Articles | Volume 12, issue 8
https://doi.org/10.5194/gmd-12-3439-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/gmd-12-3439-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Model evaluation paper
| 
06 Aug 2019
Model evaluation paper |
| 06 Aug 2019
| 06 Aug 2019
Revised treatment of wet scavenging processes dramatically improves GEOS-Chem 12.0.0 simulations of surface nitric acid, nitrate, and ammonium over the United States
Atmospheric Sciences Research Center, University at Albany, Albany, New York, USA
Fangqun Yu
Atmospheric Sciences Research Center, University at Albany, Albany, New York, USA
James Schwab
Atmospheric Sciences Research Center, University at Albany, Albany, New York, USA
Viewed
Total article views: 3,728 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 07 Mar 2019)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 2,576 | 1,097 | 55 | 3,728 | 196 | 64 | 70 |
- HTML: 2,576
- PDF: 1,097
- XML: 55
- Total: 3,728
- Supplement: 196
- BibTeX: 64
- EndNote: 70
Total article views: 3,075 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 06 Aug 2019)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 2,253 | 773 | 49 | 3,075 | 196 | 57 | 59 |
- HTML: 2,253
- PDF: 773
- XML: 49
- Total: 3,075
- Supplement: 196
- BibTeX: 57
- EndNote: 59
Total article views: 653 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 07 Mar 2019)
| HTML | XML | Total | BibTeX | EndNote | |
|---|---|---|---|---|---|
| 323 | 324 | 6 | 653 | 7 | 11 |
- HTML: 323
- PDF: 324
- XML: 6
- Total: 653
- BibTeX: 7
- EndNote: 11
Viewed (geographical distribution)
Total article views: 3,728 (including HTML, PDF, and XML)
Thereof 3,377 with geography defined
and 351 with unknown origin.
Total article views: 3,075 (including HTML, PDF, and XML)
Thereof 2,779 with geography defined
and 296 with unknown origin.
Total article views: 653 (including HTML, PDF, and XML)
Thereof 598 with geography defined
and 55 with unknown origin.
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
Cited
47 citations as recorded by crossref.
- Examining the competing effects of contemporary land management vs. land cover changes on global air quality A. Wong & J. Geddes 10.5194/acp-21-16479-2021
- Impact of Air Refreshing and Cloud Ice Uptake Limitations on Vertical Profiles and Wet Depositions of Nitrate, Ammonium, and Sulfate G. Luo & F. Yu 10.1029/2023GL104258
- Improving the Representation of Whitecap Fraction and Sea Salt Aerosol Emissions in the ECMWF IFS-AER S. Rémy & M. Anguelova 10.3390/rs13234856
- Exploring Deposition Observations of Oxidized Sulfur and Nitrogen as a Constraint on Emissions in the United States I. Dutta & C. Heald 10.1029/2023JD039610
- Quantification of Atmospheric Ammonia Concentrations: A Review of Its Measurement and Modeling A. Nair & F. Yu 10.3390/atmos11101092
- Investigation of the wet removal rate of black carbon in East Asia: validation of a below- and in-cloud wet removal scheme in FLEXible PARTicle (FLEXPART) model v10.4 Y. Choi et al. 10.5194/acp-20-13655-2020
- Model bias in simulating major chemical components of PM<sub>2.5</sub> in China R. Miao et al. 10.5194/acp-20-12265-2020
