Articles | Volume 10, issue 1
https://doi.org/10.5194/gmd-10-169-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/gmd-10-169-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Model description paper
| 
13 Jan 2017
Model description paper |
| 13 Jan 2017
UCLALES–SALSA v1.0: a large-eddy model with interactive sectional microphysics for aerosol, clouds and precipitation
Karlsruhe Institute of Technology, Karlsruhe, Germany
Finnish Meteorological Institute, Atmospheric Research Centre of Eastern Finland, P.O. Box 1627, 70211 Kuopio, Finland
Zubair Maalick
Department of Applied Physics, University of Eastern Finland, P.O. Box 1627, 70211 Kuopio, Finland
Tomi Raatikainen
Finnish Meteorological Institute, P.O. Box 503, 00101 Helsinki, Finland
Harri Kokkola
Finnish Meteorological Institute, Atmospheric Research Centre of Eastern Finland, P.O. Box 1627, 70211 Kuopio, Finland
Thomas Kühn
Finnish Meteorological Institute, Atmospheric Research Centre of Eastern Finland, P.O. Box 1627, 70211 Kuopio, Finland
Department of Applied Physics, University of Eastern Finland, P.O. Box 1627, 70211 Kuopio, Finland
Sami Romakkaniemi
Finnish Meteorological Institute, Atmospheric Research Centre of Eastern Finland, P.O. Box 1627, 70211 Kuopio, Finland
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We use a numerical model to study interactions between humid light-absorbing aerosol plumes, clouds, and radiation over the southeast Atlantic. We find that the warming produced by the aerosols reduces cloud cover, especially in highly polluted situations. Aerosol impacts on drizzle play a minor role. However, aerosol effects on cloud reflectivity and moisture-induced changes in cloud cover dominate the climatic response and lead to an overall cooling by the biomass burning plumes.
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Our results show that the global model is stable and it provides meaningful results. This way we can include a physics-based presentation of sub-grid physics (physics which happens on a 100 m scale) in the global model, whose resolution is on a 100 km scale.
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The spatial and temporal restrictions of observations and oversimplified aerosol representation in large eddy simulations (LES) limit our understanding of aerosol–stratocumulus interactions. In this closure study of in situ and remote sensing observations and outputs from UCLALES–SALSA, we have assessed the role of convective overturning and aerosol effects in two cloud events observed at the Puijo SMEAR IV station, Finland, a diurnal-high aerosol case and a nocturnal-low aerosol case.
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Aerosols and clouds persist as the dominant sources of uncertainty in climate projections. In this modelling study, we investigate the role of marine aerosols in influencing the lifetime of low-level clouds. Our high resolution simulations show that sea spray can both extend and shorten the lifetime of the cloud layer depending on the model setup. The impact of the primary marine organics is relatively limited while secondary aerosol from monoterpenes can have larger impact.
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Juha Tonttila, Ali Afzalifar, Harri Kokkola, Tomi Raatikainen, Hannele Korhonen, and Sami Romakkaniemi
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J. Tonttila, H. Järvinen, and P. Räisänen
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S. V. Henriksson, J.-P. Pietikäinen, A.-P. Hyvärinen, P. Räisänen, K. Kupiainen, J. Tonttila, R. Hooda, H. Lihavainen, D. O'Donnell, L. Backman, Z. Klimont, and A. Laaksonen
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Harri Kokkola, Juha Tonttila, Silvia Calderón, Sami Romakkaniemi, Antti Lipponen, Aapo Peräkorpi, Tero Mielonen, Edward Gryspeerdt, Timo H. Virtanen, Pekka Kolmonen, and Antti Arola
EGUsphere, https://doi.org/10.5194/egusphere-2024-1964, https://doi.org/10.5194/egusphere-2024-1964, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Mariya Petrenko, Ralph Kahn, Mian Chin, Susanne E. Bauer, Tommi Bergman, Huisheng Bian, Gabriele Curci, Ben Johnson, Johannes Kaiser, Zak Kipling, Harri Kokkola, Xiaohong Liu, Keren Mezuman, Tero Mielonen, Gunnar Myhre, Xiaohua Pan, Anna Protonotariou, Samuel Remy, Ragnhild Bieltvedt Skeie, Philip Stier, Toshihiko Takemura, Kostas Tsigaridis, Hailong Wang, Duncan Watson-Parris, and Kai Zhang
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Marje Prank, Juha Tonttila, Xiaoxia Shang, Sami Romakkaniemi, and Tomi Raatikainen
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Large primary bioparticles such as pollen can be abundant in the atmosphere. In humid conditions pollens can rupture and release a large number of fine sub-pollen particles (SPPs). The paper investigates what kind of birch pollen concentrations are needed for the pollen and SPPs to start playing a noticeable role in cloud processes and alter precipitation formation. In the studied cases only the largest observed pollen concentrations were able to noticeably alter the precipitation formation.
Anton Laakso, Daniele Visioni, Ulrike Niemeier, Simone Tilmes, and Harri Kokkola
Earth Syst. Dynam., 15, 405–427, https://doi.org/10.5194/esd-15-405-2024, https://doi.org/10.5194/esd-15-405-2024, 2024
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This study is the second in a two-part series in which we explore the dependency of the impacts of stratospheric sulfur injections on both the model employed and the strategy of injection utilized. The study uncovers uncertainties associated with these techniques to cool climate, highlighting how the simulated climate impacts are dependent on both the selected model and the magnitude of the injections. We also show that estimating precipitation impacts of aerosol injection is a complex task.
Alejandro Baró Pérez, Michael S. Diamond, Frida A.-M. Bender, Abhay Devasthale, Matthias Schwarz, Julien Savre, Juha Tonttila, Harri Kokkola, Hyunho Lee, David Painemal, and Annica M. L. Ekman
Atmos. Chem. Phys., 24, 4591–4610, https://doi.org/10.5194/acp-24-4591-2024, https://doi.org/10.5194/acp-24-4591-2024, 2024
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We use a numerical model to study interactions between humid light-absorbing aerosol plumes, clouds, and radiation over the southeast Atlantic. We find that the warming produced by the aerosols reduces cloud cover, especially in highly polluted situations. Aerosol impacts on drizzle play a minor role. However, aerosol effects on cloud reflectivity and moisture-induced changes in cloud cover dominate the climatic response and lead to an overall cooling by the biomass burning plumes.
Kalle Nordling, Jukka-Pekka Keskinen, Sami Romakkaniemi, Harri Kokkola, Petri Räisänen, Antti Lipponen, Antti-Ilari Partanen, Jaakko Ahola, Juha Tonttila, Muzaffer Ege Alper, Hannele Korhonen, and Tomi Raatikainen
Atmos. Chem. Phys., 24, 869–890, https://doi.org/10.5194/acp-24-869-2024, https://doi.org/10.5194/acp-24-869-2024, 2024
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Our results show that the global model is stable and it provides meaningful results. This way we can include a physics-based presentation of sub-grid physics (physics which happens on a 100 m scale) in the global model, whose resolution is on a 100 km scale.
Muhammed Irfan, Thomas Kühn, Taina Yli-Juuti, Anton Laakso, Eemeli Holopainen, Douglas R. Worsnop, Annele Virtanen, and Harri Kokkola
EGUsphere, https://doi.org/10.5194/egusphere-2023-2768, https://doi.org/10.5194/egusphere-2023-2768, 2023
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Tuuli Miinalainen, Harri Kokkola, Antti Lipponen, Antti-Pekka Hyvärinen, Vijay Kumar Soni, Kari E. J. Lehtinen, and Thomas Kühn
Atmos. Chem. Phys., 23, 3471–3491, https://doi.org/10.5194/acp-23-3471-2023, https://doi.org/10.5194/acp-23-3471-2023, 2023
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We simulated the effects of aerosol emission mitigation on both global and regional radiative forcing and city-level air quality with a global-scale climate model. We used a machine learning downscaling approach to bias-correct the PM2.5 values obtained from the global model for the Indian megacity New Delhi. Our results indicate that aerosol mitigation could result in both improved air quality and less radiative heating for India.
Ville Leinonen, Harri Kokkola, Taina Yli-Juuti, Tero Mielonen, Thomas Kühn, Tuomo Nieminen, Simo Heikkinen, Tuuli Miinalainen, Tommi Bergman, Ken Carslaw, Stefano Decesari, Markus Fiebig, Tareq Hussein, Niku Kivekäs, Radovan Krejci, Markku Kulmala, Ari Leskinen, Andreas Massling, Nikos Mihalopoulos, Jane P. Mulcahy, Steffen M. Noe, Twan van Noije, Fiona M. O'Connor, Colin O'Dowd, Dirk Olivie, Jakob B. Pernov, Tuukka Petäjä, Øyvind Seland, Michael Schulz, Catherine E. Scott, Henrik Skov, Erik Swietlicki, Thomas Tuch, Alfred Wiedensohler, Annele Virtanen, and Santtu Mikkonen
Atmos. Chem. Phys., 22, 12873–12905, https://doi.org/10.5194/acp-22-12873-2022, https://doi.org/10.5194/acp-22-12873-2022, 2022
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We provide the first extensive comparison of detailed aerosol size distribution trends between in situ observations from Europe and five different earth system models. We investigated aerosol modes (nucleation, Aitken, and accumulation) separately and were able to show the differences between measured and modeled trends and especially their seasonal patterns. The differences in model results are likely due to complex effects of several processes instead of certain specific model features.
Silvia M. Calderón, Juha Tonttila, Angela Buchholz, Jorma Joutsensaari, Mika Komppula, Ari Leskinen, Liqing Hao, Dmitri Moisseev, Iida Pullinen, Petri Tiitta, Jian Xu, Annele Virtanen, Harri Kokkola, and Sami Romakkaniemi
Atmos. Chem. Phys., 22, 12417–12441, https://doi.org/10.5194/acp-22-12417-2022, https://doi.org/10.5194/acp-22-12417-2022, 2022
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The spatial and temporal restrictions of observations and oversimplified aerosol representation in large eddy simulations (LES) limit our understanding of aerosol–stratocumulus interactions. In this closure study of in situ and remote sensing observations and outputs from UCLALES–SALSA, we have assessed the role of convective overturning and aerosol effects in two cloud events observed at the Puijo SMEAR IV station, Finland, a diurnal-high aerosol case and a nocturnal-low aerosol case.
Sini Isokääntä, Paul Kim, Santtu Mikkonen, Thomas Kühn, Harri Kokkola, Taina Yli-Juuti, Liine Heikkinen, Krista Luoma, Tuukka Petäjä, Zak Kipling, Daniel Partridge, and Annele Virtanen
Atmos. Chem. Phys., 22, 11823–11843, https://doi.org/10.5194/acp-22-11823-2022, https://doi.org/10.5194/acp-22-11823-2022, 2022
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This research employs air mass history analysis and observations to study how clouds and precipitation affect atmospheric aerosols during transport to a boreal forest site. The mass concentrations of studied chemical species showed exponential decrease as a function of accumulated rain along the air mass route. Our analysis revealed in-cloud sulfate formation, while no major changes in organic mass were seen. Most of the in-cloud-formed sulfate could be assigned to particle sizes above 200 nm.
Qirui Zhong, Nick Schutgens, Guido van der Werf, Twan van Noije, Kostas Tsigaridis, Susanne E. Bauer, Tero Mielonen, Alf Kirkevåg, Øyvind Seland, Harri Kokkola, Ramiro Checa-Garcia, David Neubauer, Zak Kipling, Hitoshi Matsui, Paul Ginoux, Toshihiko Takemura, Philippe Le Sager, Samuel Rémy, Huisheng Bian, Mian Chin, Kai Zhang, Jialei Zhu, Svetlana G. Tsyro, Gabriele Curci, Anna Protonotariou, Ben Johnson, Joyce E. Penner, Nicolas Bellouin, Ragnhild B. Skeie, and Gunnar Myhre
Atmos. Chem. Phys., 22, 11009–11032, https://doi.org/10.5194/acp-22-11009-2022, https://doi.org/10.5194/acp-22-11009-2022, 2022
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Aerosol optical depth (AOD) errors for biomass burning aerosol (BBA) are evaluated in 18 global models against satellite datasets. Notwithstanding biases in satellite products, they allow model evaluations. We observe large and diverse model biases due to errors in BBA. Further interpretations of AOD diversities suggest large biases exist in key processes for BBA which require better constraining. These results can contribute to further model improvement and development.
Marje Prank, Juha Tonttila, Jaakko Ahola, Harri Kokkola, Thomas Kühn, Sami Romakkaniemi, and Tomi Raatikainen
Atmos. Chem. Phys., 22, 10971–10992, https://doi.org/10.5194/acp-22-10971-2022, https://doi.org/10.5194/acp-22-10971-2022, 2022
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Aerosols and clouds persist as the dominant sources of uncertainty in climate projections. In this modelling study, we investigate the role of marine aerosols in influencing the lifetime of low-level clouds. Our high resolution simulations show that sea spray can both extend and shorten the lifetime of the cloud layer depending on the model setup. The impact of the primary marine organics is relatively limited while secondary aerosol from monoterpenes can have larger impact.
