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<article xmlns:xlink="http://www.w3.org/1999/xlink" xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:oasis="http://docs.oasis-open.org/ns/oasis-exchange/table" xml:lang="en" dtd-version="3.0"><?xmltex \makeatother\@nolinetrue\makeatletter?>
  <front>
    <journal-meta><journal-id journal-id-type="publisher">GMD</journal-id><journal-title-group>
    <journal-title>Geoscientific Model Development</journal-title>
    <abbrev-journal-title abbrev-type="publisher">GMD</abbrev-journal-title><abbrev-journal-title abbrev-type="nlm-ta">Geosci. Model Dev.</abbrev-journal-title>
  </journal-title-group><issn pub-type="epub">1991-9603</issn><publisher>
    <publisher-name>Copernicus Publications</publisher-name>
    <publisher-loc>Göttingen, Germany</publisher-loc>
  </publisher></journal-meta>
    <article-meta>
      <article-id pub-id-type="doi">10.5194/gmd-11-1557-2018</article-id><title-group><article-title>Prognostic parameterization of cloud ice with a single category in the aerosol-climate model ECHAM(v6.3.0)-HAM(v2.3)</article-title><alt-title>Prognostic parameterization of cloud ice in ECHAM6-HAM2</alt-title>
      </title-group><?xmltex \runningtitle{Prognostic parameterization of cloud ice in ECHAM6-HAM2}?><?xmltex \runningauthor{R. Dietlicher et al.}?>
      <contrib-group>
        <contrib contrib-type="author" corresp="yes">
          <name><surname>Dietlicher</surname><given-names>Remo</given-names></name>
          <email>remo.dietlicher@env.ethz.ch</email>
        <ext-link>https://orcid.org/0000-0003-0217-7232</ext-link></contrib>
        <contrib contrib-type="author" corresp="no">
          <name><surname>Neubauer</surname><given-names>David</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-9869-3946</ext-link></contrib>
        <contrib contrib-type="author" corresp="no">
          <name><surname>Lohmann</surname><given-names>Ulrike</given-names></name>
          
        <ext-link>https://orcid.org/0000-0001-8885-3785</ext-link></contrib>
        <aff id="aff1"><institution>Institute for Atmospheric and Climate Science, ETH Zürich, Universitätstrasse 16, 8092 Zurich, Switzerland</institution>
        </aff>
      </contrib-group>
      <author-notes><corresp id="corr1">Remo Dietlicher (remo.dietlicher@env.ethz.ch)</corresp></author-notes><pub-date><day>18</day><month>April</month><year>2018</year></pub-date>
      
      <volume>11</volume>
      <issue>4</issue>
      <fpage>1557</fpage><lpage>1576</lpage>
      <history>
        <date date-type="received"><day>7</day><month>July</month><year>2017</year></date>
           <date date-type="rev-request"><day>14</day><month>August</month><year>2017</year></date>
           <date date-type="rev-recd"><day>8</day><month>March</month><year>2018</year></date>
           <date date-type="accepted"><day>23</day><month>March</month><year>2018</year></date>
      </history>
      <permissions>
        <copyright-statement>Copyright: © 2018 Remo Dietlicher et al.</copyright-statement>
        <copyright-year>2018</copyright-year>
      <license license-type="open-access"><license-p>This work is licensed under the Creative Commons Attribution 4.0 International License. To view a copy of this licence, visit <ext-link ext-link-type="uri" xlink:href="https://creativecommons.org/licenses/by/4.0/">https://creativecommons.org/licenses/by/4.0/</ext-link></license-p></license></permissions><self-uri xlink:href="https://gmd.copernicus.org/articles/11/1557/2018/gmd-11-1557-2018.html">This article is available from https://gmd.copernicus.org/articles/11/1557/2018/gmd-11-1557-2018.html</self-uri><self-uri xlink:href="https://gmd.copernicus.org/articles/11/1557/2018/gmd-11-1557-2018.pdf">The full text article is available as a PDF file from https://gmd.copernicus.org/articles/11/1557/2018/gmd-11-1557-2018.pdf</self-uri>
      <abstract><title>Abstract</title>
    <p id="d1e95">A new scheme for stratiform cloud microphysics has been implemented in the
ECHAM6-HAM2 general circulation model. It features a widely used description
of cloud water with two categories for cloud droplets and raindrops. The
unique aspect of the new scheme is the break with the traditional approach to
describe cloud ice analogously. Here we parameterize cloud ice by a single
category that predicts bulk particle properties (P3). This method has already
been applied in a regional model and most recently also in the Community
Atmosphere Model 5 (CAM5). A single cloud ice category does not rely on
heuristic conversion rates from one category to another. Therefore, it is
conceptually easier and closer to first principles.</p>
    <p id="d1e98">This work shows that a single category is a viable approach to describe cloud
ice in climate models. Prognostic representation of sedimentation is achieved
by a nested approach for sub-stepping the cloud microphysics scheme. This
yields good results in terms of accuracy and performance as compared to
simulations with high temporal resolution. Furthermore, the new scheme allows
for a competition between various cloud processes and is thus able to
unbiasedly represent the ice formation pathway from nucleation to growth by
vapor deposition and collisions to sedimentation.</p>
    <p id="d1e101">Specific aspects of the P3 method are evaluated. We could not produce a
purely stratiform cloud where rime growth dominates growth by vapor
deposition and conclude that the lack of appropriate conditions renders the
prognostic parameters associated with the rime properties unnecessary.
Limitations inherent in a single category are examined.</p>
  </abstract>
    </article-meta>
  </front>
<body>
      

      <?xmltex \hack{\newpage}?>
<sec id="Ch1.S1" sec-type="intro">
  <title>Introduction</title>
      <p id="d1e113">Clouds are a major source of uncertainty in current climate projections as
assessed by the last IPCC report <xref ref-type="bibr" rid="bib1.bibx44" id="paren.1"/>. Apart from synoptic-scale
low pressure systems, clouds are not resolved by the coarse spatial
resolution used in climate models, which necessitates a transfer from
grid-box mean model states to the sub-grid distribution of humidity down to
the microphysical properties of clouds. The circumstances require heuristic
methods to represent the average response of clouds to natural and
anthropogenic forcing.</p>
      <p id="d1e119">Over the last 50 years the level of sophistication of the transfer methods
from resolved to parameterized scales has steadily increased.
<xref ref-type="bibr" rid="bib1.bibx17" id="text.2"/> built a scheme based on a system of continuity equations
for vapor, cloud and precipitation, which assumed that clouds form as soon as
grid-box mean supersaturation is established and precipitate proportionally
to their mass. This idea was refined by the work of <xref ref-type="bibr" rid="bib1.bibx45" id="text.3"/> to
account for sub-grid cloudiness by assuming an inhomogeneous distribution of
moisture within a model grid box. Later on, polydisperse cloud droplets were
represented <xref ref-type="bibr" rid="bib1.bibx3" id="paren.4"/>, which was the first step towards the now common transfer from grid-box mean quantities down to particle scales by
the assumption of particle size distributions in two-moment schemes. Since
then, a multitude of studies has documented the progress in both the representation
of sub-grid clouds (e.g., <xref ref-type="bibr" rid="bib1.bibx51" id="altparen.5"/>) and the extension of schemes
based on particle size distributions to ice (e.g., <xref ref-type="bibr" rid="bib1.bibx41" id="altparen.6"/>).</p>
      <p id="d1e137"><xref ref-type="bibr" rid="bib1.bibx20" id="text.7"/> assessed the ability of climate models to represent the amount
of ice in clouds from the last generation of climate models. They found that
the globally averaged, annual mean ice water path differs by a factor of
2–10 among<?pagebreak page1558?> the selected models used in the Coupled Model Intercomparison Project Phase 5 (CMIP5). While all of the models in their study are in radiative
balance, they do so at the cost of a wide variety of cloud ice contents due
to the large uncertainty in their radiative properties. At the same time, new
studies <xref ref-type="bibr" rid="bib1.bibx47" id="paren.8"/> suggest that as the phase of a cloud is
decisive for its radiative properties, it strongly impacts the equilibrium
climate sensitivity (ECS) <xref ref-type="bibr" rid="bib1.bibx48" id="paren.9"/>. Furthermore, satellite observations show that the occurrence of ice and mixed-phase clouds is tightly
linked to precipitation fields <xref ref-type="bibr" rid="bib1.bibx34 bib1.bibx8" id="paren.10"/>, which further reinforces the importance of accurately representing cloud ice
in models.</p>
      <p id="d1e151">The response of climate, and in particular clouds, to a warming world induced
by increasing carbon dioxide emissions is a highly discussed topic in the
climate research community
<xref ref-type="bibr" rid="bib1.bibx11 bib1.bibx4 bib1.bibx43 bib1.bibx48 bib1.bibx40" id="paren.11"/>. Following
<xref ref-type="bibr" rid="bib1.bibx48" id="text.12"/> we focus on improving the representation of the supercooled
liquid fraction in climate models and hence cloud ice in general. As has been
laid out by the study of <xref ref-type="bibr" rid="bib1.bibx20" id="text.13"/>, there is a lot of room for
improvement in this area.</p>
      <p id="d1e164">Many climate models represent ice by predefining categories for a given
particle characteristic, such as ice crystals, planar snow flakes, or dense
and spherical graupel and hail particles <xref ref-type="bibr" rid="bib1.bibx41" id="paren.14"/>. Widely used
categories for ice particles in models are in-cloud ice and falling snow.
With the coarse resolution employed in climate models, these categories serve
to distinguish between cloud ice and precipitation. This approach is
motivated by the analogous treatment for cloud liquid water where cloud
droplets are separated from raindrops. However, unlike for liquid water
where there is a clear scale separation between condensational growth and
growth by collision and coalescence, the criteria to divide ice into an
in-cloud category and a precipitating category is not well defined. This
classification therefore differs from model to model and, being weakly
constrained, the associated conversion rates are often used as tuning
parameters. The conversion from cloud ice to snow is usually based on a
threshold size for snow. Some models cut off the particle size distribution
at a given threshold <xref ref-type="bibr" rid="bib1.bibx32" id="paren.15"/>; others use it together
with ice growth rates to calculate the time needed to grow particles to the
threshold size <xref ref-type="bibr" rid="bib1.bibx35" id="paren.16"/>. Due to this heuristic partitioning,
cloud ice parameterizations are associated with a large uncertainty.</p>
      <p id="d1e176">New studies <xref ref-type="bibr" rid="bib1.bibx33 bib1.bibx14" id="paren.17"/> introduce
techniques to describe cloud ice in a more continuous fashion. Contrary to
the common approach of representing ice as a composition of different
particle types, they suggest using a single category whose properties adjust
smoothly to cloud conditions and formation history. This eliminates the need
to parameterize weakly constrained conversion processes among categories.</p>
      <p id="d1e182">Describing a hydrometeor species with a single category implies that the
entire category, including a potentially fast-falling part, has to be treated
prognostically. Since prognostic precipitation categories are becoming more
and more popular in multi-category schemes as well
<xref ref-type="bibr" rid="bib1.bibx9 bib1.bibx39" id="paren.18"/>, many approaches exist to locally
increase time resolution in order to achieve numeric stability. Here we
present a nested sub-stepping approach in the ECHAM6-HAM2 general circulation
model (GCM) microphysics scheme.</p>
      <p id="d1e188">In this study we focus on the pathways subsequent to ice initiation by a more
physically based description of cloud ice but acknowledge the importance of
ongoing research to understand freezing mechanisms
<xref ref-type="bibr" rid="bib1.bibx52 bib1.bibx13 bib1.bibx29" id="paren.19"/> and the resulting parameterization
development <xref ref-type="bibr" rid="bib1.bibx36 bib1.bibx12" id="paren.20"/>. We will use the
microphysical properties of ice described in <xref ref-type="bibr" rid="bib1.bibx33" id="text.21"/>
(hereafter MM15), also known as the predicted bulk particle properties (P3),
and embed them in the ECHAM6-HAM2 cloud microphysics scheme.</p>
      <p id="d1e200">The P3 method was originally implemented in the regional model Weather
Research and Forecasting Model (WRF). More recently, it has also been
included in the global context of the Community Atmosphere Model 5 (CAM5)
<xref ref-type="bibr" rid="bib1.bibx7" id="paren.22"/>. <xref ref-type="bibr" rid="bib1.bibx7" id="text.23"/> focus on the description of the particle
properties within P3 and the empirical parameter choices therein and discard
the effects of riming on the particle properties a priori. Our paper
documents the transition from diagnostic snow to a prognostic single category
in ECHAM6-HAM2 on a technical level. We use the full P3 method, including the
rime properties, and evaluate a cloud formation scenario that is consistent
with the forcing provided by a GCM and might allow for significant rime
formation. We show idealized mixed-phase cloud simulations to better
understand the cloud formation and glaciation process with the new scheme.
The intuition gained from this exercise then helps interpreting model output
where usually only temporal and global averages are available and the
information on individual clouds is lost.</p>
      <p id="d1e209">A short summary of the P3 method is given in Sect. <xref ref-type="sec" rid="Ch1.S2"/>. As
this new approach leads to a revision of the existing cloud microphysics
scheme, the entire scheme is described in Sect. <xref ref-type="sec" rid="Ch1.S3"/>. Numerical
challenges associated with the prognostic treatment of sedimenting ice are
addressed in Sect. <xref ref-type="sec" rid="Ch1.S4"/>. Section <xref ref-type="sec" rid="Ch1.S5"/> shows
results of the new microphysics scheme in a 1-D single-column setup. We
highlight conceptual differences to the original 2-category scheme,
potential simplifications in the context of a GCM and limitations inherent in
a single category. Section <xref ref-type="sec" rid="Ch1.S6"/> concludes this study by
evaluating the feasibility and benefit from using a single-category ice phase
scheme in ECHAM6-HAM2.</p>
</sec>
<?pagebreak page1559?><sec id="Ch1.S2">
  <title>Revision of the predicted bulk particle properties (P3)</title>
      <p id="d1e228">This section serves as a review of the fundamental concepts of the P3 method
presented in MM15. All the relevant aspects for the prediction of particle
properties from the grid-box mean model state are covered.</p>
      <p id="d1e231">Instead of the two categories for cloud ice and snow, the single-category
scheme uses four prognostic parameters describing a single category: the
total ice mass mixing ratio <inline-formula><mml:math id="M1" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, total ice number concentration
<inline-formula><mml:math id="M2" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, riming mass mixing ratio <inline-formula><mml:math id="M3" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>rim</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and riming volume
<inline-formula><mml:math id="M4" display="inline"><mml:mrow><mml:msub><mml:mi>b</mml:mi><mml:mtext>rim</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>. For the particle size distribution the gamma distribution
          <disp-formula id="Ch1.E1" content-type="numbered"><mml:math id="M5" display="block"><mml:mrow><mml:mi>N</mml:mi><mml:mo>(</mml:mo><mml:mi>D</mml:mi><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mtext>i</mml:mtext></mml:msub><mml:msup><mml:mi mathvariant="italic">λ</mml:mi><mml:mrow><mml:mi mathvariant="italic">μ</mml:mi><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow><mml:mrow><mml:mi mathvariant="normal">Γ</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="italic">μ</mml:mi><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>)</mml:mo></mml:mrow></mml:mfrac></mml:mstyle><mml:msup><mml:mi>D</mml:mi><mml:mrow><mml:mi mathvariant="italic">μ</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="italic">λ</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msup><mml:msup><mml:mi>e</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mi mathvariant="italic">λ</mml:mi><mml:mi>D</mml:mi></mml:mrow></mml:msup></mml:mrow></mml:math></disp-formula>
        is chosen with the gamma function <inline-formula><mml:math id="M6" display="inline"><mml:mrow><mml:mi mathvariant="normal">Γ</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="italic">μ</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> and the three free parameters
<inline-formula><mml:math id="M7" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M8" display="inline"><mml:mi mathvariant="italic">μ</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M9" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula>. An empirical relationship between <inline-formula><mml:math id="M10" display="inline"><mml:mi mathvariant="italic">μ</mml:mi></mml:math></inline-formula>
and <inline-formula><mml:math id="M11" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula> <xref ref-type="bibr" rid="bib1.bibx10" id="paren.24"/> reduces the number of free parameters
from three to two:
          <disp-formula id="Ch1.E2" content-type="numbered"><mml:math id="M12" display="block"><mml:mrow><mml:mi mathvariant="italic">μ</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.076</mml:mn><mml:msup><mml:mfenced close=")" open="("><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mi mathvariant="italic">λ</mml:mi><mml:mn mathvariant="normal">100</mml:mn></mml:mfrac></mml:mstyle></mml:mfenced><mml:mn mathvariant="normal">0.8</mml:mn></mml:msup><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>
        The parameter <inline-formula><mml:math id="M13" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula> is given in m<inline-formula><mml:math id="M14" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. The scheme defines a regime-dependent mass-to-size
relationship:

              <disp-formula specific-use="align" content-type="numbered"><mml:math id="M15" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E3"><mml:mtd/><mml:mtd><mml:mstyle class="stylechange" displaystyle="true"/></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:mi>m</mml:mi><mml:mo>(</mml:mo><mml:mi>D</mml:mi><mml:mo>)</mml:mo><mml:mo>=</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mtr><mml:mtd><mml:mstyle class="stylechange" displaystyle="true"/></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:mfenced open="{" close=""><mml:mtable class="cases" columnspacing="1em" rowspacing="0.2ex" columnalign="left left" framespacing="0em"><mml:mtr><mml:mtd><mml:mrow><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mi mathvariant="italic">π</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:mfrac></mml:mstyle><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>i</mml:mtext></mml:msub><mml:msup><mml:mi>D</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:mi mathvariant="normal">for</mml:mi><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mi mathvariant="normal">small</mml:mi><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mi mathvariant="normal">spherical</mml:mi><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mi mathvariant="normal">ice</mml:mi><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mi>D</mml:mi><mml:mo>&lt;</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mtext>th</mml:mtext></mml:msub></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd><mml:mrow><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mtext>va</mml:mtext></mml:msub><mml:msup><mml:mi>D</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mtext>va</mml:mtext></mml:msub></mml:mrow></mml:msup></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:mi mathvariant="normal">for</mml:mi><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mi mathvariant="normal">dendrites</mml:mi><mml:mo>,</mml:mo><mml:mspace width="0.25em" linebreak="nobreak"/><mml:msub><mml:mi>D</mml:mi><mml:mtext>th</mml:mtext></mml:msub><mml:mo>&lt;</mml:mo><mml:mi>D</mml:mi><mml:mo>&lt;</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mtext>gr</mml:mtext></mml:msub></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd><mml:mrow><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mi mathvariant="italic">π</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:mfrac></mml:mstyle><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>g</mml:mtext></mml:msub><mml:msup><mml:mi>D</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:mi mathvariant="normal">for</mml:mi><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mi mathvariant="normal">graupel</mml:mi><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.25em"/><mml:msub><mml:mi>D</mml:mi><mml:mtext>gr</mml:mtext></mml:msub><mml:mo>&lt;</mml:mo><mml:mi>D</mml:mi><mml:mo>&lt;</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mtext>cr</mml:mtext></mml:msub></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd><mml:mrow><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mrow><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mtext>va</mml:mtext></mml:msub></mml:mrow><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:msub><mml:mi>F</mml:mi><mml:mtext>r</mml:mtext></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:msup><mml:mi>D</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mtext>va</mml:mtext></mml:msub></mml:mrow></mml:msup></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:mi mathvariant="normal">for</mml:mi><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mi mathvariant="normal">partially</mml:mi><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mi mathvariant="normal">rimed</mml:mi><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mi mathvariant="normal">crystals</mml:mi><mml:mo>,</mml:mo><mml:mspace width="0.25em" linebreak="nobreak"/><mml:msub><mml:mi>D</mml:mi><mml:mtext>cr</mml:mtext></mml:msub><mml:mo>&lt;</mml:mo><mml:mi>D</mml:mi><mml:mo>.</mml:mo></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:mfenced></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:math></disp-formula>

          The parameters <inline-formula><mml:math id="M16" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mtext>va</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M17" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mtext>va</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> that define the mass-to-size relation for dendrites are empirical constants derived for aggregates
of unrimed bullets, columns and side planes <xref ref-type="bibr" rid="bib1.bibx5" id="paren.25"/>,
<inline-formula><mml:math id="M18" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is the density of ice, and <inline-formula><mml:math id="M19" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>g</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is the density of
graupel. The rime fraction <inline-formula><mml:math id="M20" display="inline"><mml:mrow><mml:msub><mml:mi>F</mml:mi><mml:mtext>r</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>q</mml:mi><mml:mtext>rim</mml:mtext></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>q</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is predicted
by the model. The scheme needs to predict four unknown parameters: two for
the mass-to-size relationship and two for the particle size distribution. The
mass-to-size relationship is defined by the two transition sizes
<inline-formula><mml:math id="M21" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>gr</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> separating dendrites from graupel and <inline-formula><mml:math id="M22" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>cr</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> separating
graupel from partially rimed particles; see Fig. <xref ref-type="fig" rid="Ch1.F1"/>. The
particle size distribution is defined by the total number of particles
<inline-formula><mml:math id="M23" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and one of the gamma distribution shape parameters <inline-formula><mml:math id="M24" display="inline"><mml:mi mathvariant="italic">μ</mml:mi></mml:math></inline-formula> or
<inline-formula><mml:math id="M25" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula> through the use of Eq. (<xref ref-type="disp-formula" rid="Ch1.E2"/>).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F1"><label>Figure 1</label><caption><p id="d1e801">Summary of the mechanism used in the single-category scheme with an
exemplary particle size distribution. <inline-formula><mml:math id="M26" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is the density of ice,
<inline-formula><mml:math id="M27" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mtext>va</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M28" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mtext>va</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> are empirical constants,
<inline-formula><mml:math id="M29" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>g</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is the diagnosed graupel density, and <inline-formula><mml:math id="M30" display="inline"><mml:mrow><mml:msub><mml:mi>F</mml:mi><mml:mtext>r</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>q</mml:mi><mml:mtext>rim</mml:mtext></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>q</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is the rime fraction. The dashed–dotted line between
<inline-formula><mml:math id="M31" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>gr</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M32" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>cr</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> visualizes the extrapolation of the dendritic
particles to the rimed regime for the calculation of <inline-formula><mml:math id="M33" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>g</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>
referenced in the text.</p></caption>
        <?xmltex \igopts{width=227.622047pt}?><graphic xlink:href="https://gmd.copernicus.org/articles/11/1557/2018/gmd-11-1557-2018-f01.png"/>

      </fig>

      <p id="d1e913">In the following it will be explained how those four unknown parameters are
calculated from the grid-box mean state defined by the four prognostic
parameters: the total ice mass <inline-formula><mml:math id="M34" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, the rimed ice mass
<inline-formula><mml:math id="M35" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>rim</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, the total ice number <inline-formula><mml:math id="M36" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and the rimed ice density
<inline-formula><mml:math id="M37" display="inline"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mtext>rim</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>. The threshold sizes <inline-formula><mml:math id="M38" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>gr</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M39" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>cr</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> are
defined by requiring that the mass-to-size relationship increases
monotonically with increasing particle diameter. This yields the three
equations

              <disp-formula specific-use="align" content-type="numbered"><mml:math id="M40" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E4"><mml:mtd/><mml:mtd><mml:mstyle displaystyle="true" class="stylechange"/></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mi mathvariant="italic">π</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:mfrac></mml:mstyle><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>i</mml:mtext></mml:msub><mml:msup><mml:mi>D</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msup><mml:mo>=</mml:mo><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mtext>va</mml:mtext></mml:msub><mml:msup><mml:mi>D</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mtext>va</mml:mtext></mml:msub></mml:mrow></mml:msup><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mo>⇒</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mtext>th</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:msup><mml:mfenced close=")" open="("><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="italic">π</mml:mi><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow><mml:mrow><mml:mn mathvariant="normal">6</mml:mn><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mtext>va</mml:mtext></mml:msub></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mfrac><mml:mn mathvariant="normal">1</mml:mn><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mtext>va</mml:mtext></mml:msub><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:mfrac></mml:msup><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mtr><mml:mtd><mml:mstyle class="stylechange" displaystyle="true"/></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mtext>va</mml:mtext></mml:msub><mml:msup><mml:mi>D</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mtext>va</mml:mtext></mml:msub></mml:mrow></mml:msup><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mi mathvariant="italic">π</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:mfrac></mml:mstyle><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>g</mml:mtext></mml:msub><mml:msup><mml:mi>D</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msup><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mo>⇒</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mtext>gr</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:msup><mml:mfenced open="(" close=")"><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mn mathvariant="normal">6</mml:mn><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mtext>va</mml:mtext></mml:msub></mml:mrow><mml:mrow><mml:mi mathvariant="italic">π</mml:mi><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>g</mml:mtext></mml:msub></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mfrac><mml:mn mathvariant="normal">1</mml:mn><mml:mrow><mml:mn mathvariant="normal">3</mml:mn><mml:mo>-</mml:mo><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mtext>va</mml:mtext></mml:msub></mml:mrow></mml:mfrac></mml:msup><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd><mml:mstyle class="stylechange" displaystyle="true"/></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mi mathvariant="italic">π</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:mfrac></mml:mstyle><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>g</mml:mtext></mml:msub><mml:msup><mml:mi>D</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msup><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mtext>va</mml:mtext></mml:msub></mml:mrow><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:msub><mml:mi>F</mml:mi><mml:mtext>r</mml:mtext></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:msup><mml:mi>D</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mtext>va</mml:mtext></mml:msub></mml:mrow></mml:msup><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mo>⇒</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mtext>cr</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:msup><mml:mfenced close=")" open="("><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mn mathvariant="normal">6</mml:mn><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mtext>va</mml:mtext></mml:msub></mml:mrow><mml:mrow><mml:mo>(</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:msub><mml:mi>F</mml:mi><mml:mtext>r</mml:mtext></mml:msub><mml:mo>)</mml:mo><mml:mi mathvariant="italic">π</mml:mi><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>g</mml:mtext></mml:msub></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mfrac><mml:mn mathvariant="normal">1</mml:mn><mml:mrow><mml:mn mathvariant="normal">3</mml:mn><mml:mo>-</mml:mo><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mtext>va</mml:mtext></mml:msub></mml:mrow></mml:mfrac></mml:msup><mml:mo>.</mml:mo></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:math></disp-formula>

          One directly sees that <inline-formula><mml:math id="M41" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>th</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> only depends on constants while the
others depend on the graupel density <inline-formula><mml:math id="M42" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>g</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and rime fraction
<inline-formula><mml:math id="M43" display="inline"><mml:mrow><mml:msub><mml:mi>F</mml:mi><mml:mtext>r</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>. To calculate the graupel density <inline-formula><mml:math id="M44" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>g</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, a system of
equations needs to be solved. The value of <inline-formula><mml:math id="M45" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>g</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> depends on both
the density of rimed ice <inline-formula><mml:math id="M46" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>r</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> that accumulated on a particle by
wet growth and the density of the underlying dendritic structure
<inline-formula><mml:math id="M47" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>. It is thus calculated as the average of the two, weighted by
the rime mass fraction:
          <disp-formula id="Ch1.E5" content-type="numbered"><mml:math id="M48" display="block"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>g</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>F</mml:mi><mml:mtext>r</mml:mtext></mml:msub><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>r</mml:mtext></mml:msub><mml:mo>+</mml:mo><mml:mo>(</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:msub><mml:mi>F</mml:mi><mml:mtext>r</mml:mtext></mml:msub><mml:mo>)</mml:mo><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>d</mml:mtext></mml:msub><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>
        The density of the underlying dendrite in the rimed regime (illustrated by
the dashed–dotted line in Fig. <xref ref-type="fig" rid="Ch1.F1"/>) in turn is calculated as
a mass-weighted average over the rime regime (<inline-formula><mml:math id="M49" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>gr</mml:mtext></mml:msub><mml:mo>&lt;</mml:mo><mml:mi>D</mml:mi><mml:mo>&lt;</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mtext>cr</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>):
          <disp-formula id="Ch1.E6" content-type="numbered"><mml:math id="M50" display="block"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>d</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mn mathvariant="normal">6</mml:mn><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mtext>va</mml:mtext></mml:msub><mml:mo>(</mml:mo><mml:msubsup><mml:mi>D</mml:mi><mml:mtext>cr</mml:mtext><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mtext>va</mml:mtext></mml:msub><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msubsup><mml:mo>-</mml:mo><mml:msubsup><mml:mi>D</mml:mi><mml:mtext>gr</mml:mtext><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mtext>va</mml:mtext></mml:msub><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msubsup><mml:mo>)</mml:mo></mml:mrow><mml:mrow><mml:mi mathvariant="italic">π</mml:mi><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mtext>va</mml:mtext></mml:msub><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn><mml:mo>)</mml:mo><mml:mo>(</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mtext>cr</mml:mtext></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mtext>gr</mml:mtext></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>
        Equations (<xref ref-type="disp-formula" rid="Ch1.E5"/>) and (<xref ref-type="disp-formula" rid="Ch1.E6"/>) can be solved iteratively for
<inline-formula><mml:math id="M51" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>g</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> through the use of Eq. (<xref ref-type="disp-formula" rid="Ch1.E4"/>). At this point,
the mass-to-size relation <inline-formula><mml:math id="M52" display="inline"><mml:mrow><mml:mi>m</mml:mi><mml:mo>(</mml:mo><mml:mi>D</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> is completely defined. What remains is the
shape<?pagebreak page1560?> parameter for the size distribution. For this, the integral equation
          <disp-formula id="Ch1.E7" content-type="numbered"><mml:math id="M53" display="block"><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>=</mml:mo><mml:munderover><mml:mo movablelimits="false">∫</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mi mathvariant="normal">∞</mml:mi></mml:munderover><mml:mi>m</mml:mi><mml:mo>(</mml:mo><mml:mi>D</mml:mi><mml:mo>)</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msup><mml:mi mathvariant="italic">λ</mml:mi><mml:mrow><mml:mi mathvariant="italic">μ</mml:mi><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow><mml:mrow><mml:mi mathvariant="normal">Γ</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="italic">μ</mml:mi><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>)</mml:mo></mml:mrow></mml:mfrac></mml:mstyle><mml:msup><mml:mi>D</mml:mi><mml:mi mathvariant="italic">μ</mml:mi></mml:msup><mml:msup><mml:mi>e</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mi mathvariant="italic">λ</mml:mi><mml:mi>D</mml:mi></mml:mrow></mml:msup><mml:mtext>d</mml:mtext><mml:mi>D</mml:mi></mml:mrow></mml:math></disp-formula>
        is solved for <inline-formula><mml:math id="M54" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula>. Once all the parameters for <inline-formula><mml:math id="M55" display="inline"><mml:mrow><mml:mi>N</mml:mi><mml:mo>(</mml:mo><mml:mi>D</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M56" display="inline"><mml:mrow><mml:mi>m</mml:mi><mml:mo>(</mml:mo><mml:mi>D</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> are
determined from the predicted model parameters, any size-dependant process
rate can be integrated offline and read back from a lookup table. This is
necessary since the iterative process for finding <inline-formula><mml:math id="M57" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>g</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, solving
Eq. (<xref ref-type="disp-formula" rid="Ch1.E7"/>) for <inline-formula><mml:math id="M58" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula> (or <inline-formula><mml:math id="M59" display="inline"><mml:mi mathvariant="italic">μ</mml:mi></mml:math></inline-formula>) as well as integrating
process rates such as the self-collection of ice particles over the four ice
habit regimes is computationally too expensive to be done online.</p>
      <p id="d1e1687">The weakly constrained parameters in the scheme are the <inline-formula><mml:math id="M60" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mi mathvariant="normal">va</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>
and <inline-formula><mml:math id="M61" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">va</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> parameters in the <inline-formula><mml:math id="M62" display="inline"><mml:mrow><mml:mi>m</mml:mi><mml:mo>(</mml:mo><mml:mi>D</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> relation as well as the
parameters describing the projected area <inline-formula><mml:math id="M63" display="inline"><mml:mrow><mml:mi>A</mml:mi><mml:mo>(</mml:mo><mml:mi>D</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> which is essential for the
microphysical process rate calculations. The sensitivity to the involved
parameter choices in the global context of CAM5 is elaborated in a recent
publication by <xref ref-type="bibr" rid="bib1.bibx7" id="text.26"/>.</p>
      <p id="d1e1743">For this study we implemented the lookup table closely following the original
P3 scheme and the empirical constants used therein.</p>
</sec>
<sec id="Ch1.S3">
  <title>Description of the cloud microphysics scheme</title>
      <p id="d1e1752">We developed a new cloud microphysics scheme in the framework of ECHAM6-HAM2 (echam6.3.0-ham2.3-moz1.0) <xref ref-type="bibr" rid="bib1.bibx53 bib1.bibx42" id="paren.27"/>. The
original cloud microphysics scheme solves prognostic equations for the mass
mixing ratios of cloud liquid and ice <xref ref-type="bibr" rid="bib1.bibx25" id="paren.28"/>. Snow and rain are
diagnosed from the cloud mass mixing ratios of the respective phase. Over the
years, this scheme was expanded to improve the representation of
microphysical processes by adding prognostic equations for the number
concentrations for cloud droplets and ice crystals
<xref ref-type="bibr" rid="bib1.bibx26 bib1.bibx22" id="paren.29"/>. Conversion rates involving the ice phase
date back to <xref ref-type="bibr" rid="bib1.bibx21" id="text.30"/> and <xref ref-type="bibr" rid="bib1.bibx35" id="text.31"/>. Our inclusion of a
completely new approach to describe ice properties brought changes to many
parameterizations and required a complete restructuring of the code to allow
for temporal sub-stepping. The following will describe the implementation of
the microphysics scheme with a single-category ice phase.</p>
      <p id="d1e1770">The snow category has been removed and instead, in addition to ice mass and
number, the riming mass and riming volume are introduced to make up the four-moment single-category ice described in MM15. Except for the restructuring of
the code explained in Sect. <xref ref-type="sec" rid="Ch1.S3.SS1"/>, the two-category
description of the liquid phase has not changed. With the goal of better
representing the supercooled liquid fraction, we changed the way the
Wegener–Bergeron–Findeisen (WBF) process was parameterized. The original
scheme did not allow deposition and condensation to occur simultaneously but
parameterized the WBF process based on whether or not the sub-grid-scale
updraft velocity and hence cooling rates caused super- or subsaturation
with regard to liquid water <xref ref-type="bibr" rid="bib1.bibx19" id="paren.32"/>.</p>
<sec id="Ch1.S3.SS1">
  <title>Code structure</title>
      <p id="d1e1783">To better understand the model integration, consider a cloud parameter
<inline-formula><mml:math id="M64" display="inline"><mml:mi mathvariant="italic">ϕ</mml:mi></mml:math></inline-formula>. This represents any of the prognostic parameters used in this scheme,
e.g., cloud ice <inline-formula><mml:math id="M65" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> or cloud liquid <inline-formula><mml:math id="M66" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. The model then
solves the equation
            <disp-formula id="Ch1.E8" content-type="numbered"><mml:math id="M67" display="block"><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>+</mml:mo><mml:mi mathvariant="bold-italic">u</mml:mi><mml:mo>⋅</mml:mo><mml:mi mathvariant="normal">∇</mml:mi><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mo>=</mml:mo><mml:msub><mml:mfenced close="|" open=""><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mi mathvariant="normal">micro</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mfenced close="|" open=""><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mi mathvariant="normal">vdiff</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mfenced open="" close="|"><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mi mathvariant="normal">convection</mml:mi></mml:msub><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
          where the left-hand side represents the resolved advection and the right-hand side the unresolved processes that need to be parameterized. The
tendencies due to the microphysics routine are summarized here by
<inline-formula><mml:math id="M68" display="inline"><mml:mrow><mml:msub><mml:mfenced close="|" open=""><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mo>/</mml:mo><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfenced><mml:mi mathvariant="normal">micro</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. The tendencies
<inline-formula><mml:math id="M69" display="inline"><mml:mrow><mml:msub><mml:mfenced open="" close="|"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mo>/</mml:mo><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfenced><mml:mi mathvariant="normal">vdiff</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M70" display="inline"><mml:mrow><mml:msub><mml:mfenced close="|" open=""><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mo>/</mml:mo><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfenced><mml:mi mathvariant="normal">convection</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> are calculated by ECHAM6-HAM2's vertical
diffusion and convection modules <xref ref-type="bibr" rid="bib1.bibx42" id="paren.33"/>. Cloud microphysics
modules not only include phase changes and aggregation processes but also
the vertical advection of precipitation. For the prognostic treatment of
precipitation, this aspect has strong implications for the accuracy and
performance of the scheme. To this end, we separate the cloud processes from
the prognostic advection of cloud ice. As will be elaborated carefully in
Sect. <xref ref-type="sec" rid="Ch1.S4"/>, this allows us to employ a two-step reduction in the
global model time step to (1) sufficiently resolve the computationally heavy
cloud process calculations and (2) to achieve numerical stability for the
vertical advection of cloud ice. This separation is shown in
Fig. <xref ref-type="fig" rid="Ch1.F2"/> by the local update boxes separating the
calculation of cloud processes and sedimentation. In terms of
the arbitrary cloud parameter <inline-formula><mml:math id="M71" display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi>n</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula> at time step <inline-formula><mml:math id="M72" display="inline"><mml:mi>n</mml:mi></mml:math></inline-formula>, the workflow of a
single microphysics sub-step can be expressed as