- Nitrate chemistry in the northeast US – Part 2: Oxygen isotopes reveal differences in particulate and gas-phase formation H. Kim et al. 10.5194/acp-23-4203-2023
- Aerosol‐Radiation Interactions in China in Winter: Competing Effects of Reduced Shortwave Radiation and Cloud‐Snowfall‐Albedo Feedbacks Under Rapidly Changing Emissions J. Moch et al. 10.1029/2021JD035442
- Improving Below‐Cloud Scavenging Coefficients of Sulfate, Nitrate, and Ammonium in PM2.5 and Implications for Numerical Simulation and Air Pollution Control L. Yao et al. 10.1029/2023JD039487
- Source apportionment of PM2.5 in Montréal, Canada, and health risk assessment for potentially toxic elements N. Fakhri et al. 10.5194/acp-24-1193-2024
- Further improvement of wet process treatments in GEOS-Chem v12.6.0: impact on global distributions of aerosols and aerosol precursors G. Luo et al. 10.5194/gmd-13-2879-2020
- UK Ammonia Emissions Estimated With Satellite Observations and GEOS‐Chem E. Marais et al. 10.1029/2021JD035237
- A Satellite-Based Indicator for Diagnosing Particulate Nitrate Sensitivity to Precursor Emissions: Application to East Asia, Europe, and North America R. Dang et al. 10.1021/acs.est.4c08082
- The importance of ammonia for springtime atmospheric new particle formation and aerosol number abundance over the United States A. Nair et al. 10.1016/j.scitotenv.2022.160756
- Impacts of Emissions of C2‐C5 Alkanes From the U.S. Oil and Gas Sector on Ozone and Other Secondary Species Z. Tzompa‐Sosa & E. Fischer 10.1029/2019JD031935
- Remote Aerosol Simulated During the Atmospheric Tomography (ATom) Campaign and Implications for Aerosol Lifetime C. Gao et al. 10.1029/2022JD036524
- Coarse particulate matter air quality in East Asia: implications for fine particulate nitrate S. Zhai et al. 10.5194/acp-23-4271-2023
- Enhancing Fine Aerosol Simulations in the Remote Atmosphere with Machine Learning M. Lu & C. Gao 10.3390/atmos15111356
- Contribution of brown carbon to the light absorption and radiative effect of carbonaceous aerosols from biomass burning emissions in Chiang Mai, Thailand Y. Zhang et al. 10.1016/j.atmosenv.2021.118544
- Increasing influence of Canadian anthropogenic and the Great Lakes Region shipment SO2 emission on ultrafine particle number concentrations in New York State G. Luo et al. 10.1088/2515-7620/ac82a9
- Global modeling of heterogeneous hydroxymethanesulfonate chemistry S. Song et al. 10.5194/acp-21-457-2021
- Constraining remote oxidation capacity with ATom observations K. Travis et al. 10.5194/acp-20-7753-2020
- Transboundary transport of air pollution in eastern Canada R. Stevens et al. 10.1039/D3VA00307H
- Aerosol responses to precipitation along North American air trajectories arriving at Bermuda H. Dadashazar et al. 10.5194/acp-21-16121-2021
- Compositional Constraints are Vital for Atmospheric PM2.5 Source Attribution over India S. Pai et al. 10.1021/acsearthspacechem.2c00150
- Diagnosing the Sensitivity of Particulate Nitrate to Precursor Emissions Using Satellite Observations of Ammonia and Nitrogen Dioxide R. Dang et al. 10.1029/2023GL105761
- Influence of Oil and Gas End-Use on Summertime Particulate Matter and Ozone Pollution in the Eastern US K. Vohra et al. 10.1021/acs.est.4c10032
