Articles | Volume 17, issue 20
https://doi.org/10.5194/gmd-17-7401-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/gmd-17-7401-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Development and technical paper
| 
25 Oct 2024
Development and technical paper |
| 25 Oct 2024
| 25 Oct 2024
Recommended coupling to global meteorological fields for long-term tracer simulations with WRF-GHG
Department of Biogeochemical Signals, Max Planck Institute for Biogeochemistry, Jena, Germany
Michał Gałkowski
Department of Biogeochemical Signals, Max Planck Institute for Biogeochemistry, Jena, Germany
Faculty of Physics and Applied Computer Science, AGH University of Kraków, Kraków, Poland
Friedemann Reum
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt, Oberpfaffenhofen, Germany
Santiago Botía
Department of Biogeochemical Signals, Max Planck Institute for Biogeochemistry, Jena, Germany
Julia Marshall
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt, Oberpfaffenhofen, Germany
Kai Uwe Totsche
Institute of Geosciences, Department of Hydrogeology, Friedrich Schiller University Jena, Jena, Germany
Christoph Gerbig
Department of Biogeochemical Signals, Max Planck Institute for Biogeochemistry, Jena, Germany
Related authors
Noelia R. Benavente, Santiago Botía, Luciana V. Rizzo, Angel Vara-Vela, Paulo Artaxo, Hella van Asperen, Felipe Santos da Silva, Flavio A. F. D'Oliveira, Horst Fischer, Michał Gałkowski, Theo Glauch, Alice Henkes, David Ho, Cléo Q. Dias-Júnior, Amauri C. P. Junior, Julia Marshall, Linda Ort, Ben-Hur M. Portella, and Luiz A. T. Machado
EGUsphere, https://doi.org/10.5194/egusphere-2026-979, https://doi.org/10.5194/egusphere-2026-979, 2026
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
The Amazon Basin plays a vital role in regulating Earth's climate by absorbing and releasing carbon dioxide and methane. We studied how a high-resolution atmospheric transport model captures these gases, comparing it with measurements from towers and aircraft over the forest. Adjusting for forest carbon exchange improved carbon dioxide results, while methane levels were heavily dependent on emission estimates. Remaining errors were linked to winds and atmospheric mixing.
Noelia R. Benavente, Santiago Botía, Luciana V. Rizzo, Angel Vara-Vela, Paulo Artaxo, Hella van Asperen, Felipe Santos da Silva, Flavio A. F. D'Oliveira, Horst Fischer, Michał Gałkowski, Theo Glauch, Alice Henkes, David Ho, Cléo Q. Dias-Júnior, Amauri C. P. Junior, Julia Marshall, Linda Ort, Ben-Hur M. Portella, and Luiz A. T. Machado
EGUsphere, https://doi.org/10.5194/egusphere-2026-979, https://doi.org/10.5194/egusphere-2026-979, 2026
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
The Amazon Basin plays a vital role in regulating Earth's climate by absorbing and releasing carbon dioxide and methane. We studied how a high-resolution atmospheric transport model captures these gases, comparing it with measurements from towers and aircraft over the forest. Adjusting for forest carbon exchange improved carbon dioxide results, while methane levels were heavily dependent on emission estimates. Remaining errors were linked to winds and atmospheric mixing.
Michael Weimer, Maximilian Reuter, Michael Hilker, Stefan Noël, Michael Buchwitz, Yasjka Meijer, Rüdiger Lang, Julia Marshall, Heinrich Bovensmann, John P. Burrows, and Hartmut Bösch
EGUsphere, https://doi.org/10.5194/egusphere-2026-1458, https://doi.org/10.5194/egusphere-2026-1458, 2026
This preprint is open for discussion and under review for Atmospheric Measurement Techniques (AMT).
Short summary
Short summary
Greenhouse gas column measurements from space using reflected sunlight have to make assumptions about the Earth's surface elevation. Usually, it assumed that the elevation representing the satellite's spatial sample is the unweighted average of high-resolution surface elevation data. We find and show with many examples that the surface elevation should be weighted by the surface reflectance in the respective wavelength bands. This improves errors in the retrieval of trace gases.
Fabian Maier, Christian Rödenbeck, Ute Karstens, Frank-Thomas Koch, Maksym Gachkivskyi, Andrew Smerald, and Christoph Gerbig
EGUsphere, https://doi.org/10.5194/egusphere-2026-739, https://doi.org/10.5194/egusphere-2026-739, 2026
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
Transport model errors represent a major source of uncertainty in greenhouse gas flux estimates derived from inverse modelling, yet they remain challenging to quantify. In our study, we leverage the similarities in the atmospheric transport of methane (CH4) and radon (222Rn) by performing a dual-tracer CH4-222Rn inversion over Europe, with the goal of enhancing the reliability of CH4 flux estimates. We discuss the benefits and limitations of this dual-tracer approach.
Amauri C. Prudente Jr., Luiz A. T. Machado, Felipe S. Silva, Tercio Ambrizzi, Paulo Artaxo, Santiago Botia, Luan P. Cordeiro, Cleo Q. Dias Jr., Edmilson Freitas, Demerval S. Moreira, Christopher Pöhlker, Ivan M. C. Toro, Xiyan Xu, and Luciana V. Rizzo
Biogeosciences, 23, 1771–1793, https://doi.org/10.5194/bg-23-1771-2026, https://doi.org/10.5194/bg-23-1771-2026, 2026
Short summary
Short summary
This study propoes a new method of spatialization to estimate carbon fluxes in the Brazilian Amazon biome. To do so, was used a land surface model (JULES) and two vegetation properties. The results of this spatialization resulted in a carbon fluxes of -1.34 Pg C during the year of 2021 in the entire Brazilian Amazon biome being the states of Amapa and Acre main relevant regions of carbon source.
Samuel Upton, Markus Reichstein, Wouter Peters, Santiago Botía, Jacob A. Nelson, Sophia Walther, Martin Jung, Fabian Gans, László Haszpra, and Ana Bastos
Atmos. Chem. Phys., 26, 2561–2595, https://doi.org/10.5194/acp-26-2561-2026, https://doi.org/10.5194/acp-26-2561-2026, 2026
Short summary
Short summary
We create a hybrid ecosystem-level carbon flux model using both eddy-covariance observations and observations of the atmospheric mole fraction of CO2 at three tall-tower observatories. Our study uses an atmospheric transport model (STILT) to connect the atmospheric signal to the ecosystem-level model. We show that this inclusion of atmospheric information meaningfully improves the model's representation of the interannual variability of the global net flux of CO2.
Anne-Wil van den Berg, Joram J. D. Hooghiem, Auke M. van der Woude, Pieter Rijsdijk, Roland Vernooij, Santiago Botia, Guido R. van der Werf, John B. Miller, Ingrid T. Luijkx, Maarten C. Krol, and Wouter Peters
EGUsphere, https://doi.org/10.5194/egusphere-2025-6213, https://doi.org/10.5194/egusphere-2025-6213, 2026
Short summary
Short summary
We estimate 2019 Brazilian fire carbon monoxide (CO) emissions using CO retrievals from different satellite instruments in a new top-down inversion framework. The retrievals strongly constrain fire emissions and complement existing inventories. National-scale posterior emissions align well with the new GFED5.1 inventory, supporting progress in fire emission modelling. Yet, posterior emissions in the Cerrado and Caatinga are systematically higher than inventories, we discuss potential drivers.
Paul Waldmann, Max Eckl, Leon Knez, Klaus-Dirk Gottschaldt, Alina Fiehn, Christian Mallaun, Michał Gałkowski, Christoph Kiemle, Ronald Hutjes, Thomas Röckmann, Huilin Chen, and Anke Roiger
Atmos. Meas. Tech., 19, 185–210, https://doi.org/10.5194/amt-19-185-2026, https://doi.org/10.5194/amt-19-185-2026, 2026
Short summary
Short summary
Nitrous oxide and methane emissions from agriculture need to be reduced, therefore emissions must be understood to effectively mitigate them. This is the first approach to measure those emissions aircraft-based, to assess their magnitude and drivers. We identified emission hotspots and temporal changes in agricultural emissions in the Netherlands. Our approach is applicable to further greenhouse gas emitters, therefore it builds a step towards more comprehensive emission quantification.