                <disp-formula specific-use="align" content-type="numbered"><mml:math id="M73" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E9"><mml:mtd/><mml:mtd><mml:mstyle displaystyle="true" class="stylechange"/></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mo>=</mml:mo><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi>n</mml:mi></mml:msup><mml:mo>+</mml:mo><mml:msub><mml:mfenced close="|" open=""><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi>n</mml:mi></mml:msup></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mi mathvariant="normal">cloud</mml:mi></mml:msub><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mtr><mml:mtd><mml:mstyle displaystyle="true" class="stylechange"/></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mrow><mml:mi>n</mml:mi><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup><mml:mo>=</mml:mo><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mo>+</mml:mo><mml:msub><mml:mfenced open="" close="|"><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mi mathvariant="normal">sed</mml:mi></mml:msub><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi><mml:mo>.</mml:mo></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:math></disp-formula>

            The entire scheme then consists out of <inline-formula><mml:math id="M74" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mi mathvariant="normal">out</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> iterations of
Eq. (<xref ref-type="disp-formula" rid="Ch1.E9"/>) where the calculation of the sedimentation tendency
is done iteratively as well. This iterative process is shown in
Fig. <xref ref-type="fig" rid="Ch1.F2"/>. The cloud process tendency is given by

                <disp-formula specific-use="align" content-type="numbered"><mml:math id="M75" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E10"><mml:mtd/><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:msub><mml:mfenced open="" close="|"><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mi mathvariant="normal">cloud</mml:mi></mml:msub></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mo>=</mml:mo><mml:msub><mml:mfenced open="" close="|"><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mi mathvariant="normal">iaccl</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mfenced close="|" open=""><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mi mathvariant="normal">islf</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mfenced open="" close="|"><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mi mathvariant="normal">raccc</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mfenced close="|" open=""><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mi mathvariant="normal">cautr</mml:mi></mml:msub></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mtr><mml:mtd><mml:mstyle displaystyle="true" class="stylechange"/></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:mo>+</mml:mo><mml:msub><mml:mfenced open="" close="|"><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mrow><mml:mi mathvariant="normal">e</mml:mi><mml:mo>/</mml:mo><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mfenced open="" close="|"><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mrow><mml:mi mathvariant="normal">c</mml:mi><mml:mo>/</mml:mo><mml:mi mathvariant="normal">d</mml:mi></mml:mrow></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mfenced open="" close="|"><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mi mathvariant="normal">act</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mfenced close="|" open=""><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mi mathvariant="normal">ci</mml:mi></mml:msub></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd><mml:mstyle displaystyle="true" class="stylechange"/></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:mo>+</mml:mo><mml:msub><mml:mfenced close="|" open=""><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mi mathvariant="normal">mlt</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mfenced close="|" open=""><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mi mathvariant="normal">frz</mml:mi></mml:msub><mml:mo>.</mml:mo></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:math></disp-formula>

           <?pagebreak page1561?> The individual terms are discussed in detail below. The abbreviations are as follows:</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F2"><label>Figure 2</label><caption><p id="d1e2344">Flow diagram of the new scheme. The scheme is divided into three major
parts: cloud processes, sedimentation and diagnostics.
The model state is symbolized by <inline-formula><mml:math id="M76" display="inline"><mml:mi mathvariant="italic">ϕ</mml:mi></mml:math></inline-formula> as in the text. Arrows represent the
workflow (solid) and sub-stepping (dashed). The box labeled vertical
loop represents the part of the code that is looped vertically for the
diagnostic treatment of rain. The parameters <inline-formula><mml:math id="M77" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mi mathvariant="normal">in</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and
<inline-formula><mml:math id="M78" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mi mathvariant="normal">out</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> refer to the number of iterations of the inner and outer
loop, respectively. The red numbers on the left represent the approximate
computation times of the respective parts in arbitrary units.</p></caption>
          <?xmltex \igopts{width=213.395669pt}?><graphic xlink:href="https://gmd.copernicus.org/articles/11/1557/2018/gmd-11-1557-2018-f02.png"/>

        </fig>

      <p id="d1e2382"><list list-type="bullet">
            <list-item>

      <p id="d1e2387">“iaccl”, accretion of liquid by ice</p>
            </list-item>
            <list-item>

      <p id="d1e2393">“islf”, self-collection of ice</p>
            </list-item>
            <list-item>

      <p id="d1e2399">“cautr” and “raccc”
auto-conversion and accretion of cloud
droplets to rain</p>
            </list-item>
            <list-item>

      <p id="d1e2405">“e/s”, below-cloud sublimation of rain and sedimenting ice</p>
            </list-item>
            <list-item>

      <p id="d1e2411">“c/d”, cloud formation and dissipation in response to large-scale forcing</p>
            </list-item>
            <list-item>

      <p id="d1e2418">“act”, activation of aerosol particles to cloud droplets</p>
            </list-item>
            <list-item>

      <p id="d1e2424">“ci”, nucleation and deposition in cirrus clouds allowing supersaturation with respect to ice</p>
            </list-item>
            <list-item>

      <p id="d1e2430">“mlt”, melting of ice</p>
            </list-item>
            <list-item>

