Development and technical paper 15 Jan 2021
Development and technical paper | 15 Jan 2021
Optimization of the sulfate aerosol hygroscopicity parameter in WRF-Chem
Ah-Hyun Kim et al.
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Najin Kim, Seong Soo Yum, Minsu Park, Jong Sung Park, Hye Jung Shin, and Joon Young Ahn
Atmos. Chem. Phys., 20, 11245–11262, https://doi.org/10.5194/acp-20-11245-2020, https://doi.org/10.5194/acp-20-11245-2020, 2020
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Chemical effects on the size-resolved hygroscopicity of urban aerosols were examined based on the KORUS-AQ field campaign data (HTDMA and HR-ToF-AMS). The size-resolved chemical composition data were found to be critical in explaining the size-dependent hygroscopicity, as well as the diurnal variation of κ for small particles. Aerosol mixing state information was associated with the size-resolved chemical composition data to reveal chemical information of different hygroscopicity modes.
Jiyeon Park, Manuel Dall'Osto, Kihong Park, Yeontae Gim, Hyo Jin Kang, Eunho Jang, Ki-Tae Park, Minsu Park, Seong Soo Yum, Jinyoung Jung, Bang Yong Lee, and Young Jun Yoon
Atmos. Chem. Phys., 20, 5573–5590, https://doi.org/10.5194/acp-20-5573-2020, https://doi.org/10.5194/acp-20-5573-2020, 2020
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The physical properties of aerosol particles throughout the Arctic Ocean and Pacific Ocean were measured aboard the Korean icebreaker R/V Araon during the summer of 2017. A number of new particle formation (NPF) events and growth were frequently observed in both Arctic terrestrial and Arctic marine air masses. This suggests that terrestrial ecosystems – including river outflows and tundra – strongly affect aerosol emissions in the Arctic coastal areas, affecting
radiative forcing.
Junshik Um, Greg M. McFarquhar, Jeffrey L. Stith, Chang Hoon Jung, Seoung Soo Lee, Ji Yi Lee, Younghwan Shin, Yun Gon Lee, Yiseok Isaac Yang, Seong Soo Yum, Byung-Gon Kim, Joo Wan Cha, and A-Reum Ko
Atmos. Chem. Phys., 18, 16915–16930, https://doi.org/10.5194/acp-18-16915-2018, https://doi.org/10.5194/acp-18-16915-2018, 2018
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During the 2012 Deep Convective Clouds and Chemistry experiment upper anvils of two storms were sampled. The occurrence of well-defined pristine crystals was low in the anvils, while single frozen droplets and frozen droplet aggregates (FDAs) were the dominant habits. A new algorithm was developed to automatically identify the number, size, and relative position of element frozen droplets within FDAs. The morphological characteristics of FDAs were compared with those of black carbon aggregates.
Julia Schmale, Silvia Henning, Stefano Decesari, Bas Henzing, Helmi Keskinen, Karine Sellegri, Jurgita Ovadnevaite, Mira L. Pöhlker, Joel Brito, Aikaterini Bougiatioti, Adam Kristensson, Nikos Kalivitis, Iasonas Stavroulas, Samara Carbone, Anne Jefferson, Minsu Park, Patrick Schlag, Yoko Iwamoto, Pasi Aalto, Mikko Äijälä, Nicolas Bukowiecki, Mikael Ehn, Göran Frank, Roman Fröhlich, Arnoud Frumau, Erik Herrmann, Hartmut Herrmann, Rupert Holzinger, Gerard Kos, Markku Kulmala, Nikolaos Mihalopoulos, Athanasios Nenes, Colin O'Dowd, Tuukka Petäjä, David Picard, Christopher Pöhlker, Ulrich Pöschl, Laurent Poulain, André Stephan Henry Prévôt, Erik Swietlicki, Meinrat O. Andreae, Paulo Artaxo, Alfred Wiedensohler, John Ogren, Atsushi Matsuki, Seong Soo Yum, Frank Stratmann, Urs Baltensperger, and Martin Gysel
Atmos. Chem. Phys., 18, 2853–2881, https://doi.org/10.5194/acp-18-2853-2018, https://doi.org/10.5194/acp-18-2853-2018, 2018
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Collocated long-term observations of cloud condensation nuclei (CCN) number concentrations, particle number size distributions and chemical composition from 12 sites are synthesized. Observations cover coastal environments, the Arctic, the Mediterranean, the boreal and rain forest, high alpine and continental background sites, and Monsoon-influenced areas. We interpret regional and seasonal variability. CCN concentrations are predicted with the κ–Köhler model and compared to the measurements.
J. H. Kim, S. S. Yum, S. Shim, W. J. Kim, M. Park, J.-H. Kim, M.-H. Kim, and S.-C. Yoon
Atmos. Chem. Phys., 14, 8763–8779, https://doi.org/10.5194/acp-14-8763-2014, https://doi.org/10.5194/acp-14-8763-2014, 2014
Related subject area
Climate and Earth system modeling
Evaluation of polar stratospheric clouds in the global chemistry–climate model SOCOLv3.1 by comparison with CALIPSO spaceborne lidar measurements
Lossy compression of Earth system model data based on a hierarchical tensor with Adaptive-HGFDR (v1.0)
Methane chemistry in a nutshell – the new submodels CH4 (v1.0) and TRSYNC (v1.0) in MESSy (v2.54.0)
Coordinating an operational data distribution network for CMIP6 data
Implementation of sequential cropping into JULESvn5.2 land-surface model
Development of four-dimensional variational assimilation system based on the GRAPES–CUACE adjoint model (GRAPES–CUACE-4D-Var V1.0) and its application in emission inversion
HIRM v1.0: a hybrid impulse response model for climate modeling and uncertainty analyses
CLIMADA v1.4.1: towards a globally consistent adaptation options appraisal tool
FORTE 2.0: a fast, parallel and flexible coupled climate model
Updated European hydraulic pedotransfer functions with communicated uncertainties in the predicted variables (euptfv2)
Spin-up characteristics with three types of initial fields and the restart effects on forecast accuracy in the GRAPES global forecast system
GTS v1.0: a macrophysics scheme for climate models based on a probability density function
Calibration of temperature-dependent ocean microbial processes in the cGENIE.muffin (v0.9.13) Earth system model
Description and evaluation of aerosol in UKESM1 and HadGEM3-GC3.1 CMIP6 historical simulations
DiRong1.0: a distributed implementation for improving routing network generation in model coupling
Overview of the Norwegian Earth System Model (NorESM2) and key climate response of CMIP6 DECK, historical, and scenario simulations
Geospatial input data for the PALM model system 6.0: model requirements, data sources and processing
Exploring the parameter space of the COSMO-CLM v5.0 regional climate model for the Central Asia CORDEX domain
The benefits of increasing resolution in global and regional climate simulations for European climate extremes
European daily precipitation according to EURO-CORDEX regional climate models (RCMs) and high-resolution global climate models (GCMs) from the High-Resolution Model Intercomparison Project (HighResMIP)
Harmonization of global land use change and management for the period 850–2100 (LUH2) for CMIP6
A computationally efficient method for probabilistic local warming projections constrained by history matching and pattern scaling, demonstrated by WASP–LGRTC-1.0
R2D2 v2.0: accounting for temporal dependences in multivariate bias correction via analogue rank resampling
Extending the Modular Earth Submodel System (MESSy v2.54) model hierarchy: the ECHAM/MESSy IdeaLized (EMIL) model setup
Boreal summer intraseasonal oscillation in a superparameterized general circulation model: effects of air–sea coupling and ocean mean state
Reduced Complexity Model Intercomparison Project Phase 1: introduction and evaluation of global-mean temperature response
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A new bias-correction method for precipitation over complex terrain suitable for different climate states: a case study using WRF (version 3.8.1)
A process-based evaluation of the Intermediate Complexity Atmospheric Research Model (ICAR) 1.0.1
ISSM-SLPS: geodetically compliant Sea-Level Projection System for the Ice-sheet and Sea-level System Model v4.17
Newly developed aircraft routing options for air traffic simulation in the chemistry–climate model EMAC 2.53: AirTraf 2.0
Quantifying CanESM5 and EAMv1 sensitivities to Mt. Pinatubo volcanic forcing for the CMIP6 historical experiment
Optimizing high-resolution Community Earth System Model on a heterogeneous many-core supercomputing platform
Understanding the development of systematic errors in the Asian Summer Monsoon
MIROC-INTEG-LAND version 1: a global biogeochemical land surface model with human water management, crop growth, and land-use change
Optimality-based non-Redfield plankton–ecosystem model (OPEM v1.1) in UVic-ESCM 2.9 – Part 2: Sensitivity analysis and model calibration
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Effects of Coupling a Stochastic Convective Parameterization with Zhang-McFarlane Scheme on Precipitation Simulation in the DOE E3SMv1 Atmosphere Model
The E3SM version 1 single-column model
RadNet 1.0: exploring deep learning architectures for longwave radiative transfer
Efficient ensemble data assimilation for coupled models with the Parallel Data Assimilation Framework: example of AWI-CM (AWI-CM-PDAF 1.0)
Modelling mineral dust emissions and atmospheric dispersion with MADE3 in EMAC v2.54
Evaluation of the University of Victoria Earth System Climate Model version 2.10 (UVic ESCM 2.10)
Earth System Model Evaluation Tool (ESMValTool) v2.0 – diagnostics for emergent constraints and future projections from Earth system models in CMIP
Evaluating the land-surface energy partitioning in ERA5
Robust Ecosystem Demography (RED version 1.0): a parsimonious approach to modelling vegetation dynamics in Earth system models
The GGCMI Phase 2 emulators: global gridded crop model responses to changes in CO2, temperature, water, and nitrogen (version 1.0)
Role of vegetation in representing land surface temperature in the CHTESSEL (CY45R1) and SURFEX-ISBA (v8.1) land surface models: a case study over Iberia
Simulating the mid-Holocene, Last Interglacial and mid-Pliocene climate with EC-Earth3-LR
Taiwan Earth System Model Version 1: description and evaluation of mean state
Michael Steiner, Beiping Luo, Thomas Peter, Michael C. Pitts, and Andrea Stenke
Geosci. Model Dev., 14, 935–959, https://doi.org/10.5194/gmd-14-935-2021, https://doi.org/10.5194/gmd-14-935-2021, 2021
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We evaluate polar stratospheric clouds (PSCs) as simulated by the chemistry–climate model (CCM) SOCOLv3.1 in comparison with measurements by the CALIPSO satellite. A cold bias results in an overestimated PSC area and mountain-wave ice is underestimated, but we find overall good temporal and spatial agreement of PSC occurrence and composition. This work confirms previous studies indicating that simplified PSC schemes may also achieve good approximations of the fundamental properties of PSCs.
