Articles | Volume 10, issue 2
https://doi.org/10.5194/gmd-10-673-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/gmd-10-673-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Source apportionment of atmospheric water over East Asia – a source tracer study in CAM5.1
Chen Pan
Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration, Nanjing University of Information Science & Technology, Nanjing, China
Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters, Nanjing University of Information Science & Technology, Nanjing, China
Key Laboratory of Meteorological Disaster, Ministry of Education (KLME), Nanjing University of Information Science & Technology, Nanjing, China
Joint International Research Laboratory of Climate and Environment Change (ILCEC), Nanjing University of Information Science & Technology, Nanjing, China
Bin Zhu
CORRESPONDING AUTHOR
Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration, Nanjing University of Information Science & Technology, Nanjing, China
Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters, Nanjing University of Information Science & Technology, Nanjing, China
Key Laboratory of Meteorological Disaster, Ministry of Education (KLME), Nanjing University of Information Science & Technology, Nanjing, China
Joint International Research Laboratory of Climate and Environment Change (ILCEC), Nanjing University of Information Science & Technology, Nanjing, China
Jinhui Gao
Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration, Nanjing University of Information Science & Technology, Nanjing, China
Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters, Nanjing University of Information Science & Technology, Nanjing, China
Key Laboratory of Meteorological Disaster, Ministry of Education (KLME), Nanjing University of Information Science & Technology, Nanjing, China
Joint International Research Laboratory of Climate and Environment Change (ILCEC), Nanjing University of Information Science & Technology, Nanjing, China
Hanqing Kang
Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration, Nanjing University of Information Science & Technology, Nanjing, China
Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters, Nanjing University of Information Science & Technology, Nanjing, China
Key Laboratory of Meteorological Disaster, Ministry of Education (KLME), Nanjing University of Information Science & Technology, Nanjing, China
Joint International Research Laboratory of Climate and Environment Change (ILCEC), Nanjing University of Information Science & Technology, Nanjing, China
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Qidi Li, Yuhan Luo, Yuanyuan Qian, Chen Pan, Ke Dou, Xuewei Hou, Fuqi Si, and Wenqing Liu
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-859, https://doi.org/10.5194/acp-2022-859, 2023
Revised manuscript not accepted
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We found that all instruments recorded severe ozone depletion from March 18 to April 18, 2020. The effect of the polar vortex on ozone depletion in the stratosphere was clear. Additionally, the SD-WACCM model results indicated that both ClO and BrO concentrations peaked in late March. Before chlorine activation began, bromine mainly existed as HOBr; however, after chlorine activation, bromine mainly existed in the form of BrCl.
Hanqing Kang, Bin Zhu, Jinhui Gao, Yao He, Honglei Wang, Jifeng Su, Chen Pan, Tong Zhu, and Bu Yu
Atmos. Chem. Phys., 19, 3673–3685, https://doi.org/10.5194/acp-19-3673-2019, https://doi.org/10.5194/acp-19-3673-2019, 2019
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In this study, we found that a cold front can transport air pollutants from the polluted North China Plain to the Yangtze River Delta (YRD), thereby deteriorating air quality over the YRD. Before the cold frontal passage, a warm and polluted air mass over YRD climbed to the free troposphere (1.0–2.0 km) along the frontal surface. After the cold frontal passage, high pressure behind the frontal zone resulted in a synoptic subsidence that trapped PM2.5 in the surface.
Jinhui Gao, Bin Zhu, Hui Xiao, Hanqing Kang, Chen Pan, Dongdong Wang, and Honglei Wang
Atmos. Chem. Phys., 18, 7081–7094, https://doi.org/10.5194/acp-18-7081-2018, https://doi.org/10.5194/acp-18-7081-2018, 2018
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This model study is about the effect of black carbon (BC) and the boundary layer interactions on surface ozone in an area of severe haze and ozone pollution in China. It shows the following: BC not only reduces photolysis rate, but also suppresses boundary layer (BL) development, then confines more ozone precursors. The BL suppression leads to less ozone aloft being entrained downward and finally leading to surface ozone reduction before noon.
Naifu Shao, Chunsong Lu, Xingcan Jia, Yuan Wang, Yubin Li, Yan Yin, Bin Zhu, Tianliang Zhao, Duanyang Liu, Shengjie Niu, Shuxian Fan, Shuqi Yan, and Jingjing Lv
Atmos. Chem. Phys., 23, 9873–9890, https://doi.org/10.5194/acp-23-9873-2023, https://doi.org/10.5194/acp-23-9873-2023, 2023
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Fog is an important meteorological phenomenon that affects visibility. Aerosols and the planetary boundary layer (PBL) play critical roles in the fog life cycle. In this study, aerosol-induced changes in fog properties become more remarkable in the second fog (Fog2) than in the first fog (Fog1). The reason is that aerosol–cloud interaction (ACI) delays Fog1 dissipation, leading to the PBL meteorological conditions being more conducive to Fog2 formation and to stronger ACI in Fog2.
Chenwei Fang, Jim M. Haywood, Ju Liang, Ben T. Johnson, Ying Chen, and Bin Zhu
Atmos. Chem. Phys., 23, 8341–8368, https://doi.org/10.5194/acp-23-8341-2023, https://doi.org/10.5194/acp-23-8341-2023, 2023
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The responses of Asian summer monsoon duration and intensity to air pollution mitigation are identified given the net-zero future. We show that reducing scattering aerosols makes the rainy season longer and stronger across South Asia and East Asia but that absorbing aerosol reduction has the opposite effect. Our results hint at distinct monsoon responses to emission controls that target different aerosols.
Xuewei Hou, Oliver Wild, Bin Zhu, and James Lee
EGUsphere, https://doi.org/10.5194/egusphere-2023-1592, https://doi.org/10.5194/egusphere-2023-1592, 2023
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In response to the climate crisis, many countries have committed to net zero in a certain future year. The impacts of net zero scenario on tropospheric O3 are less well studied and remain unclear. In this study, we quantified the changes of tropospheric O3 budgets, spatiotemporal distributions of future surface O3 in East Asia and regional O3 source contributions for 2060 under a net zero scenario, using the NCAR Community Earth System Model (CESM) and online O3 tagging methods.
Wen Lu, Bin Zhu, Shuqi Yan, Jie Li, and Zifa Wang
EGUsphere, https://doi.org/10.5194/egusphere-2023-1089, https://doi.org/10.5194/egusphere-2023-1089, 2023
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Parameterized the minimum turbulent diffusivity (Kzmin) by sensible heat flux and latent heat flux and embedded it into the WRF-Chem model. New scheme improved the underestimation of turbulence diffusion underestimation and overestimation of surface PM2.5 under stable boundary layer simulation over eastern China. The physical relationship between Kzmin and two factors was discussed. Process analysis showed that vertical mixing is the key process to improve surface PM2.5 simulations.
Shuqi Yan, Bin Zhu, Shuangshuang Shi, Wen Lu, Jinhui Gao, Hanqing Kang, and Duanyang Liu
Atmos. Chem. Phys., 23, 5177–5190, https://doi.org/10.5194/acp-23-5177-2023, https://doi.org/10.5194/acp-23-5177-2023, 2023
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We analyze ozone response to aerosol mixing states in the vertical direction by WRF-Chem simulations. Aerosols generally lead to turbulent suppression, precursor accumulation, low-level photolysis reduction, and upper-level photolysis enhancement under different underlying surface and pollution conditions. Thus, ozone decreases within the entire boundary layer during the daytime, and the decrease is the least in aerosol external mixing states compared to internal and core shell mixing states.