      <p id="d1e2436">“frz”, homogeneous and heterogeneous freezing of cloud droplets.</p>
            </list-item>
          </list></p>
      <p id="d1e2441">Equation (<xref ref-type="disp-formula" rid="Ch1.E10"/>) is in strong contrast to the original
scheme. Due to the long time step of the global model, cloud processes have
been calculated sequentially. This allowed us to represent a full cloud
life cycle within one time step; from condensation/deposition to collisions
and freezing/melting to evaporation/sublimation or precipitation formation.
With the sub-stepping introduced to resolve the vertical advection of cloud
ice, the new scheme also resolves the life cycle of rather short-lived clouds
and hence does not need to introduce a specific order in which the cloud
processes occur.</p>
      <p id="d1e2447">In practice, the tendencies for cirrus nucleation and deposition <inline-formula><mml:math id="M79" display="inline"><mml:mrow><mml:msub><mml:mfenced close="|" open=""><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mo>/</mml:mo><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfenced><mml:mi mathvariant="normal">ci</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and cloud droplet activation <inline-formula><mml:math id="M80" display="inline"><mml:mrow><mml:msub><mml:mfenced open="" close="|"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mo>/</mml:mo><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfenced><mml:mi mathvariant="normal">act</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> are currently computed before the outer
loop for two reasons. Both parameterizations are based on the time rate of
change in supersaturation within an adiabatic parcel ascent. Particle
formation depends on the maximal supersaturation that can be reached before
condensational/depositional growth quickly depletes all supersaturation
established by cooling. Such parameterizations are designed for global models
where the time step is large enough, such that the entire process from parcel
ascent to particle formation and subsequent depletion of supersaturation
takes place within a single time step. With a reduced time step, this
assumption does no longer hold. Furthermore, ECHAM6-HAM2 is designed in a
modular way. Therefore, aerosol-related particle formation is not calculated
within the cloud microphysics module but as part of the aerosol module HAM2
and a separate cirrus module. This approach allows us to choose the appropriate
scheme for different applications and decouples the development of different
modules by specifying a coupling interface.</p>
      <p id="d1e2492">In the following subsections the parameterizations used to calculate the
individual terms in Eq. (<xref ref-type="disp-formula" rid="Ch1.E10"/>) are presented.</p>
</sec>
<sec id="Ch1.S3.SS2">
  <title>Cloud processes</title>
<sec id="Ch1.S3.SS2.SSS1">
  <title>Cloud formation and dissipation</title>
      <p id="d1e2508">Condensation and deposition can occur
before grid-box mean supersaturation is established. The formation and
dissipation of a cloud depends on the convergence and divergence of specific
humidity and temperature <xref ref-type="bibr" rid="bib1.bibx46" id="paren.34"/>. The fractional cloud cover
<inline-formula><mml:math id="M81" display="inline"><mml:mi>b</mml:mi></mml:math></inline-formula> is related to the relative humidity, RH:
              <disp-formula id="Ch1.E11" content-type="numbered"><mml:math id="M82" display="block"><mml:mrow><mml:mi>b</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:msqrt><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="normal">RH</mml:mi><mml:mo>-</mml:mo><mml:msub><mml:mi mathvariant="normal">RH</mml:mi><mml:mtext>c</mml:mtext></mml:msub></mml:mrow><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:msub><mml:mi mathvariant="normal">RH</mml:mi><mml:mtext>c</mml:mtext></mml:msub></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:msqrt><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
            where <inline-formula><mml:math id="M83" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="normal">RH</mml:mi><mml:mtext>c</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is a threshold grid-box mean relative humidity that has
to be exceeded for cloud formation to be initiated. The previous microphysics
scheme used a threshold ice mass mixing ratio to decide whether to use the
relative humidity<?pagebreak page1562?> with regard to ice or liquid. However, this approach handles
glaciation of a cloud poorly and leads to a sudden increase in cloud cover
once the threshold is exceeded. To circumvent this problem, we introduce a
saturation-specific humidity
              <disp-formula id="Ch1.E12" content-type="numbered"><mml:math id="M84" display="block"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>s</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mi>f</mml:mi><mml:msub><mml:mi>q</mml:mi><mml:mtext>s,l</mml:mtext></mml:msub><mml:mo>+</mml:mo><mml:mo>(</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:mi>f</mml:mi><mml:mo>)</mml:mo><mml:msub><mml:mi>q</mml:mi><mml:mtext>s,i</mml:mtext></mml:msub></mml:mrow></mml:math></disp-formula>
            throughout the mixed-phase cloud regime, i.e., the temperature range from
<inline-formula><mml:math id="M85" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">35</mml:mn></mml:mrow></mml:math></inline-formula> to 0 <inline-formula><mml:math id="M86" display="inline"><mml:mrow class="unit"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup><mml:mi mathvariant="normal">C</mml:mi></mml:mrow></mml:math></inline-formula>. The parameter <inline-formula><mml:math id="M87" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula> is a weighting function,
with <inline-formula><mml:math id="M88" display="inline"><mml:mrow><mml:mi>f</mml:mi><mml:mo>(</mml:mo><mml:mo>-</mml:mo><mml:mn mathvariant="normal">35</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mrow class="unit"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup><mml:mi mathvariant="normal">C</mml:mi></mml:mrow><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M89" display="inline"><mml:mrow><mml:mi>f</mml:mi><mml:mo>(</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mrow class="unit"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup><mml:mi mathvariant="normal">C</mml:mi></mml:mrow><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula>,
and <inline-formula><mml:math id="M90" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>s,l/i</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is the saturation-specific humidities over liquid and
ice. With that, an interpolated relative humidity <inline-formula><mml:math id="M91" display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="normal">RH</mml:mi><mml:mo>*</mml:mo></mml:msup><mml:mo>=</mml:mo><mml:mi>q</mml:mi><mml:mo>/</mml:mo><mml:msub><mml:mi>q</mml:mi><mml:mtext>s</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is inserted into equation Eq. (<xref ref-type="disp-formula" rid="Ch1.E11"/>) to
calculate the cloud cover.</p>
      <p id="d1e2733">For all microphysics processes, <inline-formula><mml:math id="M92" display="inline"><mml:mi>b</mml:mi></mml:math></inline-formula> is used to calculate the in-cloud values,
e.g., <inline-formula><mml:math id="M93" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>i</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mover accent="true"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>/</mml:mo><mml:mi>b</mml:mi></mml:mrow></mml:math></inline-formula> where <inline-formula><mml:math id="M94" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is the variable
used for in-cloud processes and <inline-formula><mml:math id="M95" display="inline"><mml:mover accent="true"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> is the grid-box mean
value.</p>
      <p id="d1e2794">Sedimenting ice and rain, which are allowed to fall into cloud-free layers
where <inline-formula><mml:math id="M96" display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="normal">RH</mml:mi><mml:mo>*</mml:mo></mml:msup><mml:mo>&lt;</mml:mo><mml:msub><mml:mi mathvariant="normal">RH</mml:mi><mml:mtext>c</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, use a sedimentation cover based on the
cloud cover of the precipitating cloud. The sedimentation cover <inline-formula><mml:math id="M97" display="inline"><mml:mrow><mml:msub><mml:mi>b</mml:mi><mml:mtext>sed</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is
simply diagnosed as the cloud cover at the base of the next cloud above.</p>
      <p id="d1e2826">The water mass <inline-formula><mml:math id="M98" display="inline"><mml:mi>Q</mml:mi></mml:math></inline-formula> that is available for condensation/deposition (or required
to evaporate/sublimate) is given by
              <disp-formula id="Ch1.E13" content-type="numbered"><mml:math id="M99" display="block"><mml:mrow><mml:mi>Q</mml:mi><mml:mo>=</mml:mo><mml:mo>-</mml:mo><mml:mi>b</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>q</mml:mi><mml:mtext>f</mml:mtext></mml:msub><mml:mo>-</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>q</mml:mi><mml:mtext>s</mml:mtext></mml:msub><mml:mo>)</mml:mo><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
            where <inline-formula><mml:math id="M100" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>q</mml:mi><mml:mtext>f</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is the moisture convergence in the grid box by the
resolved transport and <inline-formula><mml:math id="M101" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>q</mml:mi><mml:mtext>s</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is the change in saturation-specific
humidity due to heat advection, which includes the change given by the
Clausius–Clapeyron equation as well as the temperature dependence of the
weighting function <inline-formula><mml:math id="M102" display="inline"><mml:mrow><mml:mi>f</mml:mi><mml:mo>(</mml:mo><mml:mi>T</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>.</p>
      <p id="d1e2914">We follow the approach of <xref ref-type="bibr" rid="bib1.bibx32" id="text.35"/> to directly include
the WBF process in mixed-phase clouds and calculate the mass of water that is
able to deposit on the existing ice crystals <xref ref-type="bibr" rid="bib1.bibx27" id="paren.36"/>
              <disp-formula id="Ch1.E14" content-type="numbered"><mml:math id="M103" display="block"><mml:mrow><mml:mi>A</mml:mi><mml:mo>=</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi><mml:msub><mml:mi>N</mml:mi><mml:mtext>i</mml:mtext></mml:msub><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mtext>m</mml:mtext></mml:msub><mml:msub><mml:mi>f</mml:mi><mml:mtext>v</mml:mtext></mml:msub><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mn mathvariant="normal">4</mml:mn><mml:mi mathvariant="italic">π</mml:mi><mml:mi>C</mml:mi><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="normal">RH</mml:mi><mml:mi>i</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>)</mml:mo></mml:mrow><mml:mrow><mml:msubsup><mml:mi>F</mml:mi><mml:mtext>k</mml:mtext><mml:mtext>i</mml:mtext></mml:msubsup><mml:mo>+</mml:mo><mml:msubsup><mml:mi>F</mml:mi><mml:mtext>d</mml:mtext><mml:mtext>i</mml:mtext></mml:msubsup></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
            where <inline-formula><mml:math id="M104" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mtext>m</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:math></inline-formula> is the probability of a water vapor molecule to
successfully be incorporated into an ice crystal, <inline-formula><mml:math id="M105" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi></mml:mrow></mml:math></inline-formula> is the model
time step, and <inline-formula><mml:math id="M106" display="inline"><mml:mi>C</mml:mi></mml:math></inline-formula> is the diameter <inline-formula><mml:math id="M107" display="inline"><mml:mi>D</mml:mi></mml:math></inline-formula>-dependant capacitance of the ice particle
(<inline-formula><mml:math id="M108" display="inline"><mml:mrow><mml:mi>C</mml:mi><mml:mo>=</mml:mo><mml:mi>D</mml:mi></mml:mrow></mml:math></inline-formula> for spherical graupel and <inline-formula><mml:math id="M109" display="inline"><mml:mrow><mml:mi>C</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.48</mml:mn><mml:mi>D</mml:mi></mml:mrow></mml:math></inline-formula> for dendritic particles). The
parameters <inline-formula><mml:math id="M110" display="inline"><mml:mrow><mml:msubsup><mml:mi>F</mml:mi><mml:mtext>k</mml:mtext><mml:mtext>i</mml:mtext></mml:msubsup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M111" display="inline"><mml:mrow><mml:msubsup><mml:mi>F</mml:mi><mml:mtext>d</mml:mtext><mml:mtext>i</mml:mtext></mml:msubsup></mml:mrow></mml:math></inline-formula> are thermodynamic parameters depending only on
temperature. The parameter <inline-formula><mml:math id="M112" display="inline"><mml:mrow><mml:msub><mml:mi>f</mml:mi><mml:mtext>v</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is the ventilation coefficient given by a
parameterization from <xref ref-type="bibr" rid="bib1.bibx49" id="text.37"/> for plate-like ice crystals
              <disp-formula id="Ch1.E15" content-type="numbered"><mml:math id="M113" display="block"><mml:mrow><mml:msub><mml:mi>f</mml:mi><mml:mtext>v</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.65</mml:mn><mml:mo>+</mml:mo><mml:mn mathvariant="normal">0.44</mml:mn><mml:msubsup><mml:mi>N</mml:mi><mml:mrow><mml:mi>S</mml:mi><mml:mi>c</mml:mi></mml:mrow><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>/</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msubsup><mml:msubsup><mml:mi>N</mml:mi><mml:mrow><mml:mi>R</mml:mi><mml:mi>e</mml:mi></mml:mrow><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>/</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msubsup><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
            with the Schmidt number <inline-formula><mml:math id="M114" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mrow><mml:mi>S</mml:mi><mml:mi>c</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> and the Reynolds number <inline-formula><mml:math id="M115" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mrow><mml:mi>R</mml:mi><mml:mi>e</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>. Since both
the Reynolds number <inline-formula><mml:math id="M116" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mrow><mml:mi>R</mml:mi><mml:mi>e</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> and the capacitance <inline-formula><mml:math id="M117" display="inline"><mml:mi>C</mml:mi></mml:math></inline-formula> are size dependant, the
respective summands are integrated offline and read back from the lookup
table. This formulation is identical to the original P3 scheme. For the
relative humidity, it is assumed that <inline-formula><mml:math id="M118" display="inline"><mml:mrow><mml:msub><mml:mtext>RH</mml:mtext><mml:mtext>i</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>q</mml:mi><mml:mtext>s,l</mml:mtext></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>q</mml:mi><mml:mtext>s,i</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> i.e., that the
cloudy portion of the grid box is at water saturation as long as liquid water
is present in mixed-phase clouds. Additionally, it is assumed that ice
crystal growth is prioritized over cloud droplet growth. With those two
assumptions, the following rules determine the condensation and deposition in
mixed-phase clouds.</p>
      <p id="d1e3226">In a cloud-forming environment (<inline-formula><mml:math id="M119" display="inline"><mml:mrow><mml:mi>Q</mml:mi><mml:mo>&gt;</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula>), the mass potentially available for
deposition is the sum of the excess water vapor <inline-formula><mml:math id="M120" display="inline"><mml:mi>Q</mml:mi></mml:math></inline-formula> and the liquid water
<inline-formula><mml:math id="M121" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>c</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>. If <inline-formula><mml:math id="M122" display="inline"><mml:mrow><mml:mi>Q</mml:mi><mml:mo>&lt;</mml:mo><mml:mi>A</mml:mi></mml:mrow></mml:math></inline-formula> the missing water is taken from the liquid phase and thus
represents the WBF process. Otherwise both cloud droplets and ice crystals
grow. In the case of a dissipating cloud (<inline-formula><mml:math id="M123" display="inline"><mml:mrow><mml:mi>Q</mml:mi><mml:mo>&lt;</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula>), cloud droplets evaporate
first and only if <inline-formula><mml:math id="M124" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>c</mml:mtext></mml:msub><mml:mo>&lt;</mml:mo><mml:mi>Q</mml:mi></mml:mrow></mml:math></inline-formula> ice crystals sublimate.</p>
      <p id="d1e3299">The growth and dissipation of pure ice clouds in the mixed-phase regime
follows that dictated by Eq. (<xref ref-type="disp-formula" rid="Ch1.E13"/>) to be consistent with
the cloud fraction in Eq. (<xref ref-type="disp-formula" rid="Ch1.E11"/>). The formation of cirrus
clouds is handled separately and is discussed in the next subsection.</p>
</sec>
<sec id="Ch1.S3.SS2.SSS2">
  <title>Cirrus clouds</title>
      <p id="d1e3312">Homogeneous freezing of solution droplets in cirrus clouds
is considered. Starting at around 140 % RH with respect to ice,
it is evident that the in-cloud deposition discussed in the previous
subsection is not suited to represent such clouds as it does not allow
supersaturation by design. To capture this effect we allow supersaturation
with respect to ice and parameterize cirrus clouds by the scheme described in
<xref ref-type="bibr" rid="bib1.bibx16" id="text.38"/>. It is based on sub-grid updraft velocity inferred
from the turbulent kinetic energy (TKE) to obtain a more physical sub-grid
distribution of saturation values. Vapor deposition is calculated explicitly
based on the supersaturation with regard to ice. Cirrus clouds dissipate the same way
as mixed-phase and liquid clouds.</p>
      <p id="d1e3318">This scheme has two main limitations. Firstly, it does not include
preexisting ice crystals that compete for available humidity with the newly
formed ones. Secondly, the use of the TKE to infer sub-grid updraft
velocities is debatable. A study by <xref ref-type="bibr" rid="bib1.bibx15" id="text.39"/> showed that this
formulation in ECHAM5 did not reproduce the observed updraft velocities and
better agreement with observation was reached by including orographic gravity
waves. A recent study with CAM5 reached better agreement with observations by
only using the large-scale updraft velocity <xref ref-type="bibr" rid="bib1.bibx54" id="paren.40"/>. Improving
the representation of cirrus clouds is work in progress in our group.</p>
</sec>
<sec id="Ch1.S3.SS2.SSS3">
  <title>Aerosol activation</title>
      <p id="d1e3333">The model ECHAM6-HAM2 used in this study is equipped
with the online aerosol model HAM version 2 <xref ref-type="bibr" rid="bib1.bibx53" id="paren.41"/>. Number
concentrations and mass mixing ratios of five<?pagebreak page1563?> aerosol species (sulfate, sea
salt, mineral dust, black carbon and organic carbon) are calculated with the
aerosol module HAM. Aerosol activation is calculated according to
<xref ref-type="bibr" rid="bib1.bibx2" id="text.42"/> and <xref ref-type="bibr" rid="bib1.bibx1" id="text.43"/> considering the
aerosol particle size and chemical composition. The transition from grid-box
mean to the physically relevant sub-grid formulation is done according to the
sub-grid updraft velocity. We apply a correction to cloud droplet number
concentrations if the mass-weighted mean droplet size is unphysically large
because aerosol activation was too weak. For that, we adjust the number
concentration such that a volume mean droplet radius of 25 <inline-formula><mml:math id="M125" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>m
is not exceeded.</p>
</sec>
<sec id="Ch1.S3.SS2.SSS4">
  <title>Freezing of cloud droplets</title>
      <p id="d1e3359">The freezing capabilities of black carbon and mineral
dust are calculated according to the parameterization developed by
<xref ref-type="bibr" rid="bib1.bibx24" id="text.44"/>. It accounts for both contact freezing of mineral
dust and immersion freezing of black carbon and mineral dust in stratiform
mixed-phase clouds.</p>
</sec>
<sec id="Ch1.S3.SS2.SSS5">
  <title>Liquid–ice interactions</title>
      <p id="d1e3372">Collisions between cloud droplets and ice crystals are calculated based on
the ice particle's projected area and fall speed. These properties are part
of the new single-category description of ice and further described in MM15.
The current diagnostic treatment of rain does not allow us to calculate raindrop collection by ice. We assume that this process can be neglected and
riming will be dominated by cloud droplets colliding with ice particles. This
is equivalent to the original microphysics scheme in ECHAM6-HAM2.</p>
</sec>
<sec id="Ch1.S3.SS2.SSS6">
  <title>Ice particle self-collection</title>
      <p id="d1e3381">With the size distribution and projected area to diameter relation intrinsic
to the single-category scheme we are able to numerically integrate the
collection kernel. The resulting process rates are stored and read from
lookup tables. This replaces the aggregation parameterization employed by the
original scheme to calculate the efficiency with which ice crystals collide
to form snow.</p>
</sec>
<sec id="Ch1.S3.SS2.SSS7">
  <title>Below-cloud evaporation/sublimation</title>
      <p id="d1e3390">The evaporation of rain is calculated according to <xref ref-type="bibr" rid="bib1.bibx37" id="text.45"/>. For
ice we use the same formulation for below-cloud sublimation as employed for
deposition by moisture convergence (Eq. <xref ref-type="disp-formula" rid="Ch1.E14"/>), where we use
the grid-box mean subsaturation with respect to ice. This implies that we
neglect a potential subgrid distribution of humidity in completely cloud-free
grid boxes.</p>
</sec>
<sec id="Ch1.S3.SS2.SSS8">
  <title>Melting of ice</title>
      <p id="d1e3404">Melting is calculated based on <xref ref-type="bibr" rid="bib1.bibx30" id="text.46"/>. It combines terms for
condensation, diffusion and riming in a heat-budget equation. Here only
condensation and diffusion are considered:

                  <disp-formula specific-use="align" content-type="numbered"><mml:math id="M126" display="block"><mml:mtable rowspacing="5.690551pt" displaystyle="true"><mml:mlabeledtr id="Ch1.E16"><mml:mtd/><mml:mtd><mml:mstyle class="stylechange" displaystyle="true"/></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:msub><mml:mfenced close="|" open=""><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:msub><mml:mi>q</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mi mathvariant="normal">mlt</mml:mi></mml:msub><mml:mo>=</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mtr><mml:mtd><mml:mstyle class="stylechange" displaystyle="true"/></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:mo>-</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mn mathvariant="normal">2</mml:mn><mml:mi mathvariant="italic">π</mml:mi><mml:mi>D</mml:mi><mml:mo>[</mml:mo><mml:mi>K</mml:mi><mml:mo>(</mml:mo><mml:mi>T</mml:mi><mml:mo>-</mml:mo><mml:msub><mml:mi>T</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub><mml:mo>)</mml:mo><mml:mo>+</mml:mo><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>air</mml:mtext></mml:msub><mml:mi mathvariant="italic">ψ</mml:mi><mml:msub><mml:mi>L</mml:mi><mml:mtext>v</mml:mtext></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mfenced open="" close="|"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi>v</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>q</mml:mi><mml:mtext>s</mml:mtext></mml:msub></mml:mrow></mml:mfenced><mml:mrow><mml:mi>t</mml:mi><mml:mo>=</mml:mo><mml:msub><mml:mi>T</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:msub><mml:mo>)</mml:mo><mml:mo>]</mml:mo><mml:msub><mml:mi>f</mml:mi><mml:mtext>v</mml:mtext></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mi>L</mml:mi><mml:mtext>f</mml:mtext></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:math></disp-formula>

              where <inline-formula><mml:math id="M127" display="inline"><mml:mrow><mml:msub><mml:mi>L</mml:mi><mml:mtext>v/f</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is the latent heat of vaporization and fusion, respectively, <inline-formula><mml:math id="M128" display="inline"><mml:mi>K</mml:mi></mml:math></inline-formula> is the thermal conductivity of air, <inline-formula><mml:math id="M129" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>air</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is
the density of air and <inline-formula><mml:math id="M130" display="inline"><mml:mi mathvariant="italic">ψ</mml:mi></mml:math></inline-formula> is the water vapor diffusivity. The melted
water is added to the cloud water mass within the cloud and to the rain water
mass below the cloud.</p>
</sec>
<sec id="Ch1.S3.SS2.SSS9">
  <title>Cloud droplet auto-conversion and accretion by rain</title>
      <p id="d1e3580">Warm-phase processes are adapted from the original microphysics scheme in
ECHAM6-HAM2 to minimize differences and enhance comparability. The
sedimentation of liquid water is diagnosed by a separate category for rain
that is assumed to fall through the whole column within one single global
time step. Rain is formed by auto-conversion and increased by accretion.
Auto-conversion from cloud water to rain is calculated from the cloud liquid
mass mixing ratio <inline-formula><mml:math id="M131" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>c</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and the number concentration of cloud droplets
<inline-formula><mml:math id="M132" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mtext>c</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> following the empirical relation <xref ref-type="bibr" rid="bib1.bibx18" id="paren.47"/>
              <disp-formula id="Ch1.E17" content-type="numbered"><mml:math id="M133" display="block"><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:msub><mml:mi>q</mml:mi><mml:mtext>r</mml:mtext></mml:msub></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:msub><mml:mo fence="true" mathsize="1.5em">|</mml:mo><mml:mi mathvariant="normal">aut</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1350</mml:mn><mml:msubsup><mml:mi>q</mml:mi><mml:mtext>c</mml:mtext><mml:mn mathvariant="normal">2.47</mml:mn></mml:msubsup><mml:msubsup><mml:mi>N</mml:mi><mml:mtext>c</mml:mtext><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.79</mml:mn></mml:mrow></mml:msubsup><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
            where <inline-formula><mml:math id="M134" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>r</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is the rain mass mixing ratio. Rain falling from above is
also able to grow by accretion of cloud droplets following
              <disp-formula id="Ch1.E18" content-type="numbered"><mml:math id="M135" display="block"><mml:mrow><mml:msub><mml:mfenced close="|" open=""><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:msub><mml:mi>q</mml:mi><mml:mtext>r</mml:mtext></mml:msub></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mi mathvariant="normal">acc</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">3.7</mml:mn><mml:msub><mml:mi>q</mml:mi><mml:mtext>c</mml:mtext></mml:msub><mml:msub><mml:mi>q</mml:mi><mml:mtext>r</mml:mtext></mml:msub><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>
            The rain flux is then given by <xref ref-type="bibr" rid="bib1.bibx42" id="paren.48"/>
              <disp-formula id="Ch1.E19" content-type="numbered"><mml:math id="M136" display="block"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">rain</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mn mathvariant="normal">1</mml:mn><mml:mi>g</mml:mi></mml:mfrac></mml:mstyle><mml:munderover><mml:mo movablelimits="false">∫</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mi>p</mml:mi></mml:munderover><mml:mo>(</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">aut</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">acc</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">mlt</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">evp</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:mtext>d</mml:mtext><mml:mi>p</mml:mi></mml:mrow></mml:math></disp-formula>
            for pressure <inline-formula><mml:math id="M137" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula> and the source and sink terms of auto-conversion from cloud
droplets to rain <inline-formula><mml:math id="M138" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">aut</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mfenced close="|" open=""><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mrow><mml:mo>∂</mml:mo><mml:msub><mml:mi>q</mml:mi><mml:mtext>r</mml:mtext></mml:msub></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mi mathvariant="normal">aut</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, accretion of cloud droplets by rain
<inline-formula><mml:math id="M139" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">acc</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mfenced open="" close="|"><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mrow><mml:mo>∂</mml:mo><mml:msub><mml:mi>q</mml:mi><mml:mtext>r</mml:mtext></mml:msub></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mfenced><mml:mi mathvariant="normal">acc</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, melting of ice <inline-formula><mml:math id="M140" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">mlt</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and evaporation of
rain <inline-formula><mml:math id="M141" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">evp</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. Given the precipitation velocity of rain, the rain
mass mixing ratio <inline-formula><mml:math id="M142" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>r</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> used for the accretion rate can be calculated
from the rain flux <inline-formula><mml:math id="M143" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">rain</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>.</p>
</sec>
</sec>
<sec id="Ch1.S3.SS3">
  <title>Sedimentation</title>
<sec id="Ch1.S3.SS3.SSS1">
  <title>Falling ice</title>
      <p id="d1e3903">Sedimentation of ice is calculated prognostically according to MM15. The rate
of change due to sedimentation is deduced from the number-weighted mean
(<inline-formula><mml:math id="M144" display="inline"><mml:mrow><mml:msub><mml:mi>v</mml:mi><mml:mtext>n</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>) and mass-weighted mean (<inline-formula><mml:math id="M145" display="inline"><mml:mrow><mml:msub><mml:mi>v</mml:mi><mml:mtext>m</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>) fall speeds