Zhaoyuan Yu, Dongshuang Li, Zhengfang Zhang, Wen Luo, Yuan Liu, Zengjie Wang, and Linwang Yuan
Geosci. Model Dev., 14, 875–887, https://doi.org/10.5194/gmd-14-875-2021, https://doi.org/10.5194/gmd-14-875-2021, 2021
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Few lossy compression methods consider both the global and local multidimensional coupling correlations, which could lead to information loss in data compression. Here we develop an adaptive lossy compression method, Adaptive-HGFDR, to capture both the global and local variation of multidimensional coupling correlations and improve approximation accuracy. The method can achieve good compression performances for most flux variables with significant spatiotemporal heterogeneity.
Franziska Winterstein and Patrick Jöckel
Geosci. Model Dev., 14, 661–674, https://doi.org/10.5194/gmd-14-661-2021, https://doi.org/10.5194/gmd-14-661-2021, 2021
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Atmospheric methane is currently a hot topic in climate research. This is partly due to its chemically active nature. We introduce a simplified approach to simulate methane in climate models to enable large sensitivity studies by reducing computational cost but including the crucial feedback of methane on stratospheric water vapour. We further provide options to simulate the isotopic content of methane and to generate output for an inverse optimization technique for emission estimation.
Ruth Petrie, Sébastien Denvil, Sasha Ames, Guillaume Levavasseur, Sandro Fiore, Chris Allen, Fabrizio Antonio, Katharina Berger, Pierre-Antoine Bretonnière, Luca Cinquini, Eli Dart, Prashanth Dwarakanath, Kelsey Druken, Ben Evans, Laurent Franchistéguy, Sébastien Gardoll, Eric Gerbier, Mark Greenslade, David Hassell, Alan Iwi, Martin Juckes, Stephan Kindermann, Lukasz Lacinski, Maria Mirto, Atef Ben Nasser, Paola Nassisi, Eric Nienhouse, Sergey Nikonov, Alessandra Nuzzo, Clare Richards, Syazwan Ridzwan, Michel Rixen, Kim Serradell, Kate Snow, Ag Stephens, Martina Stockhause, Hans Vahlenkamp, and Rick Wagner
Geosci. Model Dev., 14, 629–644, https://doi.org/10.5194/gmd-14-629-2021, https://doi.org/10.5194/gmd-14-629-2021, 2021
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This paper describes the infrastructure that is used to distribute Coupled Model Intercomparison Project Phase 6 (CMIP6) data around the world for analysis by the climate research community. It is expected that there will be ~20 PB (petabytes) of data available for analysis. The operations team performed a series of preparation "data challenges" to ensure all components of the infrastructure were operational for when the data became available for timely data distribution and subsequent analysis.
Camilla Mathison, Andrew J. Challinor, Chetan Deva, Pete Falloon, Sébastien Garrigues, Sophie Moulin, Karina Williams, and Andy Wiltshire
Geosci. Model Dev., 14, 437–471, https://doi.org/10.5194/gmd-14-437-2021, https://doi.org/10.5194/gmd-14-437-2021, 2021
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Sequential cropping (also known as multiple or double cropping) is a common cropping system, particularly in tropical regions. Typically, land surface models only simulate a single crop per year. To understand how sequential crops influence surface fluxes, we implement sequential cropping in JULES to simulate all the crops grown within a year at a given location in a seamless way. We demonstrate the method using a site in Avignon, four locations in India and a regional run for two Indian states.
Chao Wang, Xingqin An, Qing Hou, Zhaobin Sun, Yanjun Li, and Jiangtao Li
Geosci. Model Dev., 14, 337–350, https://doi.org/10.5194/gmd-14-337-2021, https://doi.org/10.5194/gmd-14-337-2021, 2021
Kalyn Dorheim, Steven J. Smith, and Ben Bond-Lamberty
Geosci. Model Dev., 14, 365–375, https://doi.org/10.5194/gmd-14-365-2021, https://doi.org/10.5194/gmd-14-365-2021, 2021
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Simple climate models are frequently used in research and decision-making communities because of their tractability and low computational cost. Simple climate models are diverse, including highly idealized and process-based models. Here we present a hybrid approach that combines the strength of two types of simple climate models in a flexible framework. This hybrid approach has provided insights into the climate system and opens an avenue for investigating radiative forcing uncertainties.
David N. Bresch and Gabriela Aznar-Siguan
Geosci. Model Dev., 14, 351–363, https://doi.org/10.5194/gmd-14-351-2021, https://doi.org/10.5194/gmd-14-351-2021, 2021
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Climate change is a fact and adaptation a necessity. The Economics of Climate Adaptation methodology provides a framework to integrate risk and reward perspectives of different stakeholders, underpinned by the CLIMADA impact modelling platform. This extended version of CLIMADA enables risk assessment and options appraisal in a modular form and occasionally bespoke fashion yet with high reusability of functionalities to foster usage in interdisciplinary studies and international collaboration.
Adam T. Blaker, Manoj Joshi, Bablu Sinha, David P. Stevens, Robin S. Smith, and Joël J.-M. Hirschi
Geosci. Model Dev., 14, 275–293, https://doi.org/10.5194/gmd-14-275-2021, https://doi.org/10.5194/gmd-14-275-2021, 2021
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FORTE 2.0 is a flexible coupled atmosphere–ocean general circulation model that can be run on modest hardware. We present two 2000-year simulations which show that FORTE 2.0 is capable of producing a stable climate. Earlier versions of FORTE were used for a wide range of studies, ranging from aquaplanet configurations to investigating the cold European winters of 2009–2010. This paper introduces the updated model for which the code and configuration are now publicly available.
Brigitta Szabó, Melanie Weynants, and Tobias K. D. Weber
Geosci. Model Dev., 14, 151–175, https://doi.org/10.5194/gmd-14-151-2021, https://doi.org/10.5194/gmd-14-151-2021, 2021
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This paper presents updated European prediction algorithms (euptf2) to compute soil hydraulic parameters from easily available soil properties. The new algorithms lead to significantly better predictions and provide a built-in prediction uncertainty computation. The influence of predictor variables on predicted soil hydraulic properties is explored and practical guidance on how to use the derived PTFs is provided. A website and an R package facilitate easy application of the updated predictions.
Zhanshan Ma, Chuanfeng Zhao, Jiandong Gong, Jin Zhang, Zhe Li, Jian Sun, Yongzhu Liu, Jiong Chen, and Qingu Jiang
Geosci. Model Dev., 14, 205–221, https://doi.org/10.5194/gmd-14-205-2021, https://doi.org/10.5194/gmd-14-205-2021, 2021
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The spin-up in GRAPES_GFS, under different initial fields, goes through a dramatic adjustment in the first half-hour of integration and slow dynamic and thermal adjustments afterwards. It lasts for at least 6 h, with model adjustment gradually completed from lower to upper layers in the model. Thus, the forecast results, at least in the first 6 h, should be avoided when used. In addition, the spin-up process should repeat when the model simulation is interrupted.
Chein-Jung Shiu, Yi-Chi Wang, Huang-Hsiung Hsu, Wei-Ting Chen, Hua-Lu Pan, Ruiyu Sun, Yi-Hsuan Chen, and Cheng-An Chen
Geosci. Model Dev., 14, 177–204, https://doi.org/10.5194/gmd-14-177-2021, https://doi.org/10.5194/gmd-14-177-2021, 2021
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A cloud macrophysics scheme utilizing grid-mean hydrometeor information is developed and evaluated for climate models. The GFS–TaiESM–Sundqvist (GTS) scheme can simulate variations of cloud fraction associated with relative humidity (RH) in a more consistent way than the default scheme of CAM5.3. Through better cloud–RH distributions, the GTS scheme helps to better represent cloud fraction, cloud radiative forcing, and thermodynamic-related climatic fields in climate simulations.
Katherine A. Crichton, Jamie D. Wilson, Andy Ridgwell, and Paul N. Pearson
Geosci. Model Dev., 14, 125–149, https://doi.org/10.5194/gmd-14-125-2021, https://doi.org/10.5194/gmd-14-125-2021, 2021
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Temperature is a controller of metabolic processes and therefore also a controller of the ocean's biological carbon pump (BCP). We calibrate a temperature-dependent version of the BCP in the cGENIE Earth system model. Since the pre-industrial period, warming has intensified near-surface nutrient recycling, supporting production and largely offsetting stratification-induced surface nutrient limitation. But at the same time less carbon that sinks out of the surface then reaches the deep ocean.
Jane P. Mulcahy, Colin Johnson, Colin G. Jones, Adam C. Povey, Catherine E. Scott, Alistair Sellar, Steven T. Turnock, Matthew T. Woodhouse, Nathan Luke Abraham, Martin B. Andrews, Nicolas Bellouin, Jo Browse, Ken S. Carslaw, Mohit Dalvi, Gerd A. Folberth, Matthew Glover, Daniel P. Grosvenor, Catherine Hardacre, Richard Hill, Ben Johnson, Andy Jones, Zak Kipling, Graham Mann, James Mollard, Fiona M. O'Connor, Julien Palmiéri, Carly Reddington, Steven T. Rumbold, Mark Richardson, Nick A. J. Schutgens, Philip Stier, Marc Stringer, Yongming Tang, Jeremy Walton, Stephanie Woodward, and Andrew Yool
Geosci. Model Dev., 13, 6383–6423, https://doi.org/10.5194/gmd-13-6383-2020, https://doi.org/10.5194/gmd-13-6383-2020, 2020
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Aerosols are an important component of the Earth system. Here, we comprehensively document and evaluate the aerosol schemes as implemented in the physical and Earth system models, HadGEM3-GC3.1 and UKESM1. This study provides a useful characterisation of the aerosol climatology in both models, facilitating the understanding of the numerous aerosol–climate interaction studies that will be conducted for CMIP6 and beyond.
Hao Yu, Li Liu, Chao Sun, Ruizhe Li, Xinzhu Yu, Cheng Zhang, Zhiyuan Zhang, and Bin Wang
Geosci. Model Dev., 13, 6253–6263, https://doi.org/10.5194/gmd-13-6253-2020, https://doi.org/10.5194/gmd-13-6253-2020, 2020
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Routing network generation is a major step for initializing the data transfer functionality for model coupling. The distributed implementation for routing network generation (DiRong1.0) proposed in this paper can significantly improve the global implementation of routing network generation used in some existing coupling software, because it does not introduce any gather–broadcast communications and achieves much lower complexity in terms of time, memory, and communication.