Qidi Li, Yuhan Luo, Yuanyuan Qian, Chen Pan, Ke Dou, Xuewei Hou, Fuqi Si, and Wenqing Liu
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-859, https://doi.org/10.5194/acp-2022-859, 2023
Revised manuscript not accepted
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We found that all instruments recorded severe ozone depletion from March 18 to April 18, 2020. The effect of the polar vortex on ozone depletion in the stratosphere was clear. Additionally, the SD-WACCM model results indicated that both ClO and BrO concentrations peaked in late March. Before chlorine activation began, bromine mainly existed as HOBr; however, after chlorine activation, bromine mainly existed in the form of BrCl.
Zefeng Zhang, Hengnan Guo, Hanqing Kang, Jing Wang, Junlin An, Xingna Yu, Jingjing Lv, and Bin Zhu
Atmos. Meas. Tech., 15, 7259–7264, https://doi.org/10.5194/amt-15-7259-2022, https://doi.org/10.5194/amt-15-7259-2022, 2022
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In this study, we first analyze the relationship between the visibility, the extinction coefficient, and atmospheric compositions. Then we propose to use the harmonic average of visibility data as the average visibility, which can better reflect changes in atmospheric extinction coefficients and aerosol concentrations. It is recommended to use the harmonic average visibility in the studies of climate change, atmospheric radiation, air pollution, environmental health, etc.
Hanqing Kang, Bin Zhu, Gerrit de Leeuw, Bu Yu, Ronald J. van der A, and Wen Lu
Atmos. Chem. Phys., 22, 10623–10634, https://doi.org/10.5194/acp-22-10623-2022, https://doi.org/10.5194/acp-22-10623-2022, 2022
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This study quantified the contribution of each urban-induced meteorological effect (temperature, humidity, and circulation) to aerosol concentration. We found that the urban heat island (UHI) circulation dominates the UHI effects on aerosol. The UHI circulation transports aerosol and its precursor gases from the warmer lower boundary layer to the colder lower free troposphere and promotes the secondary formation of ammonium nitrate aerosol in the cold atmosphere.
Ying Li, Xiangjun Zhao, Xuejiao Deng, and Jinhui Gao
Atmos. Chem. Phys., 22, 3861–3873, https://doi.org/10.5194/acp-22-3861-2022, https://doi.org/10.5194/acp-22-3861-2022, 2022
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This study finds a new phenomenon of weak wind deepening (WWD) associated with the peripheral circulation of typhoon and gives the influence mechanism of WWD on its contribution to daily variation during sustained ozone episodes. The WWD provides the premise for pollution accumulation in the whole PBL and continued enhancement of ground-level ozone via vertical mixing processes. These findings could benefit the daily daytime ozone forecast in the PRD region and other areas.
Zhenbin Wang, Bin Zhu, Hanqing Kang, Wen Lu, Shuqi Yan, Delong Zhao, Weihang Zhang, and Jinhui Gao
Atmos. Chem. Phys., 21, 15555–15567, https://doi.org/10.5194/acp-21-15555-2021, https://doi.org/10.5194/acp-21-15555-2021, 2021
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In this paper, by using WRF-Chem with a black carbon (BC) tagging technique, we investigate the formation mechanism and regional sources of a BC peak in the free troposphere observed by aircraft flights. Local sources dominated BC from the surface to about 700 m (78.5 %), while the BC peak in the free troposphere was almost entirely imported from external sources (99.8 %). Our results indicate that cyclone systems can quickly lift BC up to the free troposphere, as well as extend its lifetime.
Meng Gao, Yang Yang, Hong Liao, Bin Zhu, Yuxuan Zhang, Zirui Liu, Xiao Lu, Chen Wang, Qiming Zhou, Yuesi Wang, Qiang Zhang, Gregory R. Carmichael, and Jianlin Hu
Atmos. Chem. Phys., 21, 11405–11421, https://doi.org/10.5194/acp-21-11405-2021, https://doi.org/10.5194/acp-21-11405-2021, 2021
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Light absorption and radiative forcing of black carbon (BC) is influenced by both BC itself and its interactions with other aerosol chemical compositions. In this study, we used the online coupled WRF-Chem model to examine how emission control measures during the Asian-Pacific Economic Cooperation (APEC) conference affect the mixing state and light absorption of BC and the associated implications for BC-PBL interactions.
Hengnan Guo, Zefeng Zhang, Lin Jiang, Junlin An, Bin Zhu, Hanqing Kang, and Jing Wang
Atmos. Meas. Tech., 14, 2441–2450, https://doi.org/10.5194/amt-14-2441-2021, https://doi.org/10.5194/amt-14-2441-2021, 2021
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Visibility is an indicator of atmospheric transparency and is widely used in many research fields. Although efforts have been made to improve the performance of visibility meters, a significant error exists in measured visibility data. This is because current methods of visibility measurement include a false assumption, which leads to the long-term neglect of an important source of visibility errors. Without major adjustments to current methods, it is not possible to obtain reliable data.
Jinhui Gao, Ying Li, Bin Zhu, Bo Hu, Lili Wang, and Fangwen Bao
Atmos. Chem. Phys., 20, 10831–10844, https://doi.org/10.5194/acp-20-10831-2020, https://doi.org/10.5194/acp-20-10831-2020, 2020
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Light extinction of aerosols can decease surface ozone mainly via reducing photochemical production of ozone. However, it also leads to high levels of ozone aloft being entrained down to the surface which partly counteracts the reduction in surface ozone. The impact of aerosols is more sensitive to local ozone, which suggests that while controlling the levels of aerosols, controlling the local ozone precursors is an effective way to suppress the increase of ozone over China at present.
Zhaobing Guo, Mingyi Xu, Yuxuan He, Shuo Gao, Chenmin Xu, Bin Zhu, Qingjun Guo, Xiaoyu Shen, Shuang Zhao, and Pengxiang Qiu
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-506, https://doi.org/10.5194/acp-2020-506, 2020
Revised manuscript not accepted
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In order to gain insight into the formation mechanism of sulfate, stable sulfur isotope and Rayleigh distillation were applied to investigate the isotopic fractionations controlled by the oxidation pathways. The processes of SO2 oxidation on the surface of α-Fe2O3 with different chemical condition (NOX, O3 and NH3) were conducted in laboratory to study mechanism of SO2 oxidation. It was found that nitrogen oxides contributed primarily to the formation of sulfate among NOX, O3 and NH3 pathways.
Shuqi Yan, Bin Zhu, Yong Huang, Jun Zhu, Hanqing Kang, Chunsong Lu, and Tong Zhu
Atmos. Chem. Phys., 20, 5559–5572, https://doi.org/10.5194/acp-20-5559-2020, https://doi.org/10.5194/acp-20-5559-2020, 2020
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The development of China has caused rapid urbanization and severe air pollution. However, the extent of their individual and combined effects on fog is not well understood. Through numerical experiments, we find that urbanization suppresses low-level fog but probably promotes upper-level fog. Additional aerosols generally promote fog. Urbanization affects fog to a much larger extent than aerosols do.