                  <disp-formula specific-use="align" content-type="numbered"><mml:math id="M146" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E20"><mml:mtd/><mml:mtd><mml:mstyle displaystyle="true" class="stylechange"/></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:msub><mml:mi>v</mml:mi><mml:mtext>n</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msubsup><mml:mo>∫</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mi mathvariant="normal">∞</mml:mi></mml:msubsup><mml:mi>v</mml:mi><mml:mo>(</mml:mo><mml:mi>D</mml:mi><mml:mo>)</mml:mo><mml:mi>N</mml:mi><mml:mo>(</mml:mo><mml:mi>D</mml:mi><mml:mo>)</mml:mo><mml:mtext>d</mml:mtext><mml:mi>D</mml:mi></mml:mrow><mml:mrow><mml:msubsup><mml:mo>∫</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mi mathvariant="normal">∞</mml:mi></mml:msubsup><mml:mi>N</mml:mi><mml:mo>(</mml:mo><mml:mi>D</mml:mi><mml:mo>)</mml:mo><mml:mtext>d</mml:mtext><mml:mi>D</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E21"><mml:mtd/><mml:mtd><mml:mstyle class="stylechange" displaystyle="true"/></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:msub><mml:mi>v</mml:mi><mml:mtext>m</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msubsup><mml:mo>∫</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mi mathvariant="normal">∞</mml:mi></mml:msubsup><mml:mi>v</mml:mi><mml:mo>(</mml:mo><mml:mi>D</mml:mi><mml:mo>)</mml:mo><mml:mi>m</mml:mi><mml:mo>(</mml:mo><mml:mi>D</mml:mi><mml:mo>)</mml:mo><mml:mi>N</mml:mi><mml:mo>(</mml:mo><mml:mi>D</mml:mi><mml:mo>)</mml:mo><mml:mtext>d</mml:mtext><mml:mi>D</mml:mi></mml:mrow><mml:mrow><mml:msubsup><mml:mo>∫</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mi mathvariant="normal">∞</mml:mi></mml:msubsup><mml:mi>m</mml:mi><mml:mo>(</mml:mo><mml:mi>D</mml:mi><mml:mo>)</mml:mo><mml:mi>N</mml:mi><mml:mo>(</mml:mo><mml:mi>D</mml:mi><mml:mo>)</mml:mo><mml:mtext>d</mml:mtext><mml:mi>D</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>.</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula>

             <?pagebreak page1564?> The fall speeds are computed offline and are read back from lookup tables.</p>
      <p id="d1e4083">The rate of change due to sedimentation is given by a one-dimensional
advection equation:
              <disp-formula id="Ch1.E22" content-type="numbered"><mml:math id="M147" display="block"><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>+</mml:mo><mml:msub><mml:mi>v</mml:mi><mml:mtext>m/n</mml:mtext></mml:msub><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>z</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
            where <inline-formula><mml:math id="M148" display="inline"><mml:mi mathvariant="italic">ϕ</mml:mi></mml:math></inline-formula> represents the ice moments: number – <inline-formula><mml:math id="M149" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, ice –
<inline-formula><mml:math id="M150" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, rimed ice – <inline-formula><mml:math id="M151" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>rim</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and volume mixing ratio –
<inline-formula><mml:math id="M152" display="inline"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mtext>rim</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>. The number mixing ratio sediments according to the
number-weighted mean fall speed <inline-formula><mml:math id="M153" display="inline"><mml:mrow><mml:msub><mml:mi>v</mml:mi><mml:mtext>n</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, the other three according to
the mass-weighted mean fall speed <inline-formula><mml:math id="M154" display="inline"><mml:mrow><mml:msub><mml:mi>v</mml:mi><mml:mtext>m</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>.</p>
      <p id="d1e4203">Given the long time step of a global model, large errors will arise in the
vertical advection of cloud ice. Therefore, sub-stepping was applied to the
relevant part. This will be further explained in Sect. <xref ref-type="sec" rid="Ch1.S4"/>.</p>
</sec>
</sec>
</sec>
<sec id="Ch1.S4">
  <title>Treating prognostic sedimentation efficiently</title>
      <p id="d1e4217">The standard version of ECHAM6-HAM2 diagnoses precipitation assuming that it
reaches the surface within one global model time step. Treating sedimentation
prognostically requires much smaller time steps to resolve the vertical
motion of hydrometeors. We therefore introduce temporal sub-stepping in the
microphysics and sedimentation calculations in order to achieve numerical
stability and keep numerical errors small.</p>
      <p id="d1e4220">The perfect integration method to solve the vertical advection equation for
sedimenting ice (Eq. <xref ref-type="disp-formula" rid="Ch1.E22"/>) should be non-dispersive,
unconditionally stable and able to deal with sharp wave fronts usually
encountered at the cloud base and cloud top. Unfortunately, this integration
method does not exist. Here, we use the upstream version of an explicit Euler
method, which leads to the following discretization of
Eq. (<xref ref-type="disp-formula" rid="Ch1.E22"/>):

              <disp-formula specific-use="align" content-type="numbered"><mml:math id="M155" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E23"><mml:mtd/><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:msubsup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi>k</mml:mi><mml:mrow><mml:mi>n</mml:mi><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msubsup></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:mo>=</mml:mo><mml:msubsup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi>k</mml:mi><mml:mi>n</mml:mi></mml:msubsup><mml:mo>+</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi><mml:mfenced close=")" open="("><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msubsup><mml:mi>v</mml:mi><mml:mrow><mml:mi>k</mml:mi><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow><mml:mi>n</mml:mi></mml:msubsup><mml:msubsup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mrow><mml:mi>k</mml:mi><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow><mml:mi>n</mml:mi></mml:msubsup></mml:mrow><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>z</mml:mi><mml:mrow><mml:mi>k</mml:mi><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>-</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msubsup><mml:mi>v</mml:mi><mml:mi>k</mml:mi><mml:mi>n</mml:mi></mml:msubsup><mml:msubsup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi>k</mml:mi><mml:mi>n</mml:mi></mml:msubsup></mml:mrow><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>z</mml:mi><mml:mi>k</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:mfenced></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mtr><mml:mtd><mml:mstyle displaystyle="true" class="stylechange"/></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:mo>=</mml:mo><mml:msubsup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi>k</mml:mi><mml:mi>n</mml:mi></mml:msubsup><mml:mo>+</mml:mo><mml:msubsup><mml:mi mathvariant="italic">α</mml:mi><mml:mrow><mml:mi>k</mml:mi><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow><mml:mi>n</mml:mi></mml:msubsup><mml:msubsup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mrow><mml:mi>k</mml:mi><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow><mml:mi>n</mml:mi></mml:msubsup><mml:mo>-</mml:mo><mml:msubsup><mml:mi mathvariant="italic">α</mml:mi><mml:mi>k</mml:mi><mml:mi>n</mml:mi></mml:msubsup><mml:msubsup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi>k</mml:mi><mml:mi>n</mml:mi></mml:msubsup><mml:mo>.</mml:mo></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:math></disp-formula>

          Indices <inline-formula><mml:math id="M156" display="inline"><mml:mi>n</mml:mi></mml:math></inline-formula> represent the <inline-formula><mml:math id="M157" display="inline"><mml:mi>n</mml:mi></mml:math></inline-formula>th time step and indices <inline-formula><mml:math id="M158" display="inline"><mml:mi>k</mml:mi></mml:math></inline-formula> represent the <inline-formula><mml:math id="M159" display="inline"><mml:mi>k</mml:mi></mml:math></inline-formula>th
model level. We introduced the Courant–Friedrich–Lewy (CFL) number
<inline-formula><mml:math id="M160" display="inline"><mml:mrow><mml:mi mathvariant="italic">α</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:mi>v</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi><mml:mo>/</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>z</mml:mi></mml:mrow></mml:math></inline-formula> because it is a useful quantity to
assess the numerical stability of a method. It can be interpreted as the
number of levels that are passed within a time interval <inline-formula><mml:math id="M161" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi></mml:mrow></mml:math></inline-formula>. This
scheme is stable for <inline-formula><mml:math id="M162" display="inline"><mml:mrow><mml:mi mathvariant="italic">α</mml:mi><mml:mo>&lt;</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula> and dispersive for large time steps. In the
following we will present a method exploiting the sequential treatment of
cloud processes and sedimentation to ensure numerical stability and
reasonable accuracy while reaching optimal model performance.</p>
<sec id="Ch1.S4.SS1">
  <title>The optimization strategy</title>
      <p id="d1e4483">In this section we present an approach to find a compromise between
computational efficiency and model accuracy. The goal is to increase model
efficiency by distributing the workload between the two parts shown in
Fig. <xref ref-type="fig" rid="Ch1.F2"/>: the computationally expensive outer loop with
<inline-formula><mml:math id="M163" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mi mathvariant="normal">out</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> iterations calculating both cloud process rates and
sedimentation and the computationally cheap inner loop with <inline-formula><mml:math id="M164" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mi mathvariant="normal">in</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>
iterations calculating only the sedimentation of cloud ice. Sedimentation is
calculated roughly 100 times faster than the cloud processes. Since the loops
are nested, the number of calls to the sedimentation calculation will be
<inline-formula><mml:math id="M165" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mi mathvariant="normal">tot</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>n</mml:mi><mml:mi mathvariant="normal">out</mml:mi></mml:msub><mml:mo>×</mml:mo><mml:msub><mml:mi>n</mml:mi><mml:mi mathvariant="normal">in</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, reducing the
time step in the sedimentation calculation and cloud processes to <inline-formula><mml:math id="M166" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>t</mml:mi><mml:mi mathvariant="normal">in</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi><mml:mo>/</mml:mo><mml:msub><mml:mi>n</mml:mi><mml:mi mathvariant="normal">tot</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M167" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>t</mml:mi><mml:mi mathvariant="normal">out</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi><mml:mo>/</mml:mo><mml:msub><mml:mi>n</mml:mi><mml:mi mathvariant="normal">out</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, respectively. To achieve
numerical stability, we calculate the required number of sub-steps
<inline-formula><mml:math id="M168" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mi mathvariant="normal">tot</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> online to achieve <inline-formula><mml:math id="M169" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mi>k</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>t</mml:mi><mml:mi mathvariant="normal">in</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:msub><mml:mi>v</mml:mi><mml:mi>k</mml:mi></mml:msub><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>t</mml:mi><mml:mi mathvariant="normal">in</mml:mi></mml:msub><mml:mo>/</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>z</mml:mi><mml:mi>k</mml:mi></mml:msub><mml:mo>&lt;</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula> for every level <inline-formula><mml:math id="M170" display="inline"><mml:mi>k</mml:mi></mml:math></inline-formula>. This
requirement could be relaxed for an implicit scheme which is stable even for
<inline-formula><mml:math id="M171" display="inline"><mml:mrow><mml:mi mathvariant="italic">α</mml:mi><mml:mo>&gt;</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula>. Since the outer loop is so much slower than the inner, the
restriction to <inline-formula><mml:math id="M172" display="inline"><mml:mrow><mml:mi mathvariant="italic">α</mml:mi><mml:mo>&lt;</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula> is not our main concern because it can easily be
achieved by the inner loop. This leads to the following expression for
<inline-formula><mml:math id="M173" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mi mathvariant="normal">tot</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> on <inline-formula><mml:math id="M174" display="inline"><mml:mi>N</mml:mi></mml:math></inline-formula> model levels:
            <disp-formula id="Ch1.E24" content-type="numbered"><mml:math id="M175" display="block"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mi mathvariant="normal">tot</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:munder><mml:mi mathvariant="normal">max</mml:mi><mml:mrow><mml:mi>k</mml:mi><mml:mo>∈</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>,</mml:mo><mml:mi mathvariant="normal">…</mml:mi><mml:mo>,</mml:mo><mml:mi>N</mml:mi></mml:mrow></mml:munder><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mi>k</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi><mml:mo>)</mml:mo><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula></p>
      <p id="d1e4744">The calculation of the process rates is not subject to the same restrictions
as sedimentation. However, if we only use the inner loop
(<inline-formula><mml:math id="M176" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mi mathvariant="normal">out</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula>) to achieve numerical stability, we will not be able to
represent the process rates acting on falling particles and impair model
accuracy. On the other hand, if we set <inline-formula><mml:math id="M177" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mi mathvariant="normal">in</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula>, we will have to
achieve numerical stability solely by the expensive outer loop and impair
computational efficiency.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F3" specific-use="star"><label>Figure 3</label><caption><p id="d1e4779">Illustration of the optimization approach. Grey horizontal lines
show the level interfaces. <bold>(a)</bold> Cloud ice against height;
<bold>(b)</bold> fall speed (orange; top axis), residence times (green; bottom
axis; per level) and accumulated residence time (purple; bottom axis;
accumulated from the bottom). Residence times are given as a fraction of the
global time step <inline-formula><mml:math id="M178" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi></mml:mrow></mml:math></inline-formula>. Colored bars show the levels below which ice
only spends a fraction <inline-formula><mml:math id="M179" display="inline"><mml:mi>x</mml:mi></mml:math></inline-formula> of the time step. <bold>(c)</bold> CFL number
<inline-formula><mml:math id="M180" display="inline"><mml:mi mathvariant="italic">α</mml:mi></mml:math></inline-formula>. Colored bars show the set of levels <inline-formula><mml:math id="M181" display="inline"><mml:mrow><mml:msub><mml:mi>I</mml:mi><mml:mtext>out</mml:mtext></mml:msub><mml:mo>(</mml:mo><mml:mi>x</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> considered
for the calculation of <inline-formula><mml:math id="M182" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mi mathvariant="normal">out</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>.</p></caption>
          <?xmltex \igopts{width=426.791339pt}?><graphic xlink:href="https://gmd.copernicus.org/articles/11/1557/2018/gmd-11-1557-2018-f03.png"/>