Øyvind Seland, Mats Bentsen, Dirk Olivié, Thomas Toniazzo, Ada Gjermundsen, Lise Seland Graff, Jens Boldingh Debernard, Alok Kumar Gupta, Yan-Chun He, Alf Kirkevåg, Jörg Schwinger, Jerry Tjiputra, Kjetil Schanke Aas, Ingo Bethke, Yuanchao Fan, Jan Griesfeller, Alf Grini, Chuncheng Guo, Mehmet Ilicak, Inger Helene Hafsahl Karset, Oskar Landgren, Johan Liakka, Kine Onsum Moseid, Aleksi Nummelin, Clemens Spensberger, Hui Tang, Zhongshi Zhang, Christoph Heinze, Trond Iversen, and Michael Schulz
Geosci. Model Dev., 13, 6165–6200, https://doi.org/10.5194/gmd-13-6165-2020, https://doi.org/10.5194/gmd-13-6165-2020, 2020
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The second version of the coupled Norwegian Earth System Model (NorESM2) is presented and evaluated. The temperature and precipitation patterns has improved compared to NorESM1. The model reaches present-day warming levels to within 0.2 °C of observed temperature but with a delayed warming during the late 20th century. Under the four scenarios (SSP1-2.6, SSP2-4.5, SSP3-7.0, and SSP5-8.5), the warming in the period of 2090–2099 compared to 1850–1879 reaches 1.3, 2.2, 3.1, and 3.9 K.
Wieke Heldens, Cornelia Burmeister, Farah Kanani-Sühring, Björn Maronga, Dirk Pavlik, Matthias Sühring, Julian Zeidler, and Thomas Esch
Geosci. Model Dev., 13, 5833–5873, https://doi.org/10.5194/gmd-13-5833-2020, https://doi.org/10.5194/gmd-13-5833-2020, 2020
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For realistic microclimate simulations in urban areas with PALM 6.0, detailed description of surface types, buildings and vegetation is required. This paper shows how such input data sets can be derived with the example of three German cities. Various data sources are used, including remote sensing, municipal data collections and open data such as OpenStreetMap. The collection and preparation of input data sets is tedious. Future research aims therefore at semi-automated tools to support users.
Emmanuele Russo, Silje Lund Sørland, Ingo Kirchner, Martijn Schaap, Christoph C. Raible, and Ulrich Cubasch
Geosci. Model Dev., 13, 5779–5797, https://doi.org/10.5194/gmd-13-5779-2020, https://doi.org/10.5194/gmd-13-5779-2020, 2020
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The parameter space of the COSMO-CLM RCM is investigated for the Central Asia CORDEX domain using a perturbed physics ensemble (PPE) with different parameter values. Results show that only a subset of model parameters presents relevant changes in model performance and these changes depend on the considered region and variable: objective calibration methods are highly necessary in this case. Additionally, the results suggest the need for calibrating an RCM when targeting different domains.
Carley E. Iles, Robert Vautard, Jane Strachan, Sylvie Joussaume, Bernd R. Eggen, and Chris D. Hewitt
Geosci. Model Dev., 13, 5583–5607, https://doi.org/10.5194/gmd-13-5583-2020, https://doi.org/10.5194/gmd-13-5583-2020, 2020
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We investigate how increased resolution affects the simulation of European climate extremes for global and regional climate models to inform modelling strategies. Precipitation extremes become heavier with higher resolution, especially over mountains, wind extremes become somewhat stronger, and for temperature extremes warm biases are reduced over mountains. Differences with resolution for the global model appear to come from downscaling effects rather than improved large-scale circulation.
Marie-Estelle Demory, Ségolène Berthou, Jesús Fernández, Silje L. Sørland, Roman Brogli, Malcolm J. Roberts, Urs Beyerle, Jon Seddon, Rein Haarsma, Christoph Schär, Erasmo Buonomo, Ole B. Christensen, James M. Ciarlo ̀, Rowan Fealy, Grigory Nikulin, Daniele Peano, Dian Putrasahan, Christopher D. Roberts, Retish Senan, Christian Steger, Claas Teichmann, and Robert Vautard
Geosci. Model Dev., 13, 5485–5506, https://doi.org/10.5194/gmd-13-5485-2020, https://doi.org/10.5194/gmd-13-5485-2020, 2020
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Now that global climate models (GCMs) can run at similar resolutions to regional climate models (RCMs), one may wonder whether GCMs and RCMs provide similar regional climate information. We perform an evaluation for daily precipitation distribution in PRIMAVERA GCMs (25–50 km resolution) and CORDEX RCMs (12–50 km resolution) over Europe. We show that PRIMAVERA and CORDEX simulate similar distributions. Considering both datasets at such a resolution results in large benefits for impact studies.
George C. Hurtt, Louise Chini, Ritvik Sahajpal, Steve Frolking, Benjamin L. Bodirsky, Katherine Calvin, Jonathan C. Doelman, Justin Fisk, Shinichiro Fujimori, Kees Klein Goldewijk, Tomoko Hasegawa, Peter Havlik, Andreas Heinimann, Florian Humpenöder, Johan Jungclaus, Jed O. Kaplan, Jennifer Kennedy, Tamás Krisztin, David Lawrence, Peter Lawrence, Lei Ma, Ole Mertz, Julia Pongratz, Alexander Popp, Benjamin Poulter, Keywan Riahi, Elena Shevliakova, Elke Stehfest, Peter Thornton, Francesco N. Tubiello, Detlef P. van Vuuren, and Xin Zhang
Geosci. Model Dev., 13, 5425–5464, https://doi.org/10.5194/gmd-13-5425-2020, https://doi.org/10.5194/gmd-13-5425-2020, 2020
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To estimate the effects of human land use activities on the carbon–climate system, a new set of global gridded land use forcing datasets was developed to link historical land use data to eight future scenarios in a standard format required by climate models. This new generation of land use harmonization (LUH2) includes updated inputs, higher spatial resolution, more detailed land use transitions, and the addition of important agricultural management layers; it will be used for CMIP6 simulations.
Philip Goodwin, Martin Leduc, Antti-Ilari Partanen, H. Damon Matthews, and Alex Rogers
Geosci. Model Dev., 13, 5389–5399, https://doi.org/10.5194/gmd-13-5389-2020, https://doi.org/10.5194/gmd-13-5389-2020, 2020
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Numerical climate models are used to make projections of future surface warming for different pathways of future greenhouse gas emissions, where future surface warming will vary from place to place. However, it is so expensive to run complex models using supercomputers that future projections can only be produced for a small number of possible future emissions pathways. This study presents an efficient climate model to make projections of local surface warming using a desktop computer.
Mathieu Vrac and Soulivanh Thao
Geosci. Model Dev., 13, 5367–5387, https://doi.org/10.5194/gmd-13-5367-2020, https://doi.org/10.5194/gmd-13-5367-2020, 2020
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We propose a multivariate bias correction (MBC) method to adjust the spatial and/or inter-variable properties of climate simulations, while also accounting for their temporal dependences (e.g., autocorrelations).
It consists on a method reordering the ranks of the time series according to their multivariate distance to a reference time series.
Results show that temporal correlations are improved while spatial and inter-variable correlations are still satisfactorily corrected.
Hella Garny, Roland Walz, Matthias Nützel, and Thomas Birner
Geosci. Model Dev., 13, 5229–5257, https://doi.org/10.5194/gmd-13-5229-2020, https://doi.org/10.5194/gmd-13-5229-2020, 2020
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Numerical models of Earth's climate system have been gaining more and more complexity over the last decades. Therefore, it is important to establish simplified models to improve process understanding. In our study, we present and document the development of a new simplified model setup within the framework of a complex climate model system that uses the same routines to calculate atmospheric dynamics as the complex model but is simplified in the representation of clouds and radiation.
Yingxia Gao, Nicholas P. Klingaman, Charlotte A. DeMott, and Pang-Chi Hsu
Geosci. Model Dev., 13, 5191–5209, https://doi.org/10.5194/gmd-13-5191-2020, https://doi.org/10.5194/gmd-13-5191-2020, 2020
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Both the air–sea coupling and ocean mean state affect the fidelity of simulated boreal summer intraseasonal oscillation (BSISO). To elucidate their relative effects on the simulated BSISO, a set of experiments was conducted using a superparameterized AGCM and its coupled version. Both air–sea coupling and cold ocean mean state improve the BSISO amplitude due to the suppression of the overestimated variance, while the former (latter) could further upgrade (degrade) the BSISO propagation.
Zebedee R. J. Nicholls, Malte Meinshausen, Jared Lewis, Robert Gieseke, Dietmar Dommenget, Kalyn Dorheim, Chen-Shuo Fan, Jan S. Fuglestvedt, Thomas Gasser, Ulrich Golüke, Philip Goodwin, Corinne Hartin, Austin P. Hope, Elmar Kriegler, Nicholas J. Leach, Davide Marchegiani, Laura A. McBride, Yann Quilcaille, Joeri Rogelj, Ross J. Salawitch, Bjørn H. Samset, Marit Sandstad, Alexey N. Shiklomanov, Ragnhild B. Skeie, Christopher J. Smith, Steve Smith, Katsumasa Tanaka, Junichi Tsutsui, and Zhiang Xie
Geosci. Model Dev., 13, 5175–5190, https://doi.org/10.5194/gmd-13-5175-2020, https://doi.org/10.5194/gmd-13-5175-2020, 2020
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Computational limits mean that we cannot run our most comprehensive climate models for all applications of interest. In such cases, reduced complexity models (RCMs) are used. Here, researchers working on 15 different models present the first systematic community effort to evaluate and compare RCMs: the Reduced Complexity Model Intercomparison Project (RCMIP). Our research ensures that users of RCMs can more easily evaluate the strengths, weaknesses and limitations of their tools.
Jaeyoung Song, Gretchen R. Miller, Anthony T. Cahill, Luiza Maria T. Aparecido, and Georgianne W. Moore
Geosci. Model Dev., 13, 5147–5173, https://doi.org/10.5194/gmd-13-5147-2020, https://doi.org/10.5194/gmd-13-5147-2020, 2020
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The performance of a land surface model (CLM4.5 and 5.0) was examined against a suite of measurements from a tropical montane rainforest in Costa Rica. Both versions failed to capture the effects of frequent rainfall events and mountainous terrain on temperature, leaf wetness, photosynthesis, and transpiration. While the new model version eliminated some errors, it still cannot precisely simulate a number of processes. This suggests that two key components of the model need modification.
Patricio Velasquez, Martina Messmer, and Christoph C. Raible
Geosci. Model Dev., 13, 5007–5027, https://doi.org/10.5194/gmd-13-5007-2020, https://doi.org/10.5194/gmd-13-5007-2020, 2020
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This work presents a new bias-correction method for precipitation that considers orographic characteristics, which can be used in studies where the latter strongly changes. The three-step correction method consists of a separation into orographic features, correction of low-intensity precipitation, and application of empirical quantile mapping. Seasonal bias induced by the global climate model is fully corrected. Rigorous cross-validations illustrate the method's applicability and robustness.
