Articles | Volume 13, issue 9
https://doi.org/10.5194/gmd-13-4435-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/gmd-13-4435-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Development and technical paper
| 
22 Sep 2020
Development and technical paper |
| 22 Sep 2020
| 22 Sep 2020
A mass- and energy-conserving framework for using machine learning to speed computations: a photochemistry example
Air Quality Research Center, University of California, Davis,
CA 95616, USA
Institute of Mathematics, Technical University of Berlin, 10587 Berlin,
Germany
Anthony S. Wexler
Air Quality Research Center, University of California, Davis,
CA 95616, USA
Departments of Mechanical and Aerospace Engineering, Civil and
Environmental Engineering, and Land, Air and Water Resources, University of
California, Davis, CA 95616, USA
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Geosci. Model Dev., 15, 3417–3431, https://doi.org/10.5194/gmd-15-3417-2022, https://doi.org/10.5194/gmd-15-3417-2022, 2022
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Large air quality and climate models require vast amounts of computational power. Machine learning tools like neural networks can be used to make these models more efficient, with the downside that their results might not make physical sense or be easy to interpret. This work develops a physically interpretable neural network that obeys scientific laws like conservation of mass and models atmospheric composition more accurately than a traditional neural network.
Bruno Debus, Andrew T. Weakley, Satoshi Takahama, Kathryn M. George, Anahita Amiri-Farahani, Bret Schichtel, Scott Copeland, Anthony S. Wexler, and Ann M. Dillner
Atmos. Meas. Tech., 15, 2685–2702, https://doi.org/10.5194/amt-15-2685-2022, https://doi.org/10.5194/amt-15-2685-2022, 2022
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In the US, routine particulate matter composition is measured on samples collected on three types of filter media and analyzed using several techniques. We propose an alternate approach that uses one analytical technique, Fourier transform-infrared spectroscopy (FT-IR), and one filter type to measure the chemical composition of particulate matter in a major US monitoring network. This method could be used to add low-cost sites to the network, fill-in missing data, or for quality control.
Patrick Obin Sturm and Anthony S. Wexler
Geosci. Model Dev., 15, 3417–3431, https://doi.org/10.5194/gmd-15-3417-2022, https://doi.org/10.5194/gmd-15-3417-2022, 2022
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Large air quality and climate models require vast amounts of computational power. Machine learning tools like neural networks can be used to make these models more efficient, with the downside that their results might not make physical sense or be easy to interpret. This work develops a physically interpretable neural network that obeys scientific laws like conservation of mass and models atmospheric composition more accurately than a traditional neural network.
Christopher D. Wallis, Mason D. Leandro, Patrick Y. Chuang, and Anthony S. Wexler
Atmos. Meas. Tech., 15, 2547–2556, https://doi.org/10.5194/amt-15-2547-2022, https://doi.org/10.5194/amt-15-2547-2022, 2022
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Measuring emissions from stacks requires techniques to address a broad range of conditions and measurement challenges. Here we describe an instrument package held by a crane above a stack to characterize both wet droplet and dried aerosol emissions from cooling tower spray drift in situ. The instrument package characterizes the velocity, size distribution, and concentration of the wet droplet emissions and the mass concentration and elemental composition of the dried PM2.5 and PM10 emissions.
Seyyed Ali Davari and Anthony S. Wexler
Atmos. Meas. Tech., 13, 5369–5377, https://doi.org/10.5194/amt-13-5369-2020, https://doi.org/10.5194/amt-13-5369-2020, 2020
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Traditional instruments for detection and quantification of toxic metals in the atmosphere are expensive. In this study, we have designed, fabricated, and tested a low-cost instrument, which employs cheap components to detect and quantify toxic metals. Advanced machine learning (ML) techniques have been used to improve the instrument's performance. This study demonstrates how the combination of low-cost sensors with ML can address problems that traditionally have been too expensive to be solved.
Satoshi Takahama, Ann M. Dillner, Andrew T. Weakley, Matteo Reggente, Charlotte Bürki, Mária Lbadaoui-Darvas, Bruno Debus, Adele Kuzmiakova, and Anthony S. Wexler
Atmos. Meas. Tech., 12, 525–567, https://doi.org/10.5194/amt-12-525-2019, https://doi.org/10.5194/amt-12-525-2019, 2019
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Mid-infrared spectra of particulate matter (PM) samples are complex but chemically informative and present an opportunity for cost-effective measurement of PM provided that quantitative calibration models can be built. We review an emerging strategy for building statistical calibration models using collocated measurements, interpreting the physical bases for such models and evaluating the suitability of existing calibration models to new samples.
Christopher D. Cappa, Shantanu H. Jathar, Michael J. Kleeman, Kenneth S. Docherty, Jose L. Jimenez, John H. Seinfeld, and Anthony S. Wexler
Atmos. Chem. Phys., 16, 3041–3059, https://doi.org/10.5194/acp-16-3041-2016, https://doi.org/10.5194/acp-16-3041-2016, 2016
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Losses of vapors to walls of chambers can negatively bias SOA formation measurements, consequently leading to low predicted SOA concentrations in air quality models. Here, we show that accounting for such vapor losses leads to substantial increases in the predicted amount of SOA formed from VOCs and to notable increases in the O : C atomic ratio in two US regions. Comparison with a variety of observational data suggests generally improved model performance when vapor wall losses are accounted for.