Petri Tiitta, Ari Leskinen, Ville A. Kaikkonen, Eero O. Molkoselkä, Anssi J. Mäkynen, Jorma Joutsensaari, Silvia Calderon, Sami Romakkaniemi, and Mika Komppula
Atmos. Meas. Tech., 15, 2993–3009, https://doi.org/10.5194/amt-15-2993-2022, https://doi.org/10.5194/amt-15-2993-2022, 2022
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The novel holographic imaging instrument (ICEMET) was adapted to measure the microphysical properties of liquid clouds, and these values were compared with parallel measurements of a cloud droplet spectrometer (FM-120) and particle measurements using a twin-inlet system. When the intercomparison was carried out during isoaxial sampling, our results showed good agreement in terms of variability between the instruments. This agreement was confirmed using Mutual and Pearson correlation analyses.
Cynthia H. Whaley, Rashed Mahmood, Knut von Salzen, Barbara Winter, Sabine Eckhardt, Stephen Arnold, Stephen Beagley, Silvia Becagli, Rong-You Chien, Jesper Christensen, Sujay Manish Damani, Xinyi Dong, Konstantinos Eleftheriadis, Nikolaos Evangeliou, Gregory Faluvegi, Mark Flanner, Joshua S. Fu, Michael Gauss, Fabio Giardi, Wanmin Gong, Jens Liengaard Hjorth, Lin Huang, Ulas Im, Yugo Kanaya, Srinath Krishnan, Zbigniew Klimont, Thomas Kühn, Joakim Langner, Kathy S. Law, Louis Marelle, Andreas Massling, Dirk Olivié, Tatsuo Onishi, Naga Oshima, Yiran Peng, David A. Plummer, Olga Popovicheva, Luca Pozzoli, Jean-Christophe Raut, Maria Sand, Laura N. Saunders, Julia Schmale, Sangeeta Sharma, Ragnhild Bieltvedt Skeie, Henrik Skov, Fumikazu Taketani, Manu A. Thomas, Rita Traversi, Kostas Tsigaridis, Svetlana Tsyro, Steven Turnock, Vito Vitale, Kaley A. Walker, Minqi Wang, Duncan Watson-Parris, and Tahya Weiss-Gibbons
Atmos. Chem. Phys., 22, 5775–5828, https://doi.org/10.5194/acp-22-5775-2022, https://doi.org/10.5194/acp-22-5775-2022, 2022
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Air pollutants, like ozone and soot, play a role in both global warming and air quality. Atmospheric models are often used to provide information to policy makers about current and future conditions under different emissions scenarios. In order to have confidence in those simulations, in this study we compare simulated air pollution from 18 state-of-the-art atmospheric models to measured air pollution in order to assess how well the models perform.
Jaakko Ahola, Tomi Raatikainen, Muzaffer Ege Alper, Jukka-Pekka Keskinen, Harri Kokkola, Antti Kukkurainen, Antti Lipponen, Jia Liu, Kalle Nordling, Antti-Ilari Partanen, Sami Romakkaniemi, Petri Räisänen, Juha Tonttila, and Hannele Korhonen
Atmos. Chem. Phys., 22, 4523–4537, https://doi.org/10.5194/acp-22-4523-2022, https://doi.org/10.5194/acp-22-4523-2022, 2022
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Clouds are important for the climate, and cloud droplets have a significant role in cloud properties. Cloud droplets form when air rises and cools and water vapour condenses on small particles that can be natural or of anthropogenic origin. Currently, the updraft velocity, meaning how fast the air rises, is poorly represented in global climate models. In our study, we show three methods that will improve the depiction of updraft velocity and which properties are vital to updrafts.
Tomi Raatikainen, Marje Prank, Jaakko Ahola, Harri Kokkola, Juha Tonttila, and Sami Romakkaniemi
Atmos. Chem. Phys., 22, 3763–3778, https://doi.org/10.5194/acp-22-3763-2022, https://doi.org/10.5194/acp-22-3763-2022, 2022
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Mineral dust or similar ice-nucleating particles (INPs) are needed to initiate cloud droplet freezing at temperatures common in shallow clouds. In this work we examine how INPs that are released from the sea surface impact marine clouds. Our high-resolution simulations show that turbulent updraughts carry these particles effectively up to the clouds, where they initiate cloud droplet freezing. Sea surface INP emissions become more important with decreasing background dust INP concentrations.
Jessica Slater, Hugh Coe, Gordon McFiggans, Juha Tonttila, and Sami Romakkaniemi
Atmos. Chem. Phys., 22, 2937–2953, https://doi.org/10.5194/acp-22-2937-2022, https://doi.org/10.5194/acp-22-2937-2022, 2022
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This paper shows the specific impact of black carbon (BC) on the aerosol–planetary boundary layer (PBL) feedback and its influence on a Beijing haze episode. Overall, this paper shows that strong temperature inversions prevent BC heating within the PBL from significantly increasing PBL height, while BC above the PBL suppresses PBL development significantly through the day. From this we suggest a method by which both locally and regionally emitted BC may impact urban pollution episodes.
Ian Boutle, Wayne Angevine, Jian-Wen Bao, Thierry Bergot, Ritthik Bhattacharya, Andreas Bott, Leo Ducongé, Richard Forbes, Tobias Goecke, Evelyn Grell, Adrian Hill, Adele L. Igel, Innocent Kudzotsa, Christine Lac, Bjorn Maronga, Sami Romakkaniemi, Juerg Schmidli, Johannes Schwenkel, Gert-Jan Steeneveld, and Benoît Vié
Atmos. Chem. Phys., 22, 319–333, https://doi.org/10.5194/acp-22-319-2022, https://doi.org/10.5194/acp-22-319-2022, 2022
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Fog forecasting is one of the biggest problems for numerical weather prediction. By comparing many models used for fog forecasting with others used for fog research, we hoped to help guide forecast improvements. We show some key processes that, if improved, will help improve fog forecasting, such as how water is deposited on the ground. We also showed that research models were not themselves a suitable baseline for comparison, and we discuss what future observations are required to improve them.
Anton Laakso, Ulrike Niemeier, Daniele Visioni, Simone Tilmes, and Harri Kokkola
Atmos. Chem. Phys., 22, 93–118, https://doi.org/10.5194/acp-22-93-2022, https://doi.org/10.5194/acp-22-93-2022, 2022
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The use of different spatio-temporal sulfur injection strategies with different magnitudes to create an artificial reflective aerosol layer to cool the climate is studied using sectional and modal aerosol schemes in a climate model. There are significant differences in the results depending on the aerosol microphysical module used. Different spatio-temporal injection strategies have a significant impact on the magnitude and zonal distribution of radiative forcing and atmospheric dynamics.
Maria Sand, Bjørn H. Samset, Gunnar Myhre, Jonas Gliß, Susanne E. Bauer, Huisheng Bian, Mian Chin, Ramiro Checa-Garcia, Paul Ginoux, Zak Kipling, Alf Kirkevåg, Harri Kokkola, Philippe Le Sager, Marianne T. Lund, Hitoshi Matsui, Twan van Noije, Dirk J. L. Olivié, Samuel Remy, Michael Schulz, Philip Stier, Camilla W. Stjern, Toshihiko Takemura, Kostas Tsigaridis, Svetlana G. Tsyro, and Duncan Watson-Parris
Atmos. Chem. Phys., 21, 15929–15947, https://doi.org/10.5194/acp-21-15929-2021, https://doi.org/10.5194/acp-21-15929-2021, 2021
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Absorption of shortwave radiation by aerosols can modify precipitation and clouds but is poorly constrained in models. A total of 15 different aerosol models from AeroCom phase III have reported total aerosol absorption, and for the first time, 11 of these models have reported in a consistent experiment the contributions to absorption from black carbon, dust, and organic aerosol. Here, we document the model diversity in aerosol absorption.
Antti Ruuskanen, Sami Romakkaniemi, Harri Kokkola, Antti Arola, Santtu Mikkonen, Harri Portin, Annele Virtanen, Kari E. J. Lehtinen, Mika Komppula, and Ari Leskinen
Atmos. Chem. Phys., 21, 1683–1695, https://doi.org/10.5194/acp-21-1683-2021, https://doi.org/10.5194/acp-21-1683-2021, 2021
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The study focuses mainly on cloud-scavenging efficiency of absorbing particulate matter (mainly black carbon) but additionally covers cloud-scavenging efficiency of scattering particles and statistics of cloud condensation nuclei. The main findings give insight into how black carbon is distributed in different particle sizes and the sensitivity to cloud scavenged. The main findings are useful for large-scale modelling for evaluating cloud scavenging.
Juha Tonttila, Ali Afzalifar, Harri Kokkola, Tomi Raatikainen, Hannele Korhonen, and Sami Romakkaniemi
Atmos. Chem. Phys., 21, 1035–1048, https://doi.org/10.5194/acp-21-1035-2021, https://doi.org/10.5194/acp-21-1035-2021, 2021
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The focus of this study is on rain enhancement by deliberate injection of small particles into clouds (
cloud seeding). The particles, usually released from an aircraft, are expected to enhance cloud droplet growth, but its practical feasibility is somewhat uncertain. To improve upon this, we simulate the seeding effects with a numerical model. The model reproduces the main features seen in field observations, with a strong sensitivity to the total mass of the injected particle material.
Jonas Gliß, Augustin Mortier, Michael Schulz, Elisabeth Andrews, Yves Balkanski, Susanne E. Bauer, Anna M. K. Benedictow, Huisheng Bian, Ramiro Checa-Garcia, Mian Chin, Paul Ginoux, Jan J. Griesfeller, Andreas Heckel, Zak Kipling, Alf Kirkevåg, Harri Kokkola, Paolo Laj, Philippe Le Sager, Marianne Tronstad Lund, Cathrine Lund Myhre, Hitoshi Matsui, Gunnar Myhre, David Neubauer, Twan van Noije, Peter North, Dirk J. L. Olivié, Samuel Rémy, Larisa Sogacheva, Toshihiko Takemura, Kostas Tsigaridis, and Svetlana G. Tsyro
Atmos. Chem. Phys., 21, 87–128, https://doi.org/10.5194/acp-21-87-2021, https://doi.org/10.5194/acp-21-87-2021, 2021
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Simulated aerosol optical properties as well as the aerosol life cycle are investigated for 14 global models participating in the AeroCom initiative. Considerable diversity is found in the simulated aerosol species emissions and lifetimes, also resulting in a large diversity in the simulated aerosol mass, composition, and optical properties. A comparison with observations suggests that, on average, current models underestimate the direct effect of aerosol on the atmosphere radiation budget.
Xiaoxia Shang, Elina Giannakaki, Stephanie Bohlmann, Maria Filioglou, Annika Saarto, Antti Ruuskanen, Ari Leskinen, Sami Romakkaniemi, and Mika Komppula
Atmos. Chem. Phys., 20, 15323–15339, https://doi.org/10.5194/acp-20-15323-2020, https://doi.org/10.5194/acp-20-15323-2020, 2020
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Measurements of the multi-wavelength Raman polarization lidar PollyXT have been combined with measurements of pollen type and concentration using a traditional pollen sampler at a rural forest site in Kuopio, Finland. The depolarization ratio was enhanced when there were pollen grains in the atmosphere, illustrating the potential of lidar to track pollen grains in the atmosphere. The depolarization ratio of pure pollen particles was assessed for birch and pine pollen using a novel algorithm.
Eemeli Holopainen, Harri Kokkola, Anton Laakso, and Thomas Kühn
Geosci. Model Dev., 13, 6215–6235, https://doi.org/10.5194/gmd-13-6215-2020, https://doi.org/10.5194/gmd-13-6215-2020, 2020
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This paper introduces an in-cloud wet deposition scheme for liquid and ice phase clouds for global aerosol–climate models. With the default setup, our wet deposition scheme behaves spuriously and better representation can be achieved with this scheme when black carbon is mixed with soluble compounds at emission time. This work is done as many of the global models fail to reproduce the transport of black carbon to the Arctic, which may be due to the poor representation of wet removal in models.
Jessica Slater, Juha Tonttila, Gordon McFiggans, Paul Connolly, Sami Romakkaniemi, Thomas Kühn, and Hugh Coe
Atmos. Chem. Phys., 20, 11893–11906, https://doi.org/10.5194/acp-20-11893-2020, https://doi.org/10.5194/acp-20-11893-2020, 2020
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The feedback effect between aerosol particles, radiation and meteorology reduces turbulent motion and results in increased surface aerosol concentrations during Beijing haze. Observational analysis and regional modelling studies have examined the feedback effect but these studies are limited. In this work, we set up a high-resolution model for the Beijing environment to examine the sensitivity of the aerosol feedback effect to initial meteorological conditions and aerosol loading.
