Articles | Volume 16, issue 23
https://doi.org/10.5194/gmd-16-7037-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/gmd-16-7037-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Model evaluation paper
| 
04 Dec 2023
Model evaluation paper |
| 04 Dec 2023
| 04 Dec 2023
Simulations of 7Be and 10Be with the GEOS-Chem global model v14.0.2 using state-of-the-art production rates
Minjie Zheng
CORRESPONDING AUTHOR
Institute for Atmospheric and Climate Science, ETH Zürich, Zürich, Switzerland
Department of Geology, Lund University, Lund, Sweden
Center for Atmospheric Research, University of Oulu, Oulu, Finland
Hongyu Liu
National Institute of Aerospace, Hampton, Virginia, USA
Science Directorate, NASA Langley Research Center, Hampton, Virginia, USA
Florian Adolphi
Alfred Wegener Institute, Helmholtz Centre for Polar and Marine Research, Bremerhaven, Germany
Faculty of Geosciences, Bremen University, Bremen, Germany
Raimund Muscheler
Department of Geology, Lund University, Lund, Sweden
Zhengyao Lu
Department of Physical Geography and Ecosystem Science, Lund University, Lund, Sweden
Mousong Wu
International Institute for Earth System Science, Nanjing University, Nanjing, China
Center for Atmospheric Research, University of Oulu, Oulu, Finland
Related authors
Gargi Sengupta, Minjie Zheng, and Nønne L. Prisle
Atmos. Chem. Phys., 24, 1467–1487, https://doi.org/10.5194/acp-24-1467-2024, https://doi.org/10.5194/acp-24-1467-2024, 2024
Short summary
Short summary
The effect of organic acid aerosol on sulfur chemistry and cloud properties was investigated in an atmospheric model. Organic acid dissociation was considered using both bulk and surface-related properties. We found that organic acid dissociation leads to increased hydrogen ion concentrations and sulfate aerosol mass in aqueous aerosols, increasing cloud formation. This could be important in large-scale climate models as many organic aerosol components are both acidic and surface-active.
Arnaud Nicolas, Gesine Mollenhauer, Johannes Lachner, Konstanze Stübner, Maylin Malter, Jutta Wollenburg, Hendrik Grotheer, and Florian Adolphi
EGUsphere, https://doi.org/10.5194/egusphere-2024-1992, https://doi.org/10.5194/egusphere-2024-1992, 2024
This preprint is open for discussion and under review for Climate of the Past (CP).
Short summary
Short summary
We use the authigenic 10Be/9Be record of a Laptev Sea sediment core for the period 8–14 kyr BP and synchronize it with the 10Be records from absolutely dated ice cores. We employed a likelihood function to calculate the ΔR values. A benthic ΔR value of +345±60 14C years was estimated, which corresponds to a marine reservoir age of 848±90 14C years. This new ΔR value was used to refine the age-depth model for core PS2458-4, establishing it as a potential reference chronology for the Laptev Sea.
Xingyu Wang, Fei Jiang, Hengmao Wang, Zhengqi Zhang, Mousong Wu, Jun Wang, Wei He, Weimin Ju, and Jingming Chen
EGUsphere, https://doi.org/10.5194/egusphere-2024-1568, https://doi.org/10.5194/egusphere-2024-1568, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
The role of Orbital Carbon Observatory 3 (OCO-3) satellites in estimating the global terrestrial near-Earth environment is unclear. So we study it by assimilating OCO-3 XCO2 alone and with OCO-2 XCO2 inversion. We found that assimilation OCO-3 XCO2 underestimated land sinks at high latitudes by retrieval alone. Joint assimilation of OCO-2 and OCO-3 XCO2 needs to be retrieved to better estimate global terrestrial NEEs.
Hongyu Liu, Bo Zhang, Richard H. Moore, Luke D. Ziemba, Richard A. Ferrare, Hyundeok Choi, Armin Sorooshian, David Painemal, Hailong Wang, Michael A. Shook, Amy Jo Scarino, Johnathan W. Hair, Ewan C. Crosbie, Marta A. Fenn, Taylor J. Shingler, Chris A. Hostetler, Gao Chen, Mary M. Kleb, Gan Luo, Fangqun Yu, Jason L. Tackett, Mark A. Vaughan, Yongxiang Hu, Glenn S. Diskin, John B. Nowak, Joshua P. DiGangi, Yonghoon Choi, Christoph A. Keller, and Matthew S. Johnson
EGUsphere, https://doi.org/10.5194/egusphere-2024-1127, https://doi.org/10.5194/egusphere-2024-1127, 2024
Short summary
Short summary
We use the GEOS-Chem model to simulate aerosols over the western North Atlantic Ocean (WNAO) during the winter and summer campaigns of ACTIVATE 2020. Model results are evaluated against in situ and remote sensing measurements from two aircraft as well as ground-based and satellite observations. The improved understanding of the aerosol life cycle, composition, transport pathways, and distribution has important implications for characterizing aerosol-cloud-meteorology interactions over the WNAO.
Gargi Sengupta, Minjie Zheng, and Nønne L. Prisle
Atmos. Chem. Phys., 24, 1467–1487, https://doi.org/10.5194/acp-24-1467-2024, https://doi.org/10.5194/acp-24-1467-2024, 2024
Short summary
Short summary
The effect of organic acid aerosol on sulfur chemistry and cloud properties was investigated in an atmospheric model. Organic acid dissociation was considered using both bulk and surface-related properties. We found that organic acid dissociation leads to increased hydrogen ion concentrations and sulfate aerosol mass in aqueous aerosols, increasing cloud formation. This could be important in large-scale climate models as many organic aerosol components are both acidic and surface-active.
Huajie Zhu, Xiuli Xing, Mousong Wu, Weimin Ju, and Fei Jiang
EGUsphere, https://doi.org/10.5194/egusphere-2023-3032, https://doi.org/10.5194/egusphere-2023-3032, 2024
Short summary
Short summary
In this study, ecosystem COS fluxes data were employed to optimize GPP estimation across various ecosystems with the Boreal Ecosystem Productivity Simulator (BEPS), which was further developed for simulating the leaf COS uptake under its state-of-the-art ‘two-leaf’ framework. our results showcased the efficacy of COS in enhancing model prediction and reducing prediction uncertainty of GPP, and deepened insights into the sensitivity, identifiability, and interactions of parameters related to COS.
Sampo Vepsäläinen, Silvia M. Calderón, and Nønne L. Prisle
Atmos. Chem. Phys., 23, 15149–15164, https://doi.org/10.5194/acp-23-15149-2023, https://doi.org/10.5194/acp-23-15149-2023, 2023
Short summary
Short summary
Atmospheric aerosols act as seeds for cloud formation. Many aerosols contain surface active material that accumulates at the surface of growing droplets. This can affect cloud droplet activation, but the broad significance of the effect and the best way to model it are still debated. We compare predictions of six models to surface activity of strongly surface active aerosol and find significant differences between the models, especially with large fractions of surfactant in the dry particles.
Putian Zhou, Zhengyao Lu, Jukka-Pekka Keskinen, Qiong Zhang, Juha Lento, Jianpu Bian, Twan van Noije, Philippe Le Sager, Veli-Matti Kerminen, Markku Kulmala, Michael Boy, and Risto Makkonen
Clim. Past, 19, 2445–2462, https://doi.org/10.5194/cp-19-2445-2023, https://doi.org/10.5194/cp-19-2445-2023, 2023
Short summary
Short summary
A Green Sahara with enhanced rainfall and larger vegetation cover existed in northern Africa about 6000 years ago. Biosphere–atmosphere interactions are found to be critical to explaining this wet period. Based on modeled vegetation reconstruction data, we simulated dust emissions and aerosol formation, which are key factors in biosphere–atmosphere interactions. Our results also provide a benchmark of aerosol climatology for future paleo-climate simulation experiments.
Amit Kumar Pandit, Jean-Paul Vernier, Thomas Duncan Fairlie, Kristopher M. Bedka, Melody A. Avery, Harish Gadhavi, Madineni Venkat Ratnam, Sanjeev Dwivedi, Kasimahanthi Amar Jyothi, Frank G. Wienhold, Holger Vömel, Hongyu Liu, Bo Zhang, Buduru Suneel Kumar, Tra Dinh, and Achuthan Jayaraman
EGUsphere, https://doi.org/10.5194/egusphere-2023-2236, https://doi.org/10.5194/egusphere-2023-2236, 2023
Short summary
Short summary
This study investigates the formation mechanism of a tropopause cirrus cloud layer observed at extremely cold temperatures over Hyderabad in India during the 2017 Asian summer monsoon using balloon-borne sensors. Ice crystals smaller than 50 microns were found in this optically thin cirrus cloud layer. Combined analysis of back-trajectories, satellite, and model data revealed that the formation of this layer was influenced by gravity waves and stratospheric hydration induced by typhoon Hato.
Chiara I. Paleari, Florian Mekhaldi, Tobias Erhardt, Minjie Zheng, Marcus Christl, Florian Adolphi, Maria Hörhold, and Raimund Muscheler
Clim. Past, 19, 2409–2422, https://doi.org/10.5194/cp-19-2409-2023, https://doi.org/10.5194/cp-19-2409-2023, 2023
Short summary
Short summary
In this study, we test the use of excess meltwater from continuous flow analysis from a firn core from Greenland for the measurement of 10Be for solar activity reconstructions. We show that the quality of results is similar to the measurements on clean firn, which opens the possibility to obtain continuous 10Be records without requiring large amounts of clean ice. Furthermore, we investigate the possibility of identifying solar storm signals in 10Be records from Greenland and Antarctica.
Tobias Erhardt, Camilla Marie Jensen, Florian Adolphi, Helle Astrid Kjær, Remi Dallmayr, Birthe Twarloh, Melanie Behrens, Motohiro Hirabayashi, Kaori Fukuda, Jun Ogata, François Burgay, Federico Scoto, Ilaria Crotti, Azzurra Spagnesi, Niccoló Maffezzoli, Delia Segato, Chiara Paleari, Florian Mekhaldi, Raimund Muscheler, Sophie Darfeuil, and Hubertus Fischer
Earth Syst. Sci. Data, 15, 5079–5091, https://doi.org/10.5194/essd-15-5079-2023, https://doi.org/10.5194/essd-15-5079-2023, 2023
Short summary
Short summary
The presented paper provides a 3.8 kyr long dataset of aerosol concentrations from the East Greenland Ice coring Project (EGRIP) ice core. The data consists of 1 mm depth-resolution profiles of calcium, sodium, ammonium, nitrate, and electrolytic conductivity as well as decadal averages of these profiles. Alongside the data a detailed description of the measurement setup as well as a discussion of the uncertainties are given.
Huajie Zhu, Mousong Wu, Fei Jiang, Michael Vossbeck, Thomas Kaminski, Xiuli Xing, Jun Wang, Weimin Ju, and Jing M. Chen
EGUsphere, https://doi.org/10.5194/egusphere-2023-1955, https://doi.org/10.5194/egusphere-2023-1955, 2023
Short summary
Short summary
In this work, Nanjing University Carbon Assimilation System (NUCAS) was developed. Data assimilation experiments were conducted to demonstrate the robustness and to investigate the feasibility and applicability of NUCAS. The assimilation of COS significantly improved the model performance in gross primary productivity, sensible heat, latent heat and even soil moisture, demonstrating that COS can provide strong constraints on parameters relevant to water, energy and carbon processes.
Armin Sorooshian, Mikhail D. Alexandrov, Adam D. Bell, Ryan Bennett, Grace Betito, Sharon P. Burton, Megan E. Buzanowicz, Brian Cairns, Eduard V. Chemyakin, Gao Chen, Yonghoon Choi, Brian L. Collister, Anthony L. Cook, Andrea F. Corral, Ewan C. Crosbie, Bastiaan van Diedenhoven, Joshua P. DiGangi, Glenn S. Diskin, Sanja Dmitrovic, Eva-Lou Edwards, Marta A. Fenn, Richard A. Ferrare, David van Gilst, Johnathan W. Hair, David B. Harper, Miguel Ricardo A. Hilario, Chris A. Hostetler, Nathan Jester, Michael Jones, Simon Kirschler, Mary M. Kleb, John M. Kusterer, Sean Leavor, Joseph W. Lee, Hongyu Liu, Kayla McCauley, Richard H. Moore, Joseph Nied, Anthony Notari, John B. Nowak, David Painemal, Kasey E. Phillips, Claire E. Robinson, Amy Jo Scarino, Joseph S. Schlosser, Shane T. Seaman, Chellappan Seethala, Taylor J. Shingler, Michael A. Shook, Kenneth A. Sinclair, William L. Smith Jr., Douglas A. Spangenberg, Snorre A. Stamnes, Kenneth L. Thornhill, Christiane Voigt, Holger Vömel, Andrzej P. Wasilewski, Hailong Wang, Edward L. Winstead, Kira Zeider, Xubin Zeng, Bo Zhang, Luke D. Ziemba, and Paquita Zuidema
Earth Syst. Sci. Data, 15, 3419–3472, https://doi.org/10.5194/essd-15-3419-2023, https://doi.org/10.5194/essd-15-3419-2023, 2023
Short summary
Short summary
The NASA Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) produced a unique dataset for research into aerosol–cloud–meteorology interactions. HU-25 Falcon and King Air aircraft conducted systematic and spatially coordinated flights over the northwest Atlantic Ocean. This paper describes the ACTIVATE flight strategy, instrument and complementary dataset products, data access and usage details, and data application notes.
Giulia Sinnl, Florian Adolphi, Marcus Christl, Kees C. Welten, Thomas Woodruff, Marc Caffee, Anders Svensson, Raimund Muscheler, and Sune Olander Rasmussen
Clim. Past, 19, 1153–1175, https://doi.org/10.5194/cp-19-1153-2023, https://doi.org/10.5194/cp-19-1153-2023, 2023
Short summary
Short summary
The record of past climate is preserved by several archives from different regions, such as ice cores from Greenland or Antarctica or speleothems from caves such as the Hulu Cave in China. In this study, these archives are aligned by taking advantage of the globally synchronous production of cosmogenic radionuclides. This produces a new perspective on the global climate in the period between 20 000 and 25 000 years ago.
Robert Mulvaney, Eric W. Wolff, Mackenzie M. Grieman, Helene H. Hoffmann, Jack D. Humby, Christoph Nehrbass-Ahles, Rachael H. Rhodes, Isobel F. Rowell, Frédéric Parrenin, Loïc Schmidely, Hubertus Fischer, Thomas F. Stocker, Marcus Christl, Raimund Muscheler, Amaelle Landais, and Frédéric Prié
Clim. Past, 19, 851–864, https://doi.org/10.5194/cp-19-851-2023, https://doi.org/10.5194/cp-19-851-2023, 2023
Short summary
Short summary
We present an age scale for a new ice core drilled at Skytrain Ice Rise, an ice rise facing the Ronne Ice Shelf in Antarctica. Various measurements in the ice and air phases are used to match the ice core to other Antarctic cores that have already been dated, and a new age scale is constructed. The 651 m ice core includes ice that is confidently dated to 117 000–126 000 years ago, in the last interglacial. Older ice is found deeper down, but there are flow disturbances in the deeper ice.
Hongyue Zhang, Jesper Sjolte, Zhengyao Lu, Jian Liu, Weiyi Sun, and Lingfeng Wan
Clim. Past, 19, 665–680, https://doi.org/10.5194/cp-19-665-2023, https://doi.org/10.5194/cp-19-665-2023, 2023
Short summary
Short summary
Based on proxy data and modeling, the Arctic temperature has an asymmetric cooling trend with more cooling over the Atlantic Arctic than the Pacific Arctic during the Holocene, dominated by orbital forcing. There is a seasonal difference in the asymmetric cooling trend, which is dominated by the DJF (December, January, and February) temperature variability. The Arctic dipole mode of sea level pressure and sea ice play a major role in asymmetric temperature changes.
Hazel Vernier, Neeraj Rastogi, Hongyu Liu, Amit Kumar Pandit, Kris Bedka, Anil Patel, Madineni Venkat Ratnam, Buduru Suneel Kumar, Bo Zhang, Harish Gadhavi, Frank Wienhold, Gwenael Berthet, and Jean-Paul Vernier
Atmos. Chem. Phys., 22, 12675–12694, https://doi.org/10.5194/acp-22-12675-2022, https://doi.org/10.5194/acp-22-12675-2022, 2022
Short summary
Short summary
The chemical composition of the stratospheric aerosols collected aboard high-altitude balloons above the summer Asian monsoon reveals the presence of nitrate/nitrite. Using numerical simulations and satellite observations, we found that pollution as well as lightning could explain some of our observations.
