Articles | Volume 17, issue 21 
            
                
                    
            
            
            https://doi.org/10.5194/gmd-17-7767-2024
                    © Author(s) 2024. This work is distributed under 
the Creative Commons Attribution 4.0 License.
                the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/gmd-17-7767-2024
                    © Author(s) 2024. This work is distributed under 
the Creative Commons Attribution 4.0 License.
                the Creative Commons Attribution 4.0 License.
A fully coupled solid-particle microphysics scheme for stratospheric aerosol injections within the aerosol–chemistry–climate model SOCOL-AERv2
Sandro Vattioni
CORRESPONDING AUTHOR
                                            
                                    
                                            Institute for Atmospheric and Climate Science, ETH Zurich, 8092 Zurich, Switzerland
                                        
                                    
                                            John A. Paulson School of Engineering and Applied Sciences, Harvard University, Cambridge, MA, USA
                                        
                                    Rahel Weber
                                            Institute for Atmospheric and Climate Science, ETH Zurich, 8092 Zurich, Switzerland
                                        
                                    
                                            John A. Paulson School of Engineering and Applied Sciences, Harvard University, Cambridge, MA, USA
                                        
                                    
                                            now at: Federal Office of Meteorology and Climatology MeteoSwiss, Zurich, Switzerland
                                        
                                    Aryeh Feinberg
                                            Institute for Atmospheric and Climate Science, ETH Zurich, 8092 Zurich, Switzerland
                                        
                                    
                                            Institute of Biogeochemistry and Pollutant Dynamics, ETH Zurich, 8092 Zurich, Switzerland
                                        
                                    
                                            now at: Department of Atmospheric Chemistry and Climate, Institute of Physical Chemistry Blas Cabrera, CSIC, Madrid, Spain
                                        
                                    Andrea Stenke
                                            Institute for Atmospheric and Climate Science, ETH Zurich, 8092 Zurich, Switzerland
                                        
                                    
                                            Institute of Biogeochemistry and Pollutant Dynamics, ETH Zurich, 8092 Zurich, Switzerland
                                        
                                    
                                            Eawag, Swiss Federal Institute of Aquatic Science and Technology, Dübendorf, Switzerland
                                        
                                    John A. Dykema
                                            John A. Paulson School of Engineering and Applied Sciences, Harvard University, Cambridge, MA, USA
                                        
                                    Beiping Luo
                                            Institute for Atmospheric and Climate Science, ETH Zurich, 8092 Zurich, Switzerland
                                        
                                    Georgios A. Kelesidis
                                            Particle Technology Laboratory, ETH Zurich, 8092 Zurich, Switzerland
                                        
                                    
                                            now at: Faculty of Aerospace Engineering, Delft University of Technology, Kluyverweg 1, 2629 HS Delft, the Netherlands
                                        
                                    Christian A. Bruun
                                            Particle Technology Laboratory, ETH Zurich, 8092 Zurich, Switzerland
                                        
                                    Timofei Sukhodolov
                                            Physikalisch-Meteorologisches Observatorium Davos and World Radiation Center, Davos, Switzerland
                                        
                                    Frank N. Keutsch
                                            John A. Paulson School of Engineering and Applied Sciences, Harvard University, Cambridge, MA, USA
                                        
                                    
                                            Department of Chemistry and Chemical Biology, Harvard University, Cambridge, MA, USA
                                        
                                    
                                            Department of Earth and Planetary Sciences, Harvard University, Cambridge, MA, USA
                                        
                                    Thomas Peter
                                            Institute for Atmospheric and Climate Science, ETH Zurich, 8092 Zurich, Switzerland
                                        
                                    Gabriel Chiodo
                                            Institute for Atmospheric and Climate Science, ETH Zurich, 8092 Zurich, Switzerland
                                        
                                    
                                            Instituto de Geociencias (IGEO), CSIC-UCM, Madrid, Spain
                                        
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                            Cited
7 citations as recorded by crossref.
- Injecting solid particles into the stratosphere could mitigate global warming but currently entails great uncertainties S. Vattioni et al. 10.1038/s43247-025-02038-1
- Engineering and logistical concerns add practical limitations to stratospheric aerosol injection strategies M. Hack et al. 10.1038/s41598-025-20447-2
- Optimizing stratospheric aerosol lifetime and albedo through particle morphology and refractive index B. Vennes et al. 10.1039/D5EA00026B
- Key Gaps in Models' Physical Representation of Climate Intervention and Its Impacts S. Eastham et al. 10.1029/2024MS004872
- Stratospheric injection of solid particles reduces side effects on circulation and climate compared to SO2 injections F. Stefanetti et al. 10.1088/2752-5295/ad9f93
- Near-future rocket launches could slow ozone recovery L. Revell et al. 10.1038/s41612-025-01098-6
- A fully coupled solid-particle microphysics scheme for stratospheric aerosol injections within the aerosol–chemistry–climate model SOCOL-AERv2 S. Vattioni et al. 10.5194/gmd-17-7767-2024
6 citations as recorded by crossref.
- Injecting solid particles into the stratosphere could mitigate global warming but currently entails great uncertainties S. Vattioni et al. 10.1038/s43247-025-02038-1
- Engineering and logistical concerns add practical limitations to stratospheric aerosol injection strategies M. Hack et al. 10.1038/s41598-025-20447-2
- Optimizing stratospheric aerosol lifetime and albedo through particle morphology and refractive index B. Vennes et al. 10.1039/D5EA00026B
- Key Gaps in Models' Physical Representation of Climate Intervention and Its Impacts S. Eastham et al. 10.1029/2024MS004872
- Stratospheric injection of solid particles reduces side effects on circulation and climate compared to SO2 injections F. Stefanetti et al. 10.1088/2752-5295/ad9f93
- Near-future rocket launches could slow ozone recovery L. Revell et al. 10.1038/s41612-025-01098-6
Latest update: 30 Oct 2025
Short summary
            We quantified impacts and efficiency of stratospheric solar climate intervention via solid particle injection. Microphysical interactions of solid particles with the sulfur cycle were interactively coupled to the heterogeneous chemistry scheme and the radiative transfer code of an aerosol–chemistry–climate model. Compared to injection of SO2 we only find a stronger cooling efficiency for solid particles when normalizing to the aerosol load but not when normalizing to the injection rate.
            We quantified impacts and efficiency of stratospheric solar climate intervention via solid...
            
         
 
                             
                             
             
             
            