Articles | Volume 17, issue 3
https://doi.org/10.5194/gmd-17-1217-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/gmd-17-1217-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Review and perspective paper
| 
14 Feb 2024
Review and perspective paper |
| 14 Feb 2024
| 14 Feb 2024
Towards the definition of a solar forcing dataset for CMIP7
Instituto de Astrofísica de Andalucía, CSIC, Granada, Spain
Thierry Dudok de Wit
LPC2E, University of Orléans, Orléans, France
International Space Science Institute, Bern, Switzerland
Ilaria Ermolli
INAF Osservatorio Astronomico di Roma, Monte Porzio Catone, Italy
Margit Haberreiter
Physical-Meteorological Observatory Davos/World Radiation Center, Davos, Switzerland
Doug Kinnison
National Center for Atmospheric Research, Boulder, CO 80301, USA
Daniel Marsh
National Center for Atmospheric Research, Boulder, CO 80301, USA
School of Physics and Astronomy, University of Leeds, Leeds, LS2 9JT, UK
Hilde Nesse
Department of Physics and Technology, University of Bergen, Bergen, Norway
Annika Seppälä
Department of Physics, University of Otago, Dunedin, New Zealand
Miriam Sinnhuber
Karlsruhe Institute of Technology, Karlsruhe, Germany
Ilya Usoskin
Space Physics and Astronomy Research Unit, University of Oulu, Finland
Sodankylä Geophysical Observatory, University of Oulu, Finland
Related authors
Norbert Glatthor, Gabriele P. Stiller, Thomas von Clarmann, Bernd Funke, Sylvia Kellmann, and Andrea Linden
Atmos. Chem. Phys., 25, 1175–1208, https://doi.org/10.5194/acp-25-1175-2025, https://doi.org/10.5194/acp-25-1175-2025, 2025
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We present global upper-tropospheric distributions of the pollutants HCN, CO, C2H2, C2H6, PAN, and HCOOH, observed between 2002 and 2012 by the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) on the Environmental Satellite (Envisat). By comparing the spatial distributions of their volume mixing ratios and by global correlation and regression analyses, we draw conclusions on their sources, such as biomass burning, anthropogenic sources, and biogenic release.
Maryam Ramezani Ziarani, Miriam Sinnhuber, Thomas Reddmann, Bernd Funke, Stefan Bender, and Michael Prather
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-227, https://doi.org/10.5194/gmd-2024-227, 2025
Preprint under review for GMD
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Our study aims to present a new method for incorporating top-down solar forcing into stratospheric ozone relying on linearized ozone scheme. The addition of geomagnetic forcing led to significant ozone losses in the polar upper stratosphere of both hemispheres due to the catalytic cycles involving NOy. In addition to the particle precipitation effect, accounting for solar UV variability in the ICON-ART model leads to the changes in ozone in the tropical stratosphere.
Florian Voet, Felix Plöger, Johannes Laube, Peter Preusse, Paul Konopka, Jens-Uwe Grooß, Jörn Ungermann, Björn-Martin Sinnhuber, Michael Hoepfner, Bernd Funke, Gerald Wetzel, Sören Johansson, Gabriele Stiller, Eric Ray, and Michaela Imelda Hegglin
EGUsphere, https://doi.org/10.5194/egusphere-2024-2624, https://doi.org/10.5194/egusphere-2024-2624, 2024
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This study refines estimates of the stratospheric “age of air,” a measure of how long air circulates in the stratosphere. By analyzing correlations between trace gases measurable by satellites, the research introduces a method that reduces uncertainties and detects small-scale atmospheric features. This improved understanding of stratospheric circulation is crucial for better climate models and predictions, enhancing our ability to assess the impacts of climate change on the atmosphere.
Miriam Sinnhuber, Christina Arras, Stefan Bender, Bernd Funke, Hanli Liu, Daniel R. Marsh, Thomas Reddmann, Eugene Rozanov, Timofei Sukhodolov, Monika E. Szelag, and Jan Maik Wissing
EGUsphere, https://doi.org/10.5194/egusphere-2024-2256, https://doi.org/10.5194/egusphere-2024-2256, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Formation of nitric oxide NO in the upper atmosphere varies with solar activity. Observations show that it starts a chain of processes in the entire atmosphere affecting the ozone layer and climate system. This is often underestimated in models. We compare five models which show large differences in simulated NO. Analysis of results point out problems related to the oxygen balance, and to the impact of atmospheric waves on dynamics. Both must be modeled well to reproduce the downward coupling.
Manuel López-Puertas, Federico Fabiano, Victor Fomichev, Bernd Funke, and Daniel R. Marsh
Geosci. Model Dev., 17, 4401–4432, https://doi.org/10.5194/gmd-17-4401-2024, https://doi.org/10.5194/gmd-17-4401-2024, 2024
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The radiative infrared cooling of CO2 in the middle atmosphere is crucial for computing its thermal structure. It requires one however to include non-local thermodynamic equilibrium processes which are computationally very expensive, which cannot be afforded by climate models. In this work, we present an updated, efficient, accurate and very fast (~50 µs) parameterization of that cooling able to cope with CO2 abundances from half the pre-industrial values to 10 times the current abundance.
Norbert Glatthor, Thomas von Clarmann, Bernd Funke, Maya García-Comas, Udo Grabowski, Michael Höpfner, Sylvia Kellmann, Michael Kiefer, Alexandra Laeng, Andrea Linden, Manuel López-Puertas, and Gabriele P. Stiller
Atmos. Meas. Tech., 17, 2849–2871, https://doi.org/10.5194/amt-17-2849-2024, https://doi.org/10.5194/amt-17-2849-2024, 2024
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We present global atmospheric methane (CH4) and nitrous oxide (N2O) distributions retrieved from measurements of the MIPAS instrument on board the Environmental Satellite (Envisat) during 2002 to 2012. Monitoring of these gases is of scientific interest because both of them are strong greenhouse gases. We analyze the latest, improved version of calibrated MIPAS measurements. Further, we apply a new retrieval scheme leading to an improved CH4 and N2O data product .
Gabriele P. Stiller, Thomas von Clarmann, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Michael Kiefer, Alexandra Laeng, Andrea Linden, Bernd Funke, Maya García-Comas, and Manuel López-Puertas
Atmos. Meas. Tech., 17, 1759–1789, https://doi.org/10.5194/amt-17-1759-2024, https://doi.org/10.5194/amt-17-1759-2024, 2024
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CFC-11, CFC-12, and HCFC-22 contribute to the depletion of ozone and are potent greenhouse gases. They have been banned by the Montreal protocol. With MIPAS on Envisat the atmospheric composition could be observed between 2002 and 2012. We present here the retrieval of their atmospheric distributions for the final data version 8. We characterise the derived data by their error budget and their spatial resolution. An additional representation for direct comparison to models is also provided.
Manuel López-Puertas, Maya García-Comas, Bernd Funke, Thomas von Clarmann, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Michael Kiefer, Alexandra Laeng, Andrea Linden, and Gabriele P. Stiller
Atmos. Meas. Tech., 16, 5609–5645, https://doi.org/10.5194/amt-16-5609-2023, https://doi.org/10.5194/amt-16-5609-2023, 2023
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This paper describes a new version (V8) of ozone data from MIPAS middle-atmosphere spectra. The dataset comprises high-quality ozone profiles from 20 to 100 km, with pole-to-pole latitude coverage for the day- and nighttime, spanning 2005 until 2012. An exhaustive treatment of errors has been performed. Compared to other satellite instruments, MIPAS ozone shows a positive bias of 5 %–8 % below 70 km. In the upper mesosphere, this new version agrees much better than previous ones (within 10 %).
Maya García-Comas, Bernd Funke, Manuel López-Puertas, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Michael Kiefer, Andrea Linden, Belén Martínez-Mondéjar, Gabriele P. Stiller, and Thomas von Clarmann
Atmos. Meas. Tech., 16, 5357–5386, https://doi.org/10.5194/amt-16-5357-2023, https://doi.org/10.5194/amt-16-5357-2023, 2023
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We have released version 8 of MIPAS IMK–IAA temperatures and pointing information retrieved from MIPAS Middle and Upper Atmosphere mode version 8.03 calibrated spectra, covering 20–115 km altitude. We considered non-local thermodynamic equilibrium emission explicitly for each limb scan, essential to retrieve accurate temperatures above the mid-mesosphere. Comparisons of this temperature dataset with SABER measurements show excellent agreement, improving those of previous MIPAS versions.
Monali Borthakur, Miriam Sinnhuber, Alexandra Laeng, Thomas Reddmann, Peter Braesicke, Gabriele Stiller, Thomas von Clarmann, Bernd Funke, Ilya Usoskin, Jan Maik Wissing, and Olesya Yakovchuk
Atmos. Chem. Phys., 23, 12985–13013, https://doi.org/10.5194/acp-23-12985-2023, https://doi.org/10.5194/acp-23-12985-2023, 2023
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Reduced ozone levels resulting from ozone depletion mean more exposure to UV radiation, which has various effects on human health. We analysed solar events to see what influence it has on the chemistry of Earth's atmosphere and how this atmospheric chemistry change can affect the ozone. To do this, we used an atmospheric model considering only chemistry and compared it with satellite data. The focus was mainly on the contribution of chlorine, and we found about 10 %–20 % ozone loss due to that.
Bernd Funke, Maya García-Comas, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Michael Kiefer, Andrea Linden, Manuel López-Puertas, Gabriele P. Stiller, and Thomas von Clarmann
Atmos. Meas. Tech., 16, 2167–2196, https://doi.org/10.5194/amt-16-2167-2023, https://doi.org/10.5194/amt-16-2167-2023, 2023
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New global nitric oxide (NO) volume-mixing-ratio and lower-thermospheric temperature data products, retrieved from Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) spectra with the IMK-IAA MIPAS data processor, have been released. The dataset covers the entire Envisat mission lifetime and includes retrieval results from all MIPAS observation modes. The data are based on ESA version 8 calibration and were processed using an improved retrieval approach.
Michael Kiefer, Thomas von Clarmann, Bernd Funke, Maya García-Comas, Norbert Glatthor, Udo Grabowski, Michael Höpfner, Sylvia Kellmann, Alexandra Laeng, Andrea Linden, Manuel López-Puertas, and Gabriele P. Stiller
Atmos. Meas. Tech., 16, 1443–1460, https://doi.org/10.5194/amt-16-1443-2023, https://doi.org/10.5194/amt-16-1443-2023, 2023
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A new ozone data set, derived from radiation measurements of the space-borne instrument MIPAS, is presented. It consists of more than 2 million single ozone profiles from 2002–2012, covering virtually all latitudes and altitudes between 5 and 70 km. Progress in data calibration and processing methods allowed for significant improvement of the data quality, compared to previous data versions. Hence, the data set will help to better understand e.g. the time evolution of ozone in the stratosphere.
Thomas von Clarmann, Norbert Glatthor, Udo Grabowski, Bernd Funke, Michael Kiefer, Anne Kleinert, Gabriele P. Stiller, Andrea Linden, and Sylvia Kellmann
Atmos. Meas. Tech., 15, 6991–7018, https://doi.org/10.5194/amt-15-6991-2022, https://doi.org/10.5194/amt-15-6991-2022, 2022
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Errors of profiles of temperature and mixing ratios retrieved from spectra recorded with the Michelson Interferometer for Passive Atmospheric Sounding are estimated. All known and quantified sources of uncertainty are considered. Some ongoing uncertaities contribute to both the random and to the systematic errors. In some cases, one source of uncertainty propagates onto the error budget via multiple pathways. Problems arise when the correlations of errors to be propagated are unknown.
Irina Mironova, Miriam Sinnhuber, Galina Bazilevskaya, Mark Clilverd, Bernd Funke, Vladimir Makhmutov, Eugene Rozanov, Michelle L. Santee, Timofei Sukhodolov, and Thomas Ulich
Atmos. Chem. Phys., 22, 6703–6716, https://doi.org/10.5194/acp-22-6703-2022, https://doi.org/10.5194/acp-22-6703-2022, 2022
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From balloon measurements, we detected unprecedented, extremely powerful, electron precipitation over the middle latitudes. The robustness of this event is confirmed by satellite observations of electron fluxes and chemical composition, as well as by ground-based observations of the radio signal propagation. The applied chemistry–climate model shows the almost complete destruction of ozone in the mesosphere over the region where high-energy electrons were observed.
Michael Kiefer, Thomas von Clarmann, Bernd Funke, Maya García-Comas, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Anne Kleinert, Alexandra Laeng, Andrea Linden, Manuel López-Puertas, Daniel R. Marsh, and Gabriele P. Stiller
Atmos. Meas. Tech., 14, 4111–4138, https://doi.org/10.5194/amt-14-4111-2021, https://doi.org/10.5194/amt-14-4111-2021, 2021
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An improved dataset of vertical temperature profiles of the Earth's atmosphere in the altitude range 5–70 km is presented. These profiles are derived from measurements of the MIPAS instrument onboard ESA's Envisat satellite. The overall improvements are based on upgrades in the input data and several improvements in the data processing approach. Both of these are discussed, and an extensive error discussion is included. Enhancements of the new dataset are demonstrated by means of examples.
Michaela I. Hegglin, Susann Tegtmeier, John Anderson, Adam E. Bourassa, Samuel Brohede, Doug Degenstein, Lucien Froidevaux, Bernd Funke, John Gille, Yasuko Kasai, Erkki T. Kyrölä, Jerry Lumpe, Donal Murtagh, Jessica L. Neu, Kristell Pérot, Ellis E. Remsberg, Alexei Rozanov, Matthew Toohey, Joachim Urban, Thomas von Clarmann, Kaley A. Walker, Hsiang-Jui Wang, Carlo Arosio, Robert Damadeo, Ryan A. Fuller, Gretchen Lingenfelser, Christopher McLinden, Diane Pendlebury, Chris Roth, Niall J. Ryan, Christopher Sioris, Lesley Smith, and Katja Weigel
Earth Syst. Sci. Data, 13, 1855–1903, https://doi.org/10.5194/essd-13-1855-2021, https://doi.org/10.5194/essd-13-1855-2021, 2021
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An overview of the SPARC Data Initiative is presented, to date the most comprehensive assessment of stratospheric composition measurements spanning 1979–2018. Measurements of 26 chemical constituents obtained from an international suite of space-based limb sounders were compiled into vertically resolved, zonal monthly mean time series. The quality and consistency of these gridded datasets are then evaluated using a climatological validation approach and a range of diagnostics.
Emily M. Gordon, Annika Seppälä, Bernd Funke, Johanna Tamminen, and Kaley A. Walker
Atmos. Chem. Phys., 21, 2819–2836, https://doi.org/10.5194/acp-21-2819-2021, https://doi.org/10.5194/acp-21-2819-2021, 2021
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Energetic particle precipitation (EPP) is the rain of solar energetic particles into the Earth's atmosphere. EPP is known to deplete O3 in the polar mesosphere–upper stratosphere via the formation of NOx. NOx also causes chlorine deactivation in the lower stratosphere and has, thus, been proposed to potentially result in reduced ozone depletion in the spring. We provide the first evidence to show that NOx formed by EPP is able to remove active chlorine, resulting in enhanced total ozone column.
Francesco Grieco, Kristell Pérot, Donal Murtagh, Patrick Eriksson, Peter Forkman, Bengt Rydberg, Bernd Funke, Kaley A. Walker, and Hugh C. Pumphrey
Atmos. Meas. Tech., 13, 5013–5031, https://doi.org/10.5194/amt-13-5013-2020, https://doi.org/10.5194/amt-13-5013-2020, 2020
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We present a unique – by time extension and geographical coverage – dataset of satellite observations of carbon monoxide (CO) in the mesosphere which will allow us to study dynamical processes, since CO is a very good tracer of circulation in the mesosphere. Previously, the dataset was unusable due to instrumental artefacts that affected the measurements. We identify the cause of the artefacts, eliminate them and prove the quality of the results by comparing with other instrument measurements.
Thomas von Clarmann, Douglas A. Degenstein, Nathaniel J. Livesey, Stefan Bender, Amy Braverman, André Butz, Steven Compernolle, Robert Damadeo, Seth Dueck, Patrick Eriksson, Bernd Funke, Margaret C. Johnson, Yasuko Kasai, Arno Keppens, Anne Kleinert, Natalya A. Kramarova, Alexandra Laeng, Bavo Langerock, Vivienne H. Payne, Alexei Rozanov, Tomohiro O. Sato, Matthias Schneider, Patrick Sheese, Viktoria Sofieva, Gabriele P. Stiller, Christian von Savigny, and Daniel Zawada
Atmos. Meas. Tech., 13, 4393–4436, https://doi.org/10.5194/amt-13-4393-2020, https://doi.org/10.5194/amt-13-4393-2020, 2020
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Remote sensing of atmospheric state variables typically relies on the inverse solution of the radiative transfer equation. An adequately characterized retrieval provides information on the uncertainties of the estimated state variables as well as on how any constraint or a priori assumption affects the estimate. This paper summarizes related techniques and provides recommendations for unified error reporting.
Pavle Arsenovic, Alessandro Damiani, Eugene Rozanov, Bernd Funke, Andrea Stenke, and Thomas Peter
Atmos. Chem. Phys., 19, 9485–9494, https://doi.org/10.5194/acp-19-9485-2019, https://doi.org/10.5194/acp-19-9485-2019, 2019
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Low-energy electrons (LEE) are the dominant source of odd nitrogen, which destroys ozone, in the mesosphere and stratosphere in polar winter in the geomagnetically active periods. However, the observed stratospheric ozone anomalies can be reproduced only when accounting for both low- and middle-range energy electrons (MEE) in the chemistry-climate model. Ozone changes may induce further dynamical and thermal changes in the atmosphere. We recommend including both LEE and MEE in climate models.
Mark E. Hervig, Benjamin T. Marshall, Scott M. Bailey, David E. Siskind, James M. Russell III, Charles G. Bardeen, Kaley A. Walker, and Bernd Funke
Atmos. Meas. Tech., 12, 3111–3121, https://doi.org/10.5194/amt-12-3111-2019, https://doi.org/10.5194/amt-12-3111-2019, 2019
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The Solar Occultation for Ice Experiment (SOFIE) has measured nitric oxide (NO) from satellite since 2007. The observations are validated through error analysis and comparisons with other satellite observations. Calculated SOFIE NO uncertainties are less than 50 % for altitudes from 40 to 140 km. SOFIE agrees with other measurements to within 50 % for altitudes from roughly 50 to 105 km for spacecraft sunrise and 50 to 140 km for sunsets.
Alexandra Laeng, Ellen Eckert, Thomas von Clarmann, Michael Kiefer, Daan Hubert, Gabriele Stiller, Norbert Glatthor, Manuel López-Puertas, Bernd Funke, Udo Grabowski, Johannes Plieninger, Sylvia Kellmann, Andrea Linden, Stefan Lossow, Arne Babenhauserheide, Lucien Froidevaux, and Kaley Walker
Atmos. Meas. Tech., 11, 4693–4705, https://doi.org/10.5194/amt-11-4693-2018, https://doi.org/10.5194/amt-11-4693-2018, 2018
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MIPAS was an IR limb emission spectrometer on the Envisat platform. From 2002 to 2012, it performed pole-to-pole measurements of ozone during day and night. ESA recently released the new version 7 of Level 1 MIPAS spectra, which is expected to reduce the long-term drift of the MIPAS Level 2 data. We evaluate the long-term stability of ozone Level 2 data from the KIT IMK processor. Our results indicate that MIPAS data are now even more suited for trend studies, alone or as part of merged data.
Manuel López-Puertas, Maya García-Comas, Bernd Funke, Angela Gardini, Gabriele P. Stiller, Thomas von Clarmann, Norbert Glatthor, Alexandra Laeng, Martin Kaufmann, Viktoria F. Sofieva, Lucien Froidevaux, Kaley A. Walker, and Masato Shiotani
Atmos. Meas. Tech., 11, 2187–2212, https://doi.org/10.5194/amt-11-2187-2018, https://doi.org/10.5194/amt-11-2187-2018, 2018
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This paper describes the inversion of O3 data from MIPAS middle atmosphere spectra which requires non-LTE. The O3 dataset comprises from 20 to 100 km, has a pole-to-pole latitude coverage, day and nighttime, and span from 2005 until 2012. A validation of the data against other satellite measurements and an overall description of O3 is also presented. This is an important dataset for the community and describes the major characteristics of stratospheric and mesospheric O3.
Miriam Sinnhuber, Uwe Berger, Bernd Funke, Holger Nieder, Thomas Reddmann, Gabriele Stiller, Stefan Versick, Thomas von Clarmann, and Jan Maik Wissing
Atmos. Chem. Phys., 18, 1115–1147, https://doi.org/10.5194/acp-18-1115-2018, https://doi.org/10.5194/acp-18-1115-2018, 2018
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Results from global models are used to analyze the impact of energetic particle precipitation on the middle atmosphere (10–80 km). Model results agree well with observations, and show strong enhancements of NOy, long-lasting ozone loss, and a net heating in the uppermost stratosphere (~35–45 km) during polar winter which changes sign in spring. Energetic particle precipitation therefore has the potential to impact atmospheric dynamics, starting from a warmer winter-time upper stratosphere.
Margarita Yela, Manuel Gil-Ojeda, Mónica Navarro-Comas, David Gonzalez-Bartolomé, Olga Puentedura, Bernd Funke, Javier Iglesias, Santiago Rodríguez, Omaira García, Héctor Ochoa, and Guillermo Deferrari
Atmos. Chem. Phys., 17, 13373–13389, https://doi.org/10.5194/acp-17-13373-2017, https://doi.org/10.5194/acp-17-13373-2017, 2017
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The paper focuses on stratospheric trends of NO2, a species involved in the ozone equilibrium, using data from four NDACC stations. The global stratospheric NO2 trend has not yet been established conclusively. We analyse DOAS data from stations in the Northern Hemisphere and Southern Hemisphere during 1993–2014. The most relevant finding is the hemispheric asymmetry found in the sign of the NO2 trend, providing further evidence of changes in the stratosphere dynamics on the global scale.
Gabriele P. Stiller, Federico Fierli, Felix Ploeger, Chiara Cagnazzo, Bernd Funke, Florian J. Haenel, Thomas Reddmann, Martin Riese, and Thomas von Clarmann
Atmos. Chem. Phys., 17, 11177–11192, https://doi.org/10.5194/acp-17-11177-2017, https://doi.org/10.5194/acp-17-11177-2017, 2017
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The discrepancy between modelled and observed 25-year trends of the strength of the stratospheric Brewer–Dobson circulation (BDC) is still not resolved. With our paper we trace the observed hemispheric dipole structure of age of air trends back to natural variability in shorter-term (decadal) time frames. Beyond this we demonstrate that after correction for the decadal natural variability the remaining trend for the first decade of the 21st century is consistent with model simulations.
Ellen Eckert, Thomas von Clarmann, Alexandra Laeng, Gabriele P. Stiller, Bernd Funke, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Michael Kiefer, Andrea Linden, Arne Babenhauserheide, Gerald Wetzel, Christopher Boone, Andreas Engel, Jeremy J. Harrison, Patrick E. Sheese, Kaley A. Walker, and Peter F. Bernath
Atmos. Meas. Tech., 10, 2727–2743, https://doi.org/10.5194/amt-10-2727-2017, https://doi.org/10.5194/amt-10-2727-2017, 2017
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We retrieved vertical profiles of CCl4 from MIPAS Envisat IMK/IAA data. A detailed description of all characteristics is included in the paper as well as comparisons with historical measurements and comparisons with collocated measurements of instruments covering the same time span as MIPAS Envisat. A particular focus also lies on the usage of a new CCl4 spectroscopic dataset introduced recently, which leads to more realistic CCl4 volume mixing ratios.
Cristen Adams, Adam E. Bourassa, Chris A. McLinden, Chris E. Sioris, Thomas von Clarmann, Bernd Funke, Landon A. Rieger, and Douglas A. Degenstein
Atmos. Chem. Phys., 17, 8063–8080, https://doi.org/10.5194/acp-17-8063-2017, https://doi.org/10.5194/acp-17-8063-2017, 2017
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We measured the relationship between volcanic aerosol and trace gases in the stratosphere using the OSIRIS and MIPAS satellite instruments between 2002 and 2014. We found that levels of stratospheric NO2 and N2O5 both decreased significantly in the presence of volcanic aerosol. These decreases were consistent with the modeling results.