S. H. Jathar, C. D. Cappa, A. S. Wexler, J. H. Seinfeld, and M. J. Kleeman
Atmos. Chem. Phys., 16, 2309–2322, https://doi.org/10.5194/acp-16-2309-2016, https://doi.org/10.5194/acp-16-2309-2016, 2016
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Multi-generational chemistry schemes applied in regional models do not increase secondary organic aerosol (SOA) mass production relative to traditional "two-product" schemes when both models are fitted to the same chamber data. The multi-generational chemistry schemes do change the predicted composition of SOA and the source attribution of SOA.
C. R. Hoyle, C. Fuchs, E. Järvinen, H. Saathoff, A. Dias, I. El Haddad, M. Gysel, S. C. Coburn, J. Tröstl, A.-K. Bernhammer, F. Bianchi, M. Breitenlechner, J. C. Corbin, J. Craven, N. M. Donahue, J. Duplissy, S. Ehrhart, C. Frege, H. Gordon, N. Höppel, M. Heinritzi, T. B. Kristensen, U. Molteni, L. Nichman, T. Pinterich, A. S. H. Prévôt, M. Simon, J. G. Slowik, G. Steiner, A. Tomé, A. L. Vogel, R. Volkamer, A. C. Wagner, R. Wagner, A. S. Wexler, C. Williamson, P. M. Winkler, C. Yan, A. Amorim, J. Dommen, J. Curtius, M. W. Gallagher, R. C. Flagan, A. Hansel, J. Kirkby, M. Kulmala, O. Möhler, F. Stratmann, D. R. Worsnop, and U. Baltensperger
Atmos. Chem. Phys., 16, 1693–1712, https://doi.org/10.5194/acp-16-1693-2016, https://doi.org/10.5194/acp-16-1693-2016, 2016
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A significant portion of sulphate, an important constituent of atmospheric aerosols, is formed via the aqueous phase oxidation of sulphur dioxide by ozone. The rate of this reaction has previously only been measured over a relatively small temperature range. Here, we use the state of the art CLOUD chamber at CERN to perform the first measurements of this reaction rate in super-cooled droplets, confirming that the existing extrapolation of the reaction rate to sub-zero temperatures is accurate.
S. H. Jathar, C. D. Cappa, A. S. Wexler, J. H. Seinfeld, and M. J. Kleeman
Geosci. Model Dev., 8, 2553–2567, https://doi.org/10.5194/gmd-8-2553-2015, https://doi.org/10.5194/gmd-8-2553-2015, 2015
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Multi-generational oxidation of organic vapors can significantly alter the mass, chemical composition and properties of secondary organic aerosol (SOA). Here, we implement a semi-explicit, constrained multi-generational oxidation model of Cappa and Wilson (2012) in a 3-D air quality model. When compared with results from a current-generation SOA model, we predict similar mass concentrations of SOA but a different chemical composition. O:C ratios of SOA are in line with those measured globally.
J. G. Charrier, N. K. Richards-Henderson, K. J. Bein, A. S. McFall, A. S. Wexler, and C. Anastasio
Atmos. Chem. Phys., 15, 2327–2340, https://doi.org/10.5194/acp-15-2327-2015, https://doi.org/10.5194/acp-15-2327-2015, 2015
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We measured the oxidative potential of airborne particles – a property that has been linked to health problems caused by particles – from different emission source mixtures in Fresno, CA. Copper was responsible for the majority of the oxidative potential (as measured by the DTT assay), followed by unknown species (likely organics) and manganese. Sources of copper-rich particles, including vehicles, had higher oxidative potentials.
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Wind farms impact local wind and turbulence. To incorporate these effects in weather forecasting, the explicit wake parameterization (EWP) is added to the forecasting model HARMONIE–AROME. We evaluate EWP using flight data above and downstream of wind farms, comparing it with an alternative wind farm parameterization and another weather model. Results affirm the correct implementation of EWP, emphasizing the necessity of accounting for wind farm effects in accurate weather forecasting.
Clément Bouvier, Daan van den Broek, Madeleine Ekblom, and Victoria A. Sinclair
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An analytical initial background state has been developed for moist baroclinic wave simulation on an aquaplanet and implemented into OpenIFS. Seven parameters can be controlled, which are used to generate the background states and the development of baroclinic waves. The meteorological and numerical stability has been assessed. Resulting baroclinic waves have proven to be realistic and sensitive to the jet's width.
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Geosci. Model Dev., 17, 2901–2927, https://doi.org/10.5194/gmd-17-2901-2024, https://doi.org/10.5194/gmd-17-2901-2024, 2024
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Boundary conditions are of crucial importance for numerical model (e.g., PALM) validation studies and have a large influence on the model results, especially when studying the atmosphere of real, complex, and densely built urban environments. Our experiments with different driving conditions for the large-eddy simulation model PALM show its strong dependency on boundary conditions, which is important for the proper separation of errors coming from the boundary conditions and the model itself.