Meng Gao, Jinhui Gao, Bin Zhu, Rajesh Kumar, Xiao Lu, Shaojie Song, Yuzhong Zhang, Beixi Jia, Peng Wang, Gufran Beig, Jianlin Hu, Qi Ying, Hongliang Zhang, Peter Sherman, and Michael B. McElroy
Atmos. Chem. Phys., 20, 4399–4414, https://doi.org/10.5194/acp-20-4399-2020, https://doi.org/10.5194/acp-20-4399-2020, 2020
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A regional fully coupled meteorology–chemistry model, Weather Research and Forecasting model with Chemistry (WRF-Chem), was employed to study the seasonality of ozone (O3) pollution and its sources in both China and India.
Hanqing Kang, Bin Zhu, Jinhui Gao, Yao He, Honglei Wang, Jifeng Su, Chen Pan, Tong Zhu, and Bu Yu
Atmos. Chem. Phys., 19, 3673–3685, https://doi.org/10.5194/acp-19-3673-2019, https://doi.org/10.5194/acp-19-3673-2019, 2019
Short summary
Short summary
In this study, we found that a cold front can transport air pollutants from the polluted North China Plain to the Yangtze River Delta (YRD), thereby deteriorating air quality over the YRD. Before the cold frontal passage, a warm and polluted air mass over YRD climbed to the free troposphere (1.0–2.0 km) along the frontal surface. After the cold frontal passage, high pressure behind the frontal zone resulted in a synoptic subsidence that trapped PM2.5 in the surface.
Jinhui Gao, Bin Zhu, Hui Xiao, Hanqing Kang, Chen Pan, Dongdong Wang, and Honglei Wang
Atmos. Chem. Phys., 18, 7081–7094, https://doi.org/10.5194/acp-18-7081-2018, https://doi.org/10.5194/acp-18-7081-2018, 2018
Short summary
Short summary
This model study is about the effect of black carbon (BC) and the boundary layer interactions on surface ozone in an area of severe haze and ozone pollution in China. It shows the following: BC not only reduces photolysis rate, but also suppresses boundary layer (BL) development, then confines more ozone precursors. The BL suppression leads to less ozone aloft being entrained downward and finally leading to surface ozone reduction before noon.
Zefeng Zhang, Yan Shen, Yanwei Li, Bin Zhu, and Xingna Yu
Atmos. Chem. Phys., 17, 4147–4157, https://doi.org/10.5194/acp-17-4147-2017, https://doi.org/10.5194/acp-17-4147-2017, 2017
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Aerosol particles and relative humidity are the main factors that affect atmospheric visibility. Due to the complexity of the physicochemical properties of aerosol particles, more and more instruments and cost were put into research, which limited the development of large area observation research. Thus, it is especially important to find the key parameters which affect the visibility and to establish the observation scheme.
Related subject area
Atmospheric sciences
Use of threshold parameter variation for tropical cyclone tracking
Passive-tracer modelling at super-resolution with Weather Research and Forecasting – Advanced Research WRF (WRF-ARW) to assess mass-balance schemes
The High-resolution Intermediate Complexity Atmospheric Research (HICAR v1.1) model enables fast dynamic downscaling to the hectometer scale
A gridded air quality forecast through fusing site-available machine learning predictions from RFSML v1.0 and chemical transport model results from GEOS-Chem v13.1.0 using the ensemble Kalman filter
Plume detection and emission estimate for biomass burning plumes from TROPOMI carbon monoxide observations using APE v1.1
CHEEREIO 1.0: a versatile and user-friendly ensemble-based chemical data assimilation and emissions inversion platform for the GEOS-Chem chemical transport model
A method to derive Fourier–wavelet spectra for the characterization of global-scale waves in the mesosphere and lower thermosphere and its MATLAB and Python software (fourierwavelet v1.1)
Dynamic Meteorology-induced Emissions Coupler (MetEmis) development in the Community Multiscale Air Quality (CMAQ): CMAQ-MetEmis
Visual analysis of model parameter sensitivities along warm conveyor belt trajectories using Met.3D (1.6.0-multivar1)
Simulating heat and CO2 fluxes in Beijing using SUEWS V2020b: sensitivity to vegetation phenology and maximum conductance
A Python library for computing individual and merged non-CO2 algorithmic climate change functions: CLIMaCCF V1.0
The three-dimensional structure of fronts in mid-latitude weather systems in numerical weather prediction models
The development and validation of the Inhomogeneous Wind Scheme for Urban Street (IWSUS-v1)
GPU-HADVPPM V1.0: a high-efficiency parallel GPU design of the piecewise parabolic method (PPM) for horizontal advection in an air quality model (CAMx V6.10)
Variability and combination as an ensemble of mineral dust forecasts during the 2021 CADDIWA experiment using the WRF 3.7.1 and CHIMERE v2020r3 models
Breakups are complicated: an efficient representation of collisional breakup in the superdroplet method
An optimized semi-empirical physical approach for satellite-based PM2.5 retrieval: embedding machine learning to simulate complex physical parameters
Sensitivity of tropospheric ozone to halogen chemistry in the chemistry–climate model LMDZ-INCA vNMHC
Segmentation of XCO2 images with deep learning: application to synthetic plumes from cities and power plants
Evaluating precipitation distributions at regional scales: a benchmarking framework and application to CMIP5 and 6 models
The Fire Inventory from NCAR version 2.5: an updated global fire emissions model for climate and chemistry applications
An approach to refining the ground meteorological observation stations for improving PM2.5 forecasts in the Beijing–Tianjin–Hebei region
Assessment of WRF (v 4.2.1) dynamically downscaled precipitation on subdaily and daily timescales over CONUS
Convective-gust nowcasting based on radar reflectivity and a deep learning algorithm
Self-nested large-eddy simulations in PALM model system v21.10 for offshore wind prediction under different atmospheric stability conditions
How does cloud-radiative heating over the North Atlantic change with grid spacing, convective parameterization, and microphysics scheme in ICON version 2.1.00?
Simulations of idealised 3D atmospheric flows on terrestrial planets using LFRic-Atmosphere
Updated isoprene and terpene emission factors for the Interactive BVOC (iBVOC) emission scheme in the United Kingdom Earth System Model (UKESM1.0)
Technical descriptions of the experimental dynamical downscaling simulations over North America by the CAM–MPAS variable-resolution model
Evaluating WRF-GC v2.0 predictions of boundary layer and vertical ozone profiles during the 2021 TRACER-AQ campaign in Houston, Texas
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Emulating aerosol optics with randomly generated neural networks
Development of an ecophysiology module in the GEOS-Chem chemical transport model version 12.2.0 to represent biosphere–atmosphere fluxes relevant for ozone air quality
Comparison of ozone formation attribution techniques in the northeastern United States
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Forecasting tropical cyclone tracks in the northwestern Pacific based on a deep-learning model
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Bernhard M. Enz, Jan P. Engelmann, and Ulrike Lohmann
Geosci. Model Dev., 16, 5093–5112, https://doi.org/10.5194/gmd-16-5093-2023, https://doi.org/10.5194/gmd-16-5093-2023, 2023
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An algorithm to track tropical cyclones in model simulation data has been developed. The algorithm uses many combinations of varying parameter thresholds to detect weaker phases of tropical cyclones while still being resilient to false positives. It is shown that the algorithm performs well and adequately represents the tropical cyclone activity of the underlying simulation data. The impact of false positives on overall tropical cyclone activity is shown to be insignificant.