Katja Matthes, Bernd Funke, Monika E. Andersson, Luke Barnard, Jürg Beer, Paul Charbonneau, Mark A. Clilverd, Thierry Dudok de Wit, Margit Haberreiter, Aaron Hendry, Charles H. Jackman, Matthieu Kretzschmar, Tim Kruschke, Markus Kunze, Ulrike Langematz, Daniel R. Marsh, Amanda C. Maycock, Stergios Misios, Craig J. Rodger, Adam A. Scaife, Annika Seppälä, Ming Shangguan, Miriam Sinnhuber, Kleareti Tourpali, Ilya Usoskin, Max van de Kamp, Pekka T. Verronen, and Stefan Versick
Geosci. Model Dev., 10, 2247–2302, https://doi.org/10.5194/gmd-10-2247-2017, https://doi.org/10.5194/gmd-10-2247-2017, 2017
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The solar forcing dataset for climate model experiments performed for the upcoming IPCC report is described. This dataset provides the radiative and particle input of solar variability on a daily basis from 1850 through to 2300. With this dataset a better representation of natural climate variability with respect to the output of the Sun is provided which provides the most sophisticated and comprehensive respresentation of solar variability that has been used in climate model simulations so far.
Bernd Funke, William Ball, Stefan Bender, Angela Gardini, V. Lynn Harvey, Alyn Lambert, Manuel López-Puertas, Daniel R. Marsh, Katharina Meraner, Holger Nieder, Sanna-Mari Päivärinta, Kristell Pérot, Cora E. Randall, Thomas Reddmann, Eugene Rozanov, Hauke Schmidt, Annika Seppälä, Miriam Sinnhuber, Timofei Sukhodolov, Gabriele P. Stiller, Natalia D. Tsvetkova, Pekka T. Verronen, Stefan Versick, Thomas von Clarmann, Kaley A. Walker, and Vladimir Yushkov
Atmos. Chem. Phys., 17, 3573–3604, https://doi.org/10.5194/acp-17-3573-2017, https://doi.org/10.5194/acp-17-3573-2017, 2017
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Simulations from eight atmospheric models have been compared to tracer and temperature observations from seven satellite instruments in order to evaluate the energetic particle indirect effect (EPP IE) during the perturbed northern hemispheric (NH) winter 2008/2009. Models are capable to reproduce the EPP IE in dynamically and geomagnetically quiescent NH winter conditions. The results emphasize the need for model improvements in the dynamical representation of elevated stratopause events.
Á. Aythami Jurado-Navarro, Manuel López-Puertas, Bernd Funke, Maya García-Comas, Angela Gardini, Francisco González-Galindo, Gabriele P. Stiller, Thomas von Clarmann, Udo Grabowski, and Andrea Linden
Atmos. Meas. Tech., 9, 6081–6100, https://doi.org/10.5194/amt-9-6081-2016, https://doi.org/10.5194/amt-9-6081-2016, 2016
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We present global distributions of CO2 concentrations in the upper atmosphere (70–140 km) derived from high-resolution 4.3 µm MIPAS spectra from 2005 to 2012. CO2 relative abundances have been measured at 120–140 km for the first time. The data have an unprecedented accuracy. CO2 shows a strong seasonal behaviour. CO2 largely controls the temperature of the upper atmosphere and its measurement is very important for understanding the impact of climate change in this region.
Patrick E. Sheese, Kaley A. Walker, Chris D. Boone, Chris A. McLinden, Peter F. Bernath, Adam E. Bourassa, John P. Burrows, Doug A. Degenstein, Bernd Funke, Didier Fussen, Gloria L. Manney, C. Thomas McElroy, Donal Murtagh, Cora E. Randall, Piera Raspollini, Alexei Rozanov, James M. Russell III, Makoto Suzuki, Masato Shiotani, Joachim Urban, Thomas von Clarmann, and Joseph M. Zawodny
Atmos. Meas. Tech., 9, 5781–5810, https://doi.org/10.5194/amt-9-5781-2016, https://doi.org/10.5194/amt-9-5781-2016, 2016
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This study validates version 3.5 of the ACE-FTS NOy species data sets by comparing diurnally scaled ACE-FTS data to correlative data from 11 other satellite limb sounders. For all five species examined (NO, NO2, HNO3, N2O5, and ClONO2), there is good agreement between ACE-FTS and the other data sets in various regions of the atmosphere. In these validated regions, these NOy data products can be used for further investigation into the composition, dynamics, and climate of the stratosphere.
Nathan P. Gillett, Hideo Shiogama, Bernd Funke, Gabriele Hegerl, Reto Knutti, Katja Matthes, Benjamin D. Santer, Daithi Stone, and Claudia Tebaldi
Geosci. Model Dev., 9, 3685–3697, https://doi.org/10.5194/gmd-9-3685-2016, https://doi.org/10.5194/gmd-9-3685-2016, 2016
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Detection and attribution of climate change is the process of determining the causes of observed climate changes, which has underpinned key conclusions on the role of human influence on climate in the reports of the Intergovernmental Panel on Climate Change (IPCC). This paper describes a coordinated set of climate model experiments that will form part of the Sixth Coupled Model Intercomparison Project and will support improved attribution of climate change in the next IPCC report.
Maya García-Comas, Francisco González-Galindo, Bernd Funke, Angela Gardini, Aythami Jurado-Navarro, Manuel López-Puertas, and William E. Ward
Atmos. Chem. Phys., 16, 11019–11041, https://doi.org/10.5194/acp-16-11019-2016, https://doi.org/10.5194/acp-16-11019-2016, 2016
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In this paper, for the first time, temperature longitudinal oscillations are derived from 20 to 150 km from a single instrument. A climatology of amplitudes and phases of zonal waves with odd daily frequencies is presented on a global scale. The interannual variability in amplitudes of the migrating modes shows a QBO in the MLT, which is probably originated in the stratosphere. The results are useful for testing general circulation models considering tidal effects in the MLT region.
E. Eckert, A. Laeng, S. Lossow, S. Kellmann, G. Stiller, T. von Clarmann, N. Glatthor, M. Höpfner, M. Kiefer, H. Oelhaf, J. Orphal, B. Funke, U. Grabowski, F. Haenel, A. Linden, G. Wetzel, W. Woiwode, P. F. Bernath, C. Boone, G. S. Dutton, J. W. Elkins, A. Engel, J. C. Gille, F. Kolonjari, T. Sugita, G. C. Toon, and K. A. Walker
Atmos. Meas. Tech., 9, 3355–3389, https://doi.org/10.5194/amt-9-3355-2016, https://doi.org/10.5194/amt-9-3355-2016, 2016
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We investigate the accuracy, precision and long-term stability of the MIPAS Envisat IMK/IAA CFC-11 (CCl3F) and CFC-12 (CCl2F2) products.
For comparisons we use several data products from satellite, airplane and balloon-borne instruments as well as ground-based data.
MIPAS Envisat CFC-11 has a slight high bias at the lower end of the profile.
CFC-12 agrees well with other data products.
The temporal stability is good up to ~ 30 km, but still leaves room for improvement.
Bernd Funke, Manuel López-Puertas, Gabriele P. Stiller, Stefan Versick, and Thomas von Clarmann
Atmos. Chem. Phys., 16, 8667–8693, https://doi.org/10.5194/acp-16-8667-2016, https://doi.org/10.5194/acp-16-8667-2016, 2016
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We present a semi-empirical model for the reconstruction of polar winter descent of reactive nitrogen (NOy) produced by energetic particle precipitation (EPP) into the stratosphere. It can be used to prescribe NOy in chemistry climate models with an upper lid below the EPP source region. We also found a significant reduction of the EPP-generated NOy during the last 30 years, likely affecting the long-term NOy trend by counteracting the expected increase caused by growing N2O emission.
Maya García-Comas, Manuel López-Puertas, Bernd Funke, Á. Aythami Jurado-Navarro, Angela Gardini, Gabriele P. Stiller, Thomas von Clarmann, and Michael Höpfner
Atmos. Chem. Phys., 16, 6701–6719, https://doi.org/10.5194/acp-16-6701-2016, https://doi.org/10.5194/acp-16-6701-2016, 2016
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We have analysed IR measurements of PMCs in the NH and SH from 2005 to 2012. This technique is sensitive to the total ice volume independent of particle size. For the first time, we have measured the total ice volume from the midlatitudes to the poles. The data indicate a layer of ice from 81 to 89 km and from the poles to 50–60º in each hemisphere, increasing near the poles. The ice density is larger in the NH than in the SH and located 1 km lower. PMCs also show a diurnal variation.
S. Tegtmeier, M. I. Hegglin, J. Anderson, B. Funke, J. Gille, A. Jones, L. Smith, T. von Clarmann, and K. A. Walker
Earth Syst. Sci. Data, 8, 61–78, https://doi.org/10.5194/essd-8-61-2016, https://doi.org/10.5194/essd-8-61-2016, 2016
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The first comprehensive intercomparison of CFC-11, CFC-12, HF, and SF6 satellite data was performed as part of the SPARC Data Initiative following a new "top-down" concept of satellite measurement validation and thus providing a global picture of the data characteristics. The comparisons will provide basic information on quality and consistency of the various data sets and will serve as a guide for their use in empirical studies of climate and variability, and in model-measurement comparisons.
F. J. Haenel, G. P. Stiller, T. von Clarmann, B. Funke, E. Eckert, N. Glatthor, U. Grabowski, S. Kellmann, M. Kiefer, A. Linden, and T. Reddmann
Atmos. Chem. Phys., 15, 13161–13176, https://doi.org/10.5194/acp-15-13161-2015, https://doi.org/10.5194/acp-15-13161-2015, 2015
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Stratospheric circulation is thought to change as a consequence of climate change. Empirical evidence, however, is sparse. In this paper we present latitude- and altitude-resolved trends of the mean age of stratospheric air as derived from SF6 measurements performed by the MIPAS satellite instrument. The mean of the age of stratospheric air is a measure of the intensity of the Brewer-Dobson circulation. In this paper we discuss differences with respect to a preceding analysis by Stiller et al.
S. Bender, M. Sinnhuber, T. von Clarmann, G. Stiller, B. Funke, M. López-Puertas, J. Urban, K. Pérot, K. A. Walker, and J. P. Burrows
Atmos. Meas. Tech., 8, 4171–4195, https://doi.org/10.5194/amt-8-4171-2015, https://doi.org/10.5194/amt-8-4171-2015, 2015
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We compare the nitric oxide (NO) daily zonal mean number density data sets in the mesosphere and lower thermosphere (MLT, 60km to 150km) from four instruments: ACE-FTS (2004--2010), MIPAS (2005--2012), SCIAMACHY (2008--2012), and SMR (2003--2012). We find that these data sets from different instruments consistently constrain NO in the MLT. Thus, they offer reliable forcing inputs for climate and chemistry climate models as an initial step to include solar and geomagnetic activity.
C. McLandress, T. G. Shepherd, A. I. Jonsson, T. von Clarmann, and B. Funke
Atmos. Chem. Phys., 15, 9271–9284, https://doi.org/10.5194/acp-15-9271-2015, https://doi.org/10.5194/acp-15-9271-2015, 2015
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This is the first paper of its kind describing a method for merging the long-term satellite records of global stratospheric temperature from SSU and AMSU to yield a continuous data set from 1979 to present (and beyond). Since global-mean stratospheric temperature is close to radiative equilibrium, our "extended" SSU data set is an important climate record for the detection and attribution of anthropogenic influence.
M. Höpfner, C. D. Boone, B. Funke, N. Glatthor, U. Grabowski, A. Günther, S. Kellmann, M. Kiefer, A. Linden, S. Lossow, H. C. Pumphrey, W. G. Read, A. Roiger, G. Stiller, H. Schlager, T. von Clarmann, and K. Wissmüller
Atmos. Chem. Phys., 15, 7017–7037, https://doi.org/10.5194/acp-15-7017-2015, https://doi.org/10.5194/acp-15-7017-2015, 2015
N. Glatthor, M. Höpfner, G. P. Stiller, T. von Clarmann, B. Funke, S. Lossow, E. Eckert, U. Grabowski, S. Kellmann, A. Linden, K. A. Walker, and A. Wiegele
Atmos. Chem. Phys., 15, 563–582, https://doi.org/10.5194/acp-15-563-2015, https://doi.org/10.5194/acp-15-563-2015, 2015
M. García-Comas, B. Funke, A. Gardini, M. López-Puertas, A. Jurado-Navarro, T. von Clarmann, G. Stiller, M. Kiefer, C. D. Boone, T. Leblanc, B. T. Marshall, M. J. Schwartz, and P. E. Sheese
Atmos. Meas. Tech., 7, 3633–3651, https://doi.org/10.5194/amt-7-3633-2014, https://doi.org/10.5194/amt-7-3633-2014, 2014
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We present the new vM21 MIPAS temperatures from 20 to 102km for all of its 2005-2012 MA, UA and NLC measurements. The main upgrades are the update of ESA L1b spectra, spectroscopic database and O and CO2 climatologies, and improvement in Tk-gradient and offset regularizations and apodization accuracy. The vM21 Tk's correct the main systematic errors of previous versions and lead to remarkable improvement in their comparisons with ACE-FTS, MLS, OSIRIS, SABER and SOFIE and the MLO and TMF lidars.
M. Sinnhuber, B. Funke, T. von Clarmann, M. Lopez-Puertas, G. P. Stiller, and A. Seppälä
Atmos. Chem. Phys., 14, 7681–7692, https://doi.org/10.5194/acp-14-7681-2014, https://doi.org/10.5194/acp-14-7681-2014, 2014
F. Friederich, M. Sinnhuber, B. Funke, T. von Clarmann, and J. Orphal
Atmos. Chem. Phys., 14, 4055–4064, https://doi.org/10.5194/acp-14-4055-2014, https://doi.org/10.5194/acp-14-4055-2014, 2014
C. H. Jackman, C. E. Randall, V. L. Harvey, S. Wang, E. L. Fleming, M. López-Puertas, B. Funke, and P. F. Bernath
Atmos. Chem. Phys., 14, 1025–1038, https://doi.org/10.5194/acp-14-1025-2014, https://doi.org/10.5194/acp-14-1025-2014, 2014
M. Höpfner, N. Glatthor, U. Grabowski, S. Kellmann, M. Kiefer, A. Linden, J. Orphal, G. Stiller, T. von Clarmann, B. Funke, and C. D. Boone
Atmos. Chem. Phys., 13, 10405–10423, https://doi.org/10.5194/acp-13-10405-2013, https://doi.org/10.5194/acp-13-10405-2013, 2013
S. Bender, M. Sinnhuber, J. P. Burrows, M. Langowski, B. Funke, and M. López-Puertas
Atmos. Meas. Tech., 6, 2521–2531, https://doi.org/10.5194/amt-6-2521-2013, https://doi.org/10.5194/amt-6-2521-2013, 2013
F. Friederich, T. von Clarmann, B. Funke, H. Nieder, J. Orphal, M. Sinnhuber, G. P. Stiller, and J. M. Wissing
Atmos. Chem. Phys., 13, 2531–2539, https://doi.org/10.5194/acp-13-2531-2013, https://doi.org/10.5194/acp-13-2531-2013, 2013
S. Kellmann, T. von Clarmann, G. P. Stiller, E. Eckert, N. Glatthor, M. Höpfner, M. Kiefer, J. Orphal, B. Funke, U. Grabowski, A. Linden, G. S. Dutton, and J. W. Elkins
Atmos. Chem. Phys., 12, 11857–11875, https://doi.org/10.5194/acp-12-11857-2012, https://doi.org/10.5194/acp-12-11857-2012, 2012
Norbert Glatthor, Gabriele P. Stiller, Thomas von Clarmann, Bernd Funke, Sylvia Kellmann, and Andrea Linden
Atmos. Chem. Phys., 25, 1175–1208, https://doi.org/10.5194/acp-25-1175-2025, https://doi.org/10.5194/acp-25-1175-2025, 2025
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We present global upper-tropospheric distributions of the pollutants HCN, CO, C2H2, C2H6, PAN, and HCOOH, observed between 2002 and 2012 by the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) on the Environmental Satellite (Envisat). By comparing the spatial distributions of their volume mixing ratios and by global correlation and regression analyses, we draw conclusions on their sources, such as biomass burning, anthropogenic sources, and biogenic release.
Maryam Ramezani Ziarani, Miriam Sinnhuber, Thomas Reddmann, Bernd Funke, Stefan Bender, and Michael Prather
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-227, https://doi.org/10.5194/gmd-2024-227, 2025
Preprint under review for GMD
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Our study aims to present a new method for incorporating top-down solar forcing into stratospheric ozone relying on linearized ozone scheme. The addition of geomagnetic forcing led to significant ozone losses in the polar upper stratosphere of both hemispheres due to the catalytic cycles involving NOy. In addition to the particle precipitation effect, accounting for solar UV variability in the ICON-ART model leads to the changes in ozone in the tropical stratosphere.
Lucien Froidevaux, Douglas E. Kinnison, Benjamin Gaubert, Michael J. Schwartz, Nathaniel J. Livesey, William G. Read, Charles G. Bardeen, Jerry R. Ziemke, and Ryan A. Fuller
Atmos. Chem. Phys., 25, 597–624, https://doi.org/10.5194/acp-25-597-2025, https://doi.org/10.5194/acp-25-597-2025, 2025
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We compare observed changes in ozone (O3) and carbon monoxide (CO) in the tropical upper troposphere (10–15 km altitude) for 2005–2020 to predictions from model simulations that track the evolution of natural and industrial emissions transported to this region. An increasing trend in measured upper-tropospheric O3 is well matched by model trends. We find that changes in modeled industrial CO surface emissions lead to better model agreement with observed slight decreases in upper-tropospheric CO.
Weiyu Zhang, Kwinten Van Weverberg, Cyril J. Morcrette, Wuhu Feng, Kalli Furtado, Paul R. Field, Chih-Chieh Chen, Andrew Gettelman, Piers M. Forster, Daniel R. Marsh, and Alexandru Rap
Atmos. Chem. Phys., 25, 473–489, https://doi.org/10.5194/acp-25-473-2025, https://doi.org/10.5194/acp-25-473-2025, 2025
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Contrail cirrus is the largest, but also most uncertain, contribution of aviation to global warming. We evaluate, for the first time, the impact of the host climate model on contrail cirrus properties. Substantial differences exist between contrail cirrus formation, persistence, and radiative effects in the host climate models. Reliable contrail cirrus simulations require advanced representation of cloud optical properties and microphysics, which should be better constrained by observations.
Simone Tilmes, Ewa M. Bednarz, Andrin Jörimann, Daniele Visioni, Douglas E. Kinnison, Gabriel Chiodo, and David Plummer
EGUsphere, https://doi.org/10.5194/egusphere-2024-3586, https://doi.org/10.5194/egusphere-2024-3586, 2024
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This paper describes the details of a new multi-model intercomparison experiment to assess the effects of Stratospheric Aerosol Injections on stratospheric chemistry and dynamics and, therefore, ozone. In this experiment, all models will use the same prescribed stratospheric aerosol distribution and fixed sea-surface temperatures and sea ice. We discuss the advantages and differences of this more constrained experiment compared to previous more interactive model experiments.
Jianfei Wu, Wuhu Feng, Xianghui Xue, Daniel Robert Marsh, and John Maurice Campbell Plane
Atmos. Chem. Phys., 24, 12133–12141, https://doi.org/10.5194/acp-24-12133-2024, https://doi.org/10.5194/acp-24-12133-2024, 2024
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Metal layers occur in the mesosphere and lower thermosphere region 80–120 km from the ablation of cosmic dust. Nonmigrating diurnal tides are persistent global oscillations. We investigate nonmigrating diurnal tidal variations in metal layers using satellite observations and global climate model simulations; these have not been studied previously due to the limitations of measurements. The nonmigrating diurnal tides in temperature are strongly linked to the corresponding change in metal layers.
Theodore K. Koenig, François Hendrick, Douglas Kinnison, Christopher F. Lee, Michel Van Roozendael, and Rainer Volkamer
Atmos. Meas. Tech., 17, 5911–5934, https://doi.org/10.5194/amt-17-5911-2024, https://doi.org/10.5194/amt-17-5911-2024, 2024
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Atmospheric bromine destroys ozone, impacts oxidation capacity, and oxidizes mercury into its toxic form. We constrain bromine by remote sensing of BrO from a mountaintop. Previous measurements retrieved two to three pieces of information vertically; we apply new methods to get five and a half vertically and two more in time. We compare with aircraft measurements to validate the methods and look at variations in BrO over the Pacific.
Kane Stone, Susan Solomon, Pengfei Yu, Daniel M. Murphy, Douglas Kinnison, and Jian Guan
EGUsphere, https://doi.org/10.5194/egusphere-2024-2948, https://doi.org/10.5194/egusphere-2024-2948, 2024
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The Australian 2019/2020 wildfires injected a substantial amount of smoke into the upper atmosphere, causing unusual chemical reactions that altered the chemical makeup of the upper atmosphere. This led to ozone depletion in the Southern hemisphere midlatitudes which likely didn't fully recover until 2 years after the initial event due to the persistent chemical effects of the smoke.
Connor J. Clayton, Daniel R. Marsh, Steven T. Turnock, Ailish M. Graham, Kirsty J. Pringle, Carly L. Reddington, Rajesh Kumar, and James B. McQuaid
Atmos. Chem. Phys., 24, 10717–10740, https://doi.org/10.5194/acp-24-10717-2024, https://doi.org/10.5194/acp-24-10717-2024, 2024
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We demonstrate that strong climate mitigation could improve air quality in Europe; however, less ambitious mitigation does not result in these co-benefits. We use a high-resolution atmospheric chemistry model. This allows us to demonstrate how this varies across European countries and analyse the underlying chemistry. This may help policy-facing researchers understand which sectors and regions need to be prioritised to achieve strong air quality co-benefits of climate mitigation.
Florian Voet, Felix Plöger, Johannes Laube, Peter Preusse, Paul Konopka, Jens-Uwe Grooß, Jörn Ungermann, Björn-Martin Sinnhuber, Michael Hoepfner, Bernd Funke, Gerald Wetzel, Sören Johansson, Gabriele Stiller, Eric Ray, and Michaela Imelda Hegglin
EGUsphere, https://doi.org/10.5194/egusphere-2024-2624, https://doi.org/10.5194/egusphere-2024-2624, 2024
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This study refines estimates of the stratospheric “age of air,” a measure of how long air circulates in the stratosphere. By analyzing correlations between trace gases measurable by satellites, the research introduces a method that reduces uncertainties and detects small-scale atmospheric features. This improved understanding of stratospheric circulation is crucial for better climate models and predictions, enhancing our ability to assess the impacts of climate change on the atmosphere.
Miriam Sinnhuber, Christina Arras, Stefan Bender, Bernd Funke, Hanli Liu, Daniel R. Marsh, Thomas Reddmann, Eugene Rozanov, Timofei Sukhodolov, Monika E. Szelag, and Jan Maik Wissing
EGUsphere, https://doi.org/10.5194/egusphere-2024-2256, https://doi.org/10.5194/egusphere-2024-2256, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Formation of nitric oxide NO in the upper atmosphere varies with solar activity. Observations show that it starts a chain of processes in the entire atmosphere affecting the ozone layer and climate system. This is often underestimated in models. We compare five models which show large differences in simulated NO. Analysis of results point out problems related to the oxygen balance, and to the impact of atmospheric waves on dynamics. Both must be modeled well to reproduce the downward coupling.
Manuel López-Puertas, Federico Fabiano, Victor Fomichev, Bernd Funke, and Daniel R. Marsh
Geosci. Model Dev., 17, 4401–4432, https://doi.org/10.5194/gmd-17-4401-2024, https://doi.org/10.5194/gmd-17-4401-2024, 2024
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The radiative infrared cooling of CO2 in the middle atmosphere is crucial for computing its thermal structure. It requires one however to include non-local thermodynamic equilibrium processes which are computationally very expensive, which cannot be afforded by climate models. In this work, we present an updated, efficient, accurate and very fast (~50 µs) parameterization of that cooling able to cope with CO2 abundances from half the pre-industrial values to 10 times the current abundance.
Norbert Glatthor, Thomas von Clarmann, Bernd Funke, Maya García-Comas, Udo Grabowski, Michael Höpfner, Sylvia Kellmann, Michael Kiefer, Alexandra Laeng, Andrea Linden, Manuel López-Puertas, and Gabriele P. Stiller
Atmos. Meas. Tech., 17, 2849–2871, https://doi.org/10.5194/amt-17-2849-2024, https://doi.org/10.5194/amt-17-2849-2024, 2024
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We present global atmospheric methane (CH4) and nitrous oxide (N2O) distributions retrieved from measurements of the MIPAS instrument on board the Environmental Satellite (Envisat) during 2002 to 2012. Monitoring of these gases is of scientific interest because both of them are strong greenhouse gases. We analyze the latest, improved version of calibrated MIPAS measurements. Further, we apply a new retrieval scheme leading to an improved CH4 and N2O data product .