Fei Jiang, Weimin Ju, Wei He, Mousong Wu, Hengmao Wang, Jun Wang, Mengwei Jia, Shuzhuang Feng, Lingyu Zhang, and Jing M. Chen
Earth Syst. Sci. Data, 14, 3013–3037, https://doi.org/10.5194/essd-14-3013-2022, https://doi.org/10.5194/essd-14-3013-2022, 2022
Short summary
Short summary
A 10-year (2010–2019) global monthly terrestrial NEE dataset (GCAS2021) was inferred from the GOSAT ACOS v9 XCO2 product. It shows strong carbon sinks over eastern N. America, the Amazon, the Congo Basin, Europe, boreal forests, southern China, and Southeast Asia. It has good quality and can reflect the impacts of extreme climates and large-scale climate anomalies on carbon fluxes well. We believe that this dataset can contribute to regional carbon budget assessment and carbon dynamics research.
Giulia Sinnl, Mai Winstrup, Tobias Erhardt, Eliza Cook, Camilla Marie Jensen, Anders Svensson, Bo Møllesøe Vinther, Raimund Muscheler, and Sune Olander Rasmussen
Clim. Past, 18, 1125–1150, https://doi.org/10.5194/cp-18-1125-2022, https://doi.org/10.5194/cp-18-1125-2022, 2022
Short summary
Short summary
A new Greenland ice-core timescale, covering the last 3800 years, was produced using the machine learning algorithm StratiCounter. We synchronized the ice cores using volcanic eruptions and wildfires. We compared the new timescale to the tree-ring timescale, finding good alignment both between the common signatures of volcanic eruptions and of solar activity. Our Greenlandic timescales is safe to use for the Late Holocene, provided one uses our uncertainty estimate.
Kevin J. Sanchez, Bo Zhang, Hongyu Liu, Matthew D. Brown, Ewan C. Crosbie, Francesca Gallo, Johnathan W. Hair, Chris A. Hostetler, Carolyn E. Jordan, Claire E. Robinson, Amy Jo Scarino, Taylor J. Shingler, Michael A. Shook, Kenneth L. Thornhill, Elizabeth B. Wiggins, Edward L. Winstead, Luke D. Ziemba, Georges Saliba, Savannah L. Lewis, Lynn M. Russell, Patricia K. Quinn, Timothy S. Bates, Jack Porter, Thomas G. Bell, Peter Gaube, Eric S. Saltzman, Michael J. Behrenfeld, and Richard H. Moore
Atmos. Chem. Phys., 22, 2795–2815, https://doi.org/10.5194/acp-22-2795-2022, https://doi.org/10.5194/acp-22-2795-2022, 2022
Short summary
Short summary
Atmospheric particle concentrations impact clouds, which strongly impact the amount of sunlight reflected back into space and the overall climate. Measurements of particles over the ocean are rare and expensive to collect, so models are necessary to fill in the gaps by simulating both particle and clouds. However, some measurements are needed to test the accuracy of the models. Here, we measure changes in particles in different weather conditions, which are ideal for comparison with models.
Sampo Vepsäläinen, Silvia M. Calderón, Jussi Malila, and Nønne L. Prisle
Atmos. Chem. Phys., 22, 2669–2687, https://doi.org/10.5194/acp-22-2669-2022, https://doi.org/10.5194/acp-22-2669-2022, 2022
Short summary
Short summary
Atmospheric aerosols act as seeds for cloud formation. Many aerosols contain surface active material that accumulates at the surface of growing droplets. This can affect cloud droplet activation, but the broad significance of the effect and the best way to model it are still debated. We compare predictions of six different model approaches to surface activity of organic aerosols and find significant differences between the models, especially with large fractions of organics in the dry particles.
Erika Brattich, Hongyu Liu, Bo Zhang, Miguel Ángel Hernández-Ceballos, Jussi Paatero, Darko Sarvan, Vladimir Djurdjevic, Laura Tositti, and Jelena Ajtić
Atmos. Chem. Phys., 21, 17927–17951, https://doi.org/10.5194/acp-21-17927-2021, https://doi.org/10.5194/acp-21-17927-2021, 2021
Short summary
Short summary
In this study we analyse the output of a chemistry and transport model together with observations of different meteorological and compositional variables to demonstrate the link between sudden stratospheric warming and transport of stratospheric air to the surface in the subpolar regions of Europe during the cold season. Our findings have particular implications for atmospheric composition since climate projections indicate more frequent sudden stratospheric warming under a warmer climate.
Nønne L. Prisle
Atmos. Chem. Phys., 21, 16387–16411, https://doi.org/10.5194/acp-21-16387-2021, https://doi.org/10.5194/acp-21-16387-2021, 2021
Short summary
Short summary
A mass-based Gibbs adsorption model is presented to enable predictive Köhler calculations of droplet growth and activation with considerations of surface partitioning, surface tension, and non-ideal water activity for chemically complex and unresolved surface active aerosol mixtures, including actual atmospheric samples. The model is used to calculate cloud condensation nuclei (CCN) activity of aerosol particles comprising strongly surface-active model atmospheric humic-like substances (HULIS).
Hossein Dadashazar, Majid Alipanah, Miguel Ricardo A. Hilario, Ewan Crosbie, Simon Kirschler, Hongyu Liu, Richard H. Moore, Andrew J. Peters, Amy Jo Scarino, Michael Shook, K. Lee Thornhill, Christiane Voigt, Hailong Wang, Edward Winstead, Bo Zhang, Luke Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 21, 16121–16141, https://doi.org/10.5194/acp-21-16121-2021, https://doi.org/10.5194/acp-21-16121-2021, 2021
Short summary
Short summary
This study investigates precipitation impacts on long-range transport of North American outflow over the western North Atlantic Ocean (WNAO). Results demonstrate that precipitation scavenging plays a significant role in modifying surface aerosol concentrations over the WNAO, especially in winter and spring due to large-scale scavenging processes. This study highlights how precipitation impacts surface aerosol properties with relevance for other marine regions vulnerable to continental outflow.
Hossein Dadashazar, David Painemal, Majid Alipanah, Michael Brunke, Seethala Chellappan, Andrea F. Corral, Ewan Crosbie, Simon Kirschler, Hongyu Liu, Richard H. Moore, Claire Robinson, Amy Jo Scarino, Michael Shook, Kenneth Sinclair, K. Lee Thornhill, Christiane Voigt, Hailong Wang, Edward Winstead, Xubin Zeng, Luke Ziemba, Paquita Zuidema, and Armin Sorooshian
Atmos. Chem. Phys., 21, 10499–10526, https://doi.org/10.5194/acp-21-10499-2021, https://doi.org/10.5194/acp-21-10499-2021, 2021
Short summary
Short summary
This study investigates the seasonal cycle of cloud drop number concentration (Nd) over the western North Atlantic Ocean (WNAO) using multiple datasets. Reasons for the puzzling discrepancy between the seasonal cycles of Nd and aerosol concentration were identified. Results indicate that Nd is highest in winter (when aerosol proxy values are often lowest) due to conditions both linked to cold-air outbreaks and that promote greater droplet activation.
Nathalie Van der Putten, Florian Adolphi, Anette Mellström, Jesper Sjolte, Cyriel Verbruggen, Jan-Berend Stuut, Tobias Erhardt, Yves Frenot, and Raimund Muscheler
Clim. Past Discuss., https://doi.org/10.5194/cp-2021-69, https://doi.org/10.5194/cp-2021-69, 2021
Manuscript not accepted for further review
Short summary
Short summary
In recent decades, Southern Hemisphere westerlies (SHW) moved equator-ward during periods of low solar activity leading to increased winds/precipitation at 46° S, Indian Ocean. We present a terrestrial SHW proxy-record and find stronger SHW influence at Crozet, shortly after 2.8 ka BP, synchronous with a climate shift in the Northern Hemisphere, attributed to a major decline in solar activity. The bipolar response to solar forcing is supported by a climate model forced by solar irradiance only.
Jack J. Lin, Kamal Raj R Mundoli, Stella Wang, Esko Kokkonen, Mikko-Heikki Mikkelä, Samuli Urpelainen, and Nønne L. Prisle
Atmos. Chem. Phys., 21, 4709–4727, https://doi.org/10.5194/acp-21-4709-2021, https://doi.org/10.5194/acp-21-4709-2021, 2021
Short summary
Short summary
We used surface-sensitive X-ray photoelectron spectroscopy (XPS) to study laboratory-generated nanoparticles of atmospheric interest at 0–16 % relative humidity. XPS gives direct information about changes in the chemical state from the binding energies of probed elements. Our results indicate water adsorption and associated chemical changes at the particle surfaces well below deliquescence, with distinct features for different particle components and implications for atmospheric chemistry.
Qiong Zhang, Ellen Berntell, Josefine Axelsson, Jie Chen, Zixuan Han, Wesley de Nooijer, Zhengyao Lu, Qiang Li, Qiang Zhang, Klaus Wyser, and Shuting Yang
Geosci. Model Dev., 14, 1147–1169, https://doi.org/10.5194/gmd-14-1147-2021, https://doi.org/10.5194/gmd-14-1147-2021, 2021
Short summary
Short summary
Paleoclimate modelling has long been regarded as a strong out-of-sample test bed of the climate models that are used for the projection of future climate changes. Here, we document the model experimental setups for the three past warm periods with EC-Earth3-LR and present the results on the large-scale features. The simulations demonstrate good performance of the model in capturing the climate response under different climate forcings.
Georgia Michailoudi, Jack J. Lin, Hayato Yuzawa, Masanari Nagasaka, Marko Huttula, Nobuhiro Kosugi, Theo Kurtén, Minna Patanen, and Nønne L. Prisle
Atmos. Chem. Phys., 21, 2881–2894, https://doi.org/10.5194/acp-21-2881-2021, https://doi.org/10.5194/acp-21-2881-2021, 2021
Short summary
Short summary
This study provides insight into hydration of two significant atmospheric compounds, glyoxal and methylglyoxal. Using synchrotron radiation excited X-ray absorption spectroscopy, we confirm that glyoxal is fully hydrated in water, and for the first time, we experimentally detect enol structures in aqueous methylglyoxal. Our results support the contribution of these compounds to secondary organic aerosol formation, known to have a large uncertainty in atmospheric models and climate predictions.
Fei Jiang, Hengmao Wang, Jing M. Chen, Weimin Ju, Xiangjun Tian, Shuzhuang Feng, Guicai Li, Zhuoqi Chen, Shupeng Zhang, Xuehe Lu, Jane Liu, Haikun Wang, Jun Wang, Wei He, and Mousong Wu
Atmos. Chem. Phys., 21, 1963–1985, https://doi.org/10.5194/acp-21-1963-2021, https://doi.org/10.5194/acp-21-1963-2021, 2021
Short summary
Short summary
We present a 6-year inversion from 2010 to 2015 for the global and regional carbon fluxes using only the GOSAT XCO2 retrievals. We find that the XCO2 retrievals could significantly improve the modeling of atmospheric CO2 concentrations and that the inferred interannual variations in the terrestrial carbon fluxes in most land regions have a better relationship with the changes in severe drought area or leaf area index, or are more consistent with the previous estimates about drought impact.
Bo Zhang, Hongyu Liu, James H. Crawford, Gao Chen, T. Duncan Fairlie, Scott Chambers, Chang-Hee Kang, Alastair G. Williams, Kai Zhang, David B. Considine, Melissa P. Sulprizio, and Robert M. Yantosca
Atmos. Chem. Phys., 21, 1861–1887, https://doi.org/10.5194/acp-21-1861-2021, https://doi.org/10.5194/acp-21-1861-2021, 2021
Short summary
Short summary
We simulate atmospheric 222Rn using the GEOS-Chem model to improve understanding of 222Rn emissions and characterize convective transport in the model. We demonstrate the potential of a customized global 222Rn emission scenario to improve simulated surface 222Rn concentrations and seasonality. We assess convective transport using observed 222Rn vertical profiles. Results have important implications for using chemical transport models to interpret the transport of trace gases and aerosols.
Betty Croft, Randall V. Martin, Richard H. Moore, Luke D. Ziemba, Ewan C. Crosbie, Hongyu Liu, Lynn M. Russell, Georges Saliba, Armin Wisthaler, Markus Müller, Arne Schiller, Martí Galí, Rachel Y.-W. Chang, Erin E. McDuffie, Kelsey R. Bilsback, and Jeffrey R. Pierce
Atmos. Chem. Phys., 21, 1889–1916, https://doi.org/10.5194/acp-21-1889-2021, https://doi.org/10.5194/acp-21-1889-2021, 2021
Short summary
Short summary
North Atlantic Aerosols and Marine Ecosystems Study measurements combined with GEOS-Chem-TOMAS modeling suggest that several not-well-understood key factors control northwest Atlantic aerosol number and size. These synergetic and climate-relevant factors include particle formation near and above the marine boundary layer top, particle growth by marine secondary organic aerosol on descent, particle formation/growth related to dimethyl sulfide, sea spray aerosol, and ship emissions.
Kevin J. Sanchez, Bo Zhang, Hongyu Liu, Georges Saliba, Chia-Li Chen, Savannah L. Lewis, Lynn M. Russell, Michael A. Shook, Ewan C. Crosbie, Luke D. Ziemba, Matthew D. Brown, Taylor J. Shingler, Claire E. Robinson, Elizabeth B. Wiggins, Kenneth L. Thornhill, Edward L. Winstead, Carolyn Jordan, Patricia K. Quinn, Timothy S. Bates, Jack Porter, Thomas G. Bell, Eric S. Saltzman, Michael J. Behrenfeld, and Richard H. Moore
Atmos. Chem. Phys., 21, 831–851, https://doi.org/10.5194/acp-21-831-2021, https://doi.org/10.5194/acp-21-831-2021, 2021
Short summary
Short summary
Models describing atmospheric airflow were combined with satellite measurements representative of marine phytoplankton and other meteorological variables. These combined variables were compared to measured aerosol to identify upwind influences on aerosol concentrations. Results indicate that phytoplankton production rates upwind impact the aerosol mass. Also, results suggest that the condensation of mass onto short-lived large sea spray particles may be a significant sink of aerosol mass.
Michael Sarnthein, Kevin Küssner, Pieter M. Grootes, Blanca Ausin, Timothy Eglinton, Juan Muglia, Raimund Muscheler, and Gordon Schlolaut
Clim. Past, 16, 2547–2571, https://doi.org/10.5194/cp-16-2547-2020, https://doi.org/10.5194/cp-16-2547-2020, 2020
Short summary
Short summary
The dating technique of 14C plateau tuning uses U/Th-based model ages, refinements of the Lake Suigetsu age scale, and the link of surface ocean carbon to the globally mixed atmosphere as basis of age correlation. Our synthesis employs data of 20 sediment cores from the global ocean and offers a coherent picture of global ocean circulation evolving over glacial-to-deglacial times on semi-millennial scales to be compared with climate records stored in marine sediments, ice cores, and speleothems.
Leonie Peti, Kathryn E. Fitzsimmons, Jenni L. Hopkins, Andreas Nilsson, Toshiyuki Fujioka, David Fink, Charles Mifsud, Marcus Christl, Raimund Muscheler, and Paul C. Augustinus
Geochronology, 2, 367–410, https://doi.org/10.5194/gchron-2-367-2020, https://doi.org/10.5194/gchron-2-367-2020, 2020
Short summary
Short summary
Orakei Basin – a former maar lake in Auckland, New Zealand – provides an outstanding sediment record over the last ca. 130 000 years, but an age model is required to allow the reconstruction of climate change and volcanic eruptions contained in the sequence. To construct a relationship between depth in the sediment core and age of deposition, we combined tephrochronology, radiocarbon dating, luminescence dating, and the relative intensity of the paleomagnetic field in a Bayesian age–depth model.
Noora Hyttinen, Reyhaneh Heshmatnezhad, Jonas Elm, Theo Kurtén, and Nønne L. Prisle
Atmos. Chem. Phys., 20, 13131–13143, https://doi.org/10.5194/acp-20-13131-2020, https://doi.org/10.5194/acp-20-13131-2020, 2020
Short summary
Short summary
We present aqueous solubilities and activity coefficients of mono- and dicarboxylic acids (C1–C6 and C2–C8, respectively) estimated using the COSMOtherm program. In addition, we have calculated effective equilibrium constants of dimerization and hydration of the same acids in the condensed phase. We were also able to improve the agreement between experimental and estimated properties of monocarboxylic acids in aqueous solutions by including clustering reactions in COSMOtherm calculations.
Jesper Sjolte, Florian Adolphi, Bo M. Vinther, Raimund Muscheler, Christophe Sturm, Martin Werner, and Gerrit Lohmann
Clim. Past, 16, 1737–1758, https://doi.org/10.5194/cp-16-1737-2020, https://doi.org/10.5194/cp-16-1737-2020, 2020
Short summary
Short summary
In this study we investigate seasonal climate reconstructions produced by matching climate model output to ice core and tree-ring data, and we evaluate the model–data reconstructions against meteorological observations. The reconstructions capture the main patterns of variability in sea level pressure and temperature in summer and winter. The performance of the reconstructions depends on seasonal climate variability itself, and definitions of seasons can be optimized to capture this variability.
