia, ammonium, and total ammonia.
Chaman Gul, Shichang Kang, Siva Praveen Puppala, Xiaokang Wu, Cenlin He, Yangyang Xu, Inka Koch, Sher Muhammad, Rajesh Kumar, and Getachew Dubache
Atmos. Chem. Phys., 22, 8725–8737, https://doi.org/10.5194/acp-22-8725-2022, https://doi.org/10.5194/acp-22-8725-2022, 2022
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This work aims to understand concentrations, spatial variability, and potential source regions of light-absorbing impurities (black carbon aerosols, dust particles, and organic carbon) in the surface snow of central and western Himalayan glaciers and their impact on snow albedo and radiative forcing.
Mathew Sebastian, Sobhan Kumar Kompalli, Vasudevan Anil Kumar, Sandhya Jose, S. Suresh Babu, Govindan Pandithurai, Sachchidanand Singh, Rakesh K. Hooda, Vijay K. Soni, Jeffrey R. Pierce, Ville Vakkari, Eija Asmi, Daniel M. Westervelt, Antti-Pekka Hyvärinen, and Vijay P. Kanawade
Atmos. Chem. Phys., 22, 4491–4508, https://doi.org/10.5194/acp-22-4491-2022, https://doi.org/10.5194/acp-22-4491-2022, 2022
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Xinxin Ye, Pargoal Arab, Ravan Ahmadov, Eric James, Georg A. Grell, Bradley Pierce, Aditya Kumar, Paul Makar, Jack Chen, Didier Davignon, Greg R. Carmichael, Gonzalo Ferrada, Jeff McQueen, Jianping Huang, Rajesh Kumar, Louisa Emmons, Farren L. Herron-Thorpe, Mark Parrington, Richard Engelen, Vincent-Henri Peuch, Arlindo da Silva, Amber Soja, Emily Gargulinski, Elizabeth Wiggins, Johnathan W. Hair, Marta Fenn, Taylor Shingler, Shobha Kondragunta, Alexei Lyapustin, Yujie Wang, Brent Holben, David M. Giles, and Pablo E. Saide
Atmos. Chem. Phys., 21, 14427–14469, https://doi.org/10.5194/acp-21-14427-2021, https://doi.org/10.5194/acp-21-14427-2021, 2021
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Wildfire smoke has crucial impacts on air quality, while uncertainties in the numerical forecasts remain significant. We present an evaluation of 12 real-time forecasting systems. Comparison of predicted smoke emissions suggests a large spread in magnitudes, with temporal patterns deviating from satellite detections. The performance for AOD and surface PM2.5 and their discrepancies highlighted the role of accurately represented spatiotemporal emission profiles in improving smoke forecasts.
Ernesto Reyes-Villegas, Upasana Panda, Eoghan Darbyshire, James M. Cash, Rutambhara Joshi, Ben Langford, Chiara F. Di Marco, Neil J. Mullinger, Mohammed S. Alam, Leigh R. Crilley, Daniel J. Rooney, W. Joe F. Acton, Will Drysdale, Eiko Nemitz, Michael Flynn, Aristeidis Voliotis, Gordon McFiggans, Hugh Coe, James Lee, C. Nicholas Hewitt, Mathew R. Heal, Sachin S. Gunthe, Tuhin K. Mandal, Bhola R. Gurjar, Shivani, Ranu Gadi, Siddhartha Singh, Vijay Soni, and James D. Allan
Atmos. Chem. Phys., 21, 11655–11667, https://doi.org/10.5194/acp-21-11655-2021, https://doi.org/10.5194/acp-21-11655-2021, 2021
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This paper shows the first multisite online measurements of PM1 in Delhi, India, with measurements over different seasons in Old Delhi and New Delhi in 2018. Organic aerosol (OA) source apportionment was performed using positive matrix factorisation (PMF). Traffic was the main primary aerosol source for both OAs and black carbon, seen with PMF and Aethalometer model analysis, indicating that control of primary traffic exhaust emissions would make a significant reduction to Delhi air pollution.
Pooja V. Pawar, Sachin D. Ghude, Chinmay Jena, Andrea Móring, Mark A. Sutton, Santosh Kulkarni, Deen Mani Lal, Divya Surendran, Martin Van Damme, Lieven Clarisse, Pierre-François Coheur, Xuejun Liu, Gaurav Govardhan, Wen Xu, Jize Jiang, and Tapan Kumar Adhya
Atmos. Chem. Phys., 21, 6389–6409, https://doi.org/10.5194/acp-21-6389-2021, https://doi.org/10.5194/acp-21-6389-2021, 2021
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In this study, simulations of atmospheric ammonia (NH3) with MOZART-4 and HTAP-v2 are compared with satellite (IASI) and ground-based measurements to understand the spatial and temporal variability of NH3 over two emission hotspot regions of Asia, the IGP and the NCP. Our simulations indicate that the formation of ammonium aerosols is quicker over the NCP than the IGP, leading to smaller NH3 columns over the higher NH3-emitting NCP compared to the IGP region for comparable emissions.
Fernando Chouza, Thierry Leblanc, Mark Brewer, Patrick Wang, Sabino Piazzolla, Gabriele Pfister, Rajesh Kumar, Carl Drews, Simone Tilmes, Louisa Emmons, and Matthew Johnson
Atmos. Chem. Phys., 21, 6129–6153, https://doi.org/10.5194/acp-21-6129-2021, https://doi.org/10.5194/acp-21-6129-2021, 2021
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The tropospheric ozone lidar at the JPL Table Mountain Facility (TMF) was used to investigate the impact of Los Angeles (LA) Basin pollution transport and stratospheric intrusions in the planetary boundary layer on the San Gabriel Mountains. The results of this study indicate a dominant role of the LA Basin pollution on days when high ozone levels were observed at TMF (March–October period).
Chinmay Jena, Sachin D. Ghude, Rachana Kulkarni, Sreyashi Debnath, Rajesh Kumar, Vijay Kumar Soni, Prodip Acharja, Santosh H. Kulkarni, Manoj Khare, Akshara J. Kaginalkar, Dilip M. Chate, Kaushar Ali, Ravi S. Nanjundiah, and Madhavan N. Rajeevan
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-673, https://doi.org/10.5194/acp-2020-673, 2020
Publication in ACP not foreseen
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Simulations of atmospheric particulate matter (PM2.5) with WRF-Chem model with three different aerosol mechanisms coupled with gas-phase chemical schemes are compared to understand the spatial and temporal variability of PM2.5 over the Indo-Gangetic Plain (IGP) in the winter season. All three chemical schemes underestimate the observed concentrations of major aerosol composition and precursor gases over IGP which in turn affect the optical depth and overall performance of the model for PM2.5.
Teruyuki Nakajima, Monica Campanelli, Huizheng Che, Victor Estellés, Hitoshi Irie, Sang-Woo Kim, Jhoon Kim, Dong Liu, Tomoaki Nishizawa, Govindan Pandithurai, Vijay Kumar Soni, Boossarasiri Thana, Nas-Urt Tugjsurn, Kazuma Aoki, Sujung Go, Makiko Hashimoto, Akiko Higurashi, Stelios Kazadzis, Pradeep Khatri, Natalia Kouremeti, Rei Kudo, Franco Marenco, Masahiro Momoi, Shantikumar S. Ningombam, Claire L. Ryder, Akihiro Uchiyama, and Akihiro Yamazaki
Atmos. Meas. Tech., 13, 4195–4218, https://doi.org/10.5194/amt-13-4195-2020, https://doi.org/10.5194/amt-13-4195-2020, 2020
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This paper overviews the progress in sky radiometer technology and the development of the network called SKYNET. It is found that the technology has produced useful on-site calibration methods, retrieval algorithms, and data analyses from sky radiometer observations of aerosol, cloud, water vapor, and ozone. The paper also discusses current issues of SKYNET to provide better information for the community.