Gabriele P. Stiller, Thomas von Clarmann, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Michael Kiefer, Alexandra Laeng, Andrea Linden, Bernd Funke, Maya García-Comas, and Manuel López-Puertas
Atmos. Meas. Tech., 17, 1759–1789, https://doi.org/10.5194/amt-17-1759-2024, https://doi.org/10.5194/amt-17-1759-2024, 2024
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CFC-11, CFC-12, and HCFC-22 contribute to the depletion of ozone and are potent greenhouse gases. They have been banned by the Montreal protocol. With MIPAS on Envisat the atmospheric composition could be observed between 2002 and 2012. We present here the retrieval of their atmospheric distributions for the final data version 8. We characterise the derived data by their error budget and their spatial resolution. An additional representation for direct comparison to models is also provided.
Manuel López-Puertas, Maya García-Comas, Bernd Funke, Thomas von Clarmann, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Michael Kiefer, Alexandra Laeng, Andrea Linden, and Gabriele P. Stiller
Atmos. Meas. Tech., 16, 5609–5645, https://doi.org/10.5194/amt-16-5609-2023, https://doi.org/10.5194/amt-16-5609-2023, 2023
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This paper describes a new version (V8) of ozone data from MIPAS middle-atmosphere spectra. The dataset comprises high-quality ozone profiles from 20 to 100 km, with pole-to-pole latitude coverage for the day- and nighttime, spanning 2005 until 2012. An exhaustive treatment of errors has been performed. Compared to other satellite instruments, MIPAS ozone shows a positive bias of 5 %–8 % below 70 km. In the upper mesosphere, this new version agrees much better than previous ones (within 10 %).
Maya García-Comas, Bernd Funke, Manuel López-Puertas, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Michael Kiefer, Andrea Linden, Belén Martínez-Mondéjar, Gabriele P. Stiller, and Thomas von Clarmann
Atmos. Meas. Tech., 16, 5357–5386, https://doi.org/10.5194/amt-16-5357-2023, https://doi.org/10.5194/amt-16-5357-2023, 2023
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We have released version 8 of MIPAS IMK–IAA temperatures and pointing information retrieved from MIPAS Middle and Upper Atmosphere mode version 8.03 calibrated spectra, covering 20–115 km altitude. We considered non-local thermodynamic equilibrium emission explicitly for each limb scan, essential to retrieve accurate temperatures above the mid-mesosphere. Comparisons of this temperature dataset with SABER measurements show excellent agreement, improving those of previous MIPAS versions.
Yunqian Zhu, Robert W. Portmann, Douglas Kinnison, Owen Brian Toon, Luis Millán, Jun Zhang, Holger Vömel, Simone Tilmes, Charles G. Bardeen, Xinyue Wang, Stephanie Evan, William J. Randel, and Karen H. Rosenlof
Atmos. Chem. Phys., 23, 13355–13367, https://doi.org/10.5194/acp-23-13355-2023, https://doi.org/10.5194/acp-23-13355-2023, 2023
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The 2022 Hunga Tonga eruption injected a large amount of water into the stratosphere. Ozone depletion was observed inside the volcanic plume. Chlorine and water vapor injected by this eruption exceeded the normal range, which made the ozone chemistry during this event occur at a higher temperature than polar ozone depletion. Unlike polar ozone chemistry where chlorine nitrate is more important, hypochlorous acid plays a large role in the in-plume chlorine balance and heterogeneous processes.
John M. C. Plane, Jörg Gumbel, Konstantinos S. Kalogerakis, Daniel R. Marsh, and Christian von Savigny
Atmos. Chem. Phys., 23, 13255–13282, https://doi.org/10.5194/acp-23-13255-2023, https://doi.org/10.5194/acp-23-13255-2023, 2023
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The mesosphere or lower thermosphere region of the atmosphere borders the edge of space. It is subject to extreme ultraviolet photons and charged particles from the Sun and atmospheric gravity waves from below, which tend to break in this region. The pressure is very low, which facilitates chemistry involving species in excited states, and this is also the region where cosmic dust ablates and injects various metals. The result is a unique and exotic chemistry.
Monali Borthakur, Miriam Sinnhuber, Alexandra Laeng, Thomas Reddmann, Peter Braesicke, Gabriele Stiller, Thomas von Clarmann, Bernd Funke, Ilya Usoskin, Jan Maik Wissing, and Olesya Yakovchuk
Atmos. Chem. Phys., 23, 12985–13013, https://doi.org/10.5194/acp-23-12985-2023, https://doi.org/10.5194/acp-23-12985-2023, 2023
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Reduced ozone levels resulting from ozone depletion mean more exposure to UV radiation, which has various effects on human health. We analysed solar events to see what influence it has on the chemistry of Earth's atmosphere and how this atmospheric chemistry change can affect the ozone. To do this, we used an atmospheric model considering only chemistry and compared it with satellite data. The focus was mainly on the contribution of chlorine, and we found about 10 %–20 % ozone loss due to that.
Jian Guan, Susan Solomon, Sasha Madronich, and Douglas Kinnison
Atmos. Chem. Phys., 23, 10413–10422, https://doi.org/10.5194/acp-23-10413-2023, https://doi.org/10.5194/acp-23-10413-2023, 2023
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This paper provides a novel method to obtain a global and accurate photodissociation coefficient for NO2 (J(NO2)) based on satellite data, and the results are shown to be consistent with model results. The J(NO2) value decreases as the solar zenith angle increases and has a weak altitude dependence. A key finding is that the satellite-derived J(NO2) increases in the polar regions, in good agreement with model predictions, due to the effects of ice and snow on surface albedo.
Thomas Reddmann, Miriam Sinnhuber, Jan Maik Wissing, Olesya Yakovchuk, and Ilya Usoskin
Atmos. Chem. Phys., 23, 6989–7000, https://doi.org/10.5194/acp-23-6989-2023, https://doi.org/10.5194/acp-23-6989-2023, 2023
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Recent analyses of isotopic records of ice cores and sediments have shown that very strong explosions may occur on the Sun, perhaps about one such explosion every 1000 years. Such explosions pose a real threat to humankind. It is therefore of great interest to study the impact of such explosions on Earth. We analyzed how the explosions would affect the chemistry of the middle atmosphere and show that the related ozone loss is not dramatic and that the atmosphere will recover within 1 year.
Michael Weimer, Douglas E. Kinnison, Catherine Wilka, and Susan Solomon
Atmos. Chem. Phys., 23, 6849–6861, https://doi.org/10.5194/acp-23-6849-2023, https://doi.org/10.5194/acp-23-6849-2023, 2023
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We investigate the influence of the number density of nitric acid trihydrate (NAT) particles on associated trace gases in the lower stratosphere using data from a satellite, ozonesondes and simulations by a community chemistry climate model. By comparing probability density functions between observations and the model, we find that the standard NAT number density should be reduced for future simulations with the model.
Bernd Funke, Maya García-Comas, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Michael Kiefer, Andrea Linden, Manuel López-Puertas, Gabriele P. Stiller, and Thomas von Clarmann
Atmos. Meas. Tech., 16, 2167–2196, https://doi.org/10.5194/amt-16-2167-2023, https://doi.org/10.5194/amt-16-2167-2023, 2023
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New global nitric oxide (NO) volume-mixing-ratio and lower-thermospheric temperature data products, retrieved from Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) spectra with the IMK-IAA MIPAS data processor, have been released. The dataset covers the entire Envisat mission lifetime and includes retrieval results from all MIPAS observation modes. The data are based on ESA version 8 calibration and were processed using an improved retrieval approach.
Michael Kiefer, Thomas von Clarmann, Bernd Funke, Maya García-Comas, Norbert Glatthor, Udo Grabowski, Michael Höpfner, Sylvia Kellmann, Alexandra Laeng, Andrea Linden, Manuel López-Puertas, and Gabriele P. Stiller
Atmos. Meas. Tech., 16, 1443–1460, https://doi.org/10.5194/amt-16-1443-2023, https://doi.org/10.5194/amt-16-1443-2023, 2023
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A new ozone data set, derived from radiation measurements of the space-borne instrument MIPAS, is presented. It consists of more than 2 million single ozone profiles from 2002–2012, covering virtually all latitudes and altitudes between 5 and 70 km. Progress in data calibration and processing methods allowed for significant improvement of the data quality, compared to previous data versions. Hence, the data set will help to better understand e.g. the time evolution of ozone in the stratosphere.
Thomas von Clarmann, Norbert Glatthor, Udo Grabowski, Bernd Funke, Michael Kiefer, Anne Kleinert, Gabriele P. Stiller, Andrea Linden, and Sylvia Kellmann
Atmos. Meas. Tech., 15, 6991–7018, https://doi.org/10.5194/amt-15-6991-2022, https://doi.org/10.5194/amt-15-6991-2022, 2022
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Errors of profiles of temperature and mixing ratios retrieved from spectra recorded with the Michelson Interferometer for Passive Atmospheric Sounding are estimated. All known and quantified sources of uncertainty are considered. Some ongoing uncertaities contribute to both the random and to the systematic errors. In some cases, one source of uncertainty propagates onto the error budget via multiple pathways. Problems arise when the correlations of errors to be propagated are unknown.
Gerald Wetzel, Michael Höpfner, Hermann Oelhaf, Felix Friedl-Vallon, Anne Kleinert, Guido Maucher, Miriam Sinnhuber, Janna Abalichin, Angelika Dehn, and Piera Raspollini
Atmos. Meas. Tech., 15, 6669–6704, https://doi.org/10.5194/amt-15-6669-2022, https://doi.org/10.5194/amt-15-6669-2022, 2022
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Satellite measurements of stratospheric trace gases are essential for monitoring distributions and trends of these species on a global scale. Here, we compare the final MIPAS ESA Level 2 version 8 data (temperature and trace gases) with measurements obtained with the balloon version of MIPAS in terms of data agreement of both sensors, including combined errors. For most gases, we find a 5 % to 20 % agreement of the retrieved vertical profiles of both MIPAS instruments in the lower stratosphere.
Bingkun Yu, Xianghui Xue, Christopher J. Scott, Mingjiao Jia, Wuhu Feng, John M. C. Plane, Daniel R. Marsh, Jonas Hedin, Jörg Gumbel, and Xiankang Dou
Atmos. Chem. Phys., 22, 11485–11504, https://doi.org/10.5194/acp-22-11485-2022, https://doi.org/10.5194/acp-22-11485-2022, 2022
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We present a study on the climatology of the metal sodium layer in the upper atmosphere from the ground-based measurements obtained from a lidar network, the Odin satellite measurements, and a global model of meteoric sodium in the atmosphere. Comprehensively, comparisons show good agreement and some discrepancies between ground-based observations, satellite measurements, and global model simulations.
Ville Maliniemi, Pavle Arsenovic, Annika Seppälä, and Hilde Nesse Tyssøy
Atmos. Chem. Phys., 22, 8137–8149, https://doi.org/10.5194/acp-22-8137-2022, https://doi.org/10.5194/acp-22-8137-2022, 2022
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We simulate the effect of energetic particle precipitation (EPP) on Antarctic stratospheric ozone chemistry over the whole 20th century. We find a significant increase of reactive nitrogen due to EP, which can deplete ozone via a catalytic reaction. Furthermore, significant modulation of active chlorine is obtained related to EPP, which impacts ozone depletion by both active chlorine and EPP. Our results show that EPP has been a significant modulator of ozone chemistry during the CFC era.
Irina Mironova, Miriam Sinnhuber, Galina Bazilevskaya, Mark Clilverd, Bernd Funke, Vladimir Makhmutov, Eugene Rozanov, Michelle L. Santee, Timofei Sukhodolov, and Thomas Ulich
Atmos. Chem. Phys., 22, 6703–6716, https://doi.org/10.5194/acp-22-6703-2022, https://doi.org/10.5194/acp-22-6703-2022, 2022
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From balloon measurements, we detected unprecedented, extremely powerful, electron precipitation over the middle latitudes. The robustness of this event is confirmed by satellite observations of electron fluxes and chemical composition, as well as by ground-based observations of the radio signal propagation. The applied chemistry–climate model shows the almost complete destruction of ozone in the mesosphere over the region where high-energy electrons were observed.
Lucien Froidevaux, Douglas E. Kinnison, Michelle L. Santee, Luis F. Millán, Nathaniel J. Livesey, William G. Read, Charles G. Bardeen, John J. Orlando, and Ryan A. Fuller
Atmos. Chem. Phys., 22, 4779–4799, https://doi.org/10.5194/acp-22-4779-2022, https://doi.org/10.5194/acp-22-4779-2022, 2022
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We analyze satellite-derived distributions of chlorine monoxide (ClO) and hypochlorous acid (HOCl) in the upper atmosphere. For 2005–2020, from 50°S to 50°N and over ~30 to 45 km, ClO and HOCl decreased by −0.7 % and −0.4 % per year, respectively. A detailed model of chemistry and dynamics agrees with the results. These decreases confirm the effectiveness of the 1987 Montreal Protocol, which limited emissions of chlorine- and bromine-containing source gases, in order to protect the ozone layer.
Matthias Schneider, Benjamin Ertl, Christopher J. Diekmann, Farahnaz Khosrawi, Andreas Weber, Frank Hase, Michael Höpfner, Omaira E. García, Eliezer Sepúlveda, and Douglas Kinnison
Earth Syst. Sci. Data, 14, 709–742, https://doi.org/10.5194/essd-14-709-2022, https://doi.org/10.5194/essd-14-709-2022, 2022
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We present atmospheric H2O, HDO / H2O ratio, N2O, CH4, and HNO3 data generated by the MUSICA IASI processor using thermal nadir spectra measured by the IASI satellite instrument. The data have global daily coverage and are available for the period between October 2014 and June 2021. Multiple possibilities of data reuse are offered by providing each individual data product together with information about retrieval settings and the products' uncertainty and vertical representativeness.
Kseniia Golubenko, Eugene Rozanov, Gennady Kovaltsov, Ari-Pekka Leppänen, Timofei Sukhodolov, and Ilya Usoskin
Geosci. Model Dev., 14, 7605–7620, https://doi.org/10.5194/gmd-14-7605-2021, https://doi.org/10.5194/gmd-14-7605-2021, 2021
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A new full 3-D time-dependent model, based on SOCOL-AERv2, of beryllium atmospheric production, transport, and deposition has been developed and validated using directly measured data. The model is recommended to be used in studies related to, e.g., atmospheric dynamical patterns, extreme solar particle storms, long-term solar activity reconstruction from cosmogenic proxy data, and solar–terrestrial relations.
Ioannis A. Daglis, Loren C. Chang, Sergio Dasso, Nat Gopalswamy, Olga V. Khabarova, Emilia Kilpua, Ramon Lopez, Daniel Marsh, Katja Matthes, Dibyendu Nandy, Annika Seppälä, Kazuo Shiokawa, Rémi Thiéblemont, and Qiugang Zong
Ann. Geophys., 39, 1013–1035, https://doi.org/10.5194/angeo-39-1013-2021, https://doi.org/10.5194/angeo-39-1013-2021, 2021
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We present a detailed account of the science programme PRESTO (PREdictability of the variable Solar–Terrestrial cOupling), covering the period 2020 to 2024. PRESTO was defined by a dedicated committee established by SCOSTEP (Scientific Committee on Solar-Terrestrial Physics). We review the current state of the art and discuss future studies required for the most effective development of solar–terrestrial physics.
Catherine Wilka, Susan Solomon, Doug Kinnison, and David Tarasick
Atmos. Chem. Phys., 21, 15771–15781, https://doi.org/10.5194/acp-21-15771-2021, https://doi.org/10.5194/acp-21-15771-2021, 2021
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We use satellite and balloon measurements to evaluate modeled ozone loss seen in the unusually cold Arctic of 2020 in the real world and compare it to simulations of a world avoided. We show that extensive denitrification in 2020 provides an important test case for stratospheric model process representations. If the Montreal Protocol had not banned ozone-depleting substances, an Arctic ozone hole would have emerged for the first time in spring 2020 that is comparable to those in the Antarctic.
Jianfei Wu, Wuhu Feng, Han-Li Liu, Xianghui Xue, Daniel Robert Marsh, and John Maurice Campbell Plane
Atmos. Chem. Phys., 21, 15619–15630, https://doi.org/10.5194/acp-21-15619-2021, https://doi.org/10.5194/acp-21-15619-2021, 2021
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Metal layers occur in the MLT region (80–120 km) from the ablation of cosmic dust. The latest lidar observations show these metals can reach a height approaching 200 km, which is challenging to explain. We have developed the first global simulation incorporating the full life cycle of metal atoms and ions. The model results compare well with lidar and satellite observations of the seasonal and diurnal variation of the metals and demonstrate the importance of ion mass and ion-neutral coupling.
Viktoria J. Nordström and Annika Seppälä
Atmos. Chem. Phys., 21, 12835–12853, https://doi.org/10.5194/acp-21-12835-2021, https://doi.org/10.5194/acp-21-12835-2021, 2021
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The winter winds over Antarctica form a stable vortex. However, in 2019 the vortex was disrupted and the temperature in the polar stratosphere rose by 50°C. This event, called a sudden stratospheric warming, is a rare event in the Southern Hemisphere, with the only known major event having taken place in 2002. The 2019 event helps us unravel its causes, which are largely unknown. We have discovered a unique behaviour of the equatorial winds in 2002 and 2019 that may signal an impending SH SSW.
Ville Maliniemi, Hilde Nesse Tyssøy, Christine Smith-Johnsen, Pavle Arsenovic, and Daniel R. Marsh
Atmos. Chem. Phys., 21, 11041–11052, https://doi.org/10.5194/acp-21-11041-2021, https://doi.org/10.5194/acp-21-11041-2021, 2021
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We simulate ozone variability over the 21st century with different greenhouse gas scenarios. Our results highlight a novel mechanism of additional reactive nitrogen species descending to the Antarctic stratosphere from the thermosphere/upper mesosphere due to the accelerated residual circulation under climate change. This excess descending NOx can potentially prevent a super recovery of ozone in the Antarctic upper stratosphere.
Michael Kiefer, Thomas von Clarmann, Bernd Funke, Maya García-Comas, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Anne Kleinert, Alexandra Laeng, Andrea Linden, Manuel López-Puertas, Daniel R. Marsh, and Gabriele P. Stiller
Atmos. Meas. Tech., 14, 4111–4138, https://doi.org/10.5194/amt-14-4111-2021, https://doi.org/10.5194/amt-14-4111-2021, 2021
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An improved dataset of vertical temperature profiles of the Earth's atmosphere in the altitude range 5–70 km is presented. These profiles are derived from measurements of the MIPAS instrument onboard ESA's Envisat satellite. The overall improvements are based on upgrades in the input data and several improvements in the data processing approach. Both of these are discussed, and an extensive error discussion is included. Enhancements of the new dataset are demonstrated by means of examples.
Michaela I. Hegglin, Susann Tegtmeier, John Anderson, Adam E. Bourassa, Samuel Brohede, Doug Degenstein, Lucien Froidevaux, Bernd Funke, John Gille, Yasuko Kasai, Erkki T. Kyrölä, Jerry Lumpe, Donal Murtagh, Jessica L. Neu, Kristell Pérot, Ellis E. Remsberg, Alexei Rozanov, Matthew Toohey, Joachim Urban, Thomas von Clarmann, Kaley A. Walker, Hsiang-Jui Wang, Carlo Arosio, Robert Damadeo, Ryan A. Fuller, Gretchen Lingenfelser, Christopher McLinden, Diane Pendlebury, Chris Roth, Niall J. Ryan, Christopher Sioris, Lesley Smith, and Katja Weigel
Earth Syst. Sci. Data, 13, 1855–1903, https://doi.org/10.5194/essd-13-1855-2021, https://doi.org/10.5194/essd-13-1855-2021, 2021
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An overview of the SPARC Data Initiative is presented, to date the most comprehensive assessment of stratospheric composition measurements spanning 1979–2018. Measurements of 26 chemical constituents obtained from an international suite of space-based limb sounders were compiled into vertically resolved, zonal monthly mean time series. The quality and consistency of these gridded datasets are then evaluated using a climatological validation approach and a range of diagnostics.
Bingkun Yu, Xianghui Xue, Christopher J. Scott, Jianfei Wu, Xinan Yue, Wuhu Feng, Yutian Chi, Daniel R. Marsh, Hanli Liu, Xiankang Dou, and John M. C. Plane
Atmos. Chem. Phys., 21, 4219–4230, https://doi.org/10.5194/acp-21-4219-2021, https://doi.org/10.5194/acp-21-4219-2021, 2021
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A long-standing mystery of metal ions within Es layers in the Earth's upper atmosphere is the marked seasonal dependence, with a summer maximum and a winter minimum. We report a large-scale winter-to-summer transport of metal ions from 6-year multi-satellite observations and worldwide ground-based stations. A global atmospheric circulation is responsible for the phenomenon. Our results emphasise the effect of this atmospheric circulation on the transport of composition in the upper atmosphere.
Chaim I. Garfinkel, Ohad Harari, Shlomi Ziskin Ziv, Jian Rao, Olaf Morgenstern, Guang Zeng, Simone Tilmes, Douglas Kinnison, Fiona M. O'Connor, Neal Butchart, Makoto Deushi, Patrick Jöckel, Andrea Pozzer, and Sean Davis
Atmos. Chem. Phys., 21, 3725–3740, https://doi.org/10.5194/acp-21-3725-2021, https://doi.org/10.5194/acp-21-3725-2021, 2021
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Water vapor is the dominant greenhouse gas in the atmosphere, and El Niño is the dominant mode of variability in the ocean–atmosphere system. The connection between El Niño and water vapor above ~ 17 km is unclear, with single-model studies reaching a range of conclusions. This study examines this connection in 12 different models. While there are substantial differences among the models, all models appear to capture the fundamental physical processes correctly.
Patrick E. Sheese, Kaley A. Walker, Chris D. Boone, Doug A. Degenstein, Felicia Kolonjari, David Plummer, Douglas E. Kinnison, Patrick Jöckel, and Thomas von Clarmann
Atmos. Meas. Tech., 14, 1425–1438, https://doi.org/10.5194/amt-14-1425-2021, https://doi.org/10.5194/amt-14-1425-2021, 2021
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Output from climate chemistry models (CMAM, EMAC, and WACCM) is used to estimate the expected geophysical variability of ozone concentrations between coincident satellite instrument measurement times and geolocations. We use the Canadian ACE-FTS and OSIRIS instruments as a case study. Ensemble mean estimates are used to optimize coincidence criteria between the two instruments, allowing for the use of more coincident profiles while providing an estimate of the geophysical variation.
Emily M. Gordon, Annika Seppälä, Bernd Funke, Johanna Tamminen, and Kaley A. Walker
Atmos. Chem. Phys., 21, 2819–2836, https://doi.org/10.5194/acp-21-2819-2021, https://doi.org/10.5194/acp-21-2819-2021, 2021
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Energetic particle precipitation (EPP) is the rain of solar energetic particles into the Earth's atmosphere. EPP is known to deplete O3 in the polar mesosphere–upper stratosphere via the formation of NOx. NOx also causes chlorine deactivation in the lower stratosphere and has, thus, been proposed to potentially result in reduced ozone depletion in the spring. We provide the first evidence to show that NOx formed by EPP is able to remove active chlorine, resulting in enhanced total ozone column.
Marc von Hobe, Felix Ploeger, Paul Konopka, Corinna Kloss, Alexey Ulanowski, Vladimir Yushkov, Fabrizio Ravegnani, C. Michael Volk, Laura L. Pan, Shawn B. Honomichl, Simone Tilmes, Douglas E. Kinnison, Rolando R. Garcia, and Jonathon S. Wright
Atmos. Chem. Phys., 21, 1267–1285, https://doi.org/10.5194/acp-21-1267-2021, https://doi.org/10.5194/acp-21-1267-2021, 2021
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The Asian summer monsoon (ASM) is known to foster transport of polluted tropospheric air into the stratosphere. To test and amend our picture of ASM vertical transport, we analyse distributions of airborne trace gas observations up to 20 km altitude near the main ASM vertical conduit south of the Himalayas. We also show that a new high-resolution version of the global chemistry climate model WACCM is able to reproduce the observations well.