Anders Svensson, Dorthe Dahl-Jensen, Jørgen Peder Steffensen, Thomas Blunier, Sune O. Rasmussen, Bo M. Vinther, Paul Vallelonga, Emilie Capron, Vasileios Gkinis, Eliza Cook, Helle Astrid Kjær, Raimund Muscheler, Sepp Kipfstuhl, Frank Wilhelms, Thomas F. Stocker, Hubertus Fischer, Florian Adolphi, Tobias Erhardt, Michael Sigl, Amaelle Landais, Frédéric Parrenin, Christo Buizert, Joseph R. McConnell, Mirko Severi, Robert Mulvaney, and Matthias Bigler
Clim. Past, 16, 1565–1580, https://doi.org/10.5194/cp-16-1565-2020, https://doi.org/10.5194/cp-16-1565-2020, 2020
Short summary
Short summary
We identify signatures of large bipolar volcanic eruptions in Greenland and Antarctic ice cores during the last glacial period, which allows for a precise temporal alignment of the ice cores. Thereby the exact timing of unexplained, abrupt climatic changes occurring during the last glacial period can be determined in a global context. The study thus provides a step towards a full understanding of elements of the climate system that may also play an important role in the future.
Ashley Dinauer, Florian Adolphi, and Fortunat Joos
Clim. Past, 16, 1159–1185, https://doi.org/10.5194/cp-16-1159-2020, https://doi.org/10.5194/cp-16-1159-2020, 2020
Short summary
Short summary
Despite intense focus on the ~ 190 ‰ drop in Δ14C across the deglacial
mystery interval, the specific mechanisms responsible for the apparent Δ14C excess in the glacial atmosphere have received considerably less attention. Sensitivity experiments with the computationally efficient Bern3D Earth system model suggest that our inability to reproduce the elevated Δ14C levels during the last glacial may reflect an underestimation of 14C production and/or a biased-high reconstruction of Δ14C.
Florian Mekhaldi, Markus Czymzik, Florian Adolphi, Jesper Sjolte, Svante Björck, Ala Aldahan, Achim Brauer, Celia Martin-Puertas, Göran Possnert, and Raimund Muscheler
Clim. Past, 16, 1145–1157, https://doi.org/10.5194/cp-16-1145-2020, https://doi.org/10.5194/cp-16-1145-2020, 2020
Short summary
Short summary
Due to chronology uncertainties within paleoclimate archives, it is unclear how climate oscillations from different records relate to one another. By using radionuclides to synchronize Greenland ice cores and a German lake record over 11 000 years, we show that two oscillations observed in these records were not synchronous but terminated and began with the onset of a grand solar minimum. Both this and changes in ocean circulation could have played a role in the two climate oscillations.
Noora Hyttinen, Jonas Elm, Jussi Malila, Silvia M. Calderón, and Nønne L. Prisle
Atmos. Chem. Phys., 20, 5679–5696, https://doi.org/10.5194/acp-20-5679-2020, https://doi.org/10.5194/acp-20-5679-2020, 2020
Short summary
Short summary
Organosulfates have been identified in atmospheric secondary organic aerosol (SOA). The thermodynamic properties of SOA constituents, such as organosulfates, affect the stability and atmospheric impact of the SOA. Here we present estimated solubility, activity, pKa, saturation vapor pressure and Henry's law solubility values for several atmospherically relevant monoterpene- and isoprene-derived organosulfate compounds. These properties can be used, for example, in aerosol process modeling.
Yongyun Hu, Yan Xia, Zhengyu Liu, Yuchen Wang, Zhengyao Lu, and Tao Wang
Clim. Past, 16, 199–209, https://doi.org/10.5194/cp-16-199-2020, https://doi.org/10.5194/cp-16-199-2020, 2020
Short summary
Short summary
The paper shows, using climate simulations, that the Pacific–North American (PNA) teleconnection was distorted or completely broken at the Last Glacial Maximum (LGM). The results suggest that ENSO would have little direct impact on North American climates at the LGM.
Svante Björck, Jesper Sjolte, Karl Ljung, Florian Adolphi, Roger Flower, Rienk H. Smittenberg, Malin E. Kylander, Thomas F. Stocker, Sofia Holmgren, Hui Jiang, Raimund Muscheler, Yamoah K. K. Afrifa, Jayne E. Rattray, and Nathalie Van der Putten
Clim. Past, 15, 1939–1958, https://doi.org/10.5194/cp-15-1939-2019, https://doi.org/10.5194/cp-15-1939-2019, 2019
Short summary
Short summary
Southern Hemisphere westerlies play a key role in regulating global climate. A lake sediment record on a mid-South Atlantic island shows changes in the westerlies and hydroclimate 36.4–18.6 ka. Before 31 ka the westerlies shifted in concert with the bipolar seesaw mechanism in a fairly warm climate, followed by southerly westerlies and falling temperatures. After 27.5 ka temperatures dropped 3 °C with drier conditions and with shifting westerlies possibly triggering the variable LGM CO2 levels.
Tobias Erhardt, Emilie Capron, Sune Olander Rasmussen, Simon Schüpbach, Matthias Bigler, Florian Adolphi, and Hubertus Fischer
Clim. Past, 15, 811–825, https://doi.org/10.5194/cp-15-811-2019, https://doi.org/10.5194/cp-15-811-2019, 2019
Short summary
Short summary
The cause of the rapid warming events documented in proxy records across the Northern Hemisphere during the last glacial has been a long-standing puzzle in paleo-climate research. Here, we use high-resolution ice-core data from to cores in Greenland to investigate the progression during the onset of these events on multi-annual timescales to test their plausible triggers. We show that atmospheric circulation changes preceded the warming in Greenland and the collapse of the sea ice by a decade.
Nønne L. Prisle, Jack J. Lin, Sara Purdue, Haisheng Lin, J. Carson Meredith, and Athanasios Nenes
Atmos. Chem. Phys., 19, 4741–4761, https://doi.org/10.5194/acp-19-4741-2019, https://doi.org/10.5194/acp-19-4741-2019, 2019
Short summary
Short summary
We measure surface activity and cloud-forming potential of pollenkitt, an organic mixture coating pollen grains. Cloud droplet formation is affected through both surface tension and bulk depletion, with a consistent particle size-dependent signature. We observe nonideal solution effects in pollenkitt mixtures with ammonium sulfate salt. Our results suggest sensitivity of general water interactions, including cloud formation by pollen and their fragments, to both atmospheric humidity and aging.
Michael Boy, Erik S. Thomson, Juan-C. Acosta Navarro, Olafur Arnalds, Ekaterina Batchvarova, Jaana Bäck, Frank Berninger, Merete Bilde, Zoé Brasseur, Pavla Dagsson-Waldhauserova, Dimitri Castarède, Maryam Dalirian, Gerrit de Leeuw, Monika Dragosics, Ella-Maria Duplissy, Jonathan Duplissy, Annica M. L. Ekman, Keyan Fang, Jean-Charles Gallet, Marianne Glasius, Sven-Erik Gryning, Henrik Grythe, Hans-Christen Hansson, Margareta Hansson, Elisabeth Isaksson, Trond Iversen, Ingibjorg Jonsdottir, Ville Kasurinen, Alf Kirkevåg, Atte Korhola, Radovan Krejci, Jon Egill Kristjansson, Hanna K. Lappalainen, Antti Lauri, Matti Leppäranta, Heikki Lihavainen, Risto Makkonen, Andreas Massling, Outi Meinander, E. Douglas Nilsson, Haraldur Olafsson, Jan B. C. Pettersson, Nønne L. Prisle, Ilona Riipinen, Pontus Roldin, Meri Ruppel, Matthew Salter, Maria Sand, Øyvind Seland, Heikki Seppä, Henrik Skov, Joana Soares, Andreas Stohl, Johan Ström, Jonas Svensson, Erik Swietlicki, Ksenia Tabakova, Throstur Thorsteinsson, Aki Virkkula, Gesa A. Weyhenmeyer, Yusheng Wu, Paul Zieger, and Markku Kulmala
Atmos. Chem. Phys., 19, 2015–2061, https://doi.org/10.5194/acp-19-2015-2019, https://doi.org/10.5194/acp-19-2015-2019, 2019
Short summary
Short summary
The Nordic Centre of Excellence CRAICC (Cryosphere–Atmosphere Interactions in a Changing Arctic Climate), funded by NordForsk in the years 2011–2016, is the largest joint Nordic research and innovation initiative to date and aimed to strengthen research and innovation regarding climate change issues in the Nordic region. The paper presents an overview of the main scientific topics investigated and provides a state-of-the-art comprehensive summary of what has been achieved in CRAICC.
Theo Kurtén, Noora Hyttinen, Emma Louise D'Ambro, Joel Thornton, and Nønne Lyng Prisle
Atmos. Chem. Phys., 18, 17589–17600, https://doi.org/10.5194/acp-18-17589-2018, https://doi.org/10.5194/acp-18-17589-2018, 2018
Short summary
Short summary
We use COSMO-RS to compute saturation vapor pressures for two products of isoprene photo-oxidation and compare the results to measurements. COSMO-RS is an attractive option for calculating properties of molecules, as it is based on quantum mechanics and requires few fitting parameters. However, we show that the default implementation of this method suffers from errors related to both conformational sampling and intramolecular hydrogen bonding. We propose solutions to these problems.
Florian Adolphi, Christopher Bronk Ramsey, Tobias Erhardt, R. Lawrence Edwards, Hai Cheng, Chris S. M. Turney, Alan Cooper, Anders Svensson, Sune O. Rasmussen, Hubertus Fischer, and Raimund Muscheler
Clim. Past, 14, 1755–1781, https://doi.org/10.5194/cp-14-1755-2018, https://doi.org/10.5194/cp-14-1755-2018, 2018
Short summary
Short summary
The last glacial period was characterized by a number of rapid climate changes seen, for example, as abrupt warmings in Greenland and changes in monsoon rainfall intensity. However, due to chronological uncertainties it is challenging to know how tightly coupled these changes were. Here we exploit cosmogenic signals caused by changes in the Sun and Earth magnetic fields to link different climate archives and improve our understanding of the dynamics of abrupt climate change.
Mousong Wu, Per-Erik Jansson, Jingwei Wu, Xiao Tan, Kang Wang, Peng Chen, and Jiesheng Huang
Hydrol. Earth Syst. Sci. Discuss., https://doi.org/10.5194/hess-2018-466, https://doi.org/10.5194/hess-2018-466, 2018
Revised manuscript not accepted
Jesper Sjolte, Christophe Sturm, Florian Adolphi, Bo M. Vinther, Martin Werner, Gerrit Lohmann, and Raimund Muscheler
Clim. Past, 14, 1179–1194, https://doi.org/10.5194/cp-14-1179-2018, https://doi.org/10.5194/cp-14-1179-2018, 2018
Short summary
Short summary
Tropical volcanic eruptions and variations in solar activity have been suggested to influence the strength of westerly winds across the North Atlantic. We use Greenland ice core records together with a climate model simulation, and find stronger westerly winds for five winters following tropical volcanic eruptions. We see a delayed response to solar activity of 5 years, and the response to solar minima corresponds well to the cooling pattern during the period known as the Little Ice Age.
Minjie Zheng, Jesper Sjolte, Florian Adolphi, Bo Møllesøe Vinther, Hans Christian Steen-Larsen, Trevor James Popp, and Raimund Muscheler
Clim. Past, 14, 1067–1078, https://doi.org/10.5194/cp-14-1067-2018, https://doi.org/10.5194/cp-14-1067-2018, 2018
Short summary
Short summary
We show the seasonal δ18O data from the NEEM site in northwestern Greenland over the last 150 years. We found that the NEEM summer δ18O signal correlates well with summer temperature in western coastal Greenland, while the NEEM winter δ18O signal correlates well with sea ice concentration in Baffin Bay. In contrast with the winter δ18O data from central/southern Greenland, we find no linkage of NEEM winter δ18O to winter NAO.
Markus Czymzik, Raimund Muscheler, Florian Adolphi, Florian Mekhaldi, Nadine Dräger, Florian Ott, Michał Słowinski, Mirosław Błaszkiewicz, Ala Aldahan, Göran Possnert, and Achim Brauer
Clim. Past, 14, 687–696, https://doi.org/10.5194/cp-14-687-2018, https://doi.org/10.5194/cp-14-687-2018, 2018
Short summary
Short summary
Our results provide a proof of concept for facilitating 10Be in varved lake sediments as a novel synchronization tool required for investigating leads and lags of proxy responses to climate variability. They also point to some limitations of 10Be in these archives mainly connected to in-lake sediment resuspension processes.
Johann H. Jungclaus, Edouard Bard, Mélanie Baroni, Pascale Braconnot, Jian Cao, Louise P. Chini, Tania Egorova, Michael Evans, J. Fidel González-Rouco, Hugues Goosse, George C. Hurtt, Fortunat Joos, Jed O. Kaplan, Myriam Khodri, Kees Klein Goldewijk, Natalie Krivova, Allegra N. LeGrande, Stephan J. Lorenz, Jürg Luterbacher, Wenmin Man, Amanda C. Maycock, Malte Meinshausen, Anders Moberg, Raimund Muscheler, Christoph Nehrbass-Ahles, Bette I. Otto-Bliesner, Steven J. Phipps, Julia Pongratz, Eugene Rozanov, Gavin A. Schmidt, Hauke Schmidt, Werner Schmutz, Andrew Schurer, Alexander I. Shapiro, Michael Sigl, Jason E. Smerdon, Sami K. Solanki, Claudia Timmreck, Matthew Toohey, Ilya G. Usoskin, Sebastian Wagner, Chi-Ju Wu, Kok Leng Yeo, Davide Zanchettin, Qiong Zhang, and Eduardo Zorita
Geosci. Model Dev., 10, 4005–4033, https://doi.org/10.5194/gmd-10-4005-2017, https://doi.org/10.5194/gmd-10-4005-2017, 2017
Short summary
Short summary
Climate model simulations covering the last millennium provide context for the evolution of the modern climate and for the expected changes during the coming centuries. They can help identify plausible mechanisms underlying palaeoclimatic reconstructions. Here, we describe the forcing boundary conditions and the experimental protocol for simulations covering the pre-industrial millennium. We describe the PMIP4 past1000 simulations as contributions to CMIP6 and additional sensitivity experiments.
Hyun-Deok Choi, Hongyu Liu, James H. Crawford, David B. Considine, Dale J. Allen, Bryan N. Duncan, Larry W. Horowitz, Jose M. Rodriguez, Susan E. Strahan, Lin Zhang, Xiong Liu, Megan R. Damon, and Stephen D. Steenrod
Atmos. Chem. Phys., 17, 8429–8452, https://doi.org/10.5194/acp-17-8429-2017, https://doi.org/10.5194/acp-17-8429-2017, 2017
Short summary
Short summary
We evaluate global ozone–carbon monoxide (O3–CO) correlations in a chemistry and transport model during July–August with TES-Aura satellite observations and examine the sensitivity of model simulations to input meteorological data and emissions. Results show that O3–CO correlations may be used effectively to constrain the sources of regional tropospheric O3 in global 3-D models, especially for those regions where convective transport of pollution plays an important role.
Juan Hong, Mikko Äijälä, Silja A. K. Häme, Liqing Hao, Jonathan Duplissy, Liine M. Heikkinen, Wei Nie, Jyri Mikkilä, Markku Kulmala, Nønne L. Prisle, Annele Virtanen, Mikael Ehn, Pauli Paasonen, Douglas R. Worsnop, Ilona Riipinen, Tuukka Petäjä, and Veli-Matti Kerminen
Atmos. Chem. Phys., 17, 4387–4399, https://doi.org/10.5194/acp-17-4387-2017, https://doi.org/10.5194/acp-17-4387-2017, 2017
Short summary
Short summary
Estimates of volatility of secondary organic aerosols was characterized in a boreal forest environment of Hyytiälä, southern Finland. This was done by interpreting field measurements using a volatility tandem differential mobility analyzer (VTDMA) with a kinetic evaporation model and by applying positive matrix factorization (PMF) to high-resolution aerosol mass spectrometer data. About 16 % of the variation can be explained by the linear regression between the results from these two methods.
Erika Brattich, Hongyu Liu, Laura Tositti, David B. Considine, and James H. Crawford
Atmos. Chem. Phys., 17, 1061–1080, https://doi.org/10.5194/acp-17-1061-2017, https://doi.org/10.5194/acp-17-1061-2017, 2017
Short summary
Short summary
We apply the GMI chemistry and transport model to simulate the seasonal variations of two radionuclide aerosol tracers (terrigenous 210Pb and cosmogenic 7Be) at the WMO-GAW station of Mt. Cimone during 2005, with an aim to understand the roles of transport and precipitation scavenging processes in controlling their seasonality. Results show a dominant role of precipitation scavenging in controlling the seasonality of 210Pb and 7Be concentrations at Mt. Cimone.