Johannes Horak, Marlis Hofer, Ethan Gutmann, Alexander Gohm, and Mathias W. Rotach
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2020-317, https://doi.org/10.5194/gmd-2020-317, 2020
Revised manuscript accepted for GMD
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The presented process based evaluation of the atmospheric model ICAR is conducted to derive recommendations to increase the likelihood of its results being correct for the right reasons. We conclude that a different diagnosis of the atmospheric background state is necessary, as well as a model top at an elevation of at least 10 km. Alternative boundary conditions at the top were not found effective in reducing this model top elevation. The results have wide implications for future ICAR studies.
Eric Larour, Lambert Caron, Mathieu Morlighem, Surendra Adhikari, Thomas Frederikse, Nicole-Jeanne Schlegel, Erik Ivins, Benjamin Hamlington, Robert Kopp, and Sophie Nowicki
Geosci. Model Dev., 13, 4925–4941, https://doi.org/10.5194/gmd-13-4925-2020, https://doi.org/10.5194/gmd-13-4925-2020, 2020
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ISSM-SLPS is a new projection system for future sea level that increases the resolution and accuracy of current projection systems and improves the way uncertainty is treated in such projections. This will pave the way for better inclusion of state-of-the-art results from existing intercomparison efforts carried out by the scientific community, such as GlacierMIP2 or ISMIP6, into sea-level projections.
Hiroshi Yamashita, Feijia Yin, Volker Grewe, Patrick Jöckel, Sigrun Matthes, Bastian Kern, Katrin Dahlmann, and Christine Frömming
Geosci. Model Dev., 13, 4869–4890, https://doi.org/10.5194/gmd-13-4869-2020, https://doi.org/10.5194/gmd-13-4869-2020, 2020
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This paper describes the updated submodel AirTraf 2.0 which simulates global air traffic in the ECHAM/MESSy Atmospheric Chemistry (EMAC) model. Nine aircraft routing options have been integrated, including contrail avoidance, minimum economic costs, and minimum climate impact. Example simulations reveal characteristics of different routing options on air traffic performances. The consistency of the AirTraf simulations is verified with literature data.
Landon A. Rieger, Jason N. S. Cole, John C. Fyfe, Stephen Po-Chedley, Philip J. Cameron-Smith, Paul J. Durack, Nathan P. Gillett, and Qi Tang
Geosci. Model Dev., 13, 4831–4843, https://doi.org/10.5194/gmd-13-4831-2020, https://doi.org/10.5194/gmd-13-4831-2020, 2020
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Recently, the stratospheric aerosol forcing dataset used as an input to the Coupled Model Intercomparison Project phase 6 was updated. This work explores the impact of those changes on the modelled historical climates in the CanESM5 and EAMv1 models. Temperature differences in the stratosphere shortly after the Pinatubo eruption are found to be significant, but surface temperatures and precipitation do not show a significant change.
Shaoqing Zhang, Haohuan Fu, Lixin Wu, Yuxuan Li, Hong Wang, Yunhui Zeng, Xiaohui Duan, Wubing Wan, Li Wang, Yuan Zhuang, Hongsong Meng, Kai Xu, Ping Xu, Lin Gan, Zhao Liu, Sihai Wu, Yuhu Chen, Haining Yu, Shupeng Shi, Lanning Wang, Shiming Xu, Wei Xue, Weiguo Liu, Qiang Guo, Jie Zhang, Guanghui Zhu, Yang Tu, Jim Edwards, Allison Baker, Jianlin Yong, Man Yuan, Yangyang Yu, Qiuying Zhang, Zedong Liu, Mingkui Li, Dongning Jia, Guangwen Yang, Zhiqiang Wei, Jingshan Pan, Ping Chang, Gokhan Danabasoglu, Stephen Yeager, Nan Rosenbloom, and Ying Guo
Geosci. Model Dev., 13, 4809–4829, https://doi.org/10.5194/gmd-13-4809-2020, https://doi.org/10.5194/gmd-13-4809-2020, 2020
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Science advancement and societal needs require Earth system modelling with higher resolutions that demand tremendous computing power. We successfully scale the 10 km ocean and 25 km atmosphere high-resolution Earth system model to a new leading-edge heterogeneous supercomputer using state-of-the-art optimizing methods, promising the solution of high spatial resolution and time-varying frequency. Corresponding technical breakthroughs are of significance in modelling and HPC design communities.
Gill M. Martin, Richard C. Levine, José M. Rodriguez, and Michael Vellinga
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2020-268, https://doi.org/10.5194/gmd-2020-268, 2020
Revised manuscript accepted for GMD
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Our study highlights a number of different techniques that can be employed to investigate the sources of model error. We demonstrate how this methodology can be used to identify the regions and model components responsible for the development of long-standing errors in the Asian Summer Monsoon. Once these are known, further work can be done to explore the local processes contributing to this behaviour and their sensitivity to changes in physical parameterizations and/or model resolution.
Tokuta Yokohata, Tsuguki Kinoshita, Gen Sakurai, Yadu Pokhrel, Akihiko Ito, Masashi Okada, Yusuke Satoh, Etsushi Kato, Tomoko Nitta, Shinichiro Fujimori, Farshid Felfelani, Yoshimitsu Masaki, Toshichika Iizumi, Motoki Nishimori, Naota Hanasaki, Kiyoshi Takahashi, Yoshiki Yamagata, and Seita Emori
Geosci. Model Dev., 13, 4713–4747, https://doi.org/10.5194/gmd-13-4713-2020, https://doi.org/10.5194/gmd-13-4713-2020, 2020
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The most significant feature of MIROC-INTEG-LAND is that the land surface model that describes the processes of the energy and water balances, human water management, and crop growth incorporates a land-use decision-making model based on economic activities. The future simulations indicate that changes in climate have significant impacts on crop yields, land use, and irrigation water demand.
Chia-Te Chien, Markus Pahlow, Markus Schartau, and Andreas Oschlies
Geosci. Model Dev., 13, 4691–4712, https://doi.org/10.5194/gmd-13-4691-2020, https://doi.org/10.5194/gmd-13-4691-2020, 2020
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We demonstrate sensitivities of tracers to parameters of a new optimality-based plankton–ecosystem model (OPEM) in the UVic-ESCM. We find that changes in phytoplankton subsistence nitrogen quota strongly impact the nitrogen inventory, nitrogen fixation, and elemental stoichiometry of ordinary phytoplankton and diazotrophs. We introduce a new likelihood-based metric for model calibration, and it shows the capability of constraining globally averaged oxygen, nitrate, and DIC concentrations.
Markus Pahlow, Chia-Te Chien, Lionel A. Arteaga, and Andreas Oschlies
Geosci. Model Dev., 13, 4663–4690, https://doi.org/10.5194/gmd-13-4663-2020, https://doi.org/10.5194/gmd-13-4663-2020, 2020
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The stoichiometry of marine biotic processes is important for the regulation of atmospheric CO2 and hence the global climate. We replace a simplistic, fixed-stoichiometry plankton module in an Earth system model with an optimal-regulation model with variable stoichiometry. Our model compares better to the observed carbon transfer from the surface to depth and surface nutrient distributions. This work could aid our ability to describe and project the role of marine ecosystems in the Earth system.
Yong Wang, Guang J. Zhang, Shaocheng Xie, Wuyin Lin, George C. Craig, Qi Tang, and Hsi-Yen Ma
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2020-249, https://doi.org/10.5194/gmd-2020-249, 2020
Revised manuscript accepted for GMD
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A stochastic deep convection parameterization is implemented into the U.S. Department of Energy Energy Exascale Earth System Model Atmosphere Model version 1 (EAMv1). Compared to the default model, the well-known problem of
too much light rain and too little heavy rainis largely alleviated over the tropics with the stochastic scheme. Results from this study provide important insights into the model performance of EAMv1 when stochasticity is included in deep convective parameterization.
Peter A. Bogenschutz, Shuaiqi Tang, Peter M. Caldwell, Shaocheng Xie, Wuyin Lin, and Yao-Sheng Chen
Geosci. Model Dev., 13, 4443–4458, https://doi.org/10.5194/gmd-13-4443-2020, https://doi.org/10.5194/gmd-13-4443-2020, 2020
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This paper documents a tool that has been developed that can be used to accelerate the development and understanding of climate models. This version of the model, known as a the single-column model, is much faster to run than the full climate model, and we demonstrate that this tool can be used to quickly exploit model biases that arise due to physical processes. We show examples of how this single-column model can directly benefit the field.
Ying Liu, Rodrigo Caballero, and Joy Merwin Monteiro
Geosci. Model Dev., 13, 4399–4412, https://doi.org/10.5194/gmd-13-4399-2020, https://doi.org/10.5194/gmd-13-4399-2020, 2020
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The calculation of atmospheric radiative transfer is the most computationally expensive part of climate models. Reducing this computational burden could potentially improve our ability to simulate the earth's climate at finer scales. We propose using a statistical model – a deep neural network – to compute approximate radiative transfer in the earth's atmosphere. We demonstrate a significant reduction in computational burden as compared to a traditional scheme, especially when using GPUs.
Lars Nerger, Qi Tang, and Longjiang Mu
Geosci. Model Dev., 13, 4305–4321, https://doi.org/10.5194/gmd-13-4305-2020, https://doi.org/10.5194/gmd-13-4305-2020, 2020
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Data assimilation combines observations with numerical models to get an improved estimate of the model state. This work discusses the technical aspects of how a coupled model that simulates the ocean and the atmosphere can be augmented by data assimilation functionality provided in generic form by the open-source software PDAF (Parallel Data Assimilation Framework). A very efficient program is obtained that can be executed on high-performance computers.
Christof G. Beer, Johannes Hendricks, Mattia Righi, Bernd Heinold, Ina Tegen, Silke Groß, Daniel Sauer, Adrian Walser, and Bernadett Weinzierl
Geosci. Model Dev., 13, 4287–4303, https://doi.org/10.5194/gmd-13-4287-2020, https://doi.org/10.5194/gmd-13-4287-2020, 2020
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Mineral dust aerosol plays an important role in the climate system. Previously, dust emissions have often been represented in global models by prescribed monthly-mean emission fields representative of a specific year. We now apply an online calculation of wind-driven dust emissions. This results in an improved agreement with observations, due to a better representation of the highly variable dust emissions. Increasing the model resolution led to an additional performance gain.