Jaakko Ahola, Hannele Korhonen, Juha Tonttila, Sami Romakkaniemi, Harri Kokkola, and Tomi Raatikainen
Atmos. Chem. Phys., 20, 11639–11654, https://doi.org/10.5194/acp-20-11639-2020, https://doi.org/10.5194/acp-20-11639-2020, 2020
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In this study, we present an improved cloud model that reproduces the behaviour of mixed-phase clouds containing liquid droplets and ice crystals in more detail than before. This model is a convenient computational tool that enables the study of phenomena that cannot fit into a laboratory. These clouds have a significant role in climate, but they are not yet properly understood. Here, we show the advantages of the new model in a case study focusing on Arctic mixed-phase clouds.
Konstantinos-Matthaios Doulgeris, Mika Komppula, Sami Romakkaniemi, Antti-Pekka Hyvärinen, Veli-Matti Kerminen, and David Brus
Atmos. Meas. Tech., 13, 5129–5147, https://doi.org/10.5194/amt-13-5129-2020, https://doi.org/10.5194/amt-13-5129-2020, 2020
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We intercompared three cloud spectrometers ground setups in conditions with frequently occurring supercooled clouds. The measurements were conducted during the Pallas Cloud Experiment (PaCE) in 2013, in the Finnish sub-Arctic region at Sammaltunturi station. The main meteorological parameters influencing the spectrometers' performance was the wind direction. Final recommendations and our view on the main limitations of each spectrometer ground setup are presented.
Innocent Kudzotsa, Harri Kokkola, Juha Tonttila, Tomi Raatikainen, and Sami Romakkaniemi
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-851, https://doi.org/10.5194/acp-2020-851, 2020
Publication in ACP not foreseen
María A. Burgos, Elisabeth Andrews, Gloria Titos, Angela Benedetti, Huisheng Bian, Virginie Buchard, Gabriele Curci, Zak Kipling, Alf Kirkevåg, Harri Kokkola, Anton Laakso, Julie Letertre-Danczak, Marianne T. Lund, Hitoshi Matsui, Gunnar Myhre, Cynthia Randles, Michael Schulz, Twan van Noije, Kai Zhang, Lucas Alados-Arboledas, Urs Baltensperger, Anne Jefferson, James Sherman, Junying Sun, Ernest Weingartner, and Paul Zieger
Atmos. Chem. Phys., 20, 10231–10258, https://doi.org/10.5194/acp-20-10231-2020, https://doi.org/10.5194/acp-20-10231-2020, 2020
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We investigate how well models represent the enhancement in scattering coefficients due to particle water uptake, and perform an evaluation of several implementation schemes used in ten Earth system models. Our results show the importance of the parameterization of hygroscopicity and model chemistry as drivers of some of the observed diversity amongst model estimates. The definition of dry conditions and the phenomena taking place in this relative humidity range also impact the model evaluation.
Maria Filioglou, Elina Giannakaki, John Backman, Jutta Kesti, Anne Hirsikko, Ronny Engelmann, Ewan O'Connor, Jari T. T. Leskinen, Xiaoxia Shang, Hannele Korhonen, Heikki Lihavainen, Sami Romakkaniemi, and Mika Komppula
Atmos. Chem. Phys., 20, 8909–8922, https://doi.org/10.5194/acp-20-8909-2020, https://doi.org/10.5194/acp-20-8909-2020, 2020
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Dust optical properties are region-dependent. Saharan, Asian, and Arabian dusts do not pose similar optical properties in terms of lidar ratios; thus, a universal lidar ratio for dust particles will lead to biases. The present study analyses observations over the United Arab Emirates, quantifying the optical and geometrical extents of the aerosol layers in the area, providing at the same time the Arabian dust properties along with chemical analysis of dust samples collected in the region.
Thomas Kühn, Kaarle Kupiainen, Tuuli Miinalainen, Harri Kokkola, Ville-Veikko Paunu, Anton Laakso, Juha Tonttila, Rita Van Dingenen, Kati Kulovesi, Niko Karvosenoja, and Kari E. J. Lehtinen
Atmos. Chem. Phys., 20, 5527–5546, https://doi.org/10.5194/acp-20-5527-2020, https://doi.org/10.5194/acp-20-5527-2020, 2020
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We investigate the effects of black carbon (BC) mitigation on Arctic climate and human health, accounting for the concurrent reduction of other aerosol species. While BC is attributed a net warming effect on climate, most other aerosol species cool the planet. We find that the direct radiative effect of mitigating BC induces cooling, while aerosol–cloud effects offset this cooling and introduce large uncertainties. Furthermore, the reduced aerosol emissions reduce human mortality considerably.
Giulia Saponaro, Moa K. Sporre, David Neubauer, Harri Kokkola, Pekka Kolmonen, Larisa Sogacheva, Antti Arola, Gerrit de Leeuw, Inger H. H. Karset, Ari Laaksonen, and Ulrike Lohmann
Atmos. Chem. Phys., 20, 1607–1626, https://doi.org/10.5194/acp-20-1607-2020, https://doi.org/10.5194/acp-20-1607-2020, 2020
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The understanding of cloud processes is based on the quality of the representation of cloud properties. We compared cloud parameters from three models with satellite observations. We report on the performance of each data source, highlighting strengths and deficiencies, which should be considered when deriving the effect of aerosols on cloud properties.
Stephanie Bohlmann, Xiaoxia Shang, Elina Giannakaki, Maria Filioglou, Annika Saarto, Sami Romakkaniemi, and Mika Komppula
Atmos. Chem. Phys., 19, 14559–14569, https://doi.org/10.5194/acp-19-14559-2019, https://doi.org/10.5194/acp-19-14559-2019, 2019
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Measurements of the multiwavelength Raman polarization lidar PollyXT have been combined with measurements of pollen type and concentration using a traditional pollen sampler at the rural forest site in Vehmasmäki, Finland. High particle depolarization ratios were observed during an intense pollination event of birch pollen occasionally mixed with spruce pollen. Our observations illustrate the potential of the particle depolarization ratio to track pollen grains in the atmosphere.
Anina Gilgen, Stiig Wilkenskjeld, Jed O. Kaplan, Thomas Kühn, and Ulrike Lohmann
Clim. Past, 15, 1885–1911, https://doi.org/10.5194/cp-15-1885-2019, https://doi.org/10.5194/cp-15-1885-2019, 2019
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Using the global aerosol–climate model ECHAM-HAM-SALSA, the effect of humans on European climate in the Roman Empire was quantified. Both land use and novel estimates of anthropogenic aerosol emissions were considered. We conducted simulations with fixed sea-surface temperatures to gain a first impression about the anthropogenic impact. While land use effects induced a regional warming for one of the reconstructions, aerosol emissions led to a cooling associated with aerosol–cloud interactions.
David Neubauer, Sylvaine Ferrachat, Colombe Siegenthaler-Le Drian, Philip Stier, Daniel G. Partridge, Ina Tegen, Isabelle Bey, Tanja Stanelle, Harri Kokkola, and Ulrike Lohmann
Geosci. Model Dev., 12, 3609–3639, https://doi.org/10.5194/gmd-12-3609-2019, https://doi.org/10.5194/gmd-12-3609-2019, 2019
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The global aerosol–climate model ECHAM6.3–HAM2.3 as well as the previous model versions ECHAM5.5–HAM2.0 and ECHAM6.1–HAM2.2 are evaluated. The simulation of clouds has improved in ECHAM6.3–HAM2.3. This has an impact on effective radiative forcing due to aerosol–radiation and aerosol–cloud interactions and equilibrium climate sensitivity, which are weaker in ECHAM6.3–HAM2.3 than in the previous model versions.
Ina Tegen, David Neubauer, Sylvaine Ferrachat, Colombe Siegenthaler-Le Drian, Isabelle Bey, Nick Schutgens, Philip Stier, Duncan Watson-Parris, Tanja Stanelle, Hauke Schmidt, Sebastian Rast, Harri Kokkola, Martin Schultz, Sabine Schroeder, Nikos Daskalakis, Stefan Barthel, Bernd Heinold, and Ulrike Lohmann
Geosci. Model Dev., 12, 1643–1677, https://doi.org/10.5194/gmd-12-1643-2019, https://doi.org/10.5194/gmd-12-1643-2019, 2019
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We describe a new version of the aerosol–climate model ECHAM–HAM and show tests of the model performance by comparing different aspects of the aerosol distribution with different datasets. The updated version of HAM contains improved descriptions of aerosol processes, including updated emission fields and cloud processes. While there are regional deviations between the model and observations, the model performs well overall.
Mona Kurppa, Antti Hellsten, Pontus Roldin, Harri Kokkola, Juha Tonttila, Mikko Auvinen, Christoph Kent, Prashant Kumar, Björn Maronga, and Leena Järvi
Geosci. Model Dev., 12, 1403–1422, https://doi.org/10.5194/gmd-12-1403-2019, https://doi.org/10.5194/gmd-12-1403-2019, 2019
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This paper describes the implementation of a sectional aerosol module, SALSA, into the PALM model system 6.0. The first evaluation study shows excellent agreements with measurements. Furthermore, we show that ignoring the dry deposition of aerosol particles can overestimate aerosol number concentrations by 20 %, whereas condensation and dissolutional growth increase the total aerosol mass by over 10 % in this specific urban environment.
Harri Kokkola, Thomas Kühn, Anton Laakso, Tommi Bergman, Kari E. J. Lehtinen, Tero Mielonen, Antti Arola, Scarlet Stadtler, Hannele Korhonen, Sylvaine Ferrachat, Ulrike Lohmann, David Neubauer, Ina Tegen, Colombe Siegenthaler-Le Drian, Martin G. Schultz, Isabelle Bey, Philip Stier, Nikos Daskalakis, Colette L. Heald, and Sami Romakkaniemi
Geosci. Model Dev., 11, 3833–3863, https://doi.org/10.5194/gmd-11-3833-2018, https://doi.org/10.5194/gmd-11-3833-2018, 2018
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In this paper we present a global aerosol–chemistry–climate model with the focus on its representation for atmospheric aerosol particles. In the model, aerosols are simulated using the aerosol module SALSA2.0, which in this paper is compared to satellite, ground, and aircraft-based observations of the properties of atmospheric aerosol. Based on this study, the model simulated aerosol properties compare well with the observations.
Scarlet Stadtler, Thomas Kühn, Sabine Schröder, Domenico Taraborrelli, Martin G. Schultz, and Harri Kokkola
Geosci. Model Dev., 11, 3235–3260, https://doi.org/10.5194/gmd-11-3235-2018, https://doi.org/10.5194/gmd-11-3235-2018, 2018
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Atmospheric aerosols interact with our climate system and have adverse health effects. Nevertheless, these particles are a source of uncertainty in climate projections and the formation process of secondary aerosols formed by organic gas-phase precursors is particularly not fully understood. In order to gain a deeper understanding of secondary organic aerosol formation, this model system explicitly represents gas-phase and aerosol formation processes. Finally, this allows for process discussion.
Robin G. Stevens, Katharina Loewe, Christopher Dearden, Antonios Dimitrelos, Anna Possner, Gesa K. Eirund, Tomi Raatikainen, Adrian A. Hill, Benjamin J. Shipway, Jonathan Wilkinson, Sami Romakkaniemi, Juha Tonttila, Ari Laaksonen, Hannele Korhonen, Paul Connolly, Ulrike Lohmann, Corinna Hoose, Annica M. L. Ekman, Ken S. Carslaw, and Paul R. Field
Atmos. Chem. Phys., 18, 11041–11071, https://doi.org/10.5194/acp-18-11041-2018, https://doi.org/10.5194/acp-18-11041-2018, 2018
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We perform a model intercomparison of summertime high Arctic clouds. Observed concentrations of aerosol particles necessary for cloud formation fell to extremely low values, coincident with a transition from cloudy to nearly cloud-free conditions. Previous analyses have suggested that at these low concentrations, the radiative properties of the clouds are determined primarily by these particle concentrations. The model results strongly support this hypothesis.
Ian Boutle, Jeremy Price, Innocent Kudzotsa, Harri Kokkola, and Sami Romakkaniemi
Atmos. Chem. Phys., 18, 7827–7840, https://doi.org/10.5194/acp-18-7827-2018, https://doi.org/10.5194/acp-18-7827-2018, 2018
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Aerosol processes are a key mechanism in the development of fog. Poor representation of aerosol–fog interaction can result in large biases in fog forecasts, such as surface temperatures which are too high and fog which is too deep and long lived. A relatively simple representation of aerosol–fog interaction can actually lead to significant improvements in forecasting. Aerosol–fog interaction can have a large effect on the climate system but is poorly represented in climate models.