Zhengyao Lu, Zhengyu Liu, Guangshan Chen, and Jian Guan
Clim. Past Discuss., https://doi.org/10.5194/cp-2016-128, https://doi.org/10.5194/cp-2016-128, 2017
Revised manuscript not accepted
Short summary
Short summary
We use complex climate model simulations to study how the intensity of El Niño-Southern Oscillation (ENSO) changed for the last 300 thousand years. We consider external climatic forcings like orbital variations, greenhouse gases and ice-sheets. We find that orbital forcing dominates slow ENSO evolution by modulating the change of the coupled ocean-atmosphere instability, while the effects of GHGs and ice-sheet forcing tend to compensate each other.
Mousong Wu, Per-Erik Jansson, Xiao Tan, Jiesheng Huang, and Jingwei Wu
Hydrol. Earth Syst. Sci. Discuss., https://doi.org/10.5194/hess-2016-507, https://doi.org/10.5194/hess-2016-507, 2016
Revised manuscript not accepted
Hongyu Liu, David B. Considine, Larry W. Horowitz, James H. Crawford, Jose M. Rodriguez, Susan E. Strahan, Megan R. Damon, Stephen D. Steenrod, Xiaojing Xu, Jules Kouatchou, Claire Carouge, and Robert M. Yantosca
Atmos. Chem. Phys., 16, 4641–4659, https://doi.org/10.5194/acp-16-4641-2016, https://doi.org/10.5194/acp-16-4641-2016, 2016
Short summary
Short summary
We assess the utility of cosmogenic beryllium-7, a natural aerosol tracer, for evaluating cross-tropopause transport in global models. We show that model excessive cross-tropopause transport of beryllium-7 corresponds to overestimated stratospheric contribution to tropospheric ozone. We conclude that the observational constraints for beryllium-7 and observed beryllium-7 total deposition fluxes can be used routinely as a first-order assessment of cross-tropopause transport in global models.
Markus Czymzik, Raimund Muscheler, and Achim Brauer
Clim. Past, 12, 799–805, https://doi.org/10.5194/cp-12-799-2016, https://doi.org/10.5194/cp-12-799-2016, 2016
Short summary
Short summary
Integrating discharge data of the River Ammer back to 1926 and a 5500-year flood layer record from an annually laminated sediment core of the downstream Ammersee allowed investigating changes in the frequency of major floods in Central Europe on interannual to multi-centennial timescales. Significant correlations between flood frequency variations in both archives and changes in the activity of the Sun suggest a solar influence on the frequency of these hydrometeorological extremes.
Michael Sigl, Tyler J. Fudge, Mai Winstrup, Jihong Cole-Dai, David Ferris, Joseph R. McConnell, Ken C. Taylor, Kees C. Welten, Thomas E. Woodruff, Florian Adolphi, Marion Bisiaux, Edward J. Brook, Christo Buizert, Marc W. Caffee, Nelia W. Dunbar, Ross Edwards, Lei Geng, Nels Iverson, Bess Koffman, Lawrence Layman, Olivia J. Maselli, Kenneth McGwire, Raimund Muscheler, Kunihiko Nishiizumi, Daniel R. Pasteris, Rachael H. Rhodes, and Todd A. Sowers
Clim. Past, 12, 769–786, https://doi.org/10.5194/cp-12-769-2016, https://doi.org/10.5194/cp-12-769-2016, 2016
Short summary
Short summary
Here we present a chronology (WD2014) for the upper part (0–2850 m; 31.2 ka BP) of the West Antarctic Ice Sheet (WAIS) Divide ice core, which is based on layer counting of distinctive annual cycles preserved in the elemental, chemical and electrical conductivity records. We validated the chronology by comparing it to independent high-accuracy, absolutely dated chronologies. Given its demonstrated high accuracy, WD2014 can become a reference chronology for the Southern Hemisphere.
Bjarke Mølgaard, Jarno Vanhatalo, Pasi P. Aalto, Nønne L. Prisle, and Kaarle Hämeri
Atmos. Meas. Tech., 9, 741–751, https://doi.org/10.5194/amt-9-741-2016, https://doi.org/10.5194/amt-9-741-2016, 2016
Short summary
Short summary
We have improved the reliability of submicron aerosol particle size distributions measured in urban locations. This improvement was obtained by processing the data in a new way and avoiding a problematic assumption of a stationary aerosol during each size distribution measurement.
F. Adolphi and R. Muscheler
Clim. Past, 12, 15–30, https://doi.org/10.5194/cp-12-15-2016, https://doi.org/10.5194/cp-12-15-2016, 2016
Short summary
Short summary
Here we employ common variations in tree-ring 14C and Greenland ice core 10Be records to synchronize the Greenland ice core (GICC05) and the radiocarbon (IntCal13) timescale over the Holocene. We propose a transfer function between both timescales that allows continuous comparisons between radiocarbon dated and ice core climate records at unprecedented chronological precision.
J. Huang, H. Liu, J. H. Crawford, C. Chan, D. B. Considine, Y. Zhang, X. Zheng, C. Zhao, V. Thouret, S. J. Oltmans, S. C. Liu, D. B. A. Jones, S. D. Steenrod, and M. R. Damon
Atmos. Chem. Phys., 15, 5161–5179, https://doi.org/10.5194/acp-15-5161-2015, https://doi.org/10.5194/acp-15-5161-2015, 2015
Short summary
Short summary
High ozone concentrations (up to 94.7ppbv) were frequently observed at an altitude of ~1.5--2km over Beijing during April--May 2005. Ozone due to Asian anthropogenic pollution made major contributions to the observed ozone enhancements. These enhancements typically occurred under southerly wind and warmer conditions. An earlier onset of the Asian summer monsoon would cause more ozone enhancement events in the lower troposphere over the North China Plain in late spring and early summer.
H. Vuollekoski, M. Vogt, V. A. Sinclair, J. Duplissy, H. Järvinen, E.-M. Kyrö, R. Makkonen, T. Petäjä, N. L. Prisle, P. Räisänen, M. Sipilä, J. Ylhäisi, and M. Kulmala
Hydrol. Earth Syst. Sci., 19, 601–613, https://doi.org/10.5194/hess-19-601-2015, https://doi.org/10.5194/hess-19-601-2015, 2015
Short summary
Short summary
The global potential for collecting usable water from dew on an
artificial collector sheet was investigated by utilising 34 years of
meteorological reanalysis data as input to a dew formation model. Continental dew formation was found to be frequent and common, but daily yields were
mostly below 0.1mm.
M. Paramonov, P. P. Aalto, A. Asmi, N. Prisle, V.-M. Kerminen, M. Kulmala, and T. Petäjä
Atmos. Chem. Phys., 13, 10285–10301, https://doi.org/10.5194/acp-13-10285-2013, https://doi.org/10.5194/acp-13-10285-2013, 2013
N. L. Prisle, N. Ottosson, G. Öhrwall, J. Söderström, M. Dal Maso, and O. Björneholm
Atmos. Chem. Phys., 12, 12227–12242, https://doi.org/10.5194/acp-12-12227-2012, https://doi.org/10.5194/acp-12-12227-2012, 2012
Related subject area
Atmospheric sciences
tobac v1.5: introducing fast 3D tracking, splits and mergers, and other enhancements for identifying and analysing meteorological phenomena
Merged Observatory Data Files (MODFs): an integrated observational data product supporting process-oriented investigations and diagnostics
Simulation of marine stratocumulus using the super-droplet method: numerical convergence and comparison to a double-moment bulk scheme using SCALE-SDM 5.2.6-2.3.1
WRF-Comfort: simulating microscale variability in outdoor heat stress at the city scale with a mesoscale model
Representing effects of surface heterogeneity in a multi-plume eddy diffusivity mass flux boundary layer parameterization
Can TROPOMI NO2 satellite data be used to track the drop in and resurgence of NOx emissions in Germany between 2019–2021 using the multi-source plume method (MSPM)?
A spatiotemporally separated framework for reconstructing the sources of atmospheric radionuclide releases
A parameterization scheme for the floating wind farm in a coupled atmosphere–wave model (COAWST v3.7)
RoadSurf 1.1: open-source road weather model library
Calibrating and validating the Integrated Valuation of Ecosystem Services and Tradeoffs (InVEST) urban cooling model: case studies in France and the United States
The ddeq Python library for point source quantification from remote sensing images (version 1.0)
Incorporating Oxygen Isotopes of Oxidized Reactive Nitrogen in the Regional Atmospheric Chemistry Mechanism, version 2 (ICOIN-RACM2)
A general comprehensive evaluation method for cross-scale precipitation forecasts
Implementation of a Simple Actuator Disk for Large-Eddy Simulation in the Weather Research and Forecasting Model (WRF-SADLES v1.2) for wind turbine wake simulation
WRF-PDAF v1.0: implementation and application of an online localized ensemble data assimilation framework
Implementation and evaluation of diabatic advection in the Lagrangian transport model MPTRAC 2.6
An improved and extended parameterization of the CO2 15 µm cooling in the middle and upper atmosphere (CO2_cool_fort-1.0)
Development of a multiphase chemical mechanism to improve secondary organic aerosol formation in CAABA/MECCA (version 4.7.0)
Application of regional meteorology and air quality models based on the microprocessor without interlocked piped stages (MIPS) and LoongArch CPU platforms
Investigating ground-level ozone pollution in semi-arid and arid regions of Arizona using WRF-Chem v4.4 modeling
An objective identification technique for potential vorticity structures associated with African easterly waves
Importance of microphysical settings for climate forcing by stratospheric SO2 injections as modeled by SOCOL-AERv2
Assessment of surface ozone products from downscaled CAMS reanalysis and CAMS daily forecast using urban air quality monitoring stations in Iran
Open boundary conditions for atmospheric large-eddy simulations and their implementation in DALES4.4
Efficient and stable coupling of the SuperdropNet deep-learning-based cloud microphysics (v0.1.0) with the ICON climate and weather model (v2.6.5)
Three-dimensional variational assimilation with a multivariate background error covariance for the Model for Prediction Across Scales – Atmosphere with the Joint Effort for Data assimilation Integration (JEDI-MPAS 2.0.0-beta)
FUME 2.0 – Flexible Universal processor for Modeling Emissions
DEUCE v1.0: a neural network for probabilistic precipitation nowcasting with aleatoric and epistemic uncertainties
Evaluation of multi-season convection-permitting atmosphere – mixed-layer ocean simulations of the Maritime Continent
Investigating the impact of coupling HARMONIE-WINS50 (cy43) meteorology to LOTOS-EUROS (v2.2.002) on a simulation of NO2 concentrations over the Netherlands
Balloon drift estimation and improved position estimates for radiosondes
Emission ensemble approach to improve the development of multi-scale emission inventories
What is the relative impact of nudging and online coupling on meteorological variables, pollutant concentrations and aerosol optical properties?
Diagnosing drivers of PM2.5 simulation biases in China from meteorology, chemical composition, and emission sources using an efficient machine learning method
Validation and analysis of the Polair3D v1.11 chemical transport model over Quebec
Assimilation of GNSS tropospheric gradients into the Weather Research and Forecasting (WRF) model version 4.4.1
Identifying atmospheric rivers and their poleward latent heat transport with generalizable neural networks: ARCNNv1
Assessing acetone for the GISS ModelE2.1 Earth system model
Bergen metrics: composite error metrics for assessing performance of climate models using EURO-CORDEX simulations
A dynamic approach to three-dimensional radiative transfer in subkilometer-scale numerical weather prediction models: the dynamic TenStream solver v1.0
Evaluation and development of surface layer scheme representation of temperature inversions over boreal forests in Arctic wintertime conditions
Modelling wind farm effects in HARMONIE–AROME (cycle 43.2.2) – Part 1: Implementation and evaluation
Analytical and adaptable initial conditions for dry and moist baroclinic waves in the global hydrostatic model OpenIFS (CY43R3)
Challenges of constructing and selecting the “perfect” boundary conditions for the large-eddy simulation model PALM
Mixed-Precision Computing in the GRIST Dynamical Core for Weather and Climate Modelling
Recent improvements and maximum covariance analysis of aerosol and cloud properties in the EC-Earth3-AerChem model
A machine learning approach for evaluating Southern Ocean cloud radiative biases in a global atmosphere model
Decision Support System version 1.0 (DSS v1.0) for air quality management in Delhi, India
How non-equilibrium aerosol chemistry impacts particle acidity: the GMXe AERosol CHEMistry (GMXe–AERCHEM, v1.0) sub-submodel of MESSy
A grid model for vertical correction of precipitable water vapor over the Chinese mainland and surrounding areas using random forest
G. Alexander Sokolowsky, Sean W. Freeman, William K. Jones, Julia Kukulies, Fabian Senf, Peter J. Marinescu, Max Heikenfeld, Kelcy N. Brunner, Eric C. Bruning, Scott M. Collis, Robert C. Jackson, Gabrielle R. Leung, Nils Pfeifer, Bhupendra A. Raut, Stephen M. Saleeby, Philip Stier, and Susan C. van den Heever
Geosci. Model Dev., 17, 5309–5330, https://doi.org/10.5194/gmd-17-5309-2024, https://doi.org/10.5194/gmd-17-5309-2024, 2024
Short summary
Short summary
Building on previous analysis tools developed for atmospheric science, the original release of the Tracking and Object-Based Analysis (tobac) Python package, v1.2, was open-source, modular, and insensitive to the type of gridded input data. Here, we present the latest version of tobac, v1.5, which substantially improves scientific capabilities and computational efficiency from the previous version. These enhancements permit new uses for tobac in atmospheric science and potentially other fields.
Taneil Uttal, Leslie M. Hartten, Siri Jodha Khalsa, Barbara Casati, Gunilla Svensson, Jonathan Day, Jareth Holt, Elena Akish, Sara Morris, Ewan O'Connor, Roberta Pirazzini, Laura X. Huang, Robert Crawford, Zen Mariani, Øystein Godøy, Johanna A. K. Tjernström, Giri Prakash, Nicki Hickmon, Marion Maturilli, and Christopher J. Cox
Geosci. Model Dev., 17, 5225–5247, https://doi.org/10.5194/gmd-17-5225-2024, https://doi.org/10.5194/gmd-17-5225-2024, 2024
Short summary
Short summary
A Merged Observatory Data File (MODF) format to systematically collate complex atmosphere, ocean, and terrestrial data sets collected by multiple instruments during field campaigns is presented. The MODF format is also designed to be applied to model output data, yielding format-matching Merged Model Data Files (MMDFs). MODFs plus MMDFs will augment and accelerate the synergistic use of model results with observational data to increase understanding and predictive skill.
Chongzhi Yin, Shin-ichiro Shima, Lulin Xue, and Chunsong Lu
Geosci. Model Dev., 17, 5167–5189, https://doi.org/10.5194/gmd-17-5167-2024, https://doi.org/10.5194/gmd-17-5167-2024, 2024
Short summary
Short summary
We investigate numerical convergence properties of a particle-based numerical cloud microphysics model (SDM) and a double-moment bulk scheme for simulating a marine stratocumulus case, compare their results with model intercomparison project results, and present possible explanations for the different results of the SDM and the bulk scheme. Aerosol processes can be accurately simulated using SDM, and this may be an important factor affecting the behavior and morphology of marine stratocumulus.
Alberto Martilli, Negin Nazarian, E. Scott Krayenhoff, Jacob Lachapelle, Jiachen Lu, Esther Rivas, Alejandro Rodriguez-Sanchez, Beatriz Sanchez, and José Luis Santiago
Geosci. Model Dev., 17, 5023–5039, https://doi.org/10.5194/gmd-17-5023-2024, https://doi.org/10.5194/gmd-17-5023-2024, 2024
Short summary
Short summary
Here, we present a model that quantifies the thermal stress and its microscale variability at a city scale with a mesoscale model. This tool can have multiple applications, from early warnings of extreme heat to the vulnerable population to the evaluation of the effectiveness of heat mitigation strategies. It is the first model that includes information on microscale variability in a mesoscale model, something that is essential for fully evaluating heat stress.
Nathan P. Arnold
Geosci. Model Dev., 17, 5041–5056, https://doi.org/10.5194/gmd-17-5041-2024, https://doi.org/10.5194/gmd-17-5041-2024, 2024
Short summary
Short summary
Earth system models often represent the land surface at smaller scales than the atmosphere, but surface–atmosphere coupling uses only aggregated surface properties. This study presents a method to allow heterogeneous surface properties to modify boundary layer updrafts. The method is tested in single column experiments. Updraft properties are found to reasonably covary with surface conditions, and simulated boundary layer variability is enhanced over more heterogeneous land surfaces.
Enrico Dammers, Janot Tokaya, Christian Mielke, Kevin Hausmann, Debora Griffin, Chris McLinden, Henk Eskes, and Renske Timmermans
Geosci. Model Dev., 17, 4983–5007, https://doi.org/10.5194/gmd-17-4983-2024, https://doi.org/10.5194/gmd-17-4983-2024, 2024
Short summary
Short summary
Nitrogen dioxide (NOx) is produced by sources such as industry and traffic and is directly linked to negative impacts on health and the environment. The current construction of emission inventories to keep track of NOx emissions is slow and time-consuming. Satellite measurements provide a way to quickly and independently estimate emissions. In this study, we apply a consistent methodology to derive NOx emissions over Germany and illustrate the value of having such a method for fast projections.