Meng Gao, Jinhui Gao, Bin Zhu, Rajesh Kumar, Xiao Lu, Shaojie Song, Yuzhong Zhang, Beixi Jia, Peng Wang, Gufran Beig, Jianlin Hu, Qi Ying, Hongliang Zhang, Peter Sherman, and Michael B. McElroy
Atmos. Chem. Phys., 20, 4399–4414, https://doi.org/10.5194/acp-20-4399-2020, https://doi.org/10.5194/acp-20-4399-2020, 2020
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A regional fully coupled meteorology–chemistry model, Weather Research and Forecasting model with Chemistry (WRF-Chem), was employed to study the seasonality of ozone (O3) pollution and its sources in both China and India.
Suvarna Fadnavis, Rolf Müller, Gayatry Kalita, Matthew Rowlinson, Alexandru Rap, Jui-Lin Frank Li, Blaž Gasparini, and Anton Laakso
Atmos. Chem. Phys., 19, 9989–10008, https://doi.org/10.5194/acp-19-9989-2019, https://doi.org/10.5194/acp-19-9989-2019, 2019
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This paper highlights the impact of Asian anthropogenic emission changes in SO2 on sulfate loading in the Asian upper troposphere–lower stratosphere from a global chemistry–climate model and satellite remote sensing. Estimated seasonal mean direct radiative forcing at the top of the atmosphere induced by the increase in Indian SO2 is −0.2–−1.5 W m2 over India. Chinese SO2 emission reduction leads to a positive radiative forcing of ~0.6–6 W m2 over China. It will likely decrease Indian rainfall.
Zainab Q. Hakim, Scott Archer-Nicholls, Gufran Beig, Gerd A. Folberth, Kengo Sudo, Nathan Luke Abraham, Sachin Ghude, Daven K. Henze, and Alexander T. Archibald
Atmos. Chem. Phys., 19, 6437–6458, https://doi.org/10.5194/acp-19-6437-2019, https://doi.org/10.5194/acp-19-6437-2019, 2019
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Surface ozone is an important air pollutant and recent work has calculated that large numbers of people die prematurely because of exposure to high levels of surface ozone in India. However, these calculations require model simulations of ozone as key inputs.
Here we perform the most thorough evaluation of global model surface ozone over India to date. These analyses of model simulations and observations highlight some successes and shortcomings and the need for further process-based studies.
Marianne Tronstad Lund, Gunnar Myhre, Amund Søvde Haslerud, Ragnhild Bieltvedt Skeie, Jan Griesfeller, Stephen Matthew Platt, Rajesh Kumar, Cathrine Lund Myhre, and Michael Schulz
Geosci. Model Dev., 11, 4909–4931, https://doi.org/10.5194/gmd-11-4909-2018, https://doi.org/10.5194/gmd-11-4909-2018, 2018
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Atmospheric aerosols play a key role in the climate system, but their exact impact on the energy balance remains uncertain. Accurate representation of the geographical distribution and properties of aerosols in global models is key to reduce this uncertainty. Here we use a new emission inventory and a range of observations to carefully validate a state-of-the-art model and present an updated estimate of the net direct effect of anthropogenic aerosols since the preindustrial era.
Piyush Bhardwaj, Manish Naja, Maheswar Rupakheti, Aurelia Lupascu, Andrea Mues, Arnico Kumar Panday, Rajesh Kumar, Khadak Singh Mahata, Shyam Lal, Harish C. Chandola, and Mark G. Lawrence
Atmos. Chem. Phys., 18, 11949–11971, https://doi.org/10.5194/acp-18-11949-2018, https://doi.org/10.5194/acp-18-11949-2018, 2018
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This study provides information about the regional variabilities in some of the pollutants using observations in Nepal and India. It is shown that agricultural crop residue burning leads to a significant enhancement in ozone and CO over a wider region. Further, the wintertime higher ozone levels are shown to be largely due to local emissions, while regional transport could be important in spring and hence shows the role of regional sources versus local sources in the Kathmandu Valley.
Matthieu Pommier, Hilde Fagerli, Michael Gauss, David Simpson, Sumit Sharma, Vinay Sinha, Sachin D. Ghude, Oskar Landgren, Agnes Nyiri, and Peter Wind
Atmos. Chem. Phys., 18, 103–127, https://doi.org/10.5194/acp-18-103-2018, https://doi.org/10.5194/acp-18-103-2018, 2018
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India has to cope with a poor air quality, and this work shows a predicted increase in pollution (O3 & PM2.5) if no further policy efforts are made in the future. Climate change will modify the soil moisture leading to changes in O3. Changes in PM2.5 are related to changes in precipitation, biogenic emissions and wind speed. It is also shown that in the 2050s, the secondary inorganic aerosols will become the main component of PM2.5 over India related to the increase in anthropogenic emissions.
Youhua Tang, Mariusz Pagowski, Tianfeng Chai, Li Pan, Pius Lee, Barry Baker, Rajesh Kumar, Luca Delle Monache, Daniel Tong, and Hyun-Cheol Kim
Geosci. Model Dev., 10, 4743–4758, https://doi.org/10.5194/gmd-10-4743-2017, https://doi.org/10.5194/gmd-10-4743-2017, 2017
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In order to evaluate the data assimilation tools for regional real-time PM2.5 forecasts, we applied a 3D-Var assimilation tool to adjust the aerosol initial condition by assimilating satellite-retrieved aerosol optical depth and surface PM2.5 observations for a regional air quality model, which is compared to another assimilation method, optimal interpolation. We discuss the pros and cons of these two assimilation methods based on the comparison of their 1-month four-cycles-per-day runs.
Suvarna Fadnavis, Gayatry Kalita, K. Ravi Kumar, Blaž Gasparini, and Jui-Lin Frank Li
Atmos. Chem. Phys., 17, 11637–11654, https://doi.org/10.5194/acp-17-11637-2017, https://doi.org/10.5194/acp-17-11637-2017, 2017
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In this study, the model simulations show that monsoon convection over the Bay of Bengal, the South China Sea and southern flanks of the Himalayas transports Asian carbonaceous aerosol into the UTLS. Carbonaceous aerosol induces enhancement in heating rate, vertical velocity and water vapor transport in the UTLS. Doubling of carbonaceous aerosols creates an anomalous warming over the TP. It generates monsoon Hadley circulation and thus increases precipitation over India and northeast China.
Sarah Safieddine, Anne Boynard, Nan Hao, Fuxiang Huang, Lili Wang, Dongsheng Ji, Brice Barret, Sachin D. Ghude, Pierre-François Coheur, Daniel Hurtmans, and Cathy Clerbaux
Atmos. Chem. Phys., 16, 10489–10500, https://doi.org/10.5194/acp-16-10489-2016, https://doi.org/10.5194/acp-16-10489-2016, 2016
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The Asian Summer Monsoon has implication on the weather and climate system as well as pollutants concentration over the monsoon regions leading to effects on the global air quality. Our results, combining satellite, aircraft and ground station data, show that tropospheric ozone, decrease during the period May–August over East and South Asia due to the Monsoon. The magnitude of this drop depends largely on meteorology and geographic location.
R. Kumar, M. C. Barth, V. S. Nair, G. G. Pfister, S. Suresh Babu, S. K. Satheesh, K. Krishna Moorthy, G. R. Carmichael, Z. Lu, and D. G. Streets
Atmos. Chem. Phys., 15, 5415–5428, https://doi.org/10.5194/acp-15-5415-2015, https://doi.org/10.5194/acp-15-5415-2015, 2015
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We examine differences in the surface BC between the Bay of Bengal (BoB) and the Arabian Sea (AS) and identify dominant sources of BC in South Asia during ICARB. Anthropogenic emissions were the main source of BC during ICARB and had about 5 times stronger influence on the BoB compared to the AS. Regional-scale transport contributes up to 25% of BC mass concentrations in western and eastern India, suggesting that surface BC mass concentrations cannot be linked directly to the local emissions.
