Treatment of non-ideality in the SPACCIM multiphase model – Part 1: Model  development

Rusumdar, A. J.; Wolke, R.; Tilgner, A.; Herrmann, H.

doi:https://doi.org/10.5194/gmd-9-247-2016

Articles | Volume 9, issue 1

https://doi.org/10.5194/gmd-9-247-2016

© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

https://doi.org/10.5194/gmd-9-247-2016

© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Articles | Volume 9, issue 1

Development and technical paper

|

25 Jan 2016

Development and technical paper |

| 25 Jan 2016

Treatment of non-ideality in the SPACCIM multiphase model – Part 1: Model development

A. J. Rusumdar, R. Wolke, A. Tilgner, and H. Herrmann

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Final revised paper (published on 25 Jan 2016)
Preprint (discussion started on 01 Jun 2015)

Interactive discussion

Status: closed

AC: Author comment | RC: Referee comment | SC: Short comment | EC: Editor comment

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- Supplement

RC C1311: 'Review of Rusumdar et al', Anonymous Referee #1, 06 Jul 2015
RC C1425: 'Review of Rusumdar et al', Anonymous Referee #2, 21 Jul 2015
- AC C2494: 'Authors' response to Referee #2', Ralf Wolke, 15 Oct 2015
AC C2493: 'Authors' response to Referee #1', Ralf Wolke, 15 Oct 2015

Peer-review completion

AR: Author's response | RR: Referee report | ED: Editor decision

AR by Ralf Wolke on behalf of the Authors (15 Oct 2015) Author's response Manuscript

ED: Referee Nomination & Report Request started (02 Nov 2015) by Andrea Stenke

RR by Anonymous Referee #1 (26 Nov 2015)

ED: Publish as is (11 Dec 2015) by Andrea Stenke

AR by Ralf Wolke on behalf of the Authors (16 Dec 2015)

Short summary

The present paper was aimed at the further development of SPACCIM to treat both complex multiphase chemistry and phase transfer processes considering new non-ideality properties of concentrated solutions. Model studies showed the applicability of the new kinetic model approach for complex aerosol mixtures and detailed chemical mechanisms. Simulations have implied that the treatment of non-ideality should be mandatory for modeling multiphase chemical processes in deliquesced particles.