Nadine Mengis, David P. Keller, Andrew H. MacDougall, Michael Eby, Nesha Wright, Katrin J. Meissner, Andreas Oschlies, Andreas Schmittner, Alexander J. MacIsaac, H. Damon Matthews, and Kirsten Zickfeld
Geosci. Model Dev., 13, 4183–4204, https://doi.org/10.5194/gmd-13-4183-2020, https://doi.org/10.5194/gmd-13-4183-2020, 2020
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In this paper, we evaluate the newest version of the University of Victoria Earth System Climate Model (UVic ESCM 2.10). Combining recent model developments as a joint effort, this version is to be used in the next phase of model intercomparison and climate change studies. The UVic ESCM 2.10 is capable of reproducing changes in historical temperature and carbon fluxes well. Additionally, the model is able to reproduce the three-dimensional distribution of many ocean tracers.
Axel Lauer, Veronika Eyring, Omar Bellprat, Lisa Bock, Bettina K. Gier, Alasdair Hunter, Ruth Lorenz, Núria Pérez-Zanón, Mattia Righi, Manuel Schlund, Daniel Senftleben, Katja Weigel, and Sabrina Zechlau
Geosci. Model Dev., 13, 4205–4228, https://doi.org/10.5194/gmd-13-4205-2020, https://doi.org/10.5194/gmd-13-4205-2020, 2020
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The Earth System Model Evaluation Tool is a community software tool designed for evaluation and analysis of climate models. New features of version 2.0 include analysis scripts for important large-scale features in climate models, diagnostics for extreme events, regional model and impact evaluation. In this paper, newly implemented climate metrics, emergent constraints for climate-relevant feedbacks and diagnostics for future model projections are described and illustrated with examples.
Brecht Martens, Dominik L. Schumacher, Hendrik Wouters, Joaquín Muñoz-Sabater, Niko E. C. Verhoest, and Diego G. Miralles
Geosci. Model Dev., 13, 4159–4181, https://doi.org/10.5194/gmd-13-4159-2020, https://doi.org/10.5194/gmd-13-4159-2020, 2020
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Climate reanalyses are widely used in different fields and an in-depth evaluation of the different variables provided by reanalyses is a necessary means to provide feedback on the quality to their users and the operational centres producing these data sets. In this study, we show the improvements of ECMWF's latest climate reanalysis (ERA5) upon its predecessor (ERA-Interim) in partitioning the available energy at the land surface.
Arthur P. K. Argles, Jonathan R. Moore, Chris Huntingford, Andrew J. Wiltshire, Anna B. Harper, Chris D. Jones, and Peter M. Cox
Geosci. Model Dev., 13, 4067–4089, https://doi.org/10.5194/gmd-13-4067-2020, https://doi.org/10.5194/gmd-13-4067-2020, 2020
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The Robust Ecosystem Demography (RED) model simulates cohorts of vegetation through mass classes. RED establishes a framework for representing demographic changes through competition, growth, and mortality across the size distribution of a forest. The steady state of the model can be solved analytically, enabling initialization. When driven by mean growth rates from a land-surface model, RED is able to fit the observed global vegetation map, giving a map of implicit mortality rates.
James A. Franke, Christoph Müller, Joshua Elliott, Alex C. Ruane, Jonas Jägermeyr, Abigail Snyder, Marie Dury, Pete D. Falloon, Christian Folberth, Louis François, Tobias Hank, R. Cesar Izaurralde, Ingrid Jacquemin, Curtis Jones, Michelle Li, Wenfeng Liu, Stefan Olin, Meridel Phillips, Thomas A. M. Pugh, Ashwan Reddy, Karina Williams, Ziwei Wang, Florian Zabel, and Elisabeth J. Moyer
Geosci. Model Dev., 13, 3995–4018, https://doi.org/10.5194/gmd-13-3995-2020, https://doi.org/10.5194/gmd-13-3995-2020, 2020
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Improving our understanding of the impacts of climate change on crop yields will be critical for global food security in the next century. The models often used to study the how climate change may impact agriculture are complex and costly to run. In this work, we describe a set of global crop model emulators (simplified models) developed under the Agricultural Model Intercomparison Project. Crop model emulators make agricultural simulations more accessible to policy or decision makers.
Miguel Nogueira, Clément Albergel, Souhail Boussetta, Frederico Johannsen, Isabel F. Trigo, Sofia L. Ermida, João P. A. Martins, and Emanuel Dutra
Geosci. Model Dev., 13, 3975–3993, https://doi.org/10.5194/gmd-13-3975-2020, https://doi.org/10.5194/gmd-13-3975-2020, 2020
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We used earth observations to evaluate and improve the representation of land surface temperature (LST) and vegetation coverage over Iberia in CHTESSEL and SURFEX land surface models. We demonstrate the added value of updating the vegetation types and fractions together with the representation of vegetation coverage seasonality. Results show a large reduction in daily maximum LST systematic error during warm months, with neutral impacts in other seasons.
Qiong Zhang, Qiang Li, Qiang Zhang, Ellen Berntell, Josefine Axelsson, Jie Chen, Zixuan Han, Wesley de Nooijer, Zhengyao Lu, Klaus Wyser, and Shuting Yang
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2020-208, https://doi.org/10.5194/gmd-2020-208, 2020
Revised manuscript accepted for GMD
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Paleoclimate modelling has long been regarded as a strong out-of-sample test-bed of the climate models that are used for the projection of future climate changes. Here, we document the model experiments setup for the three past warm periods with EC-Earth3-LR and present the results on the large-scale features from the completed production simulations. The simulations demonstrate the good performance of the model to capture the climate response under different climate forcings.
Wei-Liang Lee, Yi-Chi Wang, Chein-Jung Shiu, I-chun Tsai, Chia-Ying Tu, Yung-Yao Lan, Jen-Ping Chen, Hua-Lu Pan, and Huang-Hsiung Hsu
Geosci. Model Dev., 13, 3887–3904, https://doi.org/10.5194/gmd-13-3887-2020, https://doi.org/10.5194/gmd-13-3887-2020, 2020
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The Taiwan Earth System Model (TaiESM) is a new climate model developed in Taiwan. It includes several new features, and therefore it can better simulate the occurrence of convective rainfall, solar energy received by mountainous surfaces, and more detail chemical processes in aerosols. TaiESM can capture the trend of global warming after 1950 well, and its overall performance in most meteorological quantities is better than the average of global models used in IPCC AR5.
Cited articles
Abdul-Razzak, H. and Ghan, S. J.: A parameterization of aerosol activation: 2. Multiple aerosol types, J. Geophys. Res., 105, 6837–6844, https://doi.org/10.1029/1999jd901161, 2000.
Abdul-Razzak, H., Ghan, S. J., and Rivera-Carpio, C.: A parameterization of aerosol activation. Part I: Single aerosol type, J. Geophys. Res., 103, 6123–6131, https://doi.org/10.1029/97jd03735, 1998.
Ackermann, I. J., Hass, H., Memmesheimer, M., Ebel, A., Binkowski, F. S., and Shankar U.: Modal aerosol dynamics model for Europe: Development and first applications, Atmos. Environ., 32, 2981–2999, https://doi.org/10.1016/s1352-2310(98)00006-5, 1998.
Albrecht, B. A.: Aerosols, cloud microphysics and fractional cloudiness, Science, 245, 1227–1230, https://doi.org/10.1126/science.245.4923.1227, 1989.
Al-Saadi, J., Carmichael, G., Crawford, J., Emmons, L., Song, C. K., Chang, L. S., Lee, G., Kim, J., and Park, R.: NASA contributions to KORUS-AQ: An international cooperative air quality field study in Korea, NASA White Pap., Virginia, USA, available at: https://espo.nasa.gov/sites/default/files/documents/White%20paper%20outlining%20NASA%e2%80%99s%20contribution%20to%20KORUS-AQ_0.pdf
(last access: 14 January 2021), 2016.
Andreae, M. O. and Rosenfeld, D.: Aerosol-cloud-precipitation interactions. Part 1. The nature and sources of cloud-active aerosols, Earth-Sci. Rev., 89, 13–41, 2008.
Aneja, V. P.: Natural sulfur emissions into the atmosphere. J. Air Waste Manag. Assoc., 40, 469–476, https://doi.org/10.1080/10473289.1990.10466701, 1990.
Baró, R., Jiménez-Guerrero, P., Balzarini, A., Curci, G., Forkel, R., Grell, G., Hirtl, M., Honzak, L., Langer, M., Pérez, J. L., Pirovano, G., San José, R., Tuccella, P., Werhahn, J., and Žabkar, R.: Sensitivity analysis of the microphysics scheme in WRF-Chem contributions to AQMEII phase 2, Atmos. Environ., 115, 620–629, https://doi.org/10.1016/j.atmosenv.2015.01.047, 2015.
Bessagnet, B., Pirovano, G., Mircea, M., Cuvelier, C., Aulinger, A., Calori, G., Ciarelli, G., Manders, A., Stern, R., Tsyro, S., García Vivanco, M., Thunis, P., Pay, M.-T., Colette, A., Couvidat, F., Meleux, F., Rouïl, L., Ung, A., Aksoyoglu, S., Baldasano, J. M., Bieser, J., Briganti, G., Cappelletti, A., D'Isidoro, M., Finardi, S., Kranenburg, R., Silibello, C., Carnevale, C., Aas, W., Dupont, J.-C., Fagerli, H., Gonzalez, L., Menut, L., Prévôt, A. S. H., Roberts, P., and White, L.: Presentation of the EURODELTA III intercomparison exercise – evaluation of the chemistry transport models' performance on criteria pollutants and joint analysis with meteorology, Atmos. Chem. Phys., 16, 12667–12701, https://doi.org/10.5194/acp-16-12667-2016, 2016.
Bishop, G. A. and Stedman, D. H.: Reactive Nitrogen Species Emission Trends in Three Light-/Medium-Duty United States Fleets, Environ. Sci. Technol., 49, 11234–11240, https://doi.org/10.1021/acs.est.5b02392, 2015.
Boucher, O. and Anderson, T. L.: General circulation model assessment of the sensitivity of direct climate forcing by anthropogenic sulfate aerosols to aerosol size and chemistry, J. Geophys. Res., 100, 26117–26134, https://doi.org/10.1029/95JD02531, 1995.
Boucher, O., Randall, D., Artaxo, P., Bretherton, C., Feingold, G., Forster, P., Kerminen, V.-M., Kondo, Y., Liao, H., Lohmann, U., Rasch, P., Satheesh, S. K., Sherwood, S., Stevens, B., and Zhang, X. Y.: Clouds and Aerosols, in: Climate Change 2013: The Physical Science Basis. Contribution of Working Group I to the Fifth Assessment Report of the Intergovernmental Panel on Climate Change, edited by: Stocker, T. F., Qin, D., Plattner, G.-K., Tignor, M., Allen, S. K., Boschung, J., Nauels, A., Xia, Y., Bex, V., and Midgley, P. M., Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA, 2013.