Yuhan Xu, Sheng Fang, Xinwen Dong, and Shuhan Zhuang
Geosci. Model Dev., 17, 4961–4982, https://doi.org/10.5194/gmd-17-4961-2024, https://doi.org/10.5194/gmd-17-4961-2024, 2024
Short summary
Short summary
Recent atmospheric radionuclide leakages from unknown sources have posed a new challenge in nuclear emergency assessment. Reconstruction via environmental observations is the only feasible way to identify sources, but simultaneous reconstruction of the source location and release rate yields high uncertainties. We propose a spatiotemporally separated reconstruction strategy that avoids these uncertainties and outperforms state-of-the-art methods with respect to accuracy and uncertainty ranges.
Shaokun Deng, Shengmu Yang, Shengli Chen, Daoyi Chen, Xuefeng Yang, and Shanshan Cui
Geosci. Model Dev., 17, 4891–4909, https://doi.org/10.5194/gmd-17-4891-2024, https://doi.org/10.5194/gmd-17-4891-2024, 2024
Short summary
Short summary
Global offshore wind power development is moving from offshore to deeper waters, where floating offshore wind turbines have an advantage over bottom-fixed turbines. However, current wind farm parameterization schemes in mesoscale models are not applicable to floating turbines. We propose a floating wind farm parameterization scheme that accounts for the attenuation of the significant wave height by floating turbines. The results indicate that it has a significant effect on the power output.
Virve Eveliina Karsisto
Geosci. Model Dev., 17, 4837–4853, https://doi.org/10.5194/gmd-17-4837-2024, https://doi.org/10.5194/gmd-17-4837-2024, 2024
Short summary
Short summary
RoadSurf is an open-source library that contains functions from the Finnish Meteorological Institute’s road weather model. The evaluation of the library shows that it is well suited for making road surface temperature forecasts. The evaluation was done by making forecasts for about 400 road weather stations in Finland with the library. Accurate forecasts help road authorities perform salting and plowing operations at the right time and keep roads safe for drivers.
Perrine Hamel, Martí Bosch, Léa Tardieu, Aude Lemonsu, Cécile de Munck, Chris Nootenboom, Vincent Viguié, Eric Lonsdorf, James A. Douglass, and Richard P. Sharp
Geosci. Model Dev., 17, 4755–4771, https://doi.org/10.5194/gmd-17-4755-2024, https://doi.org/10.5194/gmd-17-4755-2024, 2024
Short summary
Short summary
The InVEST Urban Cooling model estimates the cooling effect of vegetation in cities. We further developed an algorithm to facilitate model calibration and evaluation. Applying the algorithm to case studies in France and in the United States, we found that nighttime air temperature estimates compare well with reference datasets. Estimated change in temperature from a land cover scenario compares well with an alternative model estimate, supporting the use of the model for urban planning decisions.
Gerrit Kuhlmann, Erik Koene, Sandro Meier, Diego Santaren, Grégoire Broquet, Frédéric Chevallier, Janne Hakkarainen, Janne Nurmela, Laia Amorós, Johanna Tamminen, and Dominik Brunner
Geosci. Model Dev., 17, 4773–4789, https://doi.org/10.5194/gmd-17-4773-2024, https://doi.org/10.5194/gmd-17-4773-2024, 2024
Short summary
Short summary
We present a Python software library for data-driven emission quantification (ddeq). It can be used to determine the emissions of hot spots (cities, power plants and industry) from remote sensing images using different methods. ddeq can be extended for new datasets and methods, providing a powerful community tool for users and developers. The application of the methods is shown using Jupyter notebooks included in the library.
Wendell W. Walters, Masayuki Takeuchi, Nga L. Ng, and Meredith G. Hastings
Geosci. Model Dev., 17, 4673–4687, https://doi.org/10.5194/gmd-17-4673-2024, https://doi.org/10.5194/gmd-17-4673-2024, 2024
Short summary
Short summary
The study introduces a novel chemical mechanism for explicitly tracking oxygen isotope transfer in oxidized reactive nitrogen and odd oxygen using the Regional Atmospheric Chemistry Mechanism, version 2. This model enhances our ability to simulate and compare oxygen isotope compositions of reactive nitrogen, revealing insights into oxidation chemistry. The approach shows promise for improving atmospheric chemistry models and tropospheric oxidation capacity predictions.
Bing Zhang, Mingjian Zeng, Anning Huang, Zhengkun Qin, Couhua Liu, Wenru Shi, Xin Li, Kefeng Zhu, Chunlei Gu, and Jialing Zhou
Geosci. Model Dev., 17, 4579–4601, https://doi.org/10.5194/gmd-17-4579-2024, https://doi.org/10.5194/gmd-17-4579-2024, 2024
Short summary
Short summary
By directly analyzing the proximity of precipitation forecasts and observations, a precipitation accuracy score (PAS) method was constructed. This method does not utilize a traditional contingency-table-based classification verification; however, it can replace the threat score (TS), equitable threat score (ETS), and other skill score methods, and it can be used to calculate the accuracy of numerical models or quantitative precipitation forecasts.
Hai Bui, Mostafa Bakhoday-Paskyabi, and Mohammadreza Mohammadpour-Penchah
Geosci. Model Dev., 17, 4447–4465, https://doi.org/10.5194/gmd-17-4447-2024, https://doi.org/10.5194/gmd-17-4447-2024, 2024
Short summary
Short summary
We developed a new wind turbine wake model, the Simple Actuator Disc for Large Eddy Simulation (SADLES), integrated with the widely used Weather Research and Forecasting (WRF) model. WRF-SADLES accurately simulates wind turbine wakes at resolutions of a few dozen meters, aligning well with idealized simulations and observational measurements. This makes WRF-SADLES a promising tool for wind energy research, offering a balance between accuracy, computational efficiency, and ease of implementation.
Changliang Shao and Lars Nerger
Geosci. Model Dev., 17, 4433–4445, https://doi.org/10.5194/gmd-17-4433-2024, https://doi.org/10.5194/gmd-17-4433-2024, 2024
Short summary
Short summary
This paper introduces and evaluates WRF-PDAF, a fully online-coupled ensemble data assimilation (DA) system. A key advantage of the WRF-PDAF configuration is its ability to concurrently integrate all ensemble states, eliminating the need for time-consuming distribution and collection of ensembles during the coupling communication. The extra time required for DA amounts to only 20.6 % per cycle. Twin experiment results underscore the effectiveness of the WRF-PDAF system.
Jan Clemens, Lars Hoffmann, Bärbel Vogel, Sabine Grießbach, and Nicole Thomas
Geosci. Model Dev., 17, 4467–4493, https://doi.org/10.5194/gmd-17-4467-2024, https://doi.org/10.5194/gmd-17-4467-2024, 2024
Short summary
Short summary
Lagrangian transport models simulate the transport of air masses in the atmosphere. For example, one model (CLaMS) is well suited to calculating transport as it uses a special coordinate system and special vertical wind. However, it only runs inefficiently on modern supercomputers. Hence, we have implemented the benefits of CLaMS into a new model (MPTRAC), which is already highly efficient on modern supercomputers. Finally, in extensive tests, we showed that CLaMS and MPTRAC agree very well.
Manuel López-Puertas, Federico Fabiano, Victor Fomichev, Bernd Funke, and Daniel R. Marsh
Geosci. Model Dev., 17, 4401–4432, https://doi.org/10.5194/gmd-17-4401-2024, https://doi.org/10.5194/gmd-17-4401-2024, 2024
Short summary
Short summary
The radiative infrared cooling of CO2 in the middle atmosphere is crucial for computing its thermal structure. It requires one however to include non-local thermodynamic equilibrium processes which are computationally very expensive, which cannot be afforded by climate models. In this work, we present an updated, efficient, accurate and very fast (~50 µs) parameterization of that cooling able to cope with CO2 abundances from half the pre-industrial values to 10 times the current abundance.
Felix Wieser, Rolf Sander, Changmin Cho, Hendrik Fuchs, Thorsten Hohaus, Anna Novelli, Ralf Tillmann, and Domenico Taraborrelli
Geosci. Model Dev., 17, 4311–4330, https://doi.org/10.5194/gmd-17-4311-2024, https://doi.org/10.5194/gmd-17-4311-2024, 2024
Short summary
Short summary
The chemistry scheme of the atmospheric box model CAABA/MECCA is expanded to achieve an improved aerosol formation from emitted organic compounds. In addition to newly added reactions, temperature-dependent partitioning of all new species between the gas and aqueous phases is estimated and included in the pre-existing scheme. Sensitivity runs show an overestimation of key compounds from isoprene, which can be explained by a lack of aqueous-phase degradation reactions and box model limitations.
Zehua Bai, Qizhong Wu, Kai Cao, Yiming Sun, and Huaqiong Cheng
Geosci. Model Dev., 17, 4383–4399, https://doi.org/10.5194/gmd-17-4383-2024, https://doi.org/10.5194/gmd-17-4383-2024, 2024
Short summary
Short summary
There is relatively limited research on the application of scientific computing on RISC CPU platforms. The MIPS architecture CPUs, a type of RISC CPUs, have distinct advantages in energy efficiency and scalability. The air quality modeling system can run stably on the MIPS and LoongArch platforms, and the experiment results verify the stability of scientific computing on the platforms. The work provides a technical foundation for the scientific application based on MIPS and LoongArch.
Yafang Guo, Chayan Roychoudhury, Mohammad Amin Mirrezaei, Rajesh Kumar, Armin Sorooshian, and Avelino F. Arellano
Geosci. Model Dev., 17, 4331–4353, https://doi.org/10.5194/gmd-17-4331-2024, https://doi.org/10.5194/gmd-17-4331-2024, 2024
Short summary
Short summary
This research focuses on surface ozone (O3) pollution in Arizona, a historically air-quality-challenged arid and semi-arid region in the US. The unique characteristics of this kind of region, e.g., intense heat, minimal moisture, and persistent desert shrubs, play a vital role in comprehending O3 exceedances. Using the WRF-Chem model, we analyzed O3 levels in the pre-monsoon month, revealing the model's skill in capturing diurnal and MDA8 O3 levels.
Christoph Fischer, Andreas H. Fink, Elmar Schömer, Marc Rautenhaus, and Michael Riemer
Geosci. Model Dev., 17, 4213–4228, https://doi.org/10.5194/gmd-17-4213-2024, https://doi.org/10.5194/gmd-17-4213-2024, 2024
Short summary
Short summary
This study presents a method for identifying and tracking 3-D potential vorticity structures within African easterly waves (AEWs). Each identified structure is characterized by descriptors, including its 3-D position and orientation, which have been validated through composite comparisons. A trough-centric perspective on the descriptors reveals the evolution and distinct characteristics of AEWs. These descriptors serve as valuable statistical inputs for the study of AEW-related phenomena.
Sandro Vattioni, Andrea Stenke, Beiping Luo, Gabriel Chiodo, Timofei Sukhodolov, Elia Wunderlin, and Thomas Peter
Geosci. Model Dev., 17, 4181–4197, https://doi.org/10.5194/gmd-17-4181-2024, https://doi.org/10.5194/gmd-17-4181-2024, 2024
Short summary
Short summary
We investigate the sensitivity of aerosol size distributions in the presence of strong SO2 injections for climate interventions or after volcanic eruptions to the call sequence and frequency of the routines for nucleation and condensation in sectional aerosol models with operator splitting. Using the aerosol–chemistry–climate model SOCOL-AERv2, we show that the radiative and chemical outputs are sensitive to these settings at high H2SO4 supersaturations and how to obtain reliable results.
Najmeh Kaffashzadeh and Abbas-Ali Aliakbari Bidokhti
Geosci. Model Dev., 17, 4155–4179, https://doi.org/10.5194/gmd-17-4155-2024, https://doi.org/10.5194/gmd-17-4155-2024, 2024
Short summary
Short summary
This paper assesses the capability of two state-of-the-art global datasets in simulating surface ozone over Iran using a new methodology. It is found that the global model data need to be downscaled for regulatory purposes or policy applications at local scales. The method can be useful not only for the evaluation but also for the prediction of other chemical species, such as aerosols.
Franciscus Liqui Lung, Christian Jakob, A. Pier Siebesma, and Fredrik Jansson
Geosci. Model Dev., 17, 4053–4076, https://doi.org/10.5194/gmd-17-4053-2024, https://doi.org/10.5194/gmd-17-4053-2024, 2024
Short summary
Short summary
Traditionally, high-resolution atmospheric models employ periodic boundary conditions, which limit simulations to domains without horizontal variations. In this research open boundary conditions are developed to replace the periodic boundary conditions. The implementation is tested in a controlled setup, and the results show minimal disturbances. Using these boundary conditions, high-resolution models can be forced by a coarser model to study atmospheric phenomena in realistic background states.
Caroline Arnold, Shivani Sharma, Tobias Weigel, and David S. Greenberg
Geosci. Model Dev., 17, 4017–4029, https://doi.org/10.5194/gmd-17-4017-2024, https://doi.org/10.5194/gmd-17-4017-2024, 2024
Short summary
Short summary
In atmospheric models, rain formation is simplified to be computationally efficient. We trained a machine learning model, SuperdropNet, to emulate warm-rain formation based on super-droplet simulations. Here, we couple SuperdropNet with an atmospheric model in a warm-bubble experiment and find that the coupled simulation runs stable and produces reasonable results, making SuperdropNet a viable ML proxy for droplet simulations. We also present a comprehensive benchmark for coupling architectures.
Byoung-Joo Jung, Benjamin Ménétrier, Chris Snyder, Zhiquan Liu, Jonathan J. Guerrette, Junmei Ban, Ivette Hernández Baños, Yonggang G. Yu, and William C. Skamarock
Geosci. Model Dev., 17, 3879–3895, https://doi.org/10.5194/gmd-17-3879-2024, https://doi.org/10.5194/gmd-17-3879-2024, 2024
Short summary
Short summary
We describe the multivariate static background error covariance (B) for the JEDI-MPAS 3D-Var data assimilation system. With tuned B parameters, the multivariate B gives physically balanced analysis increment fields in the single-observation test framework. In the month-long cycling experiment with a global 60 km mesh, 3D-Var with static B performs stably. Due to its simple workflow and minimal computational requirements, JEDI-MPAS 3D-Var can be useful for the research community.
Michal Belda, Nina Benešová, Jaroslav Resler, Peter Huszár, Ondřej Vlček, Pavel Krč, Jan Karlický, Pavel Juruš, and Kryštof Eben
Geosci. Model Dev., 17, 3867–3878, https://doi.org/10.5194/gmd-17-3867-2024, https://doi.org/10.5194/gmd-17-3867-2024, 2024
Short summary
Short summary
For modeling atmospheric chemistry, it is necessary to provide data on emissions of pollutants. These can come from various sources and in various forms, and preprocessing of the data to be ingestible by chemistry models can be quite challenging. We developed the FUME processor to use a database layer that internally transforms all input data into a rigid structure, facilitating further processing to allow for emission processing from the continental to the street scale.
Bent Harnist, Seppo Pulkkinen, and Terhi Mäkinen
Geosci. Model Dev., 17, 3839–3866, https://doi.org/10.5194/gmd-17-3839-2024, https://doi.org/10.5194/gmd-17-3839-2024, 2024
Short summary
Short summary
Probabilistic precipitation nowcasting (local forecasting for 0–6 h) is crucial for reducing damage from events like flash floods. For this goal, we propose the DEUCE neural-network-based model which uses data and model uncertainties to generate an ensemble of potential precipitation development scenarios for the next hour. Trained and evaluated with Finnish precipitation composites, DEUCE was found to produce more skillful and reliable nowcasts than established models.
Emma Howard, Steven Woolnough, Nicholas Klingaman, Daniel Shipley, Claudio Sanchez, Simon C. Peatman, Cathryn E. Birch, and Adrian J. Matthews
Geosci. Model Dev., 17, 3815–3837, https://doi.org/10.5194/gmd-17-3815-2024, https://doi.org/10.5194/gmd-17-3815-2024, 2024
Short summary
Short summary
This paper describes a coupled atmosphere–mixed-layer ocean simulation setup that will be used to study weather processes in Southeast Asia. The set-up has been used to compare high-resolution simulations, which are able to partially resolve storms, to coarser simulations, which cannot. We compare the model performance at representing variability of rainfall and sea surface temperatures across length scales between the coarse and fine models.
Andrés Yarce Botero, Michiel van Weele, Arjo Segers, Pier Siebesma, and Henk Eskes
Geosci. Model Dev., 17, 3765–3781, https://doi.org/10.5194/gmd-17-3765-2024, https://doi.org/10.5194/gmd-17-3765-2024, 2024
Short summary
Short summary
HARMONIE WINS50 reanalysis data with 0.025° × 0.025° resolution from 2019 to 2021 were coupled with the LOTOS-EUROS Chemical Transport Model. HARMONIE and ECMWF meteorology configurations against Cabauw observations (52.0° N, 4.9° W) were evaluated as simulated NO2 concentrations with ground-level sensors. Differences in crucial meteorological input parameters (boundary layer height, vertical diffusion coefficient) between the hydrostatic and non-hydrostatic models were analysed.