Noora Partamies, Fasil Tesema, Emma Bland, Erkka Heino, Hilde Nesse Tyssøy, and Erlend Kallelid
Ann. Geophys., 39, 69–83, https://doi.org/10.5194/angeo-39-69-2021, https://doi.org/10.5194/angeo-39-69-2021, 2021
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About 200 nights of substorm activity have been analysed for their magnetic disturbance magnitude and the level of cosmic radio noise absorption. We show that substorms with a single expansion phase have limited lifetimes and spatial extents. Starting from magnetically quiet conditions, the strongest absorption occurs after 1 to 2 nights of substorm activity. This prolonged activity is thus required to accelerate particles to energies, which may affect the atmospheric chemistry.
Arseniy Karagodin-Doyennel, Eugene Rozanov, Ales Kuchar, William Ball, Pavle Arsenovic, Ellis Remsberg, Patrick Jöckel, Markus Kunze, David A. Plummer, Andrea Stenke, Daniel Marsh, Doug Kinnison, and Thomas Peter
Atmos. Chem. Phys., 21, 201–216, https://doi.org/10.5194/acp-21-201-2021, https://doi.org/10.5194/acp-21-201-2021, 2021
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The solar signal in the mesospheric H2O and CO was extracted from the CCMI-1 model simulations and satellite observations using multiple linear regression (MLR) analysis. MLR analysis shows a pronounced and statistically robust solar signal in both H2O and CO. The model results show a general agreement with observations reproducing a negative/positive solar signal in H2O/CO. The pattern of the solar signal varies among the considered models, reflecting some differences in the model setup.
Fasil Tesema, Noora Partamies, Hilde Nesse Tyssøy, and Derek McKay
Ann. Geophys., 38, 1191–1202, https://doi.org/10.5194/angeo-38-1191-2020, https://doi.org/10.5194/angeo-38-1191-2020, 2020
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In this study, we present the ionization level from EISCAT radar experiments and cosmic noise absorption level
from KAIRA riometer observations during pulsating auroras. We found thick layers of ionization that reach down
to 70 km (harder precipitation) and higher cosmic noise absorption during patchy pulsating aurora than
during amorphous pulsating and patchy auroras.
Yuanhong Zhao, Marielle Saunois, Philippe Bousquet, Xin Lin, Antoine Berchet, Michaela I. Hegglin, Josep G. Canadell, Robert B. Jackson, Makoto Deushi, Patrick Jöckel, Douglas Kinnison, Ole Kirner, Sarah Strode, Simone Tilmes, Edward J. Dlugokencky, and Bo Zheng
Atmos. Chem. Phys., 20, 13011–13022, https://doi.org/10.5194/acp-20-13011-2020, https://doi.org/10.5194/acp-20-13011-2020, 2020
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Decadal trends and variations in OH are critical for understanding atmospheric CH4 evolution. We quantify the impacts of OH trends and variations on the CH4 budget by conducting CH4 inversions on a decadal scale with an ensemble of OH fields. We find the negative OH anomalies due to enhanced fires can reduce the optimized CH4 emissions by up to 10 Tg yr−1 during El Niño years and the positive OH trend from 1986 to 2010 results in a ∼ 23 Tg yr−1 additional increase in optimized CH4 emissions.
Daniele Minganti, Simon Chabrillat, Yves Christophe, Quentin Errera, Marta Abalos, Maxime Prignon, Douglas E. Kinnison, and Emmanuel Mahieu
Atmos. Chem. Phys., 20, 12609–12631, https://doi.org/10.5194/acp-20-12609-2020, https://doi.org/10.5194/acp-20-12609-2020, 2020
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The climatology of the N2O transport budget in the stratosphere is studied in the transformed Eulerian mean framework across a variety of datasets: a chemistry climate model, a chemistry transport model driven by four reanalyses and a chemical reanalysis. The impact of vertical advection on N2O agrees well in the datasets, but horizontal mixing presents large differences above the Antarctic and in the whole Northern Hemisphere.
Francesco Grieco, Kristell Pérot, Donal Murtagh, Patrick Eriksson, Peter Forkman, Bengt Rydberg, Bernd Funke, Kaley A. Walker, and Hugh C. Pumphrey
Atmos. Meas. Tech., 13, 5013–5031, https://doi.org/10.5194/amt-13-5013-2020, https://doi.org/10.5194/amt-13-5013-2020, 2020
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We present a unique – by time extension and geographical coverage – dataset of satellite observations of carbon monoxide (CO) in the mesosphere which will allow us to study dynamical processes, since CO is a very good tracer of circulation in the mesosphere. Previously, the dataset was unusable due to instrumental artefacts that affected the measurements. We identify the cause of the artefacts, eliminate them and prove the quality of the results by comparing with other instrument measurements.
Matt Amos, Paul J. Young, J. Scott Hosking, Jean-François Lamarque, N. Luke Abraham, Hideharu Akiyoshi, Alexander T. Archibald, Slimane Bekki, Makoto Deushi, Patrick Jöckel, Douglas Kinnison, Ole Kirner, Markus Kunze, Marion Marchand, David A. Plummer, David Saint-Martin, Kengo Sudo, Simone Tilmes, and Yousuke Yamashita
Atmos. Chem. Phys., 20, 9961–9977, https://doi.org/10.5194/acp-20-9961-2020, https://doi.org/10.5194/acp-20-9961-2020, 2020
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We present an updated projection of Antarctic ozone hole recovery using an ensemble of chemistry–climate models. To do so, we employ a method, more advanced and skilful than the current multi-model mean standard, which is applicable to other ensemble analyses. It calculates the performance and similarity of the models, which we then use to weight the model. Calculating model similarity allows us to account for models which are constructed from similar components.
Thomas von Clarmann, Douglas A. Degenstein, Nathaniel J. Livesey, Stefan Bender, Amy Braverman, André Butz, Steven Compernolle, Robert Damadeo, Seth Dueck, Patrick Eriksson, Bernd Funke, Margaret C. Johnson, Yasuko Kasai, Arno Keppens, Anne Kleinert, Natalya A. Kramarova, Alexandra Laeng, Bavo Langerock, Vivienne H. Payne, Alexei Rozanov, Tomohiro O. Sato, Matthias Schneider, Patrick Sheese, Viktoria Sofieva, Gabriele P. Stiller, Christian von Savigny, and Daniel Zawada
Atmos. Meas. Tech., 13, 4393–4436, https://doi.org/10.5194/amt-13-4393-2020, https://doi.org/10.5194/amt-13-4393-2020, 2020
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Remote sensing of atmospheric state variables typically relies on the inverse solution of the radiative transfer equation. An adequately characterized retrieval provides information on the uncertainties of the estimated state variables as well as on how any constraint or a priori assumption affects the estimate. This paper summarizes related techniques and provides recommendations for unified error reporting.
Niilo Kalakoski, Pekka T. Verronen, Annika Seppälä, Monika E. Szeląg, Antti Kero, and Daniel R. Marsh
Atmos. Chem. Phys., 20, 8923–8938, https://doi.org/10.5194/acp-20-8923-2020, https://doi.org/10.5194/acp-20-8923-2020, 2020
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Effects of solar proton events (SPEs) on middle atmosphere chemistry were studied using the WACCM-D chemistry–climate model, including an improved representation of lower ionosphere ion chemistry. This study includes 66 events in the years 1989–2012 and uses a statistical approach to determine the impact of the improved chemistry scheme. The differences shown highlight the importance of ion chemistry in models used to study energetic particle precipitation.
Pekka T. Verronen, Daniel R. Marsh, Monika E. Szeląg, and Niilo Kalakoski
Ann. Geophys., 38, 833–844, https://doi.org/10.5194/angeo-38-833-2020, https://doi.org/10.5194/angeo-38-833-2020, 2020
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This paper is the first to study how the representation of the magnetic-local-time (MLT) dependency of electron precipitation impacts middle-atmospheric-ozone response on monthly timescales. We use a state-of-the-art chemistry–climate model with detailed lower-ionospheric chemistry for an advanced representation of atmospheric impacts of electron forcing. We find that the use of daily zonal-mean electron forcing will provide an accurate ozone response in long-term climate simulations.
Daniele Visioni, Giovanni Pitari, Vincenzo Rizi, Marco Iarlori, Irene Cionni, Ilaria Quaglia, Hideharu Akiyoshi, Slimane Bekki, Neal Butchart, Martin Chipperfield, Makoto Deushi, Sandip S. Dhomse, Rolando Garcia, Patrick Joeckel, Douglas Kinnison, Jean-François Lamarque, Marion Marchand, Martine Michou, Olaf Morgenstern, Tatsuya Nagashima, Fiona M. O'Connor, Luke D. Oman, David Plummer, Eugene Rozanov, David Saint-Martin, Robyn Schofield, John Scinocca, Andrea Stenke, Kane Stone, Kengo Sudo, Taichu Y. Tanaka, Simone Tilmes, Holger Tost, Yousuke Yamashita, and Guang Zeng
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-525, https://doi.org/10.5194/acp-2020-525, 2020
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In this work we analyse the trend in ozone profiles taken at L'Aquila (Italy, 42.4° N) for seventeen years, between 2000 and 2016 and compare them against already available measured ozone trends. We try to understand and explain the observed trends at various heights in light of the simulations from seventeen different model, highlighting the contribution of changes in circulation and chemical ozone loss during this time period.
Markus Kunze, Tim Kruschke, Ulrike Langematz, Miriam Sinnhuber, Thomas Reddmann, and Katja Matthes
Atmos. Chem. Phys., 20, 6991–7019, https://doi.org/10.5194/acp-20-6991-2020, https://doi.org/10.5194/acp-20-6991-2020, 2020
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Modelling the response of the atmosphere and its constituents to 11-year solar variations is subject to a certain uncertainty arising from the solar irradiance data set used in the chemistry–climate model (CCM) and the applied CCM itself.
This study reveals significant influences from both sources on the variations in the solar response in the stratosphere and mesosphere.
However, there are also regions where the random, unexplained part of the variations in the solar response is largest.
Marta Abalos, Clara Orbe, Douglas E. Kinnison, David Plummer, Luke D. Oman, Patrick Jöckel, Olaf Morgenstern, Rolando R. Garcia, Guang Zeng, Kane A. Stone, and Martin Dameris
Atmos. Chem. Phys., 20, 6883–6901, https://doi.org/10.5194/acp-20-6883-2020, https://doi.org/10.5194/acp-20-6883-2020, 2020
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A set of state-of-the art chemistry–climate models is used to examine future changes in downward transport from the stratosphere, a key contributor to tropospheric ozone. The acceleration of the stratospheric circulation results in increased stratosphere-to-troposphere transport. In the subtropics, downward advection into the troposphere is enhanced due to climate change. At higher latitudes, the ozone reservoir above the tropopause is enlarged due to the stronger circulation and ozone recovery.
Emily M. Gordon, Annika Seppälä, and Johanna Tamminen
Atmos. Chem. Phys., 20, 6259–6271, https://doi.org/10.5194/acp-20-6259-2020, https://doi.org/10.5194/acp-20-6259-2020, 2020
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The Sun constantly emits high-energy charged particles that produce the ozone destroying chemical NOx in the polar atmosphere. NOx is transported to the stratosphere, where the ozone layer is. Satellite observations show that the NOx gases remain in the atmosphere longer than previously reported. This is influenced by the strength of atmospheric large-scale dynamics, suggesting that there are specific times when this type of solar influence on the Antarctic atmosphere becomes more pronounced.
Clara Orbe, David A. Plummer, Darryn W. Waugh, Huang Yang, Patrick Jöckel, Douglas E. Kinnison, Beatrice Josse, Virginie Marecal, Makoto Deushi, Nathan Luke Abraham, Alexander T. Archibald, Martyn P. Chipperfield, Sandip Dhomse, Wuhu Feng, and Slimane Bekki
Atmos. Chem. Phys., 20, 3809–3840, https://doi.org/10.5194/acp-20-3809-2020, https://doi.org/10.5194/acp-20-3809-2020, 2020
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Atmospheric composition is strongly influenced by global-scale winds that are not always properly simulated in computer models. A common approach to correct for this bias is to relax or
nudgeto the observed winds. Here we systematically evaluate how well this technique performs across a large suite of chemistry–climate models in terms of its ability to reproduce key aspects of both the tropospheric and stratospheric circulations.
Julie M. Nicely, Bryan N. Duncan, Thomas F. Hanisco, Glenn M. Wolfe, Ross J. Salawitch, Makoto Deushi, Amund S. Haslerud, Patrick Jöckel, Béatrice Josse, Douglas E. Kinnison, Andrew Klekociuk, Michael E. Manyin, Virginie Marécal, Olaf Morgenstern, Lee T. Murray, Gunnar Myhre, Luke D. Oman, Giovanni Pitari, Andrea Pozzer, Ilaria Quaglia, Laura E. Revell, Eugene Rozanov, Andrea Stenke, Kane Stone, Susan Strahan, Simone Tilmes, Holger Tost, Daniel M. Westervelt, and Guang Zeng
Atmos. Chem. Phys., 20, 1341–1361, https://doi.org/10.5194/acp-20-1341-2020, https://doi.org/10.5194/acp-20-1341-2020, 2020
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Differences in methane lifetime among global models are large and poorly understood. We use a neural network method and simulations from the Chemistry Climate Model Initiative to quantify the factors influencing methane lifetime spread among models and variations over time. UV photolysis, tropospheric ozone, and nitrogen oxides drive large model differences, while the same factors plus specific humidity contribute to a decreasing trend in methane lifetime between 1980 and 2015.
Elizabeth Asher, Rebecca S. Hornbrook, Britton B. Stephens, Doug Kinnison, Eric J. Morgan, Ralph F. Keeling, Elliot L. Atlas, Sue M. Schauffler, Simone Tilmes, Eric A. Kort, Martin S. Hoecker-Martínez, Matt C. Long, Jean-François Lamarque, Alfonso Saiz-Lopez, Kathryn McKain, Colm Sweeney, Alan J. Hills, and Eric C. Apel
Atmos. Chem. Phys., 19, 14071–14090, https://doi.org/10.5194/acp-19-14071-2019, https://doi.org/10.5194/acp-19-14071-2019, 2019
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Halogenated organic trace gases, which are a source of reactive halogens to the atmosphere, exert a disproportionately large influence on atmospheric chemistry and climate. This paper reports novel aircraft observations of halogenated compounds over the Southern Ocean in summer and evaluates hypothesized regional sources and emissions of these trace gases through their relationships to additional aircraft observations.
Yuanhong Zhao, Marielle Saunois, Philippe Bousquet, Xin Lin, Antoine Berchet, Michaela I. Hegglin, Josep G. Canadell, Robert B. Jackson, Didier A. Hauglustaine, Sophie Szopa, Ann R. Stavert, Nathan Luke Abraham, Alex T. Archibald, Slimane Bekki, Makoto Deushi, Patrick Jöckel, Béatrice Josse, Douglas Kinnison, Ole Kirner, Virginie Marécal, Fiona M. O'Connor, David A. Plummer, Laura E. Revell, Eugene Rozanov, Andrea Stenke, Sarah Strode, Simone Tilmes, Edward J. Dlugokencky, and Bo Zheng
Atmos. Chem. Phys., 19, 13701–13723, https://doi.org/10.5194/acp-19-13701-2019, https://doi.org/10.5194/acp-19-13701-2019, 2019
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The role of hydroxyl radical changes in methane trends is debated, hindering our understanding of the methane cycle. This study quantifies how uncertainties in the hydroxyl radical may influence methane abundance in the atmosphere based on the inter-model comparison of hydroxyl radical fields and model simulations of CH4 abundance with different hydroxyl radical scenarios during 2000–2016. We show that hydroxyl radical changes could contribute up to 54 % of model-simulated methane biases.
Andreas Chrysanthou, Amanda C. Maycock, Martyn P. Chipperfield, Sandip Dhomse, Hella Garny, Douglas Kinnison, Hideharu Akiyoshi, Makoto Deushi, Rolando R. Garcia, Patrick Jöckel, Oliver Kirner, Giovanni Pitari, David A. Plummer, Laura Revell, Eugene Rozanov, Andrea Stenke, Taichu Y. Tanaka, Daniele Visioni, and Yousuke Yamashita
Atmos. Chem. Phys., 19, 11559–11586, https://doi.org/10.5194/acp-19-11559-2019, https://doi.org/10.5194/acp-19-11559-2019, 2019
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We perform the first multi-model comparison of the impact of nudged meteorology on the stratospheric residual circulation (RC) in chemistry–climate models. Nudging meteorology does not constrain the mean strength of RC compared to free-running simulations, and despite the lack of agreement in the mean circulation, nudging tightly constrains the inter-annual variability in the tropical upward mass flux in the lower stratosphere. In summary, nudging strongly affects the representation of RC.
Kévin Lamy, Thierry Portafaix, Béatrice Josse, Colette Brogniez, Sophie Godin-Beekmann, Hassan Bencherif, Laura Revell, Hideharu Akiyoshi, Slimane Bekki, Michaela I. Hegglin, Patrick Jöckel, Oliver Kirner, Ben Liley, Virginie Marecal, Olaf Morgenstern, Andrea Stenke, Guang Zeng, N. Luke Abraham, Alexander T. Archibald, Neil Butchart, Martyn P. Chipperfield, Glauco Di Genova, Makoto Deushi, Sandip S. Dhomse, Rong-Ming Hu, Douglas Kinnison, Michael Kotkamp, Richard McKenzie, Martine Michou, Fiona M. O'Connor, Luke D. Oman, Giovanni Pitari, David A. Plummer, John A. Pyle, Eugene Rozanov, David Saint-Martin, Kengo Sudo, Taichu Y. Tanaka, Daniele Visioni, and Kohei Yoshida
Atmos. Chem. Phys., 19, 10087–10110, https://doi.org/10.5194/acp-19-10087-2019, https://doi.org/10.5194/acp-19-10087-2019, 2019
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In this study, we simulate the ultraviolet radiation evolution during the 21st century on Earth's surface using the output from several numerical models which participated in the Chemistry-Climate Model Initiative. We present four possible futures which depend on greenhouse gases emissions. The role of ozone-depleting substances, greenhouse gases and aerosols are investigated. Our results emphasize the important role of aerosols for future ultraviolet radiation in the Northern Hemisphere.
Pavle Arsenovic, Alessandro Damiani, Eugene Rozanov, Bernd Funke, Andrea Stenke, and Thomas Peter
Atmos. Chem. Phys., 19, 9485–9494, https://doi.org/10.5194/acp-19-9485-2019, https://doi.org/10.5194/acp-19-9485-2019, 2019
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Low-energy electrons (LEE) are the dominant source of odd nitrogen, which destroys ozone, in the mesosphere and stratosphere in polar winter in the geomagnetically active periods. However, the observed stratospheric ozone anomalies can be reproduced only when accounting for both low- and middle-range energy electrons (MEE) in the chemistry-climate model. Ozone changes may induce further dynamical and thermal changes in the atmosphere. We recommend including both LEE and MEE in climate models.
Ohad Harari, Chaim I. Garfinkel, Shlomi Ziskin Ziv, Olaf Morgenstern, Guang Zeng, Simone Tilmes, Douglas Kinnison, Makoto Deushi, Patrick Jöckel, Andrea Pozzer, Fiona M. O'Connor, and Sean Davis
Atmos. Chem. Phys., 19, 9253–9268, https://doi.org/10.5194/acp-19-9253-2019, https://doi.org/10.5194/acp-19-9253-2019, 2019
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Ozone depletion in the Antarctic has been shown to influence surface conditions, but the effects of ozone depletion in the Arctic on surface climate are unclear. We show that Arctic ozone does influence surface climate in both polar regions and tropical regions, though the proximate cause of these surface impacts is not yet clear.
Mark E. Hervig, Benjamin T. Marshall, Scott M. Bailey, David E. Siskind, James M. Russell III, Charles G. Bardeen, Kaley A. Walker, and Bernd Funke
Atmos. Meas. Tech., 12, 3111–3121, https://doi.org/10.5194/amt-12-3111-2019, https://doi.org/10.5194/amt-12-3111-2019, 2019
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The Solar Occultation for Ice Experiment (SOFIE) has measured nitric oxide (NO) from satellite since 2007. The observations are validated through error analysis and comparisons with other satellite observations. Calculated SOFIE NO uncertainties are less than 50 % for altitudes from 40 to 140 km. SOFIE agrees with other measurements to within 50 % for altitudes from roughly 50 to 105 km for spacecraft sunrise and 50 to 140 km for sunsets.
Huang Yang, Darryn W. Waugh, Clara Orbe, Guang Zeng, Olaf Morgenstern, Douglas E. Kinnison, Jean-Francois Lamarque, Simone Tilmes, David A. Plummer, Patrick Jöckel, Susan E. Strahan, Kane A. Stone, and Robyn Schofield
Atmos. Chem. Phys., 19, 5511–5528, https://doi.org/10.5194/acp-19-5511-2019, https://doi.org/10.5194/acp-19-5511-2019, 2019
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We evaluate the performance of a suite of models in simulating the large-scale transport from the northern midlatitudes to the Arctic using a CO-like idealized tracer. We find a large multi-model spread of the Arctic concentration of this CO-like tracer that is well correlated with the differences in the location of the midlatitude jet as well as the northern Hadley Cell edge. Our results suggest the Hadley Cell is key and zonal-mean transport by surface meridional flow needs better constraint.
Marianna Linz, Marta Abalos, Anne Sasha Glanville, Douglas E. Kinnison, Alison Ming, and Jessica L. Neu
Atmos. Chem. Phys., 19, 5069–5090, https://doi.org/10.5194/acp-19-5069-2019, https://doi.org/10.5194/acp-19-5069-2019, 2019
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The stratospheric circulation is important for transporting ozone and water vapor, and models of the stratosphere differ. The metrics used to compare models are inconsistent between studies and cannot be calculated from observational data. In this paper, we explore a metric for the circulation that can be calculated from observations and examine how it relates to the more commonly used metrics. We find substantial differences in the upper and lower stratosphere depending on the choice of metric.
Lucien Froidevaux, Douglas E. Kinnison, Ray Wang, John Anderson, and Ryan A. Fuller
Atmos. Chem. Phys., 19, 4783–4821, https://doi.org/10.5194/acp-19-4783-2019, https://doi.org/10.5194/acp-19-4783-2019, 2019
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This work evaluates two versions of a 3-D global model of upper-atmospheric composition for recent decades. The two versions differ mainly in their dynamical (wind) constraints. Model–data differences, variability, and trends in five gases (ozone, H2O, HCl, HNO3, and N2O) are compared. While the match between models and observations is impressive, a few areas of discrepancy are noted. This work also updates trends in composition based on recent satellite-based measurements (through 2018).
Tao Yuan, Wuhu Feng, John M. C. Plane, and Daniel R. Marsh
Atmos. Chem. Phys., 19, 3769–3777, https://doi.org/10.5194/acp-19-3769-2019, https://doi.org/10.5194/acp-19-3769-2019, 2019
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The Na layer in the upper atmosphere is very sensitive to solar radiation and varies considerably during sunrise and sunset. In this paper, we use the lidar observations and an advanced model to investigate this process. We found that the variation is mostly due to the changes in several photochemical reactions involving Na compounds, especially NaHCO3. We also reveal that the Fe layer in the same region changes more quickly than the Na layer due to a faster reaction rate of FeOH to sunlight.
David A. Newnham, Mark A. Clilverd, Michael Kosch, Annika Seppälä, and Pekka T. Verronen
Atmos. Meas. Tech., 12, 1375–1392, https://doi.org/10.5194/amt-12-1375-2019, https://doi.org/10.5194/amt-12-1375-2019, 2019
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A simulation study has been carried out to investigate the potential for observing ozone and hydroxyl radical abundances in the mesosphere and lower thermosphere using ground-based passive microwave radiometry. In the polar middle atmosphere these chemical species respond strongly to geomagnetic activity associated with space weather. The results show that measuring diurnal variations in ozone and hydroxyl from high-latitude Northern Hemisphere and Antarctic locations would be possible.
Stefan Bender, Miriam Sinnhuber, Patrick J. Espy, and John P. Burrows
Atmos. Chem. Phys., 19, 2135–2147, https://doi.org/10.5194/acp-19-2135-2019, https://doi.org/10.5194/acp-19-2135-2019, 2019
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We present an empirical model for nitric oxide (NO) in the mesosphere (60–90 km) derived from SCIAMACHY limb scan data. Our model relates the daily (longitudinally) averaged NO number densities from SCIAMACHY as a function of geomagnetic latitude to the solar Lyman-alpha and the geomagnetic AE indices. We use a non-linear regression model, incorporating a finite and seasonally varying lifetime for the geomagnetically induced NO.