Sepehr Fathi, Mark Gordon, and Yongsheng Chen
Geosci. Model Dev., 16, 5069–5091, https://doi.org/10.5194/gmd-16-5069-2023, https://doi.org/10.5194/gmd-16-5069-2023, 2023
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We have combined various capabilities within a WRF model to generate simulations of atmospheric pollutant dispersion at 50 m resolution. The study objective was to resolve transport processes at the scale of measurements to assess and optimize aircraft-based emission rate retrievals. Model performance evaluation resulted in agreement within 5 % of observed meteorological and within 1–2 standard deviations of observed wind fields. Mass was conserved in the model within 5 % of input emissions.
Dylan Reynolds, Ethan Gutmann, Bert Kruyt, Michael Haugeneder, Tobias Jonas, Franziska Gerber, Michael Lehning, and Rebecca Mott
Geosci. Model Dev., 16, 5049–5068, https://doi.org/10.5194/gmd-16-5049-2023, https://doi.org/10.5194/gmd-16-5049-2023, 2023
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The challenge of running geophysical models is often compounded by the question of where to obtain appropriate data to give as input to a model. Here we present the HICAR model, a simplified atmospheric model capable of running at spatial resolutions of hectometers for long time series or over large domains. This makes physically consistent atmospheric data available at the spatial and temporal scales needed for some terrestrial modeling applications, for example seasonal snow forecasting.
Li Fang, Jianbing Jin, Arjo Segers, Hong Liao, Ke Li, Bufan Xu, Wei Han, Mijie Pang, and Hai Xiang Lin
Geosci. Model Dev., 16, 4867–4882, https://doi.org/10.5194/gmd-16-4867-2023, https://doi.org/10.5194/gmd-16-4867-2023, 2023
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Machine learning models have gained great popularity in air quality prediction. However, they are only available at air quality monitoring stations. In contrast, chemical transport models (CTM) provide predictions that are continuous in the 3D field. Owing to complex error sources, they are typically biased. In this study, we proposed a gridded prediction with high accuracy by fusing predictions from our regional feature selection machine learning prediction (RFSML v1.0) and a CTM prediction.
Manu Goudar, Juliëtte C. S. Anema, Rajesh Kumar, Tobias Borsdorff, and Jochen Landgraf
Geosci. Model Dev., 16, 4835–4852, https://doi.org/10.5194/gmd-16-4835-2023, https://doi.org/10.5194/gmd-16-4835-2023, 2023
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A framework was developed to automatically detect plumes and compute emission estimates with cross-sectional flux method (CFM) for biomass burning events in TROPOMI CO datasets using Visible Infrared Imaging Radiometer Suite active fire data. The emissions were more reliable when changing plume height in downwind direction was used instead of constant injection height. The CFM had uncertainty even when the meteorological conditions were accurate; thus there is a need for better inversion models.
Drew C. Pendergrass, Daniel J. Jacob, Hannah Nesser, Daniel J. Varon, Melissa Sulprizio, Kazuyuki Miyazaki, and Kevin W. Bowman
Geosci. Model Dev., 16, 4793–4810, https://doi.org/10.5194/gmd-16-4793-2023, https://doi.org/10.5194/gmd-16-4793-2023, 2023
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We have built a tool called CHEEREIO that allows scientists to use observations of pollutants or gases in the atmosphere, such as from satellites or surface stations, to update supercomputer models that simulate the Earth. CHEEREIO uses the difference between the model simulations of the atmosphere and real-world observations to come up with a good guess for the actual composition of our atmosphere, the true emissions of various pollutants, and whatever else they may want to study.
Yosuke Yamazaki
Geosci. Model Dev., 16, 4749–4766, https://doi.org/10.5194/gmd-16-4749-2023, https://doi.org/10.5194/gmd-16-4749-2023, 2023
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The Earth's atmosphere can support various types of global-scale waves. Some waves propagate eastward and others westward, and they can have different zonal wavenumbers. The Fourier–wavelet analysis is a useful technique for identifying different components of global-scale waves and their temporal variability. This paper introduces an easy-to-implement method to derive Fourier–wavelet spectra from 2-D space–time data. Application examples are presented using atmospheric models.
Bok H. Baek, Carlie Coats, Siqi Ma, Chi-Tsan Wang, Yunyao Li, Jia Xing, Daniel Tong, Soontae Kim, and Jung-Hun Woo
Geosci. Model Dev., 16, 4659–4676, https://doi.org/10.5194/gmd-16-4659-2023, https://doi.org/10.5194/gmd-16-4659-2023, 2023
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To enable the direct feedback effects of aerosols and local meteorology in an air quality modeling system without any computational bottleneck, we have developed an inline meteorology-induced emissions coupler module within the U.S. Environmental Protection Agency’s Community Multiscale Air Quality modeling system to dynamically model the complex MOtor Vehicle Emission Simulator (MOVES) on-road mobile emissions inline without a separate dedicated emissions processing model like SMOKE.
Christoph Neuhauser, Maicon Hieronymus, Michael Kern, Marc Rautenhaus, Annika Oertel, and Rüdiger Westermann
Geosci. Model Dev., 16, 4617–4638, https://doi.org/10.5194/gmd-16-4617-2023, https://doi.org/10.5194/gmd-16-4617-2023, 2023
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Numerical weather prediction models rely on parameterizations for sub-grid-scale processes, which are a source of uncertainty. We present novel visual analytics solutions to analyze interactively the sensitivities of a selected prognostic variable to multiple model parameters along trajectories regarding similarities in temporal development and spatiotemporal relationships. The proposed workflow is applied to cloud microphysical sensitivities along coherent strongly ascending trajectories.
Yingqi Zheng, Minttu Havu, Huizhi Liu, Xueling Cheng, Yifan Wen, Hei Shing Lee, Joyson Ahongshangbam, and Leena Järvi
Geosci. Model Dev., 16, 4551–4579, https://doi.org/10.5194/gmd-16-4551-2023, https://doi.org/10.5194/gmd-16-4551-2023, 2023
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The performance of the Surface Urban Energy and Water Balance Scheme (SUEWS) is evaluated against the observed surface exchanges (fluxes) of heat and carbon dioxide in a densely built neighborhood in Beijing. The heat flux modeling is noticeably improved by using the observed maximum conductance and by optimizing the vegetation phenology modeling. SUEWS also performs well in simulating carbon dioxide flux.
Simone Dietmüller, Sigrun Matthes, Katrin Dahlmann, Hiroshi Yamashita, Abolfazl Simorgh, Manuel Soler, Florian Linke, Benjamin Lührs, Maximilian M. Meuser, Christian Weder, Volker Grewe, Feijia Yin, and Federica Castino
Geosci. Model Dev., 16, 4405–4425, https://doi.org/10.5194/gmd-16-4405-2023, https://doi.org/10.5194/gmd-16-4405-2023, 2023
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Climate-optimized aircraft trajectories avoid atmospheric regions with a large climate impact due to aviation emissions. This requires spatially and temporally resolved information on aviation's climate impact. We propose using algorithmic climate change functions (aCCFs) for CO2 and non-CO2 effects (ozone, methane, water vapor, contrail cirrus). Merged aCCFs combine individual aCCFs by assuming aircraft-specific parameters and climate metrics. Technically this is done with a Python library.