Ulrich Voggenberger, Leopold Haimberger, Federico Ambrogi, and Paul Poli
Geosci. Model Dev., 17, 3783–3799, https://doi.org/10.5194/gmd-17-3783-2024, https://doi.org/10.5194/gmd-17-3783-2024, 2024
Short summary
Short summary
This paper presents a method for calculating balloon drift from historical radiosonde ascent data. The drift can reach distances of several hundred kilometres and is often neglected. Verification shows the beneficial impact of the more accurate balloon position on model assimilation. The method is not limited to radiosondes but would also work for dropsondes, ozonesondes, or any other in situ sonde carried by the wind in the pre-GNSS era, provided the necessary information is available.
Philippe Thunis, Jeroen Kuenen, Enrico Pisoni, Bertrand Bessagnet, Manjola Banja, Lech Gawuc, Karol Szymankiewicz, Diego Guizardi, Monica Crippa, Susana Lopez-Aparicio, Marc Guevara, Alexander De Meij, Sabine Schindlbacher, and Alain Clappier
Geosci. Model Dev., 17, 3631–3643, https://doi.org/10.5194/gmd-17-3631-2024, https://doi.org/10.5194/gmd-17-3631-2024, 2024
Short summary
Short summary
An ensemble emission inventory is created with the aim of monitoring the status and progress made with the development of EU-wide inventories. This emission ensemble serves as a common benchmark for the screening and allows for the comparison of more than two inventories at a time. Because the emission “truth” is unknown, the approach does not tell which inventory is the closest to reality, but it identifies inconsistencies that require special attention.
Laurent Menut, Bertrand Bessagnet, Arineh Cholakian, Guillaume Siour, Sylvain Mailler, and Romain Pennel
Geosci. Model Dev., 17, 3645–3665, https://doi.org/10.5194/gmd-17-3645-2024, https://doi.org/10.5194/gmd-17-3645-2024, 2024
Short summary
Short summary
This study is about the modelling of the atmospheric composition in Europe during the summer of 2022, when massive wildfires were observed. It is a sensitivity study dedicated to the relative impacts of two modelling processes that are able to modify the meteorology used for the calculation of the atmospheric chemistry and transport of pollutants.
Shuai Wang, Mengyuan Zhang, Yueqi Gao, Peng Wang, Qingyan Fu, and Hongliang Zhang
Geosci. Model Dev., 17, 3617–3629, https://doi.org/10.5194/gmd-17-3617-2024, https://doi.org/10.5194/gmd-17-3617-2024, 2024
Short summary
Short summary
Numerical models are widely used in air pollution modeling but suffer from significant biases. The machine learning model designed in this study shows high efficiency in identifying such biases. Meteorology (relative humidity and cloud cover), chemical composition (secondary organic components and dust aerosols), and emission sources (residential activities) are diagnosed as the main drivers of bias in modeling PM2.5, a typical air pollutant. The results will help to improve numerical models.
Shoma Yamanouchi, Shayamilla Mahagammulla Gamage, Sara Torbatian, Jad Zalzal, Laura Minet, Audrey Smargiassi, Ying Liu, Ling Liu, Forood Azargoshasbi, Jinwoong Kim, Youngseob Kim, Daniel Yazgi, and Marianne Hatzopoulou
Geosci. Model Dev., 17, 3579–3597, https://doi.org/10.5194/gmd-17-3579-2024, https://doi.org/10.5194/gmd-17-3579-2024, 2024
Short summary
Short summary
Air pollution is a major health hazard, and chemical transport models (CTMs) are valuable tools that aid in our understanding of the risks of air pollution at both local and regional scales. In this study, the Polair3D CTM of the Polyphemus air quality modeling platform was set up over Quebec, Canada, to assess the model’s capability in predicting key air pollutant species over the region, at seasonal temporal scales and at regional spatial scales.
Rohith Thundathil, Florian Zus, Galina Dick, and Jens Wickert
Geosci. Model Dev., 17, 3599–3616, https://doi.org/10.5194/gmd-17-3599-2024, https://doi.org/10.5194/gmd-17-3599-2024, 2024
Short summary
Short summary
Global Navigation Satellite Systems (GNSS) provides moisture observations through its densely distributed ground station network. In this research, we assimilate a new type of observation called tropospheric gradient observations, which has never been incorporated into a weather model. We develop a forward operator for gradient-based observations and conduct an assimilation impact study. The study shows significant improvements in the model's humidity fields.
Ankur Mahesh, Travis A. O'Brien, Burlen Loring, Abdelrahman Elbashandy, William Boos, and William D. Collins
Geosci. Model Dev., 17, 3533–3557, https://doi.org/10.5194/gmd-17-3533-2024, https://doi.org/10.5194/gmd-17-3533-2024, 2024
Short summary
Short summary
Atmospheric rivers (ARs) are extreme weather events that can alleviate drought or cause billions of US dollars in flood damage. We train convolutional neural networks (CNNs) to detect ARs with an estimate of the uncertainty. We present a framework to generalize these CNNs to a variety of datasets of past, present, and future climate. Using a simplified simulation of the Earth's atmosphere, we validate the CNNs. We explore the role of ARs in maintaining energy balance in the Earth system.
Alexandra Rivera, Kostas Tsigaridis, Gregory Faluvegi, and Drew Shindell
Geosci. Model Dev., 17, 3487–3505, https://doi.org/10.5194/gmd-17-3487-2024, https://doi.org/10.5194/gmd-17-3487-2024, 2024
Short summary
Short summary
This paper describes and evaluates an improvement to the representation of acetone in the GISS ModelE2.1 Earth system model. We simulate acetone's concentration and transport across the atmosphere as well as its dependence on chemistry, the ocean, and various global emissions. Comparisons of our model’s estimates to past modeling studies and field measurements have shown encouraging results. Ultimately, this paper contributes to a broader understanding of acetone's role in the atmosphere.
Alok K. Samantaray, Priscilla A. Mooney, and Carla A. Vivacqua
Geosci. Model Dev., 17, 3321–3339, https://doi.org/10.5194/gmd-17-3321-2024, https://doi.org/10.5194/gmd-17-3321-2024, 2024
Short summary
Short summary
Any interpretation of climate model data requires a comprehensive evaluation of the model performance. Numerous error metrics exist for this purpose, and each focuses on a specific aspect of the relationship between reference and model data. Thus, a comprehensive evaluation demands the use of multiple error metrics. However, this can lead to confusion. We propose a clustering technique to reduce the number of error metrics needed and a composite error metric to simplify the interpretation.
Richard Maier, Fabian Jakub, Claudia Emde, Mihail Manev, Aiko Voigt, and Bernhard Mayer
Geosci. Model Dev., 17, 3357–3383, https://doi.org/10.5194/gmd-17-3357-2024, https://doi.org/10.5194/gmd-17-3357-2024, 2024
Short summary
Short summary
Based on the TenStream solver, we present a new method to accelerate 3D radiative transfer towards the speed of currently used 1D solvers. Using a shallow-cumulus-cloud time series, we evaluate the performance of this new solver in terms of both speed and accuracy. Compared to a 3D benchmark simulation, we show that our new solver is able to determine much more accurate irradiances and heating rates than a 1D δ-Eddington solver, even when operated with a similar computational demand.
Julia Maillard, Jean-Christophe Raut, and François Ravetta
Geosci. Model Dev., 17, 3303–3320, https://doi.org/10.5194/gmd-17-3303-2024, https://doi.org/10.5194/gmd-17-3303-2024, 2024
Short summary
Short summary
Atmospheric models struggle to reproduce the strong temperature inversions in the vicinity of the surface over forested areas in the Arctic winter. In this paper, we develop modified simplified versions of surface layer schemes widely used by the community. Our modifications are used to correct the fact that original schemes place strong limits on the turbulent collapse, leading to a lower surface temperature gradient at low wind speeds. Modified versions show a better performance.
Jana Fischereit, Henrik Vedel, Xiaoli Guo Larsén, Natalie E. Theeuwes, Gregor Giebel, and Eigil Kaas
Geosci. Model Dev., 17, 2855–2875, https://doi.org/10.5194/gmd-17-2855-2024, https://doi.org/10.5194/gmd-17-2855-2024, 2024
Short summary
Short summary
Wind farms impact local wind and turbulence. To incorporate these effects in weather forecasting, the explicit wake parameterization (EWP) is added to the forecasting model HARMONIE–AROME. We evaluate EWP using flight data above and downstream of wind farms, comparing it with an alternative wind farm parameterization and another weather model. Results affirm the correct implementation of EWP, emphasizing the necessity of accounting for wind farm effects in accurate weather forecasting.
Clément Bouvier, Daan van den Broek, Madeleine Ekblom, and Victoria A. Sinclair
Geosci. Model Dev., 17, 2961–2986, https://doi.org/10.5194/gmd-17-2961-2024, https://doi.org/10.5194/gmd-17-2961-2024, 2024
Short summary
Short summary
An analytical initial background state has been developed for moist baroclinic wave simulation on an aquaplanet and implemented into OpenIFS. Seven parameters can be controlled, which are used to generate the background states and the development of baroclinic waves. The meteorological and numerical stability has been assessed. Resulting baroclinic waves have proven to be realistic and sensitive to the jet's width.
Jelena Radović, Michal Belda, Jaroslav Resler, Kryštof Eben, Martin Bureš, Jan Geletič, Pavel Krč, Hynek Řezníček, and Vladimír Fuka
Geosci. Model Dev., 17, 2901–2927, https://doi.org/10.5194/gmd-17-2901-2024, https://doi.org/10.5194/gmd-17-2901-2024, 2024
Short summary
Short summary
Boundary conditions are of crucial importance for numerical model (e.g., PALM) validation studies and have a large influence on the model results, especially when studying the atmosphere of real, complex, and densely built urban environments. Our experiments with different driving conditions for the large-eddy simulation model PALM show its strong dependency on boundary conditions, which is important for the proper separation of errors coming from the boundary conditions and the model itself.
Siyuan Chen, Yi Zhang, Yiming Wang, Zhuang Liu, Xiaohan Li, and Wei Xue
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-68, https://doi.org/10.5194/gmd-2024-68, 2024
Revised manuscript accepted for GMD
Short summary
Short summary
This study explores strategies and techniques for implementing mixed-precision code optimization within an atmosphere model dynamical core. The equation terms in the governing equations that are sensitive (insensitive) to the precision level have been identified. The performance of mixed-precision computing for weather and climate simulations was analyzed.
Manu Anna Thomas, Klaus Wyser, Shiyu Wang, Marios Chatziparaschos, Paraskevi Georgakaki, Montserrat Costa-Surós, Maria Gonçalves Ageitos, Maria Kanakidou, Carlos Pérez García-Pando, Athanasios Nenes, Twan van Noije, Philippe Le Sager, and Abhay Devasthale
EGUsphere, https://doi.org/10.5194/egusphere-2024-248, https://doi.org/10.5194/egusphere-2024-248, 2024
Short summary
Short summary
Aerosol-cloud interactions occur at a range of spatio-temporal scales. While evaluating recent developments in EC-Earth3-AerChem model, this study aims to understand the extent to which Twomey effect manifests itself at larger scales. We report a reduction in the warm bias over the Southern Ocean due to model improvements. While we do see footprints of Twomey effect at larger scales, the negative relationship between cloud droplet number and liquid water drives the shortwave radiative effect.
Sonya L. Fiddes, Marc D. Mallet, Alain Protat, Matthew T. Woodhouse, Simon P. Alexander, and Kalli Furtado
Geosci. Model Dev., 17, 2641–2662, https://doi.org/10.5194/gmd-17-2641-2024, https://doi.org/10.5194/gmd-17-2641-2024, 2024
Short summary
Short summary
In this study we present an evaluation that considers complex, non-linear systems in a holistic manner. This study uses XGBoost, a machine learning algorithm, to predict the simulated Southern Ocean shortwave radiation bias in the ACCESS model using cloud property biases as predictors. We then used a novel feature importance analysis to quantify the role that each cloud bias plays in predicting the radiative bias, laying the foundation for advanced Earth system model evaluation and development.
Gaurav Govardhan, Sachin D. Ghude, Rajesh Kumar, Sumit Sharma, Preeti Gunwani, Chinmay Jena, Prafull Yadav, Shubhangi Ingle, Sreyashi Debnath, Pooja Pawar, Prodip Acharja, Rajmal Jat, Gayatry Kalita, Rupal Ambulkar, Santosh Kulkarni, Akshara Kaginalkar, Vijay K. Soni, Ravi S. Nanjundiah, and Madhavan Rajeevan
Geosci. Model Dev., 17, 2617–2640, https://doi.org/10.5194/gmd-17-2617-2024, https://doi.org/10.5194/gmd-17-2617-2024, 2024
Short summary
Short summary
A newly developed air quality forecasting framework, Decision Support System (DSS), for air quality management in Delhi, India, provides source attribution with numerous emission reduction scenarios besides forecasts. DSS shows that during post-monsoon and winter seasons, Delhi and its neighboring districts contribute to 30 %–40 % each to pollution in Delhi. On average, a 40 % reduction in the emissions in Delhi and the surrounding districts would result in a 24 % reduction in Delhi's pollution.
Simon Rosanka, Holger Tost, Rolf Sander, Patrick Jöckel, Astrid Kerkweg, and Domenico Taraborrelli
Geosci. Model Dev., 17, 2597–2615, https://doi.org/10.5194/gmd-17-2597-2024, https://doi.org/10.5194/gmd-17-2597-2024, 2024
Short summary
Short summary
The capabilities of the Modular Earth Submodel System (MESSy) are extended to account for non-equilibrium aqueous-phase chemistry in the representation of deliquescent aerosols. When applying the new development in a global simulation, we find that MESSy's bias in modelling routinely observed reduced inorganic aerosol mass concentrations, especially in the United States. Furthermore, the representation of fine-aerosol pH is particularly improved in the marine boundary layer.
Junyu Li, Yuxin Wang, Lilong Liu, Yibin Yao, Liangke Huang, and Feijuan Li
Geosci. Model Dev., 17, 2569–2581, https://doi.org/10.5194/gmd-17-2569-2024, https://doi.org/10.5194/gmd-17-2569-2024, 2024
Short summary
Short summary
In this study, we have developed a model (RF-PWV) to characterize precipitable water vapor (PWV) variation with altitude in the study area. RF-PWV can significantly reduce errors in vertical correction, enhance PWV fusion product accuracy, and provide insights into PWV vertical distribution, thereby contributing to climate research.
Cited articles
Ajtić, J., Brattich, E., Sarvan, D., Djurdjevic, V., and Hernandez-Ceballos, M. A.: Factors affecting the 7Be surface concentration and its extremely high occurrences over the Scandinavian Peninsula during autumn and winter, Chemosphere, 199, 278–285, https://doi.org/10.1016/j.chemosphere.2018.02.052, 2018.
Ajtić, J., Zorko, B., Nečemer, M., Sarvan, D., Rajačić, M., Krneta Nikolić, J., Todorović, D., Djurdjevic, V., Vodenik, B., Glavič Cindro, D., and Kožar Logar, J.: Characteristics of radioactivity in the surface air along the 45°N zonal belt in South-Eastern Europe, Int. J. Environ. Sci. Technol., 19, 9719–9730, https://doi.org/10.1007/s13762-021-03814-0, 2022.
Aldahan, A., Possnert, G., Johnsen, S. J., Clausen, H. B., Isaksson, E., Karlen, W., and Hansson, M.: Sixty year 10Be record from Greenland and Antarctica, Earth Planet. Sci., 107, 139–147, https://doi.org/10.1007/BF02840464, 1998.
Aldahan, A., Possnert, G., and Vintersved, I.: Atmospheric interactions at northern high latitudes from weekly Be-isotopes in surface air, Appl. Radiat. Isot., 54, 345–353, https://doi.org/10.1016/S0969-8043(00)00163-9, 2001.
Aldahan, A., Hedfors, J., Possnert, G., Kulan, A., Berggren, A. M., and Söderström, C.: Atmospheric impact on beryllium isotopes as solar activity proxy, Geophys. Res. Lett., 35, L21812, https://doi.org/10.1029/2008gl035189, 2008.
Auer, M., Wagenbach, D., Wild, E. M., Wallner, A., Priller, A., Miller, H., Schlosser, C., and Kutschera, W.: Cosmogenic 26Al in the atmosphere and the prospect of a 26Al/10Be chronometer to date old ice, Earth Planet. Sc. Lett., 287, 453–462, https://doi.org/10.1016/j.epsl.2009.08.030, 2009.