        </fig>

      <?pagebreak page1565?><p id="d1e4850">We found a compromise between the two extremes by considering the trajectory
of a falling ice crystals. For model accuracy, it is important that the cloud
processes are calculated every time the ice crystals reach a new model level
and are thus exposed to a new environment. This is equivalent to the
requirement <inline-formula><mml:math id="M183" display="inline"><mml:mrow><mml:mi mathvariant="italic">α</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>t</mml:mi><mml:mi mathvariant="normal">out</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:mo>&lt;</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula>. However, if fall speeds are
very high and/or the level is very thin, the total rate of change in cloud
ice will be dominated by sedimentation. Processes like sublimation and
melting will not have enough time to significantly change the cloud ice
content on those levels. Therefore, we neglect the last part of the
trajectory where the ice only spends a fraction of a global model time step
and calculate the number of outer iterations:
            <disp-formula id="Ch1.E25" content-type="numbered"><mml:math id="M184" display="block"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mi mathvariant="normal">out</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mi mathvariant="normal">max</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:munder><mml:mi mathvariant="normal">max</mml:mi><mml:mrow><mml:mi>k</mml:mi><mml:mo>∈</mml:mo><mml:msub><mml:mi>I</mml:mi><mml:mi mathvariant="normal">out</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>x</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:munder><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mi>k</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></disp-formula>
          for the set <inline-formula><mml:math id="M185" display="inline"><mml:mrow><mml:msub><mml:mi>I</mml:mi><mml:mi mathvariant="normal">out</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>x</mml:mi><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:mo mathvariant="italic">{</mml:mo><mml:mi>k</mml:mi><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mo>|</mml:mo><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mi>k</mml:mi><mml:mo>∈</mml:mo><mml:mo mathvariant="italic">{</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>,</mml:mo><mml:mi mathvariant="normal">…</mml:mi><mml:mo>,</mml:mo><mml:mi>N</mml:mi><mml:mo mathvariant="italic">}</mml:mo><mml:mo>∧</mml:mo><mml:mspace linebreak="nobreak" width="0.25em"/><mml:msubsup><mml:mi mathvariant="normal">Σ</mml:mi><mml:mrow><mml:mi>i</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow><mml:mi>k</mml:mi></mml:msubsup><mml:msub><mml:mi mathvariant="italic">τ</mml:mi><mml:mi>k</mml:mi></mml:msub><mml:mo>&gt;</mml:mo><mml:mi>x</mml:mi><mml:mo mathvariant="italic">}</mml:mo></mml:mrow></mml:math></inline-formula> for the time spent on level <inline-formula><mml:math id="M186" display="inline"><mml:mi>k</mml:mi></mml:math></inline-formula>, <inline-formula><mml:math id="M187" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">τ</mml:mi><mml:mi>k</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, a
specified threshold time <inline-formula><mml:math id="M188" display="inline"><mml:mi>x</mml:mi></mml:math></inline-formula> and a model with <inline-formula><mml:math id="M189" display="inline"><mml:mi>N</mml:mi></mml:math></inline-formula> levels. Numerical stability
is then achieved on all levels by using
<inline-formula><mml:math id="M190" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mi mathvariant="normal">in</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>n</mml:mi><mml:mi mathvariant="normal">tot</mml:mi></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>n</mml:mi><mml:mi mathvariant="normal">out</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> inner iterations.</p>
      <p id="d1e5060">We illustrate our approach using the test case properly described in the next
section. For the purpose of this section, the exact model setup is not
important. Given the distribution of cloud ice in
Fig. <xref ref-type="fig" rid="Ch1.F3"/>a and fall speed in Fig. <xref ref-type="fig" rid="Ch1.F3"/>b, we can calculate the time that cloud ice will spend in each level. Since the
thickness of model levels varies from 90 m at the surface to 700 m at
8 km height and since gravitational size sorting and self-collection lead
to the fastest fall speeds close to the surface, <inline-formula><mml:math id="M191" display="inline"><mml:mi mathvariant="italic">α</mml:mi></mml:math></inline-formula> varies from 57 at
the surface to 1 at 8 km (Fig. <xref ref-type="fig" rid="Ch1.F3"/>c). At the same
time the accumulated time spent below a certain height is only a fraction of
a global time step (Fig. <xref ref-type="fig" rid="Ch1.F3"/>b).</p>
      <p id="d1e5078">The colored bars in Fig. <xref ref-type="fig" rid="Ch1.F3"/>c show different choices for
the threshold time <inline-formula><mml:math id="M192" display="inline"><mml:mi>x</mml:mi></mml:math></inline-formula> in units of the global model time step <inline-formula><mml:math id="M193" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi></mml:mrow></mml:math></inline-formula>. Its
value ranges from 0 (orange bar), meaning that the entire trajectory is
considered, to 1 (brown bar), neglecting the part of the trajectory where
ice does not spend at least one global model time step.</p>
      <p id="d1e5100">For the following estimation of the model error, we chose the strategy
corresponding to the purple bar <inline-formula><mml:math id="M194" display="inline"><mml:mrow><mml:msub><mml:mi>I</mml:mi><mml:mi mathvariant="normal">out</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mn mathvariant="normal">0.2</mml:mn><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>. We neglect the last
part of the trajectory where cloud ice spends less than 20 % of
the global model time step. This choice represents a compromise between
performance and accuracy; this will be further elaborated below.</p>
</sec>
<sec id="Ch1.S4.SS2">
  <title>Estimating the model error</title>
      <p id="d1e5126">To demonstrate the power of the sub-stepping described above, we employ a
simple single-column setup with 31 vertical levels. At one single model level
at around 8 km height, a constant ice source term with specified tendencies
for all four ice moments is prescribed at every time step. The source terms are
chosen such that the ice particles reach very high fall speeds, and thus
sub-stepping is fundamentally important. The forcing is representative of
hail formation and thus an extreme case that is probably not produced very
often by the global model. However, it highlights the need for sub-stepping
while the general conclusions are also true for smaller or dendritic
particles.</p>
      <p id="d1e5129">We prescribe the tendencies for cloud ice with <inline-formula><mml:math id="M195" display="inline"><mml:mrow><mml:mo>∂</mml:mo><mml:msub><mml:mi>q</mml:mi><mml:mtext>i</mml:mtext></mml:msub><mml:mo>/</mml:mo><mml:mo>∂</mml:mo><mml:mi>t</mml:mi><mml:mo>=</mml:mo><mml:mo>∂</mml:mo><mml:msub><mml:mi>q</mml:mi><mml:mtext>rim</mml:mtext></mml:msub><mml:mo>/</mml:mo><mml:mo>∂</mml:mo><mml:mi>t</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">5</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>g kg<inline-formula><mml:math id="M196" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> s<inline-formula><mml:math id="M197" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>,
<inline-formula><mml:math id="M198" display="inline"><mml:mrow><mml:mo>∂</mml:mo><mml:msub><mml:mi>n</mml:mi><mml:mi>i</mml:mi></mml:msub><mml:mo>/</mml:mo><mml:mo>∂</mml:mo><mml:mi>t</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> kg<inline-formula><mml:math id="M199" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> s<inline-formula><mml:math id="M200" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> and
<inline-formula><mml:math id="M201" display="inline"><mml:mrow><mml:mo>∂</mml:mo><mml:msub><mml:mi>b</mml:mi><mml:mtext>rim</mml:mtext></mml:msub><mml:mo>/</mml:mo><mml:mo>∂</mml:mo><mml:mi>t</mml:mi><mml:mo>=</mml:mo><mml:mo>∂</mml:mo><mml:msub><mml:mi>q</mml:mi><mml:mtext>rim</mml:mtext></mml:msub><mml:mo>/</mml:mo><mml:mo>∂</mml:mo><mml:mi>t</mml:mi><mml:msubsup><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>rim</mml:mtext><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msubsup></mml:mrow></mml:math></inline-formula>, where we set the rime density to
<inline-formula><mml:math id="M202" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>rim</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">900</mml:mn></mml:mrow></mml:math></inline-formula> kg m<inline-formula><mml:math id="M203" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. This forcing implies a rime fraction
<inline-formula><mml:math id="M204" display="inline"><mml:mrow><mml:msub><mml:mi>F</mml:mi><mml:mtext>r</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula>. The temperature profile is prescribed, constant in time and
decreases linearly from 0 <inline-formula><mml:math id="M205" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C at the ground to <inline-formula><mml:math id="M206" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>55 <inline-formula><mml:math id="M207" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C
at 8 km. Relative humidity is set to 50 % with regard to liquid water. The
relevant microphysical processes are sedimentation, sublimation and
self-collection. The resulting ice profile undergoes a buildup phase until
it reaches an equilibrium such that the source term is balanced by the
precipitation sink.</p>
      <p id="d1e5373">Results from this idealized experiment are shown in
Figs. <xref ref-type="fig" rid="Ch1.F4"/> and <xref ref-type="fig" rid="Ch1.F5"/>. Since we
are investigating numerical errors due to insufficient time resolution, the
high-resolution run (T6; black, dashed line) with a time step of
6 s is regarded as the truth in the following analysis. We did not change
the vertical resolution; therefore, CFL numbers <inline-formula><mml:math id="M208" display="inline"><mml:mrow><mml:mi mathvariant="italic">α</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">6</mml:mn></mml:mrow></mml:math></inline-formula> s) are
very small throughout the column and no sub-stepping needs to be applied in
the T6 case. With the large CFL numbers for the<?pagebreak page1566?> global time step,
errors in the sedimentation calculation are huge. The simulation without
sub-stepping (NO) shows that the large errors in the sedimentation
calculation lead to a numerical deceleration of sedimentation. This in turn
strongly delays surface precipitation and leads to an accumulation of ice in
the atmosphere; see Fig. <xref ref-type="fig" rid="Ch1.F4"/> (orange lines). The
opposite problem is encountered when only the inner loop is acting to reduce
<inline-formula><mml:math id="M209" display="inline"><mml:mi mathvariant="italic">α</mml:mi></mml:math></inline-formula> (IN; purple line). While the error in the sedimentation
calculation is reduced, the sequential treatment of cloud processes and
sedimentation leads to an underestimation of sublimation and thus
overestimation of surface precipitation.</p>
      <p id="d1e5407">The simulations OUT (green line) and FL (light blue line)
reproduce the results of the high-resolution simulation T6 much
better. The two simulations only differ by the fact that the FL
simulation further reduces <inline-formula><mml:math id="M210" display="inline"><mml:mi mathvariant="italic">α</mml:mi></mml:math></inline-formula> by the additional sub-stepping of the
sedimentation calculation to achieve <inline-formula><mml:math id="M211" display="inline"><mml:mrow><mml:mi mathvariant="italic">α</mml:mi><mml:mo>&lt;</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula> throughout the column by the
inner loop. This difference is most pronounced in the low, thin levels where
<inline-formula><mml:math id="M212" display="inline"><mml:mi mathvariant="italic">α</mml:mi></mml:math></inline-formula> can still be very large even if it is reduced by the outer loop
already. The effect of this can be seen by comparing the vertical profiles of
the process rates of the two simulations in
Fig. <xref ref-type="fig" rid="Ch1.F5"/>. In the lowest levels, the simulation
OUT deviates from the reference T6, which leads to an overall
error in the surface precipitation and the cloud ice profile. The simulation
FL reaches very good agreement with the reference at all levels by
ensuring <inline-formula><mml:math id="M213" display="inline"><mml:mrow><mml:mi mathvariant="italic">α</mml:mi><mml:mo>&lt;</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula> and thus achieving numerical stability throughout the
column.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F4"><label>Figure 4</label><caption><p id="d1e5453">Results from a sedimentation test case in the single-column model.
<bold>(a)</bold> Cloud ice and <bold>(b)</bold> surface precipitation. Colors
indicate different simulation setups: T6 uses a time step of 6 s. In the
simulations NO, IN, OUT and FL, a global time step of 600 s is used. They
differ in their sub-stepping: FL has full sub-stepping with online
computation of <inline-formula><mml:math id="M214" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mtext>in</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M215" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mtext>out</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>; IN sets <inline-formula><mml:math id="M216" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mtext>out</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula> and
only uses the inner loop with online computation of <inline-formula><mml:math id="M217" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mtext>in</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and vice
versa for the simulation OUT. NO does not use any sub-stepping with constant
<inline-formula><mml:math id="M218" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mtext>in</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>n</mml:mi><mml:mtext>out</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula>.</p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://gmd.copernicus.org/articles/11/1557/2018/gmd-11-1557-2018-f04.png"/>

        </fig>

<?xmltex \hack{\newpage}?><?xmltex \floatpos{t}?><fig id="Ch1.F5"><label>Figure 5</label><caption><p id="d1e5542">Simulations as in Fig. <xref ref-type="fig" rid="Ch1.F4"/> but for vertical
profiles at equilibrium, evaluated after 12 h of the
simulation.<bold>(a)</bold> cloud ice, <bold>(b)</bold> sublimation rate and
<bold>(c)</bold> self-collection rate.</p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://gmd.copernicus.org/articles/11/1557/2018/gmd-11-1557-2018-f05.png"/>

        </fig>

</sec>
<sec id="Ch1.S4.SS3">
  <title>Linking performance and accuracy</title>
      <?pagebreak page1567?><p id="d1e5569">The test case presented above allows us to use the optimization strategy to find
a compromise between performance and accuracy. To assess performance, we
measure the computation time of the cloud microphysics routine. Specifically
the two parts cloud processes and sedimentation shown in
Fig. <xref ref-type="fig" rid="Ch1.F2"/>. We then define the speedup as the ratio
<inline-formula><mml:math id="M219" display="inline"><mml:mrow><mml:msub><mml:mi>t</mml:mi><mml:mrow><mml:mi mathvariant="normal">T</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:mrow></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>t</mml:mi><mml:mi mathvariant="normal">SIM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> of the computation times <inline-formula><mml:math id="M220" display="inline"><mml:mi>t</mml:mi></mml:math></inline-formula> of any
simulation SIM and the reference high-resolution simulation.
Figure <xref ref-type="fig" rid="Ch1.F6"/>a shows the relative errors in surface
precipitation and ice water path at equilibrium together with the speedup
for each simulation. A new simulation OUT100 is introduced to provide
a further benchmark. It uses only the outer loop to achieve <inline-formula><mml:math id="M221" display="inline"><mml:mrow><mml:mi mathvariant="italic">α</mml:mi><mml:mo>&lt;</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula>
throughout the column; i.e., it puts all the work into the expensive cloud
processes iteration. This is equivalent to the strategy illustrated by the
orange bar in Fig. <xref ref-type="fig" rid="Ch1.F3"/>c.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F6"><label>Figure 6</label><caption><p id="d1e5621">Relative errors
<inline-formula><mml:math id="M222" display="inline"><mml:mrow><mml:mo>|</mml:mo><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="italic">SIM</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mrow><mml:mi>T</mml:mi><mml:mn mathvariant="italic">6</mml:mn></mml:mrow></mml:msub><mml:mo>)</mml:mo><mml:mo>/</mml:mo><mml:msub><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mrow><mml:mi>T</mml:mi><mml:mn mathvariant="italic">6</mml:mn></mml:mrow></mml:msub><mml:mo>|</mml:mo></mml:mrow></mml:math></inline-formula> and speedup factor
<inline-formula><mml:math id="M223" display="inline"><mml:mrow><mml:msub><mml:mi>t</mml:mi><mml:mrow><mml:mi>T</mml:mi><mml:mn mathvariant="italic">6</mml:mn></mml:mrow></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>t</mml:mi><mml:mi mathvariant="italic">SIM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> within the cloud microphysics scheme for the
simulations SIM shown in Figs. <xref ref-type="fig" rid="Ch1.F4"/>
and <xref ref-type="fig" rid="Ch1.F5"/> together with a new simulation
OUT100 that achieves <inline-formula><mml:math id="M224" display="inline"><mml:mrow><mml:mi mathvariant="italic">α</mml:mi><mml:mo>&lt;</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula> throughout the column only by using
the outer loop. <bold>(a)</bold> Blue and yellow bars show the relative error of
the ice water path and surface precipitation at equilibrium.
<bold>(b)</bold> Relative errors as in <bold>(a)</bold> (orange and blue lines).
Purple lines show the number of outer (solid; right axis) and inner (dashed;
right axis) iterations. The green line shows the speedup (right axis).</p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://gmd.copernicus.org/articles/11/1557/2018/gmd-11-1557-2018-f06.png"/>

        </fig>

      <p id="d1e5716">Figure <xref ref-type="fig" rid="Ch1.F6"/>a illustrates that the optimization strategy works
as expected and a speedup of around 7 can be achieved by only considering
part of the column to calculate the number of outer iterations. It also
confirms the finding from the last section; using the inner loop is essential
to reduce the error from more than 15 % in the OUT simulation to
well below 5 % in the FL simulation while keeping the speedup
almost identical. The simulation OUT100 achieves an almost exact match
with the high-resolution simulation. However, it comes at the cost of
drastically reducing model performance. Thus, the benefit of the sequential
treatment of cloud processes and nested sub-stepping becomes clear.</p>
      <p id="d1e5721">Figure <xref ref-type="fig" rid="Ch1.F6"/>b adds more depth to the optimization strategy. By
considering a range of different threshold times <inline-formula><mml:math id="M225" display="inline"><mml:mi>x</mml:mi></mml:math></inline-formula>, we can choose to trade
accuracy for performance. By setting a high threshold time, we can achieve a
speedup of up to 15 if we accept the larger error.</p>
      <p id="d1e5734">This analysis has been performed on a series of different test cases (varying
particle size and density as well as varying temperature and relative
humidity profiles; not shown), including one where ice melts to form rain.
This last test is particularly interesting because the melting layer
represents a sharp change in process rates from one level to the next.
However, since the calculation of rain is largely independent of the
sub-stepping (see the section below) and since melting is represented by a
finite, physically based timescale, the optimization strategy did not lead
to large errors. We chose to show a different test case here because we
wanted to highlight the treatment of the sedimentation of cloud ice in the
lowest levels where model levels are very thin.</p>
      <p id="d1e5737">While the values for the relative error vary roughly between 0 and
5 % depending on the test case and threshold values, the overall
correspondence of relative error and speedup has been shown to be a robust result
of our optimization strategy.</p>
</sec>
<sec id="Ch1.S4.SS4">
  <title>Sub-stepping and the diagnostic treatment of rain</title>
      <p id="d1e5746">This section provides a closer look at the rain flux within the sub-stepping
environment. A diagnostic treatment of precipitation is designed for very
large time steps where the vertical movement of raindrops cannot be
resolved. Since the new scheme in principle allows us to resolve falling hail
particles, we are outside of the realm the rain flux scheme was originally
designed for. Since this work focuses on the representation of cloud ice, we
will not discuss potential improvements to the liquid phase that would
benefit from the newly employed sub-stepping. The obvious improvement would
be using prognostic rain as was done by <xref ref-type="bibr" rid="bib1.bibx38" id="text.49"/>. However,
since their approach was different in terms of treating the cloud droplet and
raindrop size distribution, a merging of these two approaches is beyond the
scope of this paper but will be envisioned in future. Sticking with the rain
flux approach, it is important to rule out any systematic biases of rain
production associated with the sub-stepping employed for cloud ice.</p>
      <?pagebreak page1568?><p id="d1e5752">To estimate the sensitivity of rain production to the number of outer
iterations, we use a similar setup as for the ice sedimentation: a single-column simulation with an isothermal atmosphere at 20 <inline-formula><mml:math id="M226" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C and a
relative humidity of 100 % throughout the column. A humidity tendency
of <inline-formula><mml:math id="M227" display="inline"><mml:mrow><mml:mn mathvariant="normal">5</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">7</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> kg kg<inline-formula><mml:math id="M228" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> s<inline-formula><mml:math id="M229" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> is applied to the model levels
between 16 and 26 (corresponding to 900 and 400 hPa in pressure levels).
This forcing is representative of stratiform cloud formation in the global
setup of the model and corresponds to a water column tendency of
2 mm h<inline-formula><mml:math id="M230" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. For this experiment we fixed the cloud droplet number
concentrations but vary their (constant) values from 50 to
1000 cm<inline-formula><mml:math id="M231" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> to represent clouds with stronger and weaker rain
production rates.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F7" specific-use="star"><label>Figure 7</label><caption><p id="d1e5833">Rain production rates for the simulations described in the text.
Solid lines are simulations with <inline-formula><mml:math id="M232" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mtext>out</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula>, and dashed lines are
simulations with <inline-formula><mml:math id="M233" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mtext>out</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">100</mml:mn></mml:mrow></mml:math></inline-formula>. Different colors represent simulations
with different cloud droplet number concentrations reaching from 50 to
1000 cm<inline-formula><mml:math id="M234" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. The left column shows the total rain production rate and
its constituents auto-conversion of cloud droplets to raindrops and accretion
of cloud droplets by raindrops. The right column shows the differences
(<inline-formula><mml:math id="M235" display="inline"><mml:mrow><mml:msup><mml:mi>R</mml:mi><mml:mn mathvariant="normal">1</mml:mn></mml:msup><mml:mo>-</mml:mo><mml:msup><mml:mi>R</mml:mi><mml:mn mathvariant="normal">100</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula>, for <inline-formula><mml:math id="M236" display="inline"><mml:mrow><mml:msup><mml:mi>R</mml:mi><mml:mi>n</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula> being any of the rates above) between the
simulations with <inline-formula><mml:math id="M237" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mtext>out</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M238" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mtext>out</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">100</mml:mn></mml:mrow></mml:math></inline-formula> for every process.</p></caption>
          <?xmltex \igopts{width=398.338583pt}?><graphic xlink:href="https://gmd.copernicus.org/articles/11/1557/2018/gmd-11-1557-2018-f07.png"/>