Carslaw, K. S., Lee, L. A., Reddington, C. L., Pringle, K. J., Rap, A., Forster, P. M., Mann, G. W., Spracklen, D. V., Woodhouse, M. T., Regayre, L. A., and Pierce, J. R.: Large contribution of natural aerosols to uncertainty in indirect forcing, Nature, 503, 67–71, https://doi.org/10.1038/nature12674, 2013.
Ceburnis, D., Rinaldi, M., Ovadnevaite, J., Martucci, G., Giulianelli, L., and O'Dowd, C. D.: Marine submicron aerosol gradients, sources and sinks, Atmos. Chem. Phys., 16, 12425–12439, https://doi.org/10.5194/acp-16-12425-2016, 2016.
Chang, D., Lelieveld, J., Tost, H., Steil, B., Pozzer, A., and Yoon, J.: Aerosol physicochemical effects on CCN activation simulated with the chemistry-climate model EMAC, Atmos. Environ., 162, 127–140, https://doi.org/10.1016/j.atmosenv.2017.03.036, 2017.
Chang, J. S., Binkowski, F. S., Seaman, N. L., McHenry, J. N., Samson, P. J., Stockwell, W. R., Walcek, C. J., Madronich, S., Middleton, P. B., Pleim, J. E., and Lansford, H. H.: The regional acid deposition model and engineering model, State-of-Science/Technology, Report 4, National Acid Precipitation Assessment Program, Washington, D.C., 1989.
Chapman, E. G., Gustafson Jr., W. I., Easter, R. C., Barnard, J. C., Ghan, S. J., Pekour, M. S., and Fast, J. D.: Coupling aerosol-cloud-radiative processes in the WRF-Chem model: Investigating the radiative impact of elevated point sources, Atmos. Chem. Phys., 9, 945–964, https://doi.org/10.5194/acp-9-945-2009, 2009.
Charlson, R. J. and Wigley, T. M. L.: Sulfate Aerosol and Climatic Change, Sci. Am., 270, 48–57, https://doi.org/10.1038/scientificamerican0294-48, 1994.
Clegg, S. L., Brimblecombe, P., and Wexler, A. S.: Thermodynamic model of the system at 298.15 K, J. Phys. Chem. A., 102, 2155–2171, https://doi.org/10.1021/jp973043j, 1998.
Dibb, J. E., Talbot, R. W., Scheuer, E. M., Seid, G., Avery, M. A., and Singh, H. B.: Aerosol chemical composition in Asian continental outflow during the TRACE-P campaign: Comparison with PEM-West B, J. Geophys. Res., 108, 8815, https://doi.org/10.1029/2002JD003111, 2003.
Dusek, U., Frank, G. P., Hildebrandt, L., Curtius, J., Schneider, J., Walter, S., Chand, D., Drewnick, F., Hings, S., Jung, D., Borrmann, S., and Andreae, M. O.: Size matters more than chemistry for cloud nucleating ability of aerosol particles, Science, 312, 1375–1378, https://doi.org/10.1126/science.1125261, 2006.
Elleman, R. A. and Covert, D. S.: Aerosol size distribution modeling with the Community Multiscale Air Quality modeling system in the Pacific Northwest: 2. Parameterizations for ternary nucleation and nucleation mode processes, J. Geophys. Res., 114, D11207, https://doi.org/10.1029/2009JD012187, 2009.
Fast, J. D., Gustafson, W. I. Jr, Easter, R. C., Zaveri, R. A., Barnard, J. C., Chapman, E. G., and Grell, G. A.: Evolution of ozone, particulates, and aerosol direct forcing in an urban area using a new fully coupled meteorology, chemistry, and aerosol model, J. Geophys. Res., 111, D21305, https://doi.org/10.1029/2005jd006721, 2006.
Fisher, J. A., Jacob, D. J., Wang, Q., Bahreini, R., Carouge, C. C., Cubison, M. J., Dibb, J. E., Diehl, T., Jimenez, J. L., Leibensperger, E. M., Lu, Z., Meinders, M. B. J., Pye, H. O. T., Quinn, P. K., Sharma, S., Streets, D. G., van Donkelaar, A., and Yantosca, R. M.: Sources, distribution, and acidity of sulfate–ammonium aerosol in the Arctic in winter–spring, Atmos. Environ., 45, 7301–7318, https://doi.org/10.1016/j.atmosenv.2011.08.030, 2011.
Fountoukis, C. and Nenes, A.: Continued development of a cloud droplet formation parameterization for global climate models, J. Geophys. Res., 110, D11212, https://doi.org/10.1029/2004JD005591, 2005.
Fujita, S.-I., Takahashi, A., Weng, J.-H., Huang, L.-F., Kim, H.-K., Li, C.-K., Huang, F. T. C., and Jeng, F.-T.: Precipitation chemistry in East Asia, Atmos. Environ., 34, 525–537, https://doi.org/10.1016/S1352-2310(99)00261-7, 2000.
Gasteiger, J. and Wiegner, M.: MOPSMAP v1.0: a versatile tool for the modeling of aerosol optical properties, Geosci. Model Dev., 11, 2739–2762, https://doi.org/10.5194/gmd-11-2739-2018, 2018.
Georgiou, G. K., Christoudias, T., Proestos, Y., Kushta, J., Hadjinicolaou, P., and Lelieveld, J.: Air quality modelling in the summer over the eastern Mediterranean using WRF-Chem: chemistry and aerosol mechanism intercomparison, Atmos. Chem. Phys., 18, 1555–1571, https://doi.org/10.5194/acp-18-1555-2018, 2018.
Ghan, S. J., Abdul-Razzak, H., Nenes, A., Ming, Y., Liu, X., Ovchinnikov, M., Shipway, B., Meskhidze, N., Xu, J., and Shi, X.: Droplet nucleation: Physically-based parameterizations and comparative evaluation, J. Adv. Model. Earth Syst., 3, M10001, https://doi.org/10.1029/2011MS000074, 2011.
Good, N., Topping, D. O., Allan, J. D., Flynn, M., Fuentes, E., Irwin, M., Williams, P. I., Coe, H., and McFiggans, G.: Consistency between parameterisations of aerosol hygroscopicity and CCN activity during the RHaMBLe discovery cruise, Atmos. Chem. Phys., 10, 3189–3203, https://doi.org/10.5194/acp-10-3189-2010, 2010.
Goren, T. and Rosenfeld, D.: Decomposing aerosol cloud radiative effects into cloud cover, liquid water path and Twomey components in marine stratocumulus, Atmos. Res., 138, 378–393, https://doi.org/10.1016/j.atmosres.2013.12.008, 2014.
Grell, G. A. and Baklanov, A.: Integrated modeling for forecasting weather and air quality: A call for fully coupled approaches, Atmos. Environ., 45, 6845–6851, https://doi.org/10.1016/j.atmosenv.2011.01.017, 2011.
Grell, G. A., Knoche, R., Schmitz, R., McKeen, S. A., Frost, G., Skamarock, W. C., and Eder, B.: Fully-coupled “online” chemistry within the WRF model, Atmos. Environ., 39, 6957–6976, https://doi.org/10.1016/j.atmosenv.2005.04.027, 2005.
Guenther, A., Karl, T., Harley, P., Wiedinmyer, C., Palmer, P. I., and Geron, C.: Estimates of global terrestrial isoprene emissions using MEGAN (Model of Emissions of Gases and Aerosols from Nature), Atmos. Chem. Phys., 6, 3181–3210, https://doi.org/10.5194/acp-6-3181-2006, 2006.
Gustafson, W. I., Chapman, E. G., Ghan, S. J., Easter, R. C., and Fast, J. D.: Impact on modeled cloud characteristics due to simplified treatment of uniform cloud condensation nuclei during NEAQS 2004, Geophys. Res. Lett., 34, L19809, https://doi.org/10.1029/2007GL030021, 2007.
Hartmann, D. L.: Global physical climatology, 2nd edn., Elsevier Science, Amsterdam, the Netherlands, 485 pp., 2016.
Hong, S.-Y., Noh, Y., and Dudhia, J.: A new vertical diffusion package with an explicit treatment of entrainment processes, Mon. Weather Rev., 134, 2318–2341, https://doi.org/10.1175/MWR3199.1, 2006.
Iacono, M. J., Delamere, J. S., Mlawer, E. J., Shephard, M. W., Clough, S. A., and Collins, W. D.: Radiative forcing by long-lived greenhouse gases: Calculations with the AER radiative transfer models, J. Geophys. Res., 113, D13103, https://doi.org/10.1029/2008JD009944, 2008.
Im, U., Bianconi, R., Solazzo, E., Kioutsioukis, I., Badia, A., Balzarini, A., Baro, R., Bellasio, R., Brunner, D., Chemel, C., Curci, G., Denier van der Gon, H., Flemming, J., Forkel, R., Giordano, L., Jimenez-Guerrero, P., Hirtl, M., Hodzic, A., Honzak, L., Jorba, O., Knote, C., Makar, P. A., Manders-Groot, A., Neal, L., Perez, J. L., Pirovano, G., Pouliot, G., San Jose, R., Savage, N., Schroder, W., Sokhi, R. S., Syrakov, D., Torian, A., Tuccella, P., Wang, K., Werhahn, J., Wolke, R., Zabkar, R., Zhang, Y., Zhang, J., Hogrefe, C., and Galmarini, S.: Evaluation of operational online-coupled regional air quality models over Europe and North America in the context of AQMEII phase 2. Part II: Particulate Matter, Atmos. Environ., 115, 421–441, https://doi.org/10.1016/j.atmosenv.2014.08.072, 2015.
Janssens-Maenhout, G., Crippa, M., Guizzardi, D., Dentener, F., Muntean, M., Pouliot, G., Keating, T., Zhang, Q., Kurokawa, J., Wankmüller, R., Denier van der Gon, H., Kuenen, J. J. P., Klimont, Z., Frost, G., Darras, S., Koffi, B., and Li, M.: HTAP_v2.2: a mosaic of regional and global emission grid maps for 2008 and 2010 to study hemispheric transport of air pollution, Atmos. Chem. Phys., 15, 11411–11432, https://doi.org/10.5194/acp-15-11411-2015, 2015.