Carla Souza, Anne C. S. Mendonça, Hella Van Asperen, Flávio A. D’Oliveira, Santiago Botía, Luís G. N. Martins, Denisi H. Hall, Raoni A. Santana, Gilberto Fisch, Leonardo R. Oliveira, Jailson R. Mata, Ranyelli Figueiredo, Bruno T. T. Portela, Carlos A. Quesada, and Cléo Q. Dias-Júnior
EGUsphere, https://doi.org/10.5194/egusphere-2025-6531, https://doi.org/10.5194/egusphere-2025-6531, 2026
Short summary
Short summary
We investigated how the height of the nocturnal air layer (hn) above the Amazon forest changes over the year and how this influences gas measurements. Using two years of tower observations, we found that this layer is higher during wetter periods and much lower during dry periods linked to large climate events. hn can controls how gases accumulate or disperse at night, which affects how we interpret observations and improve weather and climate predictions.
Eleftherios Ioannidis, Antoon Meesters, Michael Steiner, Dominik Brunner, Friedemann Reum, Isabelle Pison, Antoine Berchet, Rona Thompson, Espen Sollum, Frank-Thomas Koch, Christoph Gerbig, Fenjuan Wang, Shamil Maksyutov, Aki Tsuruta, Maria Tenkanen, Tuula Aalto, Guillaume Monteil, Hong Lin, Ge Ren, Marko Scholze, and Sander Houweling
Earth Syst. Sci. Data, 18, 167–198, https://doi.org/10.5194/essd-18-167-2026, https://doi.org/10.5194/essd-18-167-2026, 2026
Short summary
Short summary
This paper describes a detailed study on CH4 European emissions, using different methodologies (9 total inverse models). The study spans over 15 years and provides detailed information on European CH4 emission trends and seasonality, using in-situ data, including Integrated Carbon Observation System (ICOS) network. Our results highlight the importance of improving details in the inversion setup, such as the treatment of lateral boundary conditions to narrow the uncertainty ranges further.
Martijn M. T. A. Pallandt, Abhishek Chatterjee, Lesley E. Ott, Julia Marshall, and Mathias Göckede
Atmos. Meas. Tech., 18, 7053–7073, https://doi.org/10.5194/amt-18-7053-2025, https://doi.org/10.5194/amt-18-7053-2025, 2025
Short summary
Short summary
Climate change is greatly affecting the Arctic. Among these changes is the thawing of permanently frozen soil, which may increase the release of methane, a powerful greenhouse gas (GHG). In this study we investigated the capabilities of tall GHG measuring towers and two satellite systems to detect this methane release. We find that these systems have different strengths and weaknesses, and that individually they struggle to detect these changes, though combined they might cover their weak spots.
Dieu Anh Tran, Jordi Vilà-Guerau de Arellano, Ingrid T. Luijkx, Christoph Gerbig, Michał Gałkowski, Santiago Botía, Kim Faassen, and Sönke Zaehle
Atmos. Chem. Phys., 25, 16553–16588, https://doi.org/10.5194/acp-25-16553-2025, https://doi.org/10.5194/acp-25-16553-2025, 2025
Short summary
Short summary
Analysis of CH4 data (2010–2021) from ZOtino Tall Tower Observatory in Central Siberia shows an increase in the late summer diurnal amplitude, driven by nighttime emissions. These trends correlate with rising soil temperature and moisture during the late summer and snow depth of the preceding spring. Peaks in 2012 and 2019 emission link to wildfires activity. Findings suggest wetlands as key CH4 sources and underscore the need for ongoing high-resolution monitoring in this region.
Sven Krautwurst, Christian Fruck, Sebastian Wolff, Jakob Borchardt, Oke Huhs, Konstantin Gerilowski, Michał Gałkowski, Christoph Kiemle, Mathieu Quatrevalet, Martin Wirth, Christian Mallaun, John P. Burrows, Christoph Gerbig, Andreas Fix, Hartmut Bösch, and Heinrich Bovensmann
Atmos. Chem. Phys., 25, 14669–14702, https://doi.org/10.5194/acp-25-14669-2025, https://doi.org/10.5194/acp-25-14669-2025, 2025
Short summary
Short summary
Anomalously high CH4 emissions from landfills in Madrid, Spain, have been observed by satellite measurements in recent years. Our investigations of these waste facilities, using passive and active airborne remote sensing measurements, confirm these high emission rates with values of up to 13 th−1 during the overflight and show excellent agreement between the two techniques. A large fraction of the emissions is attributed to active landfill sites.
Carlos A. Sierra, Ingrid Chanca, Meinrat O. Andreae, Alessandro Carioca de Araújo, Hella van Asperen, Lars Borchardt, Santiago Botía, Luiz Antonio Candido, Caio S. C. Correa, Cléo Quaresma Dias-Junior, Markus Eritt, Annica Fröhlich, Luciana V. Gatti, Marcus Guderle, Samuel Hammer, Martin Heimann, Viviana Horna, Armin Jordan, Steffen Knabe, Richard Kneißl, Jost Valentin Lavric, Ingeborg Levin, Kita Macario, Juliana Menger, Heiko Moossen, Carlos Alberto Quesada, Michael Rothe, Christian Rödenbeck, Yago Santos, Axel Steinhof, Bruno Takeshi, Susan Trumbore, and Sönke Zaehle
Earth Syst. Sci. Data, 17, 5871–5884, https://doi.org/10.5194/essd-17-5871-2025, https://doi.org/10.5194/essd-17-5871-2025, 2025
Short summary
Short summary
We present here a unique dataset of atmospheric observations of greenhouse gases and isotopes that provide key information on land-atmosphere interactions for the Amazon forests of central Brazil. The data show a relatively large level of variability, but also important trends in greenhouse gases, and signals from fires as well as seasonal biological activity.
Michał Gałkowski, Julia Marshall, Blanca Fuentes Andrade, and Christoph Gerbig
Atmos. Chem. Phys., 25, 13831–13848, https://doi.org/10.5194/acp-25-13831-2025, https://doi.org/10.5194/acp-25-13831-2025, 2025
Short summary
Short summary
Observations of greenhouse gas emissions are needed to monitor the progress towards Paris Agreement goals. Remote sensing instruments have been used to estimate emissions from the strongest anthropogenic sources. Here, we study the impact of atmospheric turbulence on the estimation of CO₂ with a realistic atmospheric model, and we show that the formation of persistent plume structures causes uncertainty on the order of 10 % of total emission that cannot be avoided.
Fabian Maier, Eva Falge, Maksym Gachkivskyi, Stephan Henne, Ute Karstens, Dafina Kikaj, Ingeborg Levin, Alistair Manning, Christian Rödenbeck, and Christoph Gerbig
Atmos. Chem. Phys., 25, 12779–12809, https://doi.org/10.5194/acp-25-12779-2025, https://doi.org/10.5194/acp-25-12779-2025, 2025
Short summary
Short summary
The radioactive noble gas radon (222Rn) is a suitable natural tracer for atmospheric transport and mixing processes that can be used to validate and calibrate atmospheric transport models. However, this requires accurate estimates of the 222Rn flux from the soil into the atmosphere. In our study, we evaluate the reliability of process-based 222Rn flux maps for Europe using a 222Rn inversion. Our inversion results can give some indications on how to improve the process-based 222Rn flux maps.
Theo Glauch, Julia Marshall, Christoph Gerbig, Santiago Botía, Michał Gałkowski, Sanam N. Vardag, and André Butz
Geosci. Model Dev., 18, 4713–4742, https://doi.org/10.5194/gmd-18-4713-2025, https://doi.org/10.5194/gmd-18-4713-2025, 2025
Short summary
Short summary
The Vegetation Photosynthesis and Respiration Model (VPRM) estimates carbon exchange between the atmosphere and biosphere by modeling gross primary production and respiration using satellite data and weather variables. Our new version, pyVPRM, supports diverse satellite products like Sentinel-2, MODIS, VIIRS, and new land cover maps, enabling high spatial and temporal resolution. This improves flux estimates, especially in complex landscapes, and ensures continuity as MODIS nears decommissioning.
Theertha Kariyathan, Ana Bastos, Markus Reichstein, Wouter Peters, and Julia Marshall
Atmos. Chem. Phys., 25, 7863–7878, https://doi.org/10.5194/acp-25-7863-2025, https://doi.org/10.5194/acp-25-7863-2025, 2025
Short summary
Short summary
The carbon uptake period (CUP) is the time period when land absorbs more CO2 than it emits. While atmospheric CO2 mole fraction measurements can be used to assess CUP changes, atmospheric transport and asynchronous timing across regions reduce the accuracy of the estimates. Forward model experiments show that only ~ 50 % of prescribed shifts in CUP timing applied to surface fluxes (ΔCUPNEE) are captured in simulated CO2 mole fraction data at monitoring sites like the Barrow Atmospheric Baseline Observatory.
