Articles | Volume 11, issue 9
https://doi.org/10.5194/gmd-11-3623-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/gmd-11-3623-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Model description paper
| 
06 Sep 2018
Model description paper |
| 06 Sep 2018
| 06 Sep 2018
libcloudph++ 2.0: aqueous-phase chemistry extension of the particle-based cloud microphysics scheme
Institute of Geophysics, Faculty of Physics, University of Warsaw, Warsaw, Poland
Hanna Pawlowska
Institute of Geophysics, Faculty of Physics, University of Warsaw, Warsaw, Poland
Related authors
Emily de Jong, John Ben Mackay, Oleksii Bulenok, Anna Jaruga, and Sylwester Arabas
Geosci. Model Dev., 16, 4193–4211, https://doi.org/10.5194/gmd-16-4193-2023, https://doi.org/10.5194/gmd-16-4193-2023, 2023
Short summary
Short summary
In clouds, collisional breakup occurs when two colliding droplets splinter into new, smaller fragments. Particle-based modeling approaches often do not represent breakup because of the computational demands of creating new droplets. We present a particle-based breakup method that preserves the computational efficiency of these methods. In a series of simple demonstrations, we show that this representation alters cloud processes in reasonable and expected ways.
S. Arabas, A. Jaruga, H. Pawlowska, and W. W. Grabowski
Geosci. Model Dev., 8, 1677–1707, https://doi.org/10.5194/gmd-8-1677-2015, https://doi.org/10.5194/gmd-8-1677-2015, 2015
Short summary
Short summary
This paper introduces a free and open-source C++ library of algorithms for representing cloud microphysics in numerical models. In the current release, the library covers three warm-rain schemes: the single- and double-moment bulk schemes, and the particle-based scheme with Monte Carlo coalescence. The three schemes are intended for modelling frameworks of different dimensionalities and complexities ranging from parcel models to multi-dimensional cloud-resolving (e.g. large-eddy) simulations.
A. Jaruga, S. Arabas, D. Jarecka, H. Pawlowska, P. K. Smolarkiewicz, and M. Waruszewski
Geosci. Model Dev., 8, 1005–1032, https://doi.org/10.5194/gmd-8-1005-2015, https://doi.org/10.5194/gmd-8-1005-2015, 2015
Short summary
Short summary
This paper accompanies the first release of libmpdata++, a C++ library implementing the multidimensional positive-definite advection transport algorithm (MPDATA) on a regular structured grid. The library offers basic numerical solvers for systems of generalised transport equations. All solvers offer parallelisation through domain decomposition using shared-memory parallelisation. The paper describes the library programming interface, and serves as a user guide.
Hans Segura, Xabier Pedruzo-Bagazgoitia, Philipp Weiss, Sebastian K. Müller, Thomas Rackow, Junhong Lee, Edgar Dolores-Tesillos, Imme Benedict, Matthias Aengenheyster, Razvan Aguridan, Gabriele Arduini, Alexander J. Baker, Jiawei Bao, Swantje Bastin, Eulàlia Baulenas, Tobias Becker, Sebastian Beyer, Hendryk Bockelmann, Nils Brüggemann, Lukas Brunner, Suvarchal K. Cheedela, Sushant Das, Jasper Denissen, Ian Dragaud, Piotr Dziekan, Madeleine Ekblom, Jan Frederik Engels, Monika Esch, Richard Forbes, Claudia Frauen, Lilli Freischem, Diego García-Maroto, Philipp Geier, Paul Gierz, Álvaro González-Cervera, Katherine Grayson, Matthew Griffith, Oliver Gutjahr, Helmuth Haak, Ioan Hadade, Kerstin Haslehner, Shabeh ul Hasson, Jan Hegewald, Lukas Kluft, Aleksei Koldunov, Nikolay Koldunov, Tobias Kölling, Shunya Koseki, Sergey Kosukhin, Josh Kousal, Peter Kuma, Arjun U. Kumar, Rumeng Li, Nicolas Maury, Maximilian Meindl, Sebastian Milinski, Kristian Mogensen, Bimochan Niraula, Jakub Nowak, Divya Sri Praturi, Ulrike Proske, Dian Putrasahan, René Redler, David Santuy, Domokos Sármány, Reiner Schnur, Patrick Scholz, Dmitry Sidorenko, Dorian Spät, Birgit Sützl, Daisuke Takasuka, Adrian Tompkins, Alejandro Uribe, Mirco Valentini, Menno Veerman, Aiko Voigt, Sarah Warnau, Fabian Wachsmann, Marta Wacławczyk, Nils Wedi, Karl-Hermann Wieners, Jonathan Wille, Marius Winkler, Yuting Wu, Florian Ziemen, Janos Zimmermann, Frida A.-M. Bender, Dragana Bojovic, Sandrine Bony, Simona Bordoni, Patrice Brehmer, Marcus Dengler, Emanuel Dutra, Saliou Faye, Erich Fischer, Chiel van Heerwaarden, Cathy Hohenegger, Heikki Järvinen, Markus Jochum, Thomas Jung, Johann H. Jungclaus, Noel S. Keenlyside, Daniel Klocke, Heike Konow, Martina Klose, Szymon Malinowski, Olivia Martius, Thorsten Mauritsen, Juan Pedro Mellado, Theresa Mieslinger, Elsa Mohino, Hanna Pawłowska, Karsten Peters-von Gehlen, Abdoulaye Sarré, Pajam Sobhani, Philip Stier, Lauri Tuppi, Pier Luigi Vidale, Irina Sandu, and Bjorn Stevens
EGUsphere, https://doi.org/10.5194/egusphere-2025-509, https://doi.org/10.5194/egusphere-2025-509, 2025
This preprint is open for discussion and under review for Geoscientific Model Development (GMD).
Short summary
Short summary
The nextGEMS project developed two Earth system models that resolve processes of the order of 10 km, giving more fidelity to the representation of local phenomena, globally. In its fourth cycle, nextGEMS performed simulations with coupled ocean, land, and atmosphere over the 2020–2049 period under the SSP3-7.0 scenario. Here, we provide an overview of nextGEMS, insights into the model development, and the realism of multi-decadal, kilometer-scale simulations.
Wojciech W. Grabowski and Hanna Pawlowska
EGUsphere, https://doi.org/10.5194/egusphere-2024-4104, https://doi.org/10.5194/egusphere-2024-4104, 2025
Short summary
Short summary
A simple diagram to depict cloud droplets formation via activation of cloud condensation nuclei (CCN) as well as their subsequent growth and evaporation is presented.
Piotr Zmijewski, Piotr Dziekan, and Hanna Pawlowska
Geosci. Model Dev., 17, 759–780, https://doi.org/10.5194/gmd-17-759-2024, https://doi.org/10.5194/gmd-17-759-2024, 2024
Short summary
Short summary
In computer simulations of clouds it is necessary to model the myriad of droplets that constitute a cloud. A popular method for this is to use so-called super-droplets (SDs), each representing many real droplets. It has remained a challenge to model collisions of SDs. We study how precipitation in a cumulus cloud depends on the number of SDs. Surprisingly, we do not find convergence in mean precipitation even for numbers of SDs much larger than typically used in simulations.
Emily de Jong, John Ben Mackay, Oleksii Bulenok, Anna Jaruga, and Sylwester Arabas
Geosci. Model Dev., 16, 4193–4211, https://doi.org/10.5194/gmd-16-4193-2023, https://doi.org/10.5194/gmd-16-4193-2023, 2023
Short summary
Short summary
In clouds, collisional breakup occurs when two colliding droplets splinter into new, smaller fragments. Particle-based modeling approaches often do not represent breakup because of the computational demands of creating new droplets. We present a particle-based breakup method that preserves the computational efficiency of these methods. In a series of simple demonstrations, we show that this representation alters cloud processes in reasonable and expected ways.
Piotr Dziekan, Maciej Waruszewski, and Hanna Pawlowska
Geosci. Model Dev., 12, 2587–2606, https://doi.org/10.5194/gmd-12-2587-2019, https://doi.org/10.5194/gmd-12-2587-2019, 2019
Short summary
Short summary
A new numerical model for clouds is presented. It is designed for detailed studies of the small-scale behavior of cloud droplets within a domain large enough to model cloud field. To achieve this, droplets are modeled in a Lagrangian manner and calculations are done on GPU accelerators. Comparison with models that use Eulerian descriptions of droplets reveals discrepancies in the amount of precipitation. This suggests that some effects important for rain production are missing in current models.
Wojciech W. Grabowski, Piotr Dziekan, and Hanna Pawlowska
Geosci. Model Dev., 11, 103–120, https://doi.org/10.5194/gmd-11-103-2018, https://doi.org/10.5194/gmd-11-103-2018, 2018
Short summary
Short summary
This paper introduces a novel approach to simulating ice-free clouds. The key process is formation and transport of cloud droplets that are represented through Lagrangian particles referred to as super-droplets. Each super-droplet represents a multitude of natural cloud droplets. The essential component of the scheme that makes it different and more efficient from previous approaches is the presence of super-droplets only within a cloud.
Piotr Dziekan and Hanna Pawlowska
Atmos. Chem. Phys., 17, 13509–13520, https://doi.org/10.5194/acp-17-13509-2017, https://doi.org/10.5194/acp-17-13509-2017, 2017
Short summary
Short summary
Raindrops form when small cloud droplets collide with each other. In most computer models of clouds, this process is described using the Smoluchowski equation. We compare the Smoluchowski equation with computer simulations in which each droplet within a small part of the cloud is modeled. We show, depending on the simulation setup, that the Smoluchowski equation can give overly slow or fast rain formation. This implies that many cloud models used do not correctly represent rain formation.