S. Fadnavis, M. G. Schultz, K. Semeniuk, A. S. Mahajan, L. Pozzoli, S. Sonbawne, S. D. Ghude, M. Kiefer, and E. Eckert
Atmos. Chem. Phys., 14, 12725–12743, https://doi.org/10.5194/acp-14-12725-2014, https://doi.org/10.5194/acp-14-12725-2014, 2014
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The Asian summer monsoon transports pollutants from local emission sources to the upper troposphere and lower stratosphere (UTLS). The increasing trend of these pollutants may have climatic impact. This study addresses the impact of convectively lifted Indian and Chinese emissions on the ULTS. Sensitivity experiments with emission changes in particular regions show that Chinese emissions have a greater impact on the concentrations of NOY species than Indian emissions.
R. Kumar, M. C. Barth, S. Madronich, M. Naja, G. R. Carmichael, G. G. Pfister, C. Knote, G. P. Brasseur, N. Ojha, and T. Sarangi
Atmos. Chem. Phys., 14, 6813–6834, https://doi.org/10.5194/acp-14-6813-2014, https://doi.org/10.5194/acp-14-6813-2014, 2014
R. Kumar, M. C. Barth, G. G. Pfister, M. Naja, and G. P. Brasseur
Atmos. Chem. Phys., 14, 2431–2446, https://doi.org/10.5194/acp-14-2431-2014, https://doi.org/10.5194/acp-14-2431-2014, 2014
Related subject area
Atmospheric sciences
Modeling of polycyclic aromatic hydrocarbons (PAHs) from global to regional scales: model development (IAP-AACM_PAH v1.0) and investigation of health risks in 2013 and 2018 in China
LIMA (v2.0): A full two-moment cloud microphysical scheme for the mesoscale non-hydrostatic model Meso-NH v5-6
SLUCM+BEM (v1.0): a simple parameterisation for dynamic anthropogenic heat and electricity consumption in WRF-Urban (v4.3.2)
NAQPMS-PDAF v2.0: a novel hybrid nonlinear data assimilation system for improved simulation of PM2.5 chemical components
Source-specific bias correction of US background and anthropogenic ozone modeled in CMAQ
Observational operator for fair model evaluation with ground NO2 measurements
Valid time shifting ensemble Kalman filter (VTS-EnKF) for dust storm forecasting
An updated parameterization of the unstable atmospheric surface layer in the Weather Research and Forecasting (WRF) modeling system
The impact of cloud microphysics and ice nucleation on Southern Ocean clouds assessed with single-column modeling and instrument simulators
An updated aerosol simulation in the Community Earth System Model (v2.1.3): dust and marine aerosol emissions and secondary organic aerosol formation
Exploring ship track spreading rates with a physics-informed Langevin particle parameterization
Do data-driven models beat numerical models in forecasting weather extremes? A comparison of IFS HRES, Pangu-Weather, and GraphCast
Development of the MPAS-CMAQ coupled system (V1.0) for multiscale global air quality modeling
Assessment of object-based indices to identify convective organization
The Global Forest Fire Emissions Prediction System version 1.0
NEIVAv1.0: Next-generation Emissions InVentory expansion of Akagi et al. (2011) version 1.0
FLEXPART version 11: improved accuracy, efficiency, and flexibility
Challenges of high-fidelity air quality modeling in urban environments – PALM sensitivity study during stable conditions
Air quality modeling intercomparison and multiscale ensemble chain for Latin America
Recommended coupling to global meteorological fields for long-term tracer simulations with WRF-GHG
Selecting CMIP6 global climate models (GCMs) for Coordinated Regional Climate Downscaling Experiment (CORDEX) dynamical downscaling over Southeast Asia using a standardised benchmarking framework
Improved definition of prior uncertainties in CO2 and CO fossil fuel fluxes and its impact on multi-species inversion with GEOS-Chem (v12.5)
RASCAL v1.0: an open-source tool for climatological time series reconstruction and extension
Introducing graupel density prediction in Weather Research and Forecasting (WRF) double-moment 6-class (WDM6) microphysics and evaluation of the modified scheme during the ICE-POP field campaign
Enabling high-performance cloud computing for the Community Multiscale Air Quality Model (CMAQ) version 5.3.3: performance evaluation and benefits for the user community
Atmospheric-river-induced precipitation in California as simulated by the regionally refined Simple Convective Resolving E3SM Atmosphere Model (SCREAM) Version 0
Recent improvements and maximum covariance analysis of aerosol and cloud properties in the EC-Earth3-AerChem model
GPU-HADVPPM4HIP V1.0: using the heterogeneous-compute interface for portability (HIP) to speed up the piecewise parabolic method in the CAMx (v6.10) air quality model on China's domestic GPU-like accelerator
Preliminary evaluation of the effect of electro-coalescence with conducting sphere approximation on the formation of warm cumulus clouds using SCALE-SDM version 0.2.5–2.3.0
Exploring the footprint representation of microwave radiance observations in an Arctic limited-area data assimilation system
Orbital-Radar v1.0.0: A tool to transform suborbital radar observations to synthetic EarthCARE cloud radar data
Analysis of model error in forecast errors of extended atmospheric Lorenz 05 systems and the ECMWF system
Description and validation of Vehicular Emissions from Road Traffic (VERT) 1.0, an R-based framework for estimating road transport emissions from traffic flows
AeroMix v1.0.1: a Python package for modeling aerosol optical properties and mixing states
Impact of ITCZ width on global climate: ITCZ-MIP
Deep-learning-driven simulations of boundary layer clouds over the Southern Great Plains
Mixed-precision computing in the GRIST dynamical core for weather and climate modelling
A conservative immersed boundary method for the multi-physics urban large-eddy simulation model uDALES v2.0
Accurate space-based NOx emission estimates with the flux divergence approach require fine-scale model information on local oxidation chemistry and profile shapes
RCEMIP-II: mock-Walker simulations as phase II of the radiative–convective equilibrium model intercomparison project
The MESSy DWARF (based on MESSy v2.55.2)
Objective identification of meteorological fronts and climatologies from ERA-Interim and ERA5
TAMS: a tracking, classifying, and variable-assigning algorithm for mesoscale convective systems in simulated and satellite-derived datasets
Development of the adjoint of the unified tropospheric–stratospheric chemistry extension (UCX) in GEOS-Chem adjoint v36
New explicit formulae for the settling speed of prolate spheroids in the atmosphere: theoretical background and implementation in AerSett v2.0.2
ZJU-AERO V0.5: an Accurate and Efficient Radar Operator designed for CMA-GFS/MESO with the capability to simulate non-spherical hydrometeors
The Year of Polar Prediction site Model Intercomparison Project (YOPPsiteMIP) phase 1: project overview and Arctic winter forecast evaluation
Evaluating CHASER V4.0 global formaldehyde (HCHO) simulations using satellite, aircraft, and ground-based remote-sensing observations
Global variable-resolution simulations of extreme precipitation over Henan, China, in 2021 with MPAS-Atmosphere v7.3
The CHIMERE chemistry-transport model v2023r1
Zichen Wu, Xueshun Chen, Zifa Wang, Huansheng Chen, Zhe Wang, Qing Mu, Lin Wu, Wending Wang, Xiao Tang, Jie Li, Ying Li, Qizhong Wu, Yang Wang, Zhiyin Zou, and Zijian Jiang
Geosci. Model Dev., 17, 8885–8907, https://doi.org/10.5194/gmd-17-8885-2024, https://doi.org/10.5194/gmd-17-8885-2024, 2024
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We developed a model to simulate polycyclic aromatic hydrocarbons (PAHs) from global to regional scales. The model can reproduce PAH distribution well. The concentration of BaP (indicator species for PAHs) could exceed the target values of 1 ng m-3 over some areas (e.g., in central Europe, India, and eastern China). The change in BaP is lower than that in PM2.5 from 2013 to 2018. China still faces significant potential health risks posed by BaP although the Action Plan has been implemented.