Santiago Botía, Saqr Munassar, Thomas Koch, Danilo Custodio, Luana S. Basso, Shujiro Komiya, Jost V. Lavric, David Walter, Manuel Gloor, Giordane Martins, Stijn Naus, Gerbrand Koren, Ingrid T. Luijkx, Stijn Hantson, John B. Miller, Wouter Peters, Christian Rödenbeck, and Christoph Gerbig
Atmos. Chem. Phys., 25, 6219–6255, https://doi.org/10.5194/acp-25-6219-2025, https://doi.org/10.5194/acp-25-6219-2025, 2025
Short summary
Short summary
This study uses dry CO2 mole fractions from the Amazon Tall Tower Observatory together with airborne profiles to estimate net carbon exchange in tropical South America. We found that the biogeographic Amazon is a net carbon sink, while the Cerrado and Caatinga biomes are net carbon sources, resulting in an overall neutral balance. Finally, to further reduce the uncertainty in our estimates we call for an expansion of the monitoring capacity, especially in the Amazon–Andes foothills.
Joël Thanwerdas, Antoine Berchet, Lionel Constantin, Aki Tsuruta, Michael Steiner, Friedemann Reum, Stephan Henne, and Dominik Brunner
Geosci. Model Dev., 18, 1505–1544, https://doi.org/10.5194/gmd-18-1505-2025, https://doi.org/10.5194/gmd-18-1505-2025, 2025
Short summary
Short summary
The Community Inversion Framework (CIF) brings together methods for estimating greenhouse gas fluxes from atmospheric observations. The initial ensemble method implemented in CIF was found to be incomplete and could hardly be compared to other ensemble methods employed in the inversion community. In this paper, we present and evaluate a new implementation of the ensemble mode, building upon the initial developments.
Saqr Munassar, Christian Rödenbeck, Michał Gałkowski, Frank-Thomas Koch, Kai U. Totsche, Santiago Botía, and Christoph Gerbig
Atmos. Chem. Phys., 25, 639–656, https://doi.org/10.5194/acp-25-639-2025, https://doi.org/10.5194/acp-25-639-2025, 2025
Short summary
Short summary
CO2 mole fractions simulated over a global set of stations showed an overestimation of CO2 if the diurnal cycle is missing in biogenic fluxes. This leads to biases in the estimated fluxes derived from the regional-scale inversions. Interannual variability of estimated biogenic fluxes is also affected by the exclusion of the CO2 diurnal cycle. The findings point to the importance of including the diurnal variations of CO2 in the biogenic fluxes used as priors in global and regional inversions.
Luiz A. T. Machado, Jürgen Kesselmeier, Santiago Botía, Hella van Asperen, Meinrat O. Andreae, Alessandro C. de Araújo, Paulo Artaxo, Achim Edtbauer, Rosaria R. Ferreira, Marco A. Franco, Hartwig Harder, Sam P. Jones, Cléo Q. Dias-Júnior, Guido G. Haytzmann, Carlos A. Quesada, Shujiro Komiya, Jost Lavric, Jos Lelieveld, Ingeborg Levin, Anke Nölscher, Eva Pfannerstill, Mira L. Pöhlker, Ulrich Pöschl, Akima Ringsdorf, Luciana Rizzo, Ana M. Yáñez-Serrano, Susan Trumbore, Wanda I. D. Valenti, Jordi Vila-Guerau de Arellano, David Walter, Jonathan Williams, Stefan Wolff, and Christopher Pöhlker
Atmos. Chem. Phys., 24, 8893–8910, https://doi.org/10.5194/acp-24-8893-2024, https://doi.org/10.5194/acp-24-8893-2024, 2024
Short summary
Short summary
Composite analysis of gas concentration before and after rainfall, during the day and night, gives insight into the complex relationship between trace gas variability and precipitation. The analysis helps us to understand the sources and sinks of trace gases within a forest ecosystem. It elucidates processes that are not discernible under undisturbed conditions and contributes to a deeper understanding of the trace gas life cycle and its intricate interactions with cloud dynamics in the Amazon.
Dieu Anh Tran, Christoph Gerbig, Christian Rödenbeck, and Sönke Zaehle
Atmos. Chem. Phys., 24, 8413–8440, https://doi.org/10.5194/acp-24-8413-2024, https://doi.org/10.5194/acp-24-8413-2024, 2024
Short summary
Short summary
The analysis of the atmospheric CO2 record from the Zotino Tall Tower Observatory (ZOTTO) in central Siberia shows significant increases in the length and amplitude of the CO2 uptake and release in the 2010–2021 period. The trend shows a stronger increase in carbon release amplitude compared to the uptake, suggesting that, despite enhanced growing season uptake, during this period climate warming did not elevate the annual net CO2 uptake as cold-season respirations also responded to the warming.
Fabian Maier, Christian Rödenbeck, Ingeborg Levin, Christoph Gerbig, Maksym Gachkivskyi, and Samuel Hammer
Atmos. Chem. Phys., 24, 8183–8203, https://doi.org/10.5194/acp-24-8183-2024, https://doi.org/10.5194/acp-24-8183-2024, 2024
Short summary
Short summary
We investigate the usage of discrete radiocarbon (14C)-based fossil fuel carbon dioxide (ffCO2) concentration estimates vs. continuous carbon monoxide (CO)-based ffCO2 estimates to evaluate the seasonal cycle of ffCO2 emissions in an urban region with an inverse modeling framework. We find that the CO-based ffCO2 estimates allow us to reconstruct robust seasonal cycles, which show the distinct COVID-19 drawdown in 2020 and can be used to validate emission inventories.
Vishnu Thilakan, Dhanyalekshmi Pillai, Jithin Sukumaran, Christoph Gerbig, Haseeb Hakkim, Vinayak Sinha, Yukio Terao, Manish Naja, and Monish Vijay Deshpande
Atmos. Chem. Phys., 24, 5315–5335, https://doi.org/10.5194/acp-24-5315-2024, https://doi.org/10.5194/acp-24-5315-2024, 2024
Short summary
Short summary
This study investigates the usability of CO2 mixing ratio observations over India to infer regional carbon sources and sinks. We demonstrate that a high-resolution modelling system can represent the observed CO2 variations reasonably well by improving the transport and flux variations at a fine scale. Future carbon data assimilation systems can thus benefit from these recently available CO2 observations when fine-scale variations are adequately represented in the models.
Mirosław Zimnoch, Michał Gałkowski, Piotr Sekuła, Łukasz Chmura, Jakub Bartyzel, Alina Jasek-Kamińska, Alicja Skiba, Jarosław Nęcki, Przemysław Wachniew, and Paweł Jagoda
EGUsphere, https://doi.org/10.5194/egusphere-2024-1167, https://doi.org/10.5194/egusphere-2024-1167, 2024
Short summary
Short summary
The manuscript presents the dataset collected in the urban area of Krakow city containing several measurement campaigns focused on the investigation of vertical CO2 and CH4 profiles supplemented by set of meteorological parameters (e.g. temperature, pressure) measured along the profiles up to ca. 280 m a.g.l. The presented data collection explains the dynamics of the lower atmosphere on a daily and seasonal scale providing the three dimensional dataset that can be used for model validation.
Christian Rödenbeck, Karina E. Adcock, Markus Eritt, Maksym Gachkivskyi, Christoph Gerbig, Samuel Hammer, Armin Jordan, Ralph F. Keeling, Ingeborg Levin, Fabian Maier, Andrew C. Manning, Heiko Moossen, Saqr Munassar, Penelope A. Pickers, Michael Rothe, Yasunori Tohjima, and Sönke Zaehle
Atmos. Chem. Phys., 23, 15767–15782, https://doi.org/10.5194/acp-23-15767-2023, https://doi.org/10.5194/acp-23-15767-2023, 2023
Short summary
Short summary
The carbon dioxide content of the Earth atmosphere is increasing due to human emissions from burning of fossil fuels, causing global climate change. The strength of the fossil-fuel emissions is estimated by inventories based on energy data, but independent validation of these inventories has been recommended by the Intergovernmental Panel on Climate Change. Here we investigate the potential to validate inventories based on measurements of small changes in the atmospheric oxygen content.
Alina Fiehn, Maximilian Eckl, Julian Kostinek, Michał Gałkowski, Christoph Gerbig, Michael Rothe, Thomas Röckmann, Malika Menoud, Hossein Maazallahi, Martina Schmidt, Piotr Korbeń, Jarosław Neçki, Mila Stanisavljević, Justyna Swolkień, Andreas Fix, and Anke Roiger
Atmos. Chem. Phys., 23, 15749–15765, https://doi.org/10.5194/acp-23-15749-2023, https://doi.org/10.5194/acp-23-15749-2023, 2023
Short summary
Short summary
During the CoMet mission in the Upper Silesian Coal Basin (USCB) ground-based and airborne air samples were taken and analyzed for the isotopic composition of CH4 to derive the mean signature of the USCB and source signatures of individual coal mines. Using δ2H signatures, the biogenic emissions from the USCB account for 15 %–50 % of total emissions, which is underestimated in common emission inventories. This demonstrates the importance of δ2H-CH4 observations for methane source apportionment.