Andreas A. Beckert, Lea Eisenstein, Annika Oertel, Tim Hewson, George C. Craig, and Marc Rautenhaus
Geosci. Model Dev., 16, 4427–4450, https://doi.org/10.5194/gmd-16-4427-2023, https://doi.org/10.5194/gmd-16-4427-2023, 2023
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We investigate the benefit of objective 3-D front detection with modern interactive visual analysis techniques for case studies of extra-tropical cyclones and comparisons of frontal structures between different numerical weather prediction models. The 3-D frontal structures show agreement with 2-D fronts from surface analysis charts and augment them in the vertical dimension. We see great potential for more complex studies of atmospheric dynamics and for operational weather forecasting.
Zhenxin Liu, Yuanhao Chen, Yuhang Wang, Cheng Liu, Shuhua Liu, and Hong Liao
Geosci. Model Dev., 16, 4385–4403, https://doi.org/10.5194/gmd-16-4385-2023, https://doi.org/10.5194/gmd-16-4385-2023, 2023
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The heterogeneous layout of urban buildings leads to the complex wind field in and over the urban canopy. Large discrepancies between the observations and the current simulations result from misunderstanding the character of the wind field. The Inhomogeneous Wind Scheme in Urban Street (IWSUS) was developed to simulate the heterogeneity of the wind speed in a typical street and then improve the simulated energy budget in the lower atmospheric layer over the urban canopy.
Kai Cao, Qizhong Wu, Lingling Wang, Nan Wang, Huaqiong Cheng, Xiao Tang, Dongqing Li, and Lanning Wang
Geosci. Model Dev., 16, 4367–4383, https://doi.org/10.5194/gmd-16-4367-2023, https://doi.org/10.5194/gmd-16-4367-2023, 2023
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Offline performance experiment results show that the GPU-HADVPPM on a V100 GPU can achieve up to 1113.6 × speedups to its original version on an E5-2682 v4 CPU. A series of optimization measures are taken, and the CAMx-CUDA model improves the computing efficiency by 128.4 × on a single V100 GPU card. A parallel architecture with an MPI plus CUDA hybrid paradigm is presented, and it can achieve up to 4.5 × speedup when launching eight CPU cores and eight GPU cards.
Laurent Menut
Geosci. Model Dev., 16, 4265–4281, https://doi.org/10.5194/gmd-16-4265-2023, https://doi.org/10.5194/gmd-16-4265-2023, 2023
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This study analyzes forecasts that were made in 2021 to help trigger measurements during the CADDIWA experiment. The WRF and CHIMERE models were run each day, and the first goal is to quantify the variability of the forecast as a function of forecast leads and forecast location. The possibility of using the different leads as an ensemble is also tested. For some locations, the correlation scores are better with this approach. This could be tested on operational forecast chains in the future.
Emily de Jong, John Ben Mackay, Oleksii Bulenok, Anna Jaruga, and Sylwester Arabas
Geosci. Model Dev., 16, 4193–4211, https://doi.org/10.5194/gmd-16-4193-2023, https://doi.org/10.5194/gmd-16-4193-2023, 2023
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In clouds, collisional breakup occurs when two colliding droplets splinter into new, smaller fragments. Particle-based modeling approaches often do not represent breakup because of the computational demands of creating new droplets. We present a particle-based breakup method that preserves the computational efficiency of these methods. In a series of simple demonstrations, we show that this representation alters cloud processes in reasonable and expected ways.
Caiyi Jin, Qiangqiang Yuan, Tongwen Li, Yuan Wang, and Liangpei Zhang
Geosci. Model Dev., 16, 4137–4154, https://doi.org/10.5194/gmd-16-4137-2023, https://doi.org/10.5194/gmd-16-4137-2023, 2023
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The semi-empirical physical approach derives PM2.5 with strong physical significance. However, due to the complex optical characteristic, the physical parameters are difficult to express accurately. Thus, combining the atmospheric physical mechanism and machine learning, we propose an optimized model. It creatively embeds the random forest model into the physical PM2.5 remote sensing approach to simulate a physical parameter. Our method shows great optimized performance in the validations.
Cyril Caram, Sophie Szopa, Anne Cozic, Slimane Bekki, Carlos A. Cuevas, and Alfonso Saiz-Lopez
Geosci. Model Dev., 16, 4041–4062, https://doi.org/10.5194/gmd-16-4041-2023, https://doi.org/10.5194/gmd-16-4041-2023, 2023
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We studied the role of halogenated compounds (containing chlorine, bromine and iodine), emitted by natural processes (mainly above the oceans), in the chemistry of the lower layers of the atmosphere. We introduced this relatively new chemistry in a three-dimensional climate–chemistry model and looked at how this chemistry will disrupt the ozone. We showed that the concentration of ozone decreases by 22 % worldwide and that of the atmospheric detergent, OH, by 8 %.
Joffrey Dumont Le Brazidec, Pierre Vanderbecken, Alban Farchi, Marc Bocquet, Jinghui Lian, Grégoire Broquet, Gerrit Kuhlmann, Alexandre Danjou, and Thomas Lauvaux
Geosci. Model Dev., 16, 3997–4016, https://doi.org/10.5194/gmd-16-3997-2023, https://doi.org/10.5194/gmd-16-3997-2023, 2023
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Monitoring of CO2 emissions is key to the development of reduction policies. Local emissions, from cities or power plants, may be estimated from CO2 plumes detected in satellite images. CO2 plumes generally have a weak signal and are partially concealed by highly variable background concentrations and instrument errors, which hampers their detection. To address this problem, we propose and apply deep learning methods to detect the contour of a plume in simulated CO2 satellite images.
Min-Seop Ahn, Paul A. Ullrich, Peter J. Gleckler, Jiwoo Lee, Ana C. Ordonez, and Angeline G. Pendergrass
Geosci. Model Dev., 16, 3927–3951, https://doi.org/10.5194/gmd-16-3927-2023, https://doi.org/10.5194/gmd-16-3927-2023, 2023
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We introduce a framework for regional-scale evaluation of simulated precipitation distributions with 62 climate reference regions and 10 metrics and apply it to evaluate CMIP5 and CMIP6 models against multiple satellite-based precipitation products. The common model biases identified in this study are mainly associated with the overestimated light precipitation and underestimated heavy precipitation. These biases persist from earlier-generation models and have been slightly improved in CMIP6.
Christine Wiedinmyer, Yosuke Kimura, Elena C. McDonald-Buller, Louisa K. Emmons, Rebecca R. Buchholz, Wenfu Tang, Keenan Seto, Maxwell B. Joseph, Kelley C. Barsanti, Annmarie G. Carlton, and Robert Yokelson
Geosci. Model Dev., 16, 3873–3891, https://doi.org/10.5194/gmd-16-3873-2023, https://doi.org/10.5194/gmd-16-3873-2023, 2023
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The Fire INventory from NCAR (FINN) provides daily global estimates of emissions from open fires based on satellite detections of hot spots. This version has been updated to apply MODIS and VIIRS satellite fire detection and better represents both large and small fires. FINNv2.5 generates more emissions than FINNv1 and is in general agreement with other fire emissions inventories. The new estimates are consistent with satellite observations, but uncertainties remain regionally and by pollutant.