Sonya L. Fiddes, Marc D. Mallet, Alain Protat, Matthew T. Woodhouse, Simon P. Alexander, and Kalli Furtado
Geosci. Model Dev., 17, 2641–2662, https://doi.org/10.5194/gmd-17-2641-2024, https://doi.org/10.5194/gmd-17-2641-2024, 2024
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Gaurav Govardhan, Sachin D. Ghude, Rajesh Kumar, Sumit Sharma, Preeti Gunwani, Chinmay Jena, Prafull Yadav, Shubhangi Ingle, Sreyashi Debnath, Pooja Pawar, Prodip Acharja, Rajmal Jat, Gayatry Kalita, Rupal Ambulkar, Santosh Kulkarni, Akshara Kaginalkar, Vijay K. Soni, Ravi S. Nanjundiah, and Madhavan Rajeevan
Geosci. Model Dev., 17, 2617–2640, https://doi.org/10.5194/gmd-17-2617-2024, https://doi.org/10.5194/gmd-17-2617-2024, 2024
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A newly developed air quality forecasting framework, Decision Support System (DSS), for air quality management in Delhi, India, provides source attribution with numerous emission reduction scenarios besides forecasts. DSS shows that during post-monsoon and winter seasons, Delhi and its neighboring districts contribute to 30 %–40 % each to pollution in Delhi. On average, a 40 % reduction in the emissions in Delhi and the surrounding districts would result in a 24 % reduction in Delhi's pollution.
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Geosci. Model Dev., 17, 2597–2615, https://doi.org/10.5194/gmd-17-2597-2024, https://doi.org/10.5194/gmd-17-2597-2024, 2024
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Junyu Li, Yuxin Wang, Lilong Liu, Yibin Yao, Liangke Huang, and Feijuan Li
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Rolf Sander
Geosci. Model Dev., 17, 2419–2425, https://doi.org/10.5194/gmd-17-2419-2024, https://doi.org/10.5194/gmd-17-2419-2024, 2024
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The open-source software MEXPLORER 1.0.0 is presented here. The program can be used to analyze, reduce, and visualize complex chemical reaction mechanisms. The mathematics behind the tool is based on graph theory: chemical species are represented as vertices, and reactions as edges. MEXPLORER is a community model published under the GNU General Public License.
Leonardo Olivetti and Gabriele Messori
Geosci. Model Dev., 17, 2347–2358, https://doi.org/10.5194/gmd-17-2347-2024, https://doi.org/10.5194/gmd-17-2347-2024, 2024
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In the last decades, weather forecasting up to 15 d into the future has been dominated by physics-based numerical models. Recently, deep learning models have challenged this paradigm. However, the latter models may struggle when forecasting weather extremes. In this article, we argue for deep learning models specifically designed to handle extreme events, and we propose a foundational framework to develop such models.
Stefan Rahimi, Lei Huang, Jesse Norris, Alex Hall, Naomi Goldenson, Will Krantz, Benjamin Bass, Chad Thackeray, Henry Lin, Di Chen, Eli Dennis, Ethan Collins, Zachary J. Lebo, Emily Slinskey, Sara Graves, Surabhi Biyani, Bowen Wang, Stephen Cropper, and the UCLA Center for Climate Science Team
Geosci. Model Dev., 17, 2265–2286, https://doi.org/10.5194/gmd-17-2265-2024, https://doi.org/10.5194/gmd-17-2265-2024, 2024
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Romain Pilon and Daniela I. V. Domeisen
Geosci. Model Dev., 17, 2247–2264, https://doi.org/10.5194/gmd-17-2247-2024, https://doi.org/10.5194/gmd-17-2247-2024, 2024
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This paper introduces a new method for detecting atmospheric cloud bands to identify long convective cloud bands that extend from the tropics to the midlatitudes. The algorithm allows for easy use and enables researchers to study the life cycle and climatology of cloud bands and associated rainfall. This method provides insights into the large-scale processes involved in cloud band formation and their connections between different regions, as well as differences across ocean basins.
Salvatore Larosa, Domenico Cimini, Donatello Gallucci, Saverio Teodosio Nilo, and Filomena Romano
Geosci. Model Dev., 17, 2053–2076, https://doi.org/10.5194/gmd-17-2053-2024, https://doi.org/10.5194/gmd-17-2053-2024, 2024
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PyRTlib is an attractive educational tool because it provides a flexible and user-friendly way to broadly simulate how electromagnetic radiation travels through the atmosphere as it interacts with atmospheric constituents (such as gases, aerosols, and hydrometeors). PyRTlib is a so-called radiative transfer model; these are commonly used to simulate and understand remote sensing observations from ground-based, airborne, or satellite instruments.
Joffrey Dumont Le Brazidec, Pierre Vanderbecken, Alban Farchi, Grégoire Broquet, Gerrit Kuhlmann, and Marc Bocquet
Geosci. Model Dev., 17, 1995–2014, https://doi.org/10.5194/gmd-17-1995-2024, https://doi.org/10.5194/gmd-17-1995-2024, 2024
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Our research presents an innovative approach to estimating power plant CO2 emissions from satellite images of the corresponding plumes such as those from the forthcoming CO2M satellite constellation. The exploitation of these images is challenging due to noise and meteorological uncertainties. To overcome these obstacles, we use a deep learning neural network trained on simulated CO2 images. Our method outperforms alternatives, providing a positive perspective for the analysis of CO2M images.