Marie Taufour, Jean-Pierre Pinty, Christelle Barthe, Benoît Vié, and Chien Wang
Geosci. Model Dev., 17, 8773–8798, https://doi.org/10.5194/gmd-17-8773-2024, https://doi.org/10.5194/gmd-17-8773-2024, 2024
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We have developed a complete two-moment version of the LIMA (Liquid Ice Multiple Aerosols) microphysics scheme. We have focused on collection processes, where the hydrometeor number transfer is often estimated in proportion to the mass transfer. The impact of these parameterizations on a convective system and the prospects for more realistic estimates of secondary parameters (reflectivity, hydrometeor size) are shown in a first test on an idealized case.
Yuya Takane, Yukihiro Kikegawa, Ko Nakajima, and Hiroyuki Kusaka
Geosci. Model Dev., 17, 8639–8664, https://doi.org/10.5194/gmd-17-8639-2024, https://doi.org/10.5194/gmd-17-8639-2024, 2024
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A new parameterisation for dynamic anthropogenic heat and electricity consumption is described. The model reproduced the temporal variation in and spatial distributions of electricity consumption and temperature well in summer and winter. The partial air conditioning was the most critical factor, significantly affecting the value of anthropogenic heat emission.
Hongyi Li, Ting Yang, Lars Nerger, Dawei Zhang, Di Zhang, Guigang Tang, Haibo Wang, Yele Sun, Pingqing Fu, Hang Su, and Zifa Wang
Geosci. Model Dev., 17, 8495–8519, https://doi.org/10.5194/gmd-17-8495-2024, https://doi.org/10.5194/gmd-17-8495-2024, 2024
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To accurately characterize the spatiotemporal distribution of particulate matter <2.5 µm chemical components, we developed the Nested Air Quality Prediction Model System with the Parallel Data Assimilation Framework (NAQPMS-PDAF) v2.0 for chemical components with non-Gaussian and nonlinear properties. NAQPMS-PDAF v2.0 has better computing efficiency, excels when used with a small ensemble size, and can significantly improve the simulation performance of chemical components.
T. Nash Skipper, Christian Hogrefe, Barron H. Henderson, Rohit Mathur, Kristen M. Foley, and Armistead G. Russell
Geosci. Model Dev., 17, 8373–8397, https://doi.org/10.5194/gmd-17-8373-2024, https://doi.org/10.5194/gmd-17-8373-2024, 2024
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Chemical transport model simulations are combined with ozone observations to estimate the bias in ozone attributable to US anthropogenic sources and individual sources of US background ozone: natural sources, non-US anthropogenic sources, and stratospheric ozone. Results indicate a positive bias correlated with US anthropogenic emissions during summer in the eastern US and a negative bias correlated with stratospheric ozone during spring.
Li Fang, Jianbing Jin, Arjo Segers, Ke Li, Ji Xia, Wei Han, Baojie Li, Hai Xiang Lin, Lei Zhu, Song Liu, and Hong Liao
Geosci. Model Dev., 17, 8267–8282, https://doi.org/10.5194/gmd-17-8267-2024, https://doi.org/10.5194/gmd-17-8267-2024, 2024
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Model evaluations against ground observations are usually unfair. The former simulates mean status over coarse grids and the latter the surrounding atmosphere. To solve this, we proposed the new land-use-based representative (LUBR) operator that considers intra-grid variance. The LUBR operator is validated to provide insights that align with satellite measurements. The results highlight the importance of considering fine-scale urban–rural differences when comparing models and observation.
Mijie Pang, Jianbing Jin, Arjo Segers, Huiya Jiang, Wei Han, Batjargal Buyantogtokh, Ji Xia, Li Fang, Jiandong Li, Hai Xiang Lin, and Hong Liao
Geosci. Model Dev., 17, 8223–8242, https://doi.org/10.5194/gmd-17-8223-2024, https://doi.org/10.5194/gmd-17-8223-2024, 2024
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The ensemble Kalman filter (EnKF) improves dust storm forecasts but faces challenges with position errors. The valid time shifting EnKF (VTS-EnKF) addresses this by adjusting for position errors, enhancing accuracy in forecasting dust storms, as proven in tests on 2021 events, even with smaller ensembles and time intervals.
Prabhakar Namdev, Maithili Sharan, Piyush Srivastava, and Saroj Kanta Mishra
Geosci. Model Dev., 17, 8093–8114, https://doi.org/10.5194/gmd-17-8093-2024, https://doi.org/10.5194/gmd-17-8093-2024, 2024
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Inadequate representation of surface–atmosphere interaction processes is a major source of uncertainty in numerical weather prediction models. Here, an effort has been made to improve the Weather Research and Forecasting (WRF) model version 4.2.2 by introducing a unique theoretical framework under convective conditions. In addition, to enhance the potential applicability of the WRF modeling system, various commonly used similarity functions under convective conditions have also been installed.
Andrew Gettelman, Richard Forbes, Roger Marchand, Chih-Chieh Chen, and Mark Fielding
Geosci. Model Dev., 17, 8069–8092, https://doi.org/10.5194/gmd-17-8069-2024, https://doi.org/10.5194/gmd-17-8069-2024, 2024
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Supercooled liquid clouds (liquid clouds colder than 0°C) are common at higher latitudes (especially over the Southern Ocean) and are critical for constraining climate projections. We compare a single-column version of a weather model to observations with two different cloud schemes and find that both the dynamical environment and atmospheric aerosols are important for reproducing observations.
Yujuan Wang, Peng Zhang, Jie Li, Yaman Liu, Yanxu Zhang, Jiawei Li, and Zhiwei Han
Geosci. Model Dev., 17, 7995–8021, https://doi.org/10.5194/gmd-17-7995-2024, https://doi.org/10.5194/gmd-17-7995-2024, 2024
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This study updates the CESM's aerosol schemes, focusing on dust, marine aerosol emissions, and secondary organic aerosol (SOA) . Dust emission modifications make deflation areas more continuous, improving results in North America and the sub-Arctic. Humidity correction to sea-salt emissions has a minor effect. Introducing marine organic aerosol emissions, coupled with ocean biogeochemical processes, and adding aqueous reactions for SOA formation advance the CESM's aerosol modelling results.
Lucas A. McMichael, Michael J. Schmidt, Robert Wood, Peter N. Blossey, and Lekha Patel
Geosci. Model Dev., 17, 7867–7888, https://doi.org/10.5194/gmd-17-7867-2024, https://doi.org/10.5194/gmd-17-7867-2024, 2024
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Marine cloud brightening (MCB) is a climate intervention technique to potentially cool the climate. Climate models used to gauge regional climate impacts associated with MCB often assume large areas of the ocean are uniformly perturbed. However, a more realistic representation of MCB application would require information about how an injected particle plume spreads. This work aims to develop such a plume-spreading model.
Leonardo Olivetti and Gabriele Messori
Geosci. Model Dev., 17, 7915–7962, https://doi.org/10.5194/gmd-17-7915-2024, https://doi.org/10.5194/gmd-17-7915-2024, 2024
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Data-driven models are becoming a viable alternative to physics-based models for weather forecasting up to 15 d into the future. However, it is unclear whether they are as reliable as physics-based models when forecasting weather extremes. We evaluate their performance in forecasting near-surface cold, hot, and windy extremes globally. We find that data-driven models can compete with physics-based models and that the choice of the best model mainly depends on the region and type of extreme.