Lichao Yang, Wansuo Duan, and Zifa Wang
Geosci. Model Dev., 16, 3827–3848, https://doi.org/10.5194/gmd-16-3827-2023, https://doi.org/10.5194/gmd-16-3827-2023, 2023
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An approach is proposed to refine a ground meteorological observation network to improve the PM2.5 forecasts in the Beijing–Tianjin–Hebei region. A cost-effective observation network is obtained and makes the relevant PM2.5 forecasts assimilate fewer observations but achieve the forecasting skill comparable to or higher than that obtained by assimilating all ground station observations, suggesting that many of the current ground stations can be greatly scattered to avoid much unnecessary work.
Abhishekh Kumar Srivastava, Paul Aaron Ullrich, Deeksha Rastogi, Pouya Vahmani, Andrew Jones, and Richard Grotjahn
Geosci. Model Dev., 16, 3699–3722, https://doi.org/10.5194/gmd-16-3699-2023, https://doi.org/10.5194/gmd-16-3699-2023, 2023
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Stakeholders need high-resolution regional climate data for applications such as assessing water availability and mountain snowpack. This study examines 3 h and 24 h historical precipitation over the contiguous United States in the 12 km WRF version 4.2.1-based dynamical downscaling of the ERA5 reanalysis. WRF improves precipitation characteristics such as the annual cycle and distribution of the precipitation maxima, but it also displays regionally and seasonally varying precipitation biases.
Haixia Xiao, Yaqiang Wang, Yu Zheng, Yuanyuan Zheng, Xiaoran Zhuang, Hongyan Wang, and Mei Gao
Geosci. Model Dev., 16, 3611–3628, https://doi.org/10.5194/gmd-16-3611-2023, https://doi.org/10.5194/gmd-16-3611-2023, 2023
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Due to the small-scale and nonstationary nature of convective wind gusts (CGs), reliable CG nowcasting has remained unattainable. Here, we developed a deep learning model — namely CGsNet — for 0—2 h of quantitative CG nowcasting, first achieving minute—kilometer-level forecasts. Based on the CGsNet model, the average surface wind speed (ASWS) and peak wind gust speed (PWGS) predictions are obtained. Experiments indicate that CGsNet exhibits higher accuracy than the traditional method.
Maria Krutova, Mostafa Bakhoday-Paskyabi, Joachim Reuder, and Finn Gunnar Nielsen
Geosci. Model Dev., 16, 3553–3564, https://doi.org/10.5194/gmd-16-3553-2023, https://doi.org/10.5194/gmd-16-3553-2023, 2023
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Local refinement of the grid is a powerful method allowing us to reduce the computational time while preserving the accuracy in the area of interest. Depending on the implementation, the local refinement may introduce unwanted numerical effects into the results. We study the wind speed common to the wind turbine operational speeds and confirm strong alteration of the result when the heat fluxes are present, except for the specific refinement scheme used.
Sylvia Sullivan, Behrooz Keshtgar, Nicole Albern, Elzina Bala, Christoph Braun, Anubhav Choudhary, Johannes Hörner, Hilke Lentink, Georgios Papavasileiou, and Aiko Voigt
Geosci. Model Dev., 16, 3535–3551, https://doi.org/10.5194/gmd-16-3535-2023, https://doi.org/10.5194/gmd-16-3535-2023, 2023
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Clouds absorb and re-emit infrared radiation from Earth's surface and absorb and reflect incoming solar radiation. As a result, they change atmospheric temperature gradients that drive large-scale circulation. To better simulate this circulation, we study how the radiative heating and cooling from clouds depends on model settings like grid spacing; whether we describe convection approximately or exactly; and the level of detail used to describe small-scale processes, or microphysics, in clouds.
Denis E. Sergeev, Nathan J. Mayne, Thomas Bendall, Ian A. Boutle, Alex Brown, Iva Kavcic, James Kent, Krisztian Kohary, James Manners, Thomas Melvin, Enrico Olivier, Lokesh K. Ragta, Ben J. Shipway, Jon Wakelin, Nigel Wood, and Mohamed Zerroukat
EGUsphere, https://doi.org/10.5194/egusphere-2023-647, https://doi.org/10.5194/egusphere-2023-647, 2023
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3D climate models are one of the best tools we have to study planetary atmospheres. Here, we apply LFRic-Atmosphere, a new model developed by the Met Office, to seven different scenarios for terrestrial planetary climates, including four for the exoplanet TRAPPIST-1e, a primary target for future observations. LFRic-Atmosphere reproduces these scenarios within the spread of the existing models across a range of key climatic variables, justifying its use in future exoplanet studies.
James Weber, James A. King, Katerina Sindelarova, and Maria Val Martin
Geosci. Model Dev., 16, 3083–3101, https://doi.org/10.5194/gmd-16-3083-2023, https://doi.org/10.5194/gmd-16-3083-2023, 2023
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The emissions of volatile organic compounds from vegetation (BVOCs) influence atmospheric composition and contribute to certain gases and aerosols (tiny airborne particles) which play a role in climate change. BVOC emissions are likely to change in the future due to changes in climate and land use. Therefore, accurate simulation of BVOC emission is important, and this study describes an update to the simulation of BVOC emissions in the United Kingdom Earth System Model (UKESM).
Koichi Sakaguchi, L. Ruby Leung, Colin M. Zarzycki, Jihyeon Jang, Seth McGinnis, Bryce E. Harrop, William C. Skamarock, Andrew Gettelman, Chun Zhao, William J. Gutowski, Stephen Leak, and Linda Mearns
Geosci. Model Dev., 16, 3029–3081, https://doi.org/10.5194/gmd-16-3029-2023, https://doi.org/10.5194/gmd-16-3029-2023, 2023
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We document details of the regional climate downscaling dataset produced by a global variable-resolution model. The experiment is unique in that it follows a standard protocol designed for coordinated experiments of regional models. We found negligible influence of post-processing on statistical analysis, importance of simulation quality outside of the target region, and computational challenges that our model code faced due to rapidly changing super computer systems.
Xueying Liu, Yuxuan Wang, Shailaja Wasti, Wei Li, Ehsan Soleimanian, James Flynn, Travis Griggs, Sergio Alvarez, John T. Sullivan, Maurice Roots, Laurence Twigg, Guillaume Gronoff, Timothy Berkoff, Paul Walter, Mark Estes, Johnathan W. Hair, Taylor Shingler, Amy Jo Scarino, Marta Fenn, and Laura Judd
EGUsphere, https://doi.org/10.5194/egusphere-2023-892, https://doi.org/10.5194/egusphere-2023-892, 2023
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With a comprehensive suite of ground-based and airborne remote sensing measurements during the 2021 Tracking Aerosol Convection Experiment Air Quality (TRACER-AQ) campaign in Houston, this study evaluates the simulation of the planetary boundary layer (PBL) height and the ozone vertical profile by a high-resolution (1.33 km) 3-D photochemical model Weather Research and Forecasting-driven GEOS-Chem (WRF-GC).