Tilo Fytterer, Christian von Savigny, Martin Mlynczak, and Miriam Sinnhuber
Atmos. Chem. Phys., 19, 1835–1851, https://doi.org/10.5194/acp-19-1835-2019, https://doi.org/10.5194/acp-19-1835-2019, 2019
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A model was developed to derive night-time atomic oxygen (O(3P)) and atomic hydrogen (H) from satellite observations in the altitude region between 75 km and 100 km. Comparisons between the
best-fit modeland the measurements suggest that chemical reactions involving O2 and O(3P) might occur differently than is usually assumed in literature. This considerably affects the derived abundances of O(3P) and H, which in turn might influence air temperature and winds of the whole atmosphere.
David E. Siskind, McArthur Jones Jr., Douglas P. Drob, John P. McCormack, Mark E. Hervig, Daniel R. Marsh, Martin G. Mlynczak, Scott M. Bailey, Astrid Maute, and Nicholas J. Mitchell
Ann. Geophys., 37, 37–48, https://doi.org/10.5194/angeo-37-37-2019, https://doi.org/10.5194/angeo-37-37-2019, 2019
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We use data from two NASA satellites and a general circulation model of the upper atmosphere to elucidate the key factors governing the abundance and diurnal variation of nitric oxide (NO) at near-solar minimum conditions and low latitudes. This has been difficult to do previously, because NO data are typically taken from satellites in sun-synchronous orbits, meaning that they only acquire data in fixed local times. We overcome this limitation through model simulations of the NO diurnal cycle.
Roland Eichinger, Simone Dietmüller, Hella Garny, Petr Šácha, Thomas Birner, Harald Bönisch, Giovanni Pitari, Daniele Visioni, Andrea Stenke, Eugene Rozanov, Laura Revell, David A. Plummer, Patrick Jöckel, Luke Oman, Makoto Deushi, Douglas E. Kinnison, Rolando Garcia, Olaf Morgenstern, Guang Zeng, Kane Adam Stone, and Robyn Schofield
Atmos. Chem. Phys., 19, 921–940, https://doi.org/10.5194/acp-19-921-2019, https://doi.org/10.5194/acp-19-921-2019, 2019
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To shed more light upon the changes in stratospheric circulation in the 21st century, climate projection simulations of 10 state-of-the-art global climate models, spanning from 1960 to 2100, are analyzed. The study shows that in addition to changes in transport, mixing also plays an important role in stratospheric circulation and that the properties of mixing vary over time. Furthermore, the influence of mixing is quantified and a dynamical framework is provided to understand the changes.
Laura E. Revell, Andrea Stenke, Fiona Tummon, Aryeh Feinberg, Eugene Rozanov, Thomas Peter, N. Luke Abraham, Hideharu Akiyoshi, Alexander T. Archibald, Neal Butchart, Makoto Deushi, Patrick Jöckel, Douglas Kinnison, Martine Michou, Olaf Morgenstern, Fiona M. O'Connor, Luke D. Oman, Giovanni Pitari, David A. Plummer, Robyn Schofield, Kane Stone, Simone Tilmes, Daniele Visioni, Yousuke Yamashita, and Guang Zeng
Atmos. Chem. Phys., 18, 16155–16172, https://doi.org/10.5194/acp-18-16155-2018, https://doi.org/10.5194/acp-18-16155-2018, 2018
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Global models such as those participating in the Chemistry-Climate Model Initiative (CCMI) consistently simulate biases in tropospheric ozone compared with observations. We performed an advanced statistical analysis with one of the CCMI models to understand the cause of the bias. We found that emissions of ozone precursor gases are the dominant driver of the bias, implying either that the emissions are too large, or that the way in which the model handles emissions needs to be improved.
Tao Li, Chao Ban, Xin Fang, Jing Li, Zhaopeng Wu, Wuhu Feng, John M. C. Plane, Jiangang Xiong, Daniel R. Marsh, Michael J. Mills, and Xiankang Dou
Atmos. Chem. Phys., 18, 11683–11695, https://doi.org/10.5194/acp-18-11683-2018, https://doi.org/10.5194/acp-18-11683-2018, 2018
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A total of 154 nights of observations by the USTC Na temperature and wind lidar (32° N, 117° E) suggest significant seasonal variability in the mesopause. Chemistry plays an important role in Na atom formation. More than half of the observed gravity wave (GW) momentum flux (MF), whose divergence determines the GW forcing, is induced by short-period (10 min–2 h) waves. The anticorrelation between MF and zonal wind (U) suggests strong filtering of short-period GWs by semiannual oscillation U.
Amanda C. Maycock, Katja Matthes, Susann Tegtmeier, Hauke Schmidt, Rémi Thiéblemont, Lon Hood, Hideharu Akiyoshi, Slimane Bekki, Makoto Deushi, Patrick Jöckel, Oliver Kirner, Markus Kunze, Marion Marchand, Daniel R. Marsh, Martine Michou, David Plummer, Laura E. Revell, Eugene Rozanov, Andrea Stenke, Yousuke Yamashita, and Kohei Yoshida
Atmos. Chem. Phys., 18, 11323–11343, https://doi.org/10.5194/acp-18-11323-2018, https://doi.org/10.5194/acp-18-11323-2018, 2018
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The 11-year solar cycle is an important driver of climate variability. Changes in incoming solar ultraviolet radiation affect atmospheric ozone, which in turn influences atmospheric temperatures. Constraining the impact of the solar cycle on ozone is therefore important for understanding climate variability. This study examines the representation of the solar influence on ozone in numerical models used to simulate past and future climate. We highlight important differences among model datasets.
Alexandra Laeng, Ellen Eckert, Thomas von Clarmann, Michael Kiefer, Daan Hubert, Gabriele Stiller, Norbert Glatthor, Manuel López-Puertas, Bernd Funke, Udo Grabowski, Johannes Plieninger, Sylvia Kellmann, Andrea Linden, Stefan Lossow, Arne Babenhauserheide, Lucien Froidevaux, and Kaley Walker
Atmos. Meas. Tech., 11, 4693–4705, https://doi.org/10.5194/amt-11-4693-2018, https://doi.org/10.5194/amt-11-4693-2018, 2018
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MIPAS was an IR limb emission spectrometer on the Envisat platform. From 2002 to 2012, it performed pole-to-pole measurements of ozone during day and night. ESA recently released the new version 7 of Level 1 MIPAS spectra, which is expected to reduce the long-term drift of the MIPAS Level 2 data. We evaluate the long-term stability of ozone Level 2 data from the KIT IMK processor. Our results indicate that MIPAS data are now even more suited for trend studies, alone or as part of merged data.
Koen Hendrickx, Linda Megner, Daniel R. Marsh, and Christine Smith-Johnsen
Atmos. Chem. Phys., 18, 9075–9089, https://doi.org/10.5194/acp-18-9075-2018, https://doi.org/10.5194/acp-18-9075-2018, 2018
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The mechanisms that produce, destroy and transport nitric oxide (NO) in the Antarctic mesosphere and lower thermosphere are investigated in AIM-SOFIE satellite observations and compared to SD-WACCM simulations. During winter, NO concentrations are most similar while the altitude of maximum NO number densities is most separated. Even though the rate of descent is similar in both datasets, the simulated descending NO flux is too low in concentration, which reflects a missing source of NO.
Jens-Uwe Grooß, Rolf Müller, Reinhold Spang, Ines Tritscher, Tobias Wegner, Martyn P. Chipperfield, Wuhu Feng, Douglas E. Kinnison, and Sasha Madronich
Atmos. Chem. Phys., 18, 8647–8666, https://doi.org/10.5194/acp-18-8647-2018, https://doi.org/10.5194/acp-18-8647-2018, 2018
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We investigate a discrepancy between model simulations and observations of HCl in the dark polar stratosphere. In early winter, the less-well-studied period of the onset of chlorine activation, observations show a much faster depletion of HCl than simulations of three models. This points to some unknown process that is currently not represented in the models. Various hypotheses for potential causes are investigated that partly reduce the discrepancy. The impact on polar ozone depletion is low.
Sandip S. Dhomse, Douglas Kinnison, Martyn P. Chipperfield, Ross J. Salawitch, Irene Cionni, Michaela I. Hegglin, N. Luke Abraham, Hideharu Akiyoshi, Alex T. Archibald, Ewa M. Bednarz, Slimane Bekki, Peter Braesicke, Neal Butchart, Martin Dameris, Makoto Deushi, Stacey Frith, Steven C. Hardiman, Birgit Hassler, Larry W. Horowitz, Rong-Ming Hu, Patrick Jöckel, Beatrice Josse, Oliver Kirner, Stefanie Kremser, Ulrike Langematz, Jared Lewis, Marion Marchand, Meiyun Lin, Eva Mancini, Virginie Marécal, Martine Michou, Olaf Morgenstern, Fiona M. O'Connor, Luke Oman, Giovanni Pitari, David A. Plummer, John A. Pyle, Laura E. Revell, Eugene Rozanov, Robyn Schofield, Andrea Stenke, Kane Stone, Kengo Sudo, Simone Tilmes, Daniele Visioni, Yousuke Yamashita, and Guang Zeng
Atmos. Chem. Phys., 18, 8409–8438, https://doi.org/10.5194/acp-18-8409-2018, https://doi.org/10.5194/acp-18-8409-2018, 2018
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We analyse simulations from the Chemistry-Climate Model Initiative (CCMI) to estimate the return dates of the stratospheric ozone layer from depletion by anthropogenic chlorine and bromine. The simulations from 20 models project that global column ozone will return to 1980 values in 2047 (uncertainty range 2042–2052). Return dates in other regions vary depending on factors related to climate change and importance of chlorine and bromine. Column ozone in the tropics may continue to decline.
Stefan Lossow, Dale F. Hurst, Karen H. Rosenlof, Gabriele P. Stiller, Thomas von Clarmann, Sabine Brinkop, Martin Dameris, Patrick Jöckel, Doug E. Kinnison, Johannes Plieninger, David A. Plummer, Felix Ploeger, William G. Read, Ellis E. Remsberg, James M. Russell, and Mengchu Tao
Atmos. Chem. Phys., 18, 8331–8351, https://doi.org/10.5194/acp-18-8331-2018, https://doi.org/10.5194/acp-18-8331-2018, 2018
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Trend estimates of lower stratospheric H2O derived from the FPH observations at Boulder and a merged zonal mean satellite data set clearly differ for the time period from the late 1980s to 2010. We investigate if a sampling bias between Boulder and the zonal mean around the Boulder latitude can explain these trend discrepancies. Typically they are small and not sufficient to explain the trend discrepancies in the observational database.
Clara Orbe, Huang Yang, Darryn W. Waugh, Guang Zeng, Olaf Morgenstern, Douglas E. Kinnison, Jean-Francois Lamarque, Simone Tilmes, David A. Plummer, John F. Scinocca, Beatrice Josse, Virginie Marecal, Patrick Jöckel, Luke D. Oman, Susan E. Strahan, Makoto Deushi, Taichu Y. Tanaka, Kohei Yoshida, Hideharu Akiyoshi, Yousuke Yamashita, Andreas Stenke, Laura Revell, Timofei Sukhodolov, Eugene Rozanov, Giovanni Pitari, Daniele Visioni, Kane A. Stone, Robyn Schofield, and Antara Banerjee
Atmos. Chem. Phys., 18, 7217–7235, https://doi.org/10.5194/acp-18-7217-2018, https://doi.org/10.5194/acp-18-7217-2018, 2018
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In this study we compare a few atmospheric transport properties among several numerical models that are used to study the influence of atmospheric chemistry on climate. We show that there are large differences among models in terms of the timescales that connect the Northern Hemisphere midlatitudes, where greenhouse gases and ozone-depleting substances are emitted, to the Southern Hemisphere. Our results may have important implications for how models represent atmospheric composition.
Simone Dietmüller, Roland Eichinger, Hella Garny, Thomas Birner, Harald Boenisch, Giovanni Pitari, Eva Mancini, Daniele Visioni, Andrea Stenke, Laura Revell, Eugene Rozanov, David A. Plummer, John Scinocca, Patrick Jöckel, Luke Oman, Makoto Deushi, Shibata Kiyotaka, Douglas E. Kinnison, Rolando Garcia, Olaf Morgenstern, Guang Zeng, Kane Adam Stone, and Robyn Schofield
Atmos. Chem. Phys., 18, 6699–6720, https://doi.org/10.5194/acp-18-6699-2018, https://doi.org/10.5194/acp-18-6699-2018, 2018
Martin G. Schultz, Scarlet Stadtler, Sabine Schröder, Domenico Taraborrelli, Bruno Franco, Jonathan Krefting, Alexandra Henrot, Sylvaine Ferrachat, Ulrike Lohmann, David Neubauer, Colombe Siegenthaler-Le Drian, Sebastian Wahl, Harri Kokkola, Thomas Kühn, Sebastian Rast, Hauke Schmidt, Philip Stier, Doug Kinnison, Geoffrey S. Tyndall, John J. Orlando, and Catherine Wespes
Geosci. Model Dev., 11, 1695–1723, https://doi.org/10.5194/gmd-11-1695-2018, https://doi.org/10.5194/gmd-11-1695-2018, 2018
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The chemistry–climate model ECHAM-HAMMOZ contains a detailed representation of tropospheric and stratospheric reactive chemistry and state-of-the-art parameterizations of aerosols. It thus allows for detailed investigations of chemical processes in the climate system. Evaluation of the model with various observational data yields good results, but the model has a tendency to produce too much OH in the tropics. This highlights the important interplay between atmospheric chemistry and dynamics.
Fernando Iglesias-Suarez, Douglas E. Kinnison, Alexandru Rap, Amanda C. Maycock, Oliver Wild, and Paul J. Young
Atmos. Chem. Phys., 18, 6121–6139, https://doi.org/10.5194/acp-18-6121-2018, https://doi.org/10.5194/acp-18-6121-2018, 2018
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This study explores future ozone radiative forcing (RF) and the relative contribution due to different drivers. Climate-induced ozone RF is largely the result of the interplay between lightning-produced ozone and enhanced ozone destruction in a warmer and wetter atmosphere. These results demonstrate the importance of stratospheric–tropospheric interactions and the stratosphere as a key region controlling a large fraction of the tropospheric ozone RF.
Manuel López-Puertas, Maya García-Comas, Bernd Funke, Angela Gardini, Gabriele P. Stiller, Thomas von Clarmann, Norbert Glatthor, Alexandra Laeng, Martin Kaufmann, Viktoria F. Sofieva, Lucien Froidevaux, Kaley A. Walker, and Masato Shiotani
Atmos. Meas. Tech., 11, 2187–2212, https://doi.org/10.5194/amt-11-2187-2018, https://doi.org/10.5194/amt-11-2187-2018, 2018
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This paper describes the inversion of O3 data from MIPAS middle atmosphere spectra which requires non-LTE. The O3 dataset comprises from 20 to 100 km, has a pole-to-pole latitude coverage, day and nighttime, and span from 2005 until 2012. A validation of the data against other satellite measurements and an overall description of O3 is also presented. This is an important dataset for the community and describes the major characteristics of stratospheric and mesospheric O3.
Erkki Kyrölä, Monika E. Andersson, Pekka T. Verronen, Marko Laine, Simo Tukiainen, and Daniel R. Marsh
Atmos. Chem. Phys., 18, 5001–5019, https://doi.org/10.5194/acp-18-5001-2018, https://doi.org/10.5194/acp-18-5001-2018, 2018
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In this work we compare three key constituents of the middle atmosphere (ozone, NO2, and NO3) from the GOMOS satellite instrument with the WACCM model. We find that in the stratosphere (below 50 km) ozone differences are very small, but in the mesosphere large deviations are found. GOMOS and WACCM NO2 agree reasonably well except in the polar areas. These differences can be connected to the solar particle storms. For NO3, WACCM results agree with GOMOS with a very high correlation.
Niall J. Ryan, Douglas E. Kinnison, Rolando R. Garcia, Christoph G. Hoffmann, Mathias Palm, Uwe Raffalski, and Justus Notholt
Atmos. Chem. Phys., 18, 1457–1474, https://doi.org/10.5194/acp-18-1457-2018, https://doi.org/10.5194/acp-18-1457-2018, 2018
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We used model output and instrument data to assess how well polar atmospheric descent rates can be derived using concentration measurements of long-lived gases in the atmosphere. The results indicate that the method incurs errors as large as the descent rates, and often leads to a misinterpretation of the direction of air motion. The rates derived using this method do not appear to represent the mean vertical wind in the middle atmosphere, and we suggest an alternate definition.
Miriam Sinnhuber, Uwe Berger, Bernd Funke, Holger Nieder, Thomas Reddmann, Gabriele Stiller, Stefan Versick, Thomas von Clarmann, and Jan Maik Wissing
Atmos. Chem. Phys., 18, 1115–1147, https://doi.org/10.5194/acp-18-1115-2018, https://doi.org/10.5194/acp-18-1115-2018, 2018
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Results from global models are used to analyze the impact of energetic particle precipitation on the middle atmosphere (10–80 km). Model results agree well with observations, and show strong enhancements of NOy, long-lasting ozone loss, and a net heating in the uppermost stratosphere (~35–45 km) during polar winter which changes sign in spring. Energetic particle precipitation therefore has the potential to impact atmospheric dynamics, starting from a warmer winter-time upper stratosphere.
Olaf Morgenstern, Kane A. Stone, Robyn Schofield, Hideharu Akiyoshi, Yousuke Yamashita, Douglas E. Kinnison, Rolando R. Garcia, Kengo Sudo, David A. Plummer, John Scinocca, Luke D. Oman, Michael E. Manyin, Guang Zeng, Eugene Rozanov, Andrea Stenke, Laura E. Revell, Giovanni Pitari, Eva Mancini, Glauco Di Genova, Daniele Visioni, Sandip S. Dhomse, and Martyn P. Chipperfield
Atmos. Chem. Phys., 18, 1091–1114, https://doi.org/10.5194/acp-18-1091-2018, https://doi.org/10.5194/acp-18-1091-2018, 2018
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We assess how ozone as simulated by a group of chemistry–climate models responds to variations in man-made climate gases and ozone-depleting substances. We find some agreement, particularly in the middle and upper stratosphere, but also considerable disagreement elsewhere. Such disagreement affects the reliability of future ozone projections based on these models, and also constitutes a source of uncertainty in climate projections using prescribed ozone derived from these simulations.
Amirmahdi Zarboo, Stefan Bender, John P. Burrows, Johannes Orphal, and Miriam Sinnhuber
Atmos. Meas. Tech., 11, 473–487, https://doi.org/10.5194/amt-11-473-2018, https://doi.org/10.5194/amt-11-473-2018, 2018
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We present the retrieved volume emission rates (VERs) from the airglow of both the daytime and twilight O2(1Σ) band and O2(1Δ) band emissions in the mesosphere and lower thermosphere (MLT). We have investigated the daily mean latitudinal distributions and the time series of the retrieved VER in the altitude range from 53 to 149 km. These observations provide information about the chemistry and dynamics and can be used to infer ozone, solar heating rates, and temperature in the MLT.
Justin Bandoro, Susan Solomon, Benjamin D. Santer, Douglas E. Kinnison, and Michael J. Mills
Atmos. Chem. Phys., 18, 143–166, https://doi.org/10.5194/acp-18-143-2018, https://doi.org/10.5194/acp-18-143-2018, 2018
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We studied the attribution of stratospheric ozone changes and identified similarities between observations and human fingerprints from both emissions of ozone-depleting substances (ODSs) and greenhouse gases (GHGs). We developed an improvement on the traditional pattern correlation method that accounts for nonlinearities in the climate forcing time evolution. Use of the latter resulted in increased S / N ratios for the ODS fingerprint. The GHG fingerprint was not identifiable.
Theodore K. Koenig, Rainer Volkamer, Sunil Baidar, Barbara Dix, Siyuan Wang, Daniel C. Anderson, Ross J. Salawitch, Pamela A. Wales, Carlos A. Cuevas, Rafael P. Fernandez, Alfonso Saiz-Lopez, Mathew J. Evans, Tomás Sherwen, Daniel J. Jacob, Johan Schmidt, Douglas Kinnison, Jean-François Lamarque, Eric C. Apel, James C. Bresch, Teresa Campos, Frank M. Flocke, Samuel R. Hall, Shawn B. Honomichl, Rebecca Hornbrook, Jørgen B. Jensen, Richard Lueb, Denise D. Montzka, Laura L. Pan, J. Michael Reeves, Sue M. Schauffler, Kirk Ullmann, Andrew J. Weinheimer, Elliot L. Atlas, Valeria Donets, Maria A. Navarro, Daniel Riemer, Nicola J. Blake, Dexian Chen, L. Gregory Huey, David J. Tanner, Thomas F. Hanisco, and Glenn M. Wolfe
Atmos. Chem. Phys., 17, 15245–15270, https://doi.org/10.5194/acp-17-15245-2017, https://doi.org/10.5194/acp-17-15245-2017, 2017
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Tropospheric inorganic bromine (BrO and Bry) shows a C-shaped profile over the tropical western Pacific Ocean, and supports previous speculation that marine convection is a source for inorganic bromine from sea salt to the upper troposphere. The Bry profile in the tropical tropopause layer (TTL) is complex, suggesting that the total Bry budget in the TTL is not closed without considering aerosol bromide. The implications for atmospheric composition and bromine sources are discussed.
Margarita Yela, Manuel Gil-Ojeda, Mónica Navarro-Comas, David Gonzalez-Bartolomé, Olga Puentedura, Bernd Funke, Javier Iglesias, Santiago Rodríguez, Omaira García, Héctor Ochoa, and Guillermo Deferrari
Atmos. Chem. Phys., 17, 13373–13389, https://doi.org/10.5194/acp-17-13373-2017, https://doi.org/10.5194/acp-17-13373-2017, 2017
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The paper focuses on stratospheric trends of NO2, a species involved in the ozone equilibrium, using data from four NDACC stations. The global stratospheric NO2 trend has not yet been established conclusively. We analyse DOAS data from stations in the Northern Hemisphere and Southern Hemisphere during 1993–2014. The most relevant finding is the hemispheric asymmetry found in the sign of the NO2 trend, providing further evidence of changes in the stratosphere dynamics on the global scale.
Johann H. Jungclaus, Edouard Bard, Mélanie Baroni, Pascale Braconnot, Jian Cao, Louise P. Chini, Tania Egorova, Michael Evans, J. Fidel González-Rouco, Hugues Goosse, George C. Hurtt, Fortunat Joos, Jed O. Kaplan, Myriam Khodri, Kees Klein Goldewijk, Natalie Krivova, Allegra N. LeGrande, Stephan J. Lorenz, Jürg Luterbacher, Wenmin Man, Amanda C. Maycock, Malte Meinshausen, Anders Moberg, Raimund Muscheler, Christoph Nehrbass-Ahles, Bette I. Otto-Bliesner, Steven J. Phipps, Julia Pongratz, Eugene Rozanov, Gavin A. Schmidt, Hauke Schmidt, Werner Schmutz, Andrew Schurer, Alexander I. Shapiro, Michael Sigl, Jason E. Smerdon, Sami K. Solanki, Claudia Timmreck, Matthew Toohey, Ilya G. Usoskin, Sebastian Wagner, Chi-Ju Wu, Kok Leng Yeo, Davide Zanchettin, Qiong Zhang, and Eduardo Zorita
Geosci. Model Dev., 10, 4005–4033, https://doi.org/10.5194/gmd-10-4005-2017, https://doi.org/10.5194/gmd-10-4005-2017, 2017
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Climate model simulations covering the last millennium provide context for the evolution of the modern climate and for the expected changes during the coming centuries. They can help identify plausible mechanisms underlying palaeoclimatic reconstructions. Here, we describe the forcing boundary conditions and the experimental protocol for simulations covering the pre-industrial millennium. We describe the PMIP4 past1000 simulations as contributions to CMIP6 and additional sensitivity experiments.
Gabriele P. Stiller, Federico Fierli, Felix Ploeger, Chiara Cagnazzo, Bernd Funke, Florian J. Haenel, Thomas Reddmann, Martin Riese, and Thomas von Clarmann
Atmos. Chem. Phys., 17, 11177–11192, https://doi.org/10.5194/acp-17-11177-2017, https://doi.org/10.5194/acp-17-11177-2017, 2017
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The discrepancy between modelled and observed 25-year trends of the strength of the stratospheric Brewer–Dobson circulation (BDC) is still not resolved. With our paper we trace the observed hemispheric dipole structure of age of air trends back to natural variability in shorter-term (decadal) time frames. Beyond this we demonstrate that after correction for the decadal natural variability the remaining trend for the first decade of the 21st century is consistent with model simulations.