Baroni, M., Bard, E., Petit, J.-R., Magand, O., and Bourlès, D.: Volcanic and solar activity, and atmospheric circulation influences on cosmogenic 10Be fallout at Vostok and Concordia (Antarctica) over the last 60 years, Geochim. Cosmochim. Ac., 75, 7132–7145, https://doi.org/10.1016/j.gca.2011.09.002, 2011.
Beer, J., McCracken, K., and Von Steiger, R.: Cosmogenic Radionuclides: Theory and Applications in the Terrestrial and Space Environments, Springer Berlin, Heidelberg, 428 pp., https://doi.org/10.1007/978-3-642-14651-0, 2012.
Berggren, A. M., Beer, J., Possnert, G., Aldahan, A., Kubik, P., Christl, M., Johnsen, S. J., Abreu, J., and Vinther, B. M.: A 600-year annual 10Be record from the NGRIP ice core, Greenland, Geophys. Res. Lett., 36, L11801, https://doi.org/10.1029/2009gl038004, 2009.
Bey, I., Jacob, D. J., Yantosca, R. M., Logan, J. A., Field, B. D., Fiore, A. M., Li, Q., Liu, H. Y., Mickley, L. J., and Schultz, M. G.: Global modeling of tropospheric chemistry with assimilated meteorology: Model description and evaluation, J. Geophys. Res.-Atmos., 106, 23073–23095, https://doi.org/10.1029/2001JD000807, 2001.
Bleichrodt, J. F.: Mean tropospheric residence time of cosmic-ray-produced beryllium 7 at north temperate latitudes, J. Geophys. Res.-Oceans, 83, 3058–3062, https://doi.org/10.1029/JC083iC06p03058, 1978.
Brattich, E., Liu, H., Tositti, L., Considine, D. B., and Crawford, J. H.: Processes controlling the seasonal variations in 210Pb and 7Be at the Mt. Cimone WMO-GAW global station, Italy: a model analysis, Atmos. Chem. Phys., 17, 1061–1080, https://doi.org/10.5194/acp-17-1061-2017, 2017.
Brattich, E., Liu, H., Zhang, B., Hernández-Ceballos, M. Á., Paatero, J., Sarvan, D., Djurdjevic, V., Tositti, L., and Ajtić, J.: Observation and modeling of high-7Be concentration events at the surface in northern Europe associated with the instability of the Arctic polar vortex in early 2003, Atmos. Chem. Phys., 21, 17927–17951, https://doi.org/10.5194/acp-21-17927-2021, 2021.
Burakowska, A., Kubicki, M., Myslek-Laurikainen, B., Piotrowski, M., Trzaskowska, H., and Sosnowiec, R.: Concentration of 7Be, 210Pb, 40K, 137Cs, 134Cs radionuclides in the ground layer of the atmosphere in the polar (Hornsund, Spitsbergen) and mid-latitudes (Otwock-Swider, Poland) regions, J. Environ. Radioact., 240, 106739, https://doi.org/10.1016/j.jenvrad.2021.106739, 2021.
Chabrillat, S., Vigouroux, C., Christophe, Y., Engel, A., Errera, Q., Minganti, D., Monge-Sanz, B. M., Segers, A., and Mahieu, E.: Comparison of mean age of air in five reanalyses using the BASCOE transport model, Atmos. Chem. Phys., 18, 14715–14735, https://doi.org/10.5194/acp-18-14715-2018, 2018.
Chae, J.-S. and Kim, G.: Large seasonal variations in fine aerosol precipitation rates revealed using cosmogenic 7Be as a tracer, Sci. Total Environ., 673, 1–6, https://doi.org/10.1016/j.scitotenv.2019.03.482, 2019.
Chang, J. C. and Hanna, S. R.: Air quality model performance evaluation, Meteorol. Atmos. Phys., 87, 167–196, https://doi.org/10.1007/s00703-003-0070-7, 2004.
Chmeleff, J., von Blanckenburg, F., Kossert, K., and Jakob, D.: Determination of the 10Be half-life by multicollector ICP-MS and liquid scintillation counting, Nuclear Instruments and Methods in Physics Research Section B, 268, 192–199, https://doi.org/10.1016/j.nimb.2009.09.012, 2010.
Copeland, K.: CARI-7 Documentation: Geomagnetic Cutoff Rigidity Calculations and Tables for 1965–2010, United States, Department of Transportation, Federal Aviation Administration, https://rosap.ntl.bts.gov/view/dot/57079 (last access: 1 December 2023), 2018.
Courtier, J., Sdraulig, S., and Hirth, G.: 7Be and 210Pb wet/dry deposition in Melbourne, Australia and the development of deployable units for radiological emergency monitoring, J. Environ. Radioact., 178–179, 419–425, https://doi.org/10.1016/j.jenvrad.2017.07.004, 2017.
Delaygue, G., Bekki, S., and Bard, E.: Modelling the stratospheric budget of beryllium isotopes, Tellus B, 67, 28582, https://doi.org/10.3402/tellusb.v67.28582, 2015.
Dibb, J. E., Talbot, R. W., and Gregory, G. L.: Beryllium 7 and Lead 210 in the western hemisphere Arctic atmosphere: Observations from three recent aircraft-based sampling programs, J. Geophys. Res.-Atmos., 97, 16709–16715, https://doi.org/10.1029/91JD01807, 1992.
Dibb, J. E., Meeker, L. D., Finkel, R. C., Southon, J. R., Caffee, M. W., and Barrie, L. A.: Estimation of stratospheric input to the Arctic troposphere: 7Be and 10Be in aerosols at Alert, Canada, 99, 12855–12864, https://doi.org/10.1029/94jd00742, 1994.
Du, J., Du, J., Baskaran, M., Bi, Q., Huang, D., and Jiang, Y.: Temporal variations of atmospheric depositional fluxes of 7Be and 210Pb over 8 years (2006–2013) at Shanghai, China, and synthesis of global fallout data, J. Geophys. Res.-Atmos., 120, 4323–4339, https://doi.org/10.1002/2014jd022807, 2015.
Dueñas, C., Gordo, E., Liger, E., Cabello, M., Cañete, S., Pérez, M., and Torre-Luque, P. D. L.: 7Be, 210Pb and 40K depositions over 11 years in Málaga, J. Environ. Radioact., 178–179, 325–334, https://doi.org/10.1016/j.jenvrad.2017.09.010, 2017.
Dutkiewicz, V. A. and Husain, L.: Stratospheric and tropospheric components of 7Be in surface air, J. Geophys. Res.-Atmos., 90, 5783–5788, https://doi.org/10.1029/JD090iD03p05783, 1985.
Eastham, S. D., Weisenstein, D. K., and Barrett, S. R. H.: Development and evaluation of the unified tropospheric–stratospheric chemistry extension (UCX) for the global chemistry-transport model GEOS-Chem, Atmos. Environ., 89, 52–63, https://doi.org/10.1016/j.atmosenv.2014.02.001, 2014.
Elsässer, C.: Exploration of 10Be ice core records using a climatological model approach: Cosmogenic production versus climate variability, heiDOK, https://doi.org/10.11588/heidok.00016349, 2013.
Elsässer, C., Wagenbach, D., Weller, R., Auer, M., Wallner, A., and Christl, M.: Continuous 25-yr aerosol records at coastal Antarctica, Tellus B, 63, 920–934, https://doi.org/10.1111/j.1600-0889.2011.00543.x, 2011.
Field, C. V., Schmidt, G. A., Koch, D., and Salyk, C.: Modeling production and climate-related impacts on 10Be concentration in ice cores, J. Geophys. Res., 111, D15107, https://doi.org/10.1029/2005jd006410, 2006.
Gao, J., Korte, M., Panovska, S., Rong, Z., and Wei, Y.: Effects of the Laschamps Excursion on Geomagnetic Cutoff Rigidities, Geochem. Geophys. Geosyst., 23, e2021GC010261, https://doi.org/10.1029/2021GC010261, 2022.
Gelaro, R., McCarty, W., Suarez, M. J., Todling, R., Molod, A., Takacs, L., Randles, C., Darmenov, A., Bosilovich, M. G., Reichle, R., Wargan, K., Coy, L., Cullather, R., Draper, C., Akella, S., Buchard, V., Conaty, A., da Silva, A., Gu, W., Kim, G. K., Koster, R., Lucchesi, R., Merkova, D., Nielsen, J. E., Partyka, G., Pawson, S., Putman, W., Rienecker, M., Schubert, S. D., Sienkiewicz, M., and Zhao, B.: The Modern-Era Retrospective Analysis for Research and Applications, Version 2 (MERRA-2), J. Climate, 30, 5419–5454, https://doi.org/10.1175/JCLI-D-16-0758.1, 2017a.
Gelaro, R., McCarty, W., Suárez, M. J., Todling, R., Molod, A., Takacs, L., Randles, C. A., Darmenov, A., Bosilovich, M. G., Reichle, R., Wargan, K., Coy, L., Cullather, R., Draper, C., Akella, S., Buchard, V., Conaty, A., da Silva, A. M., Gu, W., Kim, G.-K., Koster, R., Lucchesi, R., Merkova, D., Nielsen, J. E., Partyka, G., Pawson, S., Putman, W., Rienecker, M., Schubert, S. D., Sienkiewicz, M., and Zhao, B.: The Modern-Era Retrospective Analysis for Research and Applications, Version 2 (MERRA-2), J. Climate, 30, 5419–5454, https://doi.org/10.1175/JCLI-D-16-0758.1, 2017b.
Gfeller, G., Fischer, H., Bigler, M., Schüpbach, S., Leuenberger, D., and Mini, O.: Representativeness and seasonality of major ion records derived from NEEM firn cores, The Cryosphere, 8, 1855–1870, https://doi.org/10.5194/tc-8-1855-2014, 2014.
Golubenko, K., Rozanov, E., Kovaltsov, G., and Usoskin, I.: Zonal Mean Distribution of Cosmogenic Isotope (7Be, 10Be, 14C, and 36Cl) Production in Stratosphere and Troposphere, J. Geophys. Res.-Atmos., 127, e2022JD036726, https://doi.org/10.1029/2022JD036726, 2022.
Golubenko, K., Rozanov, E., Kovaltsov, G., Leppänen, A.-P., Sukhodolov, T., and Usoskin, I.: Application of CCM SOCOL-AERv2-BE to cosmogenic beryllium isotopes: description and validation for polar regions, Geosci. Model Dev., 14, 7605–7620, https://doi.org/10.5194/gmd-14-7605-2021, 2021.
Graham, I., Ditchburn, R., and Barry, B.: Atmospheric deposition of 7Be and 10Be in New Zealand rain (1996–98), Geochim. Cosmochim. Ac., 67, 361–373, https://doi.org/10.1016/S0016-7037(02)01092-X, 2003.
Heikkilä, U. and Smith, A. M.: Influence of model resolution on the atmospheric transport of 10Be, Atmos. Chem. Phys., 12, 10601–10612, https://doi.org/10.5194/acp-12-10601-2012, 2012.
Heikkilä, U. and Smith, A. M.: Production rate and climate influences on the variability of 10Be deposition simulated by ECHAM5-HAM: Globally, in Greenland, and in Antarctica, J. Geophys. Res.-Atmos., 118, 2506–2520, https://doi.org/10.1002/jgrd.50217, 2013.
Heikkilä, U., Beer, J., and Alfimov, V.: Beryllium-10 and beryllium-7 in precipitation in Dübendorf (440 m) and at Jungfraujoch (3580 m), Switzerland (1998–2005), J. Geophys. Res., 113, D11104, https://doi.org/10.1029/2007jd009160, 2008a.
Heikkilä, U., Beer, J., and Feichter, J.: Modeling cosmogenic radionuclides 10Be and 7Be during the Maunder Minimum using the ECHAM5-HAM General Circulation Model, Atmos. Chem. Phys., 8, 2797–2809, https://doi.org/10.5194/acp-8-2797-2008, 2008b.
Heikkilä, U., Beer, J., Jouzel, J., Feichter, J., and Kubik, P.: 10Be measured in a GRIP snow pit and modeled using the ECHAM5-HAM general circulation model, Geophys. Res. Lett., 35, L05817, https://doi.org/10.1029/2007gl033067, 2008c.
Heikkilä, U., Beer, J., and Feichter, J.: Meridional transport and deposition of atmospheric 10Be, Atmos. Chem. Phys., 9, 515–527, https://doi.org/10.5194/acp-9-515-2009, 2009.
Heikkilä, U., Beer, J., Abreu, J. A., and Steinhilber, F.: On the Atmospheric Transport and Deposition of the Cosmogenic Radionuclides (10Be): A Review, Space Sci. Rev., 176, 321–332, https://doi.org/10.1007/s11214-011-9838-0, 2013.
Herbst, K., Muscheler, R., and Heber, B.: The new local interstellar spectra and their influence on the production rates of the cosmogenic radionuclides 10Be and 14C, J. Geophys. Res.-Space Phys., 122, 23–34, https://doi.org/10.1002/2016ja023207, 2017.
Hernandez-Ceballos, M. A., Cinelli, G., Ferrer, M. M., Tollefsen, T., De Felice, L., Nweke, E., Tognoli, P. V., Vanzo, S., and De Cort, M.: A climatology of 7Be in surface air in European Union, J. Environ. Radioact., 141, 62–70, https://doi.org/10.1016/j.jenvrad.2014.12.003, 2015.
Hernández-Ceballos, M. A., Brattich, E., Cinelli, G., Ajtić, J., and Djurdjevic, V.: Seasonality of 7Be concentrations in Europe and influence of tropopause height, Tellus B, 68, 29534, https://doi.org/10.3402/tellusb.v68.29534, 2016.
Hernández-Ceballos, M. A., Brattich, E., and Ajtić, J.: Airflow and teleconnection patterns driving the spatial and temporal variability of high 7Be air concentrations in Europe, Chemosphere, 303, 135194, https://doi.org/10.1016/j.chemosphere.2022.135194, 2022.
Hu, J., Sha, Z., Wang, J., Du, J., and Ma, Y.: Atmospheric deposition of 7Be, 210Pb in Xining, a typical city on the Qinghai-Tibet Plateau, China, J. Radioanal. Nucl. Ch., 324, 1141–1150, https://doi.org/10.1007/s10967-020-07127-3, 2020.
Huang, J., Kang, S., Shen, C., Cong, Z., Liu, K., Wang, W., and Liu, L.: Concentration and seasonal variation of 10Be in surface aerosols of Lhasa, Tibet, Chinese Sci. Bull., 55, 2572–2578, https://doi.org/10.1007/s11434-010-3233-1, 2010.
Huh, C.-A., Su, C.-C., and Shiau, L.-J.: Factors controlling temporal and spatial variations of atmospheric deposition of 7Be and 210Pb in northern Taiwan, J. Geophys. Res., 111, D16304, https://doi.org/10.1029/2006jd007180, 2006.
Ioannidou, A. and Papastefanou, C.: Precipitation scavenging of 7Be and 137Cs radionuclides in air, J. Environ. Radioact., 85, 121–136, https://doi.org/10.1016/j.jenvrad.2005.06.005, 2006.
Jordan, C. E., Dibb, J. E., and Finkel, R. C.:
Koch, D. and Rind, D.: Beryllium 10/beryllium 7 as a tracer of stratospheric transport, J. Geophys. Res.-Atmos., 103, 3907–3917, https://doi.org/10.1029/97JD03117, 1998.
Koch, D. M., Jacob, D. J., and Graustein, W. C.: Vertical transport of tropospheric aerosols as indicated by 7Be and 210Pb in a chemical tracer model, J. Geophys. Res.-Atmos., 101, 18651–18666, https://doi.org/10.1029/96JD01176, 1996.
Koldobskiy, S. A., Bindi, V., Corti, C., Kovaltsov, G. A., and Usoskin, I. G.: Validation of the Neutron Monitor Yield Function Using Data From AMS-02 Experiment, 2011–2017, J. Geophys. Res.-Space Phys., 124, 2367–2379, https://doi.org/10.1029/2018ja026340, 2019.
Kong, Y. C., Lee, O. S. M., and Yung, C. H.: Study of the naturally occurring radionuclide Beryllium-7 (Be-7) in Hong Kong, J. Environ. Radioact., 246, 106850, https://doi.org/10.1016/j.jenvrad.2022.106850, 2022.
Kusmierczyk-Michulec, J., Gheddou, A., and Nikkinen, M.: Influence of precipitation on 7Be concentrations in air as measured by CTBTO global monitoring system, J. Environ. Radioact., 144, 140–151, https://doi.org/10.1016/j.jenvrad.2015.03.014, 2015.
Lal, D. and Peters, B.: Cosmic Ray Produced Radioactivity on the Earth, in: Kosmische Strahlung II / Cosmic Rays II, edited by: Sitte, K., Springer Berlin Heidelberg, Berlin, Heidelberg, 551–612, https://doi.org/10.1007/978-3-642-46079-1_7, 1967.
Lee, H. I., Huh, C. A., Lee, T., and Huang, N. E.: Time series study of a 17-year record of 7Be and 210Pb fluxes in northern Taiwan using ensemble empirical mode decomposition, J. Environ. Radioact., 147, 14–21, https://doi.org/10.1016/j.jenvrad.2015.04.017, 2015.