Xinxu Zhao, Jia Chen, Julia Marshall, Michal Gałkowski, Stephan Hachinger, Florian Dietrich, Ankit Shekhar, Johannes Gensheimer, Adrian Wenzel, and Christoph Gerbig
Atmos. Chem. Phys., 23, 14325–14347, https://doi.org/10.5194/acp-23-14325-2023, https://doi.org/10.5194/acp-23-14325-2023, 2023
Short summary
Short summary
We develop a modeling framework using the Weather Research and Forecasting model at a high spatial resolution (up to 400 m) to simulate atmospheric transport of greenhouse gases and interpret column observations. Output is validated against weather stations and column measurements in August 2018. The differential column method is applied, aided by air-mass transport tracing with the Stochastic Time-Inverted Lagrangian Transport (STILT) model, also for an exploratory measurement interpretation.
Matthew J. McGrath, Ana Maria Roxana Petrescu, Philippe Peylin, Robbie M. Andrew, Bradley Matthews, Frank Dentener, Juraj Balkovič, Vladislav Bastrikov, Meike Becker, Gregoire Broquet, Philippe Ciais, Audrey Fortems-Cheiney, Raphael Ganzenmüller, Giacomo Grassi, Ian Harris, Matthew Jones, Jürgen Knauer, Matthias Kuhnert, Guillaume Monteil, Saqr Munassar, Paul I. Palmer, Glen P. Peters, Chunjing Qiu, Mart-Jan Schelhaas, Oksana Tarasova, Matteo Vizzarri, Karina Winkler, Gianpaolo Balsamo, Antoine Berchet, Peter Briggs, Patrick Brockmann, Frédéric Chevallier, Giulia Conchedda, Monica Crippa, Stijn N. C. Dellaert, Hugo A. C. Denier van der Gon, Sara Filipek, Pierre Friedlingstein, Richard Fuchs, Michael Gauss, Christoph Gerbig, Diego Guizzardi, Dirk Günther, Richard A. Houghton, Greet Janssens-Maenhout, Ronny Lauerwald, Bas Lerink, Ingrid T. Luijkx, Géraud Moulas, Marilena Muntean, Gert-Jan Nabuurs, Aurélie Paquirissamy, Lucia Perugini, Wouter Peters, Roberto Pilli, Julia Pongratz, Pierre Regnier, Marko Scholze, Yusuf Serengil, Pete Smith, Efisio Solazzo, Rona L. Thompson, Francesco N. Tubiello, Timo Vesala, and Sophia Walther
Earth Syst. Sci. Data, 15, 4295–4370, https://doi.org/10.5194/essd-15-4295-2023, https://doi.org/10.5194/essd-15-4295-2023, 2023
Short summary
Short summary
Accurate estimation of fluxes of carbon dioxide from the land surface is essential for understanding future impacts of greenhouse gas emissions on the climate system. A wide variety of methods currently exist to estimate these sources and sinks. We are continuing work to develop annual comparisons of these diverse methods in order to clarify what they all actually calculate and to resolve apparent disagreement, in addition to highlighting opportunities for increased understanding.
Eliane Gomes Alves, Raoni Aquino Santana, Cléo Quaresma Dias-Júnior, Santiago Botía, Tyeen Taylor, Ana Maria Yáñez-Serrano, Jürgen Kesselmeier, Efstratios Bourtsoukidis, Jonathan Williams, Pedro Ivo Lembo Silveira de Assis, Giordane Martins, Rodrigo de Souza, Sérgio Duvoisin Júnior, Alex Guenther, Dasa Gu, Anywhere Tsokankunku, Matthias Sörgel, Bruce Nelson, Davieliton Pinto, Shujiro Komiya, Diogo Martins Rosa, Bettina Weber, Cybelli Barbosa, Michelle Robin, Kenneth J. Feeley, Alvaro Duque, Viviana Londoño Lemos, Maria Paula Contreras, Alvaro Idarraga, Norberto López, Chad Husby, Brett Jestrow, and Iván Mauricio Cely Toro
Atmos. Chem. Phys., 23, 8149–8168, https://doi.org/10.5194/acp-23-8149-2023, https://doi.org/10.5194/acp-23-8149-2023, 2023
Short summary
Short summary
Isoprene is emitted mainly by plants and can influence atmospheric chemistry and air quality. But, there are uncertainties in model emission estimates and follow-up atmospheric processes. In our study, with long-term observational datasets of isoprene and biological and environmental factors from central Amazonia, we show that isoprene emission estimates could be improved when biological processes were mechanistically incorporated into the model.
Theertha Kariyathan, Ana Bastos, Julia Marshall, Wouter Peters, Pieter Tans, and Markus Reichstein
Atmos. Meas. Tech., 16, 3299–3312, https://doi.org/10.5194/amt-16-3299-2023, https://doi.org/10.5194/amt-16-3299-2023, 2023
Short summary
Short summary
The timing and duration of the carbon uptake period (CUP) are sensitive to the occurrence of major phenological events, which are influenced by recent climate change. This study presents an ensemble-based approach for quantifying the timing and duration of the CUP and their uncertainty when derived from atmospheric CO2 measurements with noise and gaps. The CUP metrics derived with the approach are more robust and have less uncertainty than when estimated with the conventional methods.
Aparnna Ravi, Dhanyalekshmi Pillai, Christoph Gerbig, Stephen Sitch, Sönke Zaehle, Vishnu Thilakan, and Chandra Shekhar Jha
EGUsphere, https://doi.org/10.5194/egusphere-2023-817, https://doi.org/10.5194/egusphere-2023-817, 2023
Preprint archived
Short summary
Short summary
We derive high-resolution terrestrial CO2 fluxes over India from 2012 to 2020. This is achieved by utilizing satellite-based vegetation indices and meteorological data in a data-driven biospheric model. The model simulations are improved by incorporating soil variables and SIF retrievals from satellite instruments and relate them to ecosystem productivity across different biomes. The derived flux products better explain the flux variability compared to other existing model estimates.
Saqr Munassar, Guillaume Monteil, Marko Scholze, Ute Karstens, Christian Rödenbeck, Frank-Thomas Koch, Kai U. Totsche, and Christoph Gerbig
Atmos. Chem. Phys., 23, 2813–2828, https://doi.org/10.5194/acp-23-2813-2023, https://doi.org/10.5194/acp-23-2813-2023, 2023
Short summary
Short summary
Using different transport models results in large errors in optimized fluxes in the atmospheric inversions. Boundary conditions and inversion system configurations lead to a smaller but non-negligible impact. The findings highlight the importance to validate transport models for further developments but also to properly account for such errors in inverse modelling. This will help narrow the convergence of gas estimates reported in the scientific literature from different inversion frameworks.
Dominik Brunner, Gerrit Kuhlmann, Stephan Henne, Erik Koene, Bastian Kern, Sebastian Wolff, Christiane Voigt, Patrick Jöckel, Christoph Kiemle, Anke Roiger, Alina Fiehn, Sven Krautwurst, Konstantin Gerilowski, Heinrich Bovensmann, Jakob Borchardt, Michal Galkowski, Christoph Gerbig, Julia Marshall, Andrzej Klonecki, Pascal Prunet, Robert Hanfland, Margit Pattantyús-Ábrahám, Andrzej Wyszogrodzki, and Andreas Fix
Atmos. Chem. Phys., 23, 2699–2728, https://doi.org/10.5194/acp-23-2699-2023, https://doi.org/10.5194/acp-23-2699-2023, 2023
Short summary
Short summary
We evaluated six atmospheric transport models for their capability to simulate the CO2 plumes from two of the largest power plants in Europe by comparing the models against aircraft observations collected during the CoMet (Carbon Dioxide and Methane Mission) campaign in 2018. The study analyzed how realistically such plumes can be simulated at different model resolutions and how well the planned European satellite mission CO2M will be able to quantify emissions from power plants.
Auke M. van der Woude, Remco de Kok, Naomi Smith, Ingrid T. Luijkx, Santiago Botía, Ute Karstens, Linda M. J. Kooijmans, Gerbrand Koren, Harro A. J. Meijer, Gert-Jan Steeneveld, Ida Storm, Ingrid Super, Hubertus A. Scheeren, Alex Vermeulen, and Wouter Peters
Earth Syst. Sci. Data, 15, 579–605, https://doi.org/10.5194/essd-15-579-2023, https://doi.org/10.5194/essd-15-579-2023, 2023
Short summary
Short summary
To monitor the progress towards the CO2 emission goals set out in the Paris Agreement, the European Union requires an independent validation of emitted CO2. For this validation, atmospheric measurements of CO2 can be used, together with first-guess estimates of CO2 emissions and uptake. To quickly inform end users, it is imperative that this happens in near real-time. To aid these efforts, we create estimates of European CO2 exchange at high resolution in near real time.