Kyoung-Min Kim, Si-Wan Kim, Seunghwan Seo, Donald R. Blake, Seogju Cho, James H. Crawford, Louisa K. Emmons, Alan Fried, Jay R. Herman, Jinkyu Hong, Jinsang Jung, Gabriele G. Pfister, Andrew J. Weinheimer, Jung-Hun Woo, and Qiang Zhang
Geosci. Model Dev., 17, 1931–1955, https://doi.org/10.5194/gmd-17-1931-2024, https://doi.org/10.5194/gmd-17-1931-2024, 2024
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Three emission inventories were evaluated for East Asia using data acquired during a field campaign in 2016. The inventories successfully reproduced the daily variations of ozone and nitrogen dioxide. However, the spatial distributions of model ozone did not fully agree with the observations. Additionally, all simulations underestimated carbon monoxide and volatile organic compound (VOC) levels. Increasing VOC emissions over South Korea resulted in improved ozone simulations.
Sanam Noreen Vardag and Robert Maiwald
Geosci. Model Dev., 17, 1885–1902, https://doi.org/10.5194/gmd-17-1885-2024, https://doi.org/10.5194/gmd-17-1885-2024, 2024
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We use the atmospheric transport model GRAMM/GRAL in a Bayesian inversion to estimate urban CO2 emissions on a neighbourhood scale. We analyse the effect of varying number, precision and location of CO2 sensors for CO2 flux estimation. We further test the inclusion of co-emitted species and correlation in the inversion. The study showcases the general usefulness of GRAMM/GRAL in measurement network design.
Abhishek Savita, Joakim Kjellsson, Robin Pilch Kedzierski, Mojib Latif, Tabea Rahm, Sebastian Wahl, and Wonsun Park
Geosci. Model Dev., 17, 1813–1829, https://doi.org/10.5194/gmd-17-1813-2024, https://doi.org/10.5194/gmd-17-1813-2024, 2024
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The OpenIFS model is used to examine the impact of horizontal resolutions (HR) and model time steps. We find that the surface wind biases over the oceans, in particular the Southern Ocean, are sensitive to the model time step and HR, with the HR having the smallest biases. When using a coarse-resolution model with a shorter time step, a similar improvement is also found. Climate biases can be reduced in the OpenIFS model at a cheaper cost by reducing the time step rather than increasing the HR.
Ferdinand Briegel, Jonas Wehrle, Dirk Schindler, and Andreas Christen
Geosci. Model Dev., 17, 1667–1688, https://doi.org/10.5194/gmd-17-1667-2024, https://doi.org/10.5194/gmd-17-1667-2024, 2024
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We present a new approach to model heat stress in cities using artificial intelligence (AI). We show that the AI model is fast in terms of prediction but accurate when evaluated with measurements. The fast-predictive AI model enables several new potential applications, including heat stress prediction and warning; downscaling of potential future climates; evaluation of adaptation effectiveness; and, more fundamentally, development of guidelines to support urban planning and policymaking.
Hauke Schmidt, Sebastian Rast, Jiawei Bao, Amrit Cassim, Shih-Wei Fang, Diego Jimenez-de la Cuesta, Paul Keil, Lukas Kluft, Clarissa Kroll, Theresa Lang, Ulrike Niemeier, Andrea Schneidereit, Andrew I. L. Williams, and Bjorn Stevens
Geosci. Model Dev., 17, 1563–1584, https://doi.org/10.5194/gmd-17-1563-2024, https://doi.org/10.5194/gmd-17-1563-2024, 2024
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A recent development in numerical simulations of the global atmosphere is the increase in horizontal resolution to grid spacings of a few kilometers. However, the vertical grid spacing of these models has not been reduced at the same rate as the horizontal grid spacing. Here, we assess the effects of much finer vertical grid spacings, in particular the impacts on cloud quantities and the atmospheric energy balance.
Tao Zheng, Sha Feng, Jeffrey Steward, Xiaoxu Tian, David Baker, and Martin Baxter
Geosci. Model Dev., 17, 1543–1562, https://doi.org/10.5194/gmd-17-1543-2024, https://doi.org/10.5194/gmd-17-1543-2024, 2024
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The tangent linear and adjoint models have been successfully implemented in the MPAS-CO2 system, which has undergone rigorous accuracy testing. This development lays the groundwork for a global carbon flux data assimilation system, which offers the flexibility of high-resolution focus on specific areas, while maintaining a coarser resolution elsewhere. This approach significantly reduces computational costs and is thus perfectly suited for future CO2 geostationery and imager satellites.
Kelvin H. Bates, Mathew J. Evans, Barron H. Henderson, and Daniel J. Jacob
Geosci. Model Dev., 17, 1511–1524, https://doi.org/10.5194/gmd-17-1511-2024, https://doi.org/10.5194/gmd-17-1511-2024, 2024
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Accurate representation of rates and products of chemical reactions in atmospheric models is crucial for simulating concentrations of pollutants and climate forcers. We update the widely used GEOS-Chem atmospheric chemistry model with reaction parameters from recent compilations of experimental data and demonstrate the implications for key atmospheric chemical species. The updates decrease tropospheric CO mixing ratios and increase stratospheric nitrogen oxide mixing ratios, among other changes.