Martin G. Schultz, Scarlet Stadtler, Sabine Schröder, Domenico Taraborrelli, Bruno Franco, Jonathan Krefting, Alexandra Henrot, Sylvaine Ferrachat, Ulrike Lohmann, David Neubauer, Colombe Siegenthaler-Le Drian, Sebastian Wahl, Harri Kokkola, Thomas Kühn, Sebastian Rast, Hauke Schmidt, Philip Stier, Doug Kinnison, Geoffrey S. Tyndall, John J. Orlando, and Catherine Wespes
Geosci. Model Dev., 11, 1695–1723, https://doi.org/10.5194/gmd-11-1695-2018, https://doi.org/10.5194/gmd-11-1695-2018, 2018
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The chemistry–climate model ECHAM-HAMMOZ contains a detailed representation of tropospheric and stratospheric reactive chemistry and state-of-the-art parameterizations of aerosols. It thus allows for detailed investigations of chemical processes in the climate system. Evaluation of the model with various observational data yields good results, but the model has a tendency to produce too much OH in the tropics. This highlights the important interplay between atmospheric chemistry and dynamics.
Antti Lipponen, Tero Mielonen, Mikko R. A. Pitkänen, Robert C. Levy, Virginia R. Sawyer, Sami Romakkaniemi, Ville Kolehmainen, and Antti Arola
Atmos. Meas. Tech., 11, 1529–1547, https://doi.org/10.5194/amt-11-1529-2018, https://doi.org/10.5194/amt-11-1529-2018, 2018
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Atmospheric aerosols are small solid or liquid particles suspended in the atmosphere and they have a significant effect on the climate. Satellite data are used to get global estimates of atmospheric aerosols. In this work, a statistics-based Bayesian aerosol retrieval algorithm was developed to improve the accuracy and quantify the uncertainties related to the aerosol estimates. The algorithm is tested with NASA's Moderate Resolution Imaging Spectroradiometer (MODIS) satellite data.
Lukas Pichelstorfer, Dominik Stolzenburg, John Ortega, Thomas Karl, Harri Kokkola, Anton Laakso, Kari E. J. Lehtinen, James N. Smith, Peter H. McMurry, and Paul M. Winkler
Atmos. Chem. Phys., 18, 1307–1323, https://doi.org/10.5194/acp-18-1307-2018, https://doi.org/10.5194/acp-18-1307-2018, 2018
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Quantification of new particle formation as a source of atmospheric aerosol is clearly of importance for climate and health aspects. In our new study we developed two analysis methods that allow retrieval of nanoparticle growth dynamics at much higher precision than it was possible so far. Our results clearly demonstrate that growth rates show much more variation than is currently known and suggest that the Kelvin effect governs growth in the sub-10 nm size range.
Maria Filioglou, Anna Nikandrova, Sami Niemelä, Holger Baars, Tero Mielonen, Ari Leskinen, David Brus, Sami Romakkaniemi, Elina Giannakaki, and Mika Komppula
Atmos. Meas. Tech., 10, 4303–4316, https://doi.org/10.5194/amt-10-4303-2017, https://doi.org/10.5194/amt-10-4303-2017, 2017
Sami Romakkaniemi, Zubair Maalick, Antti Hellsten, Antti Ruuskanen, Olli Väisänen, Irshad Ahmad, Juha Tonttila, Santtu Mikkonen, Mika Komppula, and Thomas Kühn
Atmos. Chem. Phys., 17, 7955–7964, https://doi.org/10.5194/acp-17-7955-2017, https://doi.org/10.5194/acp-17-7955-2017, 2017
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Surface topography affects aerosol–cloud interactions in boundary layer clouds. Local topography effects should be screened out from in situ observations before results can be generalised into a larger scale. Here we present modelling and observational results from a measurement station residing in a 75 m tower on top of a 150 m hill, and analyse how landscape affects the cloud formation, and which factors should be taken into account when aerosol effect on cloud droplet formation is studied.
Anton Laakso, Hannele Korhonen, Sami Romakkaniemi, and Harri Kokkola
Atmos. Chem. Phys., 17, 6957–6974, https://doi.org/10.5194/acp-17-6957-2017, https://doi.org/10.5194/acp-17-6957-2017, 2017
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Based on simulations, equatorial stratospheric sulfur injections have shown to be an efficient strategy to counteract ongoing global warming. However, equatorial injections would result in relatively larger cooling in low latitudes than in high latitudes. This together with greenhouse-gas-induced warming would lead to cooling in the Equator and warming in the high latitudes. Results of this study show that a more optimal cooling effect is achieved by varying the injection area seasonally.
Antti Arola, Thomas F. Eck, Harri Kokkola, Mikko R. A. Pitkänen, and Sami Romakkaniemi
Atmos. Chem. Phys., 17, 5991–6001, https://doi.org/10.5194/acp-17-5991-2017, https://doi.org/10.5194/acp-17-5991-2017, 2017
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One of the issues that hinder the measurement-based assessment of aerosol–cloud interactions by remote sensing methods is that typically aerosols and clouds cannot be measured simultaneously by passive remote sensing methods. AERONET includes the SDA product that provides the fine-mode AOD also in mixed cloud–aerosol observations. These measurements have not yet been fully exploited in studies of aerosol–cloud interactions. We applied SDA for this kind of analysis.
Tomi Raatikainen, David Brus, Rakesh K. Hooda, Antti-Pekka Hyvärinen, Eija Asmi, Ved P. Sharma, Antti Arola, and Heikki Lihavainen
Atmos. Chem. Phys., 17, 371–383, https://doi.org/10.5194/acp-17-371-2017, https://doi.org/10.5194/acp-17-371-2017, 2017
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We have measured black carbon aerosol properties in northern India at two sites: the first site is located at the polluted Indo-Gangetic Plain, while the second site is at the Himalayan foothills in a significantly cleaner environment. The observations show a clear difference in black carbon concentrations, but individual aerosol particles seem to be similar in both sites. Indirect evidence suggests that the particles are highly irregular resembling freshly emitted soot.
Olli Väisänen, Antti Ruuskanen, Arttu Ylisirniö, Pasi Miettinen, Harri Portin, Liqing Hao, Ari Leskinen, Mika Komppula, Sami Romakkaniemi, Kari E. J. Lehtinen, and Annele Virtanen
Atmos. Chem. Phys., 16, 10385–10398, https://doi.org/10.5194/acp-16-10385-2016, https://doi.org/10.5194/acp-16-10385-2016, 2016
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In-cloud measurements of aerosol hygroscopicity and cloud droplet activation were conducted in Kuopio, Finland. According to the observations, the less hygroscopic accumulation mode particles were present in the non-activated aerosol, whereas the more hygroscopic particles were scavenged into cloud droplets. The results illustrate the sensitivity of cloud droplet formation to varying chemical composition and highlight the need for proper treatment of anthropogenic aerosols in CCN predictions.
Tero Mielonen, Anca Hienola, Thomas Kühn, Joonas Merikanto, Antti Lipponen, Tommi Bergman, Hannele Korhonen, Pekka Kolmonen, Larisa Sogacheva, Darren Ghent, Antti Arola, Gerrit de Leeuw, and Harri Kokkola
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-625, https://doi.org/10.5194/acp-2016-625, 2016
Revised manuscript not accepted
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We studied the temperature dependence of AOD and its radiative effects over the southeastern US. We used spaceborne observations of AOD, LST and tropospheric NO2 with simulations of ECHAM-HAMMOZ. The level of AOD in this region is governed by anthropogenic emissions but the temperature dependency is most likely caused by BVOC emissions. According to the observations and simulations, the regional clear-sky DRE for biogenic aerosols is −0.43 ± 0.88 W/m2/K and −0.86 ± 0.06 W/m2/K, respectively.
Jani Huttunen, Harri Kokkola, Tero Mielonen, Mika Esa Juhani Mononen, Antti Lipponen, Juha Reunanen, Anders Vilhelm Lindfors, Santtu Mikkonen, Kari Erkki Juhani Lehtinen, Natalia Kouremeti, Alkiviadis Bais, Harri Niska, and Antti Arola
Atmos. Chem. Phys., 16, 8181–8191, https://doi.org/10.5194/acp-16-8181-2016, https://doi.org/10.5194/acp-16-8181-2016, 2016
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For a good estimate of the current forcing by anthropogenic aerosols, knowledge in past is needed. One option to lengthen time series is to retrieve aerosol optical depth from solar radiation measurements. We have evaluated several methods for this task. Most of the methods produce aerosol optical depth estimates with a good accuracy. However, machine learning methods seem to be the most applicable not to produce any systematic biases, since they do not need constrain the aerosol properties.
N. I. Kristiansen, A. Stohl, D. J. L. Olivié, B. Croft, O. A. Søvde, H. Klein, T. Christoudias, D. Kunkel, S. J. Leadbetter, Y. H. Lee, K. Zhang, K. Tsigaridis, T. Bergman, N. Evangeliou, H. Wang, P.-L. Ma, R. C. Easter, P. J. Rasch, X. Liu, G. Pitari, G. Di Genova, S. Y. Zhao, Y. Balkanski, S. E. Bauer, G. S. Faluvegi, H. Kokkola, R. V. Martin, J. R. Pierce, M. Schulz, D. Shindell, H. Tost, and H. Zhang
Atmos. Chem. Phys., 16, 3525–3561, https://doi.org/10.5194/acp-16-3525-2016, https://doi.org/10.5194/acp-16-3525-2016, 2016
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Processes affecting aerosol removal from the atmosphere are not fully understood. In this study we investigate to what extent atmospheric transport models can reproduce observed loss of aerosols. We compare measurements of radioactive isotopes, that attached to ambient sulfate aerosols during the 2011 Fukushima nuclear accident, to 19 models using identical emissions. Results indicate aerosol removal that is too fast in most models, and apply to aerosols that have undergone long-range transport.
Zak Kipling, Philip Stier, Colin E. Johnson, Graham W. Mann, Nicolas Bellouin, Susanne E. Bauer, Tommi Bergman, Mian Chin, Thomas Diehl, Steven J. Ghan, Trond Iversen, Alf Kirkevåg, Harri Kokkola, Xiaohong Liu, Gan Luo, Twan van Noije, Kirsty J. Pringle, Knut von Salzen, Michael Schulz, Øyvind Seland, Ragnhild B. Skeie, Toshihiko Takemura, Kostas Tsigaridis, and Kai Zhang
Atmos. Chem. Phys., 16, 2221–2241, https://doi.org/10.5194/acp-16-2221-2016, https://doi.org/10.5194/acp-16-2221-2016, 2016
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The vertical distribution of atmospheric aerosol is an important factor in its effects on climate. In this study we use a sophisticated model of the many interacting processes affecting aerosol in the atmosphere to show that the vertical distribution is typically dominated by only a few of these processes. Constraining these physical processes may help to reduce the large differences between models. However, the important processes are not always the same for different types of aerosol.
A. Laakso, H. Kokkola, A.-I. Partanen, U. Niemeier, C. Timmreck, K. E. J. Lehtinen, H. Hakkarainen, and H. Korhonen
Atmos. Chem. Phys., 16, 305–323, https://doi.org/10.5194/acp-16-305-2016, https://doi.org/10.5194/acp-16-305-2016, 2016
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We have studied the impacts of a volcanic eruption during solar radiation management (SRM) using an aerosol-climate model ECHAM5-HAM-SALSA and an Earth system model MPI-ESM. A volcanic eruption during stratospheric sulfur geoengineering would lead to larger particles and smaller amount of new particles than if an volcano erupts in normal atmospheric conditions. Thus, volcanic eruption during SRM would lead to only a small additional cooling which would last for a significantly shorter period.
A. M. K. Hansen, J. Hong, T. Raatikainen, K. Kristensen, A. Ylisirniö, A. Virtanen, T. Petäjä, M. Glasius, and N. L. Prisle
Atmos. Chem. Phys., 15, 14071–14089, https://doi.org/10.5194/acp-15-14071-2015, https://doi.org/10.5194/acp-15-14071-2015, 2015
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This paper presents the first study of the hygroscopic properties of limonene derived organosulfates (L-OS 250). The results showed that L-OS 250 particles are weakly hygroscopic and able to activate into cloud droplets. Particles of L-OS 250 mixed with ammonium sulfate were much more hygroscopic than expected from model parametrizations and the ZSR mixing rule, indicating that solubility and non-ideal droplet interactions could be important for the hygroscopic properties of the mixed particles.
A. Arola, G. L. Schuster, M. R. A. Pitkänen, O. Dubovik, H. Kokkola, A. V. Lindfors, T. Mielonen, T. Raatikainen, S. Romakkaniemi, S. N. Tripathi, and H. Lihavainen
Atmos. Chem. Phys., 15, 12731–12740, https://doi.org/10.5194/acp-15-12731-2015, https://doi.org/10.5194/acp-15-12731-2015, 2015
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There have been relatively few measurement-based estimates for the direct radiative effect of brown carbon so far. This is first time that the direct radiative effect of brown carbon is estimated by exploiting the AERONET-retrieved imaginary indices. We estimated it for four sites in the Indo-Gangetic Plain: Karachi, Lahore,
Kanpur and Gandhi College.