Justyna Swolkień, Andreas Fix, and Michał Gałkowski
Atmos. Chem. Phys., 22, 16031–16052, https://doi.org/10.5194/acp-22-16031-2022, https://doi.org/10.5194/acp-22-16031-2022, 2022
Short summary
Short summary
Determination of emissions from coal mines on a local scale requires instantaneous data. We analysed temporal emission data for ventilation shafts and factors influencing their variability. They were saturation of the seams with methane, the permeability of the rock mass, and coal output. The data for the verification should reflect the actual values of emissions from point sources. It is recommended to achieve this by using a standardised emission measurement system for all coal mines.
Vishnu Thilakan, Dhanyalekshmi Pillai, Christoph Gerbig, Michal Galkowski, Aparnna Ravi, and Thara Anna Mathew
Atmos. Chem. Phys., 22, 15287–15312, https://doi.org/10.5194/acp-22-15287-2022, https://doi.org/10.5194/acp-22-15287-2022, 2022
Short summary
Short summary
This paper demonstrates how we can use atmospheric observations to improve the CO2 flux estimates in India. This is achieved by improving the representation of terrain, mesoscale transport, and flux variations. We quantify the impact of the unresolved variations in the current models on optimally estimated fluxes via inverse modelling and quantify the associated flux uncertainty. We illustrate how a parameterization scheme captures this variability in the coarse models.
Elise Potier, Grégoire Broquet, Yilong Wang, Diego Santaren, Antoine Berchet, Isabelle Pison, Julia Marshall, Philippe Ciais, François-Marie Bréon, and Frédéric Chevallier
Atmos. Meas. Tech., 15, 5261–5288, https://doi.org/10.5194/amt-15-5261-2022, https://doi.org/10.5194/amt-15-5261-2022, 2022
Short summary
Short summary
Atmospheric inversion at local–regional scales over Europe and pseudo-data assimilation are used to evaluate how CO2 and 14CO2 ground-based measurement networks could complement satellite CO2 imagers to monitor fossil fuel (FF) CO2 emissions. This combination significantly improves precision in the FF emission estimates in areas with a dense network but does not strongly support the separation of the FF from the biogenic signals or the spatio-temporal extrapolation of the satellite information.
Simone M. Pieber, Béla Tuzson, Stephan Henne, Ute Karstens, Christoph Gerbig, Frank-Thomas Koch, Dominik Brunner, Martin Steinbacher, and Lukas Emmenegger
Atmos. Chem. Phys., 22, 10721–10749, https://doi.org/10.5194/acp-22-10721-2022, https://doi.org/10.5194/acp-22-10721-2022, 2022
Short summary
Short summary
Understanding regional greenhouse gas emissions into the atmosphere is a prerequisite to mitigate climate change. In this study, we investigated the regional contributions of carbon dioxide (CO2) at the location of the high Alpine observatory Jungfraujoch (JFJ, Switzerland, 3580 m a.s.l.). To this purpose, we combined receptor-oriented atmospheric transport simulations for CO2 concentration in the period 2009–2017 with stable carbon isotope (δ13C–CO2) information.
Fabian Maier, Christoph Gerbig, Ingeborg Levin, Ingrid Super, Julia Marshall, and Samuel Hammer
Geosci. Model Dev., 15, 5391–5406, https://doi.org/10.5194/gmd-15-5391-2022, https://doi.org/10.5194/gmd-15-5391-2022, 2022
Short summary
Short summary
We show that the default representation of point source emissions in WRF–STILT leads to large overestimations when modelling fossil fuel CO2 concentrations for a 30 m high observation site during stable atmospheric conditions. We therefore introduce a novel point source modelling approach in WRF-STILT that takes into account their effective emission heights and results in a much better agreement with observations.
Saqr Munassar, Christian Rödenbeck, Frank-Thomas Koch, Kai U. Totsche, Michał Gałkowski, Sophia Walther, and Christoph Gerbig
Atmos. Chem. Phys., 22, 7875–7892, https://doi.org/10.5194/acp-22-7875-2022, https://doi.org/10.5194/acp-22-7875-2022, 2022
Short summary
Short summary
The results obtained from ensembles of inversions over 13 years show the largest spread in the a posteriori fluxes over the station set ensemble. Using different prior fluxes in the inversions led to a smaller impact. Drought occurrences in 2018 and 2019 affected CO2 fluxes as seen in net ecosystem exchange estimates. Our study highlights the importance of expanding the atmospheric site network across Europe to better constrain CO2 fluxes in inverse modelling.
Sven Krautwurst, Konstantin Gerilowski, Jakob Borchardt, Norman Wildmann, Michał Gałkowski, Justyna Swolkień, Julia Marshall, Alina Fiehn, Anke Roiger, Thomas Ruhtz, Christoph Gerbig, Jaroslaw Necki, John P. Burrows, Andreas Fix, and Heinrich Bovensmann
Atmos. Chem. Phys., 21, 17345–17371, https://doi.org/10.5194/acp-21-17345-2021, https://doi.org/10.5194/acp-21-17345-2021, 2021
Short summary
Short summary
Quantification of anthropogenic CH4 emissions remains challenging, but it is essential for near-term climate mitigation strategies. We use airborne remote sensing observations to assess bottom-up estimates of coal mining emissions from one of Europe's largest CH4 emission hot spots located in Poland. The analysis reveals that emissions from small groups of shafts can be disentangled, but caution is advised when comparing observations to commonly reported annual emissions.
Antoine Berchet, Espen Sollum, Rona L. Thompson, Isabelle Pison, Joël Thanwerdas, Grégoire Broquet, Frédéric Chevallier, Tuula Aalto, Adrien Berchet, Peter Bergamaschi, Dominik Brunner, Richard Engelen, Audrey Fortems-Cheiney, Christoph Gerbig, Christine D. Groot Zwaaftink, Jean-Matthieu Haussaire, Stephan Henne, Sander Houweling, Ute Karstens, Werner L. Kutsch, Ingrid T. Luijkx, Guillaume Monteil, Paul I. Palmer, Jacob C. A. van Peet, Wouter Peters, Philippe Peylin, Elise Potier, Christian Rödenbeck, Marielle Saunois, Marko Scholze, Aki Tsuruta, and Yuanhong Zhao
Geosci. Model Dev., 14, 5331–5354, https://doi.org/10.5194/gmd-14-5331-2021, https://doi.org/10.5194/gmd-14-5331-2021, 2021
Short summary
Short summary
We present here the Community Inversion Framework (CIF) to help rationalize development efforts and leverage the strengths of individual inversion systems into a comprehensive framework. The CIF is a programming protocol to allow various inversion bricks to be exchanged among researchers.
The ensemble of bricks makes a flexible, transparent and open-source Python-based tool. We describe the main structure and functionalities and demonstrate it in a simple academic case.
Piotr Sekuła, Anita Bokwa, Jakub Bartyzel, Bogdan Bochenek, Łukasz Chmura, Michał Gałkowski, and Mirosław Zimnoch
Atmos. Chem. Phys., 21, 12113–12139, https://doi.org/10.5194/acp-21-12113-2021, https://doi.org/10.5194/acp-21-12113-2021, 2021
Short summary
Short summary
The wind shear generated on a local scale by the diversified relief’s impact can be a factor which significantly modifies the spatial pattern of PM10 concentration. The vertical profile of PM10 over a city located in a large valley during the events with high surface-level PM10 concentrations may show a sudden decrease with height not only due to the increase in wind speed, but also due to the change in wind direction alone. Vertical aerosanitary urban zones can be distinguished.