David C. Wong, Jeff Willison, Jonathan E. Pleim, Golam Sarwar, James Beidler, Russ Bullock, Jerold A. Herwehe, Rob Gilliam, Daiwen Kang, Christian Hogrefe, George Pouliot, and Hosein Foroutan
Geosci. Model Dev., 17, 7855–7866, https://doi.org/10.5194/gmd-17-7855-2024, https://doi.org/10.5194/gmd-17-7855-2024, 2024
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This work describe how we linked the meteorological Model for Prediction Across Scales – Atmosphere (MPAS-A) with the Community Multiscale Air Quality (CMAQ) air quality model to form a coupled modelling system. This could be used to study air quality or climate and air quality interaction at a global scale. This new model scales well in high-performance computing environments and performs well with respect to ground surface networks in terms of ozone and PM2.5.
Giulio Mandorli and Claudia J. Stubenrauch
Geosci. Model Dev., 17, 7795–7813, https://doi.org/10.5194/gmd-17-7795-2024, https://doi.org/10.5194/gmd-17-7795-2024, 2024
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In recent years, several studies focused their attention on the disposition of convection. Lots of methods, called indices, have been developed to quantify the amount of convection clustering. These indices are evaluated in this study by defining criteria that must be satisfied and then evaluating the indices against these standards. None of the indices meet all criteria, with some only partially meeting them.
Kerry Anderson, Jack Chen, Peter Englefield, Debora Griffin, Paul A. Makar, and Dan Thompson
Geosci. Model Dev., 17, 7713–7749, https://doi.org/10.5194/gmd-17-7713-2024, https://doi.org/10.5194/gmd-17-7713-2024, 2024
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The Global Forest Fire Emissions Prediction System (GFFEPS) is a model that predicts smoke and carbon emissions from wildland fires. The model calculates emissions from the ground up based on satellite-detected fires, modelled weather and fire characteristics. Unlike other global models, GFFEPS uses daily weather conditions to capture changing burning conditions on a day-to-day basis. GFFEPS produced lower carbon emissions due to the changing weather not captured by the other models.
Samiha Binte Shahid, Forrest G. Lacey, Christine Wiedinmyer, Robert J. Yokelson, and Kelley C. Barsanti
Geosci. Model Dev., 17, 7679–7711, https://doi.org/10.5194/gmd-17-7679-2024, https://doi.org/10.5194/gmd-17-7679-2024, 2024
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The Next-generation Emissions InVentory expansion of Akagi (NEIVA) v.1.0 is a comprehensive biomass burning emissions database that allows integration of new data and flexible querying. Data are stored in connected datasets, including recommended averages of ~1500 constituents for 14 globally relevant fire types. Individual compounds were mapped to common model species to allow better attribution of emissions in modeling studies that predict the effects of fires on air quality and climate.
Lucie Bakels, Daria Tatsii, Anne Tipka, Rona Thompson, Marina Dütsch, Michael Blaschek, Petra Seibert, Katharina Baier, Silvia Bucci, Massimo Cassiani, Sabine Eckhardt, Christine Groot Zwaaftink, Stephan Henne, Pirmin Kaufmann, Vincent Lechner, Christian Maurer, Marie D. Mulder, Ignacio Pisso, Andreas Plach, Rakesh Subramanian, Martin Vojta, and Andreas Stohl
Geosci. Model Dev., 17, 7595–7627, https://doi.org/10.5194/gmd-17-7595-2024, https://doi.org/10.5194/gmd-17-7595-2024, 2024
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Computer models are essential for improving our understanding of how gases and particles move in the atmosphere. We present an update of the atmospheric transport model FLEXPART. FLEXPART 11 is more accurate due to a reduced number of interpolations and a new scheme for wet deposition. It can simulate non-spherical aerosols and includes linear chemical reactions. It is parallelised using OpenMP and includes new user options. A new user manual details how to use FLEXPART 11.
Jaroslav Resler, Petra Bauerová, Michal Belda, Martin Bureš, Kryštof Eben, Vladimír Fuka, Jan Geletič, Radek Jareš, Jan Karel, Josef Keder, Pavel Krč, William Patiño, Jelena Radović, Hynek Řezníček, Matthias Sühring, Adriana Šindelářová, and Ondřej Vlček
Geosci. Model Dev., 17, 7513–7537, https://doi.org/10.5194/gmd-17-7513-2024, https://doi.org/10.5194/gmd-17-7513-2024, 2024
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Detailed modeling of urban air quality in stable conditions is a challenge. We show the unprecedented sensitivity of a large eddy simulation (LES) model to meteorological boundary conditions and model parameters in an urban environment under stable conditions. We demonstrate the crucial role of boundary conditions for the comparability of results with observations. The study reveals a strong sensitivity of the results to model parameters and model numerical instabilities during such conditions.
Jorge E. Pachón, Mariel A. Opazo, Pablo Lichtig, Nicolas Huneeus, Idir Bouarar, Guy Brasseur, Cathy W. Y. Li, Johannes Flemming, Laurent Menut, Camilo Menares, Laura Gallardo, Michael Gauss, Mikhail Sofiev, Rostislav Kouznetsov, Julia Palamarchuk, Andreas Uppstu, Laura Dawidowski, Nestor Y. Rojas, María de Fátima Andrade, Mario E. Gavidia-Calderón, Alejandro H. Delgado Peralta, and Daniel Schuch
Geosci. Model Dev., 17, 7467–7512, https://doi.org/10.5194/gmd-17-7467-2024, https://doi.org/10.5194/gmd-17-7467-2024, 2024
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Latin America (LAC) has some of the most populated urban areas in the world, with high levels of air pollution. Air quality management in LAC has been traditionally focused on surveillance and building emission inventories. This study performed the first intercomparison and model evaluation in LAC, with interesting and insightful findings for the region. A multiscale modeling ensemble chain was assembled as a first step towards an air quality forecasting system.
David Ho, Michał Gałkowski, Friedemann Reum, Santiago Botía, Julia Marshall, Kai Uwe Totsche, and Christoph Gerbig
Geosci. Model Dev., 17, 7401–7422, https://doi.org/10.5194/gmd-17-7401-2024, https://doi.org/10.5194/gmd-17-7401-2024, 2024
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Atmospheric model users often overlook the impact of the land–atmosphere interaction. This study accessed various setups of WRF-GHG simulations that ensure consistency between the model and driving reanalysis fields. We found that a combination of nudging and frequent re-initialization allows certain improvement by constraining the soil moisture fields and, through its impact on atmospheric mixing, improves atmospheric transport.
Phuong Loan Nguyen, Lisa V. Alexander, Marcus J. Thatcher, Son C. H. Truong, Rachael N. Isphording, and John L. McGregor
Geosci. Model Dev., 17, 7285–7315, https://doi.org/10.5194/gmd-17-7285-2024, https://doi.org/10.5194/gmd-17-7285-2024, 2024
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We use a comprehensive approach to select a subset of CMIP6 models for dynamical downscaling over Southeast Asia, taking into account model performance, model independence, data availability and the range of future climate projections. The standardised benchmarking framework is applied to assess model performance through both statistical and process-based metrics. Ultimately, we identify two independent model groups that are suitable for dynamical downscaling in the Southeast Asian region.
Ingrid Super, Tia Scarpelli, Arjan Droste, and Paul I. Palmer
Geosci. Model Dev., 17, 7263–7284, https://doi.org/10.5194/gmd-17-7263-2024, https://doi.org/10.5194/gmd-17-7263-2024, 2024
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Monitoring greenhouse gas emission reductions requires a combination of models and observations, as well as an initial emission estimate. Each component provides information with a certain level of certainty and is weighted to yield the most reliable estimate of actual emissions. We describe efforts for estimating the uncertainty in the initial emission estimate, which significantly impacts the outcome. Hence, a good uncertainty estimate is key for obtaining reliable information on emissions.