Maria A. Navarro, Alfonso Saiz-Lopez, Carlos A. Cuevas, Rafael P. Fernandez, Elliot Atlas, Xavier Rodriguez-Lloveras, Douglas Kinnison, Jean-Francois Lamarque, Simone Tilmes, Troy Thornberry, Andrew Rollins, James W. Elkins, Eric J. Hintsa, and Fred L. Moore
Atmos. Chem. Phys., 17, 9917–9930, https://doi.org/10.5194/acp-17-9917-2017, https://doi.org/10.5194/acp-17-9917-2017, 2017
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Inorganic bromine (Bry) plays an important role in ozone layer depletion. Based on aircraft observations of organic bromine species and chemistry simulations, we model the Bry abundances over the Pacific tropical tropopause. Our results show BrO and Br as the dominant species during daytime hours, and BrCl and BrONO2 as the nighttime dominant species over the western and eastern Pacific, respectively. The difference in the partitioning is due to changes in the abundance of O3, NO2, and Cly.
Martin P. Langowski, Christian von Savigny, John P. Burrows, Didier Fussen, Erin C. M. Dawkins, Wuhu Feng, John M. C. Plane, and Daniel R. Marsh
Atmos. Meas. Tech., 10, 2989–3006, https://doi.org/10.5194/amt-10-2989-2017, https://doi.org/10.5194/amt-10-2989-2017, 2017
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Meteoric metals form metal layers in the upper atmosphere anandplay a role in the formation of middle-atmospheric clouds and aerosols. However, the total metal influx rate is not well known. Global Na datasets from measurements and a model are available, which had not been compared yet on a global scale until this paper. Overall the agreement is good, and many differences between measurements are also found in the model simulations. However, the modeled layer altitude is too low.
Ellen Eckert, Thomas von Clarmann, Alexandra Laeng, Gabriele P. Stiller, Bernd Funke, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Michael Kiefer, Andrea Linden, Arne Babenhauserheide, Gerald Wetzel, Christopher Boone, Andreas Engel, Jeremy J. Harrison, Patrick E. Sheese, Kaley A. Walker, and Peter F. Bernath
Atmos. Meas. Tech., 10, 2727–2743, https://doi.org/10.5194/amt-10-2727-2017, https://doi.org/10.5194/amt-10-2727-2017, 2017
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We retrieved vertical profiles of CCl4 from MIPAS Envisat IMK/IAA data. A detailed description of all characteristics is included in the paper as well as comparisons with historical measurements and comparisons with collocated measurements of instruments covering the same time span as MIPAS Envisat. A particular focus also lies on the usage of a new CCl4 spectroscopic dataset introduced recently, which leads to more realistic CCl4 volume mixing ratios.
Cristen Adams, Adam E. Bourassa, Chris A. McLinden, Chris E. Sioris, Thomas von Clarmann, Bernd Funke, Landon A. Rieger, and Douglas A. Degenstein
Atmos. Chem. Phys., 17, 8063–8080, https://doi.org/10.5194/acp-17-8063-2017, https://doi.org/10.5194/acp-17-8063-2017, 2017
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We measured the relationship between volcanic aerosol and trace gases in the stratosphere using the OSIRIS and MIPAS satellite instruments between 2002 and 2014. We found that levels of stratospheric NO2 and N2O5 both decreased significantly in the presence of volcanic aerosol. These decreases were consistent with the modeling results.
Katja Matthes, Bernd Funke, Monika E. Andersson, Luke Barnard, Jürg Beer, Paul Charbonneau, Mark A. Clilverd, Thierry Dudok de Wit, Margit Haberreiter, Aaron Hendry, Charles H. Jackman, Matthieu Kretzschmar, Tim Kruschke, Markus Kunze, Ulrike Langematz, Daniel R. Marsh, Amanda C. Maycock, Stergios Misios, Craig J. Rodger, Adam A. Scaife, Annika Seppälä, Ming Shangguan, Miriam Sinnhuber, Kleareti Tourpali, Ilya Usoskin, Max van de Kamp, Pekka T. Verronen, and Stefan Versick
Geosci. Model Dev., 10, 2247–2302, https://doi.org/10.5194/gmd-10-2247-2017, https://doi.org/10.5194/gmd-10-2247-2017, 2017
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The solar forcing dataset for climate model experiments performed for the upcoming IPCC report is described. This dataset provides the radiative and particle input of solar variability on a daily basis from 1850 through to 2300. With this dataset a better representation of natural climate variability with respect to the output of the Sun is provided which provides the most sophisticated and comprehensive respresentation of solar variability that has been used in climate model simulations so far.
Bernd Funke, William Ball, Stefan Bender, Angela Gardini, V. Lynn Harvey, Alyn Lambert, Manuel López-Puertas, Daniel R. Marsh, Katharina Meraner, Holger Nieder, Sanna-Mari Päivärinta, Kristell Pérot, Cora E. Randall, Thomas Reddmann, Eugene Rozanov, Hauke Schmidt, Annika Seppälä, Miriam Sinnhuber, Timofei Sukhodolov, Gabriele P. Stiller, Natalia D. Tsvetkova, Pekka T. Verronen, Stefan Versick, Thomas von Clarmann, Kaley A. Walker, and Vladimir Yushkov
Atmos. Chem. Phys., 17, 3573–3604, https://doi.org/10.5194/acp-17-3573-2017, https://doi.org/10.5194/acp-17-3573-2017, 2017
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Simulations from eight atmospheric models have been compared to tracer and temperature observations from seven satellite instruments in order to evaluate the energetic particle indirect effect (EPP IE) during the perturbed northern hemispheric (NH) winter 2008/2009. Models are capable to reproduce the EPP IE in dynamically and geomagnetically quiescent NH winter conditions. The results emphasize the need for model improvements in the dynamical representation of elevated stratopause events.
Olaf Morgenstern, Michaela I. Hegglin, Eugene Rozanov, Fiona M. O'Connor, N. Luke Abraham, Hideharu Akiyoshi, Alexander T. Archibald, Slimane Bekki, Neal Butchart, Martyn P. Chipperfield, Makoto Deushi, Sandip S. Dhomse, Rolando R. Garcia, Steven C. Hardiman, Larry W. Horowitz, Patrick Jöckel, Beatrice Josse, Douglas Kinnison, Meiyun Lin, Eva Mancini, Michael E. Manyin, Marion Marchand, Virginie Marécal, Martine Michou, Luke D. Oman, Giovanni Pitari, David A. Plummer, Laura E. Revell, David Saint-Martin, Robyn Schofield, Andrea Stenke, Kane Stone, Kengo Sudo, Taichu Y. Tanaka, Simone Tilmes, Yousuke Yamashita, Kohei Yoshida, and Guang Zeng
Geosci. Model Dev., 10, 639–671, https://doi.org/10.5194/gmd-10-639-2017, https://doi.org/10.5194/gmd-10-639-2017, 2017
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We present a review of the make-up of 20 models participating in the Chemistry–Climate Model Initiative (CCMI). In comparison to earlier such activities, most of these models comprise a whole-atmosphere chemistry, and several of them include an interactive ocean module. This makes them suitable for studying the interactions of tropospheric air quality, stratospheric ozone, and climate. The paper lays the foundation for other studies using the CCMI simulations for scientific analysis.
Rafael P. Fernandez, Douglas E. Kinnison, Jean-Francois Lamarque, Simone Tilmes, and Alfonso Saiz-Lopez
Atmos. Chem. Phys., 17, 1673–1688, https://doi.org/10.5194/acp-17-1673-2017, https://doi.org/10.5194/acp-17-1673-2017, 2017
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The inclusion of biogenic very-short lived bromine (VSLBr) in a chemistry-climate model produces an expansion of the ozone hole area of ~ 5 million km2, which is equivalent in magnitude to the recently estimated Antarctic ozone healing due to the reduction of anthropogenic CFCs and halons. The maximum Antarctic ozone hole depletion increases by up to 14 % when natural VSLBr are considered, but does not introduce a significant delay of the modelled ozone return date to 1980 October levels.
Tamás Kovács, Wuhu Feng, Anna Totterdill, John M. C. Plane, Sandip Dhomse, Juan Carlos Gómez-Martín, Gabriele P. Stiller, Florian J. Haenel, Christopher Smith, Piers M. Forster, Rolando R. García, Daniel R. Marsh, and Martyn P. Chipperfield
Atmos. Chem. Phys., 17, 883–898, https://doi.org/10.5194/acp-17-883-2017, https://doi.org/10.5194/acp-17-883-2017, 2017
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Sulfur hexafluoride (SF6) is a very potent greenhouse gas, which is present in the atmosphere only through its industrial use, for example as an electrical insulator. To estimate accurately the impact of SF6 emissions on climate we need to know how long it persists in the atmosphere before being removed. Previous estimates of the SF6 lifetime indicate a large degree of uncertainty. Here we use a detailed atmospheric model to calculate a current best estimate of the SF6 lifetime.
Stefan Bender, Miriam Sinnhuber, Martin Langowski, and John P. Burrows
Atmos. Meas. Tech., 10, 209–220, https://doi.org/10.5194/amt-10-209-2017, https://doi.org/10.5194/amt-10-209-2017, 2017
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We present the retrieval of NO number densities from 60 km to 85 km from measurements of SCIAMACHY/Envisat in its nominal limb mode (0–91 km). We derive the densities from the NO gamma bands (230–300 nm). Using prior input reduces the incorrect attribution of NO from the lower thermosphere. The SCIAMACHY nominal limb scans provide almost 10 years of daily NO data in this altitude range, a unique data record to constrain NO in the mesosphere for testing and validating chemistry climate models.
Á. Aythami Jurado-Navarro, Manuel López-Puertas, Bernd Funke, Maya García-Comas, Angela Gardini, Francisco González-Galindo, Gabriele P. Stiller, Thomas von Clarmann, Udo Grabowski, and Andrea Linden
Atmos. Meas. Tech., 9, 6081–6100, https://doi.org/10.5194/amt-9-6081-2016, https://doi.org/10.5194/amt-9-6081-2016, 2016
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We present global distributions of CO2 concentrations in the upper atmosphere (70–140 km) derived from high-resolution 4.3 µm MIPAS spectra from 2005 to 2012. CO2 relative abundances have been measured at 120–140 km for the first time. The data have an unprecedented accuracy. CO2 shows a strong seasonal behaviour. CO2 largely controls the temperature of the upper atmosphere and its measurement is very important for understanding the impact of climate change in this region.
Alfonso Saiz-Lopez, John M. C. Plane, Carlos A. Cuevas, Anoop S. Mahajan, Jean-François Lamarque, and Douglas E. Kinnison
Atmos. Chem. Phys., 16, 15593–15604, https://doi.org/10.5194/acp-16-15593-2016, https://doi.org/10.5194/acp-16-15593-2016, 2016
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Electronic structure calculations are used to survey possible reactions that HOI and I2 could undergo at night in the lower troposphere, and hence reconcile measurements and models. The reactions NO3 + HOI and I2 + NO3 are included in two models to explore a new nocturnal iodine radical activation mechanism, leading to a reduction of nighttime HOI and I2. This chemistry can have a large impact on NO3 levels in the MBL, and hence upon the nocturnal oxidizing capacity of the marine atmosphere.
Patrick E. Sheese, Kaley A. Walker, Chris D. Boone, Chris A. McLinden, Peter F. Bernath, Adam E. Bourassa, John P. Burrows, Doug A. Degenstein, Bernd Funke, Didier Fussen, Gloria L. Manney, C. Thomas McElroy, Donal Murtagh, Cora E. Randall, Piera Raspollini, Alexei Rozanov, James M. Russell III, Makoto Suzuki, Masato Shiotani, Joachim Urban, Thomas von Clarmann, and Joseph M. Zawodny
Atmos. Meas. Tech., 9, 5781–5810, https://doi.org/10.5194/amt-9-5781-2016, https://doi.org/10.5194/amt-9-5781-2016, 2016
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This study validates version 3.5 of the ACE-FTS NOy species data sets by comparing diurnally scaled ACE-FTS data to correlative data from 11 other satellite limb sounders. For all five species examined (NO, NO2, HNO3, N2O5, and ClONO2), there is good agreement between ACE-FTS and the other data sets in various regions of the atmosphere. In these validated regions, these NOy data products can be used for further investigation into the composition, dynamics, and climate of the stratosphere.
Nathan P. Gillett, Hideo Shiogama, Bernd Funke, Gabriele Hegerl, Reto Knutti, Katja Matthes, Benjamin D. Santer, Daithi Stone, and Claudia Tebaldi
Geosci. Model Dev., 9, 3685–3697, https://doi.org/10.5194/gmd-9-3685-2016, https://doi.org/10.5194/gmd-9-3685-2016, 2016
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Detection and attribution of climate change is the process of determining the causes of observed climate changes, which has underpinned key conclusions on the role of human influence on climate in the reports of the Intergovernmental Panel on Climate Change (IPCC). This paper describes a coordinated set of climate model experiments that will form part of the Sixth Coupled Model Intercomparison Project and will support improved attribution of climate change in the next IPCC report.
Tamás Kovács, John M. C. Plane, Wuhu Feng, Tibor Nagy, Martyn P. Chipperfield, Pekka T. Verronen, Monika E. Andersson, David A. Newnham, Mark A. Clilverd, and Daniel R. Marsh
Geosci. Model Dev., 9, 3123–3136, https://doi.org/10.5194/gmd-9-3123-2016, https://doi.org/10.5194/gmd-9-3123-2016, 2016
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This study was completed on D-region atmospheric model development. The sophisticated 3-D Whole Atmosphere Community Climate Model (WACCM) and the 1-D Sodynkalä Ion and Neutral Chemistry Model (SIC) were combined in order to provide a detailed, accurate model (WACCM-SIC) that considers the processes taking place in solar proton events. The original SIC model was reduced by mechanism reduction, which provided an accurate sub-mechanism (rSIC, WACCM-rSIC) of the original model.
Maya García-Comas, Francisco González-Galindo, Bernd Funke, Angela Gardini, Aythami Jurado-Navarro, Manuel López-Puertas, and William E. Ward
Atmos. Chem. Phys., 16, 11019–11041, https://doi.org/10.5194/acp-16-11019-2016, https://doi.org/10.5194/acp-16-11019-2016, 2016
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In this paper, for the first time, temperature longitudinal oscillations are derived from 20 to 150 km from a single instrument. A climatology of amplitudes and phases of zonal waves with odd daily frequencies is presented on a global scale. The interannual variability in amplitudes of the migrating modes shows a QBO in the MLT, which is probably originated in the stratosphere. The results are useful for testing general circulation models considering tidal effects in the MLT region.
E. Eckert, A. Laeng, S. Lossow, S. Kellmann, G. Stiller, T. von Clarmann, N. Glatthor, M. Höpfner, M. Kiefer, H. Oelhaf, J. Orphal, B. Funke, U. Grabowski, F. Haenel, A. Linden, G. Wetzel, W. Woiwode, P. F. Bernath, C. Boone, G. S. Dutton, J. W. Elkins, A. Engel, J. C. Gille, F. Kolonjari, T. Sugita, G. C. Toon, and K. A. Walker
Atmos. Meas. Tech., 9, 3355–3389, https://doi.org/10.5194/amt-9-3355-2016, https://doi.org/10.5194/amt-9-3355-2016, 2016
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We investigate the accuracy, precision and long-term stability of the MIPAS Envisat IMK/IAA CFC-11 (CCl3F) and CFC-12 (CCl2F2) products.
For comparisons we use several data products from satellite, airplane and balloon-borne instruments as well as ground-based data.
MIPAS Envisat CFC-11 has a slight high bias at the lower end of the profile.
CFC-12 agrees well with other data products.
The temporal stability is good up to ~ 30 km, but still leaves room for improvement.
Bernd Funke, Manuel López-Puertas, Gabriele P. Stiller, Stefan Versick, and Thomas von Clarmann
Atmos. Chem. Phys., 16, 8667–8693, https://doi.org/10.5194/acp-16-8667-2016, https://doi.org/10.5194/acp-16-8667-2016, 2016
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We present a semi-empirical model for the reconstruction of polar winter descent of reactive nitrogen (NOy) produced by energetic particle precipitation (EPP) into the stratosphere. It can be used to prescribe NOy in chemistry climate models with an upper lid below the EPP source region. We also found a significant reduction of the EPP-generated NOy during the last 30 years, likely affecting the long-term NOy trend by counteracting the expected increase caused by growing N2O emission.
Khalil Karami, Peter Braesicke, Miriam Sinnhuber, and Stefan Versick
Atmos. Chem. Phys., 16, 8447–8460, https://doi.org/10.5194/acp-16-8447-2016, https://doi.org/10.5194/acp-16-8447-2016, 2016
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We introduce a diagnostic tool to assess in a climatological framework the optimal propagation conditions for stationary planetary waves. Analyzing 50 winters using NCEP/NCAR reanalysis data we demonstrate several problematic features of the refractive index of Rossby waves. We introduced the Rossby waves membership value function to calculate the optimal propagation conditions for Rossby waves. Sensitivity of our diagnostic tool to strong and weak vortex regimes are examined.
Maya García-Comas, Manuel López-Puertas, Bernd Funke, Á. Aythami Jurado-Navarro, Angela Gardini, Gabriele P. Stiller, Thomas von Clarmann, and Michael Höpfner
Atmos. Chem. Phys., 16, 6701–6719, https://doi.org/10.5194/acp-16-6701-2016, https://doi.org/10.5194/acp-16-6701-2016, 2016
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We have analysed IR measurements of PMCs in the NH and SH from 2005 to 2012. This technique is sensitive to the total ice volume independent of particle size. For the first time, we have measured the total ice volume from the midlatitudes to the poles. The data indicate a layer of ice from 81 to 89 km and from the poles to 50–60º in each hemisphere, increasing near the poles. The ice density is larger in the NH than in the SH and located 1 km lower. PMCs also show a diurnal variation.
Simone Tilmes, Jean-Francois Lamarque, Louisa K. Emmons, Doug E. Kinnison, Dan Marsh, Rolando R. Garcia, Anne K. Smith, Ryan R. Neely, Andrew Conley, Francis Vitt, Maria Val Martin, Hiroshi Tanimoto, Isobel Simpson, Don R. Blake, and Nicola Blake
Geosci. Model Dev., 9, 1853–1890, https://doi.org/10.5194/gmd-9-1853-2016, https://doi.org/10.5194/gmd-9-1853-2016, 2016
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The state of the art Community Earth System Model, CESM1 CAM4-chem has been used to perform reference and sensitivity simulations as part of the Chemistry Climate Model Initiative (CCMI). Specifics of the model and details regarding the setup of the simulations are described. In additions, the main behavior of the model, including selected chemical species have been evaluated with climatological datasets. This paper is therefore a references for studies that use the provided model results.
Charles H. Jackman, Daniel R. Marsh, Douglas E. Kinnison, Christopher J. Mertens, and Eric L. Fleming
Atmos. Chem. Phys., 16, 5853–5866, https://doi.org/10.5194/acp-16-5853-2016, https://doi.org/10.5194/acp-16-5853-2016, 2016
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Two global models were used to investigate the impact of galactic cosmic ray (GCRs) on the atmosphere over the 1960-2010 time period. The primary impact of the naturally occurring GCRs on ozone was found to be due to their production of NOx and this impact varies with the atmospheric chlorine loading, sulfate aerosol loading, and solar cycle variation. GCR-caused decreases of annual average global total ozone were computed to be 0.2 % or less.
Sean Coburn, Barbara Dix, Eric Edgerton, Christopher D. Holmes, Douglas Kinnison, Qing Liang, Arnout ter Schure, Siyuan Wang, and Rainer Volkamer
Atmos. Chem. Phys., 16, 3743–3760, https://doi.org/10.5194/acp-16-3743-2016, https://doi.org/10.5194/acp-16-3743-2016, 2016
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Here we present a day of case study measurements of the vertical distribution of bromine monoxide over the coastal region of the Gulf of Mexico. These measurements are used to assess the contribution of bromine radicals to the oxidation of elemental mercury in the troposphere. We find that the measured levels of bromine in the troposphere are sufficient to quickly oxidize mercury, which has significant implications for our understanding of atmospheric mercury processes.
S. Tegtmeier, M. I. Hegglin, J. Anderson, B. Funke, J. Gille, A. Jones, L. Smith, T. von Clarmann, and K. A. Walker
Earth Syst. Sci. Data, 8, 61–78, https://doi.org/10.5194/essd-8-61-2016, https://doi.org/10.5194/essd-8-61-2016, 2016
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The first comprehensive intercomparison of CFC-11, CFC-12, HF, and SF6 satellite data was performed as part of the SPARC Data Initiative following a new "top-down" concept of satellite measurement validation and thus providing a global picture of the data characteristics. The comparisons will provide basic information on quality and consistency of the various data sets and will serve as a guide for their use in empirical studies of climate and variability, and in model-measurement comparisons.
M. P. Langowski, C. von Savigny, J. P. Burrows, V. V. Rozanov, T. Dunker, U.-P. Hoppe, M. Sinnhuber, and A. C. Aikin
Atmos. Meas. Tech., 9, 295–311, https://doi.org/10.5194/amt-9-295-2016, https://doi.org/10.5194/amt-9-295-2016, 2016
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An algorithm has been developed for the retrieval of sodium atom (Na) number density on a latitude and altitude grid from SCIAMACHY limb measurements of the Na resonance fluorescence (multiannual means 2008–2012). The Na layer peaks at 90 to 93 km altitude and has a FWHM of 5 to 15 km. A summer minimum in peak density and width is observed at high latitudes. At low latitudes, a semiannual oscillation is found. The results are compared with other measurements and models and agree well with these.
F. J. Haenel, G. P. Stiller, T. von Clarmann, B. Funke, E. Eckert, N. Glatthor, U. Grabowski, S. Kellmann, M. Kiefer, A. Linden, and T. Reddmann
Atmos. Chem. Phys., 15, 13161–13176, https://doi.org/10.5194/acp-15-13161-2015, https://doi.org/10.5194/acp-15-13161-2015, 2015
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Stratospheric circulation is thought to change as a consequence of climate change. Empirical evidence, however, is sparse. In this paper we present latitude- and altitude-resolved trends of the mean age of stratospheric air as derived from SF6 measurements performed by the MIPAS satellite instrument. The mean of the age of stratospheric air is a measure of the intensity of the Brewer-Dobson circulation. In this paper we discuss differences with respect to a preceding analysis by Stiller et al.
K. Karami, P. Braesicke, M. Kunze, U. Langematz, M. Sinnhuber, and S. Versick
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-15-33283-2015, https://doi.org/10.5194/acpd-15-33283-2015, 2015
Revised manuscript has not been submitted
S. Bender, M. Sinnhuber, T. von Clarmann, G. Stiller, B. Funke, M. López-Puertas, J. Urban, K. Pérot, K. A. Walker, and J. P. Burrows
Atmos. Meas. Tech., 8, 4171–4195, https://doi.org/10.5194/amt-8-4171-2015, https://doi.org/10.5194/amt-8-4171-2015, 2015
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We compare the nitric oxide (NO) daily zonal mean number density data sets in the mesosphere and lower thermosphere (MLT, 60km to 150km) from four instruments: ACE-FTS (2004--2010), MIPAS (2005--2012), SCIAMACHY (2008--2012), and SMR (2003--2012). We find that these data sets from different instruments consistently constrain NO in the MLT. Thus, they offer reliable forcing inputs for climate and chemistry climate models as an initial step to include solar and geomagnetic activity.
M. Gil-Ojeda, M. Navarro-Comas, L. Gómez-Martín, J. A. Adame, A. Saiz-Lopez, C. A. Cuevas, Y. González, O. Puentedura, E. Cuevas, J.-F. Lamarque, D. Kinninson, and S. Tilmes
Atmos. Chem. Phys., 15, 10567–10579, https://doi.org/10.5194/acp-15-10567-2015, https://doi.org/10.5194/acp-15-10567-2015, 2015
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The NO2 seasonal evolution in the free troposphere (FT) has been established for the first time, based on a remote sensing technique (MAXDOAS) and thus avoiding the problems of the local pollution of in situ instruments. A clear seasonality has been found, with background levels of 20-40pptv. Evidence has been found on fast, direct injection of surface air into the free troposphere. This result might have implications on the FT distribution of halogens and other species with marine sources.
C. McLandress, T. G. Shepherd, A. I. Jonsson, T. von Clarmann, and B. Funke
Atmos. Chem. Phys., 15, 9271–9284, https://doi.org/10.5194/acp-15-9271-2015, https://doi.org/10.5194/acp-15-9271-2015, 2015
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This is the first paper of its kind describing a method for merging the long-term satellite records of global stratospheric temperature from SSU and AMSU to yield a continuous data set from 1979 to present (and beyond). Since global-mean stratospheric temperature is close to radiative equilibrium, our "extended" SSU data set is an important climate record for the detection and attribution of anthropogenic influence.