Ana Maria Roxana Petrescu, Matthew J. McGrath, Robbie M. Andrew, Philippe Peylin, Glen P. Peters, Philippe Ciais, Gregoire Broquet, Francesco N. Tubiello, Christoph Gerbig, Julia Pongratz, Greet Janssens-Maenhout, Giacomo Grassi, Gert-Jan Nabuurs, Pierre Regnier, Ronny Lauerwald, Matthias Kuhnert, Juraj Balkovič, Mart-Jan Schelhaas, Hugo A. C. Denier van der
Gon, Efisio Solazzo, Chunjing Qiu, Roberto Pilli, Igor B. Konovalov, Richard A. Houghton, Dirk Günther, Lucia Perugini, Monica Crippa, Raphael Ganzenmüller, Ingrid T. Luijkx, Pete Smith, Saqr Munassar, Rona L. Thompson, Giulia Conchedda, Guillaume Monteil, Marko Scholze, Ute Karstens, Patrick Brockmann, and Albertus Johannes Dolman
Earth Syst. Sci. Data, 13, 2363–2406, https://doi.org/10.5194/essd-13-2363-2021, https://doi.org/10.5194/essd-13-2363-2021, 2021
Short summary
Short summary
This study is topical and provides a state-of-the-art scientific overview of data availability from bottom-up and top-down CO2 fossil emissions and CO2 land fluxes in the EU27+UK. The data integrate recent emission inventories with ecosystem data, land carbon models and regional/global inversions for the European domain, aiming at reconciling CO2 estimates with official country-level UNFCCC national GHG inventories in support to policy and facilitating real-time verification procedures.
Vishnu Thilakan, Dhanyalekshmi Pillai, Christoph Gerbig, Michal Galkowski, Aparnna Ravi, and Thara Anna Mathew
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-392, https://doi.org/10.5194/acp-2021-392, 2021
Revised manuscript not accepted
Short summary
Short summary
This paper demonstrates how we can make use of atmospheric observations to improve the CO2 flux estimates of India. This is achieved by improving the representation of terrain, mesoscale transport and flux variations. We quantify the impact of unresolved variations in the current models on optimally estimated fluxes via inverse modelling and quantify the associated flux uncertainty. We illustrate how a parameterization scheme captures this variability in the coarse models.
Cited articles
Agusti-Panareda, A., Diamantakis, M., Bayona, V., Klappenbach, F., and Butz, A.: Improving the inter-hemispheric gradient of total column atmospheric CO2 and CH4 in simulations with the ECMWF semi-Lagrangian atmospheric global model, Geosci. Model Dev., 10, 1–18, https://doi.org/10.5194/gmd-10-1-2017, 2017. a
Ahmadov, R., Gerbig, C., Kretschmer, R., Koerner, S., Neininger, B., Dolman, A. J., and Sarrat, C.: Mesoscale covariance of transport and CO2 fluxes: Evidence from observations and simulations using the WRF-VPRM coupled atmosphere-biosphere model, J. Geophys. Res.-Atmos., 112, D22107, https://doi.org/10.1029/2007JD008552, 2007. a, b
Ahmadov, R., McKeen, S. A., Robinson, A. L., Bahreini, R., Middlebrook, A. M., de Gouw, J. A., Meagher, J., Hsie, E.-Y., Edgerton, E., Shaw, S., and Trainer, M.: A volatility basis set model for summertime secondary organic aerosols over the eastern United States in 2006: A volatility basis set model for SOA, J. Geophys. Res.-Atmos., 117, D06301, https://doi.org/10.1029/2011JD016831, 2012. a
Baker, D. F., Law, R. M., Gurney, K. R., Rayner, P., Peylin, P., Denning, A. S., Bousquet, P., Bruhwiler, L., Chen, Y.-H., Ciais, P., Fung, I. Y., Heimann, M., John, J., Maki, T., Maksyutov, S., Masarie, K., Prather, M., Pak, B., Taguchi, S., and Zhu, Z.: TransCom 3 inversion intercomparison: Impact of transport model errors on the interannual variability of regional CO2 fluxes, 1988–2003: Transcom 3 – Interannual variability of CO2 sources, Global Biogeochem. Cy., 20, GB1002, https://doi.org/10.1029/2004GB002439, 2006. a
Beck, V., Koch, T., Kretschmer, R., Marshall, J., Ahmadov, R., Gerbig, C., Pillai, D., and Heimann, M.: The WRF Greenhouse Gas Model (WRF-GHG). Technical Report No. 25, Tech. rep., Max Planck Institute for Biogeochemistry, Jena, Germany, https://www.bgc-jena.mpg.de/bgc-systems/uploads/Wrf-ghg/Technical Reports 2011 Beck.pdf (last access: Feburary 2020), 2011. a, b
Beck, V., Gerbig, C., Koch, T., Bela, M. M., Longo, K. M., Freitas, S. R., Kaplan, J. O., Prigent, C., Bergamaschi, P., and Heimann, M.: WRF-Chem simulations in the Amazon region during wet and dry season transitions: evaluation of methane models and wetland inundation maps, Atmos. Chem. Phys., 13, 7961–7982, https://doi.org/10.5194/acp-13-7961-2013, 2013. a
Benjamin, S. G., Weygandt, S. S., Brown, J. M., Hu, M., Alexander, C. R., Smirnova, T. G., Olson, J. B., James, E. P., Dowell, D. C., Grell, G. A., Lin, H., Peckham, S. E., Smith, T. L., Moninger, W. R., Kenyon, J. S., and Manikin, G. S.: A North American Hourly Assimilation and Model Forecast Cycle: The Rapid Refresh, Mon. Weather Rev., 144, 1669–1694, https://doi.org/10.1175/MWR-D-15-0242.1, 2016. a, b, c
Bowden, J. H., Otte, T. L., Nolte, C. G., and Otte, M. J.: Examining Interior Grid Nudging Techniques Using Two-Way Nesting in the WRF Model for Regional Climate Modeling, J. Climate, 25, 2805–2823, https://doi.org/10.1175/JCLI-D-11-00167.1, 2012. a
Bowden, J. H., Nolte, C. G., and Otte, T. L.: Simulating the impact of the large-scale circulation on the 2 m temperature and precipitation climatology, Clim. Dynam., 40, 1903–1920, https://doi.org/10.1007/s00382-012-1440-y, 2013. a
Brunner, D., Kuhlmann, G., Marshall, J., Clément, V., Fuhrer, O., Broquet, G., Löscher, A., and Meijer, Y.: Accounting for the vertical distribution of emissions in atmospheric CO2 simulations, Atmos. Chem. Phys., 19, 4541–4559, https://doi.org/10.5194/acp-19-4541-2019, 2019. a
Bullock, O. R., Alapaty, K., Herwehe, J. A., Mallard, M. S., Otte, T. L., Gilliam, R. C., and Nolte, C. G.: An Observation-Based Investigation of Nudging in WRF for Downscaling Surface Climate Information to 12 km Grid Spacing, J. Appl. Meteorol. Clim., 53, 20–33, https://doi.org/10.1175/JAMC-D-13-030.1, 2014. a, b, c
Capecchi, V. and Brocca, L.: A simple assimilation method to ingest satellite soil moisture into a limited-area NWP model, Meteorol. Z., 23, 105–121, https://doi.org/10.1127/0941-2948/2014/0585, 2014. a
Chen, F. and Dudhia, J.: Coupling an Advanced Land Surface–Hydrology Model with the Penn State–NCAR MM5 Modeling System. Part I: Model Implementation and Sensitivity, Mon. Weather Rev., 129, 569–585, 2001. a
Chen, H. W., Zhang, F., Lauvaux, T., Davis, K. J., Feng, S., Butler, M. P., and Alley, R. B.: Characterization of Regional-Scale CO2 Transport Uncertainties in an Ensemble with Flow-Dependent Transport Errors, Geophys. Res. Lett., 46, 4049–4058, 2019. a
Danforth, C. M., Kalnay, E., and Miyoshi, T.: Estimating and Correcting Global Weather Model Error, Mon. Weather Rev., 135, 281–299, 2007. a
DelSole, T. and Hou, A. Y.: Empirical Correction of a Dynamical Model. Part I: Fundamental Issues, Mon. Weather Rev., 127, 2533–2545, 1999. a
Diamantakis, M. and Augusti-Panareda, A.: A positive definite tracer mass fixer for high resolution weather and atmospheric composition forecasts, ECMWF Technical Memorandum, 819, https://www.ecmwf.int/en/elibrary/17914-positive-definite-tracer-mass-fixer-high-resolution-weather-andatmospheric (last access: March 2021), 2017. a