Jardine, K., Yañez-Serrano, A. M., Williams, J., Kunert, N., Jardine, A., Taylor, T., Abrell, L., Artaxo, P., Guenther, A., Hewitt, C. N., House, E., Florentino, A. P., Manzi, A., Higuchi, N., Kesselmeier, J., Behrendt, T., Veres, P. R., Derstroff, B., Fuentes, J. D., Martin, S. T., and Andreae, M. O.: Dimethylsulfide in the Amazon rainforest, Global Biogeochem. Cycles, 29, 19–32, https://doi.org/10.1002/2014GB004969, 2015.
Kang, Y., Liu, M., Song, Y., Huang, X., Yao, H., Cai, X., Zhang, H., Kang, L., Liu, X., Yan, X., He, H., Zhang, Q., Shao, M., and Zhu, T.: High-resolution ammonia emissions inventories in China from 1980 to 2012, Atmos. Chem. Phys., 16, 2043–2058, https://doi.org/10.5194/acp-16-2043-2016, 2016.
Kazil, J. and Lovejoy, E. R.: A semi-analytical method for calculating rates of new sulfate aerosol formation from the gas phase, Atmos. Chem. Phys., 7, 3447–3459, https://doi.org/10.5194/acp-7-3447-2007, 2007.
Khvorostyanov, V. I. and Curry, J. A.: Parameterization of cloud drop activation based on analytical asymptotic solutions to the supersaturation equation, J. Atmos. Sci., 66, 1905–1925, https://doi.org/10.1175/2009JAS2811.1, 2009.
Kiehl, J. T., Schneider, T. L., Rasch, P. J., Barth, M. C., and Wong, J.: Radiative forcing due to sulfate aerosols from simulations with the National Center for Atmospheric Research Community Climate Model, Version 3, J. Geophys. Res., 105, 1441–1457, https://doi.org/10.1029/1999JD900495, 2000.
Kim, A.-H.: kimah3/optimization_so4: Source code for Optimization of Sulfate Aerosol Hygroscopicity Parameter in WRF-Chem v.3.8.1 (Version 0.1.0), Zenodo, https://doi.org/10.5281/zenodo.3899838, 2020.
Köhler, H.: The nucleus in and the growth of hygroscopic droplets, Trans. Farad. Soc., 32, 1152–1161, https://doi.org/10.1039/tf9363201152, 1936.
Korhonen, H., Carslaw, K. S., Spracklen, D. V., Mann, G. W., and Woodhouse, M. T.: Influence of oceanic dimethyl sulfide emissions on cloud condensation nuclei concentrations and seasonality over the remote Southern Hemisphere oceans: A global model study, J. Geophys. Res., 113, D15204, https://doi.org/10.1029/2007JD009718, 2008.
Kristjánsson, J. E.: Studies of the aerosol indirect effect from sulfate and black carbon aerosols, J. Geophys. Res., 107, D154246, https://doi.org/10.1029/2001JD000887, 2002.
Kukkonen, J., Olsson, T., Schultz, D. M., Baklanov, A., Klein, T., Miranda, A. I., Monteiro, A., Hirtl, M., Tarvainen, V., Boy, M., Peuch, V.-H., Poupkou, A., Kioutsioukis, I., Finardi, S., Sofiev, M., Sokhi, R., Lehtinen, K. E. J., Karatzas, K., San José, R., Astitha, M., Kallos, G., Schaap, M., Reimer, E., Jakobs, H., and Eben, K.: A review of operational, regional-scale, chemical weather forecasting models in Europe, Atmos. Chem. Phys., 12, 1–87, https://doi.org/10.5194/acp-12-1-2012, 2012.
Kulmala, M., Laaksonen, A., and Pirjola, L.: Parameterizations for sulphric acid/water nucleation rates, J. Geophys. Res., 103, 8301–8308, https://doi.org/10.1029/97jd03718, 1998.
Kulmala, M., Korhonen, P., Napari, I., Karlsson, A., Berresheim, H., and O'Dowd, C. D.: Aerosol formation during PARFORCE: Ternary nucleation of H2SO4, NH3, and H2O, J. Geophys. Res., 107, 8111, https://doi.org/10.1029/2001JD000900, 2002.
Kumar, A., Luo, J., and Bennett, G.: Statistical Evaluation of Lower Flammability Distance (LFD) using Four Hazardous Release Models, Process. Saf. Prog., 12, 11, https://doi.org/10.1002/prs.680120103, 1993.
Kurokawa, J., Ohara, T., Morikawa, T., Hanayama, S., Janssens-Maenhout, G., Fukui, T., Kawashima, K., and Akimoto, H.: Emissions of air pollutants and greenhouse gases over Asian regions during 2000–2008: Regional Emission inventory in ASia (REAS) version 2, Atmos. Chem. Phys., 13, 11019–11058, https://doi.org/10.5194/acp-13-11019-2013, 2013.
Lewis, E. R.: An examination of Köhler theory resulting in an accurate expression for the equilibrium radius ratio of a hygroscopic aerosol particle valid up to and including relative humidity 100 %, J. Geophys. Res., 113, D03205, https://doi.org/10.1029/2007JD008590, 2008.
Liu, J., Mauzerall, D. L., and Horowitz, L. W.: Source-receptor relationships between East Asian sulfur dioxide emissions and Northern Hemisphere sulfate concentrations, Atmos. Chem. Phys., 8, 3721–3733, https://doi.org/10.5194/acp-8-3721-2008, 2008.
Liu, L., , Zhang, X., Xu, W., Liu, X., Lu, X., Wang, S., Zhang, W., and Zhao, L.: Ground Ammonia Concentrations over China Derived from Satellite and Atmospheric Transport Modeling, Remote Sens., 9, 467, https://doi.org/10.3390/rs9050467, 2017.
Liu, T., Wang, X., Deng, W., Zhang, Y., Chu, B., Ding, X., Hu, Q., He, H., and Hao, J.: Role of ammonia in forming secondary aerosols from gasoline vehicle exhaust, Sci. China Chem., 58, 1377–1384, https://doi.org/10.1007/s11426-015-5414-x, 2015.
Mann, G. W., Carslaw, K. S., Spracklen, D. V., Ridley, D. A., Manktelow, P. T., Chipperfield, M. P., Pickering, S. J., and Johnson, C. E.: Description and evaluation of GLOMAP-mode: a modal global aerosol microphysics model for the UKCA composition-climate model, Geosci. Model Dev., 3, 519–551, https://doi.org/10.5194/gmd-3-519-2010, 2010.
Moore, R. H., Bahreini, R., Brock, C. A., Froyd, K. D., Cozic, J., Holloway, J. S., Middlebrook, A. M., Murphy, D. M., and Nenes, A.: Hygroscopicity and composition of Alaskan Arctic CCN during April 2008, Atmos. Chem. Phys., 11, 11807–11825, https://doi.org/10.5194/acp-11-11807-2011, 2011.
Moore, R. H., Cerully, K., Bahreini, R., Brock, C. A., Middlebrook, A. M., and Nenes, A.: Hygroscopicity and composition of California CCN during summer 2010, J. Geophys. Res., 117, D00V12, https://doi.org/10.1029/2011JD017352, 2012.
Morrison, H., Thompson, G., and Tatarskii, V.: Impact of Cloud Microphysics on the Development of Trailing Stratiform Precipitation in a Simulated Squall Line: Comparison of One- and Two-Moment Schemes, Mon. Weather Rev., 137, 991–1007, https://doi.org/10.1175/2008MWR2556.1, 2009.
Myhre, G., Shindell, D., Bréon, F.-M., Collins, W., Fuglestvedt, J., Huang, J., Koch, D., Lamarque, J.-F., Lee, D., Mendoza, B., Nakajima, T., Robock, A., Stephens, G., Takemura, T., and Zhang, H.: Anthropogenic and natural radiative forcing, in: Clim. Chang. 2013 Phys. Sci. basis. Contrib. Work. Gr. I to fifth Assess. Rep. Intergov. panel Clim. Chang., 659–740, Cambridge University Press, Cambridge, UK and New York, NY, USA, 2013.
Napari, I., Noppel, M., Vehkamaki, H., and Kulmala, M.: Parametrization of ternary nucleation rates for vapors, J. Geophys. Res., 107, 4381, https://doi.org/10.1029/2002JD002132, 2002.
Nenes, A., Pandis, S. N., and Pilinis, C.: ISORROPIA: A new thermodynamic equilibrium model for multiphase multicomponent aerosols, Aquat. Geochem., 4, 123–152, https://doi.org/10.1023/A:1009604003981, 1998.
Nenes, A., Charlson, R. J., Facchini, M. C., Kulmala, M., Laaksonen, A., and Seinfeld, J. H.: Can chemical effects on cloud droplet number rival the first indirect effect?, Geophys. Res. Lett., 29, 1848, https://doi.org/10.1029/2002GL015295, 2002.
Pan, Z., Gong, W., Mao, F., Li, J., Wang, W., Li, C., and Min, Q.: Macrophysical and optical properties of clouds over East Asia measured by CALIPSO, J. Geophys. Res.-Atmos., 120, 11653–11668, https://doi.org/10.1002/2015JD023735, 2015.
Park, M., Yum, S. S., Kim, N., Anderson, B. E., Beyersdorf, A., and Thornhill, K. L.: On the submicron aerosol distributions and CCN activity in and around the Korean Peninsula measured onboard the NASA DC-8 research aircraft during the KORUS-AQ field campaign, Atmos. Res., 243, 105004, https://doi.org/10.1016/j.atmosres.2020.105004, 2020.
Paulot, F., Jacob, D. J., Pinder, R. W., Bash, J. O., Travis, K., and Henze, D. K.: Ammonia emissions in the United States, European Union, and China derived by high-resolution inversion of ammonium wet deposition data: Interpretation with a new agricultural emissions inventory (MASAGE_NH3), J. Geophys. Res.-Atmos., 119, 4343–4364, https://doi.org/10.1002/2013jd021130, 2014.
Paulot, F., Jacob, D. J., Johnson, M. T., Bell, T. G., Baker, A. R., Keene, W. C., Lima, I. D., Doney, S. C., and Stock, C. A.: Global oceanic emission of ammonia: Constraints from seawater and atmospheric observations, Global Biogeochem. Cycles, 29, 1165–1178, https://doi.org/10.1002/2015GB005106, 2015.
Peckham, S., Grell, G. A., McKeen, S. A., Barth, M., Pfister, G., Wiedinmyer, C., Fast, J. D., Gustafson, W. I., Zaveri, R., Easter, R. C., Barnard, J., Chapman, E., Hewson, M., Schmitz, R., Salzmann, M., and Freitas, S.: WRF-Chem Version 3.3 User's Guide, NOAA Technical Memo., Washington D.C., USA, 98 pp., 2011.
Petters, M. D. and Kreidenweis, S. M.: A single parameter representation of hygroscopic growth and cloud condensation nucleus activity, Atmos. Chem. Phys., 7, 1961–1971, https://doi.org/10.5194/acp-7-1961-2007, 2007.