        </fig>

      <p id="d1e5944">The simulations are run for 1 day with the humidity forcing active
throughout the whole simulation. Every simulation is run once with
<inline-formula><mml:math id="M239" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mtext>out</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula>, i.e., without sub-stepping affecting rain production, and
once with <inline-formula><mml:math id="M240" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mtext>out</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">100</mml:mn></mml:mrow></mml:math></inline-formula>, i.e., with a very large number of outer
iterations. Figure <xref ref-type="fig" rid="Ch1.F7"/> shows the vertically integrated
rain production rate together with its constituents: rain enhancement by
accretion of cloud droplets by raindrops and auto-conversion of cloud
droplets to raindrops.</p>
      <p id="d1e5980">The first row in Fig. <xref ref-type="fig" rid="Ch1.F7"/> indicates that different
numbers of sub-steps and thus different time step lengths can lead to
differences in the rain production rate. The simulation with one sub-step has
a slightly delayed the onset of precipitation and tends to overshoot the total
rain production by up to 10 % before reaching an equilibrium. For the
simulations with the highest number concentrations and therefore weakest rain
production rates, both the delay in onset and relative strength of
overshooting is less pronounced. Eventually, every simulation reaches an
equilibrium where the humidity input is balanced by the rain sink. This
external constraint leads to vanishing differences in equilibrium rain
production rates for different numbers of sub-steps. The second and third
rows show the constituents of the total rain production rate. These rates
show that there is no compensation of errors by the accretion and
auto-conversion rates but rather that the differences are due to the
overestimation of precipitation production by the linearized numerical
integration method employed by the core model. The local update of
<inline-formula><mml:math id="M241" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>c</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M242" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mtext>c</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> by sub-stepping Eqs. (<xref ref-type="disp-formula" rid="Ch1.E17"/>)
and (<xref ref-type="disp-formula" rid="Ch1.E18"/>) reduces the numerical error of the accretion and
auto-conversion rates and prevents the overshooting of precipitation formation
that can be seen in the <inline-formula><mml:math id="M243" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mtext>out</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula> simulations. This claim is backed up
by a simulation with high temporal resolution which is almost identical to
the simulation with <inline-formula><mml:math id="M244" display="inline"><mml:mn mathvariant="normal">100</mml:mn></mml:math></inline-formula> sub-steps and therefore not shown. We conclude that
sub-stepping is beneficial for the representation of the rain flux but the
effect is small.</p>
      <p id="d1e6034">Varying the number of outer iterations from 1 to 100 is an extreme case. In
the global model setup the number of outer iterations ranges on average from
5 in the tropics to 25 in midlatitudes. Since the model converges quickly
with increasing number of outer iterations, the delayed onset and
overshooting effects discussed here are an upper limit. We conclude that for
our purpose a diagnostic scheme for liquid water is compatible with the
prognostic treatment of cloud ice and no systematic biases are induced by the
number of outer iterations used. This is important as the number of outer
iterations is computed online and may vary between columns.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F8" specific-use="star"><label>Figure 8</label><caption><p id="d1e6039">Vertical profiles of the single-column model initial conditions and
forcing terms. <bold>(a)</bold> The temperature is initially set to the
international standard atmosphere temperature profile. <bold>(b)</bold> The
humidity profile allows for cloudy regions in cirrus and mixed-phase regimes.
<bold>(c)</bold> The humidity forcing terms that are applied to initiate cloud
formation. Solid lines show the forcing during cloud formation, dotted lines
show the stable phase without forcing, and the dashed lines show the forcing
of cloud dissipation.</p></caption>
          <?xmltex \igopts{width=398.338583pt}?><graphic xlink:href="https://gmd.copernicus.org/articles/11/1557/2018/gmd-11-1557-2018-f08.png"/>

        </fig>

</sec>
</sec>
<sec id="Ch1.S5">
  <title>Simulations of an idealized mixed-phase cloud</title>
      <p id="d1e6064">To demonstrate the behavior of the new scheme, we look at results from a more
elaborate single-column simulation than the ones used in
Sect. <xref ref-type="sec" rid="Ch1.S4"/>. The setup is summarized by the initial and forcing
profiles shown in Fig. <xref ref-type="fig" rid="Ch1.F8"/>. It allows for an isolated
examination of the microphysics scheme by deactivating the convection,
vertical diffusion and radiation parameterizations and allowing no surface
evaporation. The forcing terms are chosen such that there are two cloudy
regions: one in the cirrus and one in the mixed-phase regime
(Fig. <xref ref-type="fig" rid="Ch1.F8"/>c). We run the simulations for 36 h. The cirrus
cloud forcing is applied from hours 3 to 4. In the mixed-phase cloud
regime, the forcing is applied throughout the first 12 h (solid lines in
Fig. <xref ref-type="fig" rid="Ch1.F8"/>c). After 12 h the humidity tendencies are set
to 0 for another 12 h. Finally, tendencies equal in magnitude and
duration but with opposite sign (dashed lines in Fig. <xref ref-type="fig" rid="Ch1.F8"/>c)
are applied after 24 h such that the total water content is the same for
simulation times 0 and 36 h. The temperature is kept constant throughout
the simulation to compensate for latent heating by condensation/evaporation
and deposition/sublimation. Since the vertical diffusion and convection
parameterizations are turned off, this ensures that the melting layer remains
at the same level throughout the simulation, which facilitates the
interpretation of the results.</p>
      <p id="d1e6077">We prescribe mineral dust and sulfate aerosols which dominate heterogeneous
freezing in mixed-phase conditions and homogeneous nucleation in cirrus
clouds, respectively. Cloud droplet number concentration is fixed at a
constant value representative of marine clouds of 100 cm<inline-formula><mml:math id="M245" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> since we
are mainly interested in the evolution of cloud ice.</p>
<sec id="Ch1.S5.SS1">
  <title>Comparison to the original scheme</title>
      <p id="d1e6097">The standard version of ECHAM6-HAM2 is equipped with a two-moment scheme for
both cloud liquid water and ice and diagnostic equations for snow and rain
mass mixing ratios. For comparability, the new scheme can switch between
calculating in-cloud and sedimentation tendencies based on the new single
category and the original 2-category scheme. This way we are able to
consider only the differences between the schemes that are due to the
conversion of cloud ice to snow in the original scheme and the single-category approach while all compatible cloud processes (vapor deposition,
melting and freezing) are identical.</p>

<table-wrap id="Ch1.T1" specific-use="star"><label>Table 1</label><caption><p id="d1e6102">Summary of the ice description for the three schemes mentioned in
the text. Ice crystals are abbreviated by IC. P3 represents a
description of particle properties according to Sect. <xref ref-type="sec" rid="Ch1.S2"/>.
Since this analysis is focused on the different cloud ice schemes (prognostic
single category vs. diagnostic two category), we use the P3 properties for ice
crystals also in the 2- and 2.5-category schemes, assuring comparable fall
speeds and deposition rates. Since those schemes only consider riming for
snow, P3 is reduced to pure dendritic particles (i.e., <inline-formula><mml:math id="M246" display="inline"><mml:mrow><mml:msub><mml:mi>F</mml:mi><mml:mtext>r</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mo>⇔</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mtext>gr</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mtext>cr</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>).</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="4">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="left"/>
     <oasis:colspec colnum="3" colname="col3" align="left"/>
     <oasis:colspec colnum="4" colname="col4" align="left"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">2-category scheme</oasis:entry>
         <oasis:entry colname="col3">2.5-category scheme</oasis:entry>
         <oasis:entry colname="col4">1-category scheme</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">IC properties</oasis:entry>
         <oasis:entry colname="col2">P3 (dendrites)</oasis:entry>
         <oasis:entry colname="col3">P3 (dendrites)</oasis:entry>
         <oasis:entry colname="col4">P3</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">IC sedimentation type</oasis:entry>
         <oasis:entry colname="col2">off</oasis:entry>
         <oasis:entry colname="col3">diagnostic</oasis:entry>
         <oasis:entry colname="col4">prognostic</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">IC sedimentation scheme</oasis:entry>
         <oasis:entry colname="col2">–</oasis:entry>
         <oasis:entry colname="col3">
                    <xref ref-type="bibr" rid="bib1.bibx37" id="text.50"/>
                  </oasis:entry>
         <oasis:entry colname="col4">upstream Euler</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Number of prognostic parameters for the ice phase</oasis:entry>
         <oasis:entry colname="col2">2</oasis:entry>
         <oasis:entry colname="col3">2</oasis:entry>
         <oasis:entry colname="col4">4</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Diagnostic snow</oasis:entry>
         <oasis:entry colname="col2">
                    <xref ref-type="bibr" rid="bib1.bibx35" id="normal.51"/>
                  </oasis:entry>
         <oasis:entry colname="col3">
                    <xref ref-type="bibr" rid="bib1.bibx35" id="normal.52"/>
                  </oasis:entry>
         <oasis:entry colname="col4">–</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

      <p id="d1e6254">In the following we will present results from three different microphysics
schemes, summarized in Table <xref ref-type="table" rid="Ch1.T1"/>. They are presented in the
order similar to the evolution within ECHAM-HAM. The 2-category scheme
treats ice and liquid water analogously by separating in-cloud and
precipitation hydrometeors. While for liquid water this separation can be
justified by the different scales on which growth by condensation and growth
by collision–coalescence are efficient, the analogous argument does not hold
for cloud ice; a perfect dendrite can reach a significant fall speed. This
deficiency has been solved by including the mass flux divergence scheme
<xref ref-type="bibr" rid="bib1.bibx37" id="paren.53"/> to allow the in-cloud part of the ice population to fall
<xref ref-type="bibr" rid="bib1.bibx28" id="paren.54"/>. Here we call this scheme the 2.5-category scheme since the falling ice mass flux resembles a separate
category. The problem with this is, that there is no physical distinction
between falling ice and snow. Sublimation and melting are parameterized for
both precipitation categories, but only for snow collisions with liquid water
is included. This leads to an artificial competition between falling ice and
snow that, depending on the cloud<?pagebreak page1570?> forcing, forms precipitation hydrometeors
that can further grow by riming or are limited to sublimation and melting.
Furthermore, other growth mechanisms (i.e., self-collection and vapor
deposition) are neglected for both precipitation categories. The 1-category scheme is the logical successor in this line of development. By
resolving the vertical advection of cloud ice, precipitation categories are
no longer necessary. The spectrum of ice particles is represented, and one
single set of cloud processes is parameterized for the entire ice hydrometeor
population. With that, the conceptual problems of the previous schemes are
solved. The cloud liquid and ice water contents of the three simulations in
Fig. <xref ref-type="fig" rid="Ch1.F9"/> highlight the differences between the schemes.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F9"><label>Figure 9</label><caption><p id="d1e6269">Time series of the vertical profiles of in-cloud ice (contour lines)
and liquid water contents (colors). For the 2-category schemes snow mass is
indicated by dashed lines. Note that snow is a vertically integrated quantity
and the profile therefore is only an approximation. Panels <bold>(a)</bold> and
<bold>(b)</bold> show two versions the original scheme with diagnostic treatment
of sedimentation as discussed in the text, and <bold>(c)</bold> shows the single
category with prognostic ice sedimentation.</p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://gmd.copernicus.org/articles/11/1557/2018/gmd-11-1557-2018-f09.png"/>

        </fig>

      <p id="d1e6288">In the 2-category scheme simulation, cloud ice is not allowed to fall.
In the single-column model, ice crystals are therefore restricted to the
level they formed in, which are the levels where heterogeneous freezing of
cloud droplets takes place. Since temperature decreases with increasing
altitude, this process is most active at the cloud top. As soon as a sufficiently
large number of ice crystals has formed, their accumulated depositional
growth is able to quickly deplete the coexisting liquid water. The large
mass transfer from the liquid to the ice phase grows the ice crystals to a
size where conversion to snow is efficient. Those snow particles partly
deplete the liquid cloud below the freezing levels by riming and subsequently
sublimate.</p>
      <p id="d1e6291">The results from the 2.5-category scheme simulation show how the
situation changes when the ice crystals themselves are allowed to fall. The
ice crystals that formed at the cloud top do not accumulate in the levels of
formation but spread throughout the cloud. An exponential tail of the ice
crystal mass flux continually falls out of the cloud where it sublimates. Due
to the steady removal of cloud ice, growth by vapor deposition is delayed
(orange lines in Fig. <xref ref-type="fig" rid="Ch1.F10"/>a and b). The snow
production rate is weak because ice sediments out of the cloud before it can
efficiently grow to the snow threshold size. Consequently, the riming rate is
virtually 0 since only collisions between snow flakes and cloud droplets
are considered (purple line in Fig. <xref ref-type="fig" rid="Ch1.F10"/>c). The low
riming and deposition rates lead to a mixed-phase cloud that is heavily
dominated by liquid water (Fig. <xref ref-type="fig" rid="Ch1.F10"/>d). The challenge
of treating the sedimentation of ice crystals diagnostically has been
discussed in <xref ref-type="bibr" rid="bib1.bibx37" id="text.55"/>. Our results support the hypothesis that a
diagnostic scheme likely overestimates sedimentation.</p>
      <p id="d1e6303">The 1-category scheme does not rely on a separate set of microphysical
processes that are calculated only for diagnostic sedimentation categories
like snow and falling ice in the<?pagebreak page1571?> 2.5-category scheme. Thus, there can
be a competition between riming, vapor deposition and the removal by
sedimentation. Residence times per level are resolved by the sub-stepping
which allows us to compute physical processes on a theoretical basis instead of
empirical relationships employed for the mass flux calculation for ice and
snow.</p>
      <p id="d1e6306">These simulations nicely illustrate the theoretical considerations at the
beginning of this section. The separation into multiple categories and the
associated conversion rates strongly influence the resulting cloud structure,
lifetime and phase fraction. A small snow threshold size leads to more snow
and thus more riming, while for the threshold size of 100 <inline-formula><mml:math id="M247" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>m
used in the 2.5-category scheme, snow formation is almost completely
inhibited by the steady removal of cloud ice by the mass flux divergence
scheme. This sensitivity to a development choice that is not constrained by
first principles is highly undesired. The problem is resolved by the
prognostic, single category that does not have this degree of freedom and
thus simulates the cloud in an objective, physically based manner.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F10" specific-use="star"><label>Figure 10</label><caption><p id="d1e6319">Time series for the vertically integrated phase change process rates
for the simulations described in the text. The solid lines show results from
the 2.5-category scheme with diagnostic snow and falling ice and the dashed
lines show the results from the single-category scheme with prognostic ice
sedimentation. Panels <bold>(a)</bold>–<bold>(c)</bold> show the rates of phase
changes; <bold>(d)</bold> shows the vertically integrated condensate. Condensation and
deposition rates are divided into changes due to transport (forcing
term), evaporation of rain and sublimation of sedimenting ice.
Ice growth at the expense of liquid is denoted by wbf.</p></caption>
          <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://gmd.copernicus.org/articles/11/1557/2018/gmd-11-1557-2018-f10.png"/>

        </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F11" specific-use="star"><label>Figure 11</label><caption><p id="d1e6340">Same as in Fig. <xref ref-type="fig" rid="Ch1.F10"/> but for simulations
with the single-category scheme where freezing in the mixed-phase cloud is
turned off and the humidity forcing in the cirrus regime is turned on. The
solid lines represent a simulation where riming affects the particle
properties, and the dashed lines represent a simulation where the mass-to-size
relation for dendrites is assumed for all particles with diameter <inline-formula><mml:math id="M248" display="inline"><mml:mrow><mml:mi>D</mml:mi><mml:mo>&gt;</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mtext>th</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>.</p></caption>
          <?xmltex \igopts{width=398.338583pt}?><graphic xlink:href="https://gmd.copernicus.org/articles/11/1557/2018/gmd-11-1557-2018-f11.png"/>