Díaz Isaac, L. I., Lauvaux, T., Davis, K. J., Miles, N. L., Richardson, S. J., Jacobson, A. R., and Andrews, A. E.: Model-data comparison of MCI field campaign atmospheric CO2 mole fractions: CO2 model-data comparison, J. Geophys. Res.-Atmos., 119, 10536–10551, https://doi.org/10.1002/2014JD021593, 2014. a
Díaz-Isaac, L. I., Lauvaux, T., Bocquet, M., and Davis, K. J.: Calibration of a multi-physics ensemble for estimating the uncertainty of a greenhouse gas atmospheric transport model, Atmos. Chem. Phys., 19, 5695–5718, https://doi.org/10.5194/acp-19-5695-2019, 2019. a
Durre, I., Yin, X., Vose, R. S., Applequist, S., Arnfield, J., Korzeniewski, B., and Hundermark, B.: Integrated Global Radiosonde Archive (IGRA), Version 2, NOAA National Centers for Environmental Information, https://doi.org/10.7289/V5X63K0Q, 2016. a, b
ECMWF: IFS Documentation CY43R1 – Part IV: Physical Processes, https://doi.org/10.21957/sqvo5yxja, 2016. a
Feng, S., Lauvaux, T., Newman, S., Rao, P., Ahmadov, R., Deng, A., Díaz-Isaac, L. I., Duren, R. M., Fischer, M. L., Gerbig, C., Gurney, K. R., Huang, J., Jeong, S., Li, Z., Miller, C. E., O'Keeffe, D., Patarasuk, R., Sander, S. P., Song, Y., Wong, K. W., and Yung, Y. L.: Los Angeles megacity: a high-resolution land–atmosphere modelling system for urban CO2 emissions, Atmos. Chem. Phys., 16, 9019–9045, https://doi.org/10.5194/acp-16-9019-2016, 2016. a
Feng, S., Lauvaux, T., Davis, K. J., Keller, K., Zhou, Y., Williams, C., Schuh, A. E., Liu, J., and Baker, I.: Seasonal Characteristics of Model Uncertainties From Biogenic Fluxes, Transport, and Large-Scale Boundary Inflow in Atmospheric CO2 Simulations Over North America, J. Geophys. Res.-Atmos., 124, 14325–14346, https://doi.org/10.1029/2019JD031165, 2019a. a, b, c
Feng, S., Lauvaux, T., Keller, K., Davis, K. J., Rayner, P., Oda, T., and Gurney, K. R.: A Road Map for Improving the Treatment of Uncertainties in High-Resolution Regional Carbon Flux Inverse Estimates, Geophys. Res. Lett., 46, 13461–13469, https://doi.org/10.1029/2019GL082987, 2019b. a, b, c
Fiehn, A., Kostinek, J., Eckl, M., Klausner, T., Gałkowski, M., Chen, J., Gerbig, C., Röckmann, T., Maazallahi, H., Schmidt, M., Korbeń, P., Neçki, J., Jagoda, P., Wildmann, N., Mallaun, C., Bun, R., Nickl, A.-L., Jöckel, P., Fix, A., and Roiger, A.: Estimating CH4, CO2 and CO emissions from coal mining and industrial activities in the Upper Silesian Coal Basin using an aircraft-based mass balance approach, Atmos. Chem. Phys., 20, 12675–12695, https://doi.org/10.5194/acp-20-12675-2020, 2020a. a
Fiehn, A., Kostinek, J., Ecki, M., Klausner, T., Gałkowski, M., Chen, J., Gerbig, C., Röckmann, T., Maazallahi, H., Schmidt, M., Korbeń, P., Nȩcki Jarosław, Jagoda, P., Wildmann, N., Mallaun, C., Bun, R., Nicki, A.-L., Jöckel, P., Fix, A., and Rolger, A.: Atmospheric measurements results archive, Upper Silesian Coal Basin, Poland, ICOS [data set], https://doi.org/10.18160/0SFH-JJ93, 2020b. a, b
Gałkowski, M., Jordan, A., Rothe, M., Marshall, J., Koch, F.-T., Chen, J., Agusti-Panareda, A., Fix, A., and Gerbig, C.: In situ observations of greenhouse gases over Europe during the CoMet 1.0 campaign aboard the HALO aircraft, Atmos. Meas. Tech., 14, 1525–1544, https://doi.org/10.5194/amt-14-1525-2021, 2021. a, b
Gerken, T., Feng, S., Keller, K., Lauvaux, T., DiGangi, J. P., Choi, Y., Baier, B., and Davis, K. J.: Examining CO2 Model Observation Residuals Using ACT-America Data, J. Geophys. Res.-Atmos., 126, e2020JD034481, https://doi.org/10.1029/2020JD034481, 2021. a
Grell, G. A. and Freitas, S. R.: A scale and aerosol aware stochastic convective parameterization for weather and air quality modeling, Atmos. Chem. Phys., 14, 5233–5250, https://doi.org/10.5194/acp-14-5233-2014, 2014. a
Grell, G. A., Peckham, S. E., Schmitz, R., McKeen, S. A., Frost, G., Skamarock, W. C., and Eder, B.: Fully coupled “online” chemistry within the WRF model, Atmos. Environ., 39, 6957–6975, https://doi.org/10.1016/j.atmosenv.2005.04.027, 2005. a
Hersbach, H., Bell, B., Berrisford, P., Hirahara, S., Horányi, A., Muñoz-Sabater, J., Nicolas, J., Peubey, C., Radu, R., Schepers, D., Simmons, A., Soci, C., Abdalla, S., Abellan, X., Balsamo, G., Bechtold, P., Biavati, G., Bidlot, J., Bonavita, M., De Chiara, G., Dahlgren, P., Dee, D., Diamantakis, M., Dragani, R., Flemming, J., Forbes, R., Fuentes, M., Geer, A., Haimberger, L., Healy, S., Hogan, R. J., Hólm, E., Janisková, M., Keeley, S., Laloyaux, P., Lopez, P., Lupu, C., Radnoti, G., de Rosnay, P., Rozum, I., Vamborg, F., Villaume, S., and Thépaut, J.-N.: The ERA5 global reanalysis, Q. J. Roy. Meteor. Soc., 146, 1999–2049, https://doi.org/10.1002/qj.3803, 2020. a, b
Ho, D.: Video supplement for “Recommended coupling to global meteorological fields for long-term tracer simulations with WRF-GHG”, Zenodo [video], https://doi.org/10.5281/zenodo.7347056, 2022. a
Ho, D.: Data and scripts used in “Recommended coupling to global meteorological fields for long-term tracer simulations with WRF-GHG”, Zenodo [data set], https://doi.org/10.5281/zenodo.10581026, 2024. a, b
ICOS RI, Bergamaschi, P., Colomb, A., De Mazière, M., Emmenegger, L., Kubistin, D., Lehner, I., Lehtinen, K., Leuenberger, M., Lund Myhre, C., Marek, M., Platt, S. M., Plaß-Dülmer, C., Ramonet, M., Schmidt, M., Apadula, F., Arnold, S., Chen, H., Conil, S., Couret, C., Cristofanelli, P., Forster, G., Hatakka, J., Heliasz, M., Hermansen, O., Hoheisel, A., Kneuer, T., Laurila, T., Leskinen, A., Levula, J., Lindauer, M., Lopez, M., Mammarella, I., Manca, G., Meinhardt, F., Müller-Williams, J., Ottosson-Löfvenius, M., Piacentino, S., Pitt, J., Scheeren, B., Schumacher, M., Sha, M. K., Smith, P., Steinbacher, M., Sørensen, L. L., Vítková, G., Yver-Kwok, C., di Sarra, A., Conen, F., Kazan, V., Roulet, Y.-A., Biermann, T., Delmotte, M., Heltai, D., Komínková, K., Laurent, O., Lunder, C., Marklund, P., Pichon, J.-M., Trisolino, P., ICOS Atmosphere Thematic Centre, ICOS ERIC – Carbon Portal, ICOS Flask And Calibration Laboratory (FCL), ICOS Flask And Calibration Laboratory (FCL), and ICOS Central Radiocarbon Laboratory (CRL): ICOS Atmosphere Release 2022-1 of Level 2 Greenhouse Gas Mole Fractions of CO2, CH4, N2O, CO, meteorology and 14CO2, https://doi.org/10.18160/KCYX-HA35, 2022. a, b
Janssens-Maenhout, G., Crippa, M., Guizzardi, D., Muntean, M., and Schaaf, E.: Emissions Database for Global Atmospheric Research, version v4.3.2 part I Greenhouse gases (gridmaps), European Commission, Joint Research Centre (JRC) [data set], http://data.europa.eu/89h/jrc-edgar-edgar_v432_ghg_gridmaps (last access: August 2020), 2017. a
Janssens-Maenhout, G., Crippa, M., Guizzardi, D., Muntean, M., Schaaf, E., Dentener, F., Bergamaschi, P., Pagliari, V., Olivier, J. G. J., Peters, J. A. H. W., van Aardenne, J. A., Monni, S., Doering, U., Petrescu, A. M. R., Solazzo, E., and Oreggioni, G. D.: EDGAR v4.3.2 Global Atlas of the three major greenhouse gas emissions for the period 1970–2012, Earth Syst. Sci. Data, 11, 959–1002, https://doi.org/10.5194/essd-11-959-2019, 2019. a, b
Kim, W., Yum, S. S., Hong, J., and Song, J. I.: Improvement of Fog Simulation by the Nudging of Meteorological Tower Data in the WRF and PAFOG Coupled Model, Atmosphere, 11, 311, https://doi.org/10.3390/atmos11030311, 2020. a
