Articles | Volume 13, issue 3
https://doi.org/10.5194/gmd-13-1223-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/gmd-13-1223-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Description and evaluation of the UKCA stratosphere–troposphere chemistry scheme (StratTrop vn 1.0) implemented in UKESM1
Department of Chemistry, University of Cambridge, Cambridge, CB2 1EW, UK
NCAS-Climate, University of Cambridge, CB2 1EW, UK
Fiona M. O'Connor
Met Office Hadley Centre, FitzRoy Road, Exeter, EX1 3PB, UK
Nathan Luke Abraham
Department of Chemistry, University of Cambridge, Cambridge, CB2 1EW, UK
NCAS-Climate, University of Cambridge, CB2 1EW, UK
Scott Archer-Nicholls
Department of Chemistry, University of Cambridge, Cambridge, CB2 1EW, UK
Martyn P. Chipperfield
School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UK
National Centre for Earth Observation (NCEO), University of Leeds, Leeds, UK
Mohit Dalvi
Met Office Hadley Centre, FitzRoy Road, Exeter, EX1 3PB, UK
Gerd A. Folberth
Met Office Hadley Centre, FitzRoy Road, Exeter, EX1 3PB, UK
Fraser Dennison
National Institute of Water & Atmospheric Research Ltd (NIWA), 301 Evans
Bay Parade, Greta Point, Wellington, New Zealand
now at: CSIRO Oceans and Atmosphere, Aspendale, Australia
Sandip S. Dhomse
School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UK
National Centre for Earth Observation (NCEO), University of Leeds, Leeds, UK
Paul T. Griffiths
Department of Chemistry, University of Cambridge, Cambridge, CB2 1EW, UK
NCAS-Climate, University of Cambridge, CB2 1EW, UK
Catherine Hardacre
Met Office Hadley Centre, FitzRoy Road, Exeter, EX1 3PB, UK
Alan J. Hewitt
Met Office Hadley Centre, FitzRoy Road, Exeter, EX1 3PB, UK
Richard S. Hill
Met Office Hadley Centre, FitzRoy Road, Exeter, EX1 3PB, UK
Colin E. Johnson
Met Office Hadley Centre, FitzRoy Road, Exeter, EX1 3PB, UK
James Keeble
Department of Chemistry, University of Cambridge, Cambridge, CB2 1EW, UK
NCAS-Climate, University of Cambridge, CB2 1EW, UK
Marcus O. Köhler
Department of Chemistry, University of Cambridge, Cambridge, CB2 1EW, UK
Centre for Ocean and Atmospheric Sciences, School of Environmental Sciences, University of East Anglia, Norwich, UK
now at ECMWF, Reading, UK
Olaf Morgenstern
National Institute of Water & Atmospheric Research Ltd (NIWA), 301 Evans
Bay Parade, Greta Point, Wellington, New Zealand
Jane P. Mulcahy
Met Office Hadley Centre, FitzRoy Road, Exeter, EX1 3PB, UK
Carlos Ordóñez
Met Office Hadley Centre, FitzRoy Road, Exeter, EX1 3PB, UK
now at: Departamento de Física de la Tierra y
Astrofísica, Facultad de Ciencias Físicas, Universidad Complutense
de Madrid, Madrid 28040, Spain
Richard J. Pope
School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UK
National Centre for Earth Observation (NCEO), University of Leeds, Leeds, UK
Steven T. Rumbold
NCAS-Climate, Department of Meteorology, University of Reading, Reading, RG6 6BB, UK
Maria R. Russo
Department of Chemistry, University of Cambridge, Cambridge, CB2 1EW, UK
NCAS-Climate, University of Cambridge, CB2 1EW, UK
Nicholas H. Savage
Met Office Hadley Centre, FitzRoy Road, Exeter, EX1 3PB, UK
Alistair Sellar
Met Office Hadley Centre, FitzRoy Road, Exeter, EX1 3PB, UK
Marc Stringer
NCAS-Climate, Department of Meteorology, University of Reading, Reading, RG6 6BB, UK
Steven T. Turnock
Met Office Hadley Centre, FitzRoy Road, Exeter, EX1 3PB, UK
Oliver Wild
Lancaster Environment Centre, Lancaster University, Lancaster, LA1 4YQ, UK
Guang Zeng
National Institute of Water & Atmospheric Research Ltd (NIWA), 301 Evans
Bay Parade, Greta Point, Wellington, New Zealand
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- Modulation of daily PM2.5 concentrations over China in winter by large-scale circulation and climate change Z. Jia et al. 10.5194/acp-23-2829-2023
- The Future Climate and Air Quality Response From Different Near‐Term Climate Forcer, Climate, and Land‐Use Scenarios Using UKESM1 S. Turnock et al. 10.1029/2022EF002687
- Atmospheric composition and climate impacts of a future hydrogen economy N. Warwick et al. 10.5194/acp-23-13451-2023
- Atmospheric impacts of chlorinated very short-lived substances over the recent past – Part 2: Impacts on ozone E. Bednarz et al. 10.5194/acp-23-13701-2023