M. Höpfner, C. D. Boone, B. Funke, N. Glatthor, U. Grabowski, A. Günther, S. Kellmann, M. Kiefer, A. Linden, S. Lossow, H. C. Pumphrey, W. G. Read, A. Roiger, G. Stiller, H. Schlager, T. von Clarmann, and K. Wissmüller
Atmos. Chem. Phys., 15, 7017–7037, https://doi.org/10.5194/acp-15-7017-2015, https://doi.org/10.5194/acp-15-7017-2015, 2015
S. Tilmes, J.-F. Lamarque, L. K. Emmons, D. E. Kinnison, P.-L. Ma, X. Liu, S. Ghan, C. Bardeen, S. Arnold, M. Deeter, F. Vitt, T. Ryerson, J. W. Elkins, F. Moore, J. R. Spackman, and M. Val Martin
Geosci. Model Dev., 8, 1395–1426, https://doi.org/10.5194/gmd-8-1395-2015, https://doi.org/10.5194/gmd-8-1395-2015, 2015
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The Community Atmosphere Model (CAM), version 5, is now coupled to extensive tropospheric and stratospheric chemistry, called CAM5-chem, and is available in addition to CAM4-chem in the Community Earth System Model (CESM) version 1.2. Both configurations are well suited as tools for atmospheric chemistry modeling studies in the troposphere and lower stratosphere.
T. Fytterer, M. G. Mlynczak, H. Nieder, K. Pérot, M. Sinnhuber, G. Stiller, and J. Urban
Atmos. Chem. Phys., 15, 3327–3338, https://doi.org/10.5194/acp-15-3327-2015, https://doi.org/10.5194/acp-15-3327-2015, 2015
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Energetic particles from the sun produce NOx (=N+NO+NO2) in the mesosphere/lower thermosphere. The NOx can be transported downward in the stratosphere during polar winter where NOx eventually depletes O3. This entire chain is the so-called energetic particle precipitation (EPP) indirect effect.
Here we show downward propagating negative stratospheric O3 anomalies during Antarctic polar winter. The O3 anomalies are caused by geomagnetic activity and show strong hints of the EPP indirect effect.
L. Millán, S. Wang, N. Livesey, D. Kinnison, H. Sagawa, and Y. Kasai
Atmos. Chem. Phys., 15, 2889–2902, https://doi.org/10.5194/acp-15-2889-2015, https://doi.org/10.5194/acp-15-2889-2015, 2015
P. Hess, D. Kinnison, and Q. Tang
Atmos. Chem. Phys., 15, 2341–2365, https://doi.org/10.5194/acp-15-2341-2015, https://doi.org/10.5194/acp-15-2341-2015, 2015
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Using a series of model simulations, we find that at widespread NH extratropical locations, interannual tropospheric ozone variability is largely determined by the transport of ozone from the stratosphere. This has implications in the interpretation of measured tropospheric ozone variability in light of changes in the emissions of ozone precursors and in the response of tropospheric ozone to climate change.
C. Prados-Roman, C. A. Cuevas, R. P. Fernandez, D. E. Kinnison, J-F. Lamarque, and A. Saiz-Lopez
Atmos. Chem. Phys., 15, 2215–2224, https://doi.org/10.5194/acp-15-2215-2015, https://doi.org/10.5194/acp-15-2215-2015, 2015
T. Sakazaki, M. Shiotani, M. Suzuki, D. Kinnison, J. M. Zawodny, M. McHugh, and K. A. Walker
Atmos. Chem. Phys., 15, 829–843, https://doi.org/10.5194/acp-15-829-2015, https://doi.org/10.5194/acp-15-829-2015, 2015
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The solar occultation measurements measure the atmosphere at sunrise (SR) and sunset (SS). It has been reported that there is a significant difference in the observed amount of stratospheric ozone between SR and SS. This study first revealed that this difference can be largely explained by diurnal variations in ozone, particularly those caused by vertical transport by the atmospheric tidal winds. Our results would be helpful for the construction of combined data sets from SR and SS profiles.
N. Glatthor, M. Höpfner, G. P. Stiller, T. von Clarmann, B. Funke, S. Lossow, E. Eckert, U. Grabowski, S. Kellmann, A. Linden, K. A. Walker, and A. Wiegele
Atmos. Chem. Phys., 15, 563–582, https://doi.org/10.5194/acp-15-563-2015, https://doi.org/10.5194/acp-15-563-2015, 2015
C. Prados-Roman, C. A. Cuevas, T. Hay, R. P. Fernandez, A. S. Mahajan, S.-J. Royer, M. Galí, R. Simó, J. Dachs, K. Großmann, D. E. Kinnison, J.-F. Lamarque, and A. Saiz-Lopez
Atmos. Chem. Phys., 15, 583–593, https://doi.org/10.5194/acp-15-583-2015, https://doi.org/10.5194/acp-15-583-2015, 2015
M. P. Langowski, C. von Savigny, J. P. Burrows, W. Feng, J. M. C. Plane, D. R. Marsh, D. Janches, M. Sinnhuber, A. C. Aikin, and P. Liebing
Atmos. Chem. Phys., 15, 273–295, https://doi.org/10.5194/acp-15-273-2015, https://doi.org/10.5194/acp-15-273-2015, 2015
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Global concentration fields of Mg and Mg+ in the Earth's upper mesosphere and lower thermosphere (70-150km) are presented. These are retrieved from SCIAMACHY/Envisat satellite grating spectrometer measurements in limb viewing geometry between 2008 and 2012.
These were compared with WACCM-Mg model results and a large fraction of the available measurement results for these species, and an interpretation of the results is done. The variation of these species during NLC presence is discussed.
R. P. Fernandez, R. J. Salawitch, D. E. Kinnison, J.-F. Lamarque, and A. Saiz-Lopez
Atmos. Chem. Phys., 14, 13391–13410, https://doi.org/10.5194/acp-14-13391-2014, https://doi.org/10.5194/acp-14-13391-2014, 2014
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We propose the existence of a daytime “tropical ring of atomic bromine” surrounding the tropics at a height between 15 and 19km. Our simulations show that VSL bromocarbons produce increases of 3pptv for inorganic bromine and 2pptv for organic bromine in the tropical TTL on an annual average, resulting in a total stratospheric bromine injection of 5pptv. This result suggests that the inorganic bromine injected into the stratosphere may be larger than that from VSL bromocarbons.
A. Saiz-Lopez, R. P. Fernandez, C. Ordóñez, D. E. Kinnison, J. C. Gómez Martín, J.-F. Lamarque, and S. Tilmes
Atmos. Chem. Phys., 14, 13119–13143, https://doi.org/10.5194/acp-14-13119-2014, https://doi.org/10.5194/acp-14-13119-2014, 2014
M. García-Comas, B. Funke, A. Gardini, M. López-Puertas, A. Jurado-Navarro, T. von Clarmann, G. Stiller, M. Kiefer, C. D. Boone, T. Leblanc, B. T. Marshall, M. J. Schwartz, and P. E. Sheese
Atmos. Meas. Tech., 7, 3633–3651, https://doi.org/10.5194/amt-7-3633-2014, https://doi.org/10.5194/amt-7-3633-2014, 2014
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We present the new vM21 MIPAS temperatures from 20 to 102km for all of its 2005-2012 MA, UA and NLC measurements. The main upgrades are the update of ESA L1b spectra, spectroscopic database and O and CO2 climatologies, and improvement in Tk-gradient and offset regularizations and apodization accuracy. The vM21 Tk's correct the main systematic errors of previous versions and lead to remarkable improvement in their comparisons with ACE-FTS, MLS, OSIRIS, SABER and SOFIE and the MLO and TMF lidars.
M. Sinnhuber, B. Funke, T. von Clarmann, M. Lopez-Puertas, G. P. Stiller, and A. Seppälä
Atmos. Chem. Phys., 14, 7681–7692, https://doi.org/10.5194/acp-14-7681-2014, https://doi.org/10.5194/acp-14-7681-2014, 2014
T. Wang, W. J. Randel, A. E. Dessler, M. R. Schoeberl, and D. E. Kinnison
Atmos. Chem. Phys., 14, 7135–7147, https://doi.org/10.5194/acp-14-7135-2014, https://doi.org/10.5194/acp-14-7135-2014, 2014
G. Chiodo, D. R. Marsh, R. Garcia-Herrera, N. Calvo, and J. A. García
Atmos. Chem. Phys., 14, 5251–5269, https://doi.org/10.5194/acp-14-5251-2014, https://doi.org/10.5194/acp-14-5251-2014, 2014
A. C. Kren, D. R. Marsh, A. K. Smith, and P. Pilewskie
Atmos. Chem. Phys., 14, 4843–4856, https://doi.org/10.5194/acp-14-4843-2014, https://doi.org/10.5194/acp-14-4843-2014, 2014
F. Friederich, M. Sinnhuber, B. Funke, T. von Clarmann, and J. Orphal
Atmos. Chem. Phys., 14, 4055–4064, https://doi.org/10.5194/acp-14-4055-2014, https://doi.org/10.5194/acp-14-4055-2014, 2014
C. H. Jackman, C. E. Randall, V. L. Harvey, S. Wang, E. L. Fleming, M. López-Puertas, B. Funke, and P. F. Bernath
Atmos. Chem. Phys., 14, 1025–1038, https://doi.org/10.5194/acp-14-1025-2014, https://doi.org/10.5194/acp-14-1025-2014, 2014
M. Langowski, M. Sinnhuber, A. C. Aikin, C. von Savigny, and J. P. Burrows
Atmos. Meas. Tech., 7, 29–48, https://doi.org/10.5194/amt-7-29-2014, https://doi.org/10.5194/amt-7-29-2014, 2014
M. Abalos, W. J. Randel, D. E. Kinnison, and E. Serrano
Atmos. Chem. Phys., 13, 10591–10607, https://doi.org/10.5194/acp-13-10591-2013, https://doi.org/10.5194/acp-13-10591-2013, 2013
M. Höpfner, N. Glatthor, U. Grabowski, S. Kellmann, M. Kiefer, A. Linden, J. Orphal, G. Stiller, T. von Clarmann, B. Funke, and C. D. Boone
Atmos. Chem. Phys., 13, 10405–10423, https://doi.org/10.5194/acp-13-10405-2013, https://doi.org/10.5194/acp-13-10405-2013, 2013
S. Bender, M. Sinnhuber, J. P. Burrows, M. Langowski, B. Funke, and M. López-Puertas
Atmos. Meas. Tech., 6, 2521–2531, https://doi.org/10.5194/amt-6-2521-2013, https://doi.org/10.5194/amt-6-2521-2013, 2013
I. A. Mironova and I. G. Usoskin
Atmos. Chem. Phys., 13, 8543–8550, https://doi.org/10.5194/acp-13-8543-2013, https://doi.org/10.5194/acp-13-8543-2013, 2013
I. Ermolli, K. Matthes, T. Dudok de Wit, N. A. Krivova, K. Tourpali, M. Weber, Y. C. Unruh, L. Gray, U. Langematz, P. Pilewskie, E. Rozanov, W. Schmutz, A. Shapiro, S. K. Solanki, and T. N. Woods
Atmos. Chem. Phys., 13, 3945–3977, https://doi.org/10.5194/acp-13-3945-2013, https://doi.org/10.5194/acp-13-3945-2013, 2013
F. Khosrawi, R. Müller, J. Urban, M. H. Proffitt, G. Stiller, M. Kiefer, S. Lossow, D. Kinnison, F. Olschewski, M. Riese, and D. Murtagh
Atmos. Chem. Phys., 13, 3619–3641, https://doi.org/10.5194/acp-13-3619-2013, https://doi.org/10.5194/acp-13-3619-2013, 2013
F. Friederich, T. von Clarmann, B. Funke, H. Nieder, J. Orphal, M. Sinnhuber, G. P. Stiller, and J. M. Wissing
Atmos. Chem. Phys., 13, 2531–2539, https://doi.org/10.5194/acp-13-2531-2013, https://doi.org/10.5194/acp-13-2531-2013, 2013
S. Kellmann, T. von Clarmann, G. P. Stiller, E. Eckert, N. Glatthor, M. Höpfner, M. Kiefer, J. Orphal, B. Funke, U. Grabowski, A. Linden, G. S. Dutton, and J. W. Elkins
Atmos. Chem. Phys., 12, 11857–11875, https://doi.org/10.5194/acp-12-11857-2012, https://doi.org/10.5194/acp-12-11857-2012, 2012
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Kangari Narender Reddy, Somnath Baidya Roy, Sam S. Rabin, Danica L. Lombardozzi, Gudimetla Venkateswara Varma, Ruchira Biswas, and Devavat Chiru Naik
Geosci. Model Dev., 18, 763–785, https://doi.org/10.5194/gmd-18-763-2025, https://doi.org/10.5194/gmd-18-763-2025, 2025
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The study aimed to improve the representation of wheat and rice in a land model for the Indian region. The modified model performed significantly better than the default model in simulating crop phenology, yield, and carbon, water, and energy fluxes compared to observations. The study highlights the need for global land models to use region-specific crop parameters for accurately simulating vegetation processes and land surface processes.
Giovanni Di Virgilio, Fei Ji, Eugene Tam, Jason P. Evans, Jatin Kala, Julia Andrys, Christopher Thomas, Dipayan Choudhury, Carlos Rocha, Yue Li, and Matthew L. Riley
Geosci. Model Dev., 18, 703–724, https://doi.org/10.5194/gmd-18-703-2025, https://doi.org/10.5194/gmd-18-703-2025, 2025
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We evaluate the skill in simulating the Australian climate of some of the latest generation of regional climate models. We show when and where the models simulate this climate with high skill versus model limitations. We show how new models perform relative to the previous-generation models, assessing how model design features may underlie key performance improvements. This work is of national and international relevance as it can help guide the use and interpretation of climate projections.
Giovanni Di Virgilio, Jason P. Evans, Fei Ji, Eugene Tam, Jatin Kala, Julia Andrys, Christopher Thomas, Dipayan Choudhury, Carlos Rocha, Stephen White, Yue Li, Moutassem El Rafei, Rishav Goyal, Matthew L. Riley, and Jyothi Lingala
Geosci. Model Dev., 18, 671–702, https://doi.org/10.5194/gmd-18-671-2025, https://doi.org/10.5194/gmd-18-671-2025, 2025
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We introduce new climate models that simulate Australia’s future climate at regional scales, including at an unprecedented resolution of 4 km for 1950–2100. We describe the model design process used to create these new climate models. We show how the new models perform relative to previous-generation models and compare their climate projections. This work is of national and international relevance as it can help guide climate model design and the use and interpretation of climate projections.
Jiawang Feng, Chun Zhao, Qiuyan Du, Zining Yang, and Chen Jin
Geosci. Model Dev., 18, 585–603, https://doi.org/10.5194/gmd-18-585-2025, https://doi.org/10.5194/gmd-18-585-2025, 2025
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In this study, we improved the calculation of how aerosols in the air interact with radiation in WRF-Chem. The original model used a simplified method, but we developed a more accurate approach. We found that this method significantly changes the properties of the estimated aerosols and their effects on radiation, especially for dust aerosols. It also impacts the simulated weather conditions. Our work highlights the importance of correctly representing aerosol–radiation interactions in models.
Eduardo Moreno-Chamarro, Thomas Arsouze, Mario Acosta, Pierre-Antoine Bretonnière, Miguel Castrillo, Eric Ferrer, Amanda Frigola, Daria Kuznetsova, Eneko Martin-Martinez, Pablo Ortega, and Sergi Palomas
Geosci. Model Dev., 18, 461–482, https://doi.org/10.5194/gmd-18-461-2025, https://doi.org/10.5194/gmd-18-461-2025, 2025
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We present the high-resolution model version of the EC-Earth global climate model to contribute to HighResMIP. The combined model resolution is about 10–15 km in both the ocean and atmosphere, which makes it one of the finest ever used to complete historical and scenario simulations. This model is compared with two lower-resolution versions, with a 100 km and a 25 km grid. The three models are compared with observations to study the improvements thanks to the increased resolution.
Catherine Guiavarc'h, David Storkey, Adam T. Blaker, Ed Blockley, Alex Megann, Helene Hewitt, Michael J. Bell, Daley Calvert, Dan Copsey, Bablu Sinha, Sophia Moreton, Pierre Mathiot, and Bo An
Geosci. Model Dev., 18, 377–403, https://doi.org/10.5194/gmd-18-377-2025, https://doi.org/10.5194/gmd-18-377-2025, 2025
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The Global Ocean and Sea Ice configuration version 9 (GOSI9) is the new UK hierarchy of model configurations based on the Nucleus for European Modelling of the Ocean (NEMO) and available at three resolutions. It will be used for various applications, e.g. weather forecasting and climate prediction. It improves upon the previous version by reducing global temperature and salinity biases and enhancing the representation of Arctic sea ice and the Antarctic Circumpolar Current.
Andy Richling, Jens Grieger, and Henning W. Rust
Geosci. Model Dev., 18, 361–375, https://doi.org/10.5194/gmd-18-361-2025, https://doi.org/10.5194/gmd-18-361-2025, 2025
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The performance of weather and climate prediction systems is variable in time and space. It is of interest how this performance varies in different situations. We provide a decomposition of a skill score (a measure of forecast performance) as a tool for detailed assessment of performance variability to support model development or forecast improvement. The framework is exemplified with decadal forecasts to assess the impact of different ocean states in the North Atlantic on temperature forecast.
Maria R. Russo, Sadie L. Bartholomew, David Hassell, Alex M. Mason, Erica Neininger, A. James Perman, David A. J. Sproson, Duncan Watson-Parris, and Nathan Luke Abraham
Geosci. Model Dev., 18, 181–191, https://doi.org/10.5194/gmd-18-181-2025, https://doi.org/10.5194/gmd-18-181-2025, 2025
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Observational data and modelling capabilities have expanded in recent years, but there are still barriers preventing these two data sources from being used in synergy. Proper comparison requires generating, storing, and handling a large amount of data. This work describes the first step in the development of a new set of software tools, the VISION toolkit, which can enable the easy and efficient integration of observational and model data required for model evaluation.
Bijan Fallah, Masoud Rostami, Emmanuele Russo, Paula Harder, Christoph Menz, Peter Hoffmann, Iulii Didovets, and Fred F. Hattermann
Geosci. Model Dev., 18, 161–180, https://doi.org/10.5194/gmd-18-161-2025, https://doi.org/10.5194/gmd-18-161-2025, 2025
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We tried to contribute to a local climate change impact study in central Asia, a region that is water-scarce and vulnerable to global climate change. We use regional models and machine learning to produce reliable local data from global climate models. We find that regional models show more realistic and detailed changes in heavy precipitation than global climate models. Our work can help assess the future risks of extreme events and plan adaptation strategies in central Asia.
Thomas Rackow, Xabier Pedruzo-Bagazgoitia, Tobias Becker, Sebastian Milinski, Irina Sandu, Razvan Aguridan, Peter Bechtold, Sebastian Beyer, Jean Bidlot, Souhail Boussetta, Willem Deconinck, Michail Diamantakis, Peter Dueben, Emanuel Dutra, Richard Forbes, Rohit Ghosh, Helge F. Goessling, Ioan Hadade, Jan Hegewald, Thomas Jung, Sarah Keeley, Lukas Kluft, Nikolay Koldunov, Aleksei Koldunov, Tobias Kölling, Josh Kousal, Christian Kühnlein, Pedro Maciel, Kristian Mogensen, Tiago Quintino, Inna Polichtchouk, Balthasar Reuter, Domokos Sármány, Patrick Scholz, Dmitry Sidorenko, Jan Streffing, Birgit Sützl, Daisuke Takasuka, Steffen Tietsche, Mirco Valentini, Benoît Vannière, Nils Wedi, Lorenzo Zampieri, and Florian Ziemen
Geosci. Model Dev., 18, 33–69, https://doi.org/10.5194/gmd-18-33-2025, https://doi.org/10.5194/gmd-18-33-2025, 2025
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Detailed global climate model simulations have been created based on a numerical weather prediction model, offering more accurate spatial detail down to the scale of individual cities ("kilometre-scale") and a better understanding of climate phenomena such as atmospheric storms, whirls in the ocean, and cracks in sea ice. The new model aims to provide globally consistent information on local climate change with greater precision, benefiting environmental planning and local impact modelling.
Yilin Fang, Hoang Viet Tran, and L. Ruby Leung
Geosci. Model Dev., 18, 19–32, https://doi.org/10.5194/gmd-18-19-2025, https://doi.org/10.5194/gmd-18-19-2025, 2025
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Hurricanes may worsen water quality in the lower Mississippi River basin (LMRB) by increasing nutrient runoff. We found that runoff parameterizations greatly affect nitrate–nitrogen runoff simulated using an Earth system land model. Our simulations predicted increased nitrogen runoff in the LMRB during Hurricane Ida in 2021, albeit less pronounced than the observations, indicating areas for model improvement to better understand and manage nutrient runoff loss during hurricanes in the region.
Giovanni Seijo-Ellis, Donata Giglio, Gustavo Marques, and Frank Bryan
Geosci. Model Dev., 17, 8989–9021, https://doi.org/10.5194/gmd-17-8989-2024, https://doi.org/10.5194/gmd-17-8989-2024, 2024
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A CESM–MOM6 regional configuration of the Caribbean Sea was developed in response to the rising need for high-resolution models for climate impact studies. The configuration is validated for the period 2000–2020 and improves significant errors in a low-resolution model. Oceanic properties are well represented. Patterns of freshwater associated with the Amazon River are well captured, and the mean flows of ocean waters across multiple passages in the Caribbean Sea agree with observations.
Deifilia To, Julian Quinting, Gholam Ali Hoshyaripour, Markus Götz, Achim Streit, and Charlotte Debus
Geosci. Model Dev., 17, 8873–8884, https://doi.org/10.5194/gmd-17-8873-2024, https://doi.org/10.5194/gmd-17-8873-2024, 2024
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Pangu-Weather is a breakthrough machine learning model in medium-range weather forecasting that considers 3D atmospheric information. We show that using a simpler 2D framework improves robustness, speeds up training, and reduces computational needs by 20 %–30 %. We introduce a training procedure that varies the importance of atmospheric variables over time to speed up training convergence. Decreasing computational demand increases the accessibility of training and working with the model.
Fang Li, Xiang Song, Sandy P. Harrison, Jennifer R. Marlon, Zhongda Lin, L. Ruby Leung, Jörg Schwinger, Virginie Marécal, Shiyu Wang, Daniel S. Ward, Xiao Dong, Hanna Lee, Lars Nieradzik, Sam S. Rabin, and Roland Séférian
Geosci. Model Dev., 17, 8751–8771, https://doi.org/10.5194/gmd-17-8751-2024, https://doi.org/10.5194/gmd-17-8751-2024, 2024
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This study provides the first comprehensive assessment of historical fire simulations from 19 Earth system models in phase 6 of the Coupled Model Intercomparison Project (CMIP6). Most models reproduce global totals, spatial patterns, seasonality, and regional historical changes well but fail to simulate the recent decline in global burned area and underestimate the fire response to climate variability. CMIP6 simulations address three critical issues of phase-5 models.
Seung H. Baek, Paul A. Ullrich, Bo Dong, and Jiwoo Lee
Geosci. Model Dev., 17, 8665–8681, https://doi.org/10.5194/gmd-17-8665-2024, https://doi.org/10.5194/gmd-17-8665-2024, 2024
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We evaluate downscaled products by examining locally relevant co-variances during precipitation events. Common statistical downscaling techniques preserve expected co-variances during convective precipitation (a stationary phenomenon). However, they dampen future intensification of frontal precipitation (a non-stationary phenomenon) captured in global climate models and dynamical downscaling. Our study quantifies a ramification of the stationarity assumption underlying statistical downscaling.
Emmanuel Nyenah, Petra Döll, Daniel S. Katz, and Robert Reinecke
Geosci. Model Dev., 17, 8593–8611, https://doi.org/10.5194/gmd-17-8593-2024, https://doi.org/10.5194/gmd-17-8593-2024, 2024
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Research software is vital for scientific progress but is often developed by scientists with limited skills, time, and funding, leading to challenges in usability and maintenance. Our study across 10 sectors shows strengths in version control, open-source licensing, and documentation while emphasizing the need for containerization and code quality. We recommend workshops; code quality metrics; funding; and following the findable, accessible, interoperable, and reusable (FAIR) standards.