Xiaohan Li, Yi Zhang, Xindong Peng, Baiquan Zhou, Jian Li, and Yiming Wang
Geosci. Model Dev., 16, 2975–2993, https://doi.org/10.5194/gmd-16-2975-2023, https://doi.org/10.5194/gmd-16-2975-2023, 2023
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The weather and climate physics suites used in GRIST-A22.7.28 are compared using single-column modeling. The source of their discrepancies in terms of modeling cloud and precipitation is explored. Convective parameterization is found to be a key factor responsible for the differences. The two suites also have intrinsic differences in the interaction between microphysics and other processes, resulting in different cloud features and time step sensitivities.
Virginie Marécal, Ronan Voisin-Plessis, Tjarda Jane Roberts, Alessandro Aiuppa, Herizo Narivelo, Paul David Hamer, Béatrice Josse, Jonathan Guth, Luke Surl, and Lisa Grellier
Geosci. Model Dev., 16, 2873–2898, https://doi.org/10.5194/gmd-16-2873-2023, https://doi.org/10.5194/gmd-16-2873-2023, 2023
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We implemented a halogen volcanic chemistry scheme in a one-dimensional modelling framework preparing for further use in a three-dimensional global chemistry-transport model. The results of the simulations for an eruption of Mt Etna in 2008, including various sensitivity tests, show a good consistency with previous modelling studies.
Zhe Feng, Joseph Hardin, Hannah C. Barnes, Jianfeng Li, L. Ruby Leung, Adam Varble, and Zhixiao Zhang
Geosci. Model Dev., 16, 2753–2776, https://doi.org/10.5194/gmd-16-2753-2023, https://doi.org/10.5194/gmd-16-2753-2023, 2023
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PyFLEXTRKR is a flexible atmospheric feature tracking framework with specific capabilities to track convective clouds from a variety of observations and model simulations. The package has a collection of multi-object identification algorithms and has been optimized for large datasets. This paper describes the algorithms and demonstrates applications for tracking deep convective cells and mesoscale convective systems from observations and model simulations at a wide range of scales.
Yan Ji, Bing Gong, Michael Langguth, Amirpasha Mozaffari, and Xiefei Zhi
Geosci. Model Dev., 16, 2737–2752, https://doi.org/10.5194/gmd-16-2737-2023, https://doi.org/10.5194/gmd-16-2737-2023, 2023
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Formulating short-term precipitation forecasting as a video prediction task, a novel deep learning architecture (convolutional long short-term memory generative adversarial network, CLGAN) is proposed. A benchmark dataset is built on minute-level precipitation measurements. Results show that with the GAN component the model generates predictions sharing statistical properties with observations, resulting in it outperforming the baseline in dichotomous and spatial scores for heavy precipitation.
Aleksander Lacima, Hervé Petetin, Albert Soret, Dene Bowdalo, Oriol Jorba, Zhaoyue Chen, Raúl F. Méndez Turrubiates, Hicham Achebak, Joan Ballester, and Carlos Pérez García-Pando
Geosci. Model Dev., 16, 2689–2718, https://doi.org/10.5194/gmd-16-2689-2023, https://doi.org/10.5194/gmd-16-2689-2023, 2023
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Understanding how air pollution varies across space and time is of key importance for the safeguarding of human health. This work arose in the context of the project EARLY-ADAPT, for which the Barcelona Supercomputing Center developed an air pollution database covering all of Europe. Through different statistical methods, we compared two global pollution models against measurements from ground stations and found significant discrepancies between the observed and the modeled surface pollution.
Dien Wu, Joshua L. Laughner, Junjie Liu, Paul I. Palmer, John C. Lin, and Paul O. Wennberg
EGUsphere, https://doi.org/10.5194/egusphere-2023-876, https://doi.org/10.5194/egusphere-2023-876, 2023
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To balance computational expenses and chemical complexity in extracting emission signals from tropospheric NO2 columns, we propose a simplified non-linear Lagrangian chemistry transport model and evaluate modeled results against TROPOMI v2 over multiple power plants and cities. Using this model, we then discuss how NOx chemistry affects the relationship between NOx and CO2 emissions and how studying NO2 columns helps quantify modeled biases in wind direction and prior emissions.
William Rudisill, Alejandro Flores, and Rosemary Carroll
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2023-69, https://doi.org/10.5194/gmd-2023-69, 2023
Preprint under review for GMD
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It's important to know how well atmospheric models do in the mountains, but there aren't very many weather stations. We evaluate rain and snow from a model from 1987–2020 in the Upper Colorado river basin against the data that's available. The model works pretty well but, there are still some uncertainties in remote locations. We then use snow maps collected by aircraft, streamflow measurements, and some advanced statistics to help identify how well the model works in ways we couldn't before.
Andrew Geiss, Po-Lun Ma, Balwinder Singh, and Joseph C. Hardin
Geosci. Model Dev., 16, 2355–2370, https://doi.org/10.5194/gmd-16-2355-2023, https://doi.org/10.5194/gmd-16-2355-2023, 2023
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Atmospheric aerosols play a critical role in Earth's climate, but it is too computationally expensive to directly model their interaction with radiation in climate simulations. This work develops a new neural-network-based parameterization of aerosol optical properties for use in the Energy Exascale Earth System Model that is much more accurate than the current one; it also introduces a unique model optimization method that involves randomly generating neural network architectures.
Joey C. Y. Lam, Amos P. K. Tai, Jason A. Ducker, and Christopher D. Holmes
Geosci. Model Dev., 16, 2323–2342, https://doi.org/10.5194/gmd-16-2323-2023, https://doi.org/10.5194/gmd-16-2323-2023, 2023
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We developed a new component within an atmospheric chemistry model to better simulate plant ecophysiological processes relevant for ozone air quality. We showed that it reduces simulated biases in plant uptake of ozone in prior models. The new model enables us to explore how future climatic changes affect air quality via affecting plants, examine ozone–vegetation interactions and feedbacks, and evaluate the impacts of changing atmospheric chemistry and climate on vegetation productivity.
Qian Shu, Sergey L. Napelenok, William T. Hutzell, Kirk R. Baker, Barron H. Henderson, Benjamin N. Murphy, and Christian Hogrefe
Geosci. Model Dev., 16, 2303–2322, https://doi.org/10.5194/gmd-16-2303-2023, https://doi.org/10.5194/gmd-16-2303-2023, 2023
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Source attribution methods are generally used to determine culpability of precursor emission sources to ambient pollutant concentrations. However, source attribution of secondarily formed pollutants such as ozone and its precursors cannot be explicitly measured, making evaluation of source apportionment methods challenging. In this study, multiple apportionment approach comparisons show common features but still reveal wide variations in predicted sector contribution and species dependency.
Rüdiger Brecht, Lucie Bakels, Alex Bihlo, and Andreas Stohl
Geosci. Model Dev., 16, 2181–2192, https://doi.org/10.5194/gmd-16-2181-2023, https://doi.org/10.5194/gmd-16-2181-2023, 2023
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We use neural-network-based single-image super-resolution to improve the upscaling of meteorological wind fields to be used for particle dispersion models. This deep-learning-based methodology improves the standard linear interpolation typically used in particle dispersion models. The improvement of wind fields leads to substantial improvement in the computed trajectories of the particles.