- Evaluation of interactive and prescribed agricultural ammonia emissions for simulating atmospheric composition in CAM-chem J. Vira et al. 10.5194/acp-22-1883-2022
- Assessing potential indicators of aerosol wet scavenging during long-range transport M. Hilario et al. 10.5194/amt-17-37-2024
- Multi-method determination of the below-cloud wet scavenging coefficients of aerosols in Beijing, China D. Xu et al. 10.5194/acp-19-15569-2019
- Limitations in representation of physical processes prevent successful simulation of PM<sub>2.5</sub> during KORUS-AQ K. Travis et al. 10.5194/acp-22-7933-2022
- Improvement of inorganic aerosol component in PM2.5 by constraining aqueous-phase formation of sulfate in cloud with satellite retrievals: WRF-Chem simulations T. Sha et al. 10.1016/j.scitotenv.2021.150229
- Modeling particulate nitrate in China: Current findings and future directions X. Xie et al. 10.1016/j.envint.2022.107369
- Comprehensive evaluations of diurnal NO<sub>2</sub> measurements during DISCOVER-AQ 2011: effects of resolution-dependent representation of NO<sub><i>x</i></sub> emissions J. Li et al. 10.5194/acp-21-11133-2021
- Investigating Carbonaceous Aerosol and Its Absorption Properties From Fires in the Western United States (WE‐CAN) and Southern Africa (ORACLES and CLARIFY) T. Carter et al. 10.1029/2021JD034984
- Description of the NASA GEOS Composition Forecast Modeling System GEOS‐CF v1.0 C. Keller et al. 10.1029/2020MS002413
- Empirical estimation of size-resolved scavenging coefficients derived from in-situ measurements at background sites in Korea during 2013–2020 Y. Choi et al. 10.1016/j.atmosres.2023.106971
- An improved representation of aerosol in the ECMWF IFS-COMPO 49R1 through the integration of EQSAM4Climv12 – a first attempt at simulating aerosol acidity S. Rémy et al. 10.5194/gmd-17-7539-2024
- Description and evaluation of the tropospheric aerosol scheme in the Integrated Forecasting System (IFS-AER, cycle 47R1) of ECMWF S. Rémy et al. 10.5194/gmd-15-4881-2022
- Factors controlling marine aerosol size distributions and their climate effects over the northwest Atlantic Ocean region B. Croft et al. 10.5194/acp-21-1889-2021
- Parameterization of below-cloud scavenging for polydisperse fine mode aerosols as a function of rain intensity C. Jung et al. 10.1016/j.jes.2022.07.031
- Impacts of Trans-Provincial Thermal Power Transmission on Air-Quality Recovery and Related Health Outcomes in China G. Han et al. 10.1021/acs.est.2c08925
- Relating geostationary satellite measurements of aerosol optical depth (AOD) over East Asia to fine particulate matter (PM<sub>2.5</sub>): insights from the KORUS-AQ aircraft campaign and GEOS-Chem model simulations S. Zhai et al. 10.5194/acp-21-16775-2021
- Background nitrogen dioxide (NO2) over the United States and its implications for satellite observations and trends: effects of nitrate photolysis, aircraft, and open fires R. Dang et al. 10.5194/acp-23-6271-2023
- Control of particulate nitrate air pollution in China S. Zhai et al. 10.1038/s41561-021-00726-z
- Advances in Simulating the Global Spatial Heterogeneity of Air Quality and Source Sector Contributions: Insights into the Global South D. Zhang et al. 10.1021/acs.est.2c07253
47 citations as recorded by crossref.