Álvaro González-Cervera and Luis Durán
Geosci. Model Dev., 17, 7245–7261, https://doi.org/10.5194/gmd-17-7245-2024, https://doi.org/10.5194/gmd-17-7245-2024, 2024
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RASCAL is an open-source Python tool designed for reconstructing daily climate observations, especially in regions with complex local phenomena. It merges large-scale weather patterns with local weather using the analog method. Evaluations in central Spain show that RASCAL outperforms ERA20C reanalysis in reconstructing precipitation and temperature. RASCAL offers opportunities for broad scientific applications, from short-term forecasts to local-scale climate change scenarios.
Sun-Young Park, Kyo-Sun Sunny Lim, Kwonil Kim, Gyuwon Lee, and Jason A. Milbrandt
Geosci. Model Dev., 17, 7199–7218, https://doi.org/10.5194/gmd-17-7199-2024, https://doi.org/10.5194/gmd-17-7199-2024, 2024
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We enhance the WDM6 scheme by incorporating predicted graupel density. The modification affects graupel characteristics, including fall velocity–diameter and mass–diameter relationships. Simulations highlight changes in graupel distribution and precipitation patterns, potentially influencing surface snow amounts. The study underscores the significance of integrating predicted graupel density for a more realistic portrayal of microphysical properties in weather models.
Christos I. Efstathiou, Elizabeth Adams, Carlie J. Coats, Robert Zelt, Mark Reed, John McGee, Kristen M. Foley, Fahim I. Sidi, David C. Wong, Steven Fine, and Saravanan Arunachalam
Geosci. Model Dev., 17, 7001–7027, https://doi.org/10.5194/gmd-17-7001-2024, https://doi.org/10.5194/gmd-17-7001-2024, 2024
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We present a summary of enabling high-performance computing of the Community Multiscale Air Quality Model (CMAQ) – a state-of-the-science community multiscale air quality model – on two cloud computing platforms through documenting the technologies, model performance, scaling and relative merits. This may be a new paradigm for computationally intense future model applications. We initiated this work due to a need to leverage cloud computing advances and to ease the learning curve for new users.
Peter A. Bogenschutz, Jishi Zhang, Qi Tang, and Philip Cameron-Smith
Geosci. Model Dev., 17, 7029–7050, https://doi.org/10.5194/gmd-17-7029-2024, https://doi.org/10.5194/gmd-17-7029-2024, 2024
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Using high-resolution and state-of-the-art modeling techniques we simulate five atmospheric river events for California to test the capability to represent precipitation for these events. We find that our model is able to capture the distribution of precipitation very well but suffers from overestimating the precipitation amounts over high elevation. Increasing the resolution further has no impact on reducing this bias, while increasing the domain size does have modest impacts.
Manu Anna Thomas, Klaus Wyser, Shiyu Wang, Marios Chatziparaschos, Paraskevi Georgakaki, Montserrat Costa-Surós, Maria Gonçalves Ageitos, Maria Kanakidou, Carlos Pérez García-Pando, Athanasios Nenes, Twan van Noije, Philippe Le Sager, and Abhay Devasthale
Geosci. Model Dev., 17, 6903–6927, https://doi.org/10.5194/gmd-17-6903-2024, https://doi.org/10.5194/gmd-17-6903-2024, 2024
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Aerosol–cloud interactions occur at a range of spatio-temporal scales. While evaluating recent developments in EC-Earth3-AerChem, this study aims to understand the extent to which the Twomey effect manifests itself at larger scales. We find a reduction in the warm bias over the Southern Ocean due to model improvements. While we see footprints of the Twomey effect at larger scales, the negative relationship between cloud droplet number and liquid water drives the shortwave radiative effect.
Kai Cao, Qizhong Wu, Lingling Wang, Hengliang Guo, Nan Wang, Huaqiong Cheng, Xiao Tang, Dongxing Li, Lina Liu, Dongqing Li, Hao Wu, and Lanning Wang
Geosci. Model Dev., 17, 6887–6901, https://doi.org/10.5194/gmd-17-6887-2024, https://doi.org/10.5194/gmd-17-6887-2024, 2024
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AMD’s heterogeneous-compute interface for portability was implemented to port the piecewise parabolic method solver from NVIDIA GPUs to China's GPU-like accelerators. The results show that the larger the model scale, the more acceleration effect on the GPU-like accelerator, up to 28.9 times. The multi-level parallelism achieves a speedup of 32.7 times on the heterogeneous cluster. By comparing the results, the GPU-like accelerators have more accuracy for the geoscience numerical models.
Ruyi Zhang, Limin Zhou, Shin-ichiro Shima, and Huawei Yang
Geosci. Model Dev., 17, 6761–6774, https://doi.org/10.5194/gmd-17-6761-2024, https://doi.org/10.5194/gmd-17-6761-2024, 2024
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Solar activity weakly ionises Earth's atmosphere, charging cloud droplets. Electro-coalescence is when oppositely charged droplets stick together. We introduce an analytical expression of electro-coalescence probability and use it in a warm-cumulus-cloud simulation. Results show that charge cases increase rain and droplet size, with the new method outperforming older ones. The new method requires longer computation time, but its impact on rain justifies inclusion in meteorology models.
Máté Mile, Stephanie Guedj, and Roger Randriamampianina
Geosci. Model Dev., 17, 6571–6587, https://doi.org/10.5194/gmd-17-6571-2024, https://doi.org/10.5194/gmd-17-6571-2024, 2024
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Satellite observations provide crucial information about atmospheric constituents in a global distribution that helps to better predict the weather over sparsely observed regions like the Arctic. However, the use of satellite data is usually conservative and imperfect. In this study, a better spatial representation of satellite observations is discussed and explored by a so-called footprint function or operator, highlighting its added value through a case study and diagnostics.
Lukas Pfitzenmaier, Pavlos Kollias, Nils Risse, Imke Schirmacher, Bernat Puigdomenech Treserras, and Katia Lamer
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-129, https://doi.org/10.5194/gmd-2024-129, 2024
Revised manuscript accepted for GMD
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Orbital-radar is a Python tool transferring sub-orbital radar data (ground-based, airborne, and forward-simulated NWP) into synthetical space-borne cloud profiling radar data mimicking the platform characteristics, e.g. EarthCARE or CloudSat CPR. The novelty of orbital-radar is the simulation platform characteristic noise floors and errors. By this long time data sets can be transformed into synthetic observations for Cal/Valor sensitivity studies for new or future satellite missions.
Hynek Bednář and Holger Kantz
Geosci. Model Dev., 17, 6489–6511, https://doi.org/10.5194/gmd-17-6489-2024, https://doi.org/10.5194/gmd-17-6489-2024, 2024
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The forecast error growth of atmospheric phenomena is caused by initial and model errors. When studying the initial error growth, it may turn out that small-scale phenomena, which contribute little to the forecast product, significantly affect the ability to predict this product. With a negative result, we investigate in the extended Lorenz (2005) system whether omitting these phenomena will improve predictability. A theory explaining and describing this behavior is developed.
Giorgio Veratti, Alessandro Bigi, Sergio Teggi, and Grazia Ghermandi
Geosci. Model Dev., 17, 6465–6487, https://doi.org/10.5194/gmd-17-6465-2024, https://doi.org/10.5194/gmd-17-6465-2024, 2024
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In this study, we present VERT (Vehicular Emissions from Road Traffic), an R package designed to estimate transport emissions using traffic estimates and vehicle fleet composition data. Compared to other tools available in the literature, VERT stands out for its user-friendly configuration and flexibility of user input. Case studies demonstrate its accuracy in both urban and regional contexts, making it a valuable tool for air quality management and transport scenario planning.