Alvaro Criado, Jan Mateu Armengol, Hervé Petetin, Daniel Rodriguez-Rey, Jaime Benavides, Marc Guevara, Carlos Pérez García-Pando, Albert Soret, and Oriol Jorba
Geosci. Model Dev., 16, 2193–2213, https://doi.org/10.5194/gmd-16-2193-2023, https://doi.org/10.5194/gmd-16-2193-2023, 2023
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This work aims to derive and evaluate a general statistical post-processing tool specifically designed for the street scale that can be applied to any urban air quality system. Our data fusion methodology corrects NO2 fields based on continuous hourly observations and experimental campaigns. This study enables us to obtain exceedance probability maps of air quality standards. In 2019, 13 % of the Barcelona area had a 70 % or higher probability of exceeding the annual legal NO2 limit of 40 µg/m3.
Liang Wang, Bingcheng Wan, Shaohui Zhou, Haofei Sun, and Zhiqiu Gao
Geosci. Model Dev., 16, 2167–2179, https://doi.org/10.5194/gmd-16-2167-2023, https://doi.org/10.5194/gmd-16-2167-2023, 2023
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The past 24 h TC trajectories and meteorological field data were used to forecast TC tracks in the northwestern Pacific from hours 6–72 based on GRU_CNN, which we proposed in this paper and which has better prediction results than traditional single deep-learning methods. The historical steering flow of cyclones has a significant effect on improving the accuracy of short-term forecasting, while, in long-term forecasting, the SST and geopotential height will have a particular impact.
Roland Eichinger, Sebastian Rhode, Hella Garny, Peter Preusse, Petr Pisoft, Aleš Kuchar, Patrick Jöckel, Astrid Kerkweg, and Bastian Kern
EGUsphere, https://doi.org/10.5194/egusphere-2023-270, https://doi.org/10.5194/egusphere-2023-270, 2023
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Dynamical model biases result from the columnar approach of gravity wave (GW) schemes, but parallel decomposition makes horizontal GW propagation computationally unfeasible. In the global model EMAC, we approximate it by GW redistribution at one altitude using tailor-made redistribution maps generated with a ray-tracer. More spread-out GW drag helps reconciling the model with observations and closing the 60S GW gap. Polar vortex dynamics are improved, enhancing climate model credibility.
Thibaud Sarica, Alice Maison, Yelva Roustan, Matthias Ketzel, Steen Solvang Jensen, Youngseob Kim, Christophe Chaillou, and Karine Sartelet
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2023-70, https://doi.org/10.5194/gmd-2023-70, 2023
Revised manuscript accepted for GMD
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A new version of the Model of Urban Network of Intersecting Canyons and Highways (MUNICH) is developed to represent heterogeneities of concentrations in streets. The street volume is discretized vertically and horizontally to limit the artificial dilution of emissions and concentrations. This new version is applied to street networks in Copenhagen and Paris. The comparisons to observations are improved, with higher concentrations of pollutants emitted by traffic at the bottom of the street.
Thomas Berkemeier, Matteo Krüger, Aryeh Feinberg, Marcel Müller, Ulrich Pöschl, and Ulrich K. Krieger
Geosci. Model Dev., 16, 2037–2054, https://doi.org/10.5194/gmd-16-2037-2023, https://doi.org/10.5194/gmd-16-2037-2023, 2023
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Kinetic multi-layer models (KMs) successfully describe heterogeneous and multiphase atmospheric chemistry. In applications requiring repeated execution, however, these models can be too expensive. We trained machine learning surrogate models on output of the model KM-SUB and achieved high correlations. The surrogate models run orders of magnitude faster, which suggests potential applicability in global optimization tasks and as sub-modules in large-scale atmospheric models.
Elena Fillola, Raul Santos-Rodriguez, Alistair Manning, Simon O'Doherty, and Matt Rigby
Geosci. Model Dev., 16, 1997–2009, https://doi.org/10.5194/gmd-16-1997-2023, https://doi.org/10.5194/gmd-16-1997-2023, 2023
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Lagrangian particle dispersion models are used extensively for the estimation of greenhouse gas (GHG) fluxes using atmospheric observations. However, these models do not scale well as data volumes increase. Here, we develop a proof-of-concept machine learning emulator that can produce outputs similar to those of the dispersion model, but 50 000 times faster, using only meteorological inputs. This works demonstrates the potential of machine learning to accelerate GHG estimations across the globe.
Stijn Van Leuven, Pieter De Meutter, Johan Camps, Piet Termonia, and Andy Delcloo
EGUsphere, https://doi.org/10.5194/egusphere-2023-357, https://doi.org/10.5194/egusphere-2023-357, 2023
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Precipitation collects airborne particles and deposits these on the ground. This process is called wet deposition and greatly determines how airborne radioactive particles (released routinely or accidental) contaminate the surface. In this work we present a new method to improve the calculation of wet deposition in computer models. We apply this method to the existing model FLEXPART by simulating the Fukushima nuclear accident (2011), and show that it improves the simulation of wet deposition.
Maria J. Chinita, Mikael Witte, Marcin J. Kurowski, Joao Teixeira, Kay Suselj, Georgios Matheou, and Peter Bogenschutz
Geosci. Model Dev., 16, 1909–1924, https://doi.org/10.5194/gmd-16-1909-2023, https://doi.org/10.5194/gmd-16-1909-2023, 2023
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Low clouds are one of the largest sources of uncertainty in climate prediction. In this paper, we introduce the first version of the unified turbulence and shallow convection parameterization named SHOC+MF developed to improve the representation of shallow cumulus clouds in the Simple Cloud-Resolving E3SM Atmosphere Model (SCREAM). Here, we also show promising preliminary results in a single-column model framework for two benchmark cases of shallow cumulus convection.
Kun Wang, Chao Gao, Kai Wu, Kaiyun Liu, Haofan Wang, Mo Dan, Xiaohui Ji, and Qingqing Tong
Geosci. Model Dev., 16, 1961–1973, https://doi.org/10.5194/gmd-16-1961-2023, https://doi.org/10.5194/gmd-16-1961-2023, 2023
Short summary
Short summary
This study establishes an easy-to-use and integrated framework for a model-ready emission inventory for the Weather Research and Forecasting (WRF)–Air Quality Numerical Model (AQM). A free tool called the ISAT (Inventory Spatial Allocation Tool) was developed based on this framework. ISAT helps users complete the workflow from the WRF nested-domain configuration to a model-ready emission inventory for AQM with a regional emission inventory and a shapefile for the target region.
Cited articles
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Short summary
This paper describes the implementation of the atmospheric water tracer (AWT) method in the NCAR Community Atmosphere Model version 5.1 (CAM5.1). Compared to other source apportionment methods, the AWT method was developed based on detailed physical parameterisations, and can therefore trace the behaviour of atmospheric water substances directly and exactly. Using this method, we quantitatively identify the dominant sources of precipitation and water vapour over East Asia.
This paper describes the implementation of the atmospheric water tracer (AWT) method in the NCAR...