- Examining the competing effects of contemporary land management vs. land cover changes on global air quality A. Wong & J. Geddes 10.5194/acp-21-16479-2021
- Impact of Air Refreshing and Cloud Ice Uptake Limitations on Vertical Profiles and Wet Depositions of Nitrate, Ammonium, and Sulfate G. Luo & F. Yu 10.1029/2023GL104258
- Improving the Representation of Whitecap Fraction and Sea Salt Aerosol Emissions in the ECMWF IFS-AER S. Rémy & M. Anguelova 10.3390/rs13234856
- Exploring Deposition Observations of Oxidized Sulfur and Nitrogen as a Constraint on Emissions in the United States I. Dutta & C. Heald 10.1029/2023JD039610
- Quantification of Atmospheric Ammonia Concentrations: A Review of Its Measurement and Modeling A. Nair & F. Yu 10.3390/atmos11101092
- Investigation of the wet removal rate of black carbon in East Asia: validation of a below- and in-cloud wet removal scheme in FLEXible PARTicle (FLEXPART) model v10.4 Y. Choi et al. 10.5194/acp-20-13655-2020
- Model bias in simulating major chemical components of PM<sub>2.5</sub> in China R. Miao et al. 10.5194/acp-20-12265-2020
- Nitrate chemistry in the northeast US – Part 2: Oxygen isotopes reveal differences in particulate and gas-phase formation H. Kim et al. 10.5194/acp-23-4203-2023
- Aerosol‐Radiation Interactions in China in Winter: Competing Effects of Reduced Shortwave Radiation and Cloud‐Snowfall‐Albedo Feedbacks Under Rapidly Changing Emissions J. Moch et al. 10.1029/2021JD035442
- Improving Below‐Cloud Scavenging Coefficients of Sulfate, Nitrate, and Ammonium in PM2.5 and Implications for Numerical Simulation and Air Pollution Control L. Yao et al. 10.1029/2023JD039487
- Source apportionment of PM2.5 in Montréal, Canada, and health risk assessment for potentially toxic elements N. Fakhri et al. 10.5194/acp-24-1193-2024
- Further improvement of wet process treatments in GEOS-Chem v12.6.0: impact on global distributions of aerosols and aerosol precursors G. Luo et al. 10.5194/gmd-13-2879-2020
- UK Ammonia Emissions Estimated With Satellite Observations and GEOS‐Chem E. Marais et al. 10.1029/2021JD035237
- A Satellite-Based Indicator for Diagnosing Particulate Nitrate Sensitivity to Precursor Emissions: Application to East Asia, Europe, and North America R. Dang et al. 10.1021/acs.est.4c08082
- The importance of ammonia for springtime atmospheric new particle formation and aerosol number abundance over the United States A. Nair et al. 10.1016/j.scitotenv.2022.160756
- Impacts of Emissions of C2‐C5 Alkanes From the U.S. Oil and Gas Sector on Ozone and Other Secondary Species Z. Tzompa‐Sosa & E. Fischer 10.1029/2019JD031935
- Remote Aerosol Simulated During the Atmospheric Tomography (ATom) Campaign and Implications for Aerosol Lifetime C. Gao et al. 10.1029/2022JD036524
- Coarse particulate matter air quality in East Asia: implications for fine particulate nitrate S. Zhai et al. 10.5194/acp-23-4271-2023
- Enhancing Fine Aerosol Simulations in the Remote Atmosphere with Machine Learning M. Lu & C. Gao 10.3390/atmos15111356
- Contribution of brown carbon to the light absorption and radiative effect of carbonaceous aerosols from biomass burning emissions in Chiang Mai, Thailand Y. Zhang et al. 10.1016/j.atmosenv.2021.118544
- Increasing influence of Canadian anthropogenic and the Great Lakes Region shipment SO2 emission on ultrafine particle number concentrations in New York State G. Luo et al. 10.1088/2515-7620/ac82a9
- Global modeling of heterogeneous hydroxymethanesulfonate chemistry S. Song et al. 10.5194/acp-21-457-2021
- Constraining remote oxidation capacity with ATom observations K. Travis et al. 10.5194/acp-20-7753-2020
- Transboundary transport of air pollution in eastern Canada R. Stevens et al. 10.1039/D3VA00307H
- Aerosol responses to precipitation along North American air trajectories arriving at Bermuda H. Dadashazar et al. 10.5194/acp-21-16121-2021
- Compositional Constraints are Vital for Atmospheric PM2.5 Source Attribution over India S. Pai et al. 10.1021/acsearthspacechem.2c00150