        </fig>

</sec>
<sec id="Ch1.S5.SS2">
  <title>Predicting the rime fraction and density</title>
      <p id="d1e6372">The rime variables in the single-category scheme, i.e., the rimed ice mass
mixing ratio and the rimed ice volume mixing ratio, determine the density and
shape of the particles with heavily rimed particles being spherical and
weakly rimed particles having dendritic geometry. As a result, particles with
high rime fractions have a smaller projected area and thus a higher fall
speed than their weakly rimed counterparts of the same mass.
<xref ref-type="bibr" rid="bib1.bibx33" id="text.56"/> showed in a regional model that this
adjustment of particle properties is crucial to correctly predict
precipitation rates in a squall line simulation with strong convective
updraft.</p>
      <p id="d1e6378">The ECHAM6-HAM2 GCM does not resolve those strong convective updrafts but
parameterizes convection by the <xref ref-type="bibr" rid="bib1.bibx50" id="text.57"/> scheme. In its standard
version, it employs very simplified microphysics which does not account for
the coexistence of liquid water and ice. It is therefore questionable
whether riming as such, and the resulting change in particle properties
especially, is currently adequately represented in convective clouds.</p>
      <p id="d1e6384">From a purely stratiform cloud perspective, the effect of the particle
properties on process rates is best illustrated by a seeder–feeder situation.
Ice crystals form in the cirrus cloud and quickly grow to a few
100 <inline-formula><mml:math id="M249" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>m in diameter in the highly supersaturated environment. The
largest crystals sediment quickly and subsequently interact with a
supercooled liquid cloud below by riming and the WBF process. Whether riming
or vapor deposition dominates, strongly depends on the particle size. A few
large particles will grow more strongly by riming while the growth of many
small particles will be dominated by vapor deposition. Therefore, combining
strong depositional growth in the cirrus regime with gravitational
size sorting provides the optimal conditions for rime growth within the
supercooled liquid cloud. In the following, we will explore this special case
and shed light on the particle properties within the P3 parameterization.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F12" specific-use="star"><label>Figure 12</label><caption><p id="d1e6397">Time series of the vertical profiles of the particle properties for
the seeder–feeder simulation described in the text. Panels <bold>(a)</bold>–<bold>(c)</bold> and <bold>(d)</bold>–<bold>(f)</bold> show results for
the simulations with and without taking the change in particle properties due
to riming into account, respectively. Panels <bold>(a)</bold> and <bold>(d)</bold> show the
water mixing ratios (colors for liquid, contours for ice), <bold>(b)</bold> and
<bold>(e)</bold> show ice particle fall speeds, and <bold>(c)</bold> and
<bold>(f)</bold> show ice particle density. In panels <bold>(b)</bold>, <bold>(c)</bold>,
<bold>(d)</bold> and <bold>(f)</bold>, the solid and dotted lines show regions of
significant (<inline-formula><mml:math id="M250" display="inline"><mml:mrow><mml:mo>&gt;</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">9</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> kg kg<inline-formula><mml:math id="M251" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> s<inline-formula><mml:math id="M252" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) riming and depositional
growth, respectively. Hatches mark areas where <inline-formula><mml:math id="M253" display="inline"><mml:mrow><mml:msub><mml:mi>F</mml:mi><mml:mtext>r</mml:mtext></mml:msub><mml:mo>&gt;</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:math></inline-formula>, i.e., where
particles are dominated by rimed ice.</p></caption>
          <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://gmd.copernicus.org/articles/11/1557/2018/gmd-11-1557-2018-f12.png"/>

        </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F13"><label>Figure 13</label><caption><p id="d1e6509">Time series of the vertical profile of water contents for the cirrus
cloud above a mixed-phase cloud simulation described in the text are shown
in <bold>(a)</bold> (black solid lines: ice; colors: liquid water). Panel <bold>(b)</bold> shows the same for the ice crystal number concentration. The
rectangles in <bold>(a)</bold> and <bold>(b)</bold> visualize the regions
representative of the particle size distributions in <bold>(c)</bold> (not drawn
to scale). Normalized particle size distributions for the rectangular areas
in <bold>(a)</bold> and <bold>(b)</bold> are shown in <bold>(c)</bold>. The orange and
purple lines represent the mixed-phase and cirrus particles before impact, and
the green line is the combination of the two after impact. Since the size
distribution is normalized, we give the total number <inline-formula><mml:math id="M254" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> for each
distribution in the corresponding color in L<inline-formula><mml:math id="M255" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> as well as the total ice
mass mixing ratio <inline-formula><mml:math id="M256" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> in <inline-formula><mml:math id="M257" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g kg<inline-formula><mml:math id="M258" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>.</p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://gmd.copernicus.org/articles/11/1557/2018/gmd-11-1557-2018-f13.png"/>

        </fig>

      <p id="d1e6598">The boundary and forcing profiles for the simulation are the same as in the
last section (Fig. <xref ref-type="fig" rid="Ch1.F8"/>) but with heterogeneous freezing in
the mixed-phase cloud turned off. To investigate the sensitivity to the
particle properties within the new scheme, we vary the effect that riming has
on the mass-to-size relationship of the P3 scheme described in
Sect. <xref ref-type="sec" rid="Ch1.S2"/>. Two simulations are done: the rime
properties simulation uses the regular particle properties of the P3 scheme,
and the dendritic properties simulation neglects the effect of riming
on the mass-to-size relationship. With the notation from
Sect. <xref ref-type="sec" rid="Ch1.S2"/>, this can be expressed by setting the rime fraction
<inline-formula><mml:math id="M259" display="inline"><mml:mrow><mml:msub><mml:mi>F</mml:mi><mml:mtext>r</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula>, which results in <inline-formula><mml:math id="M260" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>gr</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mtext>cr</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>. The only
remaining transition parameter then is <inline-formula><mml:math id="M261" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>th</mml:mtext></mml:msub><mml:mo>≡</mml:mo><mml:mtext>const</mml:mtext></mml:mrow></mml:math></inline-formula>,
separating the small spherical ice regime from the dendrite regime.</p>
      <p id="d1e6656">Figure <xref ref-type="fig" rid="Ch1.F11"/> shows a summary of the process rates
and column-integrated water masses. We can see that neglecting the impact of
riming on particle properties changes the thickness of the liquid cloud by
roughly 10 %. This can be attributed to the different riming and
deposition rates in the two simulations, which is ultimately a result of the
slightly longer residence times within the mixed-phase cloud due to the
smaller fall speeds in the dendritic properties simulation.</p>
      <p id="d1e6661">Figure <xref ref-type="fig" rid="Ch1.F12"/> shows the particle properties for
the two simulations. From the process rates
(Fig. <xref ref-type="fig" rid="Ch1.F11"/>b and c), we can see that rime growth
only exceeds growth by vapor deposition at about 7 h after the simulation
start and quickly diminishes after that. This is due to the gravitational
size sorting of the cirrus particles and the strong dependence on particle
fall speed and diameter of the riming rate; large particles will reach the
liquid cloud first and a significant amount of rimed ice forms upon impact
with the cloud droplets. This is the time, where the two simulations differ
most. While the particles from the rime properties simulation get
slightly more spherical by riming and their fall speeds increase up to almost
2-fold, the particles from the dendritic properties simulation
neglect the rime fraction for the fall velocity calculation. Therefore, these
particles keep their dendritic shape and fall more slowly, which gives them
more time to grow throughout the liquid cloud. The total ice particle density
is largely dominated by the particle size. A fully rimed particle could reach
a density of a several hundred kg m<inline-formula><mml:math id="M262" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. However, the maximal rime
fraction obtained here is roughly 60 %. Therefore, the particles do not
reach densities higher than 100 kg m<inline-formula><mml:math id="M263" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>.</p>
      <p id="d1e6692">The idealized, purely stratiform and turbulence-free simulations shown in
this section do not produce the conditions necessary to form heavily rimed
particles even though the setup has explicitly been designed to create an
environment that favors rime growth over depositional growth. It is therefore
questionable whether the global setup is able to provide the forcing
necessary to form heavily rimed particles at all. While this is subject to
further investigation, the simulation<?pagebreak page1572?> shown here suggests that for stratiform
clouds, the computational cost to solve prognostic equations to predict the
rime fraction and rime density could be saved.</p>
</sec>
<sec id="Ch1.S5.SS3">
  <title>Limitations of a single category</title>
      <p id="d1e6702">The single-category scheme is able to represent a wide range of particle
properties representing small in-cloud ice crystals, larger dendrites and
fast-falling structures like graupel and hail.</p>
      <p id="d1e6705">It is important to remember that the particle properties are parameterized by
the particle size distribution, mass-to-size and mass-to-projected area
relationships. Therefore, a predefined relationship between the four
prognostic ice parameters and the particle properties exists, which is laid
out in Sect. <xref ref-type="sec" rid="Ch1.S2"/>. We would like to stress the fact that it is
the four predicted ice parameters (ice mass mixing ratio <inline-formula><mml:math id="M264" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, rimed
ice mass mixing ratio <inline-formula><mml:math id="M265" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>rim</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, total ice number mixing ratio
<inline-formula><mml:math id="M266" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mtext>i</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and rimed ice volume <inline-formula><mml:math id="M267" display="inline"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mtext>rim</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>) that are prognostic and not
the particle properties themselves.</p>
      <?pagebreak page1573?><p id="d1e6754">This section provides a closer look at this peculiarity of a single-category
scheme. We use a similar seeder–feeder simulation as in the last section but
with a mixed-phase cloud instead of a pure liquid cloud as the feeder cloud.
We will focus on three particular areas in the simulation, shown in
Fig. <xref ref-type="fig" rid="Ch1.F13"/>a: (1) the mixed-phase cloud just before
the cirrus particles impact, (2) the cirrus particles just above the
mixed-phase cloud and (3) the resulting particles after impact.</p>
      <p id="d1e6759">From the corresponding particle size distributions in
Fig. <xref ref-type="fig" rid="Ch1.F13"/>b we can see how a single category handles
the addition of two ice masses with differing particle properties. The number
concentration in the tail of the very large particles from the cirrus cloud
(purple line) is lost by averaging even though it contributes almost
10 % to the total mass mixing ratio. This is because the total number
concentration is heavily dominated by the mixed-phase cloud (orange line)
with the cirrus cloud only making up a small fraction of about 1 %
thereof. Since the microphysical process rates are calculated from the
resulting particle size distribution (green line), particle collisions and
the sedimentation sink are likely underestimated.</p>
      <p id="d1e6765">A solution to this issue has been proposed by <xref ref-type="bibr" rid="bib1.bibx31" id="text.58"/> by
the use of multiple free categories. Ice of different origin will then be
sorted according to its diagnosed properties and stored in separate
variables, thus giving the properties themselves a prognostic flavor.
However, adding prognostic variables for multiple free categories is
computationally expensive. We argue that in the context of climate
projections where we are interested in global and regional mean states of the
atmosphere, the computational cost of this additional procedure likely
outweighs the benefit from an improved representation of ice particle
properties.</p>
      <p id="d1e6771">While a high-resolution model is able to produce different particle
properties within a single cloud, the global model often represents a cloud
with only a few grid boxes. Therefore, the regions where the use of multiple
free categories could improve the model results are those where the
seeder–feeder mechanism or convective anvils contribute significantly to the
ice water path. How important these situations are in the global context in
ECHAM6-HAM2 will have to be investigated in future studies. Then the benefit
of multiple free categories can be revisited.</p>
</sec>
</sec>
<sec id="Ch1.S6" sec-type="conclusions">
  <title>Conclusion</title>
      <p id="d1e6781">The single-category scheme proposed by MM15 has been successfully implemented
in the ECHAM6-HAM2 microphysics scheme. The structure of the original code
has been reworked and the large-scale deposition, cloud cover and melting
calculations have been adapted to comply with the prognostic ice category and
a variable time step. Numerical stability is achieved by sub-stepping the
cloud microphysics and sedimentation routines with an attempt to keep
computation time as low as possible by applying a nested<?pagebreak page1574?> sub-stepping
approach. It has been shown that a compromise can be reached to allow
reasonable accuracy and performance at the same time.<?xmltex \hack{\newpage}?></p>
      <p id="d1e6785">The new scheme is evaluated against its forerunner within an idealized
mixed-phase cloud simulation. The sub-stepping introduced in the new scheme
allows cloud ice sedimentation to be calculated prognostically and treats all
cloud processes equally. This means, that falling ice is now subject to all
the cloud processes, including all growth mechanisms (i.e., vapor deposition,
self-collection and riming). The artificial competition between the two
sedimentation categories that has been present in the original scheme, its
implications for the process rates and hence the cloud structure, lifetime
and phase fraction have been removed. At the same time, the continuous
treatment of cloud ice with a single category no longer requires the weakly
constrained threshold size for the conversion of ice crystals to snow.
Together, these factors make the new scheme more closely based on first
principles. This reduces its conceptual complexity and simplifies both model
development and the interpretation of model results.</p>
      <p id="d1e6788">An important feature of the original P3 scheme are the rime variables that
allow us to predict the particle shape and density. We could not produce a
purely stratiform cloud formation scenario where rime growth significantly
exceeded growth by vapor deposition. The large gap between the resolved
scales in ECHAM6-HAM2 and the scales on which hydrometeor collisions take
place raises the question to which extent riming can be represented on a
physical basis in this framework. The two additional prognostic variables
might be unnecessary for the global model used in this study. To establish
the rime fraction and density, up- and downdrafts need to be resolved on the
scales of clouds. However, any sub-grid-scale motion in the global model is
parameterized. It is therefore indispensable to include an elaborate
microphysics scheme in the convection parameterization that is able to
represent the coexistence of liquid water and ice. This is not the case for
our default scheme. While there have been approaches trying to improve this
aspect in the past <xref ref-type="bibr" rid="bib1.bibx23 bib1.bibx6" id="paren.59"/>, assessing the rime fraction
and density required for the P3 representation of cloud ice requires that the
associated cloud parameters would also need to be predicted within the
convective parameterization of ECHAM6-HAM2.</p>
      <p id="d1e6794">We evaluated limitations of the single-category scheme. The inability to
distinguish between particles from different sources, inherent in any bulk particle
scheme, persists. At the core of this problem is the fact that it is not the
ice particle properties themselves for which prognostic equations are solved
but that they are diagnosed from the prognostic ice parameters. A solution
has been proposed by <xref ref-type="bibr" rid="bib1.bibx31" id="text.60"/> by using multiple free
categories to give the particle properties themselves a prognostic flavor.</p>
      <p id="d1e6801">Reducing the number of weakly constrained parameters by going from a multi-
to a single-category scheme as well as fully resolving the ice formation
pathway by the prognostic treatment of cloud ice are clear conceptual
improvements over the original scheme. The level of sophistication to which
the single category can be implemented in a global model<?pagebreak page1575?> remains to be seen.
In the context of climate projections, the benefit from solving additional
equations to represent rimed ice properties, as is done in the P3 scheme, or
adding multiple free categories need to outweigh the associated computational
cost. As a next step we will test the performance of the single category
globally.</p>
</sec>

      
      </body>
    <back><notes notes-type="codedataavailability"><title>Code and data availability</title>

      <p id="d1e6808">The code of the cloud microphysics module (Fortran 95) is
available upon request from the corresponding author or as part of the
ECHAM6-HAMMOZ chemistry climate model through the HAMMOZ distribution
web-page <uri>https://redmine.hammoz.ethz.ch/projects/hammoz</uri>.</p>

      <p id="d1e6814">All data used to generate the plots can be found in the supplement.</p>
  </notes><app-group>
        <supplementary-material position="anchor"><p id="d1e6817">The supplement related to this article is available online at: <inline-supplementary-material xlink:href="https://doi.org/10.5194/gmd-11-1557-2018-supplement" xlink:title="zip">https://doi.org/10.5194/gmd-11-1557-2018-supplement</inline-supplementary-material>.</p></supplementary-material>
        </app-group><notes notes-type="competinginterests"><title>Competing interests</title>

      <p id="d1e6826">The authors declare that they have no conflict of
interest.</p>
  </notes><ack><title>Acknowledgements</title><p id="d1e6832">This project has been funded by the Swiss National Science Foundation
(project number 200021_160177). The authors would like to especially thank
an anonymous reviewer for valuable input which led to a significant
improvement of the model and manuscript. We thank Hugh Morrison and
Jason Milbrandt for sharing their ice particle property lookup tables and
corresponding generation code as well as their microphysics code which were
of great help to develop our own codes. Furthermore, we thank Jörg Wieder
for his work related to the WBF process parameterization. The ECHAM-HAMMOZ
model is developed by a consortium composed of ETH Zurich, the Max Planck
Institut für Meteorologie, Forschungszentrum Jülich, the University of
Oxford, the Finnish Meteorological Institute and the Leibniz Institute for
Tropospheric Research, and managed by the Center for Climate Systems Modeling
(C2SM) at ETH Zurich. Special thanks go to Sylvaine Ferrachat for technical
support regarding the model.<?xmltex \hack{\newline}?><?xmltex \hack{\newline}?> Edited by: Holger
Tost<?xmltex \hack{\newline}?> Reviewed by: two anonymous referees</p></ack><ref-list>
    <title>References</title>

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