- The Antarctic contribution to 21st-century sea-level rise predicted by the UK Earth System Model with an interactive ice sheet A. Siahaan et al. 10.5194/tc-16-4053-2022
- ACCESS-CM2-Chem: evaluation of southern hemisphere ozone and its effect on the Southern Annular Mode F. Dennison et al. 10.1071/ES22015
- The simulation of mineral dust in the United Kingdom Earth System Model UKESM1 S. Woodward et al. 10.5194/acp-22-14503-2022
- The development of the Atmospheric Measurements by Ultra-Light Spectrometer (AMULSE) greenhouse gas profiling system and application for satellite retrieval validation L. Joly et al. 10.5194/amt-13-3099-2020
- Climate Benefits of Cleaner Energy Transitions in East and South Asia Through Black Carbon Reduction S. Ramachandran et al. 10.3389/fenvs.2022.842319
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- Updated isoprene and terpene emission factors for the Interactive BVOC (iBVOC) emission scheme in the United Kingdom Earth System Model (UKESM1.0) J. Weber et al. 10.5194/gmd-16-3083-2023
- Radiative impact of improved global parameterisations of oceanic dry deposition of ozone and lightning-generated NOx A. Luhar et al. 10.5194/acp-22-13013-2022
- Description and evaluation of the new UM–UKCA (vn11.0) Double Extended Stratospheric–Tropospheric (DEST vn1.0) scheme for comprehensive modelling of halogen chemistry in the stratosphere E. Bednarz et al. 10.5194/gmd-16-6187-2023
- Assessing and improving cloud-height-based parameterisations of global lightning flash rate, and their impact on lightning-produced NO<sub><i>x</i></sub> and tropospheric composition in a chemistry–climate model A. Luhar et al. 10.5194/acp-21-7053-2021
- The impact of ozone on Earth-like exoplanet climate dynamics: the case of Proxima Centauri b P. De Luca et al. 10.1093/mnras/stae1199
- Exploring the sensitivity of atmospheric nitrate concentrations to nitric acid uptake rate using the Met Office's Unified Model A. Jones et al. 10.5194/acp-21-15901-2021
- Evaluating the simulated radiative forcings, aerosol properties, and stratospheric warmings from the 1963 Mt Agung, 1982 El Chichón, and 1991 Mt Pinatubo volcanic aerosol clouds S. Dhomse et al. 10.5194/acp-20-13627-2020
- Identifying climate model structural inconsistencies allows for tight constraint of aerosol radiative forcing L. Regayre et al. 10.5194/acp-23-8749-2023
- Historical total ozone radiative forcing derived from CMIP6 simulations R. Skeie et al. 10.1038/s41612-020-00131-0
- Opinion: Stratospheric ozone – depletion, recovery and new challenges M. Chipperfield & S. Bekki 10.5194/acp-24-2783-2024
- Description and evaluation of aerosol in UKESM1 and HadGEM3-GC3.1 CMIP6 historical simulations J. Mulcahy et al. 10.5194/gmd-13-6383-2020
- Australian wildfires cause the largest stratospheric warming since Pinatubo and extends the lifetime of the Antarctic ozone hole L. Damany-Pearce et al. 10.1038/s41598-022-15794-3
- Co-emission of volcanic sulfur and halogens amplifies volcanic effective radiative forcing J. Staunton-Sykes et al. 10.5194/acp-21-9009-2021
- Development, intercomparison, and evaluation of an improved mechanism for the oxidation of dimethyl sulfide in the UKCA model B. Cala et al. 10.5194/acp-23-14735-2023
- The role of future anthropogenic methane emissions in air quality and climate Z. Staniaszek et al. 10.1038/s41612-022-00247-5
- A multi-model assessment of the Global Warming Potential of hydrogen M. Sand et al. 10.1038/s43247-023-00857-8
- Assessment of pre-industrial to present-day anthropogenic climate forcing in UKESM1 F. O'Connor et al. 10.5194/acp-21-1211-2021
- Development of the UKESM-TOPAZ Earth System Model (Version 1.0) and Preliminary Evaluation of its Biogeochemical Simulations H. Lee et al. 10.1007/s13143-021-00263-0
- Investigation of the impact of satellite vertical sensitivity on long-term retrieved lower-tropospheric ozone trends R. Pope et al. 10.5194/acp-24-9177-2024
- Assessing the Impact of Stratospheric Aerosol Injection on US Convective Weather Environments I. Glade et al. 10.1029/2023EF004041
- Spin‐up of UK Earth System Model 1 (UKESM1) for CMIP6 A. Yool et al. 10.1029/2019MS001933
- Comparison of UKESM1 and CESM2 simulations using the same multi-target stratospheric aerosol injection strategy M. Henry et al. 10.5194/acp-23-13369-2023
- On the magnitude and sensitivity of the quasi-biennial oscillation response to a tropical volcanic eruption F. Brown et al. 10.5194/acp-23-5335-2023