Sam P. Raj, Puna Ram Sinha, Rohit Srivastava, Srinivas Bikkina, and Damu Bala Subrahamanyam
Geosci. Model Dev., 17, 6379–6399, https://doi.org/10.5194/gmd-17-6379-2024, https://doi.org/10.5194/gmd-17-6379-2024, 2024
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A Python successor to the aerosol module of the OPAC model, named AeroMix, has been developed, with enhanced capabilities to better represent real atmospheric aerosol mixing scenarios. AeroMix’s performance in modeling aerosol mixing states has been evaluated against field measurements, substantiating its potential as a versatile aerosol optical model framework for next-generation algorithms to infer aerosol mixing states and chemical composition.
Angeline G. Pendergrass, Michael P. Byrne, Oliver Watt-Meyer, Penelope Maher, and Mark J. Webb
Geosci. Model Dev., 17, 6365–6378, https://doi.org/10.5194/gmd-17-6365-2024, https://doi.org/10.5194/gmd-17-6365-2024, 2024
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The width of the tropical rain belt affects many aspects of our climate, yet we do not understand what controls it. To better understand it, we present a method to change it in numerical model experiments. We show that the method works well in four different models. The behavior of the width is unexpectedly simple in some ways, such as how strong the winds are as it changes, but in other ways, it is more complicated, especially how temperature increases with carbon dioxide.
Tianning Su and Yunyan Zhang
Geosci. Model Dev., 17, 6319–6336, https://doi.org/10.5194/gmd-17-6319-2024, https://doi.org/10.5194/gmd-17-6319-2024, 2024
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Using 2 decades of field observations over the Southern Great Plains, this study developed a deep-learning model to simulate the complex dynamics of boundary layer clouds. The deep-learning model can serve as the cloud parameterization within reanalysis frameworks, offering insights into improving the simulation of low clouds. By quantifying biases due to various meteorological factors and parameterizations, this deep-learning-driven approach helps bridge the observation–modeling divide.
Siyuan Chen, Yi Zhang, Yiming Wang, Zhuang Liu, Xiaohan Li, and Wei Xue
Geosci. Model Dev., 17, 6301–6318, https://doi.org/10.5194/gmd-17-6301-2024, https://doi.org/10.5194/gmd-17-6301-2024, 2024
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This study explores strategies and techniques for implementing mixed-precision code optimization within an atmosphere model dynamical core. The coded equation terms in the governing equations that are sensitive (or insensitive) to the precision level have been identified. The performance of mixed-precision computing in weather and climate simulations was analyzed.
Sam O. Owens, Dipanjan Majumdar, Chris E. Wilson, Paul Bartholomew, and Maarten van Reeuwijk
Geosci. Model Dev., 17, 6277–6300, https://doi.org/10.5194/gmd-17-6277-2024, https://doi.org/10.5194/gmd-17-6277-2024, 2024
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Designing cities that are resilient, sustainable, and beneficial to health requires an understanding of urban climate and air quality. This article presents an upgrade to the multi-physics numerical model uDALES, which can simulate microscale airflow, heat transfer, and pollutant dispersion in urban environments. This upgrade enables it to resolve realistic urban geometries more accurately and to take advantage of the resources available on current and future high-performance computing systems.
Felipe Cifuentes, Henk Eskes, Folkert Boersma, Enrico Dammers, and Charlotte Bryan
EGUsphere, https://doi.org/10.5194/egusphere-2024-2225, https://doi.org/10.5194/egusphere-2024-2225, 2024
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We tested the capability of the flux divergence approach (FDA) to reproduce known NOX emissions using synthetic NO2 satellite column retrievals derived from high-resolution model simulations. The FDA accurately reproduced NOX emissions when column observations were limited to the boundary layer and when the variability of NO2 lifetime, NOX:NO2 ratio, and NO2 profile shapes were correctly modeled. This introduces a strong model dependency, reducing the simplicity of the original FDA formulation.
Allison A. Wing, Levi G. Silvers, and Kevin A. Reed
Geosci. Model Dev., 17, 6195–6225, https://doi.org/10.5194/gmd-17-6195-2024, https://doi.org/10.5194/gmd-17-6195-2024, 2024
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This paper presents the experimental design for a model intercomparison project to study tropical clouds and climate. It is a follow-up from a prior project that used a simplified framework for tropical climate. The new project adds one new component – a specified pattern of sea surface temperatures as the lower boundary condition. We provide example results from one cloud-resolving model and one global climate model and test the sensitivity to the experimental parameters.
Astrid Kerkweg, Timo Kirfel, Doung H. Do, Sabine Griessbach, Patrick Jöckel, and Domenico Taraborrelli
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-117, https://doi.org/10.5194/gmd-2024-117, 2024
Revised manuscript accepted for GMD
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This article introduces the MESSy DWARF. Usually, the Modular Earth Submodel System (MESSy) is linked to full dynamical models to build chemistry climate models. However, due to the modular concept of MESSy, and the newly developed DWARF component, it is now possible to create simplified models containing just one or some process descriptions. This renders very useful for technical optimisation (e.g., GPU porting) and can be used to create less complex models, e.g., a chemical box model.
Philip G. Sansom and Jennifer L. Catto
Geosci. Model Dev., 17, 6137–6151, https://doi.org/10.5194/gmd-17-6137-2024, https://doi.org/10.5194/gmd-17-6137-2024, 2024
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Weather fronts bring a lot of rain and strong winds to many regions of the mid-latitudes. We have developed an updated method of identifying these fronts in gridded data that can be used on new datasets with small grid spacing. The method can be easily applied to different datasets due to the use of open-source software for its development and shows improvements over similar previous methods. We present an updated estimate of the average frequency of fronts over the past 40 years.
Kelly M. Núñez Ocasio and Zachary L. Moon
Geosci. Model Dev., 17, 6035–6049, https://doi.org/10.5194/gmd-17-6035-2024, https://doi.org/10.5194/gmd-17-6035-2024, 2024
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TAMS is an open-source Python-based package for tracking and classifying mesoscale convective systems that can be used to study observed and simulated systems. Each step of the algorithm is described in this paper with examples showing how to make use of visualization and post-processing tools within the package. A unique and valuable feature of this tracker is its support for unstructured grids in the identification stage and grid-independent tracking.
Irene C. Dedoussi, Daven K. Henze, Sebastian D. Eastham, Raymond L. Speth, and Steven R. H. Barrett
Geosci. Model Dev., 17, 5689–5703, https://doi.org/10.5194/gmd-17-5689-2024, https://doi.org/10.5194/gmd-17-5689-2024, 2024
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Atmospheric model gradients provide a meaningful tool for better understanding the underlying atmospheric processes. Adjoint modeling enables computationally efficient gradient calculations. We present the adjoint of the GEOS-Chem unified chemistry extension (UCX). With this development, the GEOS-Chem adjoint model can capture stratospheric ozone and other processes jointly with tropospheric processes. We apply it to characterize the Antarctic ozone depletion potential of active halogen species.
Sylvain Mailler, Sotirios Mallios, Arineh Cholakian, Vassilis Amiridis, Laurent Menut, and Romain Pennel
Geosci. Model Dev., 17, 5641–5655, https://doi.org/10.5194/gmd-17-5641-2024, https://doi.org/10.5194/gmd-17-5641-2024, 2024
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We propose two explicit expressions to calculate the settling speed of solid atmospheric particles with prolate spheroidal shapes. The first formulation is based on theoretical arguments only, while the second one is based on computational fluid dynamics calculations. We show that the first method is suitable for virtually all atmospheric aerosols, provided their shape can be adequately described as a prolate spheroid, and we provide an implementation of the first method in AerSett v2.0.2.