T. Raatikainen, D. Brus, A.-P. Hyvärinen, J. Svensson, E. Asmi, and H. Lihavainen
Atmos. Chem. Phys., 15, 10057–10070, https://doi.org/10.5194/acp-15-10057-2015, https://doi.org/10.5194/acp-15-10057-2015, 2015
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We have measured atmospheric aerosol composition by using a Single Particle Soot Photometer (SP2) in the Finnish Arctic during winter 2011-2012. SP2 can give detailed information about mass distributions and mixing state of refractory black carbon (rBC). The measurements showed varying rBC mass concentrations, but relatively constant rBC core size distributions and mixing state parameters. On average, 24% of all particles contain rBC and the observed rBC cores are always thickly coated.
M. A. Thomas, M. Kahnert, C. Andersson, H. Kokkola, U. Hansson, C. Jones, J. Langner, and A. Devasthale
Geosci. Model Dev., 8, 1885–1898, https://doi.org/10.5194/gmd-8-1885-2015, https://doi.org/10.5194/gmd-8-1885-2015, 2015
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We have showed that a coupled modelling system is beneficial in the sense that more complex processes can be included to better represent the aerosol processes starting from their formation, their interactions with clouds and provide better estimate of radiative forcing. Using this model set up, we estimated an annual mean 'indirect' radiative forcing of -0.64W/m2. This means that aerosols, solely by their capability of altering the microphysical properties of clouds can cool the Earth system.
J. Tonttila, E. J. O'Connor, A. Hellsten, A. Hirsikko, C. O'Dowd, H. Järvinen, and P. Räisänen
Atmos. Chem. Phys., 15, 5873–5885, https://doi.org/10.5194/acp-15-5873-2015, https://doi.org/10.5194/acp-15-5873-2015, 2015
M. Dalirian, H. Keskinen, L. Ahlm, A. Ylisirniö, S. Romakkaniemi, A. Laaksonen, A. Virtanen, and I. Riipinen
Atmos. Chem. Phys., 15, 3815–3829, https://doi.org/10.5194/acp-15-3815-2015, https://doi.org/10.5194/acp-15-3815-2015, 2015
C. Andersson, R. Bergström, C. Bennet, L. Robertson, M. Thomas, H. Korhonen, K. E. J. Lehtinen, and H. Kokkola
Geosci. Model Dev., 8, 171–189, https://doi.org/10.5194/gmd-8-171-2015, https://doi.org/10.5194/gmd-8-171-2015, 2015
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We have integrated the sectional aerosol dynamics model SALSA into the European scale chemistry-transport model MATCH. The combined model reproduces observed higher particle number concentration (PNCs) in central Europe and lower concentrations in remote regions; however, the total PNC is underestimated. The low nucleation rate coefficient used in this study is an important reason for the underestimation.
J. Tonttila, H. Järvinen, and P. Räisänen
Atmos. Chem. Phys., 15, 703–714, https://doi.org/10.5194/acp-15-703-2015, https://doi.org/10.5194/acp-15-703-2015, 2015
E. M. Dunne, S. Mikkonen, H. Kokkola, and H. Korhonen
Atmos. Chem. Phys., 14, 13631–13642, https://doi.org/10.5194/acp-14-13631-2014, https://doi.org/10.5194/acp-14-13631-2014, 2014
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Marine clouds have a strong effect on the Earth's radiative balance. One proposed climate feedback is that, in a warming climate, marine aerosol emissions will change due to changing wind speeds. We have examined the processes that affect aerosol emissions and removal over 15 years, and high-temporal-resolution output over 2 months. We conclude that wind trends are unlikely to cause a strong feedback in marine regions, but changes in removal processes or transport from continental regions may.
L. Q. Hao, A. Kortelainen, S. Romakkaniemi, H. Portin, A. Jaatinen, A. Leskinen, M. Komppula, P. Miettinen, D. Sueper, A. Pajunoja, J. N. Smith, K. E. J. Lehtinen, D. R. Worsnop, A. Laaksonen, and A. Virtanen
Atmos. Chem. Phys., 14, 13483–13495, https://doi.org/10.5194/acp-14-13483-2014, https://doi.org/10.5194/acp-14-13483-2014, 2014
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Positive matrix factorization (PMF) was applied to the unified high-resolution mass spectra organic species with NO+ and NO2+ ions from the measurement in a mixed region between the boreal forestland and the urban area. The PMF analysis succeeded in separating the mixed spectra into three distinct organic factors and one inorganic factor. The particulate organic nitrate was distinguished by PMF for the first time, with a contribution of one-third of the total nitrate mass.
A.-I. Partanen, E. M. Dunne, T. Bergman, A. Laakso, H. Kokkola, J. Ovadnevaite, L. Sogacheva, D. Baisnée, J. Sciare, A. Manders, C. O'Dowd, G. de Leeuw, and H. Korhonen
Atmos. Chem. Phys., 14, 11731–11752, https://doi.org/10.5194/acp-14-11731-2014, https://doi.org/10.5194/acp-14-11731-2014, 2014
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New parameterizations for the sea spray aerosol source flux and its organic fraction were incorporated into a global aerosol-climate model. The emissions of sea salt were considerably less than previous estimates. This study demonstrates that sea spray aerosol may actually decrease the number of cloud droplets, which has a warming effect on climate. Overall, sea spray aerosol was predicted to have a global cooling effect due to the scattering of solar radiation from sea spray aerosol particles.
K. Tsigaridis, N. Daskalakis, M. Kanakidou, P. J. Adams, P. Artaxo, R. Bahadur, Y. Balkanski, S. E. Bauer, N. Bellouin, A. Benedetti, T. Bergman, T. K. Berntsen, J. P. Beukes, H. Bian, K. S. Carslaw, M. Chin, G. Curci, T. Diehl, R. C. Easter, S. J. Ghan, S. L. Gong, A. Hodzic, C. R. Hoyle, T. Iversen, S. Jathar, J. L. Jimenez, J. W. Kaiser, A. Kirkevåg, D. Koch, H. Kokkola, Y. H Lee, G. Lin, X. Liu, G. Luo, X. Ma, G. W. Mann, N. Mihalopoulos, J.-J. Morcrette, J.-F. Müller, G. Myhre, S. Myriokefalitakis, N. L. Ng, D. O'Donnell, J. E. Penner, L. Pozzoli, K. J. Pringle, L. M. Russell, M. Schulz, J. Sciare, Ø. Seland, D. T. Shindell, S. Sillman, R. B. Skeie, D. Spracklen, T. Stavrakou, S. D. Steenrod, T. Takemura, P. Tiitta, S. Tilmes, H. Tost, T. van Noije, P. G. van Zyl, K. von Salzen, F. Yu, Z. Wang, Z. Wang, R. A. Zaveri, H. Zhang, K. Zhang, Q. Zhang, and X. Zhang
Atmos. Chem. Phys., 14, 10845–10895, https://doi.org/10.5194/acp-14-10845-2014, https://doi.org/10.5194/acp-14-10845-2014, 2014
S. V. Henriksson, J.-P. Pietikäinen, A.-P. Hyvärinen, P. Räisänen, K. Kupiainen, J. Tonttila, R. Hooda, H. Lihavainen, D. O'Donnell, L. Backman, Z. Klimont, and A. Laaksonen
Atmos. Chem. Phys., 14, 10177–10192, https://doi.org/10.5194/acp-14-10177-2014, https://doi.org/10.5194/acp-14-10177-2014, 2014
H. Portin, A. Leskinen, L. Hao, A. Kortelainen, P. Miettinen, A. Jaatinen, A. Laaksonen, K. E. J. Lehtinen, S. Romakkaniemi, and M. Komppula
Atmos. Chem. Phys., 14, 6021–6034, https://doi.org/10.5194/acp-14-6021-2014, https://doi.org/10.5194/acp-14-6021-2014, 2014
S. Romakkaniemi, A. Jaatinen, A. Laaksonen, A. Nenes, and T. Raatikainen
Atmos. Meas. Tech., 7, 1377–1384, https://doi.org/10.5194/amt-7-1377-2014, https://doi.org/10.5194/amt-7-1377-2014, 2014
G. W. Mann, K. S. Carslaw, C. L. Reddington, K. J. Pringle, M. Schulz, A. Asmi, D. V. Spracklen, D. A. Ridley, M. T. Woodhouse, L. A. Lee, K. Zhang, S. J. Ghan, R. C. Easter, X. Liu, P. Stier, Y. H. Lee, P. J. Adams, H. Tost, J. Lelieveld, S. E. Bauer, K. Tsigaridis, T. P. C. van Noije, A. Strunk, E. Vignati, N. Bellouin, M. Dalvi, C. E. Johnson, T. Bergman, H. Kokkola, K. von Salzen, F. Yu, G. Luo, A. Petzold, J. Heintzenberg, A. Clarke, J. A. Ogren, J. Gras, U. Baltensperger, U. Kaminski, S. G. Jennings, C. D. O'Dowd, R. M. Harrison, D. C. S. Beddows, M. Kulmala, Y. Viisanen, V. Ulevicius, N. Mihalopoulos, V. Zdimal, M. Fiebig, H.-C. Hansson, E. Swietlicki, and J. S. Henzing
Atmos. Chem. Phys., 14, 4679–4713, https://doi.org/10.5194/acp-14-4679-2014, https://doi.org/10.5194/acp-14-4679-2014, 2014
H. Kokkola, P. Yli-Pirilä, M. Vesterinen, H. Korhonen, H. Keskinen, S. Romakkaniemi, L. Hao, A. Kortelainen, J. Joutsensaari, D. R. Worsnop, A. Virtanen, and K. E. J. Lehtinen
Atmos. Chem. Phys., 14, 1689–1700, https://doi.org/10.5194/acp-14-1689-2014, https://doi.org/10.5194/acp-14-1689-2014, 2014
T. Korhola, H. Kokkola, H. Korhonen, A.-I. Partanen, A. Laaksonen, K. E. J. Lehtinen, and S. Romakkaniemi
Geosci. Model Dev., 7, 161–174, https://doi.org/10.5194/gmd-7-161-2014, https://doi.org/10.5194/gmd-7-161-2014, 2014
A. Lipponen, V. Kolehmainen, S. Romakkaniemi, and H. Kokkola
Geosci. Model Dev., 6, 2087–2098, https://doi.org/10.5194/gmd-6-2087-2013, https://doi.org/10.5194/gmd-6-2087-2013, 2013
A. I. Partanen, A. Laakso, A. Schmidt, H. Kokkola, T. Kuokkanen, J.-P. Pietikäinen, V.-M. Kerminen, K. E. J. Lehtinen, L. Laakso, and H. Korhonen
Atmos. Chem. Phys., 13, 12059–12071, https://doi.org/10.5194/acp-13-12059-2013, https://doi.org/10.5194/acp-13-12059-2013, 2013
J. Tonttila, P. Räisänen, and H. Järvinen
Atmos. Chem. Phys., 13, 7551–7565, https://doi.org/10.5194/acp-13-7551-2013, https://doi.org/10.5194/acp-13-7551-2013, 2013
S. Lance, T. Raatikainen, T. B. Onasch, D. R. Worsnop, X.-Y. Yu, M. L. Alexander, M. R. Stolzenburg, P. H. McMurry, J. N. Smith, and A. Nenes
Atmos. Chem. Phys., 13, 5049–5062, https://doi.org/10.5194/acp-13-5049-2013, https://doi.org/10.5194/acp-13-5049-2013, 2013
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The CHIMERE chemistry-transport model v2023r1
tobac v1.5: introducing fast 3D tracking, splits and mergers, and other enhancements for identifying and analysing meteorological phenomena
Merged Observatory Data Files (MODFs): an integrated observational data product supporting process-oriented investigations and diagnostics
Simulation of marine stratocumulus using the super-droplet method: numerical convergence and comparison to a double-moment bulk scheme using SCALE-SDM 5.2.6-2.3.1
WRF-Comfort: simulating microscale variability in outdoor heat stress at the city scale with a mesoscale model
Representing effects of surface heterogeneity in a multi-plume eddy diffusivity mass flux boundary layer parameterization
Can TROPOMI NO2 satellite data be used to track the drop in and resurgence of NOx emissions in Germany between 2019–2021 using the multi-source plume method (MSPM)?