Leppänen, A. P., Pacini, A. A., Usoskin, I. G., Aldahan, A., Echer, E., Evangelista, H., Klemola, S., Kovaltsov, G. A., Mursula, K., and Possnert, G.: Cosmogenic 7Be in air: A complex mixture of production and transport, J. Atmos. Solar-Terr. Phy., 72, 1036–1043, https://doi.org/10.1016/j.jastp.2010.06.006, 2010.
Lin, J.-T. and McElroy, M. B.: Impacts of boundary layer mixing on pollutant vertical profiles in the lower troposphere: Implications to satellite remote sensing, Atmos. Environ., 44, 1726–1739, https://doi.org/10.1016/j.atmosenv.2010.02.009, 2010.
Lin, S.-J. and Rood, R. B.: Multidimensional Flux-Form Semi-Lagrangian Transport Schemes, Mon. Weather Rev., 124, 2046–2070, https://doi.org/10.1175/1520-0493(1996)124<2046:MFFSLT>2.0.CO;2, 1996.
Liu, H., Jacob, D. J., Bey, I., and Yantosca, R. M.: Constraints from 210Pb and 7Be on wet deposition and transport in a global three-dimensional chemical tracer model driven by assimilated meteorological fields, J. Geophys. Res.-Atmos., 106, 12109–12128, https://doi.org/10.1029/2000jd900839, 2001.
Liu, H., Jacob, D. J., Dibb, J. E., Fiore, A. M., and Yantosca, R. M.: Constraints on the sources of tropospheric ozone from 210Pb-7Be-O3 correlations, J. Geophys. Res.-Atmos., 109, D07306, https://doi.org/10.1029/2003JD003988, 2004.
Liu, H., Considine, D. B., Horowitz, L. W., Crawford, J. H., Rodriguez, J. M., Strahan, S. E., Damon, M. R., Steenrod, S. D., Xu, X., Kouatchou, J., Carouge, C., and Yantosca, R. M.: Using beryllium-7 to assess cross-tropopause transport in global models, Atmos. Chem. Phys., 16, 4641–4659, https://doi.org/10.5194/acp-16-4641-2016, 2016.
Liu, X., Fu, Y., Bi, Y., Zhang, L., Zhao, G., Xian, F., and Zhou, W.: Monitoring Surface
Liu, X., Fu, Y., Wang, Q., Bi, Y., Zhang, L., Zhao, G., Xian, F., Cheng, P., Zhang, L., Zhou, J., and Zhou, W.: Unraveling the process of aerosols secondary formation and removal based on cosmogenic beryllium-7 and beryllium-10, Sci. Total Environ., 821, 153293, https://doi.org/10.1016/j.scitotenv.2022.153293, 2022b.
Maejima, Y., Matsuzaki, H., and Higashi, T.: Application of cosmogenic 10Be to dating soils on the raised coral reef terraces of Kikai Island, southwest Japan, Geoderma, 126, 389–399, https://doi.org/10.1016/j.geoderma.2004.10.004, 2005.
Mari, C., Jacob, D. J., and Bechtold, P.: Transport and scavenging of soluble gases in a deep convective cloud, J. Geophys. Res.-Atmos., 105, 22255–22267, https://doi.org/10.1029/2000JD900211, 2000.
Masarik, J. and Beer, J.: Simulation of particle fluxes and cosmogenic nuclide production in the Earth's atmosphere, J. Geophys. Res.-Atmos., 104, 12099–12111, https://doi.org/10.1029/1998jd200091, 1999.
Masarik, J. and Beer, J.: An updated simulation of particle fluxes and cosmogenic nuclide production in the Earth's atmosphere, J. Geophys. Res., 114, D11103, https://doi.org/10.1029/2008jd010557, 2009.
Méndez-García, C. G., Rojas-López, G., Padilla, S., Solís, C., Chávez, E., Acosta, L., and Huerta, A.: The impact of stable 27Al in 26Al/10Be meteoric ratio in PM2.5 from an urban area, J. Environ. Radioact., 246, 106832, https://doi.org/10.1016/j.jenvrad.2022.106832, 2022.
Monaghan, M. C., Krishnaswami, S., and Turekian, K. K.: The global-average production rate of 10Be, Earth Planet. Sc. Lett., 76, 279–287, https://doi.org/10.1016/0012-821X(86)90079-8, 1986.
Murray, L. T., Leibensperger, E. M., Orbe, C., Mickley, L. J., and Sulprizio, M.: GCAP 2.0: a global 3-D chemical-transport model framework for past, present, and future climate scenarios, Geosci. Model Dev., 14, 5789–5823, https://doi.org/10.5194/gmd-14-5789-2021, 2021.
Muscheler, R., Joos, F., Beer, J., Müller, S. A., Vonmoos, M., and Snowball, I.: Solar activity during the last 1000yr inferred from radionuclide records, Quaternary Sci. Rev., 26, 82–97, https://doi.org/10.1016/j.quascirev.2006.07.012, 2007.
Myers, J. L., Well, A. D., and Lorch Jr, R. F., Riegert, D. (Ed.): Research Design and Statistical Analysis, 3rd Edition, Routledge, https://doi.org/10.4324/9780203726631, 2013.
Nevalainen, J., Usoskin, I. G., and Mishev, A.: Eccentric dipole approximation of the geomagnetic field: Application to cosmic ray computations, Adv. Space Res., 52, 22–29, https://doi.org/10.1016/j.asr.2013.02.020, 2013.
Pacini, A. A., Usoskin, I. G., Mursula, K., Echer, E., and Evangelista, H.: Signature of a sudden stratospheric warming in the near-ground 7Be flux, Atmos. Environ., 113, 27–31, https://doi.org/10.1016/j.atmosenv.2015.04.065, 2015.
Padilla, S., Lopez-Gutierrez, J. M., Manjon, G., Garcia-Tenorio, R., Galvan, J. A., and Garcia-Leon, M.: Meteoric 10Be in aerosol filters in the city of Seville, J. Environ. Radioact., 196, 15–21, https://doi.org/10.1016/j.jenvrad.2018.10.009, 2019.
Pedro, J. B., Heikkilä, U. E., Klekociuk, A., Smith, A. M., van Ommen, T. D., and Curran, M. A. J.: Beryllium-10 transport to Antarctica: Results from seasonally resolved observations and modeling, J. Geophys. Res.-Atmos., 116, D23120, https://doi.org/10.1029/2011jd016530, 2011a.
Pedro, J. B., Smith, A. M., Simon, K. J., van Ommen, T. D., and Curran, M. A. J.: High-resolution records of the beryllium-10 solar activity proxy in ice from Law Dome, East Antarctica: measurement, reproducibility and principal trends, Clim. Past, 7, 707–721, https://doi.org/10.5194/cp-7-707-2011, 2011b.
Pedro, J. B., McConnell, J. R., van Ommen, T. D., Fink, D., Curran, M. A. J., Smith, A. M., Simon, K. J., Moy, A. D., and Das, S. B.: Solar and climate influences on ice core 10Be records from Antarctica and Greenland during the neutron monitor era, Earth Planet. Sc. Lett., 355–356, 174–186, https://doi.org/10.1016/j.epsl.2012.08.038, 2012.
Pilchowski, J., Kopp, A., Herbst, K., and Heber, B.: On the definition and calculation of a generalised McIlwain parameter, Astrophys. Space Sci. Trans., 6, 9–17, https://doi.org/10.5194/astra-6-9-2010, 2010.
Poluianov, S. V., Kovaltsov, G. A., Mishev, A. L., and Usoskin, I. G.: Production of cosmogenic isotopes 7Be, 10Be,14C, 22Na, and 36Cl in the atmosphere: Altitudinal profiles of yield functions, J. Geophys. Res.-Atmos., 121, 8125–8136, https://doi.org/10.1002/2016jd025034, 2016.
Raisbeck, G. M., Yiou, F., Fruneau, M., Loiseaux, J. M., Lieuvin, M., and Ravel, J. C.: Deposition rate and seasonal variations in precipitation of cosmogenic 10Be, Nature, 282, 279–280, https://doi.org/10.1038/282279a0, 1979.
Raisbeck, G. M., Yiou, F., Fruneau, M., Loiseaux, J. M., Lieuvin, M., and Ravel, J. C.: Cosmogenic
Rodriguez-Perulero, A., Baeza, A., and Guillen, J.: Seasonal evolution of 7,10Be and 22Na in the near surface atmosphere of Caceres (Spain), J. Environ. Radioact., 197, 55–61, https://doi.org/10.1016/j.jenvrad.2018.11.015, 2019.
Sangiorgi, M., Hernández Ceballos, M. A., Iurlaro, G., Cinelli, G., and de Cort, M.: 30 years of European Commission Radioactivity Environmental Monitoring data bank (REMdb) – an open door to boost environmental radioactivity research, Earth Syst. Sci. Data, 11, 589–601, https://doi.org/10.5194/essd-11-589-2019, 2019.
Smart, D. F. and Shea, M. A.: A review of geomagnetic cutoff rigidities for earth-orbiting spacecraft, Adv. Space Res., 36, 2012–2020, https://doi.org/10.1016/j.asr.2004.09.015, 2005.
Somayajulu, B. L. K., Sharma, P., Beer, J., Bonani, G., Hofmann, H. J., Morenzoni, E., Nessi, M., Suter, M., and Wölfli, W.: 10Be annual fallout in rains in India, Nuclear Instruments and Methods in Physics Research Section B, 5, 398–403, https://doi.org/10.1016/0168-583X(84)90549-4, 1984.
Spiegl, T. C., Yoden, S., Langematz, U., Sato, T., Chhin, R., Noda, S., Miyake, F., Kusano, K., Schaar, K., and Kunze, M.: Modeling the Transport and Deposition of 10Be Produced by the Strongest Solar Proton Event During the Holocene, J. Geophys. Res.-Atmos., 127, e2021JD035658, https://doi.org/10.1029/2021JD035658, 2022.
Sukhodolov, T., Usoskin, I., Rozanov, E., Asvestari, E., Ball, W. T., Curran, M. A., Fischer, H., Kovaltsov, G., Miyake, F., Peter, T., Plummer, C., Schmutz, W., Severi, M., and Traversi, R.: Atmospheric impacts of the strongest known solar particle storm of 775 AD, Sci. Rep., 7, 45257, https://doi.org/10.1038/srep45257, 2017.
Terzi, L. and Kalinowski, M.: World-wide seasonal variation of 7Be related to large-scale atmospheric circulation dynamics, J. Environ. Radioact., 178–179, 1–15, https://doi.org/10.1016/j.jenvrad.2017.06.031, 2017.
Terzi, L., Kalinowski, M., Schoeppner, M., and Wotawa, G.: How to predict seasonal weather and monsoons with radionuclide monitoring, Sci. Rep., 9, 2729, https://doi.org/10.1038/s41598-019-39664-7, 2019.
Uhlar, R., Harokova, P., Alexa, P., and Kacmarik, M.: 7Be atmospheric activity concentration and meteorological data: Statistical analysis and two-layer atmospheric model, J. Environ. Radioact., 219, 106278, https://doi.org/10.1016/j.jenvrad.2020.106278, 2020.
Usoskin, I. G., Field, C. V., Schmidt, G. A., Leppänen, A.-P., Aldahan, A., Kovaltsov, G. A., Possnert, G., and Ungar, R. K.: Short-term production and synoptic influences on atmospheric 7Be concentrations, J. Geophys. Res., 114, D06108, https://doi.org/10.1029/2008jd011333, 2009.
Villarreal, R. E., Arazi, A., and Fernandez Niello, J. O.: Correlation between the latitudinal profile of the 7Be air concentration and the Hadley cell extent in the Southern Hemisphere, J. Environ. Radioact., 244–245, 106760, https://doi.org/10.1016/j.jenvrad.2021.106760, 2022.
Wang, Q., Jacob, D. J., Fisher, J. A., Mao, J., Leibensperger, E. M., Carouge, C. C., Le Sager, P., Kondo, Y., Jimenez, J. L., Cubison, M. J., and Doherty, S. J.: Sources of carbonaceous aerosols and deposited black carbon in the Arctic in winter-spring: implications for radiative forcing, Atmos. Chem. Phys., 11, 12453–12473, https://doi.org/10.5194/acp-11-12453-2011, 2011.
Waugh, D. and Hall, T.: Age of Stratospheric Air: Theory, Observations, and Models, Rev. Geophys., 40, 1-1–1-26, https://doi.org/10.1029/2000rg000101, 2002.
Wesely, M. L.: Parameterization of surface resistances to gaseous dry deposition in regional-scale numerical models, Atmos. Environ., 23, 1293–1304, https://doi.org/10.1016/0004-6981(89)90153-4, 1989.
Wu, S., Mickley, L. J., Jacob, D. J., Logan, J. A., Yantosca, R. M., and Rind, D.: Why are there large differences between models in global budgets of tropospheric ozone?, J. Geophys. Res.-Atmos., 112, D05302, https://doi.org/10.1029/2006JD007801, 2007.
Yamagata, T., Nagai, H., Matsuzaki, H., and Narasaki, Y.: Decadal variations of atmospheric 7Be and 10Be concentrations between 1998 and 2014 in Japan, Nuclear Instruments and Methods in Physics Research Section B, 455, 265–270, https://doi.org/10.1016/j.nimb.2018.12.029, 2019.
Yu, K., Keller, C. A., Jacob, D. J., Molod, A. M., Eastham, S. D., and Long, M. S.: Errors and improvements in the use of archived meteorological data for chemical transport modeling: an analysis using GEOS-Chem v11-01 driven by GEOS-5 meteorology, Geosci. Model Dev., 11, 305–319, https://doi.org/10.5194/gmd-11-305-2018, 2018.
Zhang, B., Liu, H., Crawford, J. H., Chen, G., Fairlie, T. D., Chambers, S., Kang, C.-H., Williams, A. G., Zhang, K., Considine, D. B., Sulprizio, M. P., and Yantosca, R. M.: Simulation of radon-222 with the GEOS-Chem global model: emissions, seasonality, and convective transport, Atmos. Chem. Phys., 21, 1861–1887, https://doi.org/10.5194/acp-21-1861-2021, 2021.
Zhang, F., Wang, J., Baskaran, M., Zhong, Q., Wang, Y., Paatero, J., and Du, J.: A global dataset of atmospheric 7Be and 210Pb measurements: annual air concentration and depositional flux, Earth Syst. Sci. Data, 13, 2963–2994, https://doi.org/10.5194/essd-13-2963-2021, 2021.
Zheng, M., Adolphi, F., Sjolte, J., Aldahan, A., Possnert, G., Wu, M., Chen, P., and Muscheler, R.: Solar and climate signals revealed by seasonal 10Be data from the NEEM ice core project for the neutron monitor period, Earth Planet. Sc. Lett., 541, 116273, https://doi.org/10.1016/j.epsl.2020.116273, 2020.
Zheng, M., Adolphi, F., Sjolte, J., Aldahan, A., Possnert, G., Wu, M., Chen, P., and Muscheler, R.: Solar Activity of the Past 100 Years Inferred From 10Be in Ice Cores – Implications for Long-Term Solar Activity Reconstructions, Geophys. Res. Lett., 48, e2020GL090896, https://doi.org/10.1029/2020GL090896, 2021a.
Zheng, M., Sjolte, J., Adolphi, F., Aldahan, A., Possnert, G., Wu, M., and Muscheler, R.: Solar and meteorological influences on seasonal atmospheric 7Be in Europe for 1975 to 2018, Chemosphere, 263, 128318, https://doi.org/10.1016/j.chemosphere.2020.128318, 2021b.
Zheng, M., Adolphi, F., Paleari, C., Tao, Q., Erhardt, T., Christl, M., Wu, M., Lu, Z., Hörhold, M., Chen, P., and Muscheler, R.: Solar, Atmospheric, and Volcanic Impacts on 10Be Depositions in Greenland and Antarctica During the Last 100 Years, J. Geophys. Res.-Atmos., 128, e2022JD038392, https://doi.org/10.1029/2022JD038392, 2023a.
Zheng, M., Liu, H., Adolphi, F., Muscheler, R., Lu, Z., Wu, M., and Prisle, N. L.: Simulations of 7Be and 10Be with the GEOS-Chem global model v14.0.2 using state-of-the-art production rates, Zenodo [code and data set], https://doi.org/10.5281/zenodo.8372652, 2023b.
Short summary
The radionuclides 7Be and 10Be are useful tracers for atmospheric transport studies. Here we use the GEOS-Chem to simulate 7Be and 10Be with different production rates: the default production rate in GEOS-Chem and two from the state-of-the-art beryllium production model. We demonstrate that reduced uncertainties in the production rates can enhance the utility of 7Be and 10Be as tracers for evaluating transport and scavenging processes in global models.
The radionuclides 7Be and 10Be are useful tracers for atmospheric transport studies. Here we use...