Hejun Xie, Lei Bi, and Wei Han
Geosci. Model Dev., 17, 5657–5688, https://doi.org/10.5194/gmd-17-5657-2024, https://doi.org/10.5194/gmd-17-5657-2024, 2024
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A radar operator plays a crucial role in utilizing radar observations to enhance numerical weather forecasts. However, developing an advanced radar operator is challenging due to various complexities associated with the wave scattering by non-spherical hydrometeors, radar beam propagation, and multiple platforms. In this study, we introduce a novel radar operator named the Accurate and Efficient Radar Operator developed by ZheJiang University (ZJU-AERO) which boasts several unique features.
Jonathan J. Day, Gunilla Svensson, Barbara Casati, Taneil Uttal, Siri-Jodha Khalsa, Eric Bazile, Elena Akish, Niramson Azouz, Lara Ferrighi, Helmut Frank, Michael Gallagher, Øystein Godøy, Leslie M. Hartten, Laura X. Huang, Jareth Holt, Massimo Di Stefano, Irene Suomi, Zen Mariani, Sara Morris, Ewan O'Connor, Roberta Pirazzini, Teresa Remes, Rostislav Fadeev, Amy Solomon, Johanna Tjernström, and Mikhail Tolstykh
Geosci. Model Dev., 17, 5511–5543, https://doi.org/10.5194/gmd-17-5511-2024, https://doi.org/10.5194/gmd-17-5511-2024, 2024
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The YOPP site Model Intercomparison Project (YOPPsiteMIP), which was designed to facilitate enhanced weather forecast evaluation in polar regions, is discussed here, focussing on describing the archive of forecast data and presenting a multi-model evaluation at Arctic supersites during February and March 2018. The study highlights an underestimation in boundary layer temperature variance that is common across models and a related inability to forecast cold extremes at several of the sites.
Hossain Mohammed Syedul Hoque, Kengo Sudo, Hitoshi Irie, Yanfeng He, and Md Firoz Khan
Geosci. Model Dev., 17, 5545–5571, https://doi.org/10.5194/gmd-17-5545-2024, https://doi.org/10.5194/gmd-17-5545-2024, 2024
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Using multi-platform observations, we validated global formaldehyde (HCHO) simulations from a chemistry transport model. HCHO is a crucial intermediate in the chemical catalytic cycle that governs the ozone formation in the troposphere. The model was capable of replicating the observed spatiotemporal variability in HCHO. In a few cases, the model's capability was limited. This is attributed to the uncertainties in the observations and the model parameters.
Zijun Liu, Li Dong, Zongxu Qiu, Xingrong Li, Huiling Yuan, Dongmei Meng, Xiaobin Qiu, Dingyuan Liang, and Yafei Wang
Geosci. Model Dev., 17, 5477–5496, https://doi.org/10.5194/gmd-17-5477-2024, https://doi.org/10.5194/gmd-17-5477-2024, 2024
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In this study, we completed a series of simulations with MPAS-Atmosphere (version 7.3) to study the extreme precipitation event of Henan, China, during 20–22 July 2021. We found the different performance of two built-in parameterization scheme suites (mesoscale and convection-permitting suites) with global quasi-uniform and variable-resolution meshes. This study holds significant implications for advancing the understanding of the scale-aware capability of MPAS-Atmosphere.
Laurent Menut, Arineh Cholakian, Romain Pennel, Guillaume Siour, Sylvain Mailler, Myrto Valari, Lya Lugon, and Yann Meurdesoif
Geosci. Model Dev., 17, 5431–5457, https://doi.org/10.5194/gmd-17-5431-2024, https://doi.org/10.5194/gmd-17-5431-2024, 2024
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A new version of the CHIMERE model is presented. This version contains both computational and physico-chemical changes. The computational changes make it easy to choose the variables to be extracted as a result, including values of maximum sub-hourly concentrations. Performance tests show that the model is 1.5 to 2 times faster than the previous version for the same setup. Processes such as turbulence, transport schemes and dry deposition have been modified and updated.
Cited articles
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Clough, S. A., Shephard, M. W., Mlawer, E. J., Delamere, J. S., Iacono, M. J., Cady-Pereira, K., Boukabara, S., and Brown, P. D.: Atmospheric radiative transfer modeling: A summary of the AER codes, J. Quant. Spectrosc. Ra, 91, 233–244, https://doi.org/10.1016/j.jqsrt.2004.05.058, 2005.
Colette, A., Rouïl, L., Meleux, F., Lemaire, V., and Raux, B.: Air Control Toolbox (ACT_v1.0): a flexible surrogate model to explore mitigation scenarios in air quality forecasts, Geosci. Model Dev., 15, 1441–1465, https://doi.org/10.5194/gmd-15-1441-2022, 2022.
Cusworth, D. H., Mickley, L. J., Sulprizio, M. P., Liu, T., Marlier, M. E., DeFries, R. S., Guttikunda, S. K., and Gupta, P.: Quantifying the influence of agricultural fires in northwest India on urban air pollution in Delhi, India, Environ. Res. Lett., 13, 044018, https://doi.org/10.1088/1748-9326/aab303, 2018.
Debnath, S., Jena, C., Ghude, S. D., Kumar, R., Govardhan, G., Gunwani, P., Saha, S. K., Hazra, A., and Pokhrel, S.: Simulation of Indian Summer Monsoon Rainfall (ISMR) with fully coupled regional chemistry transport model: A case study for 2017, Atmos. Environ., 268, 118785, https://doi.org/10.1016/j.atmosenv.2021.118785, 2022.
Denby, B. R., Gauss, M., Wind, P., Mu, Q., Grøtting Wærsted, E., Fagerli, H., Valdebenito, A., and Klein, H.: Description of the uEMEP_v5 downscaling approach for the EMEP MSC-W chemistry transport model, Geosci. Model Dev., 13, 6303–6323, https://doi.org/10.5194/gmd-13-6303-2020, 2020.
Ek, M. B., Mitchell, K. E., Lin, Y., Rogers, E., Grunmann, P., Koren, V., Gayno, G., and Tarpley, J. D.: Implementation of Noah land surface model advances in the National Centers for Environmental Prediction operational mesoscale Eta model, J. Geophys. Res.-Atmos., 108, 8851, https://doi.org/10.1029/2002JD003296, 2003.
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Emmons, L. K., Walters, S., Hess, P. G., Lamarque, J.-F., Pfister, G. G., Fillmore, D., Granier, C., Guenther, A., Kinnison, D., Laepple, T., Orlando, J., Tie, X., Tyndall, G., Wiedinmyer, C., Baughcum, S. L., and Kloster, S.: Description and evaluation of the Model for Ozone and Related chemical Tracers, version 4 (MOZART-4), Geosci. Model Dev., 3, 43–67, https://doi.org/10.5194/gmd-3-43-2010, 2010.
Gadi, R., Shivani, Sharma, S. K., and Mandal, T. K.: Source apportionment and health risk assessment of organic constituents in fine ambient aerosols (PM2.5): a complete year study over National Capital Region of India, Chemosphere, 221, 583–596, https://doi.org/10.1016/j.chemosphere.2019.01.067, 2019.
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Short summary
A newly developed air quality forecasting framework, Decision Support System (DSS), for air quality management in Delhi, India, provides source attribution with numerous emission reduction scenarios besides forecasts. DSS shows that during post-monsoon and winter seasons, Delhi and its neighboring districts contribute to 30 %–40 % each to pollution in Delhi. On average, a 40 % reduction in the emissions in Delhi and the surrounding districts would result in a 24 % reduction in Delhi's pollution.
A newly developed air quality forecasting framework, Decision Support System (DSS), for air...