A spatiotemporally separated framework for reconstructing the sources of atmospheric radionuclide releases
A parameterization scheme for the floating wind farm in a coupled atmosphere–wave model (COAWST v3.7)
RoadSurf 1.1: open-source road weather model library
Calibrating and validating the Integrated Valuation of Ecosystem Services and Tradeoffs (InVEST) urban cooling model: case studies in France and the United States
The ddeq Python library for point source quantification from remote sensing images (version 1.0)
Incorporating Oxygen Isotopes of Oxidized Reactive Nitrogen in the Regional Atmospheric Chemistry Mechanism, version 2 (ICOIN-RACM2)
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Implementation of a Simple Actuator Disk for Large-Eddy Simulation in the Weather Research and Forecasting Model (WRF-SADLES v1.2) for wind turbine wake simulation
WRF-PDAF v1.0: implementation and application of an online localized ensemble data assimilation framework
Implementation and evaluation of diabatic advection in the Lagrangian transport model MPTRAC 2.6
An improved and extended parameterization of the CO2 15 µm cooling in the middle and upper atmosphere (CO2_cool_fort-1.0)
Development of a multiphase chemical mechanism to improve secondary organic aerosol formation in CAABA/MECCA (version 4.7.0)
Application of regional meteorology and air quality models based on the microprocessor without interlocked piped stages (MIPS) and LoongArch CPU platforms
Investigating ground-level ozone pollution in semi-arid and arid regions of Arizona using WRF-Chem v4.4 modeling
An objective identification technique for potential vorticity structures associated with African easterly waves
Importance of microphysical settings for climate forcing by stratospheric SO2 injections as modeled by SOCOL-AERv2
Assessment of surface ozone products from downscaled CAMS reanalysis and CAMS daily forecast using urban air quality monitoring stations in Iran
Open boundary conditions for atmospheric large-eddy simulations and their implementation in DALES4.4
Efficient and stable coupling of the SuperdropNet deep-learning-based cloud microphysics (v0.1.0) with the ICON climate and weather model (v2.6.5)
Three-dimensional variational assimilation with a multivariate background error covariance for the Model for Prediction Across Scales – Atmosphere with the Joint Effort for Data assimilation Integration (JEDI-MPAS 2.0.0-beta)
FUME 2.0 – Flexible Universal processor for Modeling Emissions
DEUCE v1.0: a neural network for probabilistic precipitation nowcasting with aleatoric and epistemic uncertainties
Evaluation of multi-season convection-permitting atmosphere – mixed-layer ocean simulations of the Maritime Continent
Investigating the impact of coupling HARMONIE-WINS50 (cy43) meteorology to LOTOS-EUROS (v2.2.002) on a simulation of NO2 concentrations over the Netherlands
Balloon drift estimation and improved position estimates for radiosondes
Emission ensemble approach to improve the development of multi-scale emission inventories
What is the relative impact of nudging and online coupling on meteorological variables, pollutant concentrations and aerosol optical properties?
Diagnosing drivers of PM2.5 simulation biases in China from meteorology, chemical composition, and emission sources using an efficient machine learning method
Validation and analysis of the Polair3D v1.11 chemical transport model over Quebec
Assimilation of GNSS tropospheric gradients into the Weather Research and Forecasting (WRF) model version 4.4.1
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Assessing acetone for the GISS ModelE2.1 Earth system model
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A dynamic approach to three-dimensional radiative transfer in subkilometer-scale numerical weather prediction models: the dynamic TenStream solver v1.0
Evaluation and development of surface layer scheme representation of temperature inversions over boreal forests in Arctic wintertime conditions
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Mixed-Precision Computing in the GRIST Dynamical Core for Weather and Climate Modelling
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Decision Support System version 1.0 (DSS v1.0) for air quality management in Delhi, India
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Laurent Menut, Arineh Cholakian, Romain Pennel, Guillaume Siour, Sylvain Mailler, Myrto Valari, Lya Lugon, and Yann Meurdesoif
Geosci. Model Dev., 17, 5431–5457, https://doi.org/10.5194/gmd-17-5431-2024, https://doi.org/10.5194/gmd-17-5431-2024, 2024
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A new version of the CHIMERE model is presented. This version contains both computational and physico-chemical changes. The computational changes make it easy to choose the variables to be extracted as a result, including values of maximum sub-hourly concentrations. Performance tests show that the model is 1.5 to 2 times faster than the previous version for the same setup. Processes such as turbulence, transport schemes and dry deposition have been modified and updated.
G. Alexander Sokolowsky, Sean W. Freeman, William K. Jones, Julia Kukulies, Fabian Senf, Peter J. Marinescu, Max Heikenfeld, Kelcy N. Brunner, Eric C. Bruning, Scott M. Collis, Robert C. Jackson, Gabrielle R. Leung, Nils Pfeifer, Bhupendra A. Raut, Stephen M. Saleeby, Philip Stier, and Susan C. van den Heever
Geosci. Model Dev., 17, 5309–5330, https://doi.org/10.5194/gmd-17-5309-2024, https://doi.org/10.5194/gmd-17-5309-2024, 2024
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Building on previous analysis tools developed for atmospheric science, the original release of the Tracking and Object-Based Analysis (tobac) Python package, v1.2, was open-source, modular, and insensitive to the type of gridded input data. Here, we present the latest version of tobac, v1.5, which substantially improves scientific capabilities and computational efficiency from the previous version. These enhancements permit new uses for tobac in atmospheric science and potentially other fields.
Taneil Uttal, Leslie M. Hartten, Siri Jodha Khalsa, Barbara Casati, Gunilla Svensson, Jonathan Day, Jareth Holt, Elena Akish, Sara Morris, Ewan O'Connor, Roberta Pirazzini, Laura X. Huang, Robert Crawford, Zen Mariani, Øystein Godøy, Johanna A. K. Tjernström, Giri Prakash, Nicki Hickmon, Marion Maturilli, and Christopher J. Cox
Geosci. Model Dev., 17, 5225–5247, https://doi.org/10.5194/gmd-17-5225-2024, https://doi.org/10.5194/gmd-17-5225-2024, 2024
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A Merged Observatory Data File (MODF) format to systematically collate complex atmosphere, ocean, and terrestrial data sets collected by multiple instruments during field campaigns is presented. The MODF format is also designed to be applied to model output data, yielding format-matching Merged Model Data Files (MMDFs). MODFs plus MMDFs will augment and accelerate the synergistic use of model results with observational data to increase understanding and predictive skill.
Chongzhi Yin, Shin-ichiro Shima, Lulin Xue, and Chunsong Lu
Geosci. Model Dev., 17, 5167–5189, https://doi.org/10.5194/gmd-17-5167-2024, https://doi.org/10.5194/gmd-17-5167-2024, 2024
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We investigate numerical convergence properties of a particle-based numerical cloud microphysics model (SDM) and a double-moment bulk scheme for simulating a marine stratocumulus case, compare their results with model intercomparison project results, and present possible explanations for the different results of the SDM and the bulk scheme. Aerosol processes can be accurately simulated using SDM, and this may be an important factor affecting the behavior and morphology of marine stratocumulus.
Alberto Martilli, Negin Nazarian, E. Scott Krayenhoff, Jacob Lachapelle, Jiachen Lu, Esther Rivas, Alejandro Rodriguez-Sanchez, Beatriz Sanchez, and José Luis Santiago
Geosci. Model Dev., 17, 5023–5039, https://doi.org/10.5194/gmd-17-5023-2024, https://doi.org/10.5194/gmd-17-5023-2024, 2024
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Here, we present a model that quantifies the thermal stress and its microscale variability at a city scale with a mesoscale model. This tool can have multiple applications, from early warnings of extreme heat to the vulnerable population to the evaluation of the effectiveness of heat mitigation strategies. It is the first model that includes information on microscale variability in a mesoscale model, something that is essential for fully evaluating heat stress.
Nathan P. Arnold
Geosci. Model Dev., 17, 5041–5056, https://doi.org/10.5194/gmd-17-5041-2024, https://doi.org/10.5194/gmd-17-5041-2024, 2024
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Earth system models often represent the land surface at smaller scales than the atmosphere, but surface–atmosphere coupling uses only aggregated surface properties. This study presents a method to allow heterogeneous surface properties to modify boundary layer updrafts. The method is tested in single column experiments. Updraft properties are found to reasonably covary with surface conditions, and simulated boundary layer variability is enhanced over more heterogeneous land surfaces.
Enrico Dammers, Janot Tokaya, Christian Mielke, Kevin Hausmann, Debora Griffin, Chris McLinden, Henk Eskes, and Renske Timmermans
Geosci. Model Dev., 17, 4983–5007, https://doi.org/10.5194/gmd-17-4983-2024, https://doi.org/10.5194/gmd-17-4983-2024, 2024
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Nitrogen dioxide (NOx) is produced by sources such as industry and traffic and is directly linked to negative impacts on health and the environment. The current construction of emission inventories to keep track of NOx emissions is slow and time-consuming. Satellite measurements provide a way to quickly and independently estimate emissions. In this study, we apply a consistent methodology to derive NOx emissions over Germany and illustrate the value of having such a method for fast projections.
Yuhan Xu, Sheng Fang, Xinwen Dong, and Shuhan Zhuang
Geosci. Model Dev., 17, 4961–4982, https://doi.org/10.5194/gmd-17-4961-2024, https://doi.org/10.5194/gmd-17-4961-2024, 2024
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Recent atmospheric radionuclide leakages from unknown sources have posed a new challenge in nuclear emergency assessment. Reconstruction via environmental observations is the only feasible way to identify sources, but simultaneous reconstruction of the source location and release rate yields high uncertainties. We propose a spatiotemporally separated reconstruction strategy that avoids these uncertainties and outperforms state-of-the-art methods with respect to accuracy and uncertainty ranges.
Shaokun Deng, Shengmu Yang, Shengli Chen, Daoyi Chen, Xuefeng Yang, and Shanshan Cui
Geosci. Model Dev., 17, 4891–4909, https://doi.org/10.5194/gmd-17-4891-2024, https://doi.org/10.5194/gmd-17-4891-2024, 2024
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Global offshore wind power development is moving from offshore to deeper waters, where floating offshore wind turbines have an advantage over bottom-fixed turbines. However, current wind farm parameterization schemes in mesoscale models are not applicable to floating turbines. We propose a floating wind farm parameterization scheme that accounts for the attenuation of the significant wave height by floating turbines. The results indicate that it has a significant effect on the power output.
Virve Eveliina Karsisto
Geosci. Model Dev., 17, 4837–4853, https://doi.org/10.5194/gmd-17-4837-2024, https://doi.org/10.5194/gmd-17-4837-2024, 2024
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RoadSurf is an open-source library that contains functions from the Finnish Meteorological Institute’s road weather model. The evaluation of the library shows that it is well suited for making road surface temperature forecasts. The evaluation was done by making forecasts for about 400 road weather stations in Finland with the library. Accurate forecasts help road authorities perform salting and plowing operations at the right time and keep roads safe for drivers.
Perrine Hamel, Martí Bosch, Léa Tardieu, Aude Lemonsu, Cécile de Munck, Chris Nootenboom, Vincent Viguié, Eric Lonsdorf, James A. Douglass, and Richard P. Sharp
Geosci. Model Dev., 17, 4755–4771, https://doi.org/10.5194/gmd-17-4755-2024, https://doi.org/10.5194/gmd-17-4755-2024, 2024
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The InVEST Urban Cooling model estimates the cooling effect of vegetation in cities. We further developed an algorithm to facilitate model calibration and evaluation. Applying the algorithm to case studies in France and in the United States, we found that nighttime air temperature estimates compare well with reference datasets. Estimated change in temperature from a land cover scenario compares well with an alternative model estimate, supporting the use of the model for urban planning decisions.
Gerrit Kuhlmann, Erik Koene, Sandro Meier, Diego Santaren, Grégoire Broquet, Frédéric Chevallier, Janne Hakkarainen, Janne Nurmela, Laia Amorós, Johanna Tamminen, and Dominik Brunner
Geosci. Model Dev., 17, 4773–4789, https://doi.org/10.5194/gmd-17-4773-2024, https://doi.org/10.5194/gmd-17-4773-2024, 2024
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We present a Python software library for data-driven emission quantification (ddeq). It can be used to determine the emissions of hot spots (cities, power plants and industry) from remote sensing images using different methods. ddeq can be extended for new datasets and methods, providing a powerful community tool for users and developers. The application of the methods is shown using Jupyter notebooks included in the library.
Wendell W. Walters, Masayuki Takeuchi, Nga L. Ng, and Meredith G. Hastings
Geosci. Model Dev., 17, 4673–4687, https://doi.org/10.5194/gmd-17-4673-2024, https://doi.org/10.5194/gmd-17-4673-2024, 2024
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The study introduces a novel chemical mechanism for explicitly tracking oxygen isotope transfer in oxidized reactive nitrogen and odd oxygen using the Regional Atmospheric Chemistry Mechanism, version 2. This model enhances our ability to simulate and compare oxygen isotope compositions of reactive nitrogen, revealing insights into oxidation chemistry. The approach shows promise for improving atmospheric chemistry models and tropospheric oxidation capacity predictions.
Bing Zhang, Mingjian Zeng, Anning Huang, Zhengkun Qin, Couhua Liu, Wenru Shi, Xin Li, Kefeng Zhu, Chunlei Gu, and Jialing Zhou
Geosci. Model Dev., 17, 4579–4601, https://doi.org/10.5194/gmd-17-4579-2024, https://doi.org/10.5194/gmd-17-4579-2024, 2024
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By directly analyzing the proximity of precipitation forecasts and observations, a precipitation accuracy score (PAS) method was constructed. This method does not utilize a traditional contingency-table-based classification verification; however, it can replace the threat score (TS), equitable threat score (ETS), and other skill score methods, and it can be used to calculate the accuracy of numerical models or quantitative precipitation forecasts.