Kuenen, J. J. P., Visschedijk, A. J. H., Jozwicka, M., and Denier van der Gon, H. A. C.: TNO-MACC_II emission inventory; a multi-year (2003–2009) consistent high-resolution European emission inventory for air quality modelling, Atmos. Chem. Phys., 14, 10963–10976, https://doi.org/10.5194/acp-14-10963-2014, 2014. a
Lauvaux, T. and Davis, K. J.: Planetary boundary layer errors in mesoscale inversions of column-integrated CO2 measurements, J. Geophys. Res.-Atmos., 119, 490–508, https://doi.org/10.1002/2013JD020175, 2014. a
Lauvaux, T., Pannekoucke, O., Sarrat, C., Chevallier, F., Ciais, P., Noilhan, J., and Rayner, P. J.: Structure of the transport uncertainty in mesoscale inversions of CO2 sources and sinks using ensemble model simulations, Biogeosciences, 6, 1089–1102, https://doi.org/10.5194/bg-6-1089-2009, 2009. a
Lin, J. C.: Accounting for the effect of transport errors on tracer inversions, Geophys. Res. Lett., 32, L01802, https://doi.org/10.1029/2004GL021127, 2005. a
Mahadevan, P., Wofsy, S. C., Matross, D. M., Xiao, X., Dunn, A. L., Lin, J. C., Gerbig, C., Munger, J. W., Chow, V. Y., and Gottlieb, E. W.: A satellite-based biosphere parameterization for net ecosystem CO2 exchange: Vegetation Photosynthesis and Respiration Model (VPRM): Net ecosystem exchange model, Global Biogeochem. Cy., 22, GB2005, https://doi.org/10.1029/2006GB002735, 2008. a, b
Markina, M., Gavrikov, A., Gulev, S., and Barnier, B.: Developing configuration of WRF model for long-term high-resolution wind wave hindcast over the North Atlantic with WAVEWATCH III, Ocean Dynam., 68, 1593–1604, https://doi.org/10.1007/s10236-018-1215-z, 2018. a
Miguez-Macho, G., Stenchikov, G. L., and Robock, A.: Spectral nudging to eliminate the effects of domain position and geometry in regional climate model simulations: Spectral nudging in regional models, J. Geophys. Res.-Atmos., 109, D13104, https://doi.org/10.1029/2003JD004495, 2004. a
Molteni, F., Buizza, R., Palmer, T. N., and Petroliagis, T.: The ECMWF Ensemble Prediction System: Methodology and validation, Q. J. Roy. Meteor. Soc., 122, 73–119, https://doi.org/10.1002/qj.49712252905, 1996. a
Nakanishi, M. and Niino, H.: An Improved Mellor–Yamada Level-3 Model: Its Numerical Stability and Application to a Regional Prediction of Advection Fog, Bound.-Lay. Meteorol., 119, 397–407, 2006. a
NOAA: NOAA Integrated Surface Database (ISD), NOAA [data set], https://registry.opendata.aws/noaa-isd, last access: May 2021. a
Pillai, D., Gerbig, C., Ahmadov, R., Rödenbeck, C., Kretschmer, R., Koch, T., Thompson, R., Neininger, B., and Lavrié, J. V.: High-resolution simulations of atmospheric CO2 over complex terrain – representing the Ochsenkopf mountain tall tower, Atmos. Chem. Phys., 11, 7445–7464, https://doi.org/10.5194/acp-11-7445-2011, 2011. a
Pleim, J. E. and Gilliam, R.: An Indirect Data Assimilation Scheme for Deep Soil Temperature in the Pleim–Xiu Land Surface Model, J. Appl. Meteorol. Clim., 48, 1362–1376, 2009. a
Rama, H.-O., Roberts, D., Tignor, M., Poloczanska, E., Mintenbeck, K., Alegría, A., Craig, M., Langsdorf, S., Löschke, S., Möller, V., Okem, A., Rama, B., and Ayanlade, S.: Climate Change 2022: Impacts, Adaptation and Vulnerability Working Group II Contribution to the Sixth Assessment Report of the Intergovernmental Panel on Climate Change, Cambridge University Press, https://doi.org/10.1017/9781009325844, 2022. a
Schuh, A. E., Denning, A. S., Corbin, K. D., Baker, I. T., Uliasz, M., Parazoo, N., Andrews, A. E., and Worthy, D. E. J.: A regional high-resolution carbon flux inversion of North America for 2004, Biogeosciences, 7, 1625–1644, https://doi.org/10.5194/bg-7-1625-2010, 2010. a
Seidel, D. J., Ao, C. O., and Li, K.: Estimating climatological planetary boundary layer heights from radiosonde observations: Comparison of methods and uncertainty analysis, J. Geophys. Res., 115, D16113, https://doi.org/10.1029/2009JD013680, 2010. a
Seidel, D. J., Zhang, Y., Beljaars, A., Golaz, J.-C., Jacobson, A. R., and Medeiros, B.: Climatology of the planetary boundary layer over the continental United States and Europe: Boundary layer climatology: U. S. and Europe, J. Geophys. Res.-Atmos., 117, D17106, https://doi.org/10.1029/2012JD018143, 2012. a
Simmons, A. J., Mureau, R., and Petroliagis, T.: Error growth and estimates of predictability from the ECMWF forecasting system, Q. J. Roy. Meteor. Soc., 121, 1739–1771, https://doi.org/10.1002/qj.49712152711, 1995. a
Skamarock, W. C., Klemp, J. B., Dudhia, J., Gill, D. O., Barker, D. M., Duda, M. G., Huang, X.-Y., Wang, W., and Powers, J. G.: A description of the Advanced Research WRF version 3, NCAR Technical note, WRF [code], https://www2.mmm.ucar.edu/wrf/users/download/get_source.html (last access: February 2020), 2008. a, b, c, d
Spero, T. L., Otte, M. J., Bowden, J. H., and Nolte, C. G.: Improving the representation of clouds, radiation, and precipitation using spectral nudging in the Weather Research and Forecasting model: Spectral Nudging of Moisture in WRF, J. Geophys. Res.-Atmos., 119, 11682–11694, https://doi.org/10.1002/2014JD022173, 2014. a, b
Spero, T. L., Nolte, C. G., Mallard, M. S., and Bowden, J. H.: A Maieutic Exploration of Nudging Strategies for Regional Climate Applications Using the WRF Model, J. Appl. Meteorol. Clim., 57, 1883–1906, https://doi.org/10.1175/JAMC-D-17-0360.1, 2018. a, b
Stauffer, D. R. and Seaman, N. L.: Use of Four-Dimensional Data Assimilation in a Limited-Area Mesoscale Model. Part I: Experiments with Synoptic-Scale Data, Mon. Weather Rev., 118, 1250–1277, https://doi.org/10.1175/1520-0493(1990)118<1250:UOFDDA>2.0.CO;2, 1990. a
Swolkień, J., Fix, A., and Gałkowski, M.: Factors influencing the temporal variability of atmospheric methane emissions from Upper Silesia coal mines: a case study from the CoMet mission, Atmos. Chem. Phys., 22, 16031–16052, https://doi.org/10.5194/acp-22-16031-2022, 2022. a, b
Vincent, C. L. and Hahmann, A. N.: The Impact of Grid and Spectral Nudging on the Variance of the Near-Surface Wind Speed, J. Appl. Meteorol. Clim., 54, 1021–1038, https://doi.org/10.1175/JAMC-D-14-0047.1, 2015. a, b, c
Vogelezang, D. H. P. and Holtslag, A. A. M.: Evaluation and model impacts of alternative boundary-layer height formulations, Bound.-Lay. Meteorol., 81, 245–269, https://doi.org/10.1007/BF02430331, 1996. a
Zittis, G., Bruggeman, A., Hadjinicolaou, P., Camera, C., and Lelieveld, J.: Effects of Meteorology Nudging in Regional Hydroclimatic Simulations of the Eastern Mediterranean, Atmosphere, 9, 470, https://doi.org/10.3390/atmos9120470, 2018. a, b, c
Short summary
Atmospheric model users often overlook the impact of the land–atmosphere interaction. This study accessed various setups of WRF-GHG simulations that ensure consistency between the model and driving reanalysis fields. We found that a combination of nudging and frequent re-initialization allows certain improvement by constraining the soil moisture fields and, through its impact on atmospheric mixing, improves atmospheric transport.
Atmospheric model users often overlook the impact of the land–atmosphere interaction. This study...
