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Geoscientific Model Development An interactive open-access journal of the European Geosciences Union
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Preprints
https://doi.org/10.5194/gmd-2019-221
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/gmd-2019-221
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.

  14 Aug 2019

14 Aug 2019

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A revised version of this preprint was accepted for the journal GMD and is expected to appear here in due course.

Simulating Forest Fire Plume Dispersion, Chemistry, and Aerosol Formation Using SAM-ASP version 1.0

Chantelle R. Lonsdale1, Matthew J. Alvarado1, Anna L. Hodshire2, Emily Ramnarine2, and Jeffrey R. Pierce2 Chantelle R. Lonsdale et al.
  • 1Atmospheric and Environmental Research (AER), Lexington, MA, 02421, USA
  • 2Department of Atmospheric Science, Colorado State University, Fort Collins, CO, 80523, USA

Abstract. Biomass burning is a major source of trace gases and aerosols that can ultimately impact health, air quality, and climate. Global and regional-scale three-dimensional Eulerian chemical transport models (CTMs) use estimates of the primary emissions from fires and can unphysically mix them across large-scale grid boxes, leading to incorrect estimates of the impact of biomass burning events. On the other hand, plume-scale process models allow for explicit simulation and examination of the chemical and physical transformations of trace gases and aerosols within biomass burning smoke plumes, and they may be used to develop parameterizations of this aging process for coarser grid-scale models. Here we describe the coupled SAM-ASP plume-scale process model, which consists of coupling the large-eddy simulation model, the System for Atmospheric Modelling (SAM) version 1.0, with the detailed gas and aerosol chemistry model, the Aerosol Simulation Program (ASP). We find that the SAM-ASP version 1.0 model is able to correctly simulate the dilution of CO in a California chaparral smoke plume, as well as the chemical loss of NOx, HONO, and NH3 within the plume, the formation of PAN and O3, the loss of OA, and the change in the size distribution of aerosols as compared to measurements and previous single-box model results. The newly coupled model is able to capture the cross-plume vertical and horizontal concentration gradients as the fire plume evolves downwind of the emission source. The integration and evaluation of SAM-ASP presented here will support the development of parameterizations of near-source biomass burning chemistry that can be used to more accurately simulate biomass burning chemical and physical transformations of trace gases and aerosols within coarser grid-scale CTMs.

Chantelle R. Lonsdale et al.

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Interactive discussion

Status: closed
Status: closed
AC: Author comment | RC: Referee comment | SC: Short comment | EC: Editor comment
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Chantelle R. Lonsdale et al.

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Simulating Forest Fire Plume Dispersion, Chemistry, and Aerosol Formation Using SAM-ASP version 1.0 C. R. Lonsdale, M. J. Alvarado, A. L. Hodshire, E. Ramnarine, and J. R. Pierce https://doi.org/10.5281/zenodo.3363995

Chantelle R. Lonsdale et al.

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Short summary
The System for Atmospheric Modelling (SAM) has been coupled with the detailed gas/aerosol chemistry model, the Aerosol Simulation Program (ASP) to capture cross-plume concentration gradients as fire plumes evolve downwind. SAM-ASP v1.0 will lead to the development of parameterizations of near-source biomass burning chemistry that can be used to more accurately simulate biomass burning chemical and physical transformations of trace gases and aerosols within coarser CTMs.
The System for Atmospheric Modelling (SAM) has been coupled with the detailed gas/aerosol...
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