Pringle, K. J., Tost, H., Pozzer, A., Pöschl, U., and Lelieveld, J.: Global distribution of the effective aerosol hygroscopicity parameter for CCN activation, Atmos. Chem. Phys., 10, 5241–5255, https://doi.org/10.5194/acp-10-5241-2010, 2010.
Qiu, Y., Zhao, C., Guo, J., and Li, J.: 8-Year ground-based observational analysis about the seasonal variation of the aerosol-cloud droplet effective radius relationship at SGP site, Atmos. Environ., 164, 139–146, https://doi.org/10.1016/j.atmosenv.2017.06.002, 2017.
Qu, Y., An, J., He, Y., and Zheng, J.: An overview of emissions of SO2 and NOx and the long-range transport of oxidized sulfur and nitrogen pollutants in East Asia, J. Env. Sci., 44, 13–25, https://doi.org/10.1016/j.jes.2015.08.028, 2016.
Raymond, T. M. and Pandis, S. N.: Formation of cloud droplets by multicomponent organic particles, J. Geophys. Res., 108, 4469, https://doi.org/10.1029/2003JD003503, 2003.
Saha, S., Moorthi, S., Wu, X., Wang, J., Nadiga, S., Tripp, P., Behringer, D., Hou, Y., Chuang, H., Iredell, M., Ek, M., Meng, J., Yang, R., Mendez, M. P., van den Dool, H., Zhang, Q., Wang, W., Chen, M., and Becker, E.: The NCEP Climate Forecast System Version 2, J. Clim., 27, 2185–2208, https://doi.org/10.1175/JCLI-D-12-00823.1, 2014.
Schell, B., Ackermann, I. J., Hass, H., Binkowski, F. S., and Ebel, A.: Modeling the formation of secondary organic aerosol within a comprehensive air quality model system, J. Geophys. Res., 106, 28275–28293, https://doi.org/10.1029/2001jd000384, 2001.
Seinfeld, J. H. and Pandis, S. N.: Atmospheric Chemistry and Physics, John Wiley and Sons, New Jersey, USA, 1203 pp., 2006.
Sengupta, M., Clothiaux, E. E., Ackerman, T. P., Kato, S., and Min, Q.: Importance of Accurate Liquid Water Path for Estimation of Solar Radiation in Warm Boundary Layer Clouds: An Observational Study, J. Clim., 16, 2997–3009, https://doi.org/10.1175/1520-0442(2003)016<2997:IOALWP>2.0.CO;2, 2003.
Shiraiwa, M., Li, Y., Tsimpidi, A. P., Karydis, V. A., Berkemeier, T., Pandis, S. N., Lelieveld, J., Koop, T., and Pöschl, U.: Global distribution of particle phase state in atmospheric secondary organic aerosols, Nat. Commun., 8, 15002, https://doi.org/10.1038/ncomms15002, 2017.
Skamarock, W. C., Klemp, J. B., Dudhia, J., Gill, D. O., Barker, D. M., Duda, M. G., Huang, X.-Y., Wang, W., and Powers, J. G.: A description of the advanced research WRF version 3, NCAR Tech. Note NCAR/TN-475+STR, University Corporation for Atmos. Res., 113 pp., https://doi.org/10.5065/D68S4MVH, 2008.
Stier, P., Feichter, J., Kloster, S., Vignati, E., and Wilson, J.: Emission-Induced Nonlinearities in the Global Aerosol System: Results from the ECHAM5-HAM Aerosol-Climate Model, J. Climate, 19, 3845–3862, https://doi.org/10.1175/jcli3772.1, 2006.
Stritzke, F., Diemel, O., and Wagner, S.: TDLAS-based NH3 mol fraction measurement for exhaust diagnostics during selective catalytic reduction using a fiber-coupled 2.2-µm DFB diode laser, Appl. Phys. B, 119, 143–152, https://doi.org/10.1007/s00340-015-6073-5, 2015.
Sutton, M. A., Reis, S., Riddick, S. N., Dragosits, U., Nemitz, E., Theobald, M. R., Tang, Y. S., Braban, C. F., Vieno, M., Dore, A. J., Mitchell, R. F., Wanless, S., Daunt, F., Fowler, D., Blackall, T. D., Milford, C., Flechard, C. R., Loubet, B., Massad, R., Cellier, P., Personne, E., Coheur, P. F., Clarisse, L., Van Damme, M., Ngadi, Y., Clerbaux, C., Skjøth, C. A., Geels, C., Hertel, O., Kruit, R. J. W., Pinder, R. W., Bash, J. O., Walker, J. T., Simpson, D., Horváth, L., Misselbrook, T. H., Bleeker, A., Dentener, F., and de Vries, W.: Towards a climate-dependent paradigm of ammonia emission and deposition, Philos. Trans. R. Soc. B, 368, 1–13, https://doi.org/10.1098/rstb.2013.0166, 2013.
Tegen, I., Neubauer, D., Ferrachat, S., Siegenthaler-Le Drian, C., Bey, I., Schutgens, N., Stier, P., Watson-Parris, D., Stanelle, T., Schmidt, H., Rast, S., Kokkola, H., Schultz, M., Schroeder, S., Daskalakis, N., Barthel, S., Heinold, B., and Lohmann, U.: The global aerosol–climate model ECHAM6.3–HAM2.3 – Part 1: Aerosol evaluation, Geosci. Model Dev., 12, 1643–1677, https://doi.org/10.5194/gmd-12-1643-2019, 2019.
Tewari, M., Chen, F., Wang, W., Dudhia, J., LeMone, M. A., Mitchell, K., Ek, M., Gayno, G., Wegiel, J., and Cuenca, R. H.: Implementation and verification of the unified NOAH land surface model in the WRF model, 20th conference on weather analysis and forecasting/16th conference on numerical weather prediction, Seattle, Washington, USA,
14 January 2004, 11–15 pp., 2004.
Tuccella, P., Curci, G., Grell, G. A., Visconti, G., Crumeyrolle, S., Schwarzenboeck, A., and Mensah, A. A.: A new chemistry option in WRF-Chem v. 3.4 for the simulation of direct and indirect aerosol effects using VBS: evaluation against IMPACT-EUCAARI data, Geosci. Model Dev., 8, 2749–2776, https://doi.org/10.5194/gmd-8-2749-2015, 2015.
Twomey, S.: Pollution and the planetary albedo, Atmos. Environ., 8, 1251–1256, 1974.
Van Damme, M., Clarisse, L., Heald, C. L., Hurtmans, D., Ngadi, Y., Clerbaux, C., Dolman, A. J., Erisman, J. W., and Coheur, P. F.: Global distributions, time series and error characterization of atmospheric ammonia (NH3) from IASI satellite observations, Atmos. Chem. Phys., 14, 2905–2922, https://doi.org/10.5194/acp-14-2905-2014, 2014.
VanReken, T. M., Rissman, T. A., Roberts, G. C., Varutbangkul, V., Jonsson, H. H., Flagan, R. C., and Seinfeld, J. H.: Toward aerosol/cloud condensation nuclei (CCN) closure during CRYSTAL-FACE, J. Geophys. Res., 108(D20), 4633, https://doi.org/10.1029/2003JD003582, 2003.
Waggoner, A. P., Weiss, R. E., and Larson, T. V.: In-situ, rapid response measurement of H2SO4/(NH4)2SO4 aerosols in urban Houston: A comparison with rural Virginia, Atmos. Environ., 17, 1723–1731, https://doi.org/10.1016/0004-6981(83)90179-8, 1967.
Warner, J. X., Dickerson, R. R., Wei, Z., Strow, L. L., Wang, Y., and Liang, Q.: Increased atmospheric ammonia over the world's major agricultural areas detected from space, Geophys. Res. Lett., 44, 2875–2884, https://doi.org/10.1002/2016GL072305, 2017.
Watanabe, M., Suzuki, T., O'ishi, R., Komuro, Y., Watanabe, S., Emori, S., Takemura, T., Chikara, M., Ogura, T., Sekiguchi, M., Takata, K., Yamazaki, D., Yokohata, T., Nozawa, T., Hasumi, H., Tatebe, H., and Kimoto, M.: Improved climate simulation by MIROC5: mean states, variability, and climate sensitivity, J. Climate, 23, 6312–6335, https://doi.org/10.1175/2010jcli3679.1, 2010.
Wexler, A. S., Lurmann, F. W., and Seinfeld, J. H.: Modelling urban and regional aerosols–I. model development, Atmos. Environ., 28, 531–546, https://doi.org/10.1016/1352-2310(94)90129-5, 1994.
Yang, Y., Wang, H., Smith, S. J., Easter, R., Ma, P.-L., Qian, Y., Yu, H., Li, C., and Rasch, P. J.: Global source attribution of sulfate concentration and direct and indirect radiative forcing, Atmos. Chem. Phys., 17, 8903–8922, https://doi.org/10.5194/acp-17-8903-2017, 2017.
Zelinka, M. D., Andrews, T., Forster, P. M., and Taylor, K. E.: Quantifying components of aerosol–cloud–radiation interactions in climate models, J. Geophys. Res. Atmos., 119, 7599–7615, https://doi.org/10.1002/2014JD021710, 2014.
Zhang, K., O'Donnell, D., Kazil, J., Stier, P., Kinne, S., Lohmann, U., Ferrachat, S., Croft, B., Quaas, J., Wan, H., Rast, S., and Feichter, J.: The global aerosol-climate model ECHAM-HAM, version 2: sensitivity to improvements in process representations, Atmos. Chem. Phys., 12, 8911–8949, https://doi.org/10.5194/acp-12-8911-2012, 2012.
Zhao, D. F., Buchholz, A., Kortner, B., Schlag, P., Rubach, F., Kiendler-Scharr, A., Tillmann, R., Wahner, A., Flores, J. M., Rudich, Y., Watne, Å. K., Hallquist, M., Wildt, J., and Mentel, T. F.: Size-dependent hygroscopicity parameter (κ) and chemical composition of secondary organic cloud condensation nuclei, Geophys. Res. Lett., 42, 10920–10928, https://doi.org/10.1002/2015GL066497, 2015.
Short summary
A new method to estimate the sulfate aerosol hygroscopicity parameter (κSO4) is suggested that can consider κSO4 for two different sulfate species instead of prescribing a single κSO4 value, as in most previous studies. The new method simulates more realistic cloud droplet concentrations and, thus, a more realistic cloud albedo effect than the original method. The new method is simple and readily applicable to modeling studies investigating sulfate aerosols’ effect in aerosol–cloud interactions.
A new method to estimate the sulfate aerosol hygroscopicity parameter (κSO4) is suggested that...