François Roberge, Alejandro Di Luca, René Laprise, Philippe Lucas-Picher, and Julie Thériault
Geosci. Model Dev., 17, 1497–1510, https://doi.org/10.5194/gmd-17-1497-2024, https://doi.org/10.5194/gmd-17-1497-2024, 2024
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Our study addresses a challenge in dynamical downscaling using regional climate models, focusing on the lack of small-scale features near the boundaries. We introduce a method to identify this “spatial spin-up” in precipitation simulations. Results show spin-up distances up to 300 km, varying by season and driving variable. Double nesting with comprehensive variables (e.g. microphysical variables) offers advantages. Findings will help optimize simulations for better climate projections.
Eloisa Raluy-López, Juan Pedro Montávez, and Pedro Jiménez-Guerrero
Geosci. Model Dev., 17, 1469–1495, https://doi.org/10.5194/gmd-17-1469-2024, https://doi.org/10.5194/gmd-17-1469-2024, 2024
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Atmospheric rivers (ARs) represent a significant source of water but are also related to extreme precipitation events. Here, we present a new regional-scale AR identification algorithm and apply it to three simulations that include aerosol interactions at different levels. The results show that aerosols modify the intensity and trajectory of ARs and redistribute the AR-related precipitation. Thus, the correct inclusion of aerosol effects is important in the simulation of AR behavior.
Sofía Gómez Maqueo Anaya, Dietrich Althausen, Matthias Faust, Holger Baars, Bernd Heinold, Julian Hofer, Ina Tegen, Albert Ansmann, Ronny Engelmann, Annett Skupin, Birgit Heese, and Kerstin Schepanski
Geosci. Model Dev., 17, 1271–1295, https://doi.org/10.5194/gmd-17-1271-2024, https://doi.org/10.5194/gmd-17-1271-2024, 2024
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Mineral dust aerosol particles vary greatly in their composition depending on source region, which leads to different physicochemical properties. Most atmosphere–aerosol models consider mineral dust aerosols to be compositionally homogeneous, which ultimately increases model uncertainty. Here, we present an approach to explicitly consider the heterogeneity of the mineralogical composition for simulations of the Saharan atmospheric dust cycle with regard to dust transport towards the Atlantic.
Alexandros Milousis, Alexandra P. Tsimpidi, Holger Tost, Spyros N. Pandis, Athanasios Nenes, Astrid Kiendler-Scharr, and Vlassis A. Karydis
Geosci. Model Dev., 17, 1111–1131, https://doi.org/10.5194/gmd-17-1111-2024, https://doi.org/10.5194/gmd-17-1111-2024, 2024
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This study aims to evaluate the newly developed ISORROPIA-lite aerosol thermodynamic module within the EMAC model and explore discrepancies in global atmospheric simulations of aerosol composition and acidity by utilizing different aerosol phase states. Even though local differences were found in regions where the RH ranged from 20 % to 60 %, on a global scale the results are similar. Therefore, ISORROPIA-lite can be a reliable and computationally effective alternative to ISORROPIA II in EMAC.
Marie-Adèle Magnaldo, Quentin Libois, Sébastien Riette, and Christine Lac
Geosci. Model Dev., 17, 1091–1109, https://doi.org/10.5194/gmd-17-1091-2024, https://doi.org/10.5194/gmd-17-1091-2024, 2024
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With the worldwide development of the solar energy sector, the need for reliable solar radiation forecasts has significantly increased. However, meteorological models that predict, among others things, solar radiation have errors. Therefore, we wanted to know in which situtaions these errors are most significant. We found that errors mostly occur in cloudy situations, and different errors were highlighted depending on the cloud altitude. Several potential sources of errors were identified.
Dongqi Lin, Jiawei Zhang, Basit Khan, Marwan Katurji, and Laura E. Revell
Geosci. Model Dev., 17, 815–845, https://doi.org/10.5194/gmd-17-815-2024, https://doi.org/10.5194/gmd-17-815-2024, 2024
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GEO4PALM is an open-source tool to generate static input for the Parallelized Large-Eddy Simulation (PALM) model system. Geospatial static input is essential for realistic PALM simulations. However, existing tools fail to generate PALM's geospatial static input for most regions. GEO4PALM is compatible with diverse geospatial data sources and provides access to free data sets. In addition, this paper presents two application examples, which show successful PALM simulations using GEO4PALM.
Piotr Zmijewski, Piotr Dziekan, and Hanna Pawlowska
Geosci. Model Dev., 17, 759–780, https://doi.org/10.5194/gmd-17-759-2024, https://doi.org/10.5194/gmd-17-759-2024, 2024
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In computer simulations of clouds it is necessary to model the myriad of droplets that constitute a cloud. A popular method for this is to use so-called super-droplets (SDs), each representing many real droplets. It has remained a challenge to model collisions of SDs. We study how precipitation in a cumulus cloud depends on the number of SDs. Surprisingly, we do not find convergence in mean precipitation even for numbers of SDs much larger than typically used in simulations.