- Diagnosing the Sensitivity of Particulate Nitrate to Precursor Emissions Using Satellite Observations of Ammonia and Nitrogen Dioxide R. Dang et al. 10.1029/2023GL105761
- Influence of Oil and Gas End-Use on Summertime Particulate Matter and Ozone Pollution in the Eastern US K. Vohra et al. 10.1021/acs.est.4c10032
- Evaluation of interactive and prescribed agricultural ammonia emissions for simulating atmospheric composition in CAM-chem J. Vira et al. 10.5194/acp-22-1883-2022
- Assessing potential indicators of aerosol wet scavenging during long-range transport M. Hilario et al. 10.5194/amt-17-37-2024
- Multi-method determination of the below-cloud wet scavenging coefficients of aerosols in Beijing, China D. Xu et al. 10.5194/acp-19-15569-2019
- Limitations in representation of physical processes prevent successful simulation of PM<sub>2.5</sub> during KORUS-AQ K. Travis et al. 10.5194/acp-22-7933-2022
- Improvement of inorganic aerosol component in PM2.5 by constraining aqueous-phase formation of sulfate in cloud with satellite retrievals: WRF-Chem simulations T. Sha et al. 10.1016/j.scitotenv.2021.150229
- Modeling particulate nitrate in China: Current findings and future directions X. Xie et al. 10.1016/j.envint.2022.107369
- Comprehensive evaluations of diurnal NO<sub>2</sub> measurements during DISCOVER-AQ 2011: effects of resolution-dependent representation of NO<sub><i>x</i></sub> emissions J. Li et al. 10.5194/acp-21-11133-2021
- Investigating Carbonaceous Aerosol and Its Absorption Properties From Fires in the Western United States (WE‐CAN) and Southern Africa (ORACLES and CLARIFY) T. Carter et al. 10.1029/2021JD034984
- Description of the NASA GEOS Composition Forecast Modeling System GEOS‐CF v1.0 C. Keller et al. 10.1029/2020MS002413
- Empirical estimation of size-resolved scavenging coefficients derived from in-situ measurements at background sites in Korea during 2013–2020 Y. Choi et al. 10.1016/j.atmosres.2023.106971
- An improved representation of aerosol in the ECMWF IFS-COMPO 49R1 through the integration of EQSAM4Climv12 – a first attempt at simulating aerosol acidity S. Rémy et al. 10.5194/gmd-17-7539-2024
- Description and evaluation of the tropospheric aerosol scheme in the Integrated Forecasting System (IFS-AER, cycle 47R1) of ECMWF S. Rémy et al. 10.5194/gmd-15-4881-2022
- Factors controlling marine aerosol size distributions and their climate effects over the northwest Atlantic Ocean region B. Croft et al. 10.5194/acp-21-1889-2021
- Parameterization of below-cloud scavenging for polydisperse fine mode aerosols as a function of rain intensity C. Jung et al. 10.1016/j.jes.2022.07.031
- Impacts of Trans-Provincial Thermal Power Transmission on Air-Quality Recovery and Related Health Outcomes in China G. Han et al. 10.1021/acs.est.2c08925
- Relating geostationary satellite measurements of aerosol optical depth (AOD) over East Asia to fine particulate matter (PM<sub>2.5</sub>): insights from the KORUS-AQ aircraft campaign and GEOS-Chem model simulations S. Zhai et al. 10.5194/acp-21-16775-2021
- Background nitrogen dioxide (NO2) over the United States and its implications for satellite observations and trends: effects of nitrate photolysis, aircraft, and open fires R. Dang et al. 10.5194/acp-23-6271-2023
- Control of particulate nitrate air pollution in China S. Zhai et al. 10.1038/s41561-021-00726-z
- Advances in Simulating the Global Spatial Heterogeneity of Air Quality and Source Sector Contributions: Insights into the Global South D. Zhang et al. 10.1021/acs.est.2c07253
Latest update: 20 Nov 2024
Short summary
GEOS-Chem 12.0.0 has been recognized to significantly overestimate the concentrations of gaseous nitric acid, aerosol nitrate, and aerosol ammonium over the United States. In this study, we show that most or all of the overestimation issue appears to be associated with wet scavenging processes. With the updated wet scavenging scheme in this work, we successfully improve the skill of the model in predicting the three species concentrations, which are important for air quality and climate studies.
GEOS-Chem 12.0.0 has been recognized to significantly overestimate the concentrations of gaseous...