Hai Bui, Mostafa Bakhoday-Paskyabi, and Mohammadreza Mohammadpour-Penchah
Geosci. Model Dev., 17, 4447–4465, https://doi.org/10.5194/gmd-17-4447-2024, https://doi.org/10.5194/gmd-17-4447-2024, 2024
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We developed a new wind turbine wake model, the Simple Actuator Disc for Large Eddy Simulation (SADLES), integrated with the widely used Weather Research and Forecasting (WRF) model. WRF-SADLES accurately simulates wind turbine wakes at resolutions of a few dozen meters, aligning well with idealized simulations and observational measurements. This makes WRF-SADLES a promising tool for wind energy research, offering a balance between accuracy, computational efficiency, and ease of implementation.
Changliang Shao and Lars Nerger
Geosci. Model Dev., 17, 4433–4445, https://doi.org/10.5194/gmd-17-4433-2024, https://doi.org/10.5194/gmd-17-4433-2024, 2024
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This paper introduces and evaluates WRF-PDAF, a fully online-coupled ensemble data assimilation (DA) system. A key advantage of the WRF-PDAF configuration is its ability to concurrently integrate all ensemble states, eliminating the need for time-consuming distribution and collection of ensembles during the coupling communication. The extra time required for DA amounts to only 20.6 % per cycle. Twin experiment results underscore the effectiveness of the WRF-PDAF system.
Jan Clemens, Lars Hoffmann, Bärbel Vogel, Sabine Grießbach, and Nicole Thomas
Geosci. Model Dev., 17, 4467–4493, https://doi.org/10.5194/gmd-17-4467-2024, https://doi.org/10.5194/gmd-17-4467-2024, 2024
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Lagrangian transport models simulate the transport of air masses in the atmosphere. For example, one model (CLaMS) is well suited to calculating transport as it uses a special coordinate system and special vertical wind. However, it only runs inefficiently on modern supercomputers. Hence, we have implemented the benefits of CLaMS into a new model (MPTRAC), which is already highly efficient on modern supercomputers. Finally, in extensive tests, we showed that CLaMS and MPTRAC agree very well.
Manuel López-Puertas, Federico Fabiano, Victor Fomichev, Bernd Funke, and Daniel R. Marsh
Geosci. Model Dev., 17, 4401–4432, https://doi.org/10.5194/gmd-17-4401-2024, https://doi.org/10.5194/gmd-17-4401-2024, 2024
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The radiative infrared cooling of CO2 in the middle atmosphere is crucial for computing its thermal structure. It requires one however to include non-local thermodynamic equilibrium processes which are computationally very expensive, which cannot be afforded by climate models. In this work, we present an updated, efficient, accurate and very fast (~50 µs) parameterization of that cooling able to cope with CO2 abundances from half the pre-industrial values to 10 times the current abundance.
Felix Wieser, Rolf Sander, Changmin Cho, Hendrik Fuchs, Thorsten Hohaus, Anna Novelli, Ralf Tillmann, and Domenico Taraborrelli
Geosci. Model Dev., 17, 4311–4330, https://doi.org/10.5194/gmd-17-4311-2024, https://doi.org/10.5194/gmd-17-4311-2024, 2024
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The chemistry scheme of the atmospheric box model CAABA/MECCA is expanded to achieve an improved aerosol formation from emitted organic compounds. In addition to newly added reactions, temperature-dependent partitioning of all new species between the gas and aqueous phases is estimated and included in the pre-existing scheme. Sensitivity runs show an overestimation of key compounds from isoprene, which can be explained by a lack of aqueous-phase degradation reactions and box model limitations.
Zehua Bai, Qizhong Wu, Kai Cao, Yiming Sun, and Huaqiong Cheng
Geosci. Model Dev., 17, 4383–4399, https://doi.org/10.5194/gmd-17-4383-2024, https://doi.org/10.5194/gmd-17-4383-2024, 2024
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There is relatively limited research on the application of scientific computing on RISC CPU platforms. The MIPS architecture CPUs, a type of RISC CPUs, have distinct advantages in energy efficiency and scalability. The air quality modeling system can run stably on the MIPS and LoongArch platforms, and the experiment results verify the stability of scientific computing on the platforms. The work provides a technical foundation for the scientific application based on MIPS and LoongArch.
Yafang Guo, Chayan Roychoudhury, Mohammad Amin Mirrezaei, Rajesh Kumar, Armin Sorooshian, and Avelino F. Arellano
Geosci. Model Dev., 17, 4331–4353, https://doi.org/10.5194/gmd-17-4331-2024, https://doi.org/10.5194/gmd-17-4331-2024, 2024
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This research focuses on surface ozone (O3) pollution in Arizona, a historically air-quality-challenged arid and semi-arid region in the US. The unique characteristics of this kind of region, e.g., intense heat, minimal moisture, and persistent desert shrubs, play a vital role in comprehending O3 exceedances. Using the WRF-Chem model, we analyzed O3 levels in the pre-monsoon month, revealing the model's skill in capturing diurnal and MDA8 O3 levels.
Christoph Fischer, Andreas H. Fink, Elmar Schömer, Marc Rautenhaus, and Michael Riemer
Geosci. Model Dev., 17, 4213–4228, https://doi.org/10.5194/gmd-17-4213-2024, https://doi.org/10.5194/gmd-17-4213-2024, 2024
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This study presents a method for identifying and tracking 3-D potential vorticity structures within African easterly waves (AEWs). Each identified structure is characterized by descriptors, including its 3-D position and orientation, which have been validated through composite comparisons. A trough-centric perspective on the descriptors reveals the evolution and distinct characteristics of AEWs. These descriptors serve as valuable statistical inputs for the study of AEW-related phenomena.
Sandro Vattioni, Andrea Stenke, Beiping Luo, Gabriel Chiodo, Timofei Sukhodolov, Elia Wunderlin, and Thomas Peter
Geosci. Model Dev., 17, 4181–4197, https://doi.org/10.5194/gmd-17-4181-2024, https://doi.org/10.5194/gmd-17-4181-2024, 2024
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We investigate the sensitivity of aerosol size distributions in the presence of strong SO2 injections for climate interventions or after volcanic eruptions to the call sequence and frequency of the routines for nucleation and condensation in sectional aerosol models with operator splitting. Using the aerosol–chemistry–climate model SOCOL-AERv2, we show that the radiative and chemical outputs are sensitive to these settings at high H2SO4 supersaturations and how to obtain reliable results.
Najmeh Kaffashzadeh and Abbas-Ali Aliakbari Bidokhti
Geosci. Model Dev., 17, 4155–4179, https://doi.org/10.5194/gmd-17-4155-2024, https://doi.org/10.5194/gmd-17-4155-2024, 2024
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This paper assesses the capability of two state-of-the-art global datasets in simulating surface ozone over Iran using a new methodology. It is found that the global model data need to be downscaled for regulatory purposes or policy applications at local scales. The method can be useful not only for the evaluation but also for the prediction of other chemical species, such as aerosols.
Franciscus Liqui Lung, Christian Jakob, A. Pier Siebesma, and Fredrik Jansson
Geosci. Model Dev., 17, 4053–4076, https://doi.org/10.5194/gmd-17-4053-2024, https://doi.org/10.5194/gmd-17-4053-2024, 2024
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Traditionally, high-resolution atmospheric models employ periodic boundary conditions, which limit simulations to domains without horizontal variations. In this research open boundary conditions are developed to replace the periodic boundary conditions. The implementation is tested in a controlled setup, and the results show minimal disturbances. Using these boundary conditions, high-resolution models can be forced by a coarser model to study atmospheric phenomena in realistic background states.
Caroline Arnold, Shivani Sharma, Tobias Weigel, and David S. Greenberg
Geosci. Model Dev., 17, 4017–4029, https://doi.org/10.5194/gmd-17-4017-2024, https://doi.org/10.5194/gmd-17-4017-2024, 2024
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In atmospheric models, rain formation is simplified to be computationally efficient. We trained a machine learning model, SuperdropNet, to emulate warm-rain formation based on super-droplet simulations. Here, we couple SuperdropNet with an atmospheric model in a warm-bubble experiment and find that the coupled simulation runs stable and produces reasonable results, making SuperdropNet a viable ML proxy for droplet simulations. We also present a comprehensive benchmark for coupling architectures.
Byoung-Joo Jung, Benjamin Ménétrier, Chris Snyder, Zhiquan Liu, Jonathan J. Guerrette, Junmei Ban, Ivette Hernández Baños, Yonggang G. Yu, and William C. Skamarock
Geosci. Model Dev., 17, 3879–3895, https://doi.org/10.5194/gmd-17-3879-2024, https://doi.org/10.5194/gmd-17-3879-2024, 2024
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We describe the multivariate static background error covariance (B) for the JEDI-MPAS 3D-Var data assimilation system. With tuned B parameters, the multivariate B gives physically balanced analysis increment fields in the single-observation test framework. In the month-long cycling experiment with a global 60 km mesh, 3D-Var with static B performs stably. Due to its simple workflow and minimal computational requirements, JEDI-MPAS 3D-Var can be useful for the research community.
Michal Belda, Nina Benešová, Jaroslav Resler, Peter Huszár, Ondřej Vlček, Pavel Krč, Jan Karlický, Pavel Juruš, and Kryštof Eben
Geosci. Model Dev., 17, 3867–3878, https://doi.org/10.5194/gmd-17-3867-2024, https://doi.org/10.5194/gmd-17-3867-2024, 2024
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For modeling atmospheric chemistry, it is necessary to provide data on emissions of pollutants. These can come from various sources and in various forms, and preprocessing of the data to be ingestible by chemistry models can be quite challenging. We developed the FUME processor to use a database layer that internally transforms all input data into a rigid structure, facilitating further processing to allow for emission processing from the continental to the street scale.
Bent Harnist, Seppo Pulkkinen, and Terhi Mäkinen
Geosci. Model Dev., 17, 3839–3866, https://doi.org/10.5194/gmd-17-3839-2024, https://doi.org/10.5194/gmd-17-3839-2024, 2024
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Probabilistic precipitation nowcasting (local forecasting for 0–6 h) is crucial for reducing damage from events like flash floods. For this goal, we propose the DEUCE neural-network-based model which uses data and model uncertainties to generate an ensemble of potential precipitation development scenarios for the next hour. Trained and evaluated with Finnish precipitation composites, DEUCE was found to produce more skillful and reliable nowcasts than established models.
Emma Howard, Steven Woolnough, Nicholas Klingaman, Daniel Shipley, Claudio Sanchez, Simon C. Peatman, Cathryn E. Birch, and Adrian J. Matthews
Geosci. Model Dev., 17, 3815–3837, https://doi.org/10.5194/gmd-17-3815-2024, https://doi.org/10.5194/gmd-17-3815-2024, 2024
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This paper describes a coupled atmosphere–mixed-layer ocean simulation setup that will be used to study weather processes in Southeast Asia. The set-up has been used to compare high-resolution simulations, which are able to partially resolve storms, to coarser simulations, which cannot. We compare the model performance at representing variability of rainfall and sea surface temperatures across length scales between the coarse and fine models.
Andrés Yarce Botero, Michiel van Weele, Arjo Segers, Pier Siebesma, and Henk Eskes
Geosci. Model Dev., 17, 3765–3781, https://doi.org/10.5194/gmd-17-3765-2024, https://doi.org/10.5194/gmd-17-3765-2024, 2024
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HARMONIE WINS50 reanalysis data with 0.025° × 0.025° resolution from 2019 to 2021 were coupled with the LOTOS-EUROS Chemical Transport Model. HARMONIE and ECMWF meteorology configurations against Cabauw observations (52.0° N, 4.9° W) were evaluated as simulated NO2 concentrations with ground-level sensors. Differences in crucial meteorological input parameters (boundary layer height, vertical diffusion coefficient) between the hydrostatic and non-hydrostatic models were analysed.
Ulrich Voggenberger, Leopold Haimberger, Federico Ambrogi, and Paul Poli
Geosci. Model Dev., 17, 3783–3799, https://doi.org/10.5194/gmd-17-3783-2024, https://doi.org/10.5194/gmd-17-3783-2024, 2024
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This paper presents a method for calculating balloon drift from historical radiosonde ascent data. The drift can reach distances of several hundred kilometres and is often neglected. Verification shows the beneficial impact of the more accurate balloon position on model assimilation. The method is not limited to radiosondes but would also work for dropsondes, ozonesondes, or any other in situ sonde carried by the wind in the pre-GNSS era, provided the necessary information is available.