S. Arabas, A. Jaruga, H. Pawlowska, and W. W. Grabowski
Geosci. Model Dev., 8, 1677–1707, https://doi.org/10.5194/gmd-8-1677-2015, https://doi.org/10.5194/gmd-8-1677-2015, 2015
Short summary
Short summary
This paper introduces a free and open-source C++ library of algorithms for representing cloud microphysics in numerical models. In the current release, the library covers three warm-rain schemes: the single- and double-moment bulk schemes, and the particle-based scheme with Monte Carlo coalescence. The three schemes are intended for modelling frameworks of different dimensionalities and complexities ranging from parcel models to multi-dimensional cloud-resolving (e.g. large-eddy) simulations.
A. Jaruga, S. Arabas, D. Jarecka, H. Pawlowska, P. K. Smolarkiewicz, and M. Waruszewski
Geosci. Model Dev., 8, 1005–1032, https://doi.org/10.5194/gmd-8-1005-2015, https://doi.org/10.5194/gmd-8-1005-2015, 2015
Short summary
Short summary
This paper accompanies the first release of libmpdata++, a C++ library implementing the multidimensional positive-definite advection transport algorithm (MPDATA) on a regular structured grid. The library offers basic numerical solvers for systems of generalised transport equations. All solvers offer parallelisation through domain decomposition using shared-memory parallelisation. The paper describes the library programming interface, and serves as a user guide.
D. Jarecka, H. Pawlowska, W. W. Grabowski, and A. A. Wyszogrodzki
Atmos. Chem. Phys., 13, 8489–8503, https://doi.org/10.5194/acp-13-8489-2013, https://doi.org/10.5194/acp-13-8489-2013, 2013
Related subject area
Atmospheric sciences
The MESSy DWARF (based on MESSy v2.55.2)
An enhanced emission module for the PALM model system 23.10 with application for PM10 emission from urban domestic heating
Identifying lightning processes in ERA5 soundings with deep learning
Sensitivity of predicted ultrafine particle size distributions in Europe to different nucleation rate parameterizations using PMCAMx-UF v2.2
Explaining neural networks for detection of tropical cyclones and atmospheric rivers in gridded atmospheric simulation data
Accurate space-based NOx emission estimates with the flux divergence approach require fine-scale model information on local oxidation chemistry and profile shapes
Exploring a high-level programming model for the NWP domain using ECMWF microphysics schemes
Quantifying uncertainties in satellite NO2 superobservations for data assimilation and model evaluation
ML-AMPSIT: Machine Learning-based Automated Multi-method Parameter Sensitivity and Importance analysis Tool
Coupling the urban canopy model TEB (SURFEXv9.0) with the radiation model SPARTACUS-Urbanv0.6.1 for more realistic urban radiative exchange calculation
Forecasting contrail climate forcing for flight planning and air traffic management applications: the CocipGrid model in pycontrails 0.51.0
Simulation of the heat mitigation potential of unsealing measures in cities by parameterizing grass grid pavers for urban microclimate modelling with ENVI-met (V5)
AI-NAOS: an AI-based nonspherical aerosol optical scheme for the chemical weather model GRAPES_Meso5.1/CUACE
Orbital-Radar v1.0.0: a tool to transform suborbital radar observations to synthetic EarthCARE cloud radar data
The Modular and Integrated Data Assimilation System at Environment and Climate Change Canada (MIDAS v3.9.1)
Modeling of polycyclic aromatic hydrocarbons (PAHs) from global to regional scales: model development (IAP-AACM_PAH v1.0) and investigation of health risks in 2013 and 2018 in China
LIMA (v2.0): A full two-moment cloud microphysical scheme for the mesoscale non-hydrostatic model Meso-NH v5-6
SLUCM+BEM (v1.0): a simple parameterisation for dynamic anthropogenic heat and electricity consumption in WRF-Urban (v4.3.2)
NAQPMS-PDAF v2.0: a novel hybrid nonlinear data assimilation system for improved simulation of PM2.5 chemical components
Source-specific bias correction of US background and anthropogenic ozone modeled in CMAQ
Observational operator for fair model evaluation with ground NO2 measurements
Valid time shifting ensemble Kalman filter (VTS-EnKF) for dust storm forecasting
An updated parameterization of the unstable atmospheric surface layer in the Weather Research and Forecasting (WRF) modeling system
The impact of cloud microphysics and ice nucleation on Southern Ocean clouds assessed with single-column modeling and instrument simulators
An updated aerosol simulation in the Community Earth System Model (v2.1.3): dust and marine aerosol emissions and secondary organic aerosol formation
Exploring ship track spreading rates with a physics-informed Langevin particle parameterization
Do data-driven models beat numerical models in forecasting weather extremes? A comparison of IFS HRES, Pangu-Weather, and GraphCast
Development of the MPAS-CMAQ coupled system (V1.0) for multiscale global air quality modeling
Assessment of object-based indices to identify convective organization
The Global Forest Fire Emissions Prediction System version 1.0
Sensitivity Studies of Four‐Dimensional Local Ensemble Transform Kalman Filter Coupled With WRF-Chem Version 3.9.1 for Improving Particulate Matter Simulation Accuracy
Development of A Fast Radiative Transfer Model for Ground-based Microwave Radiometers (ARMS-gb v1.0): Validation and Comparison to RTTOV-gb
NEIVAv1.0: Next-generation Emissions InVentory expansion of Akagi et al. (2011) version 1.0
FLEXPART version 11: improved accuracy, efficiency, and flexibility
Low-level jets in the North and Baltic Seas: Mesoscale Model Sensitivity and Climatology
Challenges of high-fidelity air quality modeling in urban environments – PALM sensitivity study during stable conditions
Knowledge-inspired fusion strategies for the inference of PM2.5 values with a Neural Network
Air quality modeling intercomparison and multiscale ensemble chain for Latin America
Recommended coupling to global meteorological fields for long-term tracer simulations with WRF-GHG
Estimation of aerosol and cloud radiative heating rate in tropical stratosphere using radiative kernel method
Selecting CMIP6 global climate models (GCMs) for Coordinated Regional Climate Downscaling Experiment (CORDEX) dynamical downscaling over Southeast Asia using a standardised benchmarking framework
Improved definition of prior uncertainties in CO2 and CO fossil fuel fluxes and its impact on multi-species inversion with GEOS-Chem (v12.5)
RASCAL v1.0: an open-source tool for climatological time series reconstruction and extension
Porting the Meso-NH atmospheric model on different GPU architectures for the next generation of supercomputers (version MESONH-v55-OpenACC)
Accounting for effects of coagulation and model uncertainties in particle number concentration estimates based on measurements from sampling lines – A Bayesian inversion approach with SLIC v1.0
Introducing graupel density prediction in Weather Research and Forecasting (WRF) double-moment 6-class (WDM6) microphysics and evaluation of the modified scheme during the ICE-POP field campaign
Enabling high-performance cloud computing for the Community Multiscale Air Quality Model (CMAQ) version 5.3.3: performance evaluation and benefits for the user community
Atmospheric-river-induced precipitation in California as simulated by the regionally refined Simple Convective Resolving E3SM Atmosphere Model (SCREAM) Version 0
Recent improvements and maximum covariance analysis of aerosol and cloud properties in the EC-Earth3-AerChem model
GPU-HADVPPM4HIP V1.0: using the heterogeneous-compute interface for portability (HIP) to speed up the piecewise parabolic method in the CAMx (v6.10) air quality model on China's domestic GPU-like accelerator
Astrid Kerkweg, Timo Kirfel, Duong H. Do, Sabine Griessbach, Patrick Jöckel, and Domenico Taraborrelli
Geosci. Model Dev., 18, 1265–1286, https://doi.org/10.5194/gmd-18-1265-2025, https://doi.org/10.5194/gmd-18-1265-2025, 2025
Short summary
Short summary
Normally, the Modular Earth Submodel System (MESSy) is linked to complete dynamic models to create chemical climate models. However, the modular concept of MESSy and the newly developed DWARF component presented here make it possible to create simplified models that contain only one or a few process descriptions. This is very useful for technical optimisation, such as porting to GPUs, and can be used to create less complex models, such as a chemical box model.
Edward C. Chan, Ilona J. Jäkel, Basit Khan, Martijn Schaap, Timothy M. Butler, Renate Forkel, and Sabine Banzhaf
Geosci. Model Dev., 18, 1119–1139, https://doi.org/10.5194/gmd-18-1119-2025, https://doi.org/10.5194/gmd-18-1119-2025, 2025
Short summary
Short summary
An enhanced emission module has been developed for the PALM model system, improving flexibility and scalability of emission source representation across different sectors. A model for parametrized domestic emissions has also been included, for which an idealized model run is conducted for particulate matter (PM10). The results show that, in addition to individual sources and diurnal variations in energy consumption, vertical transport and urban topology play a role in concentration distribution.
Gregor Ehrensperger, Thorsten Simon, Georg J. Mayr, and Tobias Hell
Geosci. Model Dev., 18, 1141–1153, https://doi.org/10.5194/gmd-18-1141-2025, https://doi.org/10.5194/gmd-18-1141-2025, 2025
Short summary
Short summary
As lightning is a brief and localized event, it is not explicitly resolved in atmospheric models. Instead, expert-based auxiliary descriptions are used to assess it. This study explores how AI can improve our understanding of lightning without relying on traditional expert knowledge. We reveal that AI independently identified the key factors known to experts as essential for lightning in the Alps region. This shows how knowledge discovery could be sped up in areas with limited expert knowledge.