- Evaluation of SO<sub>2</sub>, SO<sub>4</sub><sup>2−</sup> and an updated SO<sub>2</sub> dry deposition parameterization in the United Kingdom Earth System Model C. Hardacre et al. 10.5194/acp-21-18465-2021
- The Impacts of Aerosol Emissions on Historical Climate in UKESM1 J. Seo et al. 10.3390/atmos11101095
- Coupling interactive fire with atmospheric composition and climate in the UK Earth System Model J. Teixeira et al. 10.5194/gmd-14-6515-2021
- Decomposing the effective radiative forcing of anthropogenic aerosols based on CMIP6 Earth system models A. Kalisoras et al. 10.5194/acp-24-7837-2024
- Large-scale ozone episodes in Europe: Decreasing sizes in the last decades but diverging changes in the future R. Crespo-Miguel et al. 10.1016/j.scitotenv.2024.175071
- Tropospheric ozone in CMIP6 simulations P. Griffiths et al. 10.5194/acp-21-4187-2021
- Effective radiative forcing from emissions of reactive gases and aerosols – a multi-model comparison G. Thornhill et al. 10.5194/acp-21-853-2021
- A study of the effect of aerosols on surface ozone through meteorology feedbacks over China Y. Qu et al. 10.5194/acp-21-5705-2021
- UKESM1.1: development and evaluation of an updated configuration of the UK Earth System Model J. Mulcahy et al. 10.5194/gmd-16-1569-2023
- The Social Cost of Ozone‐Related Mortality Impacts From Methane Emissions E. McDuffie et al. 10.1029/2023EF003853
- Evaluating the physical and biogeochemical state of the global ocean component of UKESM1 in CMIP6 historical simulations A. Yool et al. 10.5194/gmd-14-3437-2021
- Trends in global tropospheric hydroxyl radical and methane lifetime since 1850 from AerChemMIP D. Stevenson et al. 10.5194/acp-20-12905-2020
- Investigating variable importance in ground-level ozone formation with supervised learning Y. Chen et al. 10.1016/j.atmosenv.2022.119148
- The decomposition of cloud–aerosol forcing in the UK Earth System Model (UKESM1) D. Grosvenor & K. Carslaw 10.5194/acp-20-15681-2020
- Interactive stratospheric aerosol models' response to different amounts and altitudes of SO2 injection during the 1991 Pinatubo eruption I. Quaglia et al. 10.5194/acp-23-921-2023
- Tropospheric Ozone Assessment Report A. Archibald et al. 10.1525/elementa.2020.034
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- Comparison of particle number size distribution trends in ground measurements and climate models V. Leinonen et al. 10.5194/acp-22-12873-2022
- Quantifying the tropospheric ozone radiative effect and its temporal evolution in the satellite era R. Pope et al. 10.5194/acp-24-3613-2024
- Climate-driven chemistry and aerosol feedbacks in CMIP6 Earth system models G. Thornhill et al. 10.5194/acp-21-1105-2021
- Atmospheric isoprene measurements reveal larger-than-expected Southern Ocean emissions V. Ferracci et al. 10.1038/s41467-024-46744-4
- Atmospheric impacts of chlorinated very short-lived substances over the recent past – Part 1: Stratospheric chlorine budget and the role of transport E. Bednarz et al. 10.5194/acp-22-10657-2022
- Chemistry-driven changes strongly influence climate forcing from vegetation emissions J. Weber et al. 10.1038/s41467-022-34944-9
- Significant human health co-benefits of mitigating African emissions C. Wells et al. 10.5194/acp-24-1025-2024
- Coupling the U.K. Earth System Model to Dynamic Models of the Greenland and Antarctic Ice Sheets R. Smith et al. 10.1029/2021MS002520
- Impacts of reducing scattering and absorbing aerosols on the temporal extent and intensity of South Asian summer monsoon and East Asian summer monsoon C. Fang et al. 10.5194/acp-23-8341-2023
- Utilising a multi-proxy to model comparison to constrain the season and regionally heterogeneous impacts of the Mt Samalas 1257 eruption L. Wainman et al. 10.5194/cp-20-951-2024
- Intercomparison of the representations of the atmospheric chemistry of pre-industrial methane and ozone in earth system and other global chemistry-transport models R. Derwent et al. 10.1016/j.atmosenv.2021.118248
- Benefits of net-zero policies for future ozone pollution in China Z. Liu et al. 10.5194/acp-23-13755-2023
- The Influence of Internal Climate Variability on Stratospheric Water Vapor Increases After Large‐Magnitude Explosive Tropical Volcanic Eruptions X. Zhou et al. 10.1029/2023GL103076