Chris Smith, Donald P. Cummins, Hege-Beate Fredriksen, Zebedee Nicholls, Malte Meinshausen, Myles Allen, Stuart Jenkins, Nicholas Leach, Camilla Mathison, and Antti-Ilari Partanen
Geosci. Model Dev., 17, 8569–8592, https://doi.org/10.5194/gmd-17-8569-2024, https://doi.org/10.5194/gmd-17-8569-2024, 2024
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Climate projections are only useful if the underlying models that produce them are well calibrated and can reproduce observed climate change. We formalise a software package that calibrates the open-source FaIR simple climate model to full-complexity Earth system models. Observations, including historical warming, and assessments of key climate variables such as that of climate sensitivity are used to constrain the model output.
Jingwei Xie, Xi Wang, Hailong Liu, Pengfei Lin, Jiangfeng Yu, Zipeng Yu, Junlin Wei, and Xiang Han
Geosci. Model Dev., 17, 8469–8493, https://doi.org/10.5194/gmd-17-8469-2024, https://doi.org/10.5194/gmd-17-8469-2024, 2024
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We propose the concept of mesoscale ocean direct numerical simulation (MODNS), which should resolve the first baroclinic deformation radius and ensure the numerical dissipative effects do not directly contaminate the mesoscale motions. It can be a benchmark for testing mesoscale ocean large eddy simulation (MOLES) methods in ocean models. We build an idealized Southern Ocean model using MITgcm to generate a type of MODNS. We also illustrate the diversity of multiscale eddy interactions.
Emily Black, John Ellis, and Ross I. Maidment
Geosci. Model Dev., 17, 8353–8372, https://doi.org/10.5194/gmd-17-8353-2024, https://doi.org/10.5194/gmd-17-8353-2024, 2024
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We present General TAMSAT-ALERT, a computationally lightweight and versatile tool for generating ensemble forecasts from time series data. General TAMSAT-ALERT is capable of combining multiple streams of monitoring and meteorological forecasting data into probabilistic hazard assessments. In this way, it complements existing systems and enhances their utility for actionable hazard assessment.
Sarah Schöngart, Lukas Gudmundsson, Mathias Hauser, Peter Pfleiderer, Quentin Lejeune, Shruti Nath, Sonia Isabelle Seneviratne, and Carl-Friedrich Schleussner
Geosci. Model Dev., 17, 8283–8320, https://doi.org/10.5194/gmd-17-8283-2024, https://doi.org/10.5194/gmd-17-8283-2024, 2024
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Precipitation and temperature are two of the most impact-relevant climatic variables. Yet, projecting future precipitation and temperature data under different emission scenarios relies on complex models that are computationally expensive. In this study, we propose a method that allows us to generate monthly means of local precipitation and temperature at low computational costs. Our modelling framework is particularly useful for all downstream applications of climate model data.
Gang Tang, Zebedee Nicholls, Chris Jones, Thomas Gasser, Alexander Norton, Tilo Ziehn, Alejandro Romero-Prieto, and Malte Meinshausen
EGUsphere, https://doi.org/10.5194/egusphere-2024-3522, https://doi.org/10.5194/egusphere-2024-3522, 2024
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We analyzed carbon and nitrogen mass conservation in data from CMIP6 Earth System Models. Our findings reveal significant discrepancies between flux and pool size data, particularly in nitrogen, where cumulative imbalances can reach hundreds of gigatons. These imbalances appear primarily due to missing or inconsistently reported fluxes – especially for land use and fire emissions. To enhance data quality, we recommend that future climate data protocols address this issue at the reporting stage.
Benjamin M. Sanderson, Ben B. B. Booth, John Dunne, Veronika Eyring, Rosie A. Fisher, Pierre Friedlingstein, Matthew J. Gidden, Tomohiro Hajima, Chris D. Jones, Colin G. Jones, Andrew King, Charles D. Koven, David M. Lawrence, Jason Lowe, Nadine Mengis, Glen P. Peters, Joeri Rogelj, Chris Smith, Abigail C. Snyder, Isla R. Simpson, Abigail L. S. Swann, Claudia Tebaldi, Tatiana Ilyina, Carl-Friedrich Schleussner, Roland Séférian, Bjørn H. Samset, Detlef van Vuuren, and Sönke Zaehle
Geosci. Model Dev., 17, 8141–8172, https://doi.org/10.5194/gmd-17-8141-2024, https://doi.org/10.5194/gmd-17-8141-2024, 2024
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We discuss how, in order to provide more relevant guidance for climate policy, coordinated climate experiments should adopt a greater focus on simulations where Earth system models are provided with carbon emissions from fossil fuels together with land use change instructions, rather than past approaches that have largely focused on experiments with prescribed atmospheric carbon dioxide concentrations. We discuss how these goals might be achieved in coordinated climate modeling experiments.
Peter Berg, Thomas Bosshard, Denica Bozhinova, Lars Bärring, Joakim Löw, Carolina Nilsson, Gustav Strandberg, Johan Södling, Johan Thuresson, Renate Wilcke, and Wei Yang
Geosci. Model Dev., 17, 8173–8179, https://doi.org/10.5194/gmd-17-8173-2024, https://doi.org/10.5194/gmd-17-8173-2024, 2024
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When bias adjusting climate model data using quantile mapping, one needs to prescribe what to do at the tails of the distribution, where a larger data range is likely encountered outside of the calibration period. The end result is highly dependent on the method used. We show that, to avoid discontinuities in the time series, one needs to exclude data in the calibration range to also activate the extrapolation functionality in that time period.
Philip J. Rasch, Haruki Hirasawa, Mingxuan Wu, Sarah J. Doherty, Robert Wood, Hailong Wang, Andy Jones, James Haywood, and Hansi Singh
Geosci. Model Dev., 17, 7963–7994, https://doi.org/10.5194/gmd-17-7963-2024, https://doi.org/10.5194/gmd-17-7963-2024, 2024
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We introduce a protocol to compare computer climate simulations to better understand a proposed strategy intended to counter warming and climate impacts from greenhouse gas increases. This slightly changes clouds in six ocean regions to reflect more sunlight and cool the Earth. Example changes in clouds and climate are shown for three climate models. Cloud changes differ between the models, but precipitation and surface temperature changes are similar when their cooling effects are made similar.
Trude Eidhammer, Andrew Gettelman, Katherine Thayer-Calder, Duncan Watson-Parris, Gregory Elsaesser, Hugh Morrison, Marcus van Lier-Walqui, Ci Song, and Daniel McCoy
Geosci. Model Dev., 17, 7835–7853, https://doi.org/10.5194/gmd-17-7835-2024, https://doi.org/10.5194/gmd-17-7835-2024, 2024
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We describe a dataset where 45 parameters related to cloud processes in the Community Earth System Model version 2 (CESM2) Community Atmosphere Model version 6 (CAM6) are perturbed. Three sets of perturbed parameter ensembles (263 members) were created: current climate, preindustrial aerosol loading and future climate with sea surface temperature increased by 4 K.
Ha Thi Minh Ho-Hagemann, Vera Maurer, Stefan Poll, and Irina Fast
Geosci. Model Dev., 17, 7815–7834, https://doi.org/10.5194/gmd-17-7815-2024, https://doi.org/10.5194/gmd-17-7815-2024, 2024
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The regional Earth system model GCOAST-AHOI v2.0 that includes the regional climate model ICON-CLM coupled to the ocean model NEMO and the hydrological discharge model HD via the OASIS3-MCT coupler can be a useful tool for conducting long-term regional climate simulations over the EURO-CORDEX domain. The new OASIS3-MCT coupling interface implemented in ICON-CLM makes it more flexible for coupling to an external ocean model and an external hydrological discharge model.
Sandro Vattioni, Rahel Weber, Aryeh Feinberg, Andrea Stenke, John A. Dykema, Beiping Luo, Georgios A. Kelesidis, Christian A. Bruun, Timofei Sukhodolov, Frank N. Keutsch, Thomas Peter, and Gabriel Chiodo
Geosci. Model Dev., 17, 7767–7793, https://doi.org/10.5194/gmd-17-7767-2024, https://doi.org/10.5194/gmd-17-7767-2024, 2024
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We quantified impacts and efficiency of stratospheric solar climate intervention via solid particle injection. Microphysical interactions of solid particles with the sulfur cycle were interactively coupled to the heterogeneous chemistry scheme and the radiative transfer code of an aerosol–chemistry–climate model. Compared to injection of SO2 we only find a stronger cooling efficiency for solid particles when normalizing to the aerosol load but not when normalizing to the injection rate.
Ingo Richter, Ping Chang, Gokhan Danabasoglu, Dietmar Dommenget, Guillaume Gastineau, Aixue Hu, Takahito Kataoka, Noel Keenlyside, Fred Kucharski, Yuko Okumura, Wonsun Park, Malte Stuecker, Andrea Taschetto, Chunzai Wang, Stephen Yeager, and Sang-Wook Yeh
EGUsphere, https://doi.org/10.5194/egusphere-2024-3110, https://doi.org/10.5194/egusphere-2024-3110, 2024
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The tropical ocean basins influence each other through multiple pathways and mechanisms, here referred to as tropical basin interaction (TBI). Many researchers have examined TBI using comprehensive climate models, but have obtained conflicting results. This may be partly due to differences in experiment protocols, and partly due to systematic model errors. TBIMIP aims to address this problem by designing a set of TBI experiments that will be performed by multiple models.
Samuel Rémy, Swen Metzger, Vincent Huijnen, Jason E. Williams, and Johannes Flemming
Geosci. Model Dev., 17, 7539–7567, https://doi.org/10.5194/gmd-17-7539-2024, https://doi.org/10.5194/gmd-17-7539-2024, 2024
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In this paper we describe the development of the future operational cycle 49R1 of the IFS-COMPO system, used for operational forecasts of atmospheric composition in the CAMS project, and focus on the implementation of the thermodynamical model EQSAM4Clim version 12. The implementation of EQSAM4Clim significantly improves the simulated secondary inorganic aerosol surface concentration. The new aerosol and precipitation acidity diagnostics showed good agreement against observational datasets.
Maximillian Van Wyk de Vries, Tom Matthews, L. Baker Perry, Nirakar Thapa, and Rob Wilby
Geosci. Model Dev., 17, 7629–7643, https://doi.org/10.5194/gmd-17-7629-2024, https://doi.org/10.5194/gmd-17-7629-2024, 2024
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This paper introduces the AtsMOS workflow, a new tool for improving weather forecasts in mountainous areas. By combining advanced statistical techniques with local weather data, AtsMOS can provide more accurate predictions of weather conditions. Using data from Mount Everest as an example, AtsMOS has shown promise in better forecasting hazardous weather conditions, making it a valuable tool for communities in mountainous regions and beyond.
Sofia Allende, Anne Marie Treguier, Camille Lique, Clément de Boyer Montégut, François Massonnet, Thierry Fichefet, and Antoine Barthélemy
Geosci. Model Dev., 17, 7445–7466, https://doi.org/10.5194/gmd-17-7445-2024, https://doi.org/10.5194/gmd-17-7445-2024, 2024
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We study the parameters of the turbulent-kinetic-energy mixed-layer-penetration scheme in the NEMO model with regard to sea-ice-covered regions of the Arctic Ocean. This evaluation reveals the impact of these parameters on mixed-layer depth, sea surface temperature and salinity, and ocean stratification. Our findings demonstrate significant impacts on sea ice thickness and sea ice concentration, emphasizing the need for accurately representing ocean mixing to understand Arctic climate dynamics.
Sabin I. Taranu, David M. Lawrence, Yoshihide Wada, Ting Tang, Erik Kluzek, Sam Rabin, Yi Yao, Steven J. De Hertog, Inne Vanderkelen, and Wim Thiery
Geosci. Model Dev., 17, 7365–7399, https://doi.org/10.5194/gmd-17-7365-2024, https://doi.org/10.5194/gmd-17-7365-2024, 2024
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In this study, we improved a climate model by adding the representation of water use sectors such as domestic, industry, and agriculture. This new feature helps us understand how water is used and supplied in various areas. We tested our model from 1971 to 2010 and found that it accurately identifies areas with water scarcity. By modelling the competition between sectors when water availability is limited, the model helps estimate the intensity and extent of individual sectors' water shortages.
Florian Börgel, Sven Karsten, Karoline Rummel, and Ulf Gräwe
EGUsphere, https://doi.org/10.5194/egusphere-2024-2685, https://doi.org/10.5194/egusphere-2024-2685, 2024
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Forecasting river runoff, crucial for managing water resources and understanding climate impacts, can be challenging. This study introduces a new method using Convolutional Long Short-Term Memory (ConvLSTM) networks, a machine learning model that processes spatial and temporal data. Focusing on the Baltic Sea region, our model uses weather data as input to predict daily river runoff for 97 rivers.
Thi Nhu Ngoc Do, Kengo Sudo, Akihiko Ito, Louisa Emmons, Vaishali Naik, Kostas Tsigaridis, Øyvind Seland, Gerd A. Folberth, and Douglas I. Kelley
EGUsphere, https://doi.org/10.5194/egusphere-2024-2313, https://doi.org/10.5194/egusphere-2024-2313, 2024
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Understanding historical isoprene emission changes is important for predicting future climate, but trends and their controlling factors remain uncertain. This study shows that long-term isoprene trends vary among Earth System Models mainly due to partially incorporating CO2 effects and land cover changes rather than climate. Future models that refine these factors’ effects on isoprene emissions, along with long-term observations, are essential for better understanding plant-climate interactions.
Michael Nole, Jonah Bartrand, Fawz Naim, and Glenn Hammond
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-162, https://doi.org/10.5194/gmd-2024-162, 2024
Revised manuscript accepted for GMD
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Safe carbon dioxide (CO2) storage is likely to be critical for mitigating some of the most dangerous effects of climate change. We present a simulation framework for modeling CO2 storage beneath the seafloor where CO2 can form a solid. This can aid in permanent CO2 storage for long periods of time. Our models show what a commercial-scale CO2 injection would look like in a marine environment. We discuss what would need to be considered when designing a sub-sea CO2 injection.
Cynthia Whaley, Montana Etten-Bohm, Courtney Schumacher, Ayodeji Akingunola, Vivek Arora, Jason Cole, Michael Lazare, David Plummer, Knut von Salzen, and Barbara Winter
Geosci. Model Dev., 17, 7141–7155, https://doi.org/10.5194/gmd-17-7141-2024, https://doi.org/10.5194/gmd-17-7141-2024, 2024
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This paper describes how lightning was added as a process in the Canadian Earth System Model in order to interactively respond to climate changes. As lightning is an important cause of global wildfires, this new model development allows for more realistic projections of how wildfires may change in the future, responding to a changing climate.
Erik Gustafsson, Bo G. Gustafsson, Martijn Hermans, Christoph Humborg, and Christian Stranne
Geosci. Model Dev., 17, 7157–7179, https://doi.org/10.5194/gmd-17-7157-2024, https://doi.org/10.5194/gmd-17-7157-2024, 2024
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Methane (CH4) cycling in the Baltic Proper is studied through model simulations, enabling a first estimate of key CH4 fluxes. A preliminary budget identifies benthic CH4 release as the dominant source and two main sinks: CH4 oxidation in the water (92 % of sinks) and outgassing to the atmosphere (8 % of sinks). This study addresses CH4 emissions from coastal seas and is a first step toward understanding the relative importance of open-water outgassing compared with local coastal hotspots.
Daniel Ries, Katherine Goode, Kellie McClernon, and Benjamin Hillman
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-133, https://doi.org/10.5194/gmd-2024-133, 2024
Revised manuscript accepted for GMD
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Machine learning has advanced research in the climate science domain, but its models are difficult to understand. In order to understand the impacts and consequences of climate interventions such as stratospheric aerosol injection, complex models are often necessary. We use a case study to illustrate how we can understand the inner workings of a complex model. We present this technique as an exploratory tool that can be used to quickly discover and assess relationships in complex climate data.
Florian Zabel, Matthias Knüttel, and Benjamin Poschlod
EGUsphere, https://doi.org/10.5194/egusphere-2024-2526, https://doi.org/10.5194/egusphere-2024-2526, 2024
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CropSuite is a fuzzy-logic based high resolution open-source crop suitability model considering the impact of climate variability. We apply CropSuite for 48 important staple and cash crops at 1 km spatial resolution for Africa. We find that climate variability significantly impacts on suitable areas, but also affects optimal sowing dates, and multiple cropping potentials. The results provide information that can be used for climate impact assessments, adaptation and land-use planning.
Kerstin Hartung, Bastian Kern, Nils-Arne Dreier, Jörn Geisbüsch, Mahnoosh Haghighatnasab, Patrick Jöckel, Astrid Kerkweg, Wilton Jaciel Loch, Florian Prill, and Daniel Rieger
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-135, https://doi.org/10.5194/gmd-2024-135, 2024
Revised manuscript accepted for GMD
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The Icosahedral Nonhydrostatic (ICON) Model Community Interface (ComIn) library supports connecting third-party modules to the ICON model. Third-party modules can range from simple diagnostic Python scripts to full chemistry models. ComIn offers a low barrier for code extensions to ICON, provides multi-language support (Fortran, C/C++ and Python) and reduces the migration effort in response to new ICON releases. This paper presents the ComIn design principles and a range of use cases.
Tridib Banerjee, Patrick Scholz, Sergey Danilov, Knut Klingbeil, and Dmitry Sidorenko
Geosci. Model Dev., 17, 7051–7065, https://doi.org/10.5194/gmd-17-7051-2024, https://doi.org/10.5194/gmd-17-7051-2024, 2024
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In this paper we propose a new alternative to one of the functionalities of the sea ice model FESOM2. The alternative we propose allows the model to capture and simulate fast changes in quantities like sea surface elevation more accurately. We also demonstrate that the new alternative is faster and more adept at taking advantages of highly parallelized computing infrastructure. We therefore show that this new alternative is a great addition to the sea ice model FESOM2.
Yuwen Fan, Zhao Yang, Min-Hui Lo, Jina Hur, and Eun-Soon Im
Geosci. Model Dev., 17, 6929–6947, https://doi.org/10.5194/gmd-17-6929-2024, https://doi.org/10.5194/gmd-17-6929-2024, 2024
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Irrigated agriculture in the North China Plain (NCP) has a significant impact on the local climate. To better understand this impact, we developed a specialized model specifically for the NCP region. This model allows us to simulate the double-cropping vegetation and the dynamic irrigation practices that are commonly employed in the NCP. This model shows improved performance in capturing the general crop growth, such as crop stages, biomass, crop yield, and vegetation greenness.
Gang Tang, Zebedee Nicholls, Alexander Norton, Sönke Zaehle, and Malte Meinshausen
EGUsphere, https://doi.org/10.5194/egusphere-2024-1941, https://doi.org/10.5194/egusphere-2024-1941, 2024
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We studied the coupled carbon-nitrogen cycle effect in Earth System Models by developing a carbon-nitrogen coupling in a reduced complexity model, MAGICC. Our model successfully emulated the global carbon-nitrogen cycle dynamics seen in CMIP6 complex models. Results indicate consistent nitrogen limitations on plant growth (net primary production) from 1850 to 2100. Our findings suggest that nitrogen deficiency could reduce future land carbon sequestration.
Ed Blockley, Emma Fiedler, Jeff Ridley, Luke Roberts, Alex West, Dan Copsey, Daniel Feltham, Tim Graham, David Livings, Clement Rousset, David Schroeder, and Martin Vancoppenolle
Geosci. Model Dev., 17, 6799–6817, https://doi.org/10.5194/gmd-17-6799-2024, https://doi.org/10.5194/gmd-17-6799-2024, 2024
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This paper documents the sea ice model component of the latest Met Office coupled model configuration, which will be used as the physical basis for UK contributions to CMIP7. Documentation of science options used in the configuration are given along with a brief model evaluation. This is the first UK configuration to use NEMO’s new SI3 sea ice model. We provide details on how SI3 was adapted to work with Met Office coupling methodology and documentation of coupling processes in the model.
Jean-François Lemieux, William H. Lipscomb, Anthony Craig, David A. Bailey, Elizabeth C. Hunke, Philippe Blain, Till A. S. Rasmussen, Mats Bentsen, Frédéric Dupont, David Hebert, and Richard Allard
Geosci. Model Dev., 17, 6703–6724, https://doi.org/10.5194/gmd-17-6703-2024, https://doi.org/10.5194/gmd-17-6703-2024, 2024
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We present the latest version of the CICE model. It solves equations that describe the dynamics and the growth and melt of sea ice. To do so, the domain is divided into grid cells and variables are positioned at specific locations in the cells. A new implementation (C-grid) is presented, with the velocity located on cell edges. Compared to the previous B-grid, the C-grid allows for a natural coupling with some oceanic and atmospheric models. It also allows for ice transport in narrow channels.
Rachid El Montassir, Olivier Pannekoucke, and Corentin Lapeyre
Geosci. Model Dev., 17, 6657–6681, https://doi.org/10.5194/gmd-17-6657-2024, https://doi.org/10.5194/gmd-17-6657-2024, 2024
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This study introduces a novel approach that combines physics and artificial intelligence (AI) for improved cloud cover forecasting. This approach outperforms traditional deep learning (DL) methods in producing realistic and physically consistent results while requiring less training data. This architecture provides a promising solution to overcome the limitations of classical AI methods and contributes to open up new possibilities for combining physical knowledge with deep learning models.
Marit Sandstad, Borgar Aamaas, Ane Nordlie Johansen, Marianne Tronstad Lund, Glen Philip Peters, Bjørn Hallvard Samset, Benjamin Mark Sanderson, and Ragnhild Bieltvedt Skeie
Geosci. Model Dev., 17, 6589–6625, https://doi.org/10.5194/gmd-17-6589-2024, https://doi.org/10.5194/gmd-17-6589-2024, 2024
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The CICERO-SCM has existed as a Fortran model since 1999 that calculates the radiative forcing and concentrations from emissions and is an upwelling diffusion energy balance model of the ocean that calculates temperature change. In this paper, we describe an updated version ported to Python and publicly available at https://github.com/ciceroOslo/ciceroscm (https://doi.org/10.5281/zenodo.10548720). This version contains functionality for parallel runs and automatic calibration.
Sébastien Masson, Swen Jullien, Eric Maisonnave, David Gill, Guillaume Samson, Mathieu Le Corre, and Lionel Renault
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-140, https://doi.org/10.5194/gmd-2024-140, 2024
Revised manuscript accepted for GMD
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This article details a new feature we implemented in the most popular regional atmospheric model (WRF). This feature allows data to be exchanged between WRF and any other model (e.g. an ocean model) using the coupling library Ocean-Atmosphere-Sea-Ice-Soil – Model Coupling Toolkit (OASIS3-MCT). This coupling interface is designed to be non-intrusive, flexible and modular. It also offers the possibility of taking into account the nested zooms used in WRF or in the models with which it is coupled.
Jordi Buckley Paules, Simone Fatichi, Bonnie Warring, and Athanasios Paschalis
EGUsphere, https://doi.org/10.5194/egusphere-2024-2072, https://doi.org/10.5194/egusphere-2024-2072, 2024
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We outline and validate developments to the pre-existing process-based model T&C to better represent cropland processes. Foreseen applications of T&C-CROP include hydrological and carbon storage implications of land-use transitions involving crop, forest, and pasture conversion, as well as studies on optimal irrigation and fertilization under a changing climate.
Zheng Xiang, Yongkang Xue, Weidong Guo, Melannie D. Hartman, Ye Liu, and William J. Parton
Geosci. Model Dev., 17, 6437–6464, https://doi.org/10.5194/gmd-17-6437-2024, https://doi.org/10.5194/gmd-17-6437-2024, 2024
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A process-based plant carbon (C)–nitrogen (N) interface coupling framework has been developed which mainly focuses on plant resistance and N-limitation effects on photosynthesis, plant respiration, and plant phenology. A dynamic C / N ratio is introduced to represent plant resistance and self-adjustment. The framework has been implemented in a coupled biophysical-ecosystem–biogeochemical model, and testing results show a general improvement in simulating plant properties with this framework.
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Executive editor
This manuscript is a timely publication necessary for preparations for CMIP7, given the importance of solar forcing to the climate system. It encourages community discussion, which will certainly be ongoing for the next several years.
This manuscript is a timely publication necessary for preparations for CMIP7, given the...
Short summary
We outline a road map for the preparation of a solar forcing dataset for the upcoming Phase 7 of the Coupled Model Intercomparison Project (CMIP7), considering the latest scientific advances made in the reconstruction of solar forcing and in the understanding of climate response while also addressing the issues that were raised during CMIP6.
We outline a road map for the preparation of a solar forcing dataset for the upcoming Phase 7 of...