David Patoulias, Kalliopi Florou, and Spyros N. Pandis
Geosci. Model Dev., 18, 1103–1118, https://doi.org/10.5194/gmd-18-1103-2025, https://doi.org/10.5194/gmd-18-1103-2025, 2025
Short summary
Short summary
The effect of the assumed atmospheric nucleation mechanism on particle number concentrations and size distribution was investigated. Two quite different mechanisms involving sulfuric acid and ammonia or a biogenic organic vapor gave quite similar results which were consistent with measurements at 26 measurement stations across Europe. The number of larger particles that serve as cloud condensation nuclei showed little sensitivity to the assumed nucleation mechanism.
Tim Radke, Susanne Fuchs, Christian Wilms, Iuliia Polkova, and Marc Rautenhaus
Geosci. Model Dev., 18, 1017–1039, https://doi.org/10.5194/gmd-18-1017-2025, https://doi.org/10.5194/gmd-18-1017-2025, 2025
Short summary
Short summary
In our study, we built upon previous work to investigate the patterns artificial intelligence (AI) learns to detect atmospheric features like tropical cyclones (TCs) and atmospheric rivers (ARs). As primary objective, we adopt a method to explain the AI used and investigate the plausibility of learned patterns. We find that plausible patterns are learned for both TCs and ARs. Hence, the chosen method is very useful for gaining confidence in the AI-based detection of atmospheric features.
Felipe Cifuentes, Henk Eskes, Enrico Dammers, Charlotte Bryan, and Folkert Boersma
Geosci. Model Dev., 18, 621–649, https://doi.org/10.5194/gmd-18-621-2025, https://doi.org/10.5194/gmd-18-621-2025, 2025
Short summary
Short summary
We tested the capability of the flux divergence approach (FDA) to reproduce known NOx emissions using synthetic NO2 satellite column retrievals from high-resolution model simulations. The FDA accurately reproduced NOx emissions when column observations were limited to the boundary layer and when the variability of the NO2 lifetime, the NOx : NO2 ratio, and NO2 profile shapes were correctly modeled. This introduces strong model dependency, reducing the simplicity of the original FDA formulation.
Stefano Ubbiali, Christian Kühnlein, Christoph Schär, Linda Schlemmer, Thomas C. Schulthess, Michael Staneker, and Heini Wernli
Geosci. Model Dev., 18, 529–546, https://doi.org/10.5194/gmd-18-529-2025, https://doi.org/10.5194/gmd-18-529-2025, 2025
Short summary
Short summary
We explore a high-level programming model for porting numerical weather prediction (NWP) model codes to graphics processing units (GPUs). We present a Python rewrite with the domain-specific library GT4Py (GridTools for Python) of two renowned cloud microphysics schemes and the associated tangent-linear and adjoint algorithms. We find excellent portability, competitive GPU performance, robust execution on diverse computing architectures, and enhanced code maintainability and user productivity.
Pieter Rijsdijk, Henk Eskes, Arlene Dingemans, K. Folkert Boersma, Takashi Sekiya, Kazuyuki Miyazaki, and Sander Houweling
Geosci. Model Dev., 18, 483–509, https://doi.org/10.5194/gmd-18-483-2025, https://doi.org/10.5194/gmd-18-483-2025, 2025
Short summary
Short summary
Clustering high-resolution satellite observations into superobservations improves model validation and data assimilation applications. In our paper, we derive quantitative uncertainties for satellite NO2 column observations based on knowledge of the retrievals, including a detailed analysis of spatial error correlations and representativity errors. The superobservations and uncertainty estimates are tested in a global chemical data assimilation system and are found to improve the forecasts.
Dario Di Santo, Cenlin He, Fei Chen, and Lorenzo Giovannini
Geosci. Model Dev., 18, 433–459, https://doi.org/10.5194/gmd-18-433-2025, https://doi.org/10.5194/gmd-18-433-2025, 2025
Short summary
Short summary
This paper presents the Machine Learning-based Automated Multi-method Parameter Sensitivity and Importance analysis Tool (ML-AMPSIT), a computationally efficient tool that uses machine learning algorithms for sensitivity analysis in atmospheric models. It is tested with the Weather Research and Forecasting (WRF) model coupled with the Noah-Multiparameterization (Noah-MP) land surface model to investigate sea breeze circulation sensitivity to vegetation-related parameters.
Robert Schoetter, Robin James Hogan, Cyril Caliot, and Valéry Masson
Geosci. Model Dev., 18, 405–431, https://doi.org/10.5194/gmd-18-405-2025, https://doi.org/10.5194/gmd-18-405-2025, 2025
Short summary
Short summary
Radiation is relevant to the atmospheric impact on people and infrastructure in cities as it can influence the urban heat island, building energy consumption, and human thermal comfort. A new urban radiation model, assuming a more realistic form of urban morphology, is coupled to the urban climate model Town Energy Balance (TEB). The new TEB is evaluated with a reference radiation model for a variety of urban morphologies, and an improvement in the simulated radiative observables is found.
Zebediah Engberg, Roger Teoh, Tristan Abbott, Thomas Dean, Marc E. J. Stettler, and Marc L. Shapiro
Geosci. Model Dev., 18, 253–286, https://doi.org/10.5194/gmd-18-253-2025, https://doi.org/10.5194/gmd-18-253-2025, 2025
Short summary
Short summary
Contrails forming in some atmospheric conditions may persist and become strongly warming cirrus, while in other conditions may be neutral or cooling. We develop a contrail forecast model to predict contrail climate forcing for any arbitrary point in space and time and explore integration into flight planning and air traffic management. This approach enables contrail interventions to target high-probability high-climate-impact regions and reduce unintended consequences of contrail management.
Nils Eingrüber, Alina Domm, Wolfgang Korres, and Karl Schneider
Geosci. Model Dev., 18, 141–160, https://doi.org/10.5194/gmd-18-141-2025, https://doi.org/10.5194/gmd-18-141-2025, 2025
Short summary
Short summary
Climate change adaptation measures like unsealings can reduce urban heat stress. As grass grid pavers have never been parameterized for microclimate model simulations with ENVI-met, a new parameterization was developed based on field measurements. To analyse the cooling potential, scenario analyses were performed for a densely developed area in Cologne. Statistically significant average cooling effects of up to −11.1 K were found for surface temperature and up to −2.9 K for 1 m air temperature.
Xuan Wang, Lei Bi, Hong Wang, Yaqiang Wang, Wei Han, Xueshun Shen, and Xiaoye Zhang
Geosci. Model Dev., 18, 117–139, https://doi.org/10.5194/gmd-18-117-2025, https://doi.org/10.5194/gmd-18-117-2025, 2025
Short summary
Short summary
The Artificial-Intelligence-based Nonspherical Aerosol Optical Scheme (AI-NAOS) was developed to improve the estimation of the aerosol direct radiation effect and was coupled online with a chemical weather model. The AI-NAOS scheme considers black carbon as fractal aggregates and soil dust as super-spheroids, encapsulated with hygroscopic aerosols. Real-case simulations emphasize the necessity of accurately representing nonspherical and inhomogeneous aerosols in chemical weather models.
Lukas Pfitzenmaier, Pavlos Kollias, Nils Risse, Imke Schirmacher, Bernat Puigdomenech Treserras, and Katia Lamer
Geosci. Model Dev., 18, 101–115, https://doi.org/10.5194/gmd-18-101-2025, https://doi.org/10.5194/gmd-18-101-2025, 2025
Short summary
Short summary
The Python tool Orbital-Radar transfers suborbital radar data (ground-based, airborne, and forward-simulated numerical weather prediction model) into synthetic spaceborne cloud profiling radar data, mimicking platform-specific instrument characteristics, e.g. EarthCARE or CloudSat. The tool's novelty lies in simulating characteristic errors and instrument noise. Thus, existing data sets are transferred into synthetic observations and can be used for satellite calibration–validation studies.
Mark Buehner, Jean-Francois Caron, Ervig Lapalme, Alain Caya, Ping Du, Yves Rochon, Sergey Skachko, Maziar Bani Shahabadi, Sylvain Heilliette, Martin Deshaies-Jacques, Weiguang Chang, and Michael Sitwell
Geosci. Model Dev., 18, 1–18, https://doi.org/10.5194/gmd-18-1-2025, https://doi.org/10.5194/gmd-18-1-2025, 2025
Short summary
Short summary
The Modular and Integrated Data Assimilation System (MIDAS) software is described. The flexible design of MIDAS enables both deterministic and ensemble prediction applications for the atmosphere and several other Earth system components. It is currently used for all main operational weather prediction systems in Canada and also for sea ice and sea surface temperature analysis. The use of MIDAS for multiple Earth system components will facilitate future research on coupled data assimilation.
Zichen Wu, Xueshun Chen, Zifa Wang, Huansheng Chen, Zhe Wang, Qing Mu, Lin Wu, Wending Wang, Xiao Tang, Jie Li, Ying Li, Qizhong Wu, Yang Wang, Zhiyin Zou, and Zijian Jiang
Geosci. Model Dev., 17, 8885–8907, https://doi.org/10.5194/gmd-17-8885-2024, https://doi.org/10.5194/gmd-17-8885-2024, 2024
Short summary
Short summary
We developed a model to simulate polycyclic aromatic hydrocarbons (PAHs) from global to regional scales. The model can reproduce PAH distribution well. The concentration of BaP (indicator species for PAHs) could exceed the target values of 1 ng m-3 over some areas (e.g., in central Europe, India, and eastern China). The change in BaP is lower than that in PM2.5 from 2013 to 2018. China still faces significant potential health risks posed by BaP although the Action Plan has been implemented.
Marie Taufour, Jean-Pierre Pinty, Christelle Barthe, Benoît Vié, and Chien Wang
Geosci. Model Dev., 17, 8773–8798, https://doi.org/10.5194/gmd-17-8773-2024, https://doi.org/10.5194/gmd-17-8773-2024, 2024
Short summary
Short summary
We have developed a complete two-moment version of the LIMA (Liquid Ice Multiple Aerosols) microphysics scheme. We have focused on collection processes, where the hydrometeor number transfer is often estimated in proportion to the mass transfer. The impact of these parameterizations on a convective system and the prospects for more realistic estimates of secondary parameters (reflectivity, hydrometeor size) are shown in a first test on an idealized case.
Yuya Takane, Yukihiro Kikegawa, Ko Nakajima, and Hiroyuki Kusaka
Geosci. Model Dev., 17, 8639–8664, https://doi.org/10.5194/gmd-17-8639-2024, https://doi.org/10.5194/gmd-17-8639-2024, 2024
Short summary
Short summary
A new parameterisation for dynamic anthropogenic heat and electricity consumption is described. The model reproduced the temporal variation in and spatial distributions of electricity consumption and temperature well in summer and winter. The partial air conditioning was the most critical factor, significantly affecting the value of anthropogenic heat emission.
Hongyi Li, Ting Yang, Lars Nerger, Dawei Zhang, Di Zhang, Guigang Tang, Haibo Wang, Yele Sun, Pingqing Fu, Hang Su, and Zifa Wang
Geosci. Model Dev., 17, 8495–8519, https://doi.org/10.5194/gmd-17-8495-2024, https://doi.org/10.5194/gmd-17-8495-2024, 2024
Short summary
Short summary
To accurately characterize the spatiotemporal distribution of particulate matter <2.5 µm chemical components, we developed the Nested Air Quality Prediction Model System with the Parallel Data Assimilation Framework (NAQPMS-PDAF) v2.0 for chemical components with non-Gaussian and nonlinear properties. NAQPMS-PDAF v2.0 has better computing efficiency, excels when used with a small ensemble size, and can significantly improve the simulation performance of chemical components.
T. Nash Skipper, Christian Hogrefe, Barron H. Henderson, Rohit Mathur, Kristen M. Foley, and Armistead G. Russell
Geosci. Model Dev., 17, 8373–8397, https://doi.org/10.5194/gmd-17-8373-2024, https://doi.org/10.5194/gmd-17-8373-2024, 2024
Short summary
Short summary
Chemical transport model simulations are combined with ozone observations to estimate the bias in ozone attributable to US anthropogenic sources and individual sources of US background ozone: natural sources, non-US anthropogenic sources, and stratospheric ozone. Results indicate a positive bias correlated with US anthropogenic emissions during summer in the eastern US and a negative bias correlated with stratospheric ozone during spring.
Li Fang, Jianbing Jin, Arjo Segers, Ke Li, Ji Xia, Wei Han, Baojie Li, Hai Xiang Lin, Lei Zhu, Song Liu, and Hong Liao
Geosci. Model Dev., 17, 8267–8282, https://doi.org/10.5194/gmd-17-8267-2024, https://doi.org/10.5194/gmd-17-8267-2024, 2024
Short summary
Short summary
Model evaluations against ground observations are usually unfair. The former simulates mean status over coarse grids and the latter the surrounding atmosphere. To solve this, we proposed the new land-use-based representative (LUBR) operator that considers intra-grid variance. The LUBR operator is validated to provide insights that align with satellite measurements. The results highlight the importance of considering fine-scale urban–rural differences when comparing models and observation.
Mijie Pang, Jianbing Jin, Arjo Segers, Huiya Jiang, Wei Han, Batjargal Buyantogtokh, Ji Xia, Li Fang, Jiandong Li, Hai Xiang Lin, and Hong Liao
Geosci. Model Dev., 17, 8223–8242, https://doi.org/10.5194/gmd-17-8223-2024, https://doi.org/10.5194/gmd-17-8223-2024, 2024
Short summary
Short summary
The ensemble Kalman filter (EnKF) improves dust storm forecasts but faces challenges with position errors. The valid time shifting EnKF (VTS-EnKF) addresses this by adjusting for position errors, enhancing accuracy in forecasting dust storms, as proven in tests on 2021 events, even with smaller ensembles and time intervals.
Prabhakar Namdev, Maithili Sharan, Piyush Srivastava, and Saroj Kanta Mishra
Geosci. Model Dev., 17, 8093–8114, https://doi.org/10.5194/gmd-17-8093-2024, https://doi.org/10.5194/gmd-17-8093-2024, 2024
Short summary
Short summary
Inadequate representation of surface–atmosphere interaction processes is a major source of uncertainty in numerical weather prediction models. Here, an effort has been made to improve the Weather Research and Forecasting (WRF) model version 4.2.2 by introducing a unique theoretical framework under convective conditions. In addition, to enhance the potential applicability of the WRF modeling system, various commonly used similarity functions under convective conditions have also been installed.
Andrew Gettelman, Richard Forbes, Roger Marchand, Chih-Chieh Chen, and Mark Fielding
Geosci. Model Dev., 17, 8069–8092, https://doi.org/10.5194/gmd-17-8069-2024, https://doi.org/10.5194/gmd-17-8069-2024, 2024
Short summary
Short summary
Supercooled liquid clouds (liquid clouds colder than 0°C) are common at higher latitudes (especially over the Southern Ocean) and are critical for constraining climate projections. We compare a single-column version of a weather model to observations with two different cloud schemes and find that both the dynamical environment and atmospheric aerosols are important for reproducing observations.
Yujuan Wang, Peng Zhang, Jie Li, Yaman Liu, Yanxu Zhang, Jiawei Li, and Zhiwei Han
Geosci. Model Dev., 17, 7995–8021, https://doi.org/10.5194/gmd-17-7995-2024, https://doi.org/10.5194/gmd-17-7995-2024, 2024
Short summary
Short summary
This study updates the CESM's aerosol schemes, focusing on dust, marine aerosol emissions, and secondary organic aerosol (SOA) . Dust emission modifications make deflation areas more continuous, improving results in North America and the sub-Arctic. Humidity correction to sea-salt emissions has a minor effect. Introducing marine organic aerosol emissions, coupled with ocean biogeochemical processes, and adding aqueous reactions for SOA formation advance the CESM's aerosol modelling results.
Lucas A. McMichael, Michael J. Schmidt, Robert Wood, Peter N. Blossey, and Lekha Patel
Geosci. Model Dev., 17, 7867–7888, https://doi.org/10.5194/gmd-17-7867-2024, https://doi.org/10.5194/gmd-17-7867-2024, 2024
Short summary
Short summary
Marine cloud brightening (MCB) is a climate intervention technique to potentially cool the climate. Climate models used to gauge regional climate impacts associated with MCB often assume large areas of the ocean are uniformly perturbed. However, a more realistic representation of MCB application would require information about how an injected particle plume spreads. This work aims to develop such a plume-spreading model.
Leonardo Olivetti and Gabriele Messori
Geosci. Model Dev., 17, 7915–7962, https://doi.org/10.5194/gmd-17-7915-2024, https://doi.org/10.5194/gmd-17-7915-2024, 2024
Short summary
Short summary
Data-driven models are becoming a viable alternative to physics-based models for weather forecasting up to 15 d into the future. However, it is unclear whether they are as reliable as physics-based models when forecasting weather extremes. We evaluate their performance in forecasting near-surface cold, hot, and windy extremes globally. We find that data-driven models can compete with physics-based models and that the choice of the best model mainly depends on the region and type of extreme.
David C. Wong, Jeff Willison, Jonathan E. Pleim, Golam Sarwar, James Beidler, Russ Bullock, Jerold A. Herwehe, Rob Gilliam, Daiwen Kang, Christian Hogrefe, George Pouliot, and Hosein Foroutan
Geosci. Model Dev., 17, 7855–7866, https://doi.org/10.5194/gmd-17-7855-2024, https://doi.org/10.5194/gmd-17-7855-2024, 2024
Short summary
Short summary
This work describe how we linked the meteorological Model for Prediction Across Scales – Atmosphere (MPAS-A) with the Community Multiscale Air Quality (CMAQ) air quality model to form a coupled modelling system. This could be used to study air quality or climate and air quality interaction at a global scale. This new model scales well in high-performance computing environments and performs well with respect to ground surface networks in terms of ozone and PM2.5.
Giulio Mandorli and Claudia J. Stubenrauch
Geosci. Model Dev., 17, 7795–7813, https://doi.org/10.5194/gmd-17-7795-2024, https://doi.org/10.5194/gmd-17-7795-2024, 2024
Short summary
Short summary
In recent years, several studies focused their attention on the disposition of convection. Lots of methods, called indices, have been developed to quantify the amount of convection clustering. These indices are evaluated in this study by defining criteria that must be satisfied and then evaluating the indices against these standards. None of the indices meet all criteria, with some only partially meeting them.
Kerry Anderson, Jack Chen, Peter Englefield, Debora Griffin, Paul A. Makar, and Dan Thompson
Geosci. Model Dev., 17, 7713–7749, https://doi.org/10.5194/gmd-17-7713-2024, https://doi.org/10.5194/gmd-17-7713-2024, 2024
Short summary
Short summary
The Global Forest Fire Emissions Prediction System (GFFEPS) is a model that predicts smoke and carbon emissions from wildland fires. The model calculates emissions from the ground up based on satellite-detected fires, modelled weather and fire characteristics. Unlike other global models, GFFEPS uses daily weather conditions to capture changing burning conditions on a day-to-day basis. GFFEPS produced lower carbon emissions due to the changing weather not captured by the other models.
Jianyu Lin, Tie Dai, Lifang Sheng, Weihang Zhang, Shangfei Hai, and Yawen Kong
EGUsphere, https://doi.org/10.5194/egusphere-2024-3321, https://doi.org/10.5194/egusphere-2024-3321, 2024
Short summary
Short summary
The effectiveness of assimilation system and its sensitivity to ensemble member size and length of assimilation window have been investigated. This study advances our understanding about the selection of basic parameters in the four-dimension local ensemble transform Kalman filter assimilation system and the performance of ensemble simulation in a particulate matter polluted environment.
Yi-Ning Shi, Jun Yang, Wei Han, Lujie Han, Jiajia Mao, Wanlin Kan, and Fuzhong Weng
EGUsphere, https://doi.org/10.5194/egusphere-2024-2884, https://doi.org/10.5194/egusphere-2024-2884, 2024
Short summary
Short summary
Assimilating Ground-based microwave radiometers' observations into numerical weather prediction models holds significant promise for enhancing forecast accuracy. Radiative transfer models (RTM) are crucial for direct data assimilation. We propose a new RTM capable of simulating brightness temperatures observed by GMRs and their Jacobians. Several improvements are introduced to achieve higher accuracy.The RTM align with RTTOV-gb well and can achieve smaller STD in water vapor absorption channels.
Samiha Binte Shahid, Forrest G. Lacey, Christine Wiedinmyer, Robert J. Yokelson, and Kelley C. Barsanti
Geosci. Model Dev., 17, 7679–7711, https://doi.org/10.5194/gmd-17-7679-2024, https://doi.org/10.5194/gmd-17-7679-2024, 2024
Short summary
Short summary
The Next-generation Emissions InVentory expansion of Akagi (NEIVA) v.1.0 is a comprehensive biomass burning emissions database that allows integration of new data and flexible querying. Data are stored in connected datasets, including recommended averages of ~1500 constituents for 14 globally relevant fire types. Individual compounds were mapped to common model species to allow better attribution of emissions in modeling studies that predict the effects of fires on air quality and climate.
Lucie Bakels, Daria Tatsii, Anne Tipka, Rona Thompson, Marina Dütsch, Michael Blaschek, Petra Seibert, Katharina Baier, Silvia Bucci, Massimo Cassiani, Sabine Eckhardt, Christine Groot Zwaaftink, Stephan Henne, Pirmin Kaufmann, Vincent Lechner, Christian Maurer, Marie D. Mulder, Ignacio Pisso, Andreas Plach, Rakesh Subramanian, Martin Vojta, and Andreas Stohl
Geosci. Model Dev., 17, 7595–7627, https://doi.org/10.5194/gmd-17-7595-2024, https://doi.org/10.5194/gmd-17-7595-2024, 2024
Short summary
Short summary
Computer models are essential for improving our understanding of how gases and particles move in the atmosphere. We present an update of the atmospheric transport model FLEXPART. FLEXPART 11 is more accurate due to a reduced number of interpolations and a new scheme for wet deposition. It can simulate non-spherical aerosols and includes linear chemical reactions. It is parallelised using OpenMP and includes new user options. A new user manual details how to use FLEXPART 11.
Bjarke Tobias Eisensøe Olsen, Andrea Noemi Hahmann, Nicolás González Alonso-de-Linaje, Mark Žagar, and Martin Dörenkämper
EGUsphere, https://doi.org/10.5194/egusphere-2024-3123, https://doi.org/10.5194/egusphere-2024-3123, 2024
Short summary
Short summary
Low-level jets (LLJs) are strong winds in the lower atmosphere, important for wind energy as turbines get taller. This study compares a weather model (WRF) with real data across five North and Baltic Sea sites. Adjusting the model improved accuracy over the widely-used ERA5. In key offshore regions, LLJs occur 10–15 % of the time and significantly boost wind power, especially in spring and summer, contributing up to 30 % of total capacity in some areas.
Jaroslav Resler, Petra Bauerová, Michal Belda, Martin Bureš, Kryštof Eben, Vladimír Fuka, Jan Geletič, Radek Jareš, Jan Karel, Josef Keder, Pavel Krč, William Patiño, Jelena Radović, Hynek Řezníček, Matthias Sühring, Adriana Šindelářová, and Ondřej Vlček
Geosci. Model Dev., 17, 7513–7537, https://doi.org/10.5194/gmd-17-7513-2024, https://doi.org/10.5194/gmd-17-7513-2024, 2024
Short summary
Short summary
Detailed modeling of urban air quality in stable conditions is a challenge. We show the unprecedented sensitivity of a large eddy simulation (LES) model to meteorological boundary conditions and model parameters in an urban environment under stable conditions. We demonstrate the crucial role of boundary conditions for the comparability of results with observations. The study reveals a strong sensitivity of the results to model parameters and model numerical instabilities during such conditions.
Matthieu Dabrowski, José Mennesson, Jérôme Riedi, Chaabane Djeraba, and Pierre Nabat
EGUsphere, https://doi.org/10.5194/egusphere-2024-2676, https://doi.org/10.5194/egusphere-2024-2676, 2024
Short summary
Short summary
This work focuses on the prediction of aerosol concentration values at ground level, which are a strong indicator of air quality, using Artificial Neural Networks. A study of different variables and their efficiency as inputs for these models is also proposed, and reveals that the best results are obtained when using all of them. Comparison of networks architectures and information fusion methods allows the extraction of knowledge on the most efficient methods in the context of this study.
Jorge E. Pachón, Mariel A. Opazo, Pablo Lichtig, Nicolas Huneeus, Idir Bouarar, Guy Brasseur, Cathy W. Y. Li, Johannes Flemming, Laurent Menut, Camilo Menares, Laura Gallardo, Michael Gauss, Mikhail Sofiev, Rostislav Kouznetsov, Julia Palamarchuk, Andreas Uppstu, Laura Dawidowski, Nestor Y. Rojas, María de Fátima Andrade, Mario E. Gavidia-Calderón, Alejandro H. Delgado Peralta, and Daniel Schuch
Geosci. Model Dev., 17, 7467–7512, https://doi.org/10.5194/gmd-17-7467-2024, https://doi.org/10.5194/gmd-17-7467-2024, 2024
Short summary
Short summary
Latin America (LAC) has some of the most populated urban areas in the world, with high levels of air pollution. Air quality management in LAC has been traditionally focused on surveillance and building emission inventories. This study performed the first intercomparison and model evaluation in LAC, with interesting and insightful findings for the region. A multiscale modeling ensemble chain was assembled as a first step towards an air quality forecasting system.
David Ho, Michał Gałkowski, Friedemann Reum, Santiago Botía, Julia Marshall, Kai Uwe Totsche, and Christoph Gerbig
Geosci. Model Dev., 17, 7401–7422, https://doi.org/10.5194/gmd-17-7401-2024, https://doi.org/10.5194/gmd-17-7401-2024, 2024
Short summary
Short summary
Atmospheric model users often overlook the impact of the land–atmosphere interaction. This study accessed various setups of WRF-GHG simulations that ensure consistency between the model and driving reanalysis fields. We found that a combination of nudging and frequent re-initialization allows certain improvement by constraining the soil moisture fields and, through its impact on atmospheric mixing, improves atmospheric transport.
Jie Gao, Yi Huang, Jonathon S. Wright, Ke Li, Tao Geng, and Qiurun Yu
EGUsphere, https://doi.org/10.5194/egusphere-2024-2815, https://doi.org/10.5194/egusphere-2024-2815, 2024
Short summary
Short summary
The aerosol in the upper troposphere and stratosphere is highly variable, and its radiative effect is poorly understood. To estimate that effect, the radiative kernel is constructed and applied. The results show that the kernels can reproduce aerosol radiative effects and are expected to simulate stratospheric aerosol radiative effects. This approach reduces computational expense and consists well with radiative model calculations and can be applied to atmospheric models with speed requirements.
Phuong Loan Nguyen, Lisa V. Alexander, Marcus J. Thatcher, Son C. H. Truong, Rachael N. Isphording, and John L. McGregor
Geosci. Model Dev., 17, 7285–7315, https://doi.org/10.5194/gmd-17-7285-2024, https://doi.org/10.5194/gmd-17-7285-2024, 2024
Short summary
Short summary
We use a comprehensive approach to select a subset of CMIP6 models for dynamical downscaling over Southeast Asia, taking into account model performance, model independence, data availability and the range of future climate projections. The standardised benchmarking framework is applied to assess model performance through both statistical and process-based metrics. Ultimately, we identify two independent model groups that are suitable for dynamical downscaling in the Southeast Asian region.
Ingrid Super, Tia Scarpelli, Arjan Droste, and Paul I. Palmer
Geosci. Model Dev., 17, 7263–7284, https://doi.org/10.5194/gmd-17-7263-2024, https://doi.org/10.5194/gmd-17-7263-2024, 2024
Short summary
Short summary
Monitoring greenhouse gas emission reductions requires a combination of models and observations, as well as an initial emission estimate. Each component provides information with a certain level of certainty and is weighted to yield the most reliable estimate of actual emissions. We describe efforts for estimating the uncertainty in the initial emission estimate, which significantly impacts the outcome. Hence, a good uncertainty estimate is key for obtaining reliable information on emissions.
Álvaro González-Cervera and Luis Durán
Geosci. Model Dev., 17, 7245–7261, https://doi.org/10.5194/gmd-17-7245-2024, https://doi.org/10.5194/gmd-17-7245-2024, 2024
Short summary
Short summary
RASCAL is an open-source Python tool designed for reconstructing daily climate observations, especially in regions with complex local phenomena. It merges large-scale weather patterns with local weather using the analog method. Evaluations in central Spain show that RASCAL outperforms ERA20C reanalysis in reconstructing precipitation and temperature. RASCAL offers opportunities for broad scientific applications, from short-term forecasts to local-scale climate change scenarios.
Juan Escobar, Philippe Wautelet, Joris Pianezze, Florian Pantillon, Thibaut Dauhut, Christelle Barthe, and Jean-Pierre Chaboureau
EGUsphere, https://doi.org/10.5194/egusphere-2024-2879, https://doi.org/10.5194/egusphere-2024-2879, 2024
Short summary
Short summary
The Meso-NH weather research code is adapted for GPUs using OpenACC, leading to significant performance and energy efficiency improvements. Called MESONH-v55-OpenACC, it includes enhanced memory management, communication optimizations, and a new solver. On the AMD MI250X Adastra platform, it achieved up to 6× speedup and 2.3× energy efficiency gain compared to CPUs. Storm simulations at 100 m resolution show successful results , positioning the code for future use on exascale supercomputers.
Matti Niskanen, Aku Seppänen, Henri Oikarinen, Miska Olin, Panu Karjalainen, Santtu Mikkonen, and Kari Lehtinen
EGUsphere, https://doi.org/10.5194/egusphere-2024-1898, https://doi.org/10.5194/egusphere-2024-1898, 2024
Short summary
Short summary
Particle size is a key factor determining the properties of aerosol particles, which have a major influence on the climate and on human health. When measuring the particle sizes, however, sometimes the sampling lines that transfer the aerosol to the measurement device distort the size distribution, making the measurement unreliable. We propose a method to correct for the distortions and estimate the true particle sizes, improving measurement accuracy.
Sun-Young Park, Kyo-Sun Sunny Lim, Kwonil Kim, Gyuwon Lee, and Jason A. Milbrandt
Geosci. Model Dev., 17, 7199–7218, https://doi.org/10.5194/gmd-17-7199-2024, https://doi.org/10.5194/gmd-17-7199-2024, 2024
Short summary
Short summary
We enhance the WDM6 scheme by incorporating predicted graupel density. The modification affects graupel characteristics, including fall velocity–diameter and mass–diameter relationships. Simulations highlight changes in graupel distribution and precipitation patterns, potentially influencing surface snow amounts. The study underscores the significance of integrating predicted graupel density for a more realistic portrayal of microphysical properties in weather models.
Christos I. Efstathiou, Elizabeth Adams, Carlie J. Coats, Robert Zelt, Mark Reed, John McGee, Kristen M. Foley, Fahim I. Sidi, David C. Wong, Steven Fine, and Saravanan Arunachalam
Geosci. Model Dev., 17, 7001–7027, https://doi.org/10.5194/gmd-17-7001-2024, https://doi.org/10.5194/gmd-17-7001-2024, 2024
Short summary
Short summary
We present a summary of enabling high-performance computing of the Community Multiscale Air Quality Model (CMAQ) – a state-of-the-science community multiscale air quality model – on two cloud computing platforms through documenting the technologies, model performance, scaling and relative merits. This may be a new paradigm for computationally intense future model applications. We initiated this work due to a need to leverage cloud computing advances and to ease the learning curve for new users.
Peter A. Bogenschutz, Jishi Zhang, Qi Tang, and Philip Cameron-Smith
Geosci. Model Dev., 17, 7029–7050, https://doi.org/10.5194/gmd-17-7029-2024, https://doi.org/10.5194/gmd-17-7029-2024, 2024
Short summary
Short summary
Using high-resolution and state-of-the-art modeling techniques we simulate five atmospheric river events for California to test the capability to represent precipitation for these events. We find that our model is able to capture the distribution of precipitation very well but suffers from overestimating the precipitation amounts over high elevation. Increasing the resolution further has no impact on reducing this bias, while increasing the domain size does have modest impacts.
Manu Anna Thomas, Klaus Wyser, Shiyu Wang, Marios Chatziparaschos, Paraskevi Georgakaki, Montserrat Costa-Surós, Maria Gonçalves Ageitos, Maria Kanakidou, Carlos Pérez García-Pando, Athanasios Nenes, Twan van Noije, Philippe Le Sager, and Abhay Devasthale
Geosci. Model Dev., 17, 6903–6927, https://doi.org/10.5194/gmd-17-6903-2024, https://doi.org/10.5194/gmd-17-6903-2024, 2024
Short summary
Short summary
Aerosol–cloud interactions occur at a range of spatio-temporal scales. While evaluating recent developments in EC-Earth3-AerChem, this study aims to understand the extent to which the Twomey effect manifests itself at larger scales. We find a reduction in the warm bias over the Southern Ocean due to model improvements. While we see footprints of the Twomey effect at larger scales, the negative relationship between cloud droplet number and liquid water drives the shortwave radiative effect.
Kai Cao, Qizhong Wu, Lingling Wang, Hengliang Guo, Nan Wang, Huaqiong Cheng, Xiao Tang, Dongxing Li, Lina Liu, Dongqing Li, Hao Wu, and Lanning Wang
Geosci. Model Dev., 17, 6887–6901, https://doi.org/10.5194/gmd-17-6887-2024, https://doi.org/10.5194/gmd-17-6887-2024, 2024
Short summary
Short summary
AMD’s heterogeneous-compute interface for portability was implemented to port the piecewise parabolic method solver from NVIDIA GPUs to China's GPU-like accelerators. The results show that the larger the model scale, the more acceleration effect on the GPU-like accelerator, up to 28.9 times. The multi-level parallelism achieves a speedup of 32.7 times on the heterogeneous cluster. By comparing the results, the GPU-like accelerators have more accuracy for the geoscience numerical models.
Cited articles
Alefeld, G. E., Potra, F. A., and Shi, Y.: Algorithm 748: Enclosing Zeros of
Continuous Functions, ACM Trans. Math. Softw., 21, 327–344,
https://doi.org/10.1145/210089.210111, 1995. a
Alfonso, L. and Raga, G.: Estimating the impact of natural and anthropogenic
emissions on cloud chemistry: Part I. Sulfur cycle, Atmos. Res., 62, 33–55,
https://doi.org/10.1016/S0169-8095(02)00022-4, 2002. a
Andrejczuk, M., Grabowski, W. W., Reisner, J., and Gadian, A.: Cloud-aerosol
interactions for boundary layer stratocumulus in the Lagrangian Cloud Model,
J. Geophys. Res.-Atmos, 115, D22, https://doi.org/10.1029/2010JD014248, 2010. a
Andrejczuk, M., Gadian, A., and Blyth, A.: Numerical simulations of
stratocumulus cloud response to aerosol perturbation, Atmos. Res., 140–141,
76–84, https://doi.org/10.1016/j.atmosres.2014.01.006, 2014. a
Arabas, S. and Pawlowska, H.: Adaptive method of lines for multi-component
aerosol condensational growth and CCN activation, Geosci. Model Dev., 4,
15–31, https://doi.org/10.5194/gmd-4-15-2011, 2011. a
Arabas, S. and Shima, S.-I.: Large-Eddy Simulations of Trade Wind Cumuli
Using
Particle-Based Microphysics with Monte Carlo Coalescence, J. Atmos. Sci., 70,
2768–2777, https://doi.org/10.1175/JAS-D-12-0295.1, 2013. a
Arabas, S., Jaruga, A., Pawlowska, H., and Grabowski, W. W.: libcloudph++
1.0:
a single-moment bulk, double-moment bulk, and particle-based warm-rain
microphysics library in C++, Geosci. Model Dev., 8, 1677–1707,
https://doi.org/10.5194/gmd-8-1677-2015, 2015. a, b, c, d, e, f, g, h, i, j, k, l, m, n
Ardon-Dryer, K., Huang, Y.-W., and Cziczo, D. J.: Laboratory studies of
collection efficiency of sub-micrometer aerosol particles by cloud droplets
on a single-droplet basis, Atmos. Chem. Phys., 15, 9159–9171,
https://doi.org/10.5194/acp-15-9159-2015, 2015. a
Barth, M. C., Rasch, P. J., Kiehl, J. T., Benkovitz, C. M., and Schwartz,
S. E.: Sulfur chemistry in the National Center for Atmospheric Research
Community Climate Model: Description, evaluation, features, and sensitivity
to aqueous chemistry, J. Geophys. Res.-Atmos., 105, 1387–1415,
https://doi.org/10.1029/1999JD900773, 2000. a
Bower, K., Choularton, T., Gallagher, M., Colvile, R., Wells, M., Beswick,
K.,
Wiedensohler, A., Hansson, H.-C., Svenningsson, B., Swietlicki, E., Wendisch,
M., Berner, A., Kruisz, C., Laj, P., Facchini, M., Fuzzi, S., Bizjak, M.,
Dollard, G., Jones, B., Acker, K., Wieprecht, W., Preiss, M., Sutton, M.,
Hargreaves, K., Storeton-West, R., Cape, J., and Arends, B.: Observations and
modelling of the processing of aerosol by a hill cap cloud, Atmos. Environ.,
31, 2527–2543, https://doi.org/10.1016/S1352-2310(96)00317-2, 1997. a
Cantrell, W., Shaw, G., and Benner, R.: Cloud properties inferred from
bimodal
aerosol number distributions, J. Geophys. Res, 104, 27615–27624,
https://doi.org/10.1029/1999JD900252, 1999. a
Chen, S., Yau, M. K., and Bartello, P.: Turbulence Effects of Collision
Efficiency and Broadening of Droplet Size Distribution in Cumulus Clouds, J.
Atmos. Sci., 75, 203–217, https://doi.org/10.1175/JAS-D-17-0123.1, 2018. a
Dianwu, Z., Jiling, X., Yu, X., and Chan, W. H.: Acid rain in southwestern
China, Atmos. Environ., 22, 349–358, https://doi.org/10.1016/0004-6981(88)90040-6,
1988. a
Dziekan, P. and Pawlowska, H.: Stochastic coalescence in Lagrangian cloud
microphysics, Atmos. Chem. Phys., 17, 13509–13520,
https://doi.org/10.5194/acp-17-13509-2017, 2017. a
Ervens, B.: Modeling the Processing of Aerosol and Trace Gases in Clouds and
Fogs, Chem. Rev., 115, 4157–4198, https://doi.org/10.1021/cr5005887, 2015. a
Faloona, I.: Sulfur processing in the marine atmospheric boundary layer: A
review and critical assessment of modeling uncertainties, Atmos. Environ.,
43, 2841–2854, https://doi.org/10.1016/j.atmosenv.2009.02.043, 2009. a, b
Feingold, G. and Kreidenweis, S. M.: Does cloud processing of aerosol enhance
droplet concentrations?, J. Geophys. Res.-Atmos., 105,
24351–24361, https://doi.org/10.1029/2000JD900369, 2000. a
Feingold, G. and Kreidenweis, S. M.: Cloud processing of aerosol as modeled
by
a large eddy simulation with coupled microphysics and aqueous chemistry, J.
Geophys. Res.-Atmos., 107, AAC 6–1–AAC 6–15,
https://doi.org/10.1029/2002JD002054, 2002. a, b, c
Flossmann, A.: A 2-D spectral model simulation of the scavenging of gaseous
and
particulate sulfate by a warm marine cloud, Atmos. Res., 32, 233–248,
https://doi.org/10.1016/0169-8095(94)90063-9, 1994. a, b
Genfa, Z., Dasgupta, P. K., Frick, G. M., and Hoppel, W. A.: Airship
Measurements of Hydrogen Peroxide and Related Parameters in the Marine
Atmosphere Along the Western U.S. Coast, Microchem. J., 62, 99–113,
https://doi.org/10.1006/mchj.1999.1715, 1999. a
Ghan, S., Easter, R., Hudson, J., and Bréon, F.-M.: Evaluation of aerosol
indirect radiative forcing in MIRAGE, J. Geophys. Res., 106, 5317–5334,
https://doi.org/10.1029/2000JD900501, 2001. a
GitHub: adiabatic parcel model based on libcloudph++,
available at: https://github.com/igfuw/parcel,
last access: 27 August 2018.
Grabowski, W. W. and Abade, G. C.: Broadening of Cloud Droplet Spectra
through
Eddy Hopping: Turbulent Adiabatic Parcel Simulations, J.
Atmos. Sci., 74, 1485–1493, https://doi.org/10.1175/JAS-D-17-0043.1, 2017. a
Grabowski, W. W., Dziekan, P., and Pawlowska, H.: Lagrangian condensation
microphysics with Twomey CCN activation, Geosci. Model Dev., 11,
103–120, https://doi.org/10.5194/gmd-11-103-2018, 2018. a
Hall, W.: A Detailed Microphysical Model Within a Two-Dimensional Dynamic
Framework: Model Description and Preliminary Results, J. Atmos. Sci., 37,
2486–2507, https://doi.org/10.1175/1520-0469(1980)037<2486:ADMMWA>2.0.CO;2, 1980. a, b, c
Hoffmann, F.: On the limits of Köhler activation theory: how do collision
and coalescence affect the activation of aerosols?, Atmos. Chem. Phys., 17,
8343–8356, https://doi.org/10.5194/acp-17-8343-2017, 2017. a
Hoffmann, M. and Calvert, J.: Chemical Transformation Modules for Eulerian
Acid
Deposition Models: Volume II, the Aqueous-phase Chemistry, U.S. Environmental
Protection Agency, Research Triangle Park, NC, 1985. a
Hoppel, W. A., Frick, G. M., and Larson, R. E.: Effect of nonprecipitating
clouds on the aerosol size distribution in the marine boundary layer,
Geophys. Res. Lett., 13, 125–128, https://doi.org/10.1029/GL013i002p00125, 1986. a
Hoppel, W. A., Frick, G. M., Fitzgerald, J. W., and Larson, R. E.: Marine
boundary layer measurements of new particle formation and the effects
nonprecipitating clouds have on aerosol size distribution, J. Geophys.
Res.-Atmos., 99, 14443–14459, https://doi.org/10.1029/94JD00797, 1994. a, b
Hudson, J. G., Noble, S., and Tabor, S.: Cloud supersaturations from CCN
spectra Hoppel minima, J. of Geophys. Res.-Atmos., 120, 3436–3452,
https://doi.org/10.1002/2014JD022669, 2015. a, b
Jaruga, A., Arabas, S., Jarecka, D., Pawlowska, H., Smolarkiewicz, P. K., and
Waruszewski, M.: libmpdata++ 1.0: a library of parallel MPDATA solvers for
systems of generalised transport equations, Geosci. Model Dev., 8,
1005–1032, https://doi.org/10.5194/gmd-8-1005-2015, 2015. a
Kessler, E.: On the continuity and distribution of water substance in
atmospheric circulations, Atmos. Res., 38, 109–145,
https://doi.org/10.1016/0169-8095(94)00090-Z, 1995. a
Kim, J., Ahlm, L., Yli-Juuti, T., Lawler, M., Keskinen, H., Tröstl, J.,
Schobesberger, S., Duplissy, J., Amorim, A., Bianchi, F., Donahue, N. M.,
Flagan, R. C., Hakala, J., Heinritzi, M., Jokinen, T., Kürten, A.,
Laaksonen, A., Lehtipalo, K., Miettinen, P., Petäjä, T., Rissanen, M. P.,
Rondo, L., Sengupta, K., Simon, M., Tomé, A., Williamson, C., Wimmer, D.,
Winkler, P. M., Ehrhart, S., Ye, P., Kirkby, J., Curtius, J., Baltensperger,
U., Kulmala, M., Lehtinen, K. E. J., Smith, J. N., Riipinen, I., and
Virtanen, A.: Hygroscopicity of nanoparticles produced from homogeneous
nucleation in the CLOUD experiments, Atmos. Chem. Phys., 16, 293–304,
https://doi.org/10.5194/acp-16-293-2016, 2016. a
Kreidenweis, S., Walcek, C., Feingold, G., Gong, W., Jacobson, M., Kim, C.,
Liu, X., Penner, J., Nenes, A., and Seinfeld, J.: Modification of aerosol
mass and size distribution due to aqueous-phase SO2 oxidation in clouds:
Comparisons of several models, J. Geophys. Res.-Atmos., 108,
https://doi.org/10.1029/2002JD002697, 2003. a, b, c, d, e, f, g, h, i, j, k, l, m, n, o, p, q
Ladino, L., Stetzer, O., Hattendorf, B., Günther, D., Croft, B., and
Lohmann,
U.: Experimental Study of Collection Efficiencies between Submicron Aerosols
and Cloud Droplets, J. Atmos. Sci., 68, 1853–1864,
https://doi.org/10.1175/JAS-D-11-012.1, 2011. a
Lebo, Z. J. and Seinfeld, J. H.: A continuous spectral aerosol-droplet
microphysics model, Atmos. Chem. Phys., 11, 12297–12316,
https://doi.org/10.5194/acp-11-12297-2011, 2011. a
Lee, J., Noh, Y., Raasch, S., Riechelmann, T., and Wang, L.: Investigation of
droplet dynamics in a convective cloud using a Lagrangian cloud model,
Meteor. Atmos. Phys., 124, 1–21, https://doi.org/10.1007/s00703-014-0311-y, 2014. a
Li, X.-Y., Brandenburg, A., Haugen, N. E. L., and Svensson, G.: Eulerian and
Lagrangian approaches to multidimensional condensation and collection, J.
Adv. Model. Earth Syst., 9, 1116–1137, https://doi.org/10.1002/2017MS000930, 2017. a
Massman, W. J.: A review of the molecular diffusivities of H2O, CO2, CH4, CO,
O3, SO2, NH3, N2O, NO, and NO2
in air, O2 and N2 near STP, Atmos. Environ.,
32, 1111–1127, https://doi.org/10.1016/S1352-2310(97)00391-9, 1998. a
Morrison, H. and Grabowski, W.: Comparison of Bulk and Bin Warm-Rain
Microphysics Models Using a Kinematic Framework, J. Atmos. Sci., 64,
2839–2861, https://doi.org/10.1175/JAS3980, 2007. a, b, c
Muhlbauer, A., Grabowski, W. W., Malinowski, S. P., Ackerman, T. P., Bryan,
G. H., Lebo, Z. J., Milbrandt, J. A., Morrison, H., Ovchinnikov, M.,
Tessendorf, S., Thériault, J. M., and Thompson, G.: Reexamination of the
State-of-the-art of Cloud Modeling Shows Real Improvements, Bull. Amer.
Meteor. Soc., 94, ES45–ES48, https://doi.org/10.1175/BAMS-D-12-00188.1, 2013. a
Myhre, G., Shindell, D., Bréon, F.-M., Collins, W., Fuglestvedt, J.,
Huang,
J., Koch, D., Lamarque, J.-F., Lee, D., Mendoza, B., Nakajima, T., Robock,
A., Stephens, G., Takemura, T., and Zhang, H.: Anthropogenic and Natural
Radiative Forcing, book section 8, 659–740, Cambridge University Press,
Cambridge, United Kingdom and New York, NY, USA,
https://doi.org/10.1017/CBO9781107415324.018, 2013. a
Naumann, A. K. and Seifert, A.: A Lagrangian drop model to study warm rain
microphysical processes in shallow cumulus, J. Adv. Model. Earth Syst., 7,
1136–1154, https://doi.org/10.1002/2015MS000456, 2015. a
Ovchinnikov, M. and Easter, R.: Modeling aerosol growth by aqueous chemistry
in a nonprecipitating stratiform cloud, J. Geophys. Res.-Atmos., 115,
D14, https://doi.org/10.1029/2009JD012816, 2010. a, b, c, d
Pawlowska, H. and Brenguier, J.-L.: An observational study of drizzle
formation
in stratocumulus clouds for general circulation model (GCM)
parameterizations, J. Geophys. Res.-Atmos., 108, D15, https://doi.org/10.1029/2002JD002679, 2003. a
Pawlowska, H., Brenguier, J., and Burnet, F.: Microphysical properties of
stratocumulus clouds, Atmos. Res., 55, 15–33,
https://doi.org/10.1016/S0169-8095(00)00054-5, 2000. a
Petters, M. and Kreidenweis, S.: A single parameter representation of
hygroscopic growth and cloud condensation nucleus activity, Atmos. Chem.
Phys., 7, 1961–1971, https://doi.org/10.5194/acp-8-6273-2008, 2007. a, b, c, d
Pinsky, M., Khain, A., and Krugliak, H.: Collisions of Cloud Droplets in a
Turbulent Flow. Part V: Application of Detailed Tables of Turbulent Collision
Rate Enhancement to Simulation of Droplet Spectra Evolution, J. Atmos. Sci.,
65, 357–374, https://doi.org/10.1175/2007JAS2358.1, 2008. a, b, c
Pruppacher, H. and Jaenicke, R.: The processing of water vapor and aerosols
by atmospheric clouds, a global estimate, Atmos. Res., 38, 283–295,
https://doi.org/10.1016/0169-8095(94)00098-X, 1995. a
Rasinski, P., Pawlowska, H., and Grabowski, W.: Observations and kinematic
modeling of drizzling marine stratocumulus, Atmos. Res., 102, 120–135,
https://doi.org/10.1016/j.atmosres.2011.06.020, 2011. a
Riechelmann, T., Noh, Y., and Raasch, S.: A new method for large-eddy
simulations of clouds with Lagrangian droplets including the effects of
turbulent collision, New J. Phys., 14, 065008,
https://doi.org/10.1088/1367-2630/14/6/065008, 2012. a
Rosenfeld, D. and Gutman, G.: Retrieving microphysical properties near the
tops of potential rain clouds by multispectral analysis of AVHRR data, Atmos.
Res., 34, 259–283, https://doi.org/10.1016/0169-8095(94)90096-5, 1994. a
Sardina, G., Poulain, S., Brandt, L., and Caballero, R.: Broadening of Cloud
Droplet Size Spectra by Stochastic Condensation: Effects of Mean Updraft
Velocity and CCN Activation, J. Atmos. Sci., 75, 451–467,
https://doi.org/10.1175/JAS-D-17-0241.1, 2018. a
Sato, Y., Shima, S., and Tomita, H.: A grid refinement study of trade wind
cumuli simulated by a Lagrangian cloud microphysical model: the super-droplet
method, Atmos. Sci. Lett., 18, 359–365, https://doi.org/10.1002/asl.764, 2017. a
Seifert, A. and Beheng, K. D.: A double-moment parameterization for
simulating
autoconversion, accretion and selfcollection, Atmos. Res., 59–60, 265–281,
https://doi.org/10.1016/S0169-8095(01)00126-0, 2001. a
Shima, S., Kusano, K., Kawano, A., Sugiyama, T., and Kawahara, S.: The
super-droplet method for the numerical simulation of clouds and
precipitation: a particle-based and probabilistic microphysics model coupled
with a non-hydrostatic model, Q. J. Roy. Meteorol. Soc., 135, 1307–1320,
https://doi.org/10.1002/qj.441, 2009. a, b, c
Sölch, I. and Kärcher, B.: A large-eddy model for cirrus clouds with
explicit aerosol and ice microphysics and Lagrangian ice particle tracking,
Q. J. Roy. Meteorol. Soc., 136, 2074–2093, https://doi.org/10.1002/qj.689, 2010. a
Stroustrup, B.: C++ Programming Language, Addison-Wesley Professional,
fourth Edn., 2013. a
Szumowski, M., Grabowski, W., and Ochs III, H.: Simple two-dimensional
kinematic framework designed to test warm rain microphysical models, Atmos.
Res., 45, 299–326, https://doi.org/10.1016/S0169-8095(97)00082-3, 1998. a
Tang, M. J., Cox, R. A., and Kalberer, M.: Compilation and evaluation of gas
phase diffusion coefficients of reactive trace gases in the atmosphere:
volume 1. Inorganic compounds, Atmos. Chem. Phys., 14, 9233–9247,
https://doi.org/10.5194/acp-14-9233-2014, 2014. a
Twohy, C. H., Austin, P. H., and Charlson, R. J.: Chemical consequences of
the
initial diffusional growth of cloud droplets: a clean marine case, Tellus B,
41B, 51–60, https://doi.org/10.1111/j.1600-0889.1989.tb00124.x, 1989. a
Unterstrasser, S. and Sölch, I.: Optimisation of the simulation particle
number in a Lagrangian ice microphysical model, Geosci. Model Dev., 7,
695–709, https://doi.org/10.5194/gmd-7-695-2014, 2014. a
Unterstrasser, S., Hoffmann, F., and Lerch, M.: Collection/aggregation
algorithms in Lagrangian cloud microphysical models: rigorous evaluation in
box model simulations, Geosci. Model Dev., 10, 1521–1548,
https://doi.org/10.5194/gmd-10-1521-2017, 2017. a
van 't Hoff, J. H.: L'équilibre chimique dans les systèmes gazeux on
dissous à l'état dilué, Recueil des Travaux Chimiques des Pays-Bas, 4, 424–427,
https://doi.org/10.1002/recl.18850041207, 1885. a
von Glasow, R. and Sander, R.: Variation of sea salt aerosol pH with relative
humidity, Geophys. Res. Lett., 28, 247–250, https://doi.org/10.1029/2000GL012387,
2001. a
Walcek, C. J. and Taylor, G. R.: A Theoretical Method for Computing Vertical
Distributions of Acidity and Sulfate Production within Cumulus Clouds, J.
Atmos. Sci., 43, 339–355,
https://doi.org/10.1175/1520-0469(1986)043<0339:ATMFCV>2.0.CO;2, 1986. a
Wang, G., Zhang, R., Gomez, M. E., Yang, L., Levy Zamora, M., Hu, M., Lin,
Y.,
Peng, J., Guo, S., Meng, J., Li, J., Cheng, C., Hu, T., Ren, Y., Wang, Y.,
Gao, J., Cao, J., An, Z., Zhou, W., Li, G., Wang, J., Tian, P.,
Marrero-Ortiz, W., Secrest, J., Du, Z., Zheng, J., Shang, D., Zeng, L., Shao,
M., Wang, W., Huang, Y., Wang, Y., Zhu, Y., Li, Y., Hu, J., Pan, B., Cai, L.,
Cheng, Y., Ji, Y., Zhang, F., Rosenfeld, D., Liss, P. S., Duce, R. A., Kolb,
C. E., and Molina, M. J.: Persistent sulfate formation from London Fog to
Chinese haze, Proc. Natl. Acad. Sci. USA, https://doi.org/10.1073/pnas.1616540113,
2016. a
Wang, J., Lee, Y.-N., Daum, P. H., Jayne, J., and Alexander, M. L.: Effects
of aerosol organics on cloud condensation nucleus (CCN) concentration and first
indirect aerosol effect, Atmos. Chem. Phys., 8, 6325–6339,
https://doi.org/10.5194/acp-8-6325-2008, 2008. a
Warneck, P.: Chemistry of the Natural Atmosphere, vol. 71 of International Geophysics Series, Academic Press, second edn., 1999. a
Werner, F., Ditas, F., Siebert, H., Simmel, M., Wehner, B., Pilewskie, P.,
Schmeissner, T., Shaw, R. A., Hartmann, S., Wex, H., Roberts, G. C., and
Wendisch, M.: Twomey effect observed from collocated microphysical and remote
sensing measurements over shallow cumulus, J. Geophys. Res.-Atmos., 119,
1534–1545, https://doi.org/10.1002/2013JD020131, 2014. a
Zhang, Q., Jimenez, J. L., Canagaratna, M. R., Allan, J. D., Coe, H.,
Ulbrich,
I., Alfarra, M. R., Takami, A., Middlebrook, A. M., Sun, Y. L., Dzepina, K.,
Dunlea, E., Docherty, K., DeCarlo, P. F., Salcedo, D., Onasch, T., Jayne,
J. T., Miyoshi, T., Shimono, A., Hatakeyama, S., Takegawa, N., Kondo, Y.,
Schneider, J., Drewnick, F., Borrmann, S., Weimer, S., Demerjian, K.,
Williams, P., Bower, K., Bahreini, R., Cottrell, L., Griffin, R. J.,
Rautiainen, J., Sun, J. Y., Zhang, Y. M., and Worsnop, D. R.: Ubiquity and
dominance of oxygenated species in organic aerosols in
anthropogenically-influenced Northern Hemisphere midlatitudes, Geophys. Res.
Lett., 34, l13801, https://doi.org/10.1029/2007GL029979, 2007.
a
Zhang, Y., Kreidenweis, S. M., and Feingold, G.: Stratocumulus processing of
gases and cloud condensation nuclei: 2. Chemistry sensitivity analysis, J.
Geophys. Res.-Atmos., 104, 16061–16080, https://doi.org/10.1029/1999JD900206,
1999. a, b
Short summary
libcloudph++ is a free and open-source library of schemes representing cloud microphysics (e.g. condensation of water vapour into cloud droplets, collisions between water drops, precipitation) in numerical models. This work adds new schemes that represent aqueous chemical reactions in water drops. The schemes focus on the oxidation of SO2 by O3 and H2O2. The libcloudph++ is now capable of resolving the changes in aerosol sizes caused by both collisions between water drops and aqueous oxidation.
libcloudph++ is a free and open-source library of schemes representing cloud microphysics (e.g....