- CRI-HOM: A novel chemical mechanism for simulating highly oxygenated organic molecules (HOMs) in global chemistry–aerosol–climate models J. Weber et al. 10.5194/acp-20-10889-2020
- Methane Emissions in a Chemistry‐Climate Model: Feedbacks and Climate Response I. Heimann et al. 10.1029/2019MS002019
- Below-cloud scavenging of aerosol by rain: a review of numerical modelling approaches and sensitivity simulations with mineral dust in the Met Office's Unified Model A. Jones et al. 10.5194/acp-22-11381-2022
- Tropospheric ozone changes and ozone sensitivity from the present day to the future under shared socio-economic pathways Z. Liu et al. 10.5194/acp-22-1209-2022
- Global agricultural N2O emission reduction strategies deliver climate benefits with minimal impact on stratospheric O3 recovery J. Weber et al. 10.1038/s41612-024-00678-2
- Change from aerosol-driven to cloud-feedback-driven trend in short-wave radiative flux over the North Atlantic D. Grosvenor & K. Carslaw 10.5194/acp-23-6743-2023
- Local and remote climate impacts of future African aerosol emissions C. Wells et al. 10.5194/acp-23-3575-2023
- Future Climate Change Impact on the Nyabugogo Catchment Water Balance in Rwanda A. Umugwaneza et al. 10.3390/w13243636
- Improvements to the representation of BVOC chemistry–climate interactions in UKCA (v11.5) with the CRI-Strat 2 mechanism: incorporation and evaluation J. Weber et al. 10.5194/gmd-14-5239-2021
- Seasonal, interannual and decadal variability of tropospheric ozone in the North Atlantic: comparison of UM-UKCA and remote sensing observations for 2005–2018 M. Russo et al. 10.5194/acp-23-6169-2023
- Methane removal and the proportional reductions in surface temperature and ozone S. Abernethy et al. 10.1098/rsta.2021.0104
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- Climate Projections Very Likely Underestimate Future Volcanic Forcing and Its Climatic Effects M. Chim et al. 10.1029/2023GL103743
- Large simulated future changes in the nitrate radical under the CMIP6 SSP scenarios: implications for oxidation chemistry S. Archer-Nicholls et al. 10.5194/acp-23-5801-2023
- Lightning-induced chemistry on tidally-locked Earth-like exoplanets M. Braam et al. 10.1093/mnras/stac2722
- Climate response to off-equatorial stratospheric sulfur injections in three Earth system models – Part 1: Experimental protocols and surface changes D. Visioni et al. 10.5194/acp-23-663-2023
- Projected future changes in extreme precipitation over China under stratospheric aerosol intervention in the UKESM1 climate model O. Wang et al. 10.5194/acp-24-12355-2024
- Including ash in UKESM1 model simulations of the Raikoke volcanic eruption reveals improved agreement with observations A. Wells et al. 10.5194/acp-23-3985-2023
- Contrasting chemical environments in summertime for atmospheric ozone across major Chinese industrial regions: the effectiveness of emission control strategies Z. Liu et al. 10.5194/acp-21-10689-2021
- The ozone–climate penalty over South America and Africa by 2100 F. Brown et al. 10.5194/acp-22-12331-2022
- On the changes in surface ozone over the twenty-first century: sensitivity to changes in surface temperature and chemical mechanisms A. Archibald et al. 10.1098/rsta.2019.0329
- Description and Evaluation of an Emission‐Driven and Fully Coupled Methane Cycle in UKESM1 G. Folberth et al. 10.1029/2021MS002982
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- An Implicit Air Quality Bias Due to the State of Pristine Aerosol X. Zhao et al. 10.1029/2021EF001979
- Climate Change Projection in the Twenty-First Century Simulated by NIMS-KMA CMIP6 Model Based on New GHGs Concentration Pathways H. Sung et al. 10.1007/s13143-021-00225-6
Latest update: 19 Nov 2024
Short summary
Here we present a description and evaluation of the UKCA stratosphere–troposphere chemistry scheme (StratTrop vn 1.0) implemented in the UK Earth System Model (UKESM1). UKCA StratTrop represents a substantial step forward compared to previous versions of UKCA. We show here that it is fully suited to the challenges of representing interactions in a coupled Earth system model and identify key areas and components for future development that will make it even better in the future.
Here we present a description and evaluation of the UKCA stratosphere–troposphere chemistry...