Roya Ghahreman, Wanmin Gong, Paul A. Makar, Alexandru Lupu, Amanda Cole, Kulbir Banwait, Colin Lee, and Ayodeji Akingunola
Geosci. Model Dev., 17, 685–707, https://doi.org/10.5194/gmd-17-685-2024, https://doi.org/10.5194/gmd-17-685-2024, 2024
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The article explores the impact of different representations of below-cloud scavenging on model biases. A new scavenging scheme and precipitation-phase partitioning improve the model's performance, with better SO42- scavenging and wet deposition of NO3- and NH4+.
Daisuke Goto, Tatsuya Seiki, Kentaroh Suzuki, Hisashi Yashiro, and Toshihiko Takemura
Geosci. Model Dev., 17, 651–684, https://doi.org/10.5194/gmd-17-651-2024, https://doi.org/10.5194/gmd-17-651-2024, 2024
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Global climate models with coarse grid sizes include uncertainties about the processes in aerosol–cloud–precipitation interactions. To reduce these uncertainties, here we performed numerical simulations using a new version of our global aerosol transport model with a finer grid size over a longer period than in our previous study. As a result, we found that the cloud microphysics module influences the aerosol distributions through both aerosol wet deposition and aerosol–cloud interactions.
Alexander de Meij, Cornelis Cuvelier, Philippe Thunis, Enrico Pisoni, and Bertrand Bessagnet
Geosci. Model Dev., 17, 587–606, https://doi.org/10.5194/gmd-17-587-2024, https://doi.org/10.5194/gmd-17-587-2024, 2024
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In our study the robustness of the model responses to emission reductions in the EU is assessed when the emission data are changed. Our findings are particularly important to better understand the uncertainties associated to the emission inventories and how these uncertainties impact the level of accuracy of the resulting air quality modelling, which is a key for designing air quality plans. Also crucial is the choice of indicator to avoid misleading interpretations of the results.
Haiqin Li, Georg A. Grell, Ravan Ahmadov, Li Zhang, Shan Sun, Jordan Schnell, and Ning Wang
Geosci. Model Dev., 17, 607–619, https://doi.org/10.5194/gmd-17-607-2024, https://doi.org/10.5194/gmd-17-607-2024, 2024
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We developed a simple and realistic method to provide aerosol emissions for aerosol-aware microphysics in a numerical weather forecast model. The cloud-radiation differences between the experimental (EXP) and control (CTL) experiments responded to the aerosol differences. The strong positive precipitation biases over North America and Europe from the CTL run were significantly reduced in the EXP run. This study shows that a realistic representation of aerosol emissions should be considered.
Nathan Patrick Arnold
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2023-245, https://doi.org/10.5194/gmd-2023-245, 2024
Revised manuscript accepted for GMD
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Earth System Models often represent the land surface at smaller scales than the atmosphere, but surface-atmosphere coupling uses only aggregated surface properties. This study presents a method to allow heterogeneous surface properties to modify boundary layer updrafts. The method is tested in single column experiments. Updraft properties are found to reasonably covary with surface conditions, and simulated boundary layer variability is enhanced over more heterogeneous land surfaces.
Giancarlo Ciarelli, Sara Tahvonen, Arineh Cholakian, Manuel Bettineschi, Bruno Vitali, Tuukka Petäjä, and Federico Bianchi
Geosci. Model Dev., 17, 545–565, https://doi.org/10.5194/gmd-17-545-2024, https://doi.org/10.5194/gmd-17-545-2024, 2024
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The terrestrial ecosystem releases large quantities of biogenic gases in the Earth's Atmosphere. These gases can effectively be converted into so-called biogenic aerosol particles and, eventually, affect the Earth's climate. Climate prediction varies greatly depending on how these processes are represented in model simulations. In this study, we present a detailed model evaluation analysis aimed at understanding the main source of uncertainty in predicting the formation of biogenic aerosols.
Jiachen Liu, Eric Chen, and Shannon L. Capps
Geosci. Model Dev., 17, 567–585, https://doi.org/10.5194/gmd-17-567-2024, https://doi.org/10.5194/gmd-17-567-2024, 2024
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Air pollution harms human life and ecosystems, but its sources are complex. Scientists and policy makers use air pollution models to advance knowledge and inform control strategies. We implemented a recently developed numeral system to relate any set of model inputs, like pollutant emissions from a given activity, to all model outputs, like concentrations of pollutants harming human health. This approach will be straightforward to update when scientists discover new processes in the atmosphere.
Gerrit Kuhlmann, Erik F. M. Koene, Sandro Meier, Diego Santaren, Grégoire Broquet, Frédéric Chevallier, Janne Hakkarainen, Janne Nurmela, Laia Amorós, Johanna Tamminen, and Dominik Brunner
EGUsphere, https://doi.org/10.5194/egusphere-2023-2936, https://doi.org/10.5194/egusphere-2023-2936, 2024
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We present a Python software library for data-driven emission quantification (ddeq). It can be used to determine the emissions of hot spots (cities, power plants and industry) from remote sensing images using different methods. ddeq can be extended for new datasets and methods, providing a powerful community tool for users and developers. The application of the methods is shown using Jupyter Notebooks included in the library.
Kun Zheng, Qiya Tan, Huihua Ruan, Jinbiao Zhang, Cong Luo, Siyu Tang, Yunlei Yi, Yugang Tian, and Jianmei Cheng
Geosci. Model Dev., 17, 399–413, https://doi.org/10.5194/gmd-17-399-2024, https://doi.org/10.5194/gmd-17-399-2024, 2024
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Radar echo extrapolation is the common method in precipitation nowcasting. Deep learning has potential in extrapolation. However, the existing models have low prediction accuracy for heavy rainfall. In this study, the prediction accuracy is improved by suppressing the blurring effect of rain distribution and reducing the negative bias. The results show that our model has better performance, which is useful for urban operation and flood prevention.
Li Pan, Partha S. Bhattacharjee, Li Zhang, Raffaele Montuoro, Barry Baker, Jeff McQueen, Georg A. Grell, Stuart A. McKeen, Shobha Kondragunta, Xiaoyang Zhang, Gregory J. Frost, Fanglin Yang, and Ivanka Stajner
Geosci. Model Dev., 17, 431–447, https://doi.org/10.5194/gmd-17-431-2024, https://doi.org/10.5194/gmd-17-431-2024, 2024
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A GEFS-Aerosols simulation was conducted from 1 September 2019 to 30 September 2020 to evaluate the model performance of GEFS-Aerosols. The purpose of this study was to understand how aerosol chemical and physical processes affect ambient aerosol concentrations by placing aerosol wet deposition, dry deposition, reactions, gravitational deposition, and emissions into the aerosol mass balance equation.
Sean Raffuse, Susan O'Neill, and Rebecca Schmidt
Geosci. Model Dev., 17, 381–397, https://doi.org/10.5194/gmd-17-381-2024, https://doi.org/10.5194/gmd-17-381-2024, 2024
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Large wildfires are increasing throughout the western United States, and wildfire smoke is hazardous to public health. We developed a suite of tools called rapidfire for estimating particle pollution during wildfires using routinely available data sets. rapidfire uses official air monitoring, satellite data, meteorology, smoke modeling, and low-cost sensors. Estimates from rapidfire compare well with ground monitors and are being used in public health studies across California.
Manuel F. Schmid, Marco G. Giometto, Gregory A. Lawrence, and Marc B. Parlange
Geosci. Model Dev., 17, 321–333, https://doi.org/10.5194/gmd-17-321-2024, https://doi.org/10.5194/gmd-17-321-2024, 2024
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Turbulence-resolving flow models have strict performance requirements, as simulations often run for weeks using hundreds of processes. Many flow scenarios also require the flexibility to modify physical and numerical models for problem-specific requirements. With a new code written in Julia we hope to make such adaptations easier without compromising on performance. In this paper we discuss the modeling approach and present validation and performance results.
Yafang Guo, Chayan Roychoudhury, Mohammad Amin Mirrezaei, Rajesh Kumar, Armin Sorooshian, and Avelino F. Arellano
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2023-234, https://doi.org/10.5194/gmd-2023-234, 2024
Revised manuscript accepted for GMD
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This research focuses on surface ozone (O3) pollution in Arizona, a historically air quality-challenged arid/semi-arid region in the US. The unique characteristics of semi-arid/arid regions, e.g., intense heat, minimal moisture, persistent desert shrubs, play a vital role in comprehending O3 exceedances. Using the WRF-Chem model, we analyzed O3 levels in the pre-monsoon month, revealing the model's skill in capturing diurnal and MDA8 O3 levels.
Marie-Noëlle Bouin, Cindy Lebeaupin Brossier, Sylvie Malardel, Aurore Voldoire, and César Sauvage
Geosci. Model Dev., 17, 117–141, https://doi.org/10.5194/gmd-17-117-2024, https://doi.org/10.5194/gmd-17-117-2024, 2024
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In numerical models, the turbulent exchanges of heat and momentum at the air–sea interface are not represented explicitly but with parameterisations depending on the surface parameters. A new parameterisation of turbulent fluxes (WASP) has been implemented in the surface model SURFEX v8.1 and validated on four case studies. It combines a close fit to observations including cyclonic winds, a dependency on the wave growth rate, and the possibility of being used in atmosphere–wave coupled models.
Michal Belda, Nina Benešová, Jaroslav Resler, Peter Huszár, Ondřej Vlček, Pavel Krč, Jan Karlický, Pavel Juruš, and Kryštof Eben
EGUsphere, https://doi.org/10.5194/egusphere-2023-2740, https://doi.org/10.5194/egusphere-2023-2740, 2024
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For modeling atmospheric chemistry, it is necessary to provide data on emissions of pollutants. These can come from various sources and in various forms and preprocessing of the data to be ingestible by chemistry models can be quite challenging. We developed the FUME processor to use a database layer that internally transforms all input data into a rigid structure facilitating further processing to allow emission processing from continental to street scale.
Najmeh Kaffashzadeh and Abbas Ali Aliakbari Bidokhti
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2023-226, https://doi.org/10.5194/gmd-2023-226, 2024
Revised manuscript accepted for GMD
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Reanalysis data have been widely used as an initial condition for the daily forecast of the atmosphere or boundary conditions in regional models, for the study of climate change, and as proxies to complement insufficient in situ measurements. This paper assesses the capability of two state-of-the-art global datasets in simulating surface ozone over Iran using a new methodology.
Zehua Bai, Qizhong Wu, Kai Cao, Yiming Sun, and Huaqiong Cheng
EGUsphere, https://doi.org/10.5194/egusphere-2023-2962, https://doi.org/10.5194/egusphere-2023-2962, 2024
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There are relatively limited researches on the application of scientific computing on RISC CPU platforms. The MIPS architecture CPUs, a type of RISC CPU, have distinct advantages in energy efficiency and scalability. In this study, the air quality modeling system can run stably on MIPS CPU platform, and the experiment results verify the stability of scientific computing on the platform. The work provides a technical foundation for the scientific application based on MIPS CPU platforms.
Lukas Fehr, Chris McLinden, Debora Griffin, Daniel Zawada, Doug Degenstein, and Adam Bourassa
Geosci. Model Dev., 16, 7491–7507, https://doi.org/10.5194/gmd-16-7491-2023, https://doi.org/10.5194/gmd-16-7491-2023, 2023
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This work highlights upgrades to SASKTRAN, a model that simulates sunlight interacting with the atmosphere to help measure trace gases. The upgrades were verified by detailed comparisons between different numerical methods. A case study was performed using SASKTRAN’s multidimensional capabilities, which found that ignoring horizontal variation in the atmosphere (a common practice in the field) can introduce non-negligible errors where there is snow or high pollution.
Sylvain Mailler, Romain Pennel, Laurent Menut, and Arineh Cholakian
Geosci. Model Dev., 16, 7509–7526, https://doi.org/10.5194/gmd-16-7509-2023, https://doi.org/10.5194/gmd-16-7509-2023, 2023
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We show that a new advection scheme named PPM + W (piecewise parabolic method + Walcek) offers geoscientific modellers an alternative, high-performance scheme designed for Cartesian-grid advection, with improved performance over the classical PPM scheme. The computational cost of PPM + W is not higher than that of PPM. With improved accuracy and controlled computational cost, this new scheme may find applications in chemistry-transport models, ocean models or atmospheric circulation models.
David R. Shaw, Toby J. Carter, Helen L. Davies, Ellen Harding-Smith, Elliott C. Crocker, Georgia Beel, Zixu Wang, and Nicola Carslaw
Geosci. Model Dev., 16, 7411–7431, https://doi.org/10.5194/gmd-16-7411-2023, https://doi.org/10.5194/gmd-16-7411-2023, 2023
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Exposure to air pollution is one of the greatest risks to human health, and it is indoors, where we spend upwards of 90 % of our time, that our exposure is greatest. The INdoor CHEMical model in Python (INCHEM-Py) is a new, community-led box model that tracks the evolution and fate of atmospheric chemical pollutants indoors. We have shown the processes simulated by INCHEM-Py, its ability to model experimental data and how it may be used to develop further understanding of indoor air chemistry.
Willem E. van Caspel, David Simpson, Jan Eiof Jonson, Anna M. K. Benedictow, Yao Ge, Alcide di Sarra, Giandomenico Pace, Massimo Vieno, Hannah L. Walker, and Mathew R. Heal
Geosci. Model Dev., 16, 7433–7459, https://doi.org/10.5194/gmd-16-7433-2023, https://doi.org/10.5194/gmd-16-7433-2023, 2023
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Radiation coming from the sun is essential to atmospheric chemistry, driving the breakup, or photodissociation, of atmospheric molecules. This in turn affects the chemical composition and reactivity of the atmosphere. The representation of photodissociation effects is therefore essential in atmospheric chemistry modeling. One such model is the EMEP MSC-W model, for which a new way of calculating the photodissociation rates is tested and evaluated in this paper.
Jungmin Lee, Walter M. Hannah, and David C. Bader
Geosci. Model Dev., 16, 7275–7287, https://doi.org/10.5194/gmd-16-7275-2023, https://doi.org/10.5194/gmd-16-7275-2023, 2023
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Representing accurate land–atmosphere interaction processes is overlooked in weather and climate models. In this study, we propose three methods to represent land–atmosphere coupling in the Energy Exascale Earth System Model (E3SM) with the Multi-scale Modeling Framework (MMF) approach. In this study, we introduce spatially homogeneous and heterogeneous land–atmosphere interaction processes within the cloud-resolving model domain. Our 5-year simulations reveal only small differences.
Laurent Menut, Bertrand Bessagnet, Arineh Cholakian, Guillaume Siour, Sylvain Mailler, and Romain Pennel
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2023-209, https://doi.org/10.5194/gmd-2023-209, 2023
Revised manuscript accepted for GMD
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This study is about the modelling of the atmospheric composition in Europe and during the summer 2022, when massive wildfires were observed. It is a sensitivity study dedicated to the relative impact of two modelling processes able to modify the meteorology used for the calculation of the atmospheric chemistry and transport of pollutants.
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Short summary
Large air quality and climate models calculate different physical and chemical phenomena in separate operators within the overall model, some of which are computationally intensive. Machine learning tools can memorize the behavior of these operators and replace them, but the replacements must still obey physical laws, like conservation principles. This work derives a mathematical framework for machine learning replacements that conserves properties, such as mass or energy, to machine precision.
Large air quality and climate models calculate different physical and chemical phenomena in...