Philippe Thunis, Jeroen Kuenen, Enrico Pisoni, Bertrand Bessagnet, Manjola Banja, Lech Gawuc, Karol Szymankiewicz, Diego Guizardi, Monica Crippa, Susana Lopez-Aparicio, Marc Guevara, Alexander De Meij, Sabine Schindlbacher, and Alain Clappier
Geosci. Model Dev., 17, 3631–3643, https://doi.org/10.5194/gmd-17-3631-2024, https://doi.org/10.5194/gmd-17-3631-2024, 2024
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An ensemble emission inventory is created with the aim of monitoring the status and progress made with the development of EU-wide inventories. This emission ensemble serves as a common benchmark for the screening and allows for the comparison of more than two inventories at a time. Because the emission “truth” is unknown, the approach does not tell which inventory is the closest to reality, but it identifies inconsistencies that require special attention.
Laurent Menut, Bertrand Bessagnet, Arineh Cholakian, Guillaume Siour, Sylvain Mailler, and Romain Pennel
Geosci. Model Dev., 17, 3645–3665, https://doi.org/10.5194/gmd-17-3645-2024, https://doi.org/10.5194/gmd-17-3645-2024, 2024
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This study is about the modelling of the atmospheric composition in Europe during the summer of 2022, when massive wildfires were observed. It is a sensitivity study dedicated to the relative impacts of two modelling processes that are able to modify the meteorology used for the calculation of the atmospheric chemistry and transport of pollutants.
Shuai Wang, Mengyuan Zhang, Yueqi Gao, Peng Wang, Qingyan Fu, and Hongliang Zhang
Geosci. Model Dev., 17, 3617–3629, https://doi.org/10.5194/gmd-17-3617-2024, https://doi.org/10.5194/gmd-17-3617-2024, 2024
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Numerical models are widely used in air pollution modeling but suffer from significant biases. The machine learning model designed in this study shows high efficiency in identifying such biases. Meteorology (relative humidity and cloud cover), chemical composition (secondary organic components and dust aerosols), and emission sources (residential activities) are diagnosed as the main drivers of bias in modeling PM2.5, a typical air pollutant. The results will help to improve numerical models.
Shoma Yamanouchi, Shayamilla Mahagammulla Gamage, Sara Torbatian, Jad Zalzal, Laura Minet, Audrey Smargiassi, Ying Liu, Ling Liu, Forood Azargoshasbi, Jinwoong Kim, Youngseob Kim, Daniel Yazgi, and Marianne Hatzopoulou
Geosci. Model Dev., 17, 3579–3597, https://doi.org/10.5194/gmd-17-3579-2024, https://doi.org/10.5194/gmd-17-3579-2024, 2024
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Air pollution is a major health hazard, and chemical transport models (CTMs) are valuable tools that aid in our understanding of the risks of air pollution at both local and regional scales. In this study, the Polair3D CTM of the Polyphemus air quality modeling platform was set up over Quebec, Canada, to assess the model’s capability in predicting key air pollutant species over the region, at seasonal temporal scales and at regional spatial scales.
Rohith Thundathil, Florian Zus, Galina Dick, and Jens Wickert
Geosci. Model Dev., 17, 3599–3616, https://doi.org/10.5194/gmd-17-3599-2024, https://doi.org/10.5194/gmd-17-3599-2024, 2024
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Global Navigation Satellite Systems (GNSS) provides moisture observations through its densely distributed ground station network. In this research, we assimilate a new type of observation called tropospheric gradient observations, which has never been incorporated into a weather model. We develop a forward operator for gradient-based observations and conduct an assimilation impact study. The study shows significant improvements in the model's humidity fields.
Ankur Mahesh, Travis A. O'Brien, Burlen Loring, Abdelrahman Elbashandy, William Boos, and William D. Collins
Geosci. Model Dev., 17, 3533–3557, https://doi.org/10.5194/gmd-17-3533-2024, https://doi.org/10.5194/gmd-17-3533-2024, 2024
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Atmospheric rivers (ARs) are extreme weather events that can alleviate drought or cause billions of US dollars in flood damage. We train convolutional neural networks (CNNs) to detect ARs with an estimate of the uncertainty. We present a framework to generalize these CNNs to a variety of datasets of past, present, and future climate. Using a simplified simulation of the Earth's atmosphere, we validate the CNNs. We explore the role of ARs in maintaining energy balance in the Earth system.
Alexandra Rivera, Kostas Tsigaridis, Gregory Faluvegi, and Drew Shindell
Geosci. Model Dev., 17, 3487–3505, https://doi.org/10.5194/gmd-17-3487-2024, https://doi.org/10.5194/gmd-17-3487-2024, 2024
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This paper describes and evaluates an improvement to the representation of acetone in the GISS ModelE2.1 Earth system model. We simulate acetone's concentration and transport across the atmosphere as well as its dependence on chemistry, the ocean, and various global emissions. Comparisons of our model’s estimates to past modeling studies and field measurements have shown encouraging results. Ultimately, this paper contributes to a broader understanding of acetone's role in the atmosphere.
Alok K. Samantaray, Priscilla A. Mooney, and Carla A. Vivacqua
Geosci. Model Dev., 17, 3321–3339, https://doi.org/10.5194/gmd-17-3321-2024, https://doi.org/10.5194/gmd-17-3321-2024, 2024
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Any interpretation of climate model data requires a comprehensive evaluation of the model performance. Numerous error metrics exist for this purpose, and each focuses on a specific aspect of the relationship between reference and model data. Thus, a comprehensive evaluation demands the use of multiple error metrics. However, this can lead to confusion. We propose a clustering technique to reduce the number of error metrics needed and a composite error metric to simplify the interpretation.
Richard Maier, Fabian Jakub, Claudia Emde, Mihail Manev, Aiko Voigt, and Bernhard Mayer
Geosci. Model Dev., 17, 3357–3383, https://doi.org/10.5194/gmd-17-3357-2024, https://doi.org/10.5194/gmd-17-3357-2024, 2024
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Based on the TenStream solver, we present a new method to accelerate 3D radiative transfer towards the speed of currently used 1D solvers. Using a shallow-cumulus-cloud time series, we evaluate the performance of this new solver in terms of both speed and accuracy. Compared to a 3D benchmark simulation, we show that our new solver is able to determine much more accurate irradiances and heating rates than a 1D δ-Eddington solver, even when operated with a similar computational demand.
Julia Maillard, Jean-Christophe Raut, and François Ravetta
Geosci. Model Dev., 17, 3303–3320, https://doi.org/10.5194/gmd-17-3303-2024, https://doi.org/10.5194/gmd-17-3303-2024, 2024
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Atmospheric models struggle to reproduce the strong temperature inversions in the vicinity of the surface over forested areas in the Arctic winter. In this paper, we develop modified simplified versions of surface layer schemes widely used by the community. Our modifications are used to correct the fact that original schemes place strong limits on the turbulent collapse, leading to a lower surface temperature gradient at low wind speeds. Modified versions show a better performance.
Jana Fischereit, Henrik Vedel, Xiaoli Guo Larsén, Natalie E. Theeuwes, Gregor Giebel, and Eigil Kaas
Geosci. Model Dev., 17, 2855–2875, https://doi.org/10.5194/gmd-17-2855-2024, https://doi.org/10.5194/gmd-17-2855-2024, 2024
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Wind farms impact local wind and turbulence. To incorporate these effects in weather forecasting, the explicit wake parameterization (EWP) is added to the forecasting model HARMONIE–AROME. We evaluate EWP using flight data above and downstream of wind farms, comparing it with an alternative wind farm parameterization and another weather model. Results affirm the correct implementation of EWP, emphasizing the necessity of accounting for wind farm effects in accurate weather forecasting.
Clément Bouvier, Daan van den Broek, Madeleine Ekblom, and Victoria A. Sinclair
Geosci. Model Dev., 17, 2961–2986, https://doi.org/10.5194/gmd-17-2961-2024, https://doi.org/10.5194/gmd-17-2961-2024, 2024
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An analytical initial background state has been developed for moist baroclinic wave simulation on an aquaplanet and implemented into OpenIFS. Seven parameters can be controlled, which are used to generate the background states and the development of baroclinic waves. The meteorological and numerical stability has been assessed. Resulting baroclinic waves have proven to be realistic and sensitive to the jet's width.
Jelena Radović, Michal Belda, Jaroslav Resler, Kryštof Eben, Martin Bureš, Jan Geletič, Pavel Krč, Hynek Řezníček, and Vladimír Fuka
Geosci. Model Dev., 17, 2901–2927, https://doi.org/10.5194/gmd-17-2901-2024, https://doi.org/10.5194/gmd-17-2901-2024, 2024
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Boundary conditions are of crucial importance for numerical model (e.g., PALM) validation studies and have a large influence on the model results, especially when studying the atmosphere of real, complex, and densely built urban environments. Our experiments with different driving conditions for the large-eddy simulation model PALM show its strong dependency on boundary conditions, which is important for the proper separation of errors coming from the boundary conditions and the model itself.
Siyuan Chen, Yi Zhang, Yiming Wang, Zhuang Liu, Xiaohan Li, and Wei Xue
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-68, https://doi.org/10.5194/gmd-2024-68, 2024
Revised manuscript accepted for GMD
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This study explores strategies and techniques for implementing mixed-precision code optimization within an atmosphere model dynamical core. The equation terms in the governing equations that are sensitive (insensitive) to the precision level have been identified. The performance of mixed-precision computing for weather and climate simulations was analyzed.
Manu Anna Thomas, Klaus Wyser, Shiyu Wang, Marios Chatziparaschos, Paraskevi Georgakaki, Montserrat Costa-Surós, Maria Gonçalves Ageitos, Maria Kanakidou, Carlos Pérez García-Pando, Athanasios Nenes, Twan van Noije, Philippe Le Sager, and Abhay Devasthale
EGUsphere, https://doi.org/10.5194/egusphere-2024-248, https://doi.org/10.5194/egusphere-2024-248, 2024
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Aerosol-cloud interactions occur at a range of spatio-temporal scales. While evaluating recent developments in EC-Earth3-AerChem model, this study aims to understand the extent to which Twomey effect manifests itself at larger scales. We report a reduction in the warm bias over the Southern Ocean due to model improvements. While we do see footprints of Twomey effect at larger scales, the negative relationship between cloud droplet number and liquid water drives the shortwave radiative effect.
Sonya L. Fiddes, Marc D. Mallet, Alain Protat, Matthew T. Woodhouse, Simon P. Alexander, and Kalli Furtado
Geosci. Model Dev., 17, 2641–2662, https://doi.org/10.5194/gmd-17-2641-2024, https://doi.org/10.5194/gmd-17-2641-2024, 2024
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In this study we present an evaluation that considers complex, non-linear systems in a holistic manner. This study uses XGBoost, a machine learning algorithm, to predict the simulated Southern Ocean shortwave radiation bias in the ACCESS model using cloud property biases as predictors. We then used a novel feature importance analysis to quantify the role that each cloud bias plays in predicting the radiative bias, laying the foundation for advanced Earth system model evaluation and development.
Gaurav Govardhan, Sachin D. Ghude, Rajesh Kumar, Sumit Sharma, Preeti Gunwani, Chinmay Jena, Prafull Yadav, Shubhangi Ingle, Sreyashi Debnath, Pooja Pawar, Prodip Acharja, Rajmal Jat, Gayatry Kalita, Rupal Ambulkar, Santosh Kulkarni, Akshara Kaginalkar, Vijay K. Soni, Ravi S. Nanjundiah, and Madhavan Rajeevan
Geosci. Model Dev., 17, 2617–2640, https://doi.org/10.5194/gmd-17-2617-2024, https://doi.org/10.5194/gmd-17-2617-2024, 2024
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A newly developed air quality forecasting framework, Decision Support System (DSS), for air quality management in Delhi, India, provides source attribution with numerous emission reduction scenarios besides forecasts. DSS shows that during post-monsoon and winter seasons, Delhi and its neighboring districts contribute to 30 %–40 % each to pollution in Delhi. On average, a 40 % reduction in the emissions in Delhi and the surrounding districts would result in a 24 % reduction in Delhi's pollution.
Simon Rosanka, Holger Tost, Rolf Sander, Patrick Jöckel, Astrid Kerkweg, and Domenico Taraborrelli
Geosci. Model Dev., 17, 2597–2615, https://doi.org/10.5194/gmd-17-2597-2024, https://doi.org/10.5194/gmd-17-2597-2024, 2024
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The capabilities of the Modular Earth Submodel System (MESSy) are extended to account for non-equilibrium aqueous-phase chemistry in the representation of deliquescent aerosols. When applying the new development in a global simulation, we find that MESSy's bias in modelling routinely observed reduced inorganic aerosol mass concentrations, especially in the United States. Furthermore, the representation of fine-aerosol pH is particularly improved in the marine boundary layer.
Cited articles
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Short summary
Novel techniques for modelling the aerosol–cloud interactions are implemented in a cloud-resolving model. The new methods improve the representation of the poorly constrained effects of cloud processing, precipitation and the wet removal of particles on the aerosol population and the associated feedbacks. The detailed representation of these processes yields more realistic simulation of the evolution of boundary layer clouds and fogs, as compared to results obtained using more simple methods.
Novel techniques for modelling the aerosol–cloud interactions are